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1.
Marine carbon cycle of the South China Sea is an important part of global carbon cycle. Researches on the air-sea CO2 flux in the South China Sea will help us understand the global carbon cycle and improve the global carbon system parameter database. This paper concisely summarized the changes of partial pressure of CO2 (pCO2), air-sea CO2 fluxes (FCO2), and related environmental factors in four regions in domains in the South China Sea. The low-salinity area of the upper reaches of the Pearl River estuary in the northern of South China Sea shelf area acted as a strong source of atmospheric CO2, with high pCO2(405.3~810.6 Pa)all year round. The lower area of the Pearl River estuary (salinity > 33.7) acted as a weak sink of CO2 in winter, with relatively low pCO2 (35.2~37.0 Pa). The northern slope/basin in the South China Sea acted as a source of CO2 in warm seasons with a relatively high pCO2 (45.0 Pa), and acted as a sink of CO2 in cold seasons with a relatively low pCO2 (34.7 Pa). The west of the Luzon Strait acted as a sink of CO2 in spring, while it acted as a source of CO2 in other seasons, with relative high pCO2 (38.4~47.5 Pa) in winter. The central/southern basin in the South China Sea acted as sources of CO2, with relative high pCO2 (41.0 Pa) all the year. Generally, the estimation of annual sea-air CO2 fluxes showed that most domains in the South China Sea served as weak sources of atmospheric CO2. In the future, more researches should be focused on the time-series of sea surface pCO2 and the remote sensing of the sea-air CO2 fluxes.  相似文献   

2.
石笋氧同位素记录具有明显的2万年周期,其他记录中广泛存在的10万年周期是否在石笋中有所表现目前还鲜有报道。通过对湖北三宝洞20支石笋的铀同位素数据的分析研究发现,石笋初始234U/238U值在序列连续性较好的640.3~299.6 ka B.P.时间段有强烈的10万年周期特征。在间冰期和冰期时,初始234U/238U值分别呈增大和减小状态。初始234U/238U值的10万年周期与全球冰量、黄土磁化率、黄土平均粒度和大气CO2变化有良好的对应关系。这些对应关系表明全球冰量、大气CO2对喀斯特区地球化学元素富集和迁移作用有重要影响。石笋氧同位素的显著岁差周期独立于石笋微量元素、高纬冰量和全球温室气体变化,暗示了太阳辐射变化对中低纬水汽环流的直接影响。石笋初始234U/238U与氧同位素、太阳辐射在冰消期时的对应变化支持北半球太阳辐射能量变化对冰期-间冰期旋回的调控作用。  相似文献   

3.
未来百年全球气候变化的影响是当前学术界激烈争议的议题,深入探讨全球气候变化的驱动机理才能正确认识全球气候变化.持续生长的青藏高原吸收了巨量的CO2,导致大气中CO2浓度大幅下降,使地球从温室气候进入到以冰期、间冰期交替出现为特征的冰室气候,青藏高原成为新生碳储库.在间冰期,青藏高原和蒙古高原将淡水输送到中低纬度内陆区(...  相似文献   

4.
Carbon dioxide records from polar ice cores and marine ocean sediments indicate that the last glacial maximum (LGM) atmosphere CO2 content was 80–90 ppm lower than the mid-Holocene. This represents a transfer of over 160 GtC into the atmosphere since the LGM. Palaeovegetation studies suggest that up to 1350 GtC was transferred from the oceans to the terrestrial biosphere at the end of the last glacial. Evidence from carbon isotopes in deep sea sediments, however, indicates a smaller shift of between 400 and 700 GtC. To understand the functioning of the carbon cycle this apparent discrepancy needs to be resolved. Thus, older data have been reassessed, new data provided and the potential errors of both methods estimated. New estimates of the expansion of terrestrial biomass between the LGM and mid-Holocene are 700 GtC ± > 300 GtC, using the ocean carbon isotope-based method, compared with of 1100 GtC ± > 500 GtC using the palaeovegetation estimate. If these estimates of the carbon shift to the terrestrial biosphere are equilibrated with the dissolved carbon in the oceans, and the CaCO3 compensation of the ocean is taken into account, then the glacial atmospheric CO2 would have been between 50 (± 30) ppm and 95 (± 50) ppm higher. The glacial atmosphere therefore should have had a CO2 partial pressure of between 330 and 375 μatm. Hence, a rise of between 130 and 175 μatm in atmospheric CO2, rather than 80 μatm, at the end of the last glacial must be accounted for.  相似文献   

5.
The δ13C of organic matter bound within the crystal lattice of foraminiferal calcite tests may provide a potential tracer of the isotopic composition of the surface water primary photosynthate. Using δ13C of the organic matter extracted from the crystal lattice and the calcite test, it is theoretically possible to estimate the paleo-surface water pCO2. We have tailored this technique initially for the subpolar planktonic foraminifera species Globigerina bulloides. Initial surface water pCO2 estimates from deep-sea core BOFS 5K (50°41.3′N, 21°51.9′W, water depth 3547 m) indicate that the northeast Atlantic Ocean may have been a greater sink for CO2 during the last glacial than during the Holocene. Greatly reduced benthic foraminifera abundances, especially phytodetritus feeders, in BOFS 5K during the last glacial indicates low surface productivity. This rules out a productivity-driven CO2 sink. The enhanced glacial CO2 sink must, therefore, have results from a southwards shift of the centre of deep water formation.  相似文献   

6.
李文宝  王汝建 《地球科学》2016,41(5):742-756
海平面的变化往往对区域生态环境、社会经济造成严重影响.通过对全球相对海平面变化(relative sea level,简称RSL)记录的再分析结果,合成了近2 Ma BP以来的全球RSL变化记录,分析了合成RSL记录对原始RSL记录数理特征的继承性,并基于频谱、滤波等数理分析验证了合成RSL记录的合理性.在此基础上,讨论了合成RSL与大气CO2浓度、中高纬度海域表层海水温度(sea surface temperature,简称SST)、全球大洋底栖氧同位素(δ18OB)等参数指标间的相关性,结果显示:(1) 合成RSL不仅与原始RSL记录的变化趋势基本一致,继承了原始RSL记录对全球气候变化的响应特征,而且显示出合成RSL记录对地球轨道参数周期变化响应明显;(2) 近2 Ma BP以来,在冰期-间冰期旋回中,合成RSL与δ18OB变化呈良好的负相关,相关系数r平均值可以达到约0.81,高于合成RSL与大气CO2浓度及中高纬度海域SST变化的相关系数;(3) 在地球轨道参数周期上,合成RSL与极地冰盖体积(δ18OB)的变化几乎同时,在偏心率周期上,合成RSL落后于SST和大气CO2浓度变化;在斜率周期上,合成RSL落后于SST变化而领先于大气CO2浓度变化.推测这些变化的诱导因素可能是在太阳辐射量改变的前提下,大气CO2浓度及大洋SST变化对极地冰盖体积产生了差异影响,进而引起海平面发生变化.   相似文献   

7.
中国第二次北极科学考察路线上温室气体瓶采样结果分析   总被引:2,自引:0,他引:2  
张东启  徐建中  汤洁  温民 《冰川冻土》2006,28(3):319-323
用气相色谱和非红外色散分析方法,分析了中国第二次北极科学考察路线上采集到的气体样品中温室气体(CO2和CH4)的浓度,对不同纬度带上CO2和CH4平均浓度变化特征进行了研究.结果表明:海洋表面不同纬度带上CO2的浓度呈现出随纬度升高而减小的趋势,这与全球范围内CO2的年平均浓度的地理分布特征相反,显示了海洋对CO2气体的吸收作用.45°N以北的海洋表面,CH4浓度有随纬度升高而增大的趋势,这与全球范围内CH4的年平均浓度的地理分布特征相同;中纬度近海岸地区温室气体浓度变化无明显规律,可能受到区域或局地气团的影响较大.  相似文献   

8.
三峡澎溪河水域CO2与CH4年总通量估算   总被引:1,自引:0,他引:1       下载免费PDF全文
李哲  白镭  蒋滔  郭劲松  刘静 《水科学进展》2013,24(4):551-559
以2010年6月~2011年5月三峡澎溪河回水区CO2与CH4通量监测数据为基础,参考澎溪河高阳平湖水域全年4次的24 h昼夜连续跟踪观测结果,对每月各采样点的日通量值进行估算。提出了水下地形划分法和环境因素控制法,将各采样点日通量数据外延至整个回水区水域,并估算了澎溪河回水区水域CO2与CH4年总通量值。研究期间,澎溪河回水区全年各采样点CO2通量均值为(3.05±0.46)mmol/(m2·h);CH4为(0.050 1±0.009 6)mmol/(m2·h)。以水下地形法为基础,该水域全年CO2和CH4总通量分别为40 060.5 t和540.9 t;以环境因素控制法为基础,全年CO2与CH4总通量分别为39 073.0 t和467.2 t。以环境要素控制法为参考,该水域CO2全年平均释放强度为43.26 mmol/(m2·d),在全球水库数据序列中处于中等略偏高水平,CH4全年平均释放强度为1.42 mmol/(m2·d),在全球水库序列中处于中等水平。  相似文献   

9.
研究青藏高原多年冻土区高寒草甸土壤CO2通量有助于准确估算该区域的土壤CO2排放, 对认识高原土壤碳循环及其对全球气候变化的响应具有重要意义. 利用静态箱-气相色谱法和LI-8100土壤CO2通量自动测量系统对疏勒河上游多年冻土区高寒草甸土壤CO2通量进行了定期观测, 结合气象和土壤环境因子进行了分析. 结果表明: 整个观测期高寒草甸土壤表现为CO2的源, 土壤CO2通量的日变化范围为2.52~532.81 mg·m-2·h-1. 土壤CO2年排放总量为1 429.88 g·m-2, 年均通量为163.23 mg·m-2·h-1; 其中, CO2通量与空气温度和相对湿度、活动层表层2 cm、10 cm、20 cm、30 cm 土壤温度、含水量和盐分均显著相关. 2 cm土壤温度、空气温度和总辐射、空气温度、2 cm土壤盐分分别是影响活动层表层2 cm土壤完全融化期、冻结过程期、完全冻结期、融化过程期土壤CO2通量的最重要因子. 在完全融化期、冻结过程期和整个观测期, 拟合最佳的温度因子变化分别能够解释土壤CO2通量变化的72.0%、82.0%和38.0%, 对应的Q10值分别为1.93、6.62和2.09. 冻融期(含融化过程期和冻结过程期)和完全冻结期的土壤CO2排放量分别占年排放总量的15.35%和11.04%, 在年排放总量估算中不容忽视.  相似文献   

10.
2030年前实现碳达峰,2060年前实现碳中和是2020年我国提出的国家重大战略目标.以当前我国的二氧化碳排放及能源结构现状,要实现这一伟大目标形势十分严峻.介绍了全球碳循环过程,阐述了碳源与碳汇对于大气CO2浓度的贡献,从减源与增汇2个方面,初步分析了地质调查在推动碳达峰与碳中和目标实现中的作用与可能的贡献,并提出了...  相似文献   

11.
通过对四川省雅安龙苍沟峨眉山玄武岩小流域的水化学组成研究,分析了不同物质来源对小流域溪水溶解质的贡献,并对该小流域岩石风化速率和CO2消耗速率进行了估算。结果表明,龙苍沟流域溪水呈中性,PH平均值为6.82。溪水中阳离子以Ca^2+为主,约占阳离子总量的56%;阴离子以HCO3^-为主,约占阴离子总量的45%。碳酸盐岩风化、硅酸盐岩风化、大气降水和人为活动对溪水阳离子平均贡献率分别为50.2%、38.2%、10.5%和1.1%。流域硅酸盐岩风化速率为37.54±24.94 t/km^2/yr,硅酸盐岩风化对大气C02消耗速率为5.4±3.6 mol C/km^2/yr。本文首次对我国峨眉山玄武岩省化学风化大气CO2消耗量进行估算,得到其年消耗通量为1.35±0.89×10^11 mol C/yr,约为全球玄武岩CO2年消耗通量的3.31±2.18%。  相似文献   

12.
Oxidized reactive nitrogen in the atmosphere mainly consists of nitrogen oxides (NO X =NO+NO2, NO3) and nitric acid. The atmospheric cycling of NO X influences the formation of ozone and hydroxyl radicals that are important for atmospheric oxidation capacity. Nitric acid, the final product of NO X oxidation, not only is an important component of particulate pollutants, but also has a direct impact on the ecosystem through dry and wet deposition. The stable nitrogen isotope (δ15N) shows the potential to study reactive nitrogen cycle, and to trace the emission, transport and deposition of reactive nitrogen from local to global scales. Here, we reviewed previous studies using δ15N to investigate NO X emission and atmospheric reactive nitrogen cycle, and discuss the uncertainties of δ15N signatures of different NO X sources from two aspects: NO X generation mechanism and NO X collection methods. We also discussed the nitrogen isotope fractionation and the consequences during the conversions of NO y molecules. We ended up with discussions on the possibility of using δ15N to trace NO X emissions. Although there are still large uncertainties in quantifying and tracing NO X emissions using nitrogen stable isotopes, such isotope tool is efficient enough to trace reactive nitrogen cycles in the atmosphere. On the basis of this, we proposed that we can combine atmospheric chemistry transmission models with isotope tracers to improve our understanding of regional and global atmospheric reactive nitrogen cycle regarding the fluxes of different emission sources, their atmospheric transformation, etc.  相似文献   

13.
人类巨量碳排放究竟导致什么后果,争议颇大,只有深入研究始新世以来大气CO2浓度与环境变化,才有可能正确认识未来人类自身巨量碳排放之后果。大量研究揭示出: 从始新世到渐新世末期,大气CO2浓度大幅下降,全球变冷,形成了大陆冰川; 中新世至今,大气CO2浓度在低浓度背景之下长周期缓慢下降。当前尚不清楚何种机制主导了这一变化过程,也不清楚形成大陆冰川的水来自何方。为此,从青藏高原深部碳循环、表层水循环和环境变化的角度探讨这些问题,再分析未来人类巨量碳排放之后果。青藏高原在生长、隆升过程中,通过硅酸岩化学风化、植物光合作用、陆内俯冲(深埋)、水岩反应等方式,持续将巨量大气CO2转化为富含碳元素的固、流体,封存在青藏高原新生的厚地壳之中,大幅降低了大气CO2浓度,导致了全球变冷、大陆内陆(含青藏高原,下同)表层失水变干,形成了大陆冰川。渐新世—中新世之交,青藏高原生长到改变大气环流的规模,形成了亚洲季风,大陆内陆进一步荒漠化,捕获CO2的量大幅下降,并与青藏高原内部所释放CO2的量达到了准动态平衡,这是中新世以来大气CO2浓度变化的主要机制。人类巨量碳排放彻底扭转了大气CO2浓度长周期缓慢下降的趋势,大陆冰川因全球变暖所形成的液态水不会长期停留在海洋里,而以大气降水的方式重新回到干冷的大陆内陆,青藏高原将因此再次成为巨型水塔,缓解30多亿人的清洁饮用水问题。持续生长的高原和当前干冷荒漠化的大陆内陆通过前述多种方式固化人类排放的巨量CO2,导致未来大气CO2浓度在较高浓度背景下保持稳定,届时沙漠变绿洲,黄土高原变成有机质丰富的黑土高原,人居环境大幅改善; 但在盆地内部,PM2.5难以扩散,易形成雾霾。全球平均海平面因海水热膨胀而缓慢上升,上升速率约为1 mm/a。水主要在大陆冰川与内陆表层之间循环,与海平面升降之间没有因果关系。因此,人类巨量碳排放所导致的全球变暖对于人类自身的发展是利大于弊。  相似文献   

14.
对取自赣南地区10个温泉的地热气体进行了气体化学成分及氦、碳、氖同位素组成的分析。该区地热气体可分为CO2型和N2型两种类型。CO2型地热气体分布在赣南东南部地区,主要成分是CO2,占总体积96.47%以上,二氧化碳气体的δ13C值为 -5.50‰~-3.49‰(PDB),平均为 -4.66‰,为幔源无机成因,其氦同位素组成为1.36~2.27 Ra,具有明显的幔源成因特征,最高约有28.2%的氦源于地幔,其N2-Ar-He关系研究表明,该型地热气体中的氮源于地幔-地壳-大气混合成因。研究揭示该区CO2型地热气体属幔源无机成因气,是地幔脱气作用的产物。N2型地热气体分布在赣南西部地区,N2含量占91.04%以上,其中二氧化碳气体的δ13C值为 -23.7‰~-12.6‰,平均为 -17.82‰,为壳源有机成因,其氦同位素组成为0.06~0.13 Ra,具有明显的壳源放射性成因特征,3He/4He 与 4He/20Ne关系和He-Ar-N2关系研究表明,N2型温泉气主要来源于大气,并有壳源气体的贡献。  相似文献   

15.
在构建分布式水文模型与生物地球化学模型的耦合模型(DTVGM-CASACNP)及应用元胞自动机-马尔科夫(CA-Markov)土地利用预测模型基础上,以滦河流域为例分析气候变化、土地利用/覆被变化(LUCC)及CO2浓度升高对径流的影响。研究结果表明: DTVGM-CASACNP耦合模型以及CA-Markov模型在滦河流域均具有较好的适用性;气候变化与土地利用/植被覆盖变化对滦河流域径流的影响较CO2浓度升高的影响程度大;未来不同情景下滦河流域2020—2049年径流呈减小趋势,大部分情景下年径流较基准年减少,与非汛期相比,滦河流域未来汛期径流对不同情景更敏感,总体上在汛期径流相对基准年减少,而在非汛期径流相对基准年增加。  相似文献   

16.
藏南碳酸岩脉成因及其气候效应   总被引:1,自引:0,他引:1  
刘焰 《地质科学》2013,48(2):384-405
始新世末期以来,全球大气CO2浓度持续下降,但长期以来不清楚为何这一时期全球大气CO2浓度下降,巨量的大气CO2赋存于何处。深入研究该问题有助于准确理解未来大气CO2浓度变化的趋势,特别是有助于进一步评估人类自身碳排放的后果。这一时期,小印度陆块持续与大亚洲陆块汇聚,导致了以喜马拉雅为代表的山脉群和青藏高原的形成。很早就有学者从地球表层碳循环的角度提出了"青藏高原的隆升导致了全球变冷"的观点,但这一观点既没有解释清楚"巨量大气CO2到何处去"的问题,也没有讨论青藏高原本身向大气圈排放CO2等问题,因此该观点最近受到了强烈的质疑。这些激烈的争论充分反映了传统的地球表层碳循环研究已不能充分满足当前社会的需求。本文从深部碳循环这个视角重新探讨青藏高原在全球碳循环中的作用。在印度与亚洲陆块持续汇聚期间,以喜马拉雅为代表的巨型山脉快速崛起,然后持续遭受化学风化作用,大量消耗大气CO2。化学风化的产物堆积在喜马拉雅山前的前陆盆地内,形成了巨量含新生碳酸盐矿物和有机碳的西瓦里克沉积杂岩,随后新生的西瓦里克杂岩又随持续平板俯冲的印度陆壳被带入青藏高原内部,与平板俯冲的印度陆壳共同经历高温变质作用。俯冲板片内的(黑)云母等含水矿物发生脱水,形成花岗岩浆。花岗岩浆再与俯冲的西瓦里克杂岩内的碳酸盐岩发生交代反应,释放出含钙、镁离子、以CO2和水为主的高温流体,本文称其为壳源火成碳酸岩浆。碳酸岩浆沿张性裂隙上侵、冷凝之后形成藏南的碳酸岩脉。虽然青藏高原内部的火山、温泉等均向大气圈排放CO2,但所排放的碳均为再循环来自大气圈的碳,并且排放量略小于吸收量,否则消耗大气CO2所新生的碳酸岩脉就不会在青藏高原内部保存下来。藏南大量晚新生代碳酸岩脉的发现充分说明了喜马拉雅山脉和藏南高原是一个巨大的碳储库,在其形成过程中将巨量大气CO2转化为流体(岩浆)的形式封存于青藏高原内部,从而大幅降低了大气CO2浓度,最终导致了全球变冷。上述过程充分说明,大气CO2浓度的变化实质上是受控于地球内部的构造运动。进一步可推论出,"全球变化"只是一个自然现象,虽然它有独特的运行轨迹,但与人类的碳排放量无因果关系。  相似文献   

17.
海表层二氧化碳分压之时间序列研究进展   总被引:1,自引:0,他引:1  
简要总结了海表层二氧化碳分压(pCO2)时间序列的研究方法,重点综述了时间序列研究在确定pCO2控制过程、揭示pCO2年际差异、监测气候事件对pCO2的影响及估算海—气二氧化碳(CO2)通量等方面的研究进展.海表层pCO2时间序列的研究方法大致可以分为2类,一类是基于船舶调查,另一类是基于浮标的CO2自动测定.时间序列研究除了能够定性地记录和追踪一些特殊和偶然的物理和生物过程对pCO2的影响外,还能够定量地给出各种过程对pCO2变化的贡献,这对揭示海洋pCO2的控制机理有着重要意义.年际尺度的时间序列观测表明:人类活动已经造成了海表层pCO2的增加,厄尔尼诺事件和拉尼娜事件对海表层pCO2和海—气CO2通量有明显影响.另外,时间序列研究能够提高海—气CO2通量估算的准确性.  相似文献   

18.
Abuse of fossil energy resources results in the excessive discharge of greenhouse gases, especially CO2, enhancing the trend of global climate warming. Carbon sequestration is an important method to lower the increasing rate of CO2 concentration in the atmosphere. Marine carbon sequestration is a novel idea for reducing CO2 emission, and its reservoir mainly includes seawater and submarine sediment, which not only possess a great potential capacity of carbon sequestration, but also have high safety in relation to continental reservoirs. In this paper, we expounded the technique principle and mechanisms of marine carbon sequestration, potential capacity and time duration of marine carbon sequestration, main factors influencing marine carbon sequestration, CO2 injection technique, impacts on marine biota from over emission of CO2 and technique monitoring the leakage of CO2. Finally, a prospect of marine carbon sequestration was proposed, and its hot topics were accordingly pointed out.  相似文献   

19.
In recent decades, humans have become a very important force in the Earth system, demonstrating that emissions (gaseous, liquid, and solid) are the cause of many of our environmental issues. These emissions are responsible for major global reorganizations of the biogeochemical cycles. The oceans are now a net sink of atmospheric CO2, whereas in their preindustrial state they were a source; the trophic state of the coastal oceans is progressively moving toward increased heterotrophy; and the terrestrial realm is now vacillating between trophic states, whereas in preindustrial times it was autotrophic. In this paper, we present model calculations that underscore the role of human-induced perturbations in changing Earth's climate, specifically the role of anthropogenic nitrogen and phosphorus in controlling processes in the global carbon cycle since the year 1850 with projections to the year 2035. Our studies show that since the late 1940's emissions of nitrogen and phosphorus have been sequestered in the terrestrial living phytomass and groundwater. This nutrient-enhanced fertilization of terrestrial biota, coupled with rising atmospheric CO2 and global temperature, has induced a sink of anthropogenic CO2 that roughly balances the emission of CO2 owing to land use change. In the year 2000, for example, the model-calculated terrestrial biotic sink was 1730 Mtons C/year, while the emission of CO2 from changes in land use was 1820 Mtons C/year, a net flux of 90 Mtons C/year emitted to the atmosphere. In the global aquatic environment, enhanced terrestrial inputs of biotically reactive phosphorus (about 8.5 Mtons P/year) and inorganic nitrogen (about 54 Mtons N/year), have induced increased new production and burial of organic carbon in marine sediments, which is a small sink of anthropogenic CO2. It is predicted that the response of the global land reservoirs of C, N, and P to sustained anthropogenic perturbations will be maintained in the same direction of change over the range of projected scenarios of global population increase and temperature change for the next 35 years. The magnitude of change is significantly larger when the global temperature increase is maximum, especially with respect to the processes of remobilization of the biotically important nutrients nitrogen and phosphorus.  相似文献   

20.
崔子恒  贺娟  贾国东 《地球科学》2021,46(1):331-340
为了讨论末次冰期以来巽他陆架东北部植被情况及巽他陆架在冰期时的碳循环意义.对位于南海西南部陆坡的18252-3站位岩心柱沉积物中长链正构烷烃组分的平均链长(ACL27-33)、碳优势指数(CPI27-33)、烷烃含量(∑oddC27-C33)、及烷烃比值等指标进行了分析.结果显示:末次冰期以来CPI27-33表现出与海...  相似文献   

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