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对可供地浸法开采的512铀矿床镭-氡放射性平衡规律进行初步研究表明,在对该矿床钻孔施工过程中,由于泥浆压力的存在,使镭-氡放射性平衡遭到破坏,严重地降低了伽玛测井的伽玛照射量率,使按伽玛测并确定的储量计算参数不准确。为此,作者对这一平衡破坏规律进行了初步研究,确定了储量计算参数的镭一氡平衡破坏修正值,既消除了伽玛测井的影响因素,又增加了20%的远景储量。建议在今后对该矿床进一步工作时,对该平衡破坏规律采用岩芯取样为主,同时辅以适量的专门物探参数观测孔进行验证的研究方案。 相似文献
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放射性平衡系数是表征铀矿床物理特性的重要参数。γ强度测量法实质上是探测铀的衰变产物氡子体的γ强度,通过它间接测铀。这只有当铀镭处于放射平衡状态时才是正确的。若铀镭的平铀状态遭到破坏,用γ法测量不加修正就不能准确地确定铀含量。因此,铀镭平衡系数及其变化规律的研究对于铀矿普查和勘探工作都有着重要的意义。 相似文献
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张锦由 《华东地质学院学报》1984,(2)
铀镭平衡系数是描述铀系中铀镭平衡状态的一个参数。它不仅关系到铀矿床储量计算的可靠性,而且关系到寻找铀矿床的某些找矿方法的应用效果。因此有必要对它作进一步的探讨。铀镭平衡系数可由下式计算: 相似文献
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氡的迁移富集及对环境的影响 总被引:1,自引:0,他引:1
氡(Rn)是镭(Ra)放射性衰变的中间产物,属于放射性惰性气体,经常溶解于水中或释放在空气中,过量则对人体健康会造成危害。地下水富集氡的程度主要取决于岩石中镭的含量和岩石的射气作用,铀矿区和含放射性元素偏高的岩石分布区,地下水氡浓度较高。地下水的运动是氡运移到地表的主要途径,空气的氡主要来源于植物的蒸发和含氡地下水的释放作用;在使用氡浓度高地下水的室内,空气的氡浓度与氡源距离和空气对流率呈负相关, 相似文献
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W. Dyck 《Journal of Geochemical Exploration》1984,20(1):85-92
Vertical profiles of 210Po in soils near the Midwest uranium deposit and an associated surficial radioactive sandstone boulder train in northern Saskatchewan show a high 210Po background in air-dried forest litter (24 pCi/g) and Ah horizon soil (11 pCi/g) relative to lower soil horizons (<1 pCi/g). These high levels mask the 210Po signal from the radioactive boulders in the near-surface soil horizons. Only in the Bf and C horizons can the existence of the radioactive boulders be inferred from 210Po determinations. For comparative purposes profiles for 226Ra, U, Ni, and other trace elements are also presented.Escape of most of the Rn from near surface soils into the atmosphere, homogenization and decay of Rn, and precipitation of decay products back onto surface soils satisfactorily explain the field observations discussed here.Compared to the highly anomalous 222Rn signal in soil gases over this boulder train the 210Po contrast is very weak and is of little use for prospecting for this type of boulder train. The relatively high 210Po background in surficial materials relative to lower soil horizons dictates that great care be taken with the 210Po method; the deepest possible horizons should be sampled. 相似文献
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David S. Vinson Avner Vengosh Daniella Hirschfeld Gary S. Dwyer 《Chemical Geology》2009,260(3-4):159-171
Naturally-occurring radionuclides (uranium, radium, and radon), major dissolved constituents, and trace elements were investigated in fresh groundwater in 117 wells in fractured crystalline rocks from the Piedmont region (North Carolina, USA). Chemical variations show a general transition between two water types: (1) slightly acidic (pH 5.0–6.0), oxic, low-total dissolved solids (TDS) waters, and (2) near neutral, oxic to anoxic, higher-TDS waters. The uranium, radium, and radon levels in groundwater associated with granite (Rolesville Granite) are systematically higher than other rock types (gneiss, metasedimentary, and metavolcanic rocks). Water chemistry plays a secondary role on radium and radon distributions as the 222Rn/226Ra activity ratio is correlated with redox-sensitive solutes such as dissolved oxygen and Mn concentrations, as well as overall dissolved solids content including major divalent cations and Ba. Since 224Ra/228Ra activity ratios in groundwater are close to 1, we suggest that mobilization of Ra and Rn is controlled by alpha recoil processes from parent nuclides on fracture surfaces, ruling out Ra sources from mineral dissolution or significant long-distance Ra transport. Alpha recoil is balanced by Ra adsorption that is influenced by redox conditions and/or ion concentrations, resulting in an approximately one order of magnitude decrease (~ 20,000 to ~ 2000) in the apparent Ra distribution coefficient between oxygen-saturated and anoxic conditions and also across the range of dissolved ion concentrations (up to ~ 7 mM). Thus, the U and Th content of rocks is the primary control on observed Ra and Rn activities in groundwater in fractured crystalline rocks, and in addition, linked dissolved solids concentrations and redox conditions impart a secondary control. 相似文献
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砂岩型铀矿是绿色经济可采的重要能源矿种,目前是世界上重要的铀矿勘探类型之一。二连盆地芒来铀矿床、鄂尔多斯盆地纳岭沟铀矿床铀矿体多呈板状产出,板状铀矿体成因备受关注。为研究砂岩型铀矿内部U、Ra和铀镭平衡系数(Kp)分布的垂向分布规律,本文以二连盆地芒来铀矿床为例,采用具有网格精度高优点的克里格插值法研究U、Ra和Kp垂向分布规律,分别利用放射性样品分析数据和定量伽马测井五点式反褶积法反演U含量数据,通过克里格法精细刻画砂岩型矿体中U、Ra和Kp分布的垂向分布规律。研究发现,该矿床板状矿体内部具有卷状的特征,Kp分布形态可以用来判断含氧含铀水的运移方向以及氧化强弱。该方法对研究铀矿体形态、铀矿成矿规律和后续地浸开采具有重要意义。 相似文献
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Américo I. Torres Carlos F. Andrade Willard S. Moore Mauricio Faleschini José L. Esteves Luis F. H. Niencheski Pedro J. Depetris 《Environmental Earth Sciences》2018,77(4):145
Submarine groundwater discharge (SGD) is herein recognized as a significant pathway of material transport from land to the coastal SW Atlantic Ocean and thus, it can be a relevant factor affecting the marine biogeochemical cycles in the region. This paper focuses on the initial measurements of 226Ra, 228Ra and 222Rn made in Patagonia’s coastal zone of Chubut and Santa Cruz provinces (42°S–48°S, Argentina). 226Ra activity ranged from 2.9 to 73.5 dpm 100 L?1, and 228Ra activity ranged from 11.9 to 311.0 dpm 100 L?1 in groundwater wells. The radium activities found in Patagonia’s marine coastal regions and adjacent shelf indicate significant enrichment throughout the coastal waters. Groundwater samples presented the largest 222Rn activity and ranged from 2.66 to 1083 dpm L?1. Conversely, in the coastal marine environment, the 222Rn activity ranged from 1.03 to 6.23 dpm L?1. The Patagonian coastal aquifer showed a larger enrichment in 228Ra than in 226Ra, which is a typical feature for sites where SGD is dominant, probably playing a significant role in the biogeochemistry of these coastal waters. 相似文献
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本文总结了706矿点水中放射性元素的富集、迁移、分布特点及其与水的化学成分的关系,作者评价了该区放射性水异常的铀成矿远景,并进一步指导了水化学找矿工作。另外,根据该矿点的水文地质条件和氡的迁移规律,定量预测了盲矿体赋存的空间位置。 相似文献
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可地浸砂岩铀矿储量计算中所需的岩矿石密度,目前用取样测定法--石蜡法获得,而放射性物探方法之一γ-γ散射测井作为参考.笔者在新疆吐哈盆地某铀矿床密度测定中,对2种方法测定的密度结果进行了资料整理、研究对比,认为后者完全可以取代前者,提供准确的岩矿石密度值. 相似文献
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The abundance and distribution of radioelements on bulk and microscopic scales were investigated in residual granitic-derived soil at a facility for investigating the movement of radon into structures. In bulk soil samples, Ra concentrations range from 0.6 to 1.3 pCi/g, and variations in Ra, Th, and K appear to be controlled mainly by heterogeneities inherited from the parent granitic rock, which contains abundant dikes and inclusions. U in soil and parent rock is concentrated in primary minerals (mainly zircon and sphene), and in secondary sites that are of greater importance for Rn emanation. The main U-bearing secondary sites are weathered sphene, grain boundary coatings, weathered biotite and plagioclase, as well as dense Fe-rich coatings and a REE-phosphate mineral present in near-vertical fracture zones in saprolite underlying shallow loam. Elevated U in these sites generally correlates with high Ti, Al, Fe, and/or P. Preferential distribution of U and Ra on grain boundaries and porous weathered minerals is reflected in relatively high Rn emanation rates in the soil. Highest emanation occurs between 1.3 and 2.3 m depth, where fine pedogenic phasesgibbsite and amorphous silica and Fe-OOH—are most abundant; it is related to fixation of Ra by these phases, which precipitate close to the surface and accumulate at these depths by illuviation. Separation of Ra from U may occur locally, given remobilization of U-series elements from secondary sites, and large differences between Ra and U sorption capabilities of several phases present in the soil. Concentration of U along permeable fracture zones in saprolite suggests that contribution of soil-gas Rn from depth (> 2 m) could be significant to Rn availability near the surface. 相似文献
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多年来我国在铀矿地质勘探取得丰硕成果的同时,也遗留了一些退役的放射性废物污染源,整治这类污染源有利于公众安全,有利于保护生态环境.整治工作中一项重要的内容,就是野外对氡(Rn)元素析出率的检测,以往的检测方法分别为局部静态法、驻极体收集积分法和活性炭吸附法.现采用HDC-90环境测氡仪可快速检测氡元素析出率. 相似文献