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1.
This study simulates how spatial variations in particle‐size emissions from a playa affect bulk and size‐resolved dust concentration profiles during two contrasting wind erosion events (a small local and a large regional event) in the Channel Country, Lake Eyre Basin, Australia. The regional event had higher dust concentration as a result of stronger frontal winds and higher erodibility across the playa. For each event, two emission scenarios are simulated to determine if measured size‐resolved dust concentration profiles can be explained by spatial variability in source area emissions. The first scenario assumes that particle‐size emissions from source areas occur at a uniform rate, while the second scenario assumes that particle‐size emissions vary between and within source areas. The uniform emission scenario, reproduced measured bulk dust concentration profiles (R2 = 0·93 regional and R2 = 0·81 local), however simulated size‐resolved dust concentration profiles had poor statistical fits to measured size‐resolved profiles for each size class (the highest were R2 = 0·5 regional and R2 = 0·3 local). For the differential particle‐size emission scenario, the fit to the measured bulk dust concentration profiles is improved (R2 = 0·97 regional and R2 = 0·83 local). However, the fit to the size‐resolved profiles improved dramatically, with the lowest being R2 = 0·89 (regional) and R2 = 0·80 (local). Particle‐size emission models should therefore be tested against both bulk and size‐resolved dust concentration profiles, since if only bulk dust concentration profiles are used model performance may be over‐stated. As the source areas in the first 90 m upwind of the tower were similar for both events, the percentage contributions of each particle‐size class to total emissions can be compared. The contribution of each particle‐size class was similar even though the wind speed, turbulence and dust concentrations were significantly different; suggesting that the contribution of each particle‐size to the total emitted dusts is not related to wind speed and turbulence. Copyright © 2012 John Wiley & Sons, Ltd.  相似文献   

2.
For the first time, vertical fluxes of mineral dust measured by Eddy Covariance in two desert sites of Northern Asia have been used to test the performances of a wind erosion model in the field. Soil parameters required by the model were obtained through field and laboratory determinations. Model predictions and direct measurements have been compared. The main finding was that the direction of the horizontal wind relative to the orientation of nebkhas played a crucial role in determining the emission of particles in one of the investigated sites. Being unable to simulate such interaction, the model generally overestimated the actual emission. It provided, instead, reliable predictions (r2 = 0·87) when the wind direction was suitable in detaching loose erodible elements placed on nebkhas thanks to their normal orientation. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

3.
Dust storms are a major contributor to soil erosion in inland Australia, and the Simpson Desert–Channel Country region is one of the most active wind erosion regions. While information is available on wind erosion rates at the land‐type level, little is known about the influence that spatial variations in the erodibility within a land type have on the resulting dust concentration profile. A Gaussian plume model, DSIS, is presented along with tower‐based dust data, to describe the influence of different spatial combinations of dust source areas, during three dust events on the Diamantina River floodplain in Western Queensland, Australia. Copyright © 2001 John Wiley & Sons, Ltd.  相似文献   

4.
Wind tunnel experiments were conducted to investigate the effects of topography on the grain size characteristics of aeolian dust deposits. Experiments were performed on three isolated hills having various size and aspect ratios. The longitudinal profile of the median grain diameter was investigated for each hill. The longitudinal dust deposition profile was also studied for nine grain size classes of between 10 and 104 µm, as were wind and dust concentration profiles in the atmosphere upwind of, over and downwind of a hill. The wind tunnel experiments show that the grain size characteristics of aeolian dust deposits are affected by topography. Most apparent is the occurrence of a zone of reduced grain size on the leeside of hills, which extends from just upwind of the summit to a distance of several times the height of the hill. Slightly coarser than normal dust is deposited on the concave windward hill slope and in a zone downwind of the area of reduced grain size, but the increase in grain size in these zones remains very small. Although the normalized dust deposition profile for a hill does not vary substantially as a function of grain size, systematic trends are observed. The most important tendencies are: (1) a progressive extension, in the downwind direction, of a zone of decreased dust deposition on the leeside of a hill (the coarser the grains, the further downwind the zone of reduced deposition extends); (2) a progressive increase in dust deposition immediately upwind of a hill (the finer the grains, the higher the deposition value upwind of a hill becomes). Both tendencies are explained by the difference in inertia of the grains, which is controlled by grain size. Copyright © 2005 John Wiley & Sons, Ltd.  相似文献   

5.
The west‐central part of South Africa's Free State Province falls within the transition zone between South Africa's sub‐humid, temperate grasslands to the east, and the semi‐arid Karoo and arid Kalahari to the south and west, respectively. The area is characterized by low rainfall (typically 500 mm or less) with high variability, but environmental conditions allow widespread dryland commercial agriculture (maize, sunflowers and stock farming). However, human activity promotes wind erosion and the area is susceptible to dust emissions. This study is the first to quantify the degree of wind erosion on the agricultural soils in the region under prevailing winter to spring climatic conditions and land management practices. Using arrays of cup anemometers, dust deposition traps and saltation impact sensors (Safires), measurements were made of the key erosivity and erodibility drivers that control the degree of wind erosion. Results demonstrate that significant quantities of dust are mobilized, particularly during the months of September and October. Thresholds of wind erosion are shown to respond particularly closely to changes in surface and aerodynamic roughness (z0) with the amount of collected dust correlating well with measures of wind erosivity that weight the impact of higher wind speeds. Given the importance of surface roughness in controlling erosion thresholds, results show that the opportunity exists for well designed farming practices to control wind erosion. However, it is likely that climatically driven environmental change will impact on some of the identified controls on erosion (wind power, moisture availability) with the result that the wind erosion hazard is likely to increase within this marginal environment. Copyright © 2010 John Wiley & Sons, Ltd.  相似文献   

6.
A conceptual model is described for the prediction of wind erosion rates dependent on the distribution of impact energy delivered to the surface by saltating grains, P[Ei], and the distribution of local surface strength, P[Es]. Methods are presented for the measurement of both distributions and consequent loss of material from the bed. It is concluded that saltating sand grains can rupture weak crusts under even moderate wind conditions, and that the rate of erosion will depend on the shape of the distribution tails. Copyright © 1999 John Wiley & Sons, Ltd.  相似文献   

7.
Deposition and erosion play a key role in the determination of the sediment budget of a river basin, as well as for floodplain sedimentation. Floodplain sedimentation, in turn, is a relevant factor for the design of flood protection measures, productivity of agro‐ecosystems, and for ecological rehabilitation plans. In the Mekong Delta, erosion and deposition are important factors for geomorphological processes like the compensation of deltaic subsidence as well as for agricultural productivity. Floodplain deposition is also counteracting the increasing climate change induced hazard by sea level rise in the delta. Despite this importance, a sediment database of the Mekong Delta is lacking, and the knowledge about erosion and deposition processes is limited. In the Vietnamese part of the Delta, the annually flooded natural floodplains have been replaced by a dense system of channels, dikes, paddy fields, and aquaculture ponds, resulting in floodplain compartments protected by ring dikes. The agricultural productivity depends on the sediment and associated nutrient input to the floodplains by the annual floods. However, no quantitative information regarding their sediment trapping efficiency has been reported yet. The present study investigates deposition and erosion based on intensive field measurements in three consecutive years (2008, 2009, and 2010). Optical backscatter sensors are used in combination with sediment traps for interpreting deposition and erosion processes in different locations. In our study area, the mean calculated deposition rate is 6.86 kg/m2 (≈ 6 mm/year). The key parameters for calculating erosion and deposition are estimated, i.e. the critical bed shear stress for deposition and erosion and the surface constant erosion rate. The bulk of the floodplain sediment deposition is found to occur during the initial stage of floodplain inundation. This finding has direct implications on the operation of sluice gates in order to optimize sediment input and distribution in the floodplains. Copyright © 2013 John Wiley & Sons, Ltd.  相似文献   

8.
Field studies conducted at Owens Lake, California, provide direct measurements of sand flux on sand sheets with zero to 20 per cent cover of salt grass. Results from 12 different sand transport events show that aerodynamic roughness length and threshold wind shear velocity increase with vegetation cover as measured by vertically projected cover and roughness density (λ). This results in a negative exponential decrease in sediment flux with increasing vegetation cover such that sand transport is effectively eliminated when the vertically projected cover of salt grass is greater than 15 per cent. A general empirical model for the relation between sand flux and vegetation cover has been derived and can be used to predict the amount of vegetation required to stabilize sand dune areas. © 1998 John Wiley & Sons, Ltd.  相似文献   

9.
Soil erosion is an important component of the global carbon cycle. However, little attention has been given to the role of aeolian processes in influencing soil organic carbon (SOC) flux and the release of greenhouse gasses, such as carbon dioxide (CO2), to the atmosphere. Understanding the magnitude and mechanisms of SOC enrichment in dust emissions is necessary to evaluate the impact of wind erosion on the carbon cycle. This research examines the SOC content and enrichment of dust emissions measured using Big Spring Number Eight (BSNE) wind‐vane samplers across five land types in the rangelands of western Queensland, Australia. Our results show that sandy soils and finer particulate quartz‐rich soils are more efficient at SOC emission and have larger SOC dust enrichment than clay‐rich aggregated soils. The SOC enrichment ratios of dusts originating from sites with sand‐rich soil ranged from 2·1–41·9, while the mean enrichment ratio for dusts originating from the clay soil was 2·1. We hypothesize that stronger inter‐particle bonds and the low grain density of the aggregated clay soil explain its reduced capacity to release SOC during saltation, relative to the particulate sandy soils. We also show that size‐selective sorting of SOC during transport may lead to further enrichment of SOC dust emissions. Two dust samples from regional transport events were found to contain 15–20% SOC. These preliminary results provide impetus for additional research into dust SOC enrichment processes to elucidate the impact of wind erosion on SOC flux and reduce uncertainty about the role of soil erosion in the global carbon cycle. Copyright © 2013 John Wiley & Sons, Ltd.  相似文献   

10.
Australian meteorological observers started using the World Meteorological Organization (WMO) weather coding system in the 1950s. This system is still in use around the world today. However, observing and recording the weather in an organized and systematic manner had been ongoing for over 100 years prior to the adoption of this coding system, and much like Australia, most countries will have historical meteorological records. In this paper we compare the wind erosion of two of the greatest droughts in Australian recorded history; the World War II (WWII) Drought (1937–1945) and the Millennium Drought (2001–2009). To do this we analysed previously unavailable meteorological observer records from the Australian Bureau of Meteorology (ABM). Wind erosion records, mostly in long‐hand written form, were translated to the modern WMO coding system for the WWII Drought and compared with the wind erosion of Australia's recently‐ended Millennium Drought, one of the longest and harshest on record. We quantify wind erosion using Dust Event Days (DED) and a modified version of a published Dust Storm Index (DSI) to show that wind erosion during the WWII Drought was up to 4.6 times higher than during the Millennium Drought. This study has international significance because it demonstrates a methodology for tracking changes in wind erosion over the past 75 years based on observer records available in every country with a history of organized weather observation. Copyright © 2014 John Wiley & Sons, Ltd.  相似文献   

11.
Seven techniques designed to measure the dry aeolian deposition of dust on a desert surface were tested during field experiments in Niger, central‐west Africa. Deposition fluxes were measured during eight periods of 3–4 days each. Experimental techniques tested were the MDCO (marble dust collector) method, the Frisbee method, the glass plate method (optical analysis of dust deposited on glass surfaces using particle imaging software), the soil surface method (deposition on a simulated desert floor) and the CAPYR (capteur pyramidal) method. Theoretical techniques tested were the inferential method and the combination method (gradient method extended with a deposition term for coarse dust particles). The results obtained by the MDCO, Frisbee, inferential and combination methods could be directly compared by converting the data to identical standard conditions (deposition on a water surface producing no resuspension). The results obtained by the other methods (glass plate, soil surface, CAPYR) were compared relatively. The study shows that the crude (unconverted) deposition fluxes of the five experimental techniques were similar, while the crude deposition fluxes calculated by the two theoretical techniques were substantially higher, of the order of four to five times as high as for the experimental techniques. Recalculation of the data to identical environmental conditions (the standard water surface) resulted in nearly identical deposition fluxes for the MDCO, Frisbee, inferential and combination techniques, although the latter two still had slightly higher values (but the differences remained small). The measurements illustrate the need to include a grain shape factor in theoretical dust deposition models. Without such a factor, theoretical models overestimate the deposition. The paper also discusses the advantages and disadvantages of the techniques tested. Copyright © 2007 John Wiley & Sons, Ltd.  相似文献   

12.
A wind tunnel study examined the effect of distributions of saltating particles on sediment surfaces which were characterized by distributions of their tensile strength. The sediments consisted of varying proportions of large sand‐sized particles with a fine particle cement. The energies of the impacting particles and the surface strengths were compared with the mass of material lost from the surface. It is important to consider distributions of parameters rather than mean values only, since abrasion and erosion may occur from surfaces not predicted from average strength and saltation velocities. At the impact velocities used in this study (mean velocity 4·4 m s?1, with standard deviation of 0·51), surfaces containing less than 12 per cent fine material were easily eroded, but insignificant erosion occurred when the fine particle content exceeded 60 per cent. Small amounts of cementing material were easily ruptured, allowing the large sand grains to be moved (largely in creep) by the bombarding particles. A significant amount of energy was lost to the bed. As the percentage of fine material increased, the surface became more difficult to break up and less energy was lost to the bed. The probability that erosion will occur for known energy distributions of impacting particles and surface strength can be calculated and the mass loss increases exponentially with a decrease in the percentage of fine cementing particles. Copyright © 2001 John Wiley & Sons, Ltd.  相似文献   

13.
Climate and land‐use changes could strongly affect wind erosion and in turn cause a series of environmental problems. Thus, the objective of this study was to assess potential wind erosion rate (PWER) response to climate and land‐use changes in the watershed of the Ningxia–Inner Mongolia Reach of the Yellow River (NIMRYR), China. The watershed of NIMRYR suffers from serious wind erosion hazards, and over recent decades, wind erosion intensity and distribution has changed, following climate and land‐use changes. To understand these processes in the NIMRYR watershed, the Integrated Wind Erosion Modelling System (IWEMS) and the Revised Wind Erosion Equation (RWEQ) were used to calculate the PWER under different climate conditions and land‐use scenarios, and to assess the influences of climate and land‐use changes on the PWER. The results show the PWER in the whole watershed had a significant declining trend from 1986 to 2013. The results of the relationship among PWER, climate change, and land‐use changes showed that climate change was the dominant control on the PWER change in this watershed. Compared to the period 1986–1995, the average PWER decreased 23.32% and 64.98% as a result of climate change in the periods 1996–2005 and 2006–2013, respectively. In contrast with climate change, the effects of land‐use changes on the average PWER were much lower, and represented a change in PWER of less than 3.3% across the whole watershed. The study method we used could provide some valuable reference for wind erosion modelling, and the research results should help climate and land‐use researchers to develop strategies to reduce wind erosion. Copyright © 2017 John Wiley & Sons, Ltd.  相似文献   

14.
As previously observed in marine sediments collected downwind of African or South American continental sources, recent studies of sediment cores collected at the bottom of Mejillones Bay in north Chile (23°S) show a laminated structure in which the amount of particles of aeolian origin and their size create significant differences between the layers. This suggests inter‐annual to inter‐decadal variations in the strength of the local southerly winds responsible for (1) the erosion of the adjacent hyperarid surface of the Mejillones Pampa, and (2) the subsequent transport of the eroded particles towards the bay. A simple model accounting for the vertical uptake, transport, and deposition of the particles initially set into motion by wind at the surface of the pampa is proposed. This model, which could be adapted to other locations, assumes that the initial rate of (vertical) uptake is proportional to the (horizontal) saltation flux quantified by means of White's equation, that particles are lifted to a height (H), increasing with the magnitude of turbulence, and that sedimentation progressively removes the coarsest particles from the air column as it moves towards the bay. In this model, the proportionality constant (A) linking the vertical flux of particles with the horizontal flux, and the injection height (H) control the magnitude and size distribution of the deposition flux in the bay. Their values are determined using the wind speed measured over the pampa and the size distribution of particles collected in sediment traps deployed in the bay as constraints. After calibration, the model is used to assess the sensitivity of the deposition flux to the wind intensity variations. The possibility of performing such quantitative studies is necessary for interpreting precisely the variability of the aeolian material in the sediment cores collected at the bottom of Mejillones Bay. Copyright © 2010 John Wiley & Sons, Ltd.  相似文献   

15.
An inexpensive, mobile field rainfall simulator and runoff plot frame were developed for use on hillside vineyards. The simulator framework and components were lightweight, readily available and easily manageable such that they can be handled by one person during transport, set–up and operation. The vineyard rainfall simulator was simpler than many of the machines in recent use for similar studies, yet offered equal or improved performance for small‐plot studies. The system developed consistent sized 2·58 mm raindrops at intensities ranging from 20 to 90 mm/h. The average distribution uniformity coefficient at an intensity of 60 mm/h was 91·7%, with a deviation of only 2·2%. This coefficient was similar to the range reported for a more complex rotating disk simulator, and was notably greater than that obtained for other similar devices. The system water capacity of 40 l allowed for 1‐h storm durations at 60 mm/h, usually sufficient time for commencement of erosion and runoff. The runoff plot frame was designed to be quickly installed, and to discourage sediment deposition in the routing of runoff to collect containers. Copyright © 2000 John Wiley & Sons, Ltd.  相似文献   

16.
Gully erosion is a significant source of fine suspended sediment (<63 μm) and associated nutrient pollution to freshwater and marine waterways. Researchers, government agencies, and monitoring groups are currently using monitoring methods designed for streams and rivers (e.g., autosamplers, rising stage samplers, and turbidity loggers) to evaluate suspended sediment in gullies. This is potentially problematic because gullies have several hydrological features and monitoring operational challenges that differ to those of continually flowing streams and rivers (e.g., short and intense flows, high suspended sediment concentrations, and rapid scouring and aggradation). Here we present a laboratory and field-based assessment of the performance of common suspended sediment monitoring techniques applied to gullies. We also evaluate a recently-described method; the pumped active suspended sediment (PASS) sampler, which has been modified for monitoring suspended sediment in gully systems. Discrete autosampling provided data at high temporal resolution, however, it had poor collection efficiency (25 ± 10%) of coarser sediment particles (i.e., sand). Rising stage sampling, while robust and cost-effective, suffered from large amounts of condensation under field conditions (25–35% of sampler volume), due to harsh climatic conditions creating large diurnal temperature differences at the field site, thereby diluting sample concentrations and introducing additional measurement uncertainty. The turbidity logger exhibited a highly variable response when calibrated at each site with physically collected suspended sediment samples (R2 = 0.17–0.83), highlighting that this approach should be used with caution. The modified PASS sampler proved to be a reliable and representative measurement method for gully sediment water quality, however, the time-integrated nature of the method limits its temporal resolution compared to the other monitoring methods. We recommend monitoring suspended sediment in alluvial gully systems using a combination of complementary techniques (e.g., PASS and RS samplers) to account for the limitations associated with individual methods.  相似文献   

17.
Wildfire is a natural component of sagebrush (Artemisia spp.) steppe rangelands that induces temporal shifts in plant community physiognomy, ground surface conditions, and erosion rates. Fire alteration of the vegetation structure and ground cover in these ecosystems commonly amplifies soil losses by wind- and water-driven erosion. Much of the fire-related erosion research for sagebrush steppe has focused on either erosion by wind over gentle terrain or water-driven erosion under high-intensity rainfall on complex topography. However, many sagebrush rangelands are geographically positioned in snow-dominated uplands with complex terrain in which runoff and sediment delivery occur primarily in winter months associated with cold-season hydrology. Current understanding is limited regarding fire effects on the interaction of wind- and cold-season hydrologic-driven erosion processes for these ecosystems. In this study, we evaluated fire impacts on vegetation, ground cover, soils, and erosion across spatial scales at a snow-dominated mountainous sagebrush site over a 2-year period post-fire. Vegetation, ground cover, and soil conditions were assessed at various plot scales (8 m2 to 3.42 ha) through standard field measures. Erosion was quantified through a network of silt fences (n = 24) spanning hillslope and side channel or swale areas, ranging from 0.003 to 3.42 ha in size. Sediment delivery at the watershed scale (129 ha) was assessed by suspended sediment samples of streamflow through a drop-box v-notch weir. Wildfire consumed nearly all above-ground live vegetation at the site and resulted in more than 60% bare ground (bare soil, ash, and rock) in the immediate post-fire period. Widespread wind-driven sediment loading of swales was observed over the first month post-fire and extensive snow drifts were formed in these swales each winter season during the study. In the first year, sediment yields from north- and south-facing aspects averaged 0.99–8.62 t ha−1 at the short-hillslope scale (~0.004 ha), 0.02–1.65 t ha−1 at the long-hillslope scale (0.02–0.46 ha), and 0.24–0.71 t ha−1 at the swale scale (0.65–3.42 ha), and watershed scale sediment yield was 2.47 t ha−1. By the second year post fire, foliar cover exceeded 120% across the site, but bare ground remained more than 60%. Sediment yield in the second year was greatly reduced across short- to long-hillslope scales (0.02–0.04 t ha−1), but was similar to first-year measures for swale plots (0.24–0.61 t ha−1) and at the watershed scale (3.05 t ha−1). Nearly all the sediment collected across all spatial scales was delivered during runoff events associated with cold-season hydrologic processes, including rain-on-snow, rain-on-frozen soils, and snowmelt runoff. Approximately 85–99% of annual sediment collected across all silt fence plots each year was from swales. The high levels of sediment delivered across hillslope to watershed scales in this study are attributed to observed preferential loading of fine sediments into swale channels by aeolian processes in the immediate post-fire period and subsequent flushing of these sediments by runoff from cold-season hydrologic processes. Our results suggest that the interaction of aeolian and cold-season hydrologic-driven erosion processes is an important component for consideration in post-fire erosion assessment and prediction and can have profound implications for soil loss from these ecosystems. © 2019 John Wiley & Sons, Ltd.  相似文献   

18.
The crater of Mount St Helens shows one of the world's highest known rates of mass wasting. On many summer days, rockfall is almost continuous, and many large rock and dirty-snow avalanches have travelled several kilometres from their sources on the crater walls. Since formation of the crater on 18 May 1980, talus cones exceeding 100 m in thickness have formed at the base of the unstable 600 m high crater walls. To estimate rates of erosion and deposition, a series of digitized topographic maps made from aerial photographs taken of the crater in 1980, 1981, 1983, 1986 and 1988 were analysed using a geographic information system. Between 1980 and 1988, 30 × 106 m3 of rock were eroded from the crater wall, representing a mean retreat rate of 2.1 m yr?1. To account for the volume increase that occurs when bedrock is transformed into scree, this volume is multiplied by 4/3; this provides an estimate of the rock-debris volume supplied to the crater floor of 40 × 106 m3. The actual volume of deposits that accumulated during this 8 year period, however, is 68 × 106 m3. The difference of 28 × 106 m3 is presumably the volume of snow intercalated between insulating layers of rock debris. Similar calculations for each of four time intervals between 1980 and 1988 suggest that wall erosion and thus talus accumulation rates are declining, but that rates will probably remain high for decades to come.  相似文献   

19.
Sediment, nutrients and pollutants discharged from sheet and interrill erosion areas by rain‐impacted flows may influence water quality in streams and rivers. The depth of water on the soil surface influences the capacity of raindrop impacts to detach soil material underlying rain‐impacted flows, and a number of so‐called process‐based and mechanistic models erroneously use equations on the basis of the effect of water depth on splash erosion to account for this effect. Also, a number of these models require complex mathematical solutions to make them operate and can only predict sediment composition and discharges well if many of their parameters are calibrated specifically to the situations where they are being applied. Experiments with rain‐impacted flows, where flow depth and velocity over eroding surfaces have been controlled, have been reported in the literature and provide more appropriate equations to account for the drop size – flow depth interactions that affect detachment and transport of particles in rain‐impacted flows. There is a need to develop modeling approaches that rely on relevant data obtained under well‐controlled flow conditions where flow depths and velocities are known. Copyright © 2012 John Wiley & Sons, Ltd.  相似文献   

20.
The inorganic silicate fraction extracted from bulk pelagic sediments from the North Pacific Ocean is eolian dust. It monitors the composition of continental crust exposed to erosion in Asia. 176Lu/177Hf ratios of modern dust are sub-chondritic between 0.011 and 0.016 but slightly elevated with respect to immature sediments. Modern dust samples display a large range in Hf isotopic composition (IC), −4.70<?Hf<+16.45, which encompasses that observed for the time series of DSDP cores 885/886 and piston core LL44-GPC3 extending back to the late Cretaceous. Hafnium and neodymium isotopic results are consistent with a dominantly binary mixture of dust contributed from island arc volcanic material and dust from central Asia. The Hf-Nd isotopic correlation for all modern dust samples, ?Hf=0.78?Nd+5.66 (n=22, R2=0.79), is flatter than those reported so far for terrestrial reservoirs. Moreover, the variability in ?Hf of Asian dust exceeds that predicted on the basis of corresponding ?Nd values (−4.7<?Hf<+2.5; −10.9<?Nd<−10.1). This is attributed to: (1) the fixing of an important unradiogenic fraction of Hf in zircons, balanced by radiogenic Hf that is mobile in the erosional cycle, (2) the elevated Lu/Hf ratio in chemical sediments which, given time, results in a Hf signature that is radiogenic compared with Hf expected from its corresponding Nd isotopic components, and (3) the possibility that diagenetic resetting of marine sediments may incorporate a significant radiogenic Hf component into diagenetically grown minerals such as illite. Together, these processes may explain the variability and more radiogenic character of Hf isotopes when compared to the Nd isotopic signatures of Asian dust. The Hf-Nd isotope time series of eolian dust are consistent with the results of modern dust except two samples that have extremely radiogenic Hf for their Nd (?Hf=+8.6 and +10.3, ?Nd=−9.5 and −9.8). These data may point to a source contribution of dust unresolved by Nd and Pb isotopes. The Hf IC of eolian dust input to the oceans may be more variable and more radiogenic than previously anticipated. The Hf signature of Pacific seawater, however, has varied little over the past 20 Myr, especially across the drastic increase of eolian dust flux from Asia around 3.5 Ma. Therefore, continental contributions to seawater Hf appear to be riverine rather than eolian. Current predictions regarding the relative proportions of source components to seawater Hf must account for the presence of a variable and radiogenic continental component. Data on the IC and flux of river-dissolved Hf to the oceans are urgently required to better estimate contributions to seawater Hf. This then would permit the use of Hf isotopes as a monitor of past changes in erosion.  相似文献   

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