天津夏季大气消光性质的研究

利用2010年夏季天津城市边界层观测站颗粒物、黑碳气溶胶、氮氧化物(NOX)浓度、地面能见度和气象梯度观测资料,分析了天津夏季大气消光特性及低能见度事件产生的原因。结果表明,天津夏季主要污染物为PM10和PM2.5,大气气溶胶消光系数为529.06M.m-1,其中,吸收系数为50.17M.m-1,散射系数为478.89M.m-1,气体吸收系数为7.74M.m-1,气溶胶单次散射反射率为0.87。天津夏季边界层大气状态有近一半的时间为中性或偏稳定层结,当出现中性或偏稳定层结大气时则有接近一半的情况出现低能见度事件(能见度<5km),影响人们的日常生活。     

利用地面水平能见度估算并分析中国地区气溶胶光学厚度长期变化特征

首先对1980年前后能见度资料非均一性进行了处理, 得到中国地区1960～2005年能见度时间序列, 并由此估算得到气溶胶光学厚度时间序列。对比已有观测及研究结果, 本文获得的气溶胶光学厚度时间序列能够较好地反映出中国地区气溶胶光学厚度长期变化特征。中国地区气溶胶光学厚度呈现逐年增加的趋势, 但1985年后增加趋势减缓, 这种变化在大城市区域表现得更为明显。中国地区气溶胶光学厚度空间分布上呈现东南部高、 西北部低的特征, 东南部地区气溶胶光学厚度普遍大于0.4, 最大值出现在四川盆地, 气溶胶光学厚度超过0.8。     

北京地区气溶胶光学厚度中长期变化特征

利用1977～1985年北京地区太阳直接辐射谱资料，分析获得了气溶胶光学厚度谱特性，使用PIS光谱仪从1993年3月到1995年3月，持续观测了北京地区晴天和少云天气的太阳直射光谱。得到了至今较为长期系统的城市大气气溶胶光学性能及特征。研究表明:（1）气溶胶光学厚度有春夏季大，秋冬季小的统计规律；（2）能见度分级后，同一能见度下气溶胶光学厚度各季节之间的差别大为减小，地面能见度对整层光学厚度表现出了较强的约束作用，文中给出了统计关系；（3）气溶胶光学厚度有逐年增高的趋势，1977年至1994年间增长了约三分之二。     

Long‐term variations in the turbidity of the arctic atmosphere in Russia

Abstract

Temporal variations of the transmission coefficient and aerosol optical depth of the atmosphere are considered using multi‐year observations at the Soviet polar stations in the Arctic. The contribution of atmospheric aerosol to the total extinction of solar radiation is estimated. A decreasing trend of atmospheric transparency due to the increase of aerosol contributing to the extinction of solar radiation during the last 25–30 years is noted. Estimates of the atmospheric aerosol influence on the incoming solar radiation indicate that a further systematic decrease of the transmission coefficient may lead to climatic changes of direct and total radiation in most polluted areas of the Arctic.     

降水现象对大气消光系数和能见度的影响

大气中各种粒子对大气消光系数和能见度有不同程度影响,除气溶胶粒子外,降水粒子对能见度影响也不可忽视。为了解降水粒子对能见度的影响,确定能见度变化与降水现象之间的关系,该文在分析降水粒子的大小、速度、形状、谱分布、光学特性等特征的基础上,忽略气溶胶粒子的影响,建立基于实测谱分布的降水与能见度的理论模型,讨论不同类型降雨、降雪对大气消光系数和能见度的影响。同时选取Parsivel降水粒子谱仪在南京地区的降雨和降雪观测记录,利用实测数据来对比验证本文所建立的降水-能见度理论模型。结果表明:能见度随着降水强度的增大呈指数降低;受降水粒子特性和天气条件等多种因素影响,能见度与降水强度之间的关系并不是唯一对应的;降雨和降雪对能见度的影响各不相同,相比而言,降雨对能见度的影响比较容易确定,而降雪对能见度的影响比较复杂,主要因为雪花或冰晶的类型复杂多变,对大气消光系数有不同程度的影响。结合理论分析和实测数据对比验证,降水现象对能见度的影响得到了证实。     

大气气溶胶散射吸湿增长特性研究进展

大气气溶胶的散射吸湿增长特性反映了相对湿度对气溶胶散射能力的影响。研究气溶胶散射吸湿增长对于评估气溶胶辐射强迫、了解气溶胶对大气能见度的影响具有重要意义。文中对气溶胶散射吸湿增长特性的研究意义、监测方法、中外研究进展、参数化拟合和模型模拟等方面进行了系统回顾和总结,并对未来发展方向做出展望。中国在该领域开展的研究数量偏少,广泛开展气溶胶散射吸湿增长特性研究十分必要。     

A study of the radiation—Climate effect of aerosol over Beijing area

In this paper, the monthly-averaged planetary albedo and equivalent blackbody temperature are calculated by using Gauss-Seidle numerical model to solve the equation or radiative transfer, based on measured aerosol data over Beijing area. With the increase of atmospheric turbidity, the planetary albedo has different characteristics in different seasons, and there is an evident decrease in the winter season. It means that the local aerosol has an heating effect to the atmosphere in winter. The correlation feature between the surface temperature and the horizontal visibility from 1963 to 1986 is analyzed, and anticorrelation is discovered in winter. It is found that surface temperature increases with the increase of aerosol.     

内蒙古东部春季三类沙尘天气气溶胶散射系数及其与PM10、能见度相关性分析

利用内蒙古东胜、锡林浩特两站2004~2006年春季（3~5月）积分浊度计的观测资料,结合同期PM10质量浓度、大气能见度等资料,分析了背景、扬沙、沙尘暴、强沙尘暴等不同强度沙尘天气气溶胶散射系数的分布特征,讨论了不同强度沙尘天气过程中散射系数、PM10、能见度的日变化规律,以及不同强度沙尘天气过程中散射系数与PM10质量浓度、散射系数与能见度的相关关系。结果表明:散射系数能够很好地反映沙尘天气强度;随沙尘天气强度增强,散射系数日变化从双峰型向单峰型转变;沙尘天气强度较弱时,PM10与散射系数的日变化不相似,强沙尘暴过程中PM10与散射系数的日变化有一定的相似性;能见度与散射系数日变化趋势相反;散射系数与PM10质量浓度呈正相关性,沙尘天气越强,相关性越好,背景、扬沙、沙尘暴、强沙尘暴相关系数分别为0.201、0.809、0.898和0.953;散射系数与能见度有指数相关关系,随沙尘天气强度增强二者相关性逐渐增强,背景、扬沙、沙尘暴、强沙尘暴相关系数分别为-0.773、-0.870、-0.918和-0.940。     

1954—2004年珠江三角洲大气能见度变化趋势

利用珠江三角洲5个城市气象观测站 (广州、深圳、台山、惠州、高要) 的长期能见度观测资料, 采用累积百分率、Ridit分析法和烟幕/霾日频率3种统计分析方法, 分析了1954—2004年珠江三角洲能见度变化趋势, 初步探讨了珠江三角洲大气环境的变化特征及其可能原因。结果表明:近50年来, 珠江三角洲城市能见度呈显著下降趋势。能见度的下降起始于20世纪70年代初, 并在经济高速发展的80—90年代初进一步恶化, 90年代中期之后虽然能见度变化趋于平缓, 但能见度下降的趋势仍未从根本上改变。珠江三角洲能见度与当地的人口增加和经济发展程度有密切的关系, 同时污染物的区域输送对西部下风向城市能见度也有很大影响。珠江三角洲能见度未得到有效改善的主要原因, 很可能是由于细粒子污染, 尤其是二次粒子前体物如SO₂和NO_X等的排放未得到有效控制。     

我国的大气透明状况

根据全国65个甲种日射站自建站起至1978年9:30,12:30,15:30各时次直接辐射的观测资料,计算了大气透明系数。为了便于各地间的比较和绘制全国分布图,所有各时次的资料都统一订正到M=2的情况下,计算中太阳常数取值S_0=1.98卡厘米~(-2)分~(-1)。 就我国的具体情况而论,地势对大气透明度的影响最为显著,直接的结果是:高原为透明度高值区,盆地为低值区。 分析了影响大气透明度的两个重要因子——水汽和气溶胶的分布特点,以及它们之间的比例关系。水汽对辐射的吸收系根据探空资料求得的整层大气的含水量按Mugge和Muller的公式计算的。     

不同场景下的交通能见度估算模型的应用

能见度监测是交通出行安全的重要保障,尤其对机场和高速公路的大范围低能见度的监测和预警更为重要。在传统人工目测方法的基础上,以激光透射能见度仪为代表的仪器测量方法更为准确,但存在探测范围小、维护成本高、全覆盖耗资大的局限性。为了克服以上缺陷,使交通能见度的估计更为灵活、高效,本文基于机场气象站点观测数据、机场大雾以及高速公路低能见度图像,构建优化三种不同场景下的能见度估计模型,并探讨了不同模型的适用性。1)基于气象站点观测的能见度估计,运用相关系数矩阵和特征重要性分析筛选出相对湿度、温度、水平风速3个变量,并考虑昼夜分别构建三元三次多项式拟合模型,模型的决定系数(R²)可达0.9以上;2)基于机场大雾图像的能见度估计深度学习模型,利用尺度不变特征变换方法提取图像关键点的特征向量,输入全连接神经网络(fully connected neural network)模型,加快训练过程并提高模型的可解释性;3)基于高速公路图像的能见度估计的反演模型,根据暗通道先验理论和能见度测量基本方程,计算大气光亮度和透射率,并根据图像距离信息得到单目图像的能见度,该方法无须预置目标物和...     

Visibility trends in six megacities in China 1973–2007

The particulate matter pollution has been serious in Chinese megacities due to the rapidly expanding economic and industrial developments, which has significant influences in atmospheric visibility. Visibility is a highly relevant factor indicating the level of atmospheric quality, and is inversely related to the optical extinction coefficient caused by gas and particle phases. In our study, visibility trends for six major megacities (Beijing, Chengdu, Guangzhou, Shanghai, Shenyang, and Xi'an) in China were evaluated during 1973–2007 on the basis of the National Climatic Data Center (NCDC) database using four measurement methods: the days per year of daily visibility < 10 km, the days per year of daily visibility > 19 km, the annual mean visibility, and the dry extinction coefficient. The annual and seasonal change trends of visibility for each city were analyzed by using a linear regression model. The annual mean visibilities for the six cities (Beijing, Chengdu, Guangzhou, Shanghai, Shenyang, and Xi'an) were 10.67, 8.60, 10.76, 8.59, 8.16, and 9.74 km respectively. Shenyang has experienced a significant increasing trend during the entire time series while visibilities for other five sites showed decreasing trends especially since the middle of 1990s. In the southern and midwestern regions (Chengdu, Guangzhou, Shanghai, and Xi'an), visibility was best in summer, whereas in the northern regions (Beijing and Shenyang), visibility was best in spring. Mean visibility in spring was worst at Guangzhou, while for the other five cities visibility in winter was worst, probably because of coal burning during the heating period. The general degradation of visibility in these megacities was probably due to the excess aerosol loading. Consequently, an urgent targeted reduction of aerosol pollution may be needed for the sake of better air quality in Chinese megacities.     

灰霾过程中的气溶胶特性观测研究

结合太阳光度计、激光雷达以及其他相关数据对河北香河县2007年4月初的一次灰霾天气过程中的气溶胶特性进行了遥感研究。研究表明,在这次灰霾的爆发期间,能见度从20 km下降到3 km左右;气溶胶光学厚度（AOD）在3个波段上都明显增加,特别是380 nm处的AOD从6日的031增长到10日的140;Angstrom指数(ALPHA)也明显下降,例如340~440 nm处的ALPHA从7日的145下降到10日的099。从AOD和ALPHA在短波处的较大变化、体积浓度谱的粗模态粒子的大量增加和PM10浓度值的变化分析来看,这次灰霾过程中的气溶胶数浓度明显增加,其中还含有大颗粒物的大量导入。激光雷达探测消光系数的垂直分布也显示气溶胶在垂直高度上达到了近3 000 m左右。从微物理特征的变化上看,这次灰霾过程中局地气溶胶的散射能力增强,吸收能力减弱。另外,通过HYSPLIT模式对后向轨迹的模拟和对NCEP数据的分析,发现这次灰霾过程中所包含的大颗粒物的主要源地可能是蒙古地区,所以气溶胶呈现了一定的沙尘气溶胶特征。     

Atmospheric transparency over central Yakutia from the sun photometer data in 2004—2014

The transparency of the atmosphere over the central part of Yakutia is classified using ground-based observations of aerosol optical depth (AOD) for the period of 2004-2014. The annual variations in monthly mean values of AOD are compared with satellite monitoring data. It is revealed that every year the days with the values of AOD corresponding to the class III of atmospheric transparency (turbid atmosphere) made up 25-30% of the total number of AOD measurement days.     

基于腔减相移光谱技术测量大气气溶胶消光系数的应用研究

基于腔减相移光谱(CAPS)技术检测灵敏度高、光源性价比好、容易控制和有效吸收光程长等优点,搭建了一套基于CAPS技术的连续测量大气气溶胶消光系数的监测系统。测试系统高反射镜片反射率约为0.9999,对应有效光程约为4.4 km;通过Allan方差测试分析系统最佳积分时间约为80 s,对应消光系数检测极限为0.06Mm-1;将系统应用于实际大气气溶胶消光系数的12个周期和48 h连续监测,显示空腔相移基本稳定,样品测量相移偏移明显,反演得到的大气能见度结果稳定可靠。由此表明,研制的基于CAPS技术的大气气溶胶消光系数连续测量系统应用于实际的测量是完全可行的。     

以黑体为目标的能见度参考标准试验研究

黑体为目标的能见度测量是从科西米德定律出发,通过工业相机对黑体目标物进行拍摄,建立黑体和背景天空的数学模型,求得能见度。分析表明:当能见度小于30 km,黑体黑度和CCD(change-coupled device)工业相机的面非均匀性对该方法测得的能见度造成的误差约为3.7%。该方法与前向散射能见度仪测量进行对比,能见度变化趋势上具有一致性;但在高能见度时,黑体能见度测量值大于前向散射能见度测量值,低能见度时,黑体测量值小于前向散射能见度测量值。     

Long-term Variability of Integral and Spectral Transparency of the Atmosphere at Mirny Observatory,Antarctica

The aerosol optical depth of the atmosphere obtained from spectral sun photometer measurements and the integral optical depth determined from standard actinometric observations of direct solar radiation are the parameters of the optical state of the atmosphere. The quantitative estimates of the integral transparency and aerosol optical depth of the atmosphere in Antarctica are presented, their long-term variability over the entire period of observations is analyzed. The comparison of obtained data with the estimates for other natural regions and conditions revealed that during the periods without the impact of volcanic eruptions, the levels of atmospheric aerosol turbidity in Antarctica over the recent decades are minimal on the planet and can be considered as global background characteristics.     

青藏高原大气气溶胶研究进展

文中综述了近30年来青藏高原大气气溶胶的研究现状,包括青藏高原大气气溶胶光学厚度、气溶胶面密度等的时空变化特征,大气气溶胶化学成分分析及气候效应的研究等。大多利用卫星、激光雷达及地面采样等资料分析研究气溶胶。青藏高原大气气溶胶研究已经取得了显著进展。文中主要综述了该领域的研究成果,并对其今后的研究进行了展望。      

Effects of additional HONO sources on visibility over the North China Plain

The objective of the present study was to better understand the impacts of the additional sources of nitrous acid （HONO） on visibility, which is an aspect not considered in current air quality models. Simulations of HONO contributions to visibility over the North China Plain （NCP） during August 2007 using the fully coupled Weather Research and Forecasting/Chemistry （WRF/Chem） model were performed, including three additional HONO sources： （1） the reaction of photo-excited nitrogen dioxide （NO~） with water vapor; （2） the NO2 heterogeneous reaction on aerosol surfaces; and （3） HONO emissions. The model generally reproduced the spatial patterns and diurnal variations of visibility over the NCP well. When the additional HONO sources were included in the simulations, the visibility was occasionally decreased by 20%-30% （3-4 km） in local urban areas of the NCP. Monthly-mean concentrations of NO3, NH＋, SO]- and PM2.5 were increased by 20%-52% （3-11μg m-3）, 10%-38%, 6%-10%, and 6%-11% （9-17 μg m-3）, respectively; and in urban areas, monthly-mean accumulation- mode number concentrations （AMNC） and surface concentrations of aerosols were enhanced by 15%-20% and 10%-20%, respectively. Overall, the results suggest that increases in concentrations of PM2.5, its hydrophilic components, and AMNC, are key factors for visibility degradation. A proposed conceptual model for the impacts of additional HONO sources on visibility also suggests that visibility estimation should consider the heterogeneous reaction on aerosol surfaces and the enhanced atmospheric oxidation capacity due to additional HONO sources, especially in areas with high mass concentrations of NOx and aerosols.     

天津冬季大气能见度与空气污染的相互关系

为探求天津冬季大气能见度特征与空气污染的相互关系,于2008年12月至2009年1月连续观测大气能见度和空气污染物浓度(PM10、PM2.5质量浓度,O_3、NO_2和SO_2体积浓度),并结合相对湿度进行相关分析。结果表明:天津冬季大气能见度平均值为11.59 km,日变化呈明显的单峰特征,其变化特征受到空气污染物,尤其是气溶胶质量浓度及相对湿度变化共同影响;观测期内霾的发生频率接近50%;采用非线性回归方程拟合能见度与气溶胶质量浓度相互关系显示,PM2.5质量浓度对水平能见度的贡献大于PM10质量浓度,并且高湿情况下,能见度与气溶胶质量浓度相关性更好。