Deposition of atmospheric mineral particles in the North Pacific Ocean

Total deposition of atmospheric mineral particles (wet plus dry) has been measured during consecutive two-week sampling intervals from January, 1981 to March, 1982 at four island stations (Midway, Oahu, Enewetak, and Fanning) of the SEAREX Asian Dust Study Network in the North Pacific. The total deposition of mineral aerosol during the period from February to June is higher than that during the period from July to January at most of the stations. A systematic geographical trend is apparent in the dust flux, with greater fluxes at higher latitudes. The deposition values are correlated with the atmospheric mineral particle concentrations at these stations. The mineral particles are transported from arid regions in Asia to the North Pacific, and the annual dust deposition to the ocean appears to be dominated by sporadic dust events of short duration. Wet deposition dominates the removal of dust particles from the atmosphere over the North Pacific. The total deposition of atmospheric mineral material to the central North Pacific is estimated to be 20×10¹² g yr^-1.     

沙尘传输路径上气溶胶浓度与干沉降通量的粒径分布特征

利用2002年春季中国北京、青岛和日本福冈3个地区的分级气溶胶浓度资料,结合改进的Wil-liams模型,分析了沙尘传输路径上空气动力学直径≤11μm气溶胶(PM11)浓度和干沉降通量的粒径分布特征,并估算了黄海海域春季PM11的干沉降通量及不同粒径气溶胶的贡献。结果表明:3个地区PM11浓度粒径分布在非沙尘时期呈双峰分布,两个峰值分别出现在细颗粒(<2.1μm)部分和粗颗粒(2.1～11μm)部分;沙尘时期,3个地区PM11浓度粒径分布均趋于单峰分布,峰值位于粗颗粒部分,并且越靠近沙尘源地,这种趋势越明显。较强沙尘天气时期,粗颗粒部分的浓度峰值粒径从沙尘源地附近到黄海西岸、东岸呈降低趋势,但在一般沙尘天气时期,这种现象并不明显。沙尘时期和非沙尘时期,3个地区粗颗粒的干沉降通量均随粒径增加而增大,细颗粒的干沉降通量随粒径的变化不明显。虽然沙尘时期粗颗粒沉降通量较非沙尘时期有明显增加,但粗颗粒对PM11干沉降通量的贡献与非沙尘时期相比,并没有明显的变化。较强沙尘天气时期,3个地区粗颗粒的干沉降通量明显高于一般沙尘天气时期;细颗粒的干沉降通量较一般沙尘天气时期略有增加。黄海海域春季沙尘时期PM11的干沉降通量约为31.70～58.59mg.m-2.d-1,非沙尘时期约为8.33～15.94mg.m-2.d-1。粗颗粒是黄海海域春季PM11干沉降通量的主要贡献者,约占PM11干沉降通量的94.2%以上。     

Characterization of nutrients in the atmospheric wet and dry deposition observed at the two monitoring sites over Yellow Sea and East China Sea

To investigate the atmospheric deposition of nutrients into the coastal and shelf regions of the northwest Pacific Ocean, observation sites were established upon Qianliyan Island (within the Yellow Sea) and the Shengsi Archipelago (within the East China Sea), respectively. Nutrient concentrations, including , were determined in both aerosols and rainwater samples. The analytical results contain clear seasonal signatures, with high values during the dry season and low values during the rainy season. Similar trends are observed for deposition fluxes. The amount of wet deposition is greater than that of dry deposition for the studied nutrient species. The influence of meteorological factors such as rainfall means that samples from Qianliyan Island record higher nutrient values than those from Shengsi. Along with riverine inputs, atmospheric deposition plays an important role in determining the biogeochemistry of nutrient species in coastal and shelf oceans. An erratum to this article can be found at     

Demarcating the worldwide monsoon

Summary The monsoon is a global climate phenomenon. This paper addresses the seasonal reversal of atmospheric circulation and the transition of dry/wet spells in the monsoon regions worldwide. The NCEP/NCAR 850 hPa wind reanalysis data for 1950–1999 and the upper-tropospheric water vapour (UTWV) band brightness temperature (BT) data observed by NOAA polar orbiting satellites for 1980–1995 are used. In the tropics, there are three large wet-UTWV centres. The summer monsoon in the subtropics can be defined as the expansion of these centres associated with the influence of cross-equatorial flows. Specifically, the dry/wet spell transition is determined by the BT values that are smaller than 244 K. The regions of the South and North African monsoons, the Asian-northwest Pacific and Australian-Southwest Pacific monsoons, and the North and South American monsoons are examined with a focus on the dry/wet spell transition and stream field features. Findings suggest that the summer monsoons over many subtropical regions can be defined by both cross-equatorial flows and dry/wet spell transitions. In the mid- and low-latitudes, there exist six major dry/wet spell transition regions with a dry or wet period lasting more than one month. The region of most significant change is located over the subtropical North Africa–Asia–northwest Pacific. The others appear over subtropical South Africa, Indonesia–Australia, southwest Pacific, the Mexico-Caribbean Sea, and subtropical South America. In addition, three regions exist where only one of the two indicators (cross-equatorial flow and dry/wet transition) is satisfied. The first is near the Equator where the directions of cross-equatorial flows alternate but a dry/wet spell transition is never experienced. The second is over North Africa where only the dry/wet spell transition can be found but not the cross-equatorial flows. The third is over the mid-latitude regions in North China, South Africa, and northern North America. These regions are influenced by cross-equatorial flows but the upper-tropospheric water vapour content is not as high as that in tropical regions. Received June 29, 2000 Revised May 15, 2001     

大气污染物SOx输送方程的尺度分析

文中用量纲分析方法分析了控制大气污染物输送方程的动力学特性。提出了 6种反映大气污染物输送过程中各种动力、物理和化学过程相对重要性的动力学参数。并以硫氧化物为例进行了各参数量级大小分析 ,尤其对 3种起汇作用 (去除机理 )的机理 (化学转化、干沉降和湿清除 )在不同尺度大气污染过程中的作用进行了详细分析。结果表明 :在一般情况下 ,SO2 的气相化学作用小于干沉降和湿清除的作用 ;干沉降作用很依赖于模式最底层厚度的选取 ;在有降雨时湿清除作用一般较大。文中还对大气污染物SOx 输送方程各项特征量的量级作了分析对比 ,得出了控制不同尺度大气污染物输送过程的零级近似方程和一级近似方程 ,并指出了这些方程的基本特征     

华东地区稻麦轮作农田生态系统N2O排放的模拟研究

利用DNDC（DeNitrification and DeComposition）模式,对华东地区典型稻麦轮作农田生态系统的N2O排放特征进行了模拟研究。结果表明：该模式能模拟出轮作周期中N2O的主要排放峰值和排放趋势,但与实测值相比,模拟结果普遍有些偏小。相对而言,该模式对旱地阶段的模拟结果比较理想,尤其是对春季小麦返青至成熟期的模拟最好。因此,我们就该阶段影响N2O排放的主要因子进行了敏感性研究。结果指出,对这一阶段N2O排放影响最大的是化肥的施用,其他比较重要的影响因子还包括犁地方式、有机肥、降水量、降水中的N含量以及温度等。     

Wet deposition of sulfate in the Inland Sea region of Japan

Precipitation chemistry data derived from a sampling network operated in the Inland Sea model region (June 1984–May 1985) are used as a basis for discussing the wet deposition of sulfate on a regional scale in Japan. Horizontal distribution, seasonal variation, relationship between wet deposition and precipitation amount, sulfate/nitrate ratio, and transport of sulfate from the ocean are discussed. Temporal trends in concentrations of atmospheric sulfur compounds and sulfate wet deposition in the model region are also covered.     

Atmospheric inorganic nitrogen in marine aerosol and precipitation and its deposition to the North and South Pacific Oceans

Aerosol and rain samples were collected between 48°N and 55°S during the KH-08-2 and MR08-06 cruises conducted over the North and South Pacific Ocean in 2008 and 2009, to estimate dry and wet deposition fluxes of atmospheric inorganic nitrogen (N). Inorganic N in aerosols was composed of ~68% NH₄⁺ and ~32% NO₃^– (median values for all data), with ~81% and ~45% of each species being present on fine mode aerosol, respectively. Concentrations of NH₄⁺ and NO₃⁻ in rainwater ranged from 1.7–55 μmol L⁻¹ and 0.16–18 μmol L⁻¹, respectively, accounting for ~87% by NH₄⁺ and ~13% by NO₃⁻ of total inorganic N (median values for all data). A significant correlation (r = 0.74, p < 0.05, n = 10) between NH₄⁺ and methanesulfonic acid (MSA) was found in rainwater samples collected over the South Pacific, whereas no significant correlations were found between NH₄⁺ and MSA in rainwater collected over the subarctic (r = 0.42, p > 0.1, n = 6) and subtropical (r = 0.33, p > 0.5, n = 6) western North Pacific, suggesting that emissions of ammonia (NH₃) by marine biological activity from the ocean could become a significant source of NH₄⁺ over the South Pacific. While NO₃⁻ was the dominant inorganic N species in dry deposition, inorganic N supplied to surface waters by wet deposition was predominantly by NH₄⁺ (42–99% of the wet deposition fluxes for total inorganic N). We estimated mean total (dry + wet) deposition fluxes of atmospheric total inorganic N in the Pacific Ocean to be 32–64 μmol m⁻² d⁻¹, with 66–99% of this by wet deposition, indicating that wet deposition plays a more important role in the supply of atmospheric inorganic N than dry deposition.     

南海季风区冰相相变潜热对中尺度对流云和降水影响作用的数值模拟研究

利用可分辨云模式及中国南海北部试验区加密探空的平均水平风场、位温场和水汽场模拟分析了1998年5月15日至6月11日中国南海北部地区中尺度对流系统(Mesoscal Convective System,简称MCS)中冰相相变潜热对云和降水、辐射传输以及大尺度环境场的影响作用。研究表明,冰相相变潜热总体上不会引起明显的大气辐射通量的变化,但会引起较明显的下垫面热通量的变化。凝华潜热释放显著地增加了大气稳定度,造成对流和下垫面热通量的减弱,从而导致地面降水减小10.11%。碰冻潜热释放也使得大气稳定度增加,不利于中尺度对流系统对流的发展,区域累积降水量减小2.2%。融化潜热的冷却效应,使得融化层以下的大气降温,从而增加了低层大气的不稳定性,有利于海面热通量的输送,导致MCS降水增加4.1%。因此,冰相相变潜热对降水的影响主要是通过影响大气环境稳定,进而影响洋面感热通量和潜热通量的垂直输送和对流的发展,导致区域降水改变。     

Sulfur budget above the Eastern Mediterranean: relative contribution of anthropogenic and biogenic sources

To access the relative contribution of anthropogenic and biogenic sulfur sources to the sulfur budget in the Eastern Mediterranean, an area characterized by very high nss-     levels, measurements of both wet and dry deposition of sulfur were performed at a remote area on the island of Crete (Finokalia) during a 3-yr period (1996–1999). The estimation of dry deposition is based on both gaseous sulfur dioxide (SO₂) and particulate phase non-sea-salt sulfate (nss-     ) and methane sulfonate (MSA) measurements. During the dry period, deposition of SO₂ from long-range transport is the main component of anthropogenic sulfur deposition in the area. The results of the wet and dry deposition obtained at Finokalia have been compared with DMS emission from seawater obtained during two yearly surveys (1997–1998) in the Cretan Sea. Our results indicate that the contribution from biogenic sources to the sulfur budget in the Eastern Mediterranean, although negligible during winter, can account for up to 26% during summer.     

南沙海域近海层大气湍流结构及输送特征研究

本文根据南沙群岛渚碧礁的一次大气湍流观测资料，分析研究南沙海域的湍流热通量输送、方差相似性、风速各分量谱、温度谱及各湍流通量协谱等大气湍流结构和输送特征，并与陆地下垫面上的结果作了比较，得到了一些有关南沙海域大气湍流输送及湍流结构的新认识。     

Some diabatic indices of the monsoon circulation in the Indian region

The influence of outgoing longwave radiation anomalies on precipitation rates is studied based on the NCEP/NCAR reanalysis during the period of the summer monsoon circulation in the Indian region. The outgoing longwave radiation data are analyzed for 1987 (dry monsoon) and 1988 (wet monsoon) separately for the Arabian Sea, India, and the Bay of Bengal. It is shown that negative outgoing longwave radiation anomalies correspond to a wet Indian monsoon, and positive anomalies are associated with a dry monsoon. Calculations using the reanalysis enable the construction of a numerical algorithm of the interaction of outgoing longwave radiation, convection, and precipitation rates in the monsoon regions. The results obtained in this work are important in the verification of corresponding parameterizations of numerical atmospheric models.     

Estimates of Large-Scale Fluxes in High Latitudes from Terrestrial Biosphere Models and an Inversion of Atmospheric CO2 Measurements

It is important to improve estimates of large-scale carbon fluxes over the boreal forest because the responses of this biome to global change may influence the dynamics of atmospheric carbon dioxide in ways that may influence the magnitude of climate change. Two methods currently being used to estimate these fluxes are process-based modeling by terrestrial biosphere models (TBMs), and atmospheric inversions in which fluxes are derived from a set of observations on atmospheric CO₂ concentrations via an atmospheric transport model. Inversions do not reveal information about processes and therefore do not allow for predictions of future fluxes, while the process-based flux estimates are not necessarily consistent with atmospheric observations of CO₂. In this study we combine the two methods by using the fluxes from four TBMs as a priori fluxes for an atmospheric Bayesian Synthesis Inversion. By doing so we learn about both approaches. The results from the inversion indicate where the results of the TBMs disagree with the atmospheric observations of CO₂, and where the results of the inversion are poorly constrained by atmospheric data, the process-based estimates determine the flux results. The analysis indicates that the TBMs are modeling the spring uptake of CO₂ too early, and that the inversion shows large uncertainty and more dependence on the initial conditions over Europe and Boreal Asia than Boreal North America. This uncertainty is related to the scarcity of data over the continents, and as this problem is not likely to be solved in the near future, TBMs will need to be developed and improved, as they are likely the best option for understanding the impact of climate variability in these regions.     

Source,transport and deposition of atmospheric phosphorus over the Northwestern Mediterranean

Atmospheric concentrations and total deposition (wet+dry) of phosphorus were measured over the northwestern Mediterranean between april 1985 and march 1988. A seasonal cycle of both atmospheric concentrations and total deposition is observed, the higher values being recorded during the dry season. Air-mass trajectory analyses allow an identification of the major sources of atmospheric phosphorus: soil-derived dust from desert areas of north Africa and anthropogenic emissions from european countries. The impact of the atmospheric input as a source of phosphorus for surface Mediterrancan waters is tentatively assessed on both annual and seasonal time scales. The results suggest that the atmospheric input of phosphorus could be significant to Mediterranean oligotrophic zones, especially during summer when phosphorus input from deeper waters into the photic layer is minimum.     

Ocean heat transport into the Arctic in the twentieth and twenty-first century in EC-Earth

The ocean heat transport into the Arctic and the heat budget of the Barents Sea are analyzed in an ensemble of historical and future climate simulations performed with the global coupled climate model EC-Earth. The zonally integrated northward heat flux in the ocean at 70°N is strongly enhanced and compensates for a reduction of its atmospheric counterpart in the twenty first century. Although an increase in the northward heat transport occurs through all of Fram Strait, Canadian Archipelago, Bering Strait and Barents Sea Opening, it is the latter which dominates the increase in ocean heat transport into the Arctic. Increased temperature of the northward transported Atlantic water masses are the main reason for the enhancement of the ocean heat transport. The natural variability in the heat transport into the Barents Sea is caused to the same extent by variations in temperature and volume transport. Large ocean heat transports lead to reduced ice and higher atmospheric temperature in the Barents Sea area and are related to the positive phase of the North Atlantic Oscillation. The net ocean heat transport into the Barents Sea grows until about year 2050. Thereafter, both heat and volume fluxes out of the Barents Sea through the section between Franz Josef Land and Novaya Zemlya are strongly enhanced and compensate for all further increase in the inflow through the Barents Sea Opening. Most of the heat transported by the ocean into the Barents Sea is passed to the atmosphere and contributes to warming of the atmosphere and Arctic temperature amplification. Latent and sensible heat fluxes are enhanced. Net surface long-wave and solar radiation are enhanced upward and downward, respectively and are almost compensating each other. We find that the changes in the surface heat fluxes are mainly caused by the vanishing sea ice in the twenty first century. The increasing ocean heat transport leads to enhanced bottom ice melt and to an extension of the area with bottom ice melt further northward. However, no indication for a substantial impact of the increased heat transport on ice melt in the Central Arctic is found. Most of the heat that is not passed to the atmosphere in the Barents Sea is stored in the Arctic intermediate layer of Atlantic water, which is increasingly pronounced in the twenty first century.     

Comparison of collection methods to determine atmospheric deposition in a rural Mediterranean site (NE Spain)

Wet-only, dry-only, bulk deposition and deposition of sedimentary particles and gases deposited after the last rain (DAR) were collected weekly at La Castanya station in the Montseny mountains (NE Spain, 41°46′N, 2°21′E) from February 2009 to July 2010. These samples were analysed for pH, alkalinity, and the concentrations of major ions (Cl^?, NO₃ ^?, SO₄ ^2?, Na⁺, K⁺, Ca²⁺, Mg²⁺, NH₄ ⁺). Significant differences were observed between bulk and wet-only precipitation, with an enrichment of ions associated to coarse particles in bulk deposition. The comparison between wet and dry fluxes revealed that the removal of compounds at Montseny occurred mainly by wet deposition, which accounted for 74 % of total deposition. The dry flux was characterised by the predominance of K⁺, Ca²⁺ and Mg²⁺, which are related to coarse particles. Bulk collection methods at Montseny were considered representative of total atmospheric deposition, since bulk deposition plus DAR accounted for 97 % of total deposition measured with wet and dry-only collection devices. Thus, bulk deposition collectors can be recommended for deposition networks at remote sites (lacking electricity connection) in environments, where coarse particles are a predominant fraction of the aerosol mass.     

Sulfur dioxide in rain clouds: Gas-liquid scavenging efficiencies and wet deposition rates in the presence of formaldehyde

The interaction of formaldehyde with SO₂ dissolved in the aqueous phase of clouds leads to the formation of hydroxymethane sulfonate. The impact of this process upon the gas-liquid equilibrium distribution of SO₂ in rain clouds and the ensuing wet SO₂ precipitation rate is explored. Model vertical SO₂ distributions are derived from observational data for three atmospheric regions: continental polluted, continental remote, and marine. The wet deposition rate for SO₂ in the polluted atmosphere increases by about a factor of two in the presence of formaldehyde compared with its absence. The effect is much stronger in the remote atmosphere leading to a potentially significant enhancement of wet SO₂ deposition. In the marine atmosphere, wet deposition of SO₂ may contribute as much as 35% to the total removal rate for SO₂ by all processes including dry deposition and chemical conversion to sulfate.     

Numerical experiments for the influence of the transition zone migration on summer climate in north china

1.IntroductionManyobservationsshowthatNorthChina,especiallythePlainofNorthChina,isoneofthemostseveredroughtareasinChina.Thedroughtdisastersoccurwithahighfrequencyandawiderange,andsustainalongtime.Moreover,thehightemperatureusuallyaccomPaniesthedroughtinthecorresPOndingPeriod.Thesummerrainfallin1997islessthanhalfofnormal.Itisthemostseveredroughtdisasterduringrecentdecades.Theregionalclimateanomaliesarenodoubtinfluencedbytheglobalclimatechange.However,manyrecentobservationsandnumericalstud…     

Determination of Sulfur Balance Between the Atmosphere and a Norway Spruce Forest Ecosystem: Comparison of Gradient Dry + Wet and Throughfall Deposition Measurements

Total sulfur deposition was determined above a Norway spruce forest, in Hungary. Two methods were applied, on one hand dry + wet deposition measurements and on the other, throughfall and stemflow deposition estimations have been carried out. Results show: total depositions are 3.3 and 3.2 g S m^–2 yr^–1 determined by dry + wet and throughfall deposition methods, respectively. The share of the dry deposition in the total S-load is 73%. The agreement between the results of the two different methods is good and suggests the needlessness of complicated dry + wet flux measurements, i.e. the total and dry deposition of sulfur compounds to forests can be determined by simple throughfall and wet deposition measurements.     

A Case Study of a Typical Dust Storm Event over the Loess Plateau of Northwest China

Enhanced observational meteorological elements,energy fluxes,and the concentration of dust aerosols collected from the Semi-Arid Climate Observatory and Laboratory(SACOL) during a typical dust storm period in March 2010 at Lanzhou were used in this paper to investigate the impact of dust aerosols on near surface atmospheric variables and energy budgets.The results show that the entire dust storm event was associated with high wind velocities and decreasing air pressure,and the air changed from cold and wet to warm and dry and then recovered to its initial state.The response of energy fluxes occurred behind meteorological elements.At high dust concentration periods,the net radiation was significantly less in the daytime and higher at night,while the heat fluxes displayed the same trend,indicating the weakening of the land-atmosphere energy exchange.The results can be used to provide verification for numerical model results in semi-arid areas.