Dust aerosols above the south polar cap of Mars as seen by OMEGA

The time evolution of atmospheric dust at high southern latitudes on Mars has been determined using observations of the south seasonal cap acquired in the near infrared (1-2.65 μm) by OMEGA/Mars Express in 2005. Observations at different solar zenith angles and one EPF sequence demonstrate that the reflectance in the 2.64 μm saturated absorption band of the surface CO₂ ice is mainly due to the light scattered by aerosols above most places of the seasonal cap. We have mapped the total optical depth of dust aerosols in the near-IR above the south seasonal cap of Mars from mid-spring to early summer with a time resolution ranging from one day to one week and a spatial resolution of a few kilometers. The optical depth above the south perennial cap is determined on a longer time range covering southern spring and summer. A constant set of optical properties of dust aerosols is consistent with OMEGA observations during the analyzed period. Strong variations of the optical depth are observed over small horizontal and temporal scales, corresponding in part to moving dust clouds. The late summer peak in dust opacity observed by Opportunity in 2005 propagated to the south pole contrarily to that observed in mid spring. This may be linked to evidence for dust scavenging by water ice-rich clouds circulating at high southern latitudes at this season.     

Pollution and eutrophication history AD 1800–2005 as recorded in sediments from five lakes in Central Chile

One of the fundamental problems to quantifying past impact of anthropogenic activities is that long series of observational data for pollutant deposition and changes in the nutrient cycling of ecosystems (eutrophication) are often not available. Lake sediments may provide suitable archives to decipher the history of local and regional pollution and eutrophication.Here we provide quantitative high-resolution data for the history of airborne pollutants and eutrophication from sediments of five lakes in Central Chile between ca. AD 1800–2005. We use spheroidal carbonaceous particles (SCPs) from fossil fuel combustion and excess atmospheric Cu deposition from mining activities as a proxy for atmospheric deposition. Organic carbon and nitrogen flux rates to the sediments and C/N ratios are used as a proxy for aquatic primary production and eutrophication.We show that the lake sediment SCP and Cu records are highly consistent and depict in great detail the local and regional history of urban, industrial and transportation history as reported in independent documentary sources and statistics. The pre-industrial and pre-1950 background concentrations (and flux rates) of the substances can be quantified. We can also show that technical measures taken in the early 1980s to trim down Cu emissions from the copper mines reduced the excess atmospheric Cu fallout to the lakes by about 50%.Eutrophication of the lakes did not start before ca. 1980. Prior to that time, warm season temperatures explain most of the variance in TOC and N flux to the sediments. The three dimictic lakes show only moderate eutrophication responses to enhanced N supply (as atmospheric fallout; enrichment factors for TOC and N 1.1–2.6), suggesting that mainly phosphorus controls aquatic primary production. The meromictic lake, where phosphorus recycling is likely, shows the largest response (enrichment factors for TOC and N between 9–20).While all five lakes show overall consistent and similar trends for the pollution history during the 19th and 20th century, there are significant differences in the details of the individual profiles. This suggests that local sources are highly important and the common regional (background) signal is relatively marginal. This is very different from Europe.     

Dust deposition at the Mars Pathfinder landing site: observations and modeling of visible/near-infrared spectra

Temporal variations in the visible/near-infrared reflectance spectra of the radiometric calibration targets on the Mars Pathfinder (MPF) lander obtained by the Imager for Mars Pathfinder (IMP) camera reveal the effects of aeolian dust deposition at the MPF site throughout the mission. Sky brightness models in combination with two-layer radiative transfer models were used with these data to track changes in dust opacity on the radiometric calibration targets (RCTs) to constrain the dust deposition rate and the spectral properties of the deposited dust. Two-layer models were run assuming both linear and nonlinear dust accumulation rates, and suggest that RCT dust optical depth at the end of the 83-sol mission was 0.08 to 0.16, or on the order of 5- to 10-μm thickness for plausible values for dust porosity and grain size. These values correspond to dust fall rates of about 20-45 μm per Earth year, consistent with previous studies of dust deposition on Mars. The single scattering albedos of the dust derived from the models fall between those previously determined for atmospheric dust and bright soils. Comparisons of relative reflectance spectra calibrated using observed RCT radiances from late in the mission versus using radiances from modeled (dust-free) RCTs also reveal distinct spectral differences consistent with dust on the RCTs. Temporal variations in RCT dust opacity are not clearly linked to known passages of vortices at the MPF site, but overall suggest that deposition of dust onto the targets by local dust devils may be favored over erosion. Analyses of temporal changes in visible/near-infrared spectra will provide valuable information for future missions by constraining how dust deposition affects landed spacecraft operability (e.g., solar power availability), instrument calibration, and interpretations of surface mineralogy and composition.     

The effect of vegetation in a climate model simulation on the Younger Dryas

The effect of vegetation on the Younger Dryas (YD) climate is studied by comparing the results of four experiments performed with the ECHAM-4 atmospheric general circulation model (AGCM): (1) modern control climate, (2) simulation with YD boundary conditions, but with modern vegetation, (3 and 4) identical to (2), but with paleo-vegetation. Prescribing paleo-vegetation instead of modern vegetation resulted in temperature anomalies (both positive and negative) of up to 4°C in the Northern Hemisphere mid-latitudes, mainly as an effect of changes in forest cover (change in albedo). Moreover, changes in precipitation and evaporation were found, most notably during December–January–February (DJF) in the tropics and were caused by the replacement of forests by grasslands. These results are consistent with other model studies on the role of vegetation changes on climate and they suggest that it is important in paleoclimate simulation studies to prescribe realistic vegetation types, belonging to the period of interest. However, in our case the addition of YD vegetation did not improve the agreement with proxy data in Europe, as the temperatures were increasing during winter compared to the YD simulation with modern vegetation. It must be noted that this increase was not statistically significant. The model-data mismatch suggests that other factors probably played an important role, such as permafrost and atmospheric dust. We infer that during the last glacial-interglacial transition, the time lag between the first temperature increase and the northward migration of trees, estimated at 500–1000 years, could have delayed the warming of the Eurasian continent. The relatively open vegetation that existed during the early stages of the last glacial-interglacial transition had a relatively high albedo, thus tempering warming up of the Eurasian land surfaces.     

Yearly and seasonal variations of low albedo surfaces on Mars in the OMEGA/MEx dataset: Constraints on aerosols properties and dust deposits

The time variations of spectral properties of dark martian surface features are investigated using the OMEGA near-IR dataset. The analyzed period covers two Mars years, spanning from early 2004 to early 2008 (includes the 2007 global dust event). Radiative transfer modeling indicates that the apparent albedo variations of low to mid-latitude dark regions are consistent with those produced by the varying optical depth of atmospheric dust as measured simultaneously from the ground by the Mars Exploration Rovers. We observe only a few significant albedo changes that can be attributed to surface phenomena. They are small-scaled and located at the boundaries between bright and dark regions. We then investigate the variations of the mean particle size of aerosols using the evolution of the observed dark region spectra between 1 and 2.5 μm. Overall, we find that the observed changes in the spectral slope are consistent with a mean particle size of aerosols varying with time between 1 and 2 μm. Observations with different solar zenith angles make it possible to characterize the aerosol layer at different altitudes, revealing a decrease of the particle size of aerosols as altitude increases.     

The ultrafine mineralogy of a molten interplanetary dust particle as an example of the quench regime of atmospheric entry heating

Abstract— Melting and degassing of interplanetary dust particle L2005B22 at ～1200 °C was due to flash heating during atmospheric entry. Preservation of the porous particle texture supports rapid quenching from the peak heating temperature whereby olivine and pyroxene nanocrystals (3 nm-26 nm) show partial devitrification of the quenched melt at T ? 450 °C–740 °C. The implied ultrahigh cooling rates are calculated at ～105 °C/h–106 °C/h, which is consistent with quench rates inferred from the temperature-time profiles based on atmospheric entry heating models. A vesicular rim on a nonstoichiometric relic forsterite grain in this particle represents either evaporative magnesium loss during flash heating or thermally annealed ion implantation texture.     

Marine ice-rafted debris records constrain maximum extent of Saalian and Weichselian ice-sheets along the northern Eurasian margin

Ice-rafted debris (IRD) (>2 mm), input in eight sediment cores along the Eurasian continental margin (Arctic Ocean), have been studied over the last two glacial/interglacial cycles. Together with the revised chronologies and new micropaleontological data of two cores from the northern Barents Sea (PS2138) and northeastern Kara Sea (PS2741) spanning Marine Isotope Stages (MIS) 6 to 1, the IRD data give new insights into the glacial history of northern Eurasian ice-sheets over the last 150 ka. The chronologies of the cores are based on stable isotope records, AMS ¹⁴C datings, paleomagnetic and biostratigraphic data.Extensive episodes of northern Barents Sea ice-sheet growth, probably to the shelf edge, occurred during the late Weichselian (MIS 2) and the Saalian (MIS 6). Major IRD discharge at the MIS 4/3-transition hints to another severe glaciation, probably onto the outer shelf, during MIS 4. IRD-based instabilities of the marine-based ice margin along the northern Barents Sea between MIS 4 and 2 are similar in timing with North Atlantic Heinrich events and Nordic Seas IRD events, suggesting similar atmospheric cooling over a broad region or linkage of ice-sheet fluctuations through small sea-level events.In the relatively low-precipitation areas of eastern Eurasia, IRD peak values during Termination II and MIS 4/3-transition suggest a Kara Sea ice-sheet advance onto the outer shelf, probably to the shelf edge, during glacial MIS 6 and 4. This suggests that during the initial cooling following the interglacials MIS 5, and possibly MIS 7, the combined effect of sustained inflow of Atlantic water into the Arctic Ocean and penetration of moisture-bearing cyclones into easterly direction supported major ice build-up during Saalian (MIS 6) and Mid-Weichselian (MIS 4) glaciation. IRD peak values in MIS 5 indicate at least two advances of the Severnaya Semlya ice-sheet to the coast line during the Early Weichselian. In contrast, a distinct Kara Sea ice advance during the Late Weichselian (MIS 2) is not documented by the IRD records along the northeastern Kara Sea margin.     

The atmospheric circulation and dust activity in different orbital epochs on Mars

A general circulation model is used to evaluate changes to the circulation and dust transport in the martian atmosphere for a range of past orbital conditions. A dust transport scheme, including parameterized dust lifting, is incorporated within the model to enable passive or radiatively active dust transport. The focus is on changes which relate to surface features, as these may potentially be verified by observations. Obliquity variations have the largest impact, as they affect the latitudinal distribution of solar heating. At low obliquities permanent CO₂ ice caps form at both poles, lowering mean surface pressures. At higher obliquities, solar insolation peaks at higher summer latitudes near solstice, producing a stronger, broader meridional circulation and a larger seasonal CO₂ ice cap in winter. Near-surface winds associated with the main meridional circulation intensify and extend polewards, with changes in cap edge position also affecting the flow. Hence the model predicts significant changes in surface wind directions as well as magnitudes. Dust lifting by wind stress increases with obliquity as the meridional circulation and associated near-surface winds strengthen. If active dust transport is used, then lifting rates increase further in response to the larger atmospheric dust opacities (hence circulation) produced. Dust lifting by dust devils increases more gradually with obliquity, having a weaker link to the meridional circulation. The primary effect of varying eccentricity is to change the impact of varying the areocentric longitude of perihelion, l, which determines when the solar forcing is strongest. The atmospheric circulation is stronger when l aligns with solstice rather than equinox, and there is also a bias from the martian topography, resulting in the strongest circulations when perihelion is at northern winter solstice. Net dust accumulation depends on both lifting and deposition. Dust which has been well mixed within the atmosphere is deposited preferentially over high topography. For wind stress lifting, the combination produces peak net removal within western boundary currents and southern midlatitude bands, and net accumulation concentrated in Arabia and Tharsis. In active dust transport experiments, dust is also scoured from northern midlatitudes during winter, further confining peak accumulation to equatorial regions. As obliquity increases, polar accumulation rates increase for wind stress lifting and are largest for high eccentricities when perihelion occurs during northern winter. For dust devil lifting, polar accumulation rates increase (though less rapidly) with obliquity above o=25°, but increase with decreasing obliquity below this, thus polar dust accumulation at low obliquities may be increasingly due to dust lifted by dust devils. For all cases discussed, the pole receiving most dust shifts from north to south as obliquity is increased.     

Solar radiation incident on Mars and the outer planets: Latitudinal,seasonal, and atmospheric effects

Calculations of the daily solar radiation incident at the tops of the atmospheres of Mars and the outer planets and its variability with latitude and season are presented in a series of figures and tables similar to those for Earth in The Smithsonian Meteorological Tables. The changes in the latitudinal and seasonal distributions of daily surface insolation during the great Martian dust storm of 1971 (when Martian atmospheric optical depth increased from about τ = 0.1 to 2.0 were significant and dramatically illustrate the effect of atmospheric aerosols on surface insolation; i.e., the mean annual daily insolation at the poles decreased by more than a factor of 100 as τ increased from 0.1 to 2.0.     

Origin of the stepped topography of the Martian poles

The circumpolar stepped topography observed within the Martian polar regions can have originated from one of a limited number of processes, including (i) erosion of resistant layers, (ii) erosion rates inversely proportional to slope gradient, (iii) basal sapping, and (iv) bistable rates of erosion and deposition. The last mechanism appears most likely to operate on the polar escarpments, driven by ablation of volatiles on the dark scarps and deposition on the icy flats. Decreasing albedo and a corresponding increase in radiation input caused by dust accumulations on the ablating layered deposits on steeper slopes provides a metastable erosion rate model sufficient to produce a stepped topography. Wind erosion is presuured later to remove the loose excess residual dust which accumulated during ablation of the scarps. The ablation of the scarps contemporaneously with ice accumulation on the flats implies the layered deposits exposed on the scarps have formed beneath overlying flats, and the observed unconformities within these deposits can due to the exposure of deposits laid down under more than one flat with different gradients. The linearity and mutual parallelism of the scarps is a result of scarp retreat on a regional slope or with a prefered direction of scarf retreat. The spiral arrangement of the scarps is probably due to more rapid retreat of scarps facing slightly west of the equatorward meridian, that is, in the direction of greatest solar and atmospheric warming. The model suggest, but does not prove, that the layered deposits are mostly water ice, with small amounts of codeposited silicate dust and volcanic ash.     

Identification and physical retrieval of dust storm using three MODIS thermal IR channels

In this paper, the dust event on 7 April 2001 in northern China is investigated with three MODIS thermal infrared (IR) bands. It is found that for the dust cloud, the observed 11 μm minus 12 μm brightness temperature difference (BTD) is always negative, while the BTD of 8.5 μm minus 11 μm varies from positive to negative depending on the dust concentration. Based on these distinguishing properties, we develop a dust mask algorithm to identify the dust storm occurrence and spatial extent. The algorithm can be used successfully in both the daytime and nighttime. Using the Mie spherical scattering theory, the thermal radiation transfer through the single dust layer is performed with the widely used forward model DISTORT. Our calculations show that the dust-like aerosols can well explain the observed BTD although both of the complex refractive index and particle size of aerosols will significantly influence the BTD. When the complex refractive index is fixed (dust-like aerosols in this paper), then the dust optical thickness and effective radii of dust particles can be retrieved from the brightness temperature (BT) of the 11 μm channel and the BTD of 11 μm minus 12 μm channels, respectively. The integral dust column density can also be derived from the retrieved dust optical thickness and effective radius.     

A numerical study of the contributions of dust source regions to the global dust budget

Contributions of the nine potential dust source regions (North and South Africa, the Arabian Peninsula, Central Asia, eastern and western China, North and South America, and Australia) to the global dust budget are investigated with a global dust transport model. A six-year simulation (1990 to 1995) indicates that the greatest contributor to the global dust budget is found to be North Africa (the Sahara Desert), which accounts for 58% of the total global dust emission and 62% of the total global dust load in the atmosphere. Australian dust dominates the southern hemisphere. The dust emission and atmospheric dust load originating from East Asia (eastern and western China) are estimated to be 214 Tg yr^− 1 and 1.1 Tg, respectively, which are 11% and 6% of the total global dust emission and dust load. Dust from East Asia dominates the atmospheric load over China and Mongolia (about 70%), Korea (60%), Japan (50%), and the North Pacific Ocean (40%). The contribution of dust originating from regions other than East Asia to the dust load over these East Asian countries and the North Pacific Ocean cannot be ignored. The simulated total dust deposition flux on Greenland suggests a possible overestimation of the Saharan dust and an underestimation of the East Asian dust in the Arctic region, which may be a common problem with global dust transport models. Possible reasons for the underestimation of the East Asian dust are discussed.     

Assessing uncertainties in dust emission in the Aral Sea region caused by meteorological fields predicted with a mesoscale model

This study investigates how the choice of the planetary boundary layer (PBL) parameterization and dust emission scheme affects the prediction of dust entrainment simulated with a regional mesoscale model. For this analysis we consider a representative dust episode which occurred on April 2001 in the Aral Sea region. The meteorological fields were simulated using the PSU/NCAR MM5 modeling system considering two different boundary layer parameterizations. In each case, emitted dust fluxes were computed off-line by incorporating MM5 meteorological fields into the dust module DuMo. Several dust emission schemes with a prescribed erodible fraction and fixed threshold wind speed were the subject of our analysis. Implications to assessment of the anthropogenic fraction of dust emitted in the Aral region were investigated by conducting the full, half, and no lake modeling experiments.Our results show that the discrepancies in dust fluxes between the two different PBLs are much higher compared to the discrepancy associated with the use of considered dust production schemes. Furthermore, the choice of the PBL affects the timing and duration of a modeled dust event. We demonstrate that different combinations of the PBL parameterization and wind- or friction velocity-driven dust emission schemes can result in up to about a 50% difference in predicted dust mass caused by the Aral Sea desiccation. We found that the drying-up of the Aral cannot only affect the dust emission by expanding the source area, but also by affecting atmospheric characteristics, especially winds. These competitive factors add further complexity to quantification of the anthropogenic dust fraction in the region.     

MEDUSA: The ExoMars experiment for in-situ monitoring of dust and water vapour

Dust and water vapour are fundamental components of the Martian atmosphere. In view of tracing the past environmental conditions on Mars, that possibly favoured the appearing of life forms, it is important to study the present climate and its evolution. Here dust and water vapour have (and have had) strong influence. Of major scientific interest is the quantity and physical, chemical and electrical properties of dust and the abundance of water vapour dispersed in the atmosphere and their exchange with the surface. Moreover, in view of the exploration of the planet with automated systems and in the future by manned missions, it is of primary importance to analyse the hazards linked to these environmental factors. The Martian Environmental Dust Systematic Analyser (MEDUSA) experiment, included in the scientific payload of the ESA ExoMars mission, accommodates a complement of sensors, based on optical detection and cumulative mass deposition, that aims to study dust and water vapour in the lower Martian atmosphere. The goals are to study, for the first time, in-situ and quantitatively, physical properties of the airborne dust, including the cumulative dust mass flux, the dust deposition rate, the physical and electrification properties, the size distribution of sampled particles and the atmospheric water vapour abundance versus time.     

Effect of charging of aerosols in the lower atmosphere of Mars during the dust storm of 2001

Aerosols are very important in the Martian climate system. Aerosols get charged by the attachment of ions in the atmosphere. Charging of aerosols reduces the conductivity of the atmosphere as the very mobile ions are lost during the ion-aerosol attachment. During a dust storm the dust opacity increases and more ion-aerosol attachment process occurs and consequently conductivity reduces further. It was found that with the background aerosols (dust opacity ∼0.2), the conductivity close to the surface of Mars was reduced by a factor of 5, but during the dust storm (opacity ∼5) of 2001 the conductivity decreased by about 2 orders of magnitude.     

Optical and chemical properties of atmospheric organic aerosols

In the light of recent field and laboratory measurements we developed a structural and chemical model for organic atmospheric aerosols. The model organic aerosol consists of an aqueous core surrounded by a hydrophobic organic layer of biological origin. The role of organic aerosols is to concentrate organic materials at the surface and transport these organic molecules in the atmosphere. The nascent hydrophobic organic aerosol is not expected to nucleate clouds efficiently. Processing by atmospheric radicals creates hydrophilic sites on the surface. The processed, aged organic aerosol is expected to accommodate water and form cloud condensation nuclei. Processing of organic atmospheric aerosols implicates them in atmospheric radiative transfer.     

Energy deposition and primary chemical products in Titan’s upper atmosphere

Cassini results indicate that solar photons dominate energy deposition in Titan’s upper atmosphere. These dissociate and ionize nitrogen and methane and drive the subsequent complex organic chemistry. The improved constraints on the atmospheric composition from Cassini measurements demand greater precision in the photochemical modeling. Therefore, in order to quantify the role of solar radiation in the primary chemical production, we have performed detailed calculations for the energy deposition of photons and photoelectrons in the atmosphere of Titan and we validate our results with the Cassini measurements for the electron fluxes and the EUV/FUV emissions. We use high-resolution cross sections for the neutral photodissociation of N₂, which we present here, and show that they provide a different picture of energy deposition compared to results based on low-resolution cross sections. Furthermore, we introduce a simple model for the energy degradation of photoelectrons based on the local deposition approximation and show that our results are in agreement with detailed calculations including transport, in the altitude region below 1200 km, where the effects of transport are negligible. Our calculated, daytime, electron fluxes are in good agreement with the measured fluxes by the Cassini Plasma Spectrometer (CAPS), and the same holds for the measured FUV emissions by the Ultraviolet Imaging Spectrometer (UVIS). Finally, we present the vertical production profiles of radicals and ions originating from the interaction of photons and electrons with the main components of Titan’s atmosphere, along with the column integrated production rates at different solar zenith angles. These can be used as basis for any further photochemical calculations.     

On the Relation Between Solar Activity and Clear-Sky Terrestrial Irradiance

The Mauna Loa Observatory record of direct-beam solar irradiance measurements for the years 1958?–?2010 is analysed to investigate the variation of clear-sky terrestrial insolation with solar activity over more than four solar cycles. The raw irradiance data exhibit a marked seasonal cycle, extended periods of lower irradiance due to emissions of volcanic aerosols, and a long-term decrease in atmospheric transmission independent of solar activity. After correcting for these effects, it is found that clear-sky terrestrial irradiance typically varies by ≈?0.2±0.1 % over the course of the solar cycle, a change of the same order of magnitude as the variations of the total solar irradiance above the atmosphere. An investigation of changes in the clear-sky atmospheric transmission fails to find a significant trend with sunspot number. Hence there is no evidence for a yet unknown effect amplifying variations of clear-sky irradiance with solar activity.     

Modeling mineral dust emissions from Chinese and Mongolian deserts

The present study investigates the frequency and intensity of mineral dust emissions over the deserts of eastern Asia from 1996 to 2001. Mineral dust emissions are simulated using a physical dust emission scheme over a region extending from 35.5°N to 47°N and from 73°E to 125°E. The input parameters required by the dust emission model are (1) surface features data including aerodynamic roughness length, soil dry size distribution and texture; and (2) meteorological surface data, mainly wind speed, soil moisture and snow cover. The way by which these surface features and meteorological data can be assessed is described and discussed. The influence of soil moisture and snow cover is taken into account and their effects on simulated dust emission are quantified.The simulations reproduce on a daily basis the location and intensity of the severe events of April 1998 and spring 2001 as recorded by the meteorological stations and/or described in various studies. Based on 6 yr of simulations, the main dust source regions are identified and their relative contributions to the total dust emissions are quantified.The seasonal cycle of the dust storms frequency is well reproduced with a maximum in spring. The simulations suggest that it is mainly controlled by the emissions occurring in the Taklimakan desert in latter spring and in summer, and by those occurring in the northern deserts of China in winter. The Taklimakan desert appears to be the most frequent and steady source of dust emissions during the studied period. On the other hand, in the Gobi desert, only a few dust emission events are simulated, but the dust amount emitted during each event is generally very large. In the northern deserts of China, dust emissions are frequent and their intensity is variable.These results show an important annual and inter-annual variability of the emitted dust (between 100 Mt yr^− 1 and 460 Mt yr^− 1), mainly controlled by the occurrence of severe events in the Gobi desert and in the northern deserts of China.