中国地区边界层大气气溶胶辐射吸收特性

采用粒子采样法对中国２３个地区边界层气溶胶的吸收系数作了测量,研究了其分布特征。结果表明：中国地区边界层气溶胶的吸收系数在１０＾－６－１０＾－３ｍ＾－１之间,明显呈北高南低的趋势,四川盆地和贵州有一相对较高的中心,吸收系数与粒子含量之间的相关系数为０．７４,吸收系数与粒子含量的分布一致性较好。小颗粒的吸收性能好于大颗粒。     

Lidar Measurements of Aerosols in the Tropical Atmosphere

Measurements of atmospheric aerosols and trace gases using the Laser radar (lidar) techniques, have been in pro-gress since 1985 at the Indian Institute of Tropical Meteorology, Pune (18o32’N, 73o51’E, 559 m AMSL), India. These observations carried out during nighttime in the lower atmosphere (up to 5.5 km AGL), employing an Argon ion / Helium-Neon lidar provided information on the nature, size, concentration and other characteristics of the constituents present in the tropical atmosphere. The time-height variations in aerosol concentration and associated layer structure exhibit marked differences between the post-sunset and pre-sunrise periods besides their seasonal va-riation with maximum concentration during pre-monsoon / winter and minimum concentration during monsoon months. These observations also revealed the influence of the terrain of the experimental site and some selected me-teorological parameters on the aerosol vertical distributions. The special observations of aerosol vertical profiles ob-tained in the nighttime atmospheric boundary layer during October 1986 through September 1989 showed that the most probable occurrence of mixing depth lies between 450 and 550 m, and the multiple stably stratified aerosol lay-ers present above the mixing depth with maximum frequency of occurrence at around 750 m. This information on nighttime mixing depth / stable layer derived from lidar aerosol observations showed good agreement with the height of the ground-based shear layer / elevated layer observed by the simultaneously operated sodar at the lidar site.     

Study of background aerosols in the Antarctic troposphere

Systematic year-round observations of submicron aerosols were carried out at Syowa Station (69°00'S, 39°35'E) in 1978. On the basis of the results of these observations, it is concluded that two types of aerosols originating from different sources are present in the Antarctic croposphere. With the intrusion of maritime air, mostly in the polar night months, sea salt particles and ammonium sulfate particles contained originally in the clean maritime air are dominant. The size distribution of such aerosols is monomodal, having a single mode at around 0.03 m in radii. On the other hand, in the sunlit months, sulfuric acid droplets are predominant and the size distribution is bimodal, having an additional mode at around 0.005 m in radii. Those sulfuric acid particles seem to be formed photochemically within a specific layer in the mid to lower troposphere over Antarctica. Most Antarctic submicron particles are of tropospheric origin, not of stratospheric nor anthropogenic origin.     

Absorbing aerosols and pre-summer monsoon hydroclimate variability over the Indian subcontinent: The challenge in investigating links

The sub-monthly evolution of the interannual variations of absorbing aerosols and related hydrometeorology over South Asia in the pre-monsoon period is investigated from the analysis of pentad-resolution observational datasets.It is shown that pre-monsoon (late April–early May) variations are characterized by increased aerosols, reduced cloudiness and precipitation, and increased downward shortwave radiation. Lead-lag regressions indicate the significant influence of synoptic scale advection (and related vertical motion) in simultaneously shaping the aerosol distribution and associated significant hydroclimate (precipitation, cloudiness, surface shortwave radiation, and 2-m air temperature) over the Indo-Gangetic Plain.The above findings can be interpreted as a manifestation of the aerosol “semi-direct” effect if one is not mindful of the prevailing circulation anomalies and their concurrent impact on aerosol and hydroclimate. The complex interplay among aerosols, dynamics and precipitation also shows the challenge of extracting the aerosol impact from an observational analysis. Finally, the analysis points to the pitfalls of a columnar, circulation-blind framework in investigating aerosol–monsoon interactions, a concern of relevance in analyses of the impact of long-term aerosol trends, as well.     

Geochemistry of regional background aerosols in the Western Mediterranean

The chemical composition of regional background aerosols, and the time variability and sources in the Western Mediterranean are interpreted in this study. To this end 2002–2007 PM speciation data from an European Supersite for Atmospheric Aerosol Research (Montseny, MSY, located 40 km NNE of Barcelona in NE Spain) were evaluated, with these data being considered representative of regional background aerosols in the Western Mediterranean Basin. The mean PM₁₀, PM_2.5 and PM₁ levels at MSY during 2002–2007 were 16, 14 and 11 µg/m³, respectively. After compiling data on regional background PM speciation from Europe to compare our data, it is evidenced that the Western Mediterranean aerosol is characterised by higher concentrations of crustal material but lower levels of OM + EC and ammonium nitrate than at central European sites. Relatively high PM_2.5 concentrations due to the transport of anthropogenic aerosols (mostly carbonaceous and sulphate) from populated coastal areas were recorded, especially during winter anticyclonic episodes and summer midday PM highs (the latter associated with the transport of the breeze and the expansion of the mixing layer). Source apportionment analyses indicated that the major contributors to PM_2.5 and PM₁₀ were secondary sulphate, secondary nitrate and crustal material, whereas the higher load of the anthropogenic component in PM_2.5 reflects the influence of regional (traffic and industrial) emissions. Levels of mineral, sulphate, sea spray and carbonaceous aerosols were higher in summer, whereas nitrate levels and Cl/Na were higher in winter. A considerably high OC/EC ratio (14 in summer, 10 in winter) was detected, which could be due to a combination of high biogenic emissions of secondary organic aerosol, SOA precursors, ozone levels and insolation, and intensive recirculation of aged air masses. Compared with more locally derived crustal geological dusts, African dust intrusions introduce relatively quartz-poor but clay mineral-rich silicate PM, with more kaolinitic clays from central North Africa in summer, and more smectitic clays from NW Africa in spring.     

Scavenging of atmospheric ions and aerosols by drifting snow in Antarctica

Measurements of the small-, intermediate-, and large-ion concentrations and the air–earth current density along with simultaneous measurements of the concentration and size distribution of aerosol particles in the size ranges 4.4–163 nm and 0.5–20 μm diameter are reported for a drifting snow period after the occurrence of a blizzard at a coastal station, Maitri, Antarctica. Ion concentrations of all categories and the air–earth current simultaneously decrease by approximately an order of magnitude as the wind speed increases from 5 to 10 ms^− 1. The rate of decrease is the highest for large ions, lowest for small ions and in-between the two for intermediate ions. Total aerosol number concentration decreases in the 4.4–163 nm size range but increases in the 0.5–20 μm size range with wind speed. The size distribution of the nanometer particles shows a dominant maximum at ~ 30 nm diameter throughout the period of observations and the height of the maximum decreases with wind speed. However, larger particles show a maximum at ~ 0.7 μm diameter but the height of the maximum increases with increasing wind speed. The results are explained in terms of scavenging of atmospheric ions and aerosols by the drifting snow particles.     

华北地区气溶胶混合状态对暖云微物理特征的影响

在UWyo单组分气溶胶的绝热气块分档云模式基础上,发展了多种化学组分气溶胶的绝热气块分档云模式。利用2006年春季华北地区地面气溶胶分级采样的离子成分分析数据和同时段高空气溶胶、云微物理飞机观测资料,研究了气溶胶混合状态对暖云微物理特征的影响。模拟结果表明,华北地区气溶胶内部混合比外部混合有利于增加云凝结核数浓度、降低气块水汽最大饱和比、增加云滴数浓度。气溶胶的混合状态不同,形成的云滴谱的特征差异较大,主要体现在云滴谱的平均尺度和峰值的突出程度;云滴谱相对离散度在0.3附近变化,且随着云滴数浓度的增加,云滴谱相对离散度呈现减小的趋势。气溶胶混合状态能够影响暖云微物理特征,从而影响大气辐射和降水过程,在天气和气候变化的研究中应予以关注。     

Origin of calcium in aerosols over the western North Pacific

Weekly aerosol samples were collected from March 1981 to June 1983 at the six stations in the western North Pacific region and analyzed for Ca and Na. By coupling data with those previously reported for Al (Tsunogai et al., 1985), the following results and conclusion have been obtained. There was a positive correlation between the atmospheric concentration of Al and the concentration of nonsea salt Ca (nssCa). The nssCa/Al ratios from the six stations, however, considerably varied (from 0.84±0.36 to 3.00±1.91), and the ratios were usally larger than those of the crustal average or of usual soil in Japan. The Ca/Al ratios of Asian desert soil and loess vary from 0.52 to 1.29, which are similar to the nssCa/Al ratios of aerosols in the surface air over the western North Pacific region except at Onna, Okinawa. The exception may be due to a local effect of coral. These results suggest that a large part of nonsea salt Ca in the surface air over the western North Pacific is derived from arid regions in Asia and that the nssCa/Al ratio in aerosol varies with that of the source material.     

2009年石家庄地区大气气溶胶的飞机探测研究

利用2009年石家庄地区不同季节的3次机载粒子探测系统PMS(Particle Measurement System)的探测资料,结合地面天气形势、风场和探空资料对石家庄地区,晴空背景下大气气溶胶的统计特征、数浓度、平均粒径的垂直分布特征以及谱分布特征进行了分析。结果表明:晴天条件下气溶胶的数浓度随高度递减,粒径随高度变化不大;在数值上,4月16日气溶胶数浓度和粒径最大,其次是10月15日,最小的是6月10日,3次粒径变化幅度都不大;逆温层底层气溶胶明显积累,气溶胶浓度在1.5 km以下大气边界层内明显高于其他层次,逆温层的高度和厚度影响气溶胶的分布;3次不同季节晴天背景下石家庄地区气溶胶谱型基本一致呈单峰分布,小于0.3μm的细粒子对气溶胶的数浓度贡献最大。     

Formation and chemical composition of atmospheric aerosols in an equatorial forest area

The physical properties and the chemical composition of atmospheric aerosols have been studied in an equatorial region in the southern Congo (Africa). Field experiments were conducted between 1978 and 1983 in the equatorial forest of the Mayombe during periods where the influence of biomass burning was minimum. The results indicate that the forest is a net source of both fine particles resulting primarily from gas-to-particle conversion and coarse particles produced by mechanical processes. Carbonaceous matter is the major component of these biogenic particles but the forest is also a significant source of sulfate, nitrate, ammonium and potassium. Half of this carbon is attached to submicron particles and likely derives from organic gaseous precursors naturally emitted by the local biosphere.Presented at the international Symposium Influence of marine and terrestrial biosphere on the chemical composition of the atmosphere, held in Mainz, F.R.G., on 16–22 March 1986.     

Chemical components of lower tropospheric aerosols in the high arctic: Six years of observations

Six years of observations (1980 to 1986) of the composition of lower tropospheric aerosols at Alert on northern Ellesmere Island in the Canadian high Arctic yield insight into the seasonal variation of Arctic air pollutants as well as of substances of natural origin. A principal component analysis of 138 observations of 21 aerosol constituents (major ions, metals, nonmetallic trace elements) for the most polluted period of December to April identified not only a soil, sea salt and anthropogenic aerosol component, but also one associated with photochemical reactions in the atmosphere that occur at polar sunrise. Depending on the source of their gaseous precursors, elements in the photochemical component can be natural or anthropogenic in origin. For instance, SO₄ ^2-, existing mostly as H₂SO₄, originates probably from both anthropogenic and natural sources while Br^– is likely of marine origin. In contrast, SO₄ ^2- in the anthropogenic component has the stoichiometry of NH₄HSO₄. In the winter months, over 90% of Arctic SO₄ ^2- is in the anthropogenic and photochemical components.In winter, a substantial portion (11 to 35%) of Na⁺ is associated with the anthropogenic aerosol component suggesting either that marine aerosols have been physically or chemically modified by interactions with air pollution or that there are anthropogenic sources of Na⁺.The aerosol soil component is controlled by both local and distant dust sources. During a year, it has two peaks at Alert, one in April/May coinciding with the Asian dust storm season and one in September.There is a marked difference in the seasonal variation of particulate Br^– and iodine concentrations in the air. Both have a peak in April/May associated with polar sunrise and, hence, photochemical reactions in the atmosphere. However, iodine also peaks in early fall. This may be a product of biogenic iodine emissions to the atmosphere during secondary blooms in northern oceans in late summer.Presented at the Second Conference on Baseline Observations in Atmospheric Chemistry (SABOAC II) in Melbourne, Australia, November 1988     

Simulation of the radiative effect of black carbon aerosols and the regional climate responses over China

As part of the development work of the Chinese new regional climate model (RIEMS), the radiative process of black carbon (BC) aerosols has been introduced into the original radiative procedures of RIEMS,and the transport model of BC aerosols has also been established and combined with the RIEMS model.Using the new model system, the distribution of black carbon aerosols and their radiative effect over the China region are investigated. The influences of BC aerosole on the atmospheric radiative transfer and on the air temperature, land surface temperature, and total rainfall are analyzed. It is found that BC aerosols induce a positive radiative forcing at the top of the atmosphere (TOA), which is dominated by shortwave radiative forcing. The maximum radiative forcing occurs in North China in July and in South China in April. At the same time, negative radiative forcing is observed on the surface. Based on the radiative forcing comparison between clear sky and cloudy sky, it is found that cloud can enforce the TOA positive radiative forcing and decrease the negative surface radiative forcing. The responses of the climate system in July to the radiative forcing due to BC aerosols are the decrease in the air temperature in the middle and lower reaches of the Changjiang River and Huaihe area and most areas of South China, and the weak increase or decrease in air temperature over North China. The total rainfall in the middle and lower reaches of the Changjiang River area is increased, but it decreased in North China in July.     

山东大风天气的低频特征及机理分析

利用山东省122个国家级地面气象观测站的风速数据与欧洲中期天气预报中心（ECMWF）提供的ERA- Interim再分析数据,采用小波分析、带通滤波等方法对2015年9月—2020年9月山东的大风天气及相应的低频大气环流形势进行分析。结果表明,近几年山东的大风天气有増加的趋势,春季大风发生频次最多,秋季最少;山东半岛东部大风频次最多,鲁南地区最少;全年只有7月偏南大风站次较偏北大风多,其余月份多以偏北大风为主。山东大风具有显著的11~13 d与20~23 d的低频振荡周期。其中,春季大风以11~13 d的振荡周期为主,秋、冬季以20~23 d的振荡周期为主,夏季大风的振荡周期不明显。振荡周期的演变与大范围的大风过程有对应关系,大范围的大风过程大致发生在振荡的波峰处。春季偏北大风盛行时,多伴有经向风自北向南的传播。秋季大约以35°N为界,对流层中高层在35°N以北,经向风自南向北传播,35°N以南,则是自北向南传播,对流层中低层反之。山东春季大风产生之前,乌拉尔山东侧低频气旋与黄海上空低频反气旋同时出现并东移,之后衍生出华北低频反气旋与渤海低频气旋,这两个系统的加强促使华北上空偏北风加大,为山东大风的产生提供了可能。同时,华北地区经向风正距平逐渐被负距平所代替,是山东大风天气产生的又一先兆。     

The evolution of Pinatubo aerosols in the Arctic stratosphere during 1994–2000

Balloon-borne aerosol measurements were performed with an optical particle counter between 1994 and 2000 at Ny-Ålesund (79°N), Svarbard. Throughout the observation period, continuous decay was found in the concentrations of particles with 0.4–0.6 μm in radius in the Arctic stratosphere, suggesting that Pinatubo aerosols remained even at the end of the 1990s. The decay rate was clearly higher for larger particle sizes, and higher at higher altitude (e-folding time of 970–526 days), suggesting a gravitational sedimentation effect. For smaller particles with R<0.4 μm, slight increases in concentration with time were found, which agreed with the measurements at mid-latitude. The sulfate mass mixing ratio in the Arctic stratosphere before 1998 showed values higher than those at middle latitude, while values were almost the same in both regions after 1998. A possible explanation of the latitudinal difference is a time lag (of 0.5–1 year) in the arrival of Pinatubo aerosols in the Arctic.     

Zonal and meridional circulations in the equatorialzone as deduced from the divergence field of the surface wind

The zonal and meridional circulations and their variability are examined on the basis of the surface wind data for 1950-1979. The climatological mean zonal wind and its divergence are examined in reference to the Walker Circulation. The role played by the meridional circulation in contributing to convergence of the surface wind field within the equatorial zone is emphasized. Regression coefficients are used to infer seasonal mean anomalies of divergence of the surface wind in years when the sea level pressure is 1 hPa above normal at Darwin, a condition representative of El Nino events. It is shown that anomalies in the divergence associated with the meridional wind component are primarily responsible for the heavy precipitation in the Central Pacific, while the anomalous divergence associated with the zonal wind component may cause the drought in the Western Pacific near Indonesia. A similar pattern of divergence anomalies is evident during three consecutive seasons beginning in northern summer and ending in northern winter. The reinforcement of the Hadley Circulation during El Nino episodes is noted. It is shown that the circulations over the Atlantic Ocean and Pacific Ocean are relatively uncorrelated. The interrelation between the dipole anticyclones and the meridional cir-culation over the central Pacific is discussed.     

中尺度区域模式层顶高度对高空风场数值模拟的影响分析

本文基于中尺度区域模式WRF,开展模式层顶高度变化对高空气象要素,特别是高空风场数值模拟影响的研究。通过设计模式顶高45、5 hPa两个试验,同化来源于NOAA-15、NOAA-18、NOAA-19和METOP-2的AMSU-A辐射计高通道数据,表明提高模式层顶能够使卫星更多的高通道样本数量进入同化系统,达到减小背景场误差,同时减小高于层顶通道辐射能量对低层通道影响的目的,一定程度上改进了同化效果,从而改善高空气象要素,特别是风场的模拟效果,与观测值的均方根误差减小了约0.4~0.5 m·s^-1。     

Water-Soluble dicarboxylic acids, ketoacids and dicarbonyls in the atmospheric aerosols over the southern ocean and western pacific ocean

Water-soluble dicarboxylic acids (DCAs), ketoacids, and α-dicarbonyls in the marine aerosol samples collected over the Southern Ocean and western Pacific Ocean were determined. Oxalic acid was the most abundant species, followed by malonic acid and then succinic acid. It is suggested that aerosol concentrations of the organics over the Southern Ocean in this work represent their global background levels. Over the Southern Ocean, total concentrations of DCAs ranged from 2.9 to 7.2 ng m⁻³ (average: 4.5 ng m⁻³), ketoacids from 0.14 to 0.40 ng m⁻³ (av.: 0.28 ng m⁻³), and dicarbonyls from 0.06 to 0.29 ng m⁻³ (av.: 0.11 ng m⁻³). Over the western Pacific, total concentrations of DCAs ranged from 1.7 to 170 ng m⁻³ (av.: 60 ng m⁻³), ketoacids from 0.08 to 5.3 ng m⁻³ (av.: 1.8 ng m⁻³), and dicarbonyls from 0.03 to 4.6 ng m⁻³ (av.: 0.95 ng m⁻³). DCAs over the western Pacific have constituted a large fraction of organic aerosols with a mean DCAs-C/TC (total carbon) of 7.0% (range: 0.59–14%). Such a high value was in contrast to the low DCAs-C/TC (av.: 1.8%; range: 0.89–4.0%) for the Southern Ocean aerosols. Based on the relative abundances and latitudinal distributions of these organics, we propose that long-range atmospheric transport is more important over the western Pacific Ocean, in contrast, in situ photochemical production is more significant over the Southern Ocean although absolute concentrations of the organics are much lower.     

山东一次飑线过程的闪电特征和大风形成机制分析

利用闪电定位资料、多普勒雷达资料和卫星资料分析2016年6月13日发生在山东的一次飑线天气过程的地闪变化特征和大风形成机制,结果表明:本次过程发生在东北冷涡影响背景下,大气层结上冷下暖,随着层结不稳定性逐渐增强和不稳定能量的积蓄,在较强的深厚垂直风切变环境下触发强对流风暴进而组织成飑线.整个飑线过程中负地闪占主导地位,...     

QuikSCAT卫星散射计矢量风检验及南海月平均风场特征分析

采用中国科学院南海海洋研究所2008年建设的,西沙海洋观测研究站上的自动气象站实测数据,对亚太数据研究中心提供的近实时QuikSCAT卫星遥感风场资料(2008年4月6日—12月31日)进行了检验和统计特征分析,得出:这两者风速的相关系数为0.86,平均偏差为-1.50 m/s,均方根误差为1.71 m/s,表明QuikSCAT卫星遥感风场资料在南海具有很高的适用性。在此基础上,利用QuikSCAT卫星遥感的月平均风场资料分析了南海月平均风场特征。结果表明:(1)南海季风10月到次年3月盛行东北风,6—8月盛行西南风,4、5、9月为季风转换季节;(2)存在两个平均风速大值中心,一个位于南海南部(10°N,108°E)附近,另一个位于台湾海峡附近,其位置和强度会随着季节变化而变动。     

Wind environment in the Lee of Kauai Island,Hawaii during trade wind conditions: weather setting for the Helios Mishap

On 26 June 2003 (approximately 1030 local time) the Helios ultralight aircraft broke apart off the west coast of Kauai Island, Hawaii as it was climbing out of the Kauai wind shadow. Following the aircraft mishap, a study was carried out to understand the conditions on the day of the crash and to better characterize the wind in the lee of Kauai. As part of this effort, both aircraft measurements and numerical modelling studies were carried out. Measurements and models showed the trade wind flow was enhanced around the island creating a region of wind shear surrounding the leeside calm zone. This wind shear region was found to be vertically oriented along the south side but tilted northward with height along the northern side of the calm zone. Several other factors on the day of the crash were investigated including water vapour gradients, diurnal Island heating, and gravity waves but their possible influences on the crash could not be confirmed. While the numerical model captured the general features of the Kauai leeside winds, the orientation of the calm zone was north of the observed one.