How much information is lost by using global-mean climate metrics? an example using the transport sector

Metrics are often used to compare the climate impacts of emissions from various sources, sectors or nations. These are usually based on global-mean input, and so there is the potential that important information on smaller scales is lost. Assuming a non-linear dependence of the climate impact on local surface temperature change, we explore the loss of information about regional variability that results from using global-mean input in the specific case of heterogeneous changes in ozone, methane and aerosol concentrations resulting from emissions from road traffic, aviation and shipping. Results from equilibrium simulations with two general circulation models are used. An alternative metric for capturing the regional climate impacts is investigated. We find that the application of a metric that is first calculated locally and then averaged globally captures a more complete and informative signal of climate impact than one that uses global-mean input. The loss of information when heterogeneity is ignored is largest in the case of aviation. Further investigation of the spatial distribution of temperature change indicates that although the pattern of temperature response does not closely match the pattern of the forcing, the forcing pattern still influences the response pattern on a hemispheric scale. When the short-lived transport forcing is superimposed on present-day anthropogenic CO₂ forcing, the heterogeneity in the temperature response to CO₂ dominates. This suggests that the importance of including regional climate impacts in global metrics depends on whether small sectors are considered in isolation or as part of the overall climate change.     

Assessment of greenhouse gases emission from civil aviation in Russia

The greenhouse gases emission (CO₂, CH₄, and N₂O) from domestic and international aviation in the Russian Federation is assessed. In 2007, the total emission of CO₂, CH₄, and N₂O amounted to 18.4 million tons of CO₂-equivalent, which is 21% below the 1990 level. Carbon dioxide dominates in the component composition of the emissions, its part in 2007 accounted for 99.1% of the emission. Taking into account the tendency towards increasing fuel consumption due to intense aircraft traffic it can be expected that compared to the present level the greenhouse gases emissions in 2012 and 2020 will increase by 15 and 45%, respectively. Accounting for the increased aircraft emissions as well as plans of foreign countries to include the international aviation into the scheme of greenhouse gases emission allowance (trade credits) it is expedient to make more precise the greenhouse gases emissions from the Russian aviation based on the detailed flight data for all types of the aircraft.     

The impact of high altitude aircraft on the ozone layer in the stratosphere

The paper discusses the potential effects on the ozone layer of gases released by the engines of proposed high altitude supersonic aircraft. The major problem arises from the emissions of nitrogen oxides which have the potential to destroy significant quantities of ozone in the stratosphere. The magnitude of the perturbation is highly dependent on the cruise altitude of the aircraft. Furthermore, the depletion of ozone is substantially reduced when heterogeneous conversion of nitrogen oxides into nitric acid on sulfate aerosol particles is taken into account in the calculation. The sensitivity of the aerosol load on stratospheric ozone is investigated. First, the model indicates that the aerosol load induced by the SO₂ released by aircraft is increased by about 10–20% above the background aerosols at mid-high latitude of the Northern Hemisphere at 15 km for the NASA emission scenario A (the NASA emission scenarios are explained in Tables I to III). This increase in aerosol has small effects on stratospheric ozone. Second, when the aerosol load is increased following a volcanic eruption similar to the eruption of El Chichon (Mexico, April 1982), the ozone column in spring increases by as much as 9% in response to the injection of NO _x from the aircraft with the NASA emission scenario A. Finally, the modeled suggests that significant ozone depletion could result from the formation of additional polar stratospheric clouds produced by the injection of H₂O and HNO₃ by the aircraft engines.     

Estimates of the Climate Response to Aircraft CO2 and NO x Emissions Scenarios

A combination of linear response models is used to estimate the transient changes in the global means of carbon dioxide (CO₂) concentration, surface temperature, and sea level due to aviation. Apart from CO₂, the forcing caused by ozone (O₃) changes due to nitrogen oxide (NO_x) emissions from aircraft is also considered. The model is applied to aviation using several CO₂ emissions scenarios, based on reported fuel consumption in the past and scenarios for the future, and corresponding NO_x emissions. Aviation CO₂ emissions from the past until 1995 enlarged the atmospheric CO₂ concentration by 1.4 ppmv (1.7% of the anthropogenic CO₂ increase since 1800). By 1995, the global mean surface temperature had increased by about 0.004 K, and the sea level had risen by 0.045 cm. In one scenario (Fa1), which assumes a threefold increase in aviation fuel consumption until 2050 and an annual increase rate of 1% thereafter until 2100, the model predicts a CO₂ concentration change of 13 ppmv by 2100, causing temperature increases of 0.01, 0.025, 0.05 K and sea level increases of 0.1, 0.3, and 0.5 cm in the years 2015, 2050, and 2100, respectively. For other recently published scenarios, the results range from 5 to 17 ppmv for CO₂ concentration increase in the year 2050, and 0.02 to 0.05 K for temperature increase. Under the assumption that present-day aircraft-induced O₃ changes cause an equilibrium surface warming of 0.05 K, the transient responses amount to 0.03 K in surface temperature for scenario Fa1 in 1995. The radiative forcing due to an aircraft-induced O₃ increase causes a larger temperature change than aircraft CO₂ forcing. Also, climate reacts more promptly to changes in O₃ than to changes in CO₂ emissions from aviation. Finally, even under the assumption of a rather small equilibrium temperature change from aircraft-induced O₃ (0.01 K for the 1992 NO_x emissions), a proposed new combustor technology which reduces specific NO_x emissions will cause a smaller temperature change during the next century than the standard technology does, despite a slightly enhanced fuel consumption. Regional effects are not considered here, but may be larger than the global mean responses.     

The effect of cloud parametrization and temperature profile on the climate sensitivity to ozone perturbations

A one-dimensional radiative-convective model extending from 0 to 70 km is used to study the sensitivity of surface temperature to perturbations in the ozone profile. Several simulations have been performed for 0₃ reductions in various altitude ranges. For each case, the resulting perturbation in the thermal structure is analysed. These calculations have been repeated for several types of cloud layers with different opacities and altitudes. It is shown that the sensitivity of the surface temperature to ozone changes is dependent on the cloudiness assumed. Ozone decreases in the lower atmosphere (0–30 km) cool the surface, since the greenhouse effect is dominant in this region, and the climate sensitivity is enhanced in the presence of a cloud layer. For higher-altitude 0₃ changes (30–70 km), the sign of the surface temperature variation depends on the cloud characteristics. In fact, the latter result is mostly the consequence of the different equilibrium temperature profiles corresponding to the various types of cloudiness. When high stratospheric ozone is reduced, positive and negative surface temperature changes of several tenths of degree are respectively associated with cold and warm climatic conditions.     

Future changes of the atmospheric composition and the impact of climate change

The development of the future atmospheric chemical composition is investigated with respect to NO _y and O₃ by means of the off‐line coupled dynamic‐chemical general circulation model ECHAM3/CHEM. Two time slice experiments have been performed for the years 1992 and 2015, which include changes in sea surface temperatures, greenhouse gas concentrations, emissions of CFCs, NO _x and other species, i.e., the 2015 simulation accounts for changes in chemically relevant emissions and for a climate change and its impact on air chemistry. The 2015 simulation clearly shows a global increase in ozone except for large areas of the lower stratosphere, where no significant changes or even decreases in the ozone concentration are found. For a better understanding of the importance of (A) emissions like NO _x and CFCs, (B) future changes of air temperature and water vapour concentration, and (C) other dynamical parameters, like precipitation and changes in the circulation, diabatic circulation, stratosphere‐troposphere‐exchange, the simulation of the future atmosphere has been performed stepwise. This method requires a climate‐chemistry model without interactive coupling of chemical species. Model results show that the direct effect of emissions (A) plays a major rôle for the composition of the future atmosphere, but they also clearly show that climate change (B and C) has a significant impact and strongly reduces the NO _y and ozone concentration in the lower stratosphere.     

Subsonic aircraft and ozone trends

Growth in subsonic air traffic over the past 20 years has been dramatic, with an annual increase of }6.1% over the decade between 1978 and 1988. Furthermore, aircraft activities in the year 2000 are predicted to be double those of 1990, with a shift towards more high-flying, longhaul subsonics. Aircraft exhaust gases increase the amount of nitrogen oxides (NO _x ) in the upper troposphere/lower stratosphere through injection at cruise altitudes. Given that NO _x is instrumental in tropospheric ozone production and stratospheric ozone destruction, it is important to determine the influence of subsonic aircraft NO _x emissions on levels of atmospheric ozone. This paper describes calculations designed to investigate the impact that subsonic aircraft may already have had on the atmosphere during the 1980s, run in a 2-D chemical-radiative-transport model. The results indicate a significant increase in upper tropospheric ozone over the decade arising from aircraft emissions. However, when comparing model results with observational data, certain discrepancies appear. Lower stratospheric ozone loss over the 1980s does not appear to be greatly altered by the inclusion of aircraft emissions in the model. However, given the trend in greater numbers of long-haul subsonic aircraft, this factor must be considered in any further calculations.     

Scenarios of possible changes in atmospheric temperatures and ozone concentrations due to man's activities,estimated with a one-dimensional coupled photochemical climate model

A one-dimensional coupled climate and chemistry model has been developed to estimate past and possible future changes in atmospheric temperatures and chemical composition due to human activities. The model takes into account heat flux into the oceans and uses a new tropospheric temperature lapse rate formulation. As found in other studies, we estimate that the combined greenhouse effect of CH₄, O₃, CF₂Cl₂, CFCl₃ and N₂O in the future will be about as large as that of CO₂. Our model calculates an increase in average global surface temperatures by about 0.6°C since the start of the industrial era and predicts for A.D. 2050 a twice as large additional rise. Substantial depletions of ozone in the upper stratosphere by between 25% and 55% are calculated, depending on scenario. Accompanying temperature changes are between 15°C and 25°C. Bromine compounds are found to be important, if no rigid international regulations on CFC emissions are effective. Our model may, however, concivably underestimate possible effects of CFCl₃, CF₂Cl₂, C₂F₃Cl₃ and other CFC and organic bromine emissions on lower stratospheric ozone, because it can not simulate the rapid breakdown of ozone which is now being observed worldwide. An uncertainty study regarding the photochemistry of stratospheric ozone, especially in the region below about 25 km, is included. We propose a reaction, involving excited molecular oxygen formation from ozone photolysis, as a possible solution to the problem of ozone concentrations calculated to be too low above 45 km. We also estimate that tropospheric ozone concentrations have grown strongly in the northern hemisphere since pre-industrial times and that further large increases may take place, especially if global emissions of NO_x from fossil fuel and biomass burning were to continue to increase. Growing NO_x emissions from aircraft may play an important role in ozone concentrations in the upper troposphere and low stratosphere.     

Relative radiative forcing consequences of global emissions of hydrocarbons, carbon monoxide and NOx from human activities estimated with a zonally-averaged two-dimensional model

A global two-dimensional (altitude-latitude) chemistry transport model is used to follow the changes in the tropospheric distribution of the two major radiatively active trace gases, methane and ozone, following step changes to the sustained emissions of the short-lived trace gases methane, carbon monoxide and non-methane hydrocarbons. The radiative impacts were dependent on the latitude chosen for the applied change in emissions. Step change global warming potentials (GWPs) were derived for a range of short-lived trace gases to describe their time-integrated radiative forcing impacts for unit emissions relative to that of carbon dioxide. The GWPs show that the tropospheric chemistry of the hydrocarbons can produce significant indirect radiative impacts through changing the tropospheric distributions of hydroxyl radicals, methane and ozone. For aircraft, the indirect radiative forcing impact of the NO _x emissions appears to be greater than that from their carbon dioxide emissions. Quantitative results from this two-dimensional model study must, however, be viewed against the known inadequacies of zonally-averaged models and their poor representation of many important tropospheric processes.     

Why radiative forcing might fail as a predictor of climate change

Radiative forcing has been widely used as a metric of climate change, i.e. as a measure by which various contributors to a net surface temperature change can be quantitatively compared. The extent to which this concept is valid for spatially inhomogeneous perturbations to the climate system is tested. A series of climate model simulations involving ozone changes of different spatial structure reveals that the climate sensitivity parameter is highly variable: for an ozone increase in the northern hemisphere lower stratosphere, it is more than twice as large as for a homogeneous CO₂ perturbation. A global ozone perturbation in the upper troposphere, however, causes a significantly smaller surface temperature response than CO₂. The variability of the climate sensitivity parameter is shown to be mostly due to the varying strength of the stratospheric water vapour feedback. The variability of the sea-ice albedo feedback modifies climate sensitivity of perturbations with the same vertical structure but a different horizontal structure. This feedback is also the origin of the comparatively larger climate sensitivity to perturbations restricted to the northern hemisphere extratropics. As cloud feedback does not operate independently from the other feedbacks, quantifying its effect is rather difficult. However, its effect on the variability of for horizontally and vertically inhomogeneous perturbations within one model framework seems to be comparatively small.This revised version was published online March 2005 with corrections to table 5.     

Introduction to special section on 'East Asia Climate and Environment'

Activities within the collaborative project East Asia Climate and Environment focus on the impact on the composition of chemically active greenhouse compounds from the rapidly growing emissions in Asia. Estimates of emissions (past and future) are discussed in light of the demand for energy in the different sectors. The impact includes regional scale contributions through short-lived climate compounds like particles and ozone, while global scale contributions are demonstrated through changes in oxidation capacity affecting compounds like CH₄. One key issue is the important and increasing contribution from China to atmospheric chemical changes.     

Latitudinal dependence of signal-to-noise patterns from two general circulation models with CO2 forcing

 Detection of an enhanced greenhouse effect on climate depends on recognition of a signal of change amidst the combined noise of climatic variability and uncertainty in the nature of the signal (functional response to changing CO₂). Using two different GCMs (one with a coupled dynamic upper ocean) and an ensemble of 20 equilibrium experiments with CO₂ ranging from 100 to 3500 ppm, we find that that two measures of signal-to-noise (S/N) for the response of surface temperature to CO₂ forcing are larger over tropical and subtropical oceans than over low-latitude landmasses and larger than at higher latitudes generally. One S/N measure has the noise based solely on inherent model variability, while the other S/N measure includes both this variability and a measure of the uncertainty in the functional nature of the signal. Although the experiments were not for transient forcing and sulphate aerosols and other potentially important forcings (e.g., ozone or solar variability) were not considered, the results suggest that the effects of enhanced greenhouse climate may be detected more readily in surface temperatures from low-latitude oceanic regions than from global or zonal temperature averages. Received: 27 June 1995/Accepted: 28 October 1996     

Emissions from Russian domestic civil aviation in 2000–2012 and integrated assessment of their impact on the climate system

Emissions from Russian domestic civil aviation for the period of 2000–2012 are assessed for the following gases: carbon dioxide, methane, nitrous oxide, carbon monoxide, nitrogen oxides, and sulfur dioxide. The integrated assessment of their impact on the climate system is performed using the values of the global warming potential. The CO₂ equivalent was used as a common measure of emissions. It is established that the modern impact of Russian civil aviation on the Earth climate is insignificant.     

Abatement of Greenhouse Gases: Does Location Matter?

Today's climate policy is based on the assumption that the location of emissions reductions has no impact on the overall climate effect. However, this may not be the case since reductions of greenhouse gases generally will lead to changes in emissions of short-lived gases and aerosols. Abatement measures may be primarily targeted at reducing CO₂, but may also simultaneously reduce emissions of NO_x, CO, CH₄ and SO₂ and aerosols. Emissions of these species may cause significant additional radiative forcing. We have used a global 3-D chemical transport model and a radiative transfer model to study the impact on climate in terms of radiative forcing for a realistic change in location of the emissions from large-scale sources. Based on an assumed 10% reduction in CO₂ emissions, reductions in the emissions of other species have been estimated. Climate impact for the SRES A1B scenario is compared to two reduction cases, with the main focus on a case with emission reductions between 2010 and 2030, but also a case with sustained emission reductions. The emission reductions are applied to four different regions (Europe, China, South Asia, and South America). In terms of integrated radiative forcing (over 100 yr), the total effect (including only the direct effect of aerosols) is always smaller than for CO₂ alone. Large variations between the regions are found (53–86% of the CO₂ effect). Inclusion of the indirect effects of sulphate aerosols reduces the net effect of measures towards zero. The global temperature responses, calculated with a simple energy balance model, show an initial additional warming of different magnitude between the regions followed by a more uniform reduction in the warming later. A major part of the regional differences can be attributed to differences related to aerosols, while ozone and changes in methane lifetime make relatively small contributions. Emission reductions in a different sector (e.g. transportation instead of large-scale sources) might change this conclusion since the NO_x to SO₂ ratio in the emissions is significantly higher for transportation than for large-scale sources. The total climate effect of abatement measures thus depends on (i) which gases and aerosols are affected by the measure, (ii) the lifetime of the measure implemented, (iii) time horizon over which the effects are considered, and (iv) the chemical, physical and meteorological conditions in the region. There are important policy implications of the results. Equal effects of a measure cannot be assumed if the measure is implemented in a different region and if several gases are affected. Thus, the design of emission reduction measures should be considered thoroughly before implementation.     

Transient Behaviour of Tropospheric Ozone Precursors in a Global 3-D CTM and Their Indirect Greenhouse Effects

The global three-dimensional Lagrangian chemistry-transport model STOCHEM has been used to follow the changes in the tropospheric distributions of the two major radiatively-active trace gases, methane and tropospheric ozone, following the emission of pulses of the short-lived tropospheric ozone precursor species, methane, carbon monoxide, NO_x and hydrogen. The radiative impacts of NO_x emissionswere dependent on the location chosen for the emission pulse, whether at the surface or in the upper troposphere or whether in the northern or southern hemispheres. Global warming potentials were derived for each of the short-lived tropospheric ozone precursor species by integrating the methane and tropospheric ozone responses over a 100 year time horizon. Indirect radiative forcing due to methane and tropospheric ozone changes appear to be significant for all of the tropospheric ozone precursor species studied. Whereas the radiative forcing from methane changes is likely to be dominated by methane emissions, that from tropospheric ozone changes is controlled by all the tropospheric ozone precursor gases, particularly NO_xemissions. The indirect radiative forcing impacts of tropospheric ozone changes may be large enough such that ozone precursors should be considered in the basket of trace gases through which policy-makers aim to combat global climate change.     

An example of fingerprint detection of greenhouse climate change

As an example of the technique of fingerprint detection of greenhouse climate change, a multivariate signal or fingerprint of the enhanced greenhouse effect is defined using the zonal mean atmospheric temperature change as a function of height and latitude between equilibrium climate model simulations with control and doubled CO₂ concentrations. This signal is compared with observed atmospheric temperature variations over the period 1963 to 1988 from radiosonde-based global analyses. There is a significant increase of this greenhouse signal in the observational data over this period.These results must be treated with caution. Upper air data are available for a short period only, possibly too short to be able to resolve any real greenhouse climate change. The greenhouse fingerprint used in this study may not be unique to the enhanced greenhouse effect and may be due to other forcing mechanisms. However, it is shown that the patterns of atmospheric temperature change associated with uniform global increases of sea surface temperature, with El NinoSouthern Oscillation events and with decreases of stratospheric ozone concentrations individually are different from the greenhouse fingerprint used here.     

欧洲地区不同温室气体背景下土地利用/覆盖变化的气候效应

通过温室气体排放和土地利用/覆盖变化,人类活动对气候变化产生显著影响。为了探究在不同温室气体浓度（Greenhouse gas concentration,GHG）背景下,相同的土地利用/覆盖变化（Land Use and Land Cover Change,LULCC）对于欧洲区域气候的影响差异,采用CESM（Community Earth System Model）耦合模式进行了模拟研究。研究发现,在1850年温室气体浓度背景下,土地利用/覆盖变化导致欧洲中东部地区降水显著增加,而在2000年温室气体浓度背景下,土地利用/覆盖变化导致欧洲中东部地区降水减少。温室气体增加后,LULCC导致该地区对流层低层大气环流由辐合变为辐散,气温以及大气水汽含量降低,这些变化能较大程度的改变LULCC对区域降水的净影响力。     

Greenhouse-gas versus aerosol forcing and African climate response

There are many indicators that human activity may change climate conditions all around the globe through emissions of greenhouse gases. In addition, aerosol particles are emitted from various natural and anthropogenic sources. One important source of aerosols arises from biomass burning, particularly in low latitudes where shifting cultivation and land degradation lead to enhanced aerosol burden. In this study the counteracting effects of greenhouse gases and aerosols on African climate are compared using climate model experiments with fully interactive aerosols from different sources. The consideration of aerosol emissions induces a remarkable decrease in short-wave solar irradiation near the surface, especially in winter and autumn in tropical West Africa and the Congo Basin where biomass burning is mainly prevailing. This directly leads to a modification of the surface energy budget with reduced sensible heat fluxes. As a consequence, temperature decreases, compensating the strong warming signal due to enhanced trace gas concentrations. While precipitation in tropical Africa is less sensitive to the greenhouse warming, it tends to decrease, if the effect of aerosols from biomass burning is taken into account. This is partly due to the local impact of enhanced aerosol burden and partly to modifications of the large-scale monsoon circulation in the lower troposphere, usually lagging behind the season with maximum aerosol emissions. In the model equilibrium experiments, the greenhouse gas impact on temperature stands out from internal variability at various time scales from daily to decadaland the same holds for precipitation under the additional aerosol forcing. Greenhouse gases and aerosols exhibit an opposite effect on daily temperature extremes, resulting in an compensation of the individual responses under the combined forcing. In terms of precipitation, daily extreme events tend to be reduced under aerosol forcing, particularly over the tropical Atlantic and the Congo basin. These results suggest that the simulation of the multiple aerosol effects from anthropogenic sources represents an important factor in tropical climate change, hence, requiring more attention in climate modelling attempts.     

Uncertainties linked to land-surface processes in climate change simulations

 The impact of climate change on the hydrology of continental surfaces is critical for human activities but the response of the surface to this perturbation may also affect the sensitivity of the climate. This complex feedback is simulated in general circulation models (GCMs) used for climate change predictions by their land-surface schemes. The present study attempts to quantify the uncertainty associated with these schemes and what impact it has on our confidence in the simulated climate anomalies. Four GCMs, each coupled to two different land-surface schemes, are used to explore the spectrum of uncertainties. It is shown that, in this sample, surface processes have a significant contribution to our ability to predict surface temperature changes and perturbations of the hydrological cycle in an environment with doubled greenhouse gas concentration. The results reveal that the uncertainty introduced by land-surface processes in the simulated climate is different from its impact on the sensitivity of GCMs to climate change, indeed an alteration of the surface parametrization with little impact on model climate can affect sensitivity significantly. This result leads us to believe that the validation of land-surface schemes should not be limited to the current climate but should also cover their sensitivity to variations in climatic forcing. Received: 24 June 1999 / Accepted: 20 April 2000     

Chemistry–Climate Interactions of Stratospheric and Mesospheric Ozone in EMAC Long-Term Simulations with Different Boundary Conditions for CO2, CH4, N2O,and ODS

Abstract

To evaluate future climate change in the middle atmosphere and the chemistry–climate interaction of stratospheric ozone, we performed a long-term simulation from 1960 to 2050 with boundary conditions from the Intergovernmental Panel on Climate Change A1B greenhouse gas scenario and the World Meteorological Organization Ab halogen scenario using the chemistry–climate model ECHAM5/MESSy Atmospheric Chemistry (EMAC). In addition to this standard simulation we performed five sensitivity simulations from 2000 to 2050 using the rerun files of the simulation mentioned above. For these sensitivity simulations we used the same model setup as in the standard simulation but changed the boundary conditions for carbon dioxide (CO₂), methane (CH₄), nitrous oxide (N₂O), and ozone-depleting substances (ODS). In the first sensitivity simulation we fixed the mixing ratios of CO₂, CH₄, and N₂O in the boundary conditions to the amounts for 2000. In each of the four other sensitivity simulations we fixed the boundary conditions of only one of CO₂, CH₄, N₂O, or ODS to the year 2000.

In our model simulations the future evolution of greenhouse gases leads to significant cooling in the stratosphere and mesosphere. Increasing CO₂ mixing ratios make the largest contributions to this radiative cooling, followed by increasing stratospheric CH₄, which also forms additional H₂O in the upper stratosphere and mesosphere. Increasing N₂O mixing ratios makes the smallest contributions to the cooling. The simulated ozone recovery leads to warming of the middle atmosphere.

In the EMAC model the future development of ozone is influenced by several factors. 1) Cooler temperatures lead to an increase in ozone in the upper stratosphere. The strongest contribution to this ozone production is cooling due to increasing CO₂ mixing ratios, followed by increasing CH₄. 2) Decreasing ODS mixing ratios lead to ozone recovery, but the contribution to the total ozone increase in the upper stratosphere is only slightly higher than the contribution of the cooling by greenhouse gases. In the polar lower stratosphere a decrease in ODS is mainly responsible for ozone recovery. 3) Higher NO_x and HO_x mixing ratios due to increased N₂O and CH₄ lead to intensified ozone destruction, primarily in the middle and upper stratosphere, from additional NO_x; in the mesosphere the intensified ozone destruction is caused by additional HO_x. In comparison to the increase in ozone due to decreasing ODS, ozone destruction caused by increased NO_x is of similar importance in some regions, especially in the middle stratosphere. 4) In the stratosphere the enhancement of the Brewer-Dobson circulation leads to a change in ozone transport. In the polar stratosphere increased downwelling leads to additional ozone in the future, especially at high northern latitudes. The dynamical impact on ozone development is higher at some altitudes in the polar stratosphere than the ozone increase due to cooler temperatures. In the tropical lower stratosphere increased residual vertical upward transport leads to a decrease in ozone.