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1.
The objective of this study was to examine a new resampling methodology for estimating reference levels of 137Cs in uneroded locations. Accurate and precise measurement of 137Cs is required from reference locations to estimate long-term (c. 40 years) sediment redistribution (SRD) and landscape stability. Without reliable long-term, quantitative erosion data it is extremely difficult for land managers to make optimal decisions to ensure landscape sustainability. To determine the influence of 137Cs reference site sampling, particularly under-sampling, on SRD and landscape stability, two statistical approaches were applied to a grid-based data set. Caesium-137 inventories in the reference location (n=36) indicated that data were normally distributed, with a mean inventory of 2150±130 Bq m−2 (±95% confidence band) and a coefficient of variation of 18%. The two approaches used to determine the effect of under sampling included: (1) one-time random subsampling from the total sample collected, subsamples ranged from n=3 to n=30; from these data means and parametric confidence bands were calculated; and (2) random subsamples (n=3 to n=36) were selected from the total 137Cs reference sample, and each subsample was in turn resampled 1000 times with replacement to establish a sampling distribution of means. Thus, an empirically derived mean and 95% confidence bands were established. Caesium-137 activities determined from each approach were input into equations to estimate SRD from two cultivated fields. Results indicate that the one-time random sampling approach for subsamples of size ≤12 significantly over- or under-estimated net SRD, particularly from the gently sloping agricultural field. Computer-intensive resampling produced significantly better estimates of net SRD when compared with the random one-sample approach, especially when a subsample of size three was used. Landscape stability, based on partitioning the agricultural fields into areas exhibiting erosion, stability and deposition, was better approximated for both fields by applying resampling. © 1998 John Wiley & Sons, Ltd.  相似文献   

2.
Floodplains comprise geomorphologically important sources and sinks for sediments and associated pollutants, yet the sedimentology of large dryland floodplains is not well understood. Processes occurring on such floodplains are often difficult to observe, and techniques used to investigate smaller perennial floodplains are often not practical in these environments. This study assesses the utility of 137Cs inventory and depth‐profile techniques for determining relative amounts of floodplain sedimentation in the Fitzroy River, northeastern Australia; a 143 000 km2 semi‐arid river system. Caesium‐137 inventories were calculated for floodplain and reference location bulk soil cores collected from four sites. Depth profiles of 137Cs concentration from each floodplain site and a reference location were recorded. The areal density of 137Cs at reference locations ranged from 13 to 978 Bq m–2 (0–1367 Bq m–2 at the 95% confidence interval), and the mean value ± 2 (standard error of the mean) was 436 ± 264 Bq m–2, similar to published data from other Southern Hemisphere locations. Floodplain inventories ranged from 68 to 1142 Bq m–2 (0–1692 Bq m–2 at the 95% confidence interval), essentially falling within the range of reference inventory values, thus preventing calculation of erosion or deposition. Depth‐profiles of 137Cs concentration indicate erosion at one site and over 66 cm of deposition at another since 1954. Analysis of 239+240Pu concentrations in a depositional core substantiated the interpretation made from 137Cs data, and depict a more tightly constrained peak in concentration. Average annual deposition rates range from 0 to 15 mm. The similarity between floodplain and reference bulk inventories does not necessarily indicate a lack of erosion or deposition, due to low 137Cs fallout in the region and associated high measurement uncertainties, and a likely influence of gully and bank eroded sediments with no or limited adsorbed 137Cs. In this low‐fallout environment, detailed depth‐profile data are necessary for investigating sedimentation using 137Cs. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

3.
Abstract

The use of the bootstrap technique to estimate the reference level of137 Cs in an uneroded site is tested. The analysis is developed using 137Cs measurements made in a small experimental Sicilian basin. In the reference area the 137Cs activity is normally distributed with a known sample mean value, m equal to 94.4 mBq cm?2. The influence of137 Cs reference site sampling was determined generating samples having a fixed size, N and six different values of the sample coefficient of variation, CV, by a Monte Carlo technique. Then, for each size N, the probability distribution of the mean μ of the sequences generated by Monte Carlo technique is defined. The soil redistribution is determined, both at morphological unit and basin scale, using the proportional method of Martz & de Jong for calculating the net soil loss. The analysis showed that the spatial distribution of the net soil loss E i, and the basin value E b are independent of the sample size, N, and the coefficient of variation, CV, of the samples drawn from the reference area, if the bootstrap technique is applied for estimating the mean μ(μ) to use as reference value. The soil redistribution is also examined using as reference value the quantiles μ2.5, μ25, μ75, μ97.5 corresponding to a frequency F(μ) equal to 2.5, 25, 75 and 97.5%, respectively. In conclusion, the analysis established that a robust estimate of the reference value can be obtained even in fields where a small number of samples was drawn (high CV of the 137Cs activity of the field samples), using the bootstrap technique for generating sequences of reference values having known mean value m (the mean value of the 137Cs activity of the drawn field samples) and large sample size (N = 50).  相似文献   

4.
The estimation of erosion and sediment delivery rates in tropical mountain watersheds is difficult and most of the methods widely used for estimating soil erosion over large areas have serious limitations. The 137Cs approach has potential for quantifying soil erosion because it can provide retrospective estimates of long‐term (since 1963) net sediment redistribution relatively quickly. Despite its great potential, 137Cs has not yet been used in an extensive, reconnaissance level survey of erosion in complex tropical mountain environments. The objective of this study was to examine the applicability of the 137Cs method to estimate erosion on steep tropical agricultural lands (23 to 80% slopes) in the Nizao watershed, a humid, tropical mountain area of the Dominican Republic. In this study we (i) examine the variation of 137Cs in ten reference sites—eight coffee groves and two forested sites—and (ii) estimate erosion from 14 cultivated fields. The soil pool of 137Cs ranged from to 150 to 192 mBq cm−2 on reference sites with minimal erosion. Variability among reference sites was less than expected for such complex mountain terrain. The variability within coffee and forested reference (average CV=28%) sites was similar to the variability found on grassland and forested reference sites in the temperate zone. The estimated annual soil loss from 14 sampled fields ranged from 6 to 61 t ha−1 year−1 with an overall mean of 26 t ha−1 year−1. Overall, the soil erosion estimates found using the 137Cs method were much lower than those often assumed for such steep tropical hillsides. These erosion estimates account for soil loss since 1963 only and it seems likely that soil losses may have been much higher in earlier decades immediately after initial forest clearing earlier in the 20th century. Copyright © 2000 John Wiley & Sons, Ltd.  相似文献   

5.
The purpose of this study was to examine the historical change in sedimentation rates in lakes that have been impacted by river regulation and agricultural activities in the Ishikari River floodplain. We dated sediment cores using caesium‐137 (137Cs) dating and tephrochronology, and we estimated sediment sources from 137Cs concentrations in the topsoil of representative land covers. We found that, between 1739 and 1963, the distance between the lake and the main river channel and whether or not the lake was connected to the river affected the sedimentation rates. After 1963, agricultural drainage systems were established in the Ishikari River floodplain. The average sedimentation rate before and after the construction of drainage ditches varied between 1–66 and 87–301 mg cm–2 a–1, respectively. The increase in the sedimentation rate after 1963 was caused by the construction of a number of drainage networks, as well as extensive cultivation activity and/or fragmentation of the swamp buffers surrounding the lakes. The 137Cs activities at the surfaces of the lake as well as the catchment‐derived 137Cs contributions and 137Cs inventory in the lake profiles were used to examine the sediment influx from the various drainage areas after the establishment of the drainage system. Our results indicate that the majority of the lake sediments were derived from cultivated areas, and therefore the catchment‐derived 137Cs contribution in the lakes was strongly correlated with the sedimentation rate. The 137Cs inventory across all of the lake profiles was also significantly greater than the atmospheric fallout. We identified a negative correlation between the 137Cs lake profile inventory and the sedimentation rate. This is because the sediment originating from the drainage areas contained low 137Cs concentrations, which diluted the overall concentration of 137Cs in the lake sediment. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

6.
Cultivated fields have been shown to be the dominant sources of sediment in almost all investigated UK catchments, typically contributing 85 to 95% of sediment inputs. As a result, most catchment management strategies are directed towards mitigating these sediment inputs. However, in many regions of the UK such as the Nene basin there is a paucity of sediment provenance data. This study used the caesium‐137 (137Cs) inventories of lake and floodplain cores as well as the 137Cs activities of present day sediment to determine sediment provenance. Sediment yields were also reconstructed in a small lake catchment. Low 137Cs inventories were present in the lake and floodplain cores in comparison to the reference inventory and inventories in cores from other UK catchments. Caesium‐137 activities in the present day sediments were low; falling close to those found in the channel bank catchment samples. It was estimated that 60 to 100% of the sediment in the Nene originated from channel banks. Pre‐1963 sediment yields were approximately 11.2 t km?2 yr?1 and post‐1963 was approximately 11.9 t km?2 yr?1. The lack of increased sediment yield post‐1963 and low sediment yield is unusual for a UK catchment (where a yield of 28 to 51 t km?2 yr?1 is typical for a lowland agricultural catchment), but is explained by the low predicted contribution of sediment from agricultural topsoils. The high channel bank contribution is likely caused by the river being starved of sediment from topsoils, increasing its capacity to entrain bank material. The good agreement between the results derived using cores and recently transported sediments, highlight the reliability of 137Cs when tracing sediment sources. However, care should be taken to assess the potential impacts of sediment particle size, sediment focusing in lakes and the possible remobilization of 137Cs from sedimentary deposits. Copyright © 2016 John Wiley & Sons, Ltd.  相似文献   

7.
Vertical profiles of the activities of 137Cs and 210Pb were measured on floodplain sediment cores and upland soil cores along the Soda Butte Creek and the Yellowstone River to determine floodplain sedimentation rates. The position of mine tailings from a 1950 impoundment failure was used as a stratigraphic marker to estimate the sedimentation rates and to make comparisons with rates provided by radionuclide‐based methods. Mass accumulation (sedimentation) rates calculated from the position of the mine tailings ranged from 0·00 to 0·17 g cm?2 yr?1 and were in good agreement with sedimentation rates calculated from the inventories of 137Cs and 210Pb. Sedimentation rates calculated from the position of the 137Cs peak generally overestimated the sedimentation rates, probably because of increased downward migration of 137Cs caused by the low pH of water moving through the mine tailings or the high permeability of floodplain sediments relative to upland reference soils. This study demonstrates that the 137Cs and 210Pb inventory methods for determining sedimentation rates can be applied to an alpine floodplain where sedimentation events are episodic and where orographic effects on precipitation generate strong downstream gradients in the delivery of atmospheric radionuclides. Copyright © 2007 John Wiley & Sons, Ltd.  相似文献   

8.
There is very thin soil layer in karst rocky desertification areas in Southwest China,sediment deposition and sediment yield in the karst area affects the development of vegetation greatly.In the present study,the 137Cs technique was used to assess the rate of sediment deposition and sediment yield in a small karst catchment.The 137Cs inventory within the depression varied between 800 m-2 and 2,200 Bq m-2,with the mean value of 1,500.1 Bq m-2.The 137Cs reference inventory at a nearby reference site was 805.9 Bq m-2.It could be inferred to that sediment deposition had occurred in the catchment.The mean depth of sediments deposition in the depression was 6 cm and the deposition rate was approximately 0.13 cm yr-1.The analysis of the topographic characteristics of the catchment revealed that the sediment deposition occurred mainly at the lower part of the small catchment.Although,there was a sinkhole in the depression,little sediment had drained out with runoff through the sinkhole,because the local people built ridges around the sinkholes for storing water.According to this,sediment yield rate in the small catchment was estimated to be approximately 19.25 to 27.5 t km-2 yr-1,and the extremely low sediment yield was maybe the main obstacle to vegetation restoration in karst rocky desertification areas.  相似文献   

9.
A rapid removal of Chernobyl137Cs from a number of large lakes has been previously reported. Our measurements of137Cs in water, sediments and pore water in the mono- and meromictic basins of Lake Lugano (Lago di Lugano) reveal generally slower half-removal times of 1.2 and 6.7 yrs, respectively. In the seasonally anoxic southern basin, this is most probably related to an intensive recycling of137Cs between water and sediments. In the permanently stratified northern basin the removal rate is much slower due to an important inventory build up in the deep anoxic part of the basin.  相似文献   

10.
The 137Cs radioactivity of soils was used as a tracer of soil erosion in a catchment in the Netherlands: 143 samples were analysed to map the 137Cs redistribution using geostatistical interpolation methods. Caesium-137 activities on grassland are significantly higher than on arable land. Also, 137Cs activities on waning slopes are higher and activities on steep slopes are lower. The soil erosion estimates, derived from the 137Cs data, are used to validate the USLE erosion model. The recent Chernobyl nuclear accident also contributed to the 137Cs activity. However, the Chernobyl input of 137Cs, with a constant ratio of 1.765:1 to 134Cs, cannot be used as a tracer of soil erosion. Because of the rapid decay of 134Cs, we will not be possible to separate the sources of 137Cs in the near future in areas significantly influenced by Chernobyl fallout and in these areas 137Cs can no longer be used as a soil erosion tracer.  相似文献   

11.
Time series of 137Cs and 99Tc activity concentrations in the brown seaweed Fucus vesiculosus and seawater, gathered at three locations on the eastern Irish coastline during the period 1988-2008, have been modelled using a novel approach incorporating a variable uptake rate in the seaweed. Seasonal variations in the time series, identified using spectral analysis, were incorporated into the model which was used to determine transfer kinetic parameters and to predict 137Cs and 99Tc concentrations in seaweed, as influenced by levels in ambient seawater. An optimisation method combining evolutionary and grid search minimisation techniques was adopted to determine the best values for the model parameters, from which concentration factors (CF) and biological half-lives (tb1/2) for 137Cs and 99Tc in F. vesiculosus were calculated. CF values of 170-179 and 1.1 × 105 l kg−1 (dry weight) were obtained for 137Cs and 99Tc, respectively, while the corresponding tb1/2 values were 39-47 and 32 days, respectively.  相似文献   

12.
238Pu,239Pu and137Cs in rain and dry fallout and90Sr in rain samples were measured at Woods Hole, Massachusetts, from June 1976 through December 1977. The dry fallout was estimated to be about 7.8% of the total deposition of239Pu and137Cs.239Pu/137Cs ratios, almost constant at about 0.011 in rain or dry fallout, February through December 1977, suggested that fractionation between the refractory and volatile radionuclides is insignificant in stratospheric fallout. This supports the idea of regional homogeneity of radionuclide ratios in fallout.  相似文献   

13.
The rate of natural removal of 137Cs from water bodies in Eastern Fennoscandia is evaluated. The half-time T of water purification from global 137Cs in lake–river systems was ~6.5 years and that for river systems was 6.5–10 years. For the 15- and 20-year exposure of 137Cs in watershed soils, its annual input in rivers was 0.021–0.120 and 0.017–0.070% of its reserve. The period of May–December 1986 showed maximal export of 137Cs, i.e., 1.1% of its reserve. 137Cs export into rivers decreased in the region from north to south because of changes in landscape and climate conditions that affect 137Cs migration on watersheds.  相似文献   

14.
At two locations in southern Lake Huron (U.S.A.), twelve 35.5-cm diameter cores of fine-grained sediments were taken for comparison of the vertical distributions of210Pb and falllout137Cs with the distributions of benthic macroinvertebrates, mainly oligochaete worms (Tubificidae) and the amphipod,Pontoporeia affinis. Locations were selected on the basis of210Pb distributions measured a year earlier which indicated contrasting depths of mixing of surface sediments. At one location the activity of210Pb is uniform down to about 6 cm and 95% of total invertebrates occur within this zone; at the other location the zone of constant activity is only 3 cm deep but 90% of the invertebrates occur within it. Comparison of published tubificid defecation rates with sediment accumulation rates based on210Pb shows that oligochaetes alone can account for mixing in one case while the effects of amphipods may be required in the case of shallower mixing. If mixing is represented as a diffusional process, eddy diffusion coefficients are at least 5.8 and 3.3 cm2 yr?1 at respective locations. In comparison with bioturbation, molecular diffusion is of minor importance in the post-depositional mobility of137Cs. The necessity for introducing a diffusion coefficient varying continuously with depth is indicated by characteristics of the distribution of137Cs. Biological reworking of near-surface sediments is an important process affecting radioactivity and chemical profiles in profundal deposits of this and probably other Great Lakes.  相似文献   

15.
The spatial distribution of 137Cs across the landscape and the processes controlling its redistribution are of interest because (i) 137Cs has been widely used to quantify the movement of soil and sediments and (ii) substantial fallout of 137Cs after the Chernobyl accident has led to contamination of foodstuffs in some places. A high‐resolution airborne geophysical radiometric survey of Northern Ireland has provided an opportunity to study the distribution and possible redistribution of 137Cs. The 137Cs activity (recorded at 1·2 million points) is distributed in a series of bands oriented approximately 160° and 115° clockwise from north. Geostatistical analysis of the data shows a strong, short‐range structure (correlation ranges between 0·6 and 8 km) in 137Cs activity across the vast majority of the region; the spatial distribution shows association with a published, coarse‐scale depositional pattern of 137Cs from Chernobyl. Two indices of land form derived from a digital elevation model, namely compound topographic index and the length–slope factor of the Revised Universal Soil Loss Equation, account for only 3% of the variance in 137Cs activity. In contrast, soil type and land cover in combination (including their interaction) account for 20% of the variance. In areas that received moderate fallout from Chernobyl, soil type alone accounts for a substantial proportion of the spatially correlated 137Cs activity. We attribute this to each soil type having a fairly uniform radiocaesium interception potential that differs from those of other soil types and that this potential controls the vertical migration of 137Cs. Over the granitic Mourne Mountains there is a strong spatial cross‐correlation between 137Cs activity and airborne estimates of soil potassium, suggesting that the latter provides a measure of the soil's radiocaesium interception potential; this is probably dominated by the quantity of the mineral illite. Copyright © 2010 John Wiley & Sons, Ltd. and British Geological Survey  相似文献   

16.
An estimated 3.5 ± 0.7 × 1015 Bq of 137Cs is thought to have been discharged into the ocean following the melt down at Fukushima Dai-ichi Nuclear Power Plant (F1NPP). While efforts have been made to monitor seafloor radiation levels, the sampling techniques used cannot capture the continuous distribution of radionuclides. In this work, we apply in situ measurement techniques using a towed gamma ray spectrometer to map the continuous distribution of 137Cs on the seafloor within 20 km of the F1NPP. The results reveal the existence of local 137Cs anomalies, with levels of 137Cs an order of magnitude higher than the surrounding seafloors. The sizes of the anomalies mapped in this work range from a few meters to a few hundreds of meters in length, and it is demonstrated that the distribution of these anomalies is strongly influenced by meter scale features of the terrain.  相似文献   

17.
On two short sediment cores from Lake Łazduny (northeastern Poland) different methods for age estimation were applied including varve counting, 210Pb, 137Cs and OSL dating. The investigated sediment consists of finely laminated, organic-rich calcareous gyttja interrupted by a sand layer. For 210Pb we tested the CFCS, CIC, CRS and SIT models and compared the results with the established varve chronology and the 137Cs distribution. The total 210Pb activity distribution is consistent between cores and shows a regular decrease with depth. However, the total inventory of unsupported 210Pb was significantly different and indicates varying rates of sediment focusing. Our results show that all 210Pb dating models used in this study produced different results, while the SIT model performed best in comparison with varve counts and 137Cs peaks. The CFCS model produced a realistic age-depth trend but obtained ages were too old compared to the varve time scale. The age estimates provided by the CRS model were too old as well with an increasing offset downcore and the CIC model failed completely by producing an unrealistic chronology with age inversions. This confirms that only systematic testing of different 210Pb dating models and routine validation using independent time markers produces reliable 210Pb chronologies. OSL dating of two samples from the sand layer provided much too old results which indicate incomplete bleaching during deposition of the analyzed quartz grains. This multiple dating approach demonstrates the considerable potential but also potential pitfalls of dating such young sediments.  相似文献   

18.
From GEOSECS stations, largely, the 1974 distributions of Pu and of137Cs are described in the Pacific Ocean north of about 20°S latitude. Changes in some of these distributions are described from 1978 cruises by the authors.The Pacific exhibited, everywhere, a shallow subsurface layer of Pu-rich water with its concentration maximum at about 465 m in 1974; over a large portion of the central North Pacific a second layer of Pu-labelled water, less concentrated than the shallow layer, lay just above the bottom. Similar features were not observed in the case of137Cs.The inventories of both Pu and137Cs in the water column at most 1974 stations are substantially greater than those to be expected from world-wide fallout alone; these inventory excesses appear to be attributable to close-in fallout, but only if the ratio Pu/137Cs in this source was much higher than in world-wide fallout. The North Pacific mean ratio of the inventories is 2.2 times that observed in world-wide fallout.Resolubilization of Pu both from sinking particles and from sediments explains peculiarities of its depth distributions.There is little evidence for tracer movement by sliding downward along density surfaces;137Cs appears to have moved to depth by downmixing at the edge of the Kuroshio, and then moved horizontally and upward alongσt contours. The shallow Pu-rich layer shows no coordination with density, salinity or O2 isopleths. The deep Pu-rich layer is restricted to a narrow range of O2 concentrations that confirm its origin in the Aleutian Trench and rapid spread southward and laterally. Near-bottom circulation processes have been much more active than here-to-fore described.  相似文献   

19.
To analyse suspended sediment sources in unmanaged Japanese cypress plantation watersheds, field measurements and fingerprinting of the suspended sediment was conducted in the Shimanto River basin in southern Japan. For sediment fingerprinting, 137Cs and 210Pbex were detected by means of gamma‐ray spectrometry in the surface soil of the forest floor, stream bank and truck trail and mobilized sediment by interrill erosion. The 137Cs and 210Pbex activities associated with the forest floor materials were considerably higher than those of the stream bank and truck trail. The 137Cs and 210Pbex activities associated with the suspended sediment were found to vary with the sampling period. Evidently, the suspended sediment can comprise materials generated from the forest floor by interrill erosion and those from the truck trail and/or stream bank. The multivariate sediment‐mixing model using 137Cs and 210Pbex showed that the contribution of the forest floor varied periodically, ranging from 23–56% in the Hinoki 156 subwatershed and from 18–85% in the Hinoki 155 subwatershed. The difference in the average contribution of the forest floor between Hinoki 156 (46%) and Hinoki 155 (69%) may relate to the presence of truck trail networks in the watershed. The truck trail network can play roles of sediment source and pathway for sediment from forest floor to stream channel due to the concentrated overland flow on the truck trail during heavy rainfall events. These results indicate that the forest floor should be recognized as a major source of suspended sediment in unmanaged Japanese cypress plantation watersheds. Copyright © 2008 John Wiley & Sons, Ltd.  相似文献   

20.
Erosion rates and processes define how mountainous landscapes evolve. This study determines the range of erosion rates in a semi‐arid landscape over decadal time spans and defines the dominant processes controlling variability in erosion rates. The varying topography and climatic regimes of the Xiying Basin (Qilian Shan Mountains, China) enables us to examine the relative roles of sheet wash versus rainsplash and the influence of vegetation on soil erosion and deposition. Soil erosion rates since 1954 were determined using 137Cs along 21 transects at four sites with varying gradient, rainfall, and vegetation cover. The mean 137Cs derived soil erosion rate ~0.42 mm/a was consistent with the catchment level erosion rate derived from total sediment yield for a 44 year record. However, there is considerable variability in 137Cs erosion rates both between transects and along transects, perhaps reflecting variation not only in the effectiveness of individual processes but also in their relative roles. We compare the 137Cs‐derived erosion rates with 1‐D models for sediment flux that incorporate sheet wash and rainsplash processes, testing them over a previously untested 60 year timescale. The variability in 137Cs erosion rates along transects is best replicated by sheet wash dominated simulations, suggesting that this is the dominant erosion process in this semi‐arid landscape. The functional form of the sheetwash model can also explain our observations that 137Cs erosion rates decrease with upslope length (i.e. distance down slope) while its variability increases. However, sparsely vegetated sites, located in slightly drier locations, have higher erosion rates, and are not as accurately modeled as densely vegetated sites, suggesting that patchiness of vegetation introduces fine scale variability in erosion rates on these slopes. Copyright © 2015 John Wiley & Sons, Ltd.  相似文献   

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