Radiative and Thermal Impacts of Smoke Aerosol Longwave Absorption during Fires in the Moscow Region in Summer 2010

The aerosol longwave radiative forcing of the atmosphere and heating rate of the near-surface aerosol layer are estimated for the extreme smoke conditions in the Moscow region in summer 2010. Thermal radiation fluxes in the atmosphere are determined using the integral transmission function and semiempirical aerosol model developed on the basis of standard aerosol models and measurements at the Zvenigorod Scientific Station, Obukhov Institute of Atmospheric Physics, Russian Academy of Sciences. The aerosol radiative forcing reached 33 W/m² at the lower atmospheric boundary and ranged between–1.0 and 1.0 W/m² at the upper atmospheric boundary. The heating rate of the 10-m atmospheric layer near surface was up to 0.2 K/h during the maximum smoke conditions on August 7–9. The sensitivity of the aerosol longwave radiative forcing to the changes in the aerosol absorption coefficient and aerosol optical thickness are estimated.     

The radiative and thermal effects of smoke aerosol over the region of Moscow during the summer fires of 2010

The shortwave radiative forcings of smoke aerosol in the cloudless atmosphere during the summer fires of 2010 in European Russia were quantitatively estimated for the land surface and the atmospheric upper boundary from measurement data obtained at the Zvenigorod Scientific Station of the Obukhov Institute of Atmospheric Physics (OIAP ZSS), Russian Academy of Sciences. Variations in the temperature of the surface air layer due to the smoke-induced attenuation of incoming solar radiation were estimated. The most intensive smoke generation in the atmosphere was observed on August 7–9, 2010, when the maximum aerosol optical thickness amounted to more than 4.0 at a wavelength of 550 nm. In this case, the albedo of single aerosol scattering amounted to ∼0.95–0.96 and the asymmetry factor amounted to ∼0.69–0.70. The maximum shortwave radiative forcing of aerosol amounted to about −360 W/m² for the land surface and almost −150 W/m² for the atmospheric upper boundary. During the period of intensive smoke generation, the cooling of the atmospheric surface layer over daylight hours (12 h) amounted, on average, to ∼6°C. The power character of the dependence of the shortwave radiative forcing of aerosol for the land surface on aerosol optical thickness up to its values exceeding 4.0, which was revealed earlier on the basis of data on aerosol optical thickness (up to 1.5) obtained at the OIAP ZSS during the summer forest and peatbog fires of 2002 in the region of Moscow, was supported.     

Brown Carbon and Black Carbon in the Smoky Atmosphere during Boreal Forest Fires

We have investigated the variability of smoke aerosol absorbing ability with variations in the content of brown carbon (BrC) and black carbon (BC). Using monitoring data on radiative characteristics of smoke aerosol at AERONET stations and the spatial distribution of aerosol optical depth (AOD) obtained by the MODIS spectrometer (Terra satellite), we have detected large-scale smokes during boreal forest fires in Russia and Canada (1995–2012). The spatial distribution (50°–70° N, 95°–125° W) and temporal variability (at AERONET station Fort McMurray) of AOD during the smoking of a part of Canada in July 2012 have been analyzed. AOD probability distributions for July 14–18, 2012, and an estimate of aerosol radiative forcing of smoke aerosol at the upper boundary of the atmosphere have been obtained. We have proposed a technique for the diagnostics of BrC and BC in smoke aerosol particles from the spectral dependence of the imaginary part of the refractive index. At a wavelength of 440 nm, the contributions of BrC and BC to the smokeaerosol absorbing abitity can be comparable in magnitude. In many cases, the absorption spectra of smoke aerosol can be adequately approximated by either power or exponential functions. The presence of BrC in smoke-aerosol particles highly extends the variety of observed absorption spectra in a smoky atmosphere and spectral dependences of single scattering albedo. In the spectral range of 440–1020 nm, the radiative characteristics of smoke aerosol are largely contributed by its fine mode.     

Evaluation of the accuracy of downward radiative flux observations at the sea surface

Observations of downward radiative flux at the sea surface generally contain uncertainty due to limited numbers of observations and limitations of auxiliary equipment. The lack of shading from direct solar radiation and ventilation systems causes bias or random errors. To evaluate the error of radiation measurements at buoys, downward shortwave and longwave radiative fluxes are compared with International Satellite Cloud Climatology Project (ISCCP), Japanese 55-year Reanalysis (JRA55), and Moderate Resolution Imaging Spectroradiometer (MODIS) retrieved model calculations of 3-h and daytime averages. Cloud masking is evaluated by a combination of MTSAT-1R and in situ observations. Coincident observations from a land-surface station located near the buoy observatories are compared with satellite and reanalysis products. The bias at buoys, compared with retrievals, approximately over- and under-estimate for longwave and shortwave fluxes, respectively. The bias at buoys is larger and smaller than the land by 23–34 W m^?2 for longwave and 13–51 W m^?2 for shortwave radiation using 3-h averages under clear-sky conditions. The differences in bias decrease when using daytime averages for longwave, but the difference for shortwave increases with daytime averages. To evaluate the effect of environmental factors on buoy observations, we compared rainfall, wind speed, and solar zenith angle with the biases. We found that rainfall and wind speed affect buoy pyrgeometers such that they overestimate the longwave flux. The cosine of solar zenith angle does not cause overestimation for longwave flux, and the effect of dome heating is small. The strong wind causes underestimation of the shortwave radiative flux due to tilting. The effect of wind is reduced when daily averages are used.     

Influence of direct sulfate-aerosol radiative forcing on the results of numerical experiments with a climate model of intermediate complexity

The climate model of intermediate complexity developed at the Institute of Atmospheric Physics of the Russian Academy of Sciences (IAP RAS CM) is extended by a block for the direct anthropogenic sulfate-aerosol (SA) radiative forcing. Numerical experiments have been performed with prescribed scenarios of the greenhouse and anthropogenic sulfate radiative forcings from observational estimates for the 19th and 20th centuries and from SRES scenarios A1B, A2, and B1 for the 21st century. The globally averaged direct anthropogenic SA radiative forcing F _ASA by the end of the 20th century relative to the preindustrial state is ?0.34 W/m², lying within the uncertainty range of the corresponding present-day estimates. The absolute value of F _ASA is the largest in Europe, North America, and southeastern Asia. A general increase in direct radiative forcing in the numerical experiments that have been performed continues until the mid-21st century. With both the greenhouse and the sulfate loadings included, the global climate warming in the model is 1.5–2.8 K by the end of the 21st century relative to the late 20th century, depending on the scenario, and 2.1–3.4 K relative to the preindustrial period. The sulfate aerosol reduces global warming by 0.1–0.4 K in different periods depending on the scenario. The largest slowdown (>1.5 K) occurs over land at middle and high latitudes in the Northern Hemisphere in the mid-21st century for scenario A2. The IAP RAS CM response to the greenhouse and the aerosol forcing is not additive.     

Field studies of the correlation between the atmospheric aerosol content and the light polarization at the zenith of the daytime sky

Results of simultaneous measurements of the direct solar radiation flux and of the degree of polarization of visible light scattered at the zenith at a different albedo of the underlying surface covered with snow after heavy snowfalls or having no snow cover are analyzed. The possibility of monitoring air turbidity on the basis of polarimetric measurements is confirmed. A procedure of remote detection of the effect of solar light polarization on atmospheric aerosol is proposed and implemented.     

全球变暖不同阶段热带辐合带的移动及其与大气能量输送的关系

基于第五次国际间耦合模式比较计划(The phase 5 of the Coupled Model Intercomparison Project,CMIP5)中在4.5 W/m^2的典型浓度路径(Representative Concentration Pathway,RCP4.5)试验结果,本文通过能量框架分析方法研究了全球变暖不同阶段热带辐合带(Intertropical Convergence Zone,ITCZ)的南北移动及其主要机制,发现在温室气体持续增加的海洋快响应和温室气体达到稳定后的海洋慢响应两个阶段,ITCZ的移动都和跨赤道的大气能量输送(Atmosphere Heat Transport,AHT)变化显著相关,但两者变化的原因在两个阶段中是不同的。在快响应阶段,ITCZ位置的移动以及跨赤道AHT受大气层顶(Top of the Atmosphere,TOA)的能量变化驱动,主要与南大洋云短波辐射响应、北半球中高纬度云和地表的短波辐射响应有关,气溶胶减少引起的辐射响应变化使得ITCZ在大多数模式中表现出向北移动的特征。在慢响应下辐射强迫保持稳定,ITCZ在大多数模式中表现出向南移动的特征。这一时期ITCZ的移动由大气表面能量通量变化驱动,主要与潜热通量变化的南北半球差异有关。全球变暖不同阶段ITCZ移动与大气能量输送变化的关系差异反映了海洋对于气候变化的重要调控作用。     

First retrieval of data regarding spatial distribution of Asian dust aerosol from the Geostationary Ocean Color Imager

Aerosol optical thickness (AOT) was retrieved from the Geostationary Ocean Color Imager (GOCI) on board the Communication, Ocean, and Meteorological Satellite (COMS) for the first time. AOT values were retrieved over the ocean at a spatial scale of 0.5 × 0.5 km² by using the look-up table (LUT)-based separation technique. The radiative transfer model (RTM) was used for different models of atmosphere-ocean environmental conditions, taking into account the realistic variability of scattering and absorption. Ocean surface properties affected by whitecaps and pigment content were also taken into account. The results show that the radiance observed by the GOCI amounts to only 5% of the radiation that penetrated the ocean and, consequently, 95% of the radiation is scattered in the atmosphere or reflected at the ocean surface in the visible wavelengths longer than 0.6 ìm. Within these wavelengths, radiance variations at the top of atmosphere (TOA) due to pigment variations are within 10%, while the radiance variation due to wind speed is considerably higher. For verification of GOCI-retrieved AOTs, comparison between GOCI and ground-based sunphotometer measurement at Gosan, Korea (126.10°E, 33.23°N)) showed good correlation (r = 0.99). The GOCI observations obtained by using the proposed technique showed promising results for the daily monitoring of atmospheric aerosol loading as well as being useful for environmental supervisory authorities.     

Optical properties and surface energy flux of spring fast ice in the Arctic

Over the past decades, sea ice in the polar regions has been significantly affecting local and even hemispheric climate through a positive ice albedo feedback mechanism. The role of fast ice, as opposed to drift ice, has not been well-studied due to its relatively small coverage over the earth. In this paper, the optical properties and surface energy balance of land fast ice in spring are studied using in situ observations in Barrow, Alaska. The results show that the albedo of the fast ice varied between 0.57 and 0.85 while the transmittance increased from 1.3×10?3 to 4.1×10?3 during the observation period. Snowfall and air temperature affected the albedo and absorbance of sea ice, but the transmittance had no obvious relationship with precipitation or snow cover. Net solar shortwave radiation contributes to the surface energy balance with a positive 99.2% of the incident flux, with sensible heat flux for the remaining 0.8%. Meanwhile, the ice surface loses energy through the net longwave radiation by 18.7% of the total emission, while the latent heat flux accounts for only 0.1%. Heat conduction is also an important factor in the overall energy budget of sea ice, contributing 81.2% of the energy loss. Results of the radiative transfer model reveal that the spectral transmittance of the fast ice is determined by the thickness of snow and sea ice as well as the amount of inclusions. As major inclusions, the ice biota and particulates have a significant influence on the magnitude and distribution of the spectral transmittance. Based on the radiative transfer model, concentrations of chlorophyll and particulate in the fast ice are estimated at 5.51 mg/m2 and 95.79 g/m2, which are typical values in the spring in Barrow.     

基于遥感的海表紫外辐射强度反演方法

Ultraviolet(UV) radiation has a significant influence on marine biological processes and primary productivity;however, the existing ocean color satellite sensors seldom contain UV bands. A look-up table of wavelengthintegrated UV irradiance(280–400 nm) on the sea surface is established using the coupled ocean atmosphere radiative transfer(COART) model. On the basis of the look-up table, the distributions of the UV irradiance at middle and low latitudes are inversed by using the satellite-derived atmospheric products from the Aqua satellite,including aerosol optical thickness at 550 nm, ozone content, liquid water path, and the total precipitable water.The validation results show that the mean relative difference of the 10 d rolling averaged UV irradiance between the satellite retrieval and field observations is 8.20% at the time of satellite passing and 13.95% for the daily dose of UV. The monthly-averaged UV irradiance and daily dose of UV retrieved by satellite data show a good correlation with the in situ data, with mean relative differences of 6.87% and 8.43%, respectively. The sensitivity analysis of satellite inputs is conducted. The liquid water path representing the condition of cloud has the highest effect on the retrieval of the UV irradiance, while ozone and aerosol have relatively lesser effect. The influence of the total precipitable water is not significant. On the basis of the satellite-derived UV irradiance on the sea surface, a preliminary simple estimation of ultraviolet radiation's effects on the global marine primary productivity is presented, and the results reveal that ultraviolet radiation has a non-negligible effect on the estimation of the marine primary productivity.     

Direct observation of radiative flux in the southern yellow sea

Direct measurements of four radiative components at air-sea boundary layer were conducted in the southern Yellow Sea during three cruises (seasons) in 2007. Simultaneous observations of meteorological (cloud cover, air temperature and humidity) and oceanographic (sea surface temperature) parameters were carried out. Observational results of radiative fluxes and meteorological and oceanographic parameters are presented. Mean diurnal cycles of four radiative components, net radiation, and sea surface albedo are calculated to achieve averages in different seasons. Net radiative fluxes in three seasons (winter, spring, autumn) are 8, 146, 60 W/m², respectively. Comparisons between the observed radiative fluxes and those estimated with formulas are taken.     

The effect that coarse particles have on estimates of both optical and radiation characteristics of dust aerosol

Based on mathematical simulation, quantitative estimates of the effect that coarse dust particles have on the accuracy of retrieving the optical characteristics of aerosol have been obtained from the results of ground-based measurements of the spectral fluxes of both direct and scattered solar radiations. The results of verifying a retrieval algorithm (used at the AERONET ground-based network) based on special test models showed that the aerosol characteristics retrieved with this algorithm are unsuitable for calculating integral solar fluxes and for simulating space spectrometric IR measurements when the concentration of dust particles in the atmosphere exceeds their concentration in the well-known CONT model of continental aerosol by a factor of two or more.     

The influence of the microphysical parameters of atmospheric aerosol particles on IR radiation extinction

The influence of the aerosol component on the total transmission of sounding IR radiation is analyzed. The emissions of both industrial and natural origins into the atmosphere were regarded as the medium. It is noted that, in studying the radiative transport through gas-aerosol mixtures, it is necessary to take into account both molecular absorption and scattering from aerosol particles. It is shown that there are certain boundary values of the microphysical parameters of aerosol where it is sufficient to take into account only one of the above-mentioned factors of radiation extinction. The quantitative values of the parameters of an aerosol medium, on the basis of which the solution of the transport equation can be significantly simplified, are given.     

热带东印度洋SST对气候变暖和变冷的响应

The response of the eastern tropical Indian Ocean(ETIO) to heat fluxes of equal amplitude but opposite sign is investigated using the Community Earth System Model(CESM). A significant positive asymmetry in sea surface temperature(SST) is found over the ETIO—the warming responses to the positive forcing exceeds the cooling to the negative forcing. A mixed layer heat budget analysis is carried out to identify the mechanisms responsible for the SST asymmetry. Results show that it is mainly ascribed to the ocean dynamical processes, including vertical advections and diffusion. The net surface heat flux, on the contrary, works to reduce the asymmetry through its shortwave radiation and latent heat flux components. The former is due to the nonlinear relationship between SST and cloud, while the latter is resulted mainly from Newtonian damping and air-sea stability effects. Changes in the SST skewness are also evaluated, with more enhanced negative SST skewness over the ETIO found for the cooling than heating scenarios due to the asymmetric thermocline-SST feedback.     

Downward longwave radiation in general circulation models: a case study at a semi‐arid continental site

The present case study evaluates the downward longwave radiation at the surface (DLR) in several high‐resolution (≈1°) general circulation models (GCMs) using surface observations from a semiarid continental site in New South Wales, Australia (Uardry, 34.39°S, 142.30°E). This site is located on a large grassland plain uniform in both its land use and landcover type, and is therefore particularly well suited for a comparison with GCM grid mean values. Monthly averages of newly constructed clear‐sky and all‐sky DLR climatologies and the resulting cloud‐radiative forcing are compared. It is shown that the GCMs exceed the observed DLR under cloud‐free conditions by 10–20 W m⁻² at this semiarid site on an annual basis, with a strong seasonal dependence. The calculated clear‐sky fluxes are overestimated during the warmer summer season, with large absolute values of DLR, while the biases are reduced in the colder and dryer winter season with smaller fluxes. This gives direct support for recent evidence that the DLR model biases depend systematically on the thermal and humidity structure of the cloudless atmosphere. Fluxes from strongly emitting atmospheres tend to be overestimated, but may be underestimated from atmospheres with smaller emission. This points to common problems inherent in the simulation of the emission from the cloudless atmosphere in current longwave radiation codes.
The comparisons of the all‐sky climatologies at Uardry show that the clear‐sky biases are partly masked in the models with an insufficient cloud‐radiative forcing, thereby counterbalancing the excessive DLR of the cloud‐free atmosphere. On the other hand, when the cloudradiative forcing is improved, the biases in the cloud‐free atmosphere become fully apparent in the all‐sky fluxes.     

我国海区SeaWiFS资料大气校正

利用光谱辐射传输理论，结合海上同步实测资料，开发出我国海区SeaWiFS资料大气校正模型。经卫星资料处理结果比对，本模型在一类水体，基本消除了412nm和443nm波段离水辐射率小于0的现象；在二类水体，利用临近一类水体的大气条件进行了有效的大气校正；同时建立了670nm,765nm,865nm波段的大气校正模型，这三个面适用于高浓度悬浮泥沙的信息提取。本模型用于处理我国海区的SeaWiFS资料比美国NASA模型更适合我国海区特定的大气和海洋环境，为SeaWiFS资料海洋水色信息提取和我国海洋一号（HY－1）及风云一号（FY－1C）卫星资料的大气校正研究提供了技术基础。     

A change in the asymmetry coefficient of Light-Scattering phase function in natural waters that contain organic particles

A semiempirical model is constructed for the relationship between the coefficient of asymmetry of Light Scattering phase function in water K and the scattering coefficient σ, which shows a mechanism of an increase in the asymmetry coefficient as the scattering coefficient grows as a result of an increase in the concentration of organic particles. The mechanism of this relationship lies in the presence in all natural waters of molecular scattering and scattering by mineral particles that create background scattering in water medium, which is overlaid by scattering by organic particles. This relationship has a regional character caused by the regional features of background scattering and the average size of organic particles in those regions. The model relationships K = f(σ) are plotted properly to the experimental ones in the various regions.     

Effect of including land-use driven radiative forcing of the surface albedo of land on climate response in the 16th–21st centuries

A change in ecosystem types, such as through natural-vegetation-agriculture conversion, alters the surface albedo and triggers attendant shortwave radiative forcing (RF). This paper describes numerical experiments performed using the climate model (CM) of the Institute of Atmospheric Physics (IAP), Russian Academy of Sciences, for the 16th–21st centuries; this model simulated the response to a change in the contents of greenhouse gases (tropospheric and stratospheric), sulfate aerosols, solar constant, as well as the response to change in surface albedo of land due to natural-vegetation-agriculture conversion. These forcing estimates relied on actual data until the late 20th century. In the 21st century, the agricultural area was specified according to scenarios of the Land Use Harmonization project and other anthropogenic impacts were specified using SRES scenarios. The change in the surface vegetation during conversion from natural vegetation to agriculture triggers a cooling RF in most regions except for those of natural semiarid vegetation. The global and annual average RF derived from the IAP RAS CM in late 20th century is ?0.11 W m^?2. Including the land-use driven RF in IAP RAS CM appreciably reconciled the model calculations to observations in this historical period. For instance, in addition to the net climate warming, IAP RAS CM predicted an annually average cooling and reduction in precipitation in the subtropics of Eurasia and North America and in Amazonia and central Africa, as well as a local maximum in annually average and summertime warming in East China. The land-use driven RF alters the sign in the dependence that the amplitude of the annual cycle of the near-surface atmospheric temperature has on the annually averaged temperature. One reason for the decrease in precipitation as a result of a change in albedo due to land use may be the suppression of the convective activity in the atmosphere in the warm period (throughout the year in the tropics) and the corresponding decrease in convective precipitation. In the 21st century, the effect that the land-use driven RF has on the climate response for scenarios of anthropogenic impact is generally small.     

A global heat and freshwater forcing dataset for ocean models

A global dataset based on the ECMWF Re-Analyses (ERA) is presented that can be used as surface boundary conditions for ocean models with sea-ice components. The definition of these conditions is based on bulk formulae. To study the mean ocean circulation, a mean annual cycle on a daily basis was constructed from ERA for all relevant parameters including wind stress. Continental runoff is considered by using information about the catchment areas of the rivers and about the main drainage basins. The bulk formulae were extended by using sea ice concentration.To estimate meridional heat transports (MHT) and to avoid any drift in ocean model simulations, the heat and fresh water budgets have been closed by applying an inverse procedure to fine-tune the fluxes towards observed transports. To improve the MHTs on the Southern Hemisphere the winds and the short wave radiation at southern higher latitudes should be corrected. Furthermore, tests were performed concerning short wave radiation which was increased in the tropics and decreased in the subsidence zones.The heat and fresh water fluxes are assessed by using a scheme of Macdonald and Wunsch based on hydrographic sections. The net heat fluxes of ERA and of the forcing dataset are consistent with the heat flux divergences and convergences estimated by this scheme except for parts of the South Atlantic and the Indian Ocean sector of the Southern Ocean where none of these datasets is consistent with these estimates. In the subtropical South Indian Ocean the forcing dataset is consistent with these estimates while ERA are not. The flux components of ERA and the forcing dataset were compared to several observational datasets (SRB, SOC, HOAPS, GPCP, and CMAP). For each component, at least one of these datasets (especially HOAPS) supports the effects of the inverse procedure and the bulk formulae almost globally with some regional exceptions: short wave radiation in the tropical oceans and the subtropical North Atlantic, latent heat flux at higher latitudes, and precipitation in the northern North Atlantic.Comparisons to the NCAR/NCEP Re-Analyses (NRA) (versions 1 and 2) and the ECHAM model in place of ERA lead to similar results. In the North Atlantic the net heat fluxes of the model based datasets approach the hydrographic estimate with increasing resolution. Applied to any ocean/sea-ice model and compared to ERA, the forcing dataset would induce only a relative small net sea-surface buoyancy loss.A comparison of the forcing dataset to measurements made using one buoy deployed in the western Pacific warm pool and five buoys deployed in the subduction region of the Northeast Atlantic shows that at the site of the first buoy the net heat fluxes of the forcing dataset are in poorer agreement than those of ERA. At the sites of two subduction buoys both datasets show the same level of agreement within the error bars specified. At the sites of the three remaining subduction buoys the forcing dataset shows a marginal improvement on ERA.     

WRF-Solar模式对山东太阳总辐射的模拟效果检验

利用专门为太阳能资源评估应用的 WRF-Solar数值模式系统,结合 MODIS 气溶胶光学厚度（AOD550 nm）数据,设置了5种山东区域总辐射模拟方案,使用山东济南、福山、吉县3个太阳辐射站总辐射观测数据,对晴天、阴天、雨天以及四季代表月等逐时总辐射模拟结果进行了对比检验。 结果表明：WRF-Solar数值模式对总辐射模拟能力在晴天和少云天最好,阴雨天较差,四季代表月中,天气过程较少的秋季和冬季模拟效果较好,春季次之,夏季相对较差;晴天和少云天、阴天和雨天以及不考虑天气过程的四季代表月所有日条件下,长、短波辐射方案分别采用RRTMG方案、new Goddard 方案,积云对流参数化方案均采用Grell 3D集合方案,同时使用AOD550 nm的气溶胶数据的总辐射模拟能力最强;WRF-Solar模式中加入 MODIS 气溶胶光学厚度资料后,山东区域晴天总辐射模拟结果明显改善,秋季、冬季代表月亦明显改善,但阴天和雨天总辐射模拟结果改善不明显,低能见度日总辐射模拟结果有所改善。