首页 | 本学科首页   官方微博 | 高级检索  
相似文献
 共查询到20条相似文献,搜索用时 15 毫秒
1.
沙尘气溶胶与气候变化   总被引:17,自引:2,他引:15  
沙尘气溶胶通过吸收和散射太阳辐射与长波辐射影响地球辐射收支和能量平衡,从而影响气候变化。另一方面,气候变化,土地利用、沙漠化和城市化等人类活动都是可能导致大气中矿物沙尘气溶胶的改变。沙尘气溶胶在全球及区域尺度气候和环境变化中起着十分重要的作用。  相似文献   

2.
The location of Central Asia,almost at the center of the global dust belt region,makes it susceptible for dust events.The studies on atmospheric impact of dust over the region are very limited despite the large area occupied by the region and its proximity to the mountain regions(Tianshan,Hindu Kush-Karakoram-Himalayas,and Tibetan Plateau).In this study,we analyse and explain the modification in aerosols'phys-ical,optical and radiative properties during various levels of aerosol loading observed over Central Asia utilizing the data collected during 2010-2018 at the AERONET station in Dushanbe,Tajikistan.Aerosol epi-sodes were classified as strong anthropogenic,strong dust and extreme dust.The mean aerosol optical depth(AOD)during these three types of events was observed a factor of~3,3.5 and 6.6,respectively,higher than the mean AOD for the period 2010-2018.The corresponding mean fine-mode fraction was 0.94,0.20 and 0.16,respectively,clearly indicating the dominance of fine-mode anthropogenic aerosol during the first type of events,whereas coarse-mode dust aerosol dominated during the other two types of events.This was corroborated by the relationships among various aerosol parameters(AOD vs.AE,and EAE vs.AAE,SSA and RRI).The mean aerosol radiative forcing(ARF)at the top of the atmosphere(ARFTOA),the bottom of the atmosphere(ARFBOA),and in the atmosphere(ARFATM)were-35±7,-73±16,and 38±17 Wm-2 during strong anthropogenic events,-48±12,-85±24,and 37±15 Wm-2 during strong dust event,and-68±19,-117±38,and 49±21 Wm-2 during extreme dust events.Increase in aerosol loading enhanced the aerosol-induced atmospheric heating rate to 0.5-1.6 K day-1(strong anthropogenic events),0.4-1.9 K day-1(strong dust events)and 0.8-2.7 K day 1(extreme dust events).The source regions of air masses to Dushanbe during the onset of such events are also identified.Our study con-tributes to the understanding of dust and anthropogenic aerosols,in particular the extreme events and their disproportionally high radiative impacts over Central Asia.  相似文献   

3.
The spatial and temporal variations in aerosols and precursor gases over oceanic regions have special importance in the estimation of radiative forcing parameters and thereby in the refinement of general circulation models. Extensive observations of the columnar aerosol optical depth (AOD), total column ozone (TCO) and precipitable water content (PWC) have been carried out using the on-line, multi-band solar radiometers onboard ORV Sagar Kanya (Cruise # SK 147B) over Bay of Bengal during 11th–28th August 1999. Aerosol optical and physical properties (optical depth and angstrom parameter) have been estimated at six wavelengths covering from UV to NIR (380–1020 nm) while TCO and PWC have been determined using the UV band around 300 nm and NIR band around 940 nm, respectively. Added, concurrent meteorological and satellite observations during this field phase of BOBMEX-99 have been utilized to investigate spectral-temporal variations of AOD, TCO and PWC in marine environment. The results indicate lower AODs (around 0.4 at characteristic wavelength of 500 nm) and size distributions with abundance of coarse-mode particles as compared to those aerosols of typical land origin. An interesting result that is found in the present study is the significant reduction in AOD at all wavelengths from initial to later part of observation period due to cloud-scavenging and rain-washout effects as well as signature of coastal aerosol loading. The clear-sky daytime diurnal variation of TCO shows gradual increase during post-sunrise hours, broad maximum during afternoon hours and gradual decrease during pre-sunset hours, which is considered to be due to photochemical reactions. The diurnal variation curve of PWC showed maximum (~ 4 cm) during morning hours and gradual decrease (~ 3.5 cm) towards evening hours, which are found to be greater as compared to typical values over land. Another interesting feature observed is that although the PWC values are very high, there was no proportionate or appreciable enhancement in AOD—a feature that can be utilized to infer composition of aerosols over the study region.  相似文献   

4.
Measurements of the submicron aerosol size distribution made at the Indian Antarctic station, Maitri (70‡45′S, 11‡44′E) from January 10th to February 24th, 1997, are reported. Total aerosol concentrations normally range from 800 to 1200 particles cm−3 which are typical values for the coastal stations at Antarctica in summer. Aerosol size distributions are generally trimodal and open-ended with a peak between 75 and 133 nm and two minima at 42 and 420 nm. Size distributions remain almost similar for several hours or even days in absence of any meteorological disturbance. Total aerosol concentration increases by approximately an order of magnitude whenever a low pressure system passes over the station. Based on the evolution of aerosol size-distributions during such aerosol enhancement periods, three types of cases have been identified. The nucleation mode in all three cases has been suggested to result from the photochemical conversion of the DMS emissions transported either by the marine air or by the air from the ice-melt regions around Maitri. Subsidence of midtropospheric air during the weakening of radiative inversion is suggested as a possible source of the nucleation mode particles in the third case. Growth of the nucleation mode particles by condensation, coagulation and/or by cloud processes has been suggested to be responsible for other modes in size distributions.  相似文献   

5.
Lidar observations of aerosol vertical distributions in the lower troposphere along with observations of horizontal and vertical winds from collocated UHF radar (Wind Profiler) over a tropical Indian station, Pune during the pre-monsoon season (March–May) of 2006 as part of an ISRO-GBP national campaign (ICARB) have been examined. Lidar vertical profiles showed high aerosol concentrations in the surface layers and a subsequent gradual decrease with height. Results showed the presence of an elevated stratified aerosol layer around 2000–3500m height which persisted throughout the months of March and April. Observed strong vertical gradients in both horizontal and vertical winds in the lower troposphere seem to be a possible cause for the formation of elevated aerosol layers. Further, high daytime temperatures accompanied by dry conditions at the surface help to enhance the aerosol loading in the lower layers over this location.  相似文献   

6.
The paper addresses influence of dust particles on the aerosol loading over the major deserts in the northern hemisphere. The role of dust aerosols in the total aerosol concentration and size distribution of the particles are analysed. It is observed that the aerosol loading is high in the northern hemisphere of which the deserts and adjoining areas in Asia and Africa play a leading role. Over the entire oceanic region, except some parts of the Atlantic Ocean near to the West coast of Africa and the Arabian Sea, aerosol loading is less. The Sahara Desert is the prominent source of dust aerosols throughout the year. The deserts of Asia are also prominent sources of dust aerosols on a global basis. Above 70% of the total aerosol optical depth (AOD) is contributed by the dust particles, reaching to around 90% during spring months March, April and May over the Sahara Desert, which is the major source of dust aerosols. Goddard Chemistry Aerosol Radiation and Transport model is used to estimate the dust aerosol concentration over the deserts of Asia and Africa. The model output almost agrees with the regions of dust loading obtained from the Envisat/SCIAMACHY. Hence, the model is reliable in estimating the dust aerosol loading over the major dust aerosol sources. The major portion of the total dust loading belongs to coarse mode particles.  相似文献   

7.
Intensive measurements were conducted in Xi’an, China before and during a COVID-19 lockdown period to investigate how changes in anthropogenic emissions affected the optical properties and radiative effects of brown carbon (BrC) aerosol. The contribution of BrC to total aerosol light absorption during the lockdown (13%–49%) was higher compared with the normal period (4%–29%). Mass absorption cross-sections (MACs) of specific organic aerosol (OA) factors were calculated from a ridge regression model. Of the primary OA (POA), coal combustion OA (CCOA) had the largest MACs at all tested wavelengths during both periods due to high molecular-weight BrC chromophores; that was followed by biomass burning OA (BBOA) and hydrocarbon-like OA (HOA). For secondary OA (SOA), the MACs of the less-oxidized oxygenated OA (OOA) species (LO-OOA) at λ = 370–590 nm were higher than those of more-oxidized OOA (MO-OOA) during both periods, presumably due to chromophore bleaching. The largest contributor to BrC absorption at the short wavelengths was CCOA during both periods, but BrC absorption by LO-OOA and MO-OOA became dominant at longer wavelengths during the lockdown. The estimated radiation forcing efficiency of BrC over 370–600 nm increased from 37.5 W·g?1 during the normal period to 50.2 W·g?1 during the lockdown, and that enhancement was mainly caused by higher MACs for both LO-OOA and MO-OOA. This study provides insights into the optical properties and radiative effects of source-specific BrC aerosol when pollution emissions are reduced.  相似文献   

8.
The present study is on the aerosol optical and radiative properties in the short-wave radiation and its climate implications at the arid city of Abu Dhabi (24.42 °N, 54.61 °E, 4.5 m MSL), in the United Arab Emirates. The direct aerosol radiative forcings (ARF) in the short-wave region at the top (TOA) and bottom of the atmosphere (BOA) are estimated using a hybrid approach, making use of discrete ordinate radiative transfer method in conjunction with the short-wave flux and spectral aerosol optical depth (AOD) measurements, over a period of 3 years (June 2012–July 2015), at Abu Dhabi located at the south-west coast of the Arabian Gulf. The inferred microphysical properties of aerosols at the measurement site indicate strong seasonal variations from the dominance of coarse mode mineral dust aerosols during spring (March–May) and summer (June–September), to the abundance of fine/accumulation mode aerosols mainly from combustion of fossil-fuel and bio-fuel during autumn (October–November) and winter (December–February) seasons. The monthly mean diurnally averaged ARF at the BOA (TOA) varies from ?13.2 Wm?2 (~?0.96 Wm?2) in November to ?39.4 Wm?2 (?11.4 Wm?2) in August with higher magnitudes of the forcing values during spring/summer seasons and lower values during autumn/winter seasons. The atmospheric aerosol forcing varies from + 12.2 Wm?2 (November) to 28.2 Wm?2 (June) with higher values throughout the spring and summer seasons, suggesting the importance of mineral dust aerosols towards the solar dimming. Seasonally, highest values of the forcing efficiency at the surface are observed in spring (?85.0 ± 4.1 W m?2 τ ?1) followed closely by winter (?79.2 ± 7.1 W m?2 τ ?1) and the lowest values during autumn season (?54 ± 4.3 W m?2 τ ?1). The study concludes with the variations of the atmospheric heating rates induced by the forcing. Highest heating rate is observed in June (0.39 K day ?1) and the lowest in November (0.17 K day ?1) and the temporal variability of this parameter is linearly associated with the aerosol absorption index.  相似文献   

9.
Satellite remote sensing provides important observational constraints for monitoring dust life cycle and improving the understanding of its effects on local to global scales. The present work analyzes the dust aerosol patterns over the arid environment of the Sistan region in southeastern Iran, by means of multiple satellite platforms aiming to reveal the spatio-temporal distribution and trends. The dataset includes records of Aerosol Index (AI) from Total Ozone Mapping Spectrometer (TOMS) (1978–2001) and 6-year AI records from the Ozone Monitoring Instrument (OMI) aboard Aura. Moreover, the aerosol optical depth is analyzed through 11-year records from Multi-angle Imaging Spectroradiometer (MISR) aboard Terra (2000–2010) and from Moderate-resolution Imaging Spectroradiometer (MODIS) onboard Terra (2000–2007) and Aqua (2002–2011). The main focus is to determine the similarities and differences in dust variability over southwest Asia, in general, and the Sistan region, in particular. The results show a marked seasonal cycle with high aerosol loading during summer and lower in winter, while MISR, MODIS, and TOMS/OMI observations agree in both terms of monthly and seasonally mean spatial and temporal patterns. The higher aerosol concentrations during summer are interpreted as a result of the combined effect of the seasonal drying of the Hamoun lakes and the strong northerly Levar winds favoring dust erosion from the alluvial deposits in Sistan. After prolonged drought period, the dust aerosol load over the area has increased in the beginning of the 2000 s and decreased after 2004, thereby leading to an overall declining trend during the last decade. Such a trend is absent during the winter period when dust emission over the region is minimal.  相似文献   

10.
Continuous and campaign-based aerosol field measurements are essential in understanding fundamental atmospheric aerosol processes and for evaluating their effect on global climate, environment and human life. Synchronous measurements of Aerosol Optical Depth (AOD), Black Carbon (BC) aerosol mass concentration and aerosol particle size distribution were carried out during the campaign period at tropical urban regions of Hyderabad, India. Daily satellite datasets of DMSP-OLS were processed for night-time forest fires over the Indian region in order to understand the additional sources (forest fires) of aerosol. The higher values in black carbon aerosol mass concentration and aerosol optical depth correlated well with forest fires occurring over the region. Ozone Monitoring Instrument (OMI) aerosol index (AI) variations showed absorbing aerosols over the region and correlated with ground measurements.  相似文献   

11.
Here we review the methods presently available and expected in the near future for retrieving the tropospheric aerosol properties using remote sensing. Since all aerosol properties cannot be derived from space, measurements performed from the surface of the Earth are used to adjust the parameters that are not directly accessible and to limit the variability of the parameters that present a weaker sensitivity. The aerosol properties derived include the column concentration (expressed by the aerosol optical depth), the size (given by distribution of the aerosol in 2 to 3 size modes or measurement of the Angström coefficient), composition (expressed by the refractive index), shape and vertical profile. The article is restricted to aerosols that are within the troposphere since the techniques used for stratospheric aerosols are very specific.  相似文献   

12.
During the field cruises of the Indian Ocean Experiment (INDOEX) extensive measurements on the atmospheric chemical and aerosol composition are undertaken to study the long-range transport of air pollution from south and southeast Asia towards the Indian Ocean during the dry monsoon season in 1998 and 1999. The present paper discusses the temporal and spatial variations in aerosols and aerosol forcing during the winter monsoon season (January-March) for INDOEX first field phase (FFP) in 1998 and INDOEX intensive field phase (IFP) in 1999. An interactive chemistry/aerosol model (LMDZ.3.3) is used to investigate the variation in the spatial distribution of tropospheric sulphate aerosols during 1998 and 1999. The model results depict major enhancement in the sulphate aerosol concentrations, radiative forcing (RF) and optical depth over the Indian subcontinent and adjoining marine areas between INDOEX-FFP and IFP. A significant increase in transport of sulphate aerosols from the continents to the Indian Ocean region has also been simulated during the winter monsoon in 1999. The mean RF over INDOEX-FFP in 1998 is found to be ?1.2 Wm–2 while it increased to ?1.85 Wm–2 during INDOEX-IFP in 1999. Model results reveal a mean sulphate aerosol optical depth (AOD) of 0.08 and 0.14 over Indian subcontinent during 1998 and 1999, respectively. The model results suggest that elevated AOD downwind of source regions in India can significantly affect the regional air quality and adjoining marine environments.  相似文献   

13.
Abstract: Twenty-four soil samples were collected at three depths from an approximately 2.5 acre contaminated site in southern Piedmont (Italy) and then analyzed. The main soil parameters determined were: pH, Cation Exchange Capacity (CEC), particle size distribution, total organic carbon (TOC) content and retained metal concentration. The mineral phases were identified by X-Ray Powder Diffraction (XRPD). All of the samples contained Zn and Cu resulting from industrial contamination during the last century, and those obtained at depths of 20-40 cm consistently showed the highest levels. To determine which size fraction was most active in the retention process, the samples were separated into four fractions (≤2 mm, ≤63 μm, ≤30 μm and ≤2 μm) and the amount of pollutant measured in each. It was found that metal retention was the highest in the clayey fraction, whose clay minerals were identified by XRPD after K+ and Mg2+ saturation, glycerol treatment and heating to 550°C. The clayey fraction was also the richest in TOC, and a direct correlation between TOC amount and metal retention was observed.  相似文献   

14.
Airborne measurements of the number concentration and size distribution of aerosols from 13 to 700 nm diameter have been made at four vertical levels across a coastline at Bhubaneswar (20°25′N, 85°83′E) during the Integrated Campaign for Aerosols, gases and Radiation Budget (ICARB) programme conducted in March–April 2006. The measurements made during the constant-level flights at 0.5, 1, 2 and 3 km altitude levels extend ~100 km over land and ~150km over ocean. Aerosol number concentrations vary from 2200 to 4500 cm?3 at 0.5 km level but are almost constant at ~ 6000 cm?3 and ~ 800 cm?3 at 2 and 3 km levels, respectively. At 1km level, aerosol number concentration shows a peak of 18,070 cm?3 around the coastline. Most of the aerosol size distribution curves at 0.5 km and 1 km levels are monomodal with a maxima at 110nm diameter which shifts to 70 nm diameter at 2 and 3 km levels. However, at the peak at 1 km level, number concentration has a bimodal distribution with an additional maximum appearing in nucleation mode. It is proposed that this maxima in nucleation mode at 1 km level may be due to the formation and transport of new particles from coastal regions.  相似文献   

15.
Mass concentration and mass size distribution of total (composite) aerosols near the surface are essential inputs needed in developing aerosol models for radiative forcing estimation as well as to infer the environment and air quality. Using extensive measurements onboard the oceanographic research vessel, Sagar Kanya, during its cruise SK223B in the second phase of the ocean segment of the Integrated Campaign for Aerosols, gases and Radiation Budget (ICARB), the spatial distribution of the mass concentration and mass size distribution of near-surface aerosols are examined for the first time over the entire Arabian Sea, going as far as 58°E and 22°N, within a span of 26 days. In general, the mass concentrations (M T ) were found to be low with the mean value for the entire Arabian Sea being 16.7 ± 7 μg m?3; almost 1/2 of the values reported in some of the earlier campaigns. Coarse mode aerosols contributed, on an average, 58% to the total mass, even though at a few pockets accumulation mode contribution dominated. Spatially, significant variations were observed over central and northern Arabian Sea as well as close to the west coast of India. In central Arabian Sea, even though the M T was quite low, contribution ofs accumulation aerosols to the total mass concentration was greater than 50%. Effective radius, a parameter important in determining scattering properties of aerosol size distribution, varied between 0.07 and 0.4 μm with a mean value of 0.2 μm. Number size distributions, deduced from the mass size distributions, were approximated to inverse power-law form and the size indices (ν) were estimated. It was found to vary in the range 3.9 to 4.2 with a mean value of 4.0 for the entire oceanic region. Extinction coefficients, estimated using the number-size distributions, were well-correlated with the accumulation mode mass concentration with a correlation coefficient of 0.82.  相似文献   

16.
文章利用2002年3月29日~4月4日在浙江临安大气本底污染监测站观测的气溶胶粒子质量谱、离子与元素成分的数据,结合TOMS卫星的气溶胶指数资料和轨迹模式,重点分析在北方沙尘暴输送影响期间临安气溶胶质量浓度尺度分布的演变特点以及气溶胶化学成分与不同空气来源的关系。初步分析结果显示,受北方沙尘暴天气影响,临安气溶胶质量浓度、离子、元素浓度有明显的尺度分布演变。这种演变与污染物来源和大气污染物的气粒转化有关。沙尘影响前和结束后临安地区气溶胶主要以细粒子为主(<2.1μm),峰值粒径0.65~2.1μm,而受北方地区的沙尘暴影响,峰值粒径偏移到2.1~3.3μm,且在7~11μm间出现另一个峰值,同时临安气溶胶粗粒子中矿物元素显著增加。从离子成分看,在整个观测期间SO2-4与NH+4在细粒子段有很好的一致性,而SO2-4,NO-3与Ca2+在粗粒子段有很好的相关,尤其是沙尘影响期间NO-3与Ca2+有很好的对应关系,表现出较明显的表面非均相反应特征  相似文献   

17.
Horizontal surface visibility range, one of the simplest measures of local atmospheric pollution, is critical for aviation, surface transport besides long-term impact on human health and climate. Long-term observations from multiple stations (including airports) across the world show statistically significant decline in visibility. We have studied climatology and trends of morning poor visibility days (PVD, visibility <4 km) and afternoon good visibility days (GVD, visibility >10 km) based on 279 surface meteorological stations well distributed over India for the period 1961–2008. During last 5 decades, all India averaged range of annual morning PVD has increased from 6.7 to 27.3 % days, while the range of afternoon GVD has decreased from 76.1 to 30.6 % days. Annually, the morning PVD increased significantly at 3.3 % days per decade, and the afternoon GVD declined significantly at ?8.6 % days per decade. Seasonally, the highest increase in morning PVD has occurred in winter (+4.3 % days per decade), while post-monsoon has the highest decrease in afternoon GVD (?9.2 % days per decade). In spatial distribution, visibility has decreased nationwide especially over Indo-Gangetic (IG) plains, central, east and northeast India which is due to increased wintertime fog, water vapor and aerosol loading. The IG plains suffer from increased fog or smog and aerosol loading during wintertime. Long-term visibility impairment over India is visible through increasing morning PVD (decreasing GVD) and decreasing afternoon GVD (increasing PVD) which are spatially well correlated with increasing relative humidity and decreasing wind speed (seasonal).  相似文献   

18.
The objective of this study is to evaluate the ability of a European chemistry transport model, ‘CHIMERE’ driven by the US meteorological model MM5, in simulating aerosol concentrations [dust, PM10 and black carbon (BC)] over the Indian region. An evaluation of a meteorological event (dust storm); impact of change in soil related parameters and meteorological input grid resolution on these aerosol concentrations has been performed. Dust storm simulation over Indo-Gangetic basin indicates ability of the model to capture dust storm events. Measured (AERONET data) and simulated parameters such as aerosol optical depth (AOD) and Angstrom exponent are used to evaluate the performance of the model to capture the dust storm event. A sensitivity study is performed to investigate the impact of change in soil characteristics (thickness of the soil layer in contact with air, volumetric water, and air content of the soil) and meteorological input grid resolution on the aerosol (dust, PM10, BC) distribution. Results show that soil parameters and meteorological input grid resolution have an important impact on spatial distribution of aerosol (dust, PM10, BC) concentrations.  相似文献   

19.
India Peninsula and East Asia are high aerosol loading regions as well as major regions influenced by Asian monsoon. The changes of monsoon intensity and precipitation have great influence on economy, especially agricultural production of monsoon regions. There are many researches of impacts of aerosol on Indian monsoon, which have achieved many comprehensive progresses. Earlier researches show that atmospheric brown cloud caused negative radiative forcing and weakened the warming induced by greenhouse gases. Current researches show that absorbing aerosol enhanced the Indian monsoon and increased rainfall in pre-monsoon season, while the scattering effect of aerosol weakened the Indian summer monsoon and the East Asian summer monsoon and rainfall in monsoon season. Due to so many factors affecting the monsoon, researches of aerosol impacts on monsoon become more complex. Thus, these results remain uncertain. This paper reviews previous researches and generalizes the mechanisms of impacts of aerosols on Asian monsoon. By comparing the East Asian summer monsoon with the Indian summer monsoon, we discussed deficiencies of the prior researches, and pointed out the direction for future researches about the impact of aerosol on the Asian summer monsoon, especially on the East Asian summer monsoon.  相似文献   

20.
In this research, a torsional cyclic shear test was modeled using the 3D discrete element method (DEM). The results are compared against experimental data and micro-mechanical aspects of the soil during the loading are discussed. The aim of the work is to study the homogeneity of strains during this laboratory test and to compare the micro-mechanical behavior of the soil sample for different strain levels. The experimental investigation was performed using a synthetic soil material made of glass beads, which simplifies the modeling and calibration since normal interaction forces do not induce rotation of the particles. Both the model and experimental tests used the same grading distribution and particle size. We showed that the hysteresis cycles can be properly reproduced in terms of shape and magnitude. Thus, we obtained a robust estimation for the secant shear modulus and damping ratio at different strain levels. With this, it was possible to build stiffness degradation and damping increase curve to compare it with experimental data obtained from torsional shear tests. Based on this validation of the DEM model, we discuss the micro-mechanical behavior of the soil and its relation with the macroscopic parameters obtained. It is shown that shear strain distribution on the sample is not uniform and that large values of strains concentrate close to the top of the sample as top rotation increases, which differs from the standard assumption of a constant value across the height of the sample. Additionally, it is observed that at 0.8 times radius, the cumulative torque reaches approximately 90% of the total torque applied to sample.  相似文献   

设为首页 | 免责声明 | 关于勤云 | 加入收藏

Copyright©北京勤云科技发展有限公司  京ICP备09084417号