Experimental study on reduction of U (Ⅵ) by an anaerobic bacterium, Shewanella putrefaciens: Application to sandstone-hosted interlayer oxidation-zone type uranium deposits, China

An experimental study on reduction of U (Ⅵ) by anaerobic bacteria, Shewane//a putrefaciens, is first reported here in China. The experimental conditions were: 35℃ and pH =7.0-7.4, corresponding to a physicochemical environments in which the sandstone-hosted interlayer oxidation-zone type uranium deposit formed in Northwest China's Xinjiang. Bacteria adopted in the present experiment, Shewanella putrefaciens, occur extensively in natural environment. Our study shows that nano-crystal precipitates of uraninite quickly occurred on the surface of the cells within one week. It was found that the pitchblende was characterized by a random arrangement of uraninite nanocrystals (2-4 nm) in it, significantly different from natural pitchblende in which uraninite nanocrystals are arranged in order. Finally, a possible mechanism of uranium biomineralization by microorganisms in the deposits is discussed. Our investigation may supply a technical train of thoughts for bioremediation of nuclear-contaminated water environments and for underground dissolving extraction of the sandstone-hosted uranium ores.     

Experimental study on reduction of U (VI) by an anaerobic bacterium, <Emphasis Type="Italic">Shewanella putrefaciens</Emphasis>: Application to sandstone-hosted interlayer oxidation-zone type uranium deposits,China

An experimental study on reduction of U (VI) by anaerobic bacteria, Shewanella putrefaciens, is first reported here in China. The experimental conditions were: 35°C and pH= 7.0-7.4, corresponding to a physicochemical environments in which the sandstone-hosted interlayer oxidation-zone type uranium deposit formed in Northwest China’s Xinjiang. Bacteria adopted in the present experiment, Shewanella putrefaciens, occur extensively in natural environment. Our study shows that nano-crystal precipitates of uraninite quickly occurred on the surface of the cells within one week. It was found that the pitchblende was characterized by a random arrangement of uraninite nanocrystals (2-4 nm) in it, significantly different from natural pitchblende in which uraninite nanocrystals are arranged in order. Finally, a possible mechanism of uranium biomineralization by microorganisms in the deposits is discussed. Our investigation may supply a technical train of thoughts for bioremediation of nuclear-contaminated water environments and for underground dissolving extraction of the sandstone-hosted uranium ores.     

Sorption behavior of U(VI), ~(234)U(VI) and ~(238)U(VI) onto fracture-filling clays in Beishan granite, Gansu: Application to selecting the site of high-level radwaste repository in China

Knowing the transport of uranium and radionu-clides through the environment is important for as-sessing the risk posed by long-term disposal of rad-waste. Granitic rocks have been selected as a host-rock type for the first high-level radwaste repository in China. According to the Chinese High-level Rad-waste Management Program, high-level radwaste (HLW) will be buried at 800―1000 m depth in a granitic pluton in Northwest China and, specifically, in the A granitic complex of Beishan area,…     

Application of ~(137)Cs fingerprinting technique to interpreting sediment production records from reservoir deposits in a small catchment of the Hilly Loess Plateau, China

According to variations of 137Cs and clay contents, 44 flood couplets were identified in a profile of res- ervoir deposit with a vertical length of 28.12 m in the Yuntaishan Gully. Couplet 27 at the middle of the profile had the highest average 137Cs content of 12.65 Bq·kg?1, which indicated the 1963s' deposits, then 137Cs content decreased both downward and upward in the profile. The second top and bottom couplets had average 137Cs contents of 2.15 Bq·kg?1 and 0.92 Bq·kg?1, respectively. By integrated analysis of reservoir construction and management history, variations of 137Cs contents over the profile, sediment yields of flood couplets and rainfall data during the period of 1958-1970, individual storms related to the flood couplets were identified. 44 floods with a total sediment yield of 2.36×104 m3 occurred and flood events in a year varied between 1 and 10 times during the period of 1960-1970. 7-10 flood events occurred during the wet period of 1961-1964 with very wet autumn, while only 1-2 events during the dry period of 1965-1969. Average annual specific sediment yield was 1.29×104 t·km?2·a?1 for the Yuntaishan Gully during the period of 1960-1970, which was slightly higher than 1.11 ×104 t·km?2·a?1 for the Upper Yanhe River Basin above the Ganguyi Hydrological Station and slightly lower than 1.40 ×104 t·km?2·a?1 for the nearby Zhifang Gully during the same period. Annual specific sediment yields for the Yuntaishan Gully were correlated to the wet season's rainfalls well.