首页 | 本学科首页   官方微博 | 高级检索  
相似文献
 共查询到20条相似文献,搜索用时 31 毫秒
1.
A screening and ranking framework (SRF) has been developed to evaluate potential geologic carbon dioxide (CO2) storage sites on the basis of health, safety, and environmental (HSE) risk arising from CO2 leakage. The approach is based on the assumption that CO2 leakage risk is dependent on three basic characteristics of a geologic CO2 storage site: (1) the potential for primary containment by the target formation; (2) the potential for secondary containment if the primary formation leaks; and (3) the potential for attenuation and dispersion of leaking CO2 if the primary formation leaks and secondary containment fails. The framework is implemented in a spreadsheet in which users enter numerical scores representing expert opinions or published information along with estimates of uncertainty. Applications to three sites in California demonstrate the approach. Refinements and extensions are possible through the use of more detailed data or model results in place of property proxies.  相似文献   

2.
Geologic carbon sequestration is the capture of anthropogenic carbon dioxide (CO2) and its storage in deep geologic formations. The processes of CO2 seepage into surface water after migration through water-saturated sediments are reviewed. Natural CO2 and CH4 fluxes are pervasive in surface-water environments and are good analogues to potential leakage and seepage of CO2. Buoyancy-driven bubble rise in surface water reaches a maximum velocity of approximately 30 cm s−1. CO2 rise in saturated porous media tends to occur as channel flow rather than bubble flow. A comparison of ebullition versus dispersive gas transport for CO2 and CH4 shows that bubble flow will dominate over dispersion in surface water. Gaseous CO2 solubility in variable-salinity waters decreases as pressure decreases leading to greater likelihood of ebullition and bubble flow in surface water as CO2 migrates upward.  相似文献   

3.
《China Geology》2022,5(3):359-371
To accelerate the achievement of China’s carbon neutrality goal and to study the factors affecting the geologic CO2 storage in the Ordos Basin, China’s National Key R&D Programs propose to select the Chang 6 oil reservoir of the Yanchang Formation in the Ordos Basin as the target reservoir to conduct the geologic carbon capture and storage (CCS) of 100000 t per year. By applying the basic theories of disciplines such as seepage mechanics, multiphase fluid mechanics, and computational fluid mechanics and quantifying the amounts of CO2 captured in gas and dissolved forms, this study investigated the effects of seven factors that influence the CO2 storage capacity of reservoirs, namely reservoir porosity, horizontal permeability, temperature, formation stress, the ratio of vertical to horizontal permeability, capillary pressure, and residual gas saturation. The results show that the sensitivity of the factors affecting the gas capture capacity of CO2 decreases in the order of formation stress, temperature, residual gas saturation, horizontal permeability, and porosity. Meanwhile, the sensitivity of the factors affecting the dissolution capture capacity of CO2 decreases in the order of formation stress, residual gas saturation, temperature, horizontal permeability, and porosity. The sensitivity of the influencing factors can serve as the basis for carrying out a reasonable assessment of sites for future CO2 storage areas and for optimizing the design of existing CO2 storage areas. The sensitivity analysis of the influencing factors will provide basic data and technical support for implementing geologic CO2 storage and will assist in improving geologic CO2 storage technologies to achieve China’s carbon neutralization goal.©2022 China Geology Editorial Office.  相似文献   

4.
The probability that storage of carbon dioxide (CO2) in deep geologic formations will become an important climate change mitigation strategy depends on a number of factors, namely (1) public acceptance, (2) the cost of geologic storage compared to other climate change mitigation options, and (3) the availability, capacity, and location of suitable sites. Whether or not a site is suitable will be determined by establishing that it can meet a set of performance requirements for safe and effective geologic storage. To date, no such performance requirements have been developed. Establishing effective requirements must start with an evaluation of how much CO2 might be stored and for how long the CO2 must remain underground to meet goals for controlling atmospheric CO2 concentrations. Answers to these questions provide a context for setting performance requirements for geologic storage projects.According to the results presented here, geologic storage could be an effective method to ease the transition away from a fossil-fuel based economy over the next several centuries, even if large amounts of CO2 are stored and some small fraction seeps from storage reservoirs back into the atmosphere. An annual seepage rate of 0.01% or 10-4/year would ensure the effectiveness of geologic carbon storage for any of the projected sequestration scenarios explored herein, even those with the largest amounts of storage (1,000 s of gigatonnes of carbon-GtC), and still provide some safety margin. Storing smaller amounts of carbon (10 s to 100 s of GtC) may allow for a slightly higher seepage rate on the order of 0.1% or 10-3/year. Based on both the large capacity of geologic storage formation and the likelihood of achieving leakage rates much lower than the rates estimated here, geologic storage appears to be a promising mitigation strategy.  相似文献   

5.
One possible way of mitigating carbon dioxide (CO2) emissions from fossil fuel combustion is using carbon dioxide capture and storage (CCS) technology. However, public perception concerning CO2 storage in the geosphere is generally negative, being particularly motivated by perceived leakage risks. Therefore, a main issue when attempting to gain public acceptance is ensuring provision of appropriate monitoring practices, aimed at providing health, safety and environmental risk assessment, so that potential risks from CO2 storage are minimized. Naturally occurring CO2 deposits provide unique natural analogues for evaluating and validating methods used for the detection and monitoring of CO2 spreading and degassing into the atmosphere. Geological and hydrological structures of the Cheb Basin (NW Bohemia, Czech Republic) represent such a natural analogue for investigating CO2 leakage and offer a perfect location at which to verify monitoring tools used for direct investigation of processes along preferential migration paths. This shallow basin dating from the Tertiary age is characterized by up to 300?m thick Neogene sediment deposits and several tectonically active faults. The objectives of this paper are to introduce the CO2 analogues concept to present the Eger Rift as a suitable location for a natural CO2 analogue site and to demonstrate to what extent such an analogue site should be used (with a case study). The case study presents the results obtained from a joint application of geoelectrical measurements in combination with soil CO2 concentration and flux determination methods, for the detection and characterization of natural CO2 releases at gas seeps (as part of a hierarchic monitoring concept). To highlight discharge-controlling structural near surface features was the initial motivation for the application of geoelectrical measurements. Soil-gas concentration and flux measurement techniques are relatively simple to employ and are valuable methods that can be used to monitor seeping CO2 along preferential pathways. Joint interpretation of both approaches yields a first insight into fluid paths and reveals that the thickness and permeability of site-specific near surface sedimentary deposits have a great influence upon the spatial distribution of the CO2 degassing pattern at surface level.  相似文献   

6.
An overview on the tectono-stratigraphic framework of the Arabian plate indicates obvious differences between two distinct areas: the hydrocarbon-prolific sector and non-hydrocarbon-prolific sector. These differences resulted from the interplay of a variety of factors; some of which are related to the paleo-geographic configuration (eustatic sea level fluctuations, climatic conditions, and salt Basins), others to differential subsidence (burial) and structural inversions. During the Paleozoic, the regional compression was caused by far field effects of the Hercynian orogeny. This led to major folded structures in central and eastern Saudi Arabia (e.g. Ghawar anticline). During the Mesozoic, the most important tectonic factor was the stretching of the crust (extension), accompanied with the increase in temperature, resulting in an increase of the accommodation space, and thicker sedimentary successions. Regional unconformities are mostly found where folded structures are dominant, and they acted as a carrier systems for the accumulation of hydrocarbon and groundwater. A good understanding of the stratigraphy and tectonic evolution is, thus, required to develop carbon capture and storage (CCS) and to design efficiently enhanced oil recovery (EOR) in both sectors. Oil and gas reservoirs offer geologic storage potential as well as the economic opportunity of better production through CO2-EOR. The world greatest hydrocarbon reservoirs mainly consist of Jurassic carbonate rocks, and are located around the Arabian Basin (including the eastern KSA and the Arabian Gulf). The Cretaceous reservoirs, which mainly consist of calcarenite and dolomite, are located around the Gotnia salt Basin (northeast of KSA). Depleted oil and gas fields, which generally have proven as geologic traps, reservoirs and seals, are ideal sites for storage of injected CO2. Each potential site for CO2-EOR or CCS should be evaluated for its potential storage with respect to the containment properties, and to ensure that conditions for safe and effective long term storage are present. The secured deep underground storage of CO2 implies appropriate geologic rock formations with suitable reservoir rocks, traps, and impermeable caprocks. Proposed targets for CCS, in the non-hydrocarbon-prolific sector, are Kharij super-aquifer (Triassic), Az-Zulfi aquifer (Middle Jurassic), Layla aquifer (Late Jurassic), and Wasia aquifer (Middle Cretaceous). Proposed targets for EOR are Safaniya oil field (Middle Cretaceous) (Safaniya, Wara and Khafji reservoirs), Manifa oil field (Las, Safaniya and Khafji reservoirs) (Late Jurassic), and Khuff reservoir (Late Permian-Early Triassic) in central to eastern KSA.  相似文献   

7.
Geologic storage of CO2 is expected to produce plumes of large areal extent, and some leakage may occur along fractures, fault zones, or improperly plugged pre-existing wellbores. A review of physical and chemical processes accompanying leakage suggests a potential for self-enhancement. The numerical simulations presented here confirm this expectation, but reveal self-limiting features as well. It seems unlikely that CO2 leakage could trigger a high-energy run-away discharge, a so-called “pneumatic eruption,” but present understanding is insufficient to rule out this possibility. The most promising avenue for increasing understanding of CO2 leakage behavior is the study of natural analogues.  相似文献   

8.
The potential for metal release associated with CO2 leakage from underground storage formations into shallow aquifers is an important consideration in assessment of risk associated with CO2 sequestration. Metal release can be driven by acidification of groundwaters caused by dissolution of CO2 and subsequent dissociation of carbonic acid. Thus, acidity is considered one of the main drivers for water quality degradation when evaluating potential impacts of CO2 leakage. Dissolution of carbonate minerals buffers the increased acidity. Thus, it is generally thought that carbonate aquifers will be less impacted by CO2 leakage than non-carbonate aquifers due to their high buffering potential. However, dissolution of carbonate minerals can also release trace metals, often present as impurities in the carbonate crystal structure, into solution. The impact of the release of trace metals through this mechanism on water quality remains relatively unknown. In a previous study we demonstrated that calcite dissolution contributed more metal release into solution than sulfide dissolution or desorption when limestone samples were dissolved in elevated CO2 conditions. The study presented in this paper expanded our work to dolomite formations and details a thorough investigation on the role of mineral composition and mechanisms on trace element release in the presence of CO2. Detailed characterization of samples from dolomite formations demonstrated stronger associations of metal releases with dissolution of carbonate mineral phases relative to sulfide minerals or surface sorption sites. Aqueous concentrations of Sr2+, CO2+, Mn2+, Ni2+, Tl+, and Zn2+ increased when these dolomite rocks were exposed to elevated concentrations of CO2. The aqueous concentrations of these metals correlate to aqueous concentrations of Ca2+ throughout the experiments. All of the experimental evidence points to carbonate minerals as the dominant source of metals from these dolomite rocks to solution under experimental CO2 leakage conditions. Aqueous concentrations of Ca2+ and Mg2+ predicted from numerical simulation of kinetic dolomite dissolution match those observed in the experiments when the surface area is three to five orders of magnitude lower than the surface area of the samples measured by gas adsorption.  相似文献   

9.
Quick-look assessments to identify optimal CO2 EOR storage sites   总被引:1,自引:0,他引:1  
A newly developed, multistage quick-look methodology allows for the efficient screening of an unmanageably large number of reservoirs to generate a workable set of sites that closely match the requirements for optimal CO2 enhanced oil recovery (EOR) storage. The objective of the study is to quickly identify miscible CO2 EOR candidates in areas that contain thousands of reservoirs and to estimate additional oil recovery and sequestration capacities of selected top options through dimensionless modeling and reservoir characterization. Quick-look assessments indicate that the CO2 EOR resource potential along the US Gulf Coast is 4.7 billion barrels, and CO2 sequestration capacity is 2.6 billion metric tons. In the first stage, oil reservoirs are screened and ranked in terms of technical and practical feasibility for miscible CO2 EOR. The second stage provides quick estimates of CO2 EOR potential and sequestration capacities. In the third stage, a dimensionless group model is applied to a selected set of sites to improve the estimates of oil recovery and storage potential using appropriate inputs for rock and fluid properties, disregarding reservoir architecture and sweep design. The fourth stage validates and refines the results by simulating flow in a model that describes the internal architecture and fluid distribution in the reservoir. The stated approach both saves time and allows more resources to be applied to the best candidate sites.  相似文献   

10.
Interpretation of carbon dioxide diffusion behavior in coals   总被引:3,自引:1,他引:3  
Storage of carbon dioxide in geological formations is for many countries one of the options to reduce greenhouse gas emissions and thus to satisfy the Kyoto agreements. The CO2 storage in unminable coal seams has the advantage that it stores CO2 emissions from industrial processes and can be used to enhance coalbed methane recovery (CO2-ECBM). For this purpose, the storage capacity of coal is an important reservoir parameter. While the amount of CO2 sorption data on various natural coals has increased in recent years, only few measurements have been performed to estimate the rate of CO2 sorption under reservoir conditions. An understanding of gas transport is crucial for processes associated with CO2 injection, storage and enhanced coalbed methane (ECBM) production.A volumetric experimental set-up has been used to determine the rate of sorption of carbon dioxide in coal particles at various pressures and various grain size fractions. The pressure history during each pressure step was measured. The measurements are interpreted in terms of temperature relaxation and transport/sorption processes within the coal particles. The characteristic times of sorption increase with increasing pressure. No clear dependence of the characteristic time with respect to the particle size was found. At low pressures (below 1 MPa) fast gas diffusion is the prevailing mechanism for sorption, whereas at higher pressures, the slow diffusion process controls the gas uptake by the coal.  相似文献   

11.
In geological formations, migration of CO2 plume is very complex and irregular. To make CO2 capture and storage technology feasible, it is important to quantify CO2 amount associated with possible leakage through natural occurring faults and fractures in geologic medium. Present work examines the fracture aperture effect on CO2 migration due to free convection. Numerical results reveal that fracture with larger-aperture intensify CO2 leakage. Mathematical formulation and equations of state for the mixture are implemented within the object-oriented finite element code OpenGeoSys developed by the authors. The volume translated Peng–Robinson equation of state is used for material properties of CO2 and water.  相似文献   

12.
A variety of structural and stratigraphic factors control geological heterogeneity, inferred to influence both sequestration capacity and effectiveness, as well as seal capacity. Structural heterogeneity factors include faults, folds, and fracture intensity. Stratigraphic heterogeneity is primarily controlled by the geometry of depositional facies and sandbody continuity, which controls permeability structure. The permeability structure, in turn, has implications for CO2 injectivity and near-term migration pathways, whereas the long-term sequestration capacity can be inferred from the production history. Examples of Gulf Coast oil and gas reservoirs with differing styles of stratigraphic heterogeneity demonstrate the impact of facies variability on fluid flow and CO2 sequestration potential. Beach and barrier-island deposits in West Ranch field in southeast Texas are homogeneous and continuous. In contrast, Seeligson and Stratton fields in south Texas, examples of major heterogeneity in fluvial systems, are composed of discontinuous, channel-fill sandstones confined to narrow, sinuous belts. These heterogeneous deposits contain limited compartments for potential CO2 storage, although CO2 sequestration effectiveness may be enhanced by the high number of intraformational shale beds. These field examples demonstrate that areas for CO2 storage can be optimized by assessing sites for enhanced oil and gas recovery in mature hydrocarbon provinces.  相似文献   

13.
In the Alban Hills area, strong areally diffuse and localised spot degassing processes occur (Tivoli, Cava dei Selci, Solforata, Tor Caldara). The gas comprises a large proportion of CO2, with minor CH4, H2S and Rn. These advective features are generated by fluid leakage from buried reservoirs hosted in the structural highs of the Mesozoic carbonate basement. Gas migration towards the surface is controlled by fault and fracture systems bordering the structural highs of the carbonate formations (e.g. Ciampino high). His release is triggered when the total pressure of the fluid phase exceeds the hydrostatic pressure, thus forming a free gas phase. Furthermore, both the sudden and catastrophic, and slow and continuous gas release at surface, of naturally occurring toxic species (CO2, H2S and Rn) poses a serious health risk to people living in this geologically active area.This paper presents data obtained from soil gas and gas flux surveys, as well as gas isotopes analyses, which suggest the presence of a deep origin gas flux enriched in carbon dioxide and minor species (CH4 and H2S), as well as a channelled migration of geogas mixtures having a Rn component which is not produced in situ.In regards to the health risk to local inhabitants, it was found that some anomalous areas had been zoned as parkland while others had been heavily developed for residential purposes. For example, many new houses were found to have been built on ground which has soil gas CO2 concentrations of over 70% and a CO2 flux of about 0.7 kg m−2 day−1, as well as radon values of more than 250 kBq/m3. In addition, an indoor radon survey has been conducted in selected houses in the town of Cava dei Selci to search for a possible correlation between the local geology and the radon concentration in indoor air. Preliminary results indicate high indoor values at ground floor levels (up to 1000 Bq/m3) and very high values in the cellars (up to 250.000 Bq/m3). It is recommended that land-use planners incorporate soil gas and/or gas flux measurements in the environmental assessment of areas of possible risk (i.e. volcanic or structurally active areas).  相似文献   

14.
Geological sequestration of CO2 in depleted oil reservoirs is a potentially useful strategy for greenhouse gas management and can be combined with enhanced oil recovery. Development of methods to estimate CO2 leakage rates is essential to assure that storage objectives are being met at sequestration facilities. Perfluorocarbon tracers (PFTs) were added as three 12 h slugs at about one week intervals during the injection of 2090 tons of CO2 into the West Pearl Queen (WPQ) depleted oil formation, sequestration pilot study site located in SE New Mexico. The CO2 was injected into the Permian Queen Formation. Leakage was monitored in soil–gas using a matrix of 40 capillary adsorbent tubes (CATs) left in the soil for periods ranging from days to months. The tracers, perfluoro-1,2-dimethylcyclohexane (PDCH), perfluorotrimethylcyclohexane (PTCH) and perfluorodimethylcyclobutane (PDCB), were analyzed using thermal desorption, and gas chromatography with electron capture detection. Monitoring was designed to look for immediate leakage, such as at the injection well bore and at nearby wells, and to develop the technology to estimate overall CO2 leak rates based on the use of PFTs. Tracers were detected in soil–gas at the monitoring sites 50 m from the injection well within days of injection. Tracers continued to escape over the following years. Leakage appears to have emanated from the vicinity of the injection well in a radial pattern to about 100 m and in directional patterns to 300 m. Leakage rates were estimated for the 3 tracers from each of the 4 sets of CATs in place following the start of CO2 injection. Leakage was fairly uniform during this period. As a first approximation, the CO2 leak rate was estimated at about 0.0085% of the total CO2 sequestered per annum.  相似文献   

15.
Carbon dioxide capture and geological storage (CCGS) is an emerging technology that is increasingly being considered for reducing greenhouse gas emissions to the atmosphere. Deep saline aquifers provide a very large capacity for CO2 storage and, unlike hydrocarbon reservoirs and coal beds, are immediately accessible and are found in all sedimentary basins. Proper understanding of the displacement character of CO2-brine systems at in-situ conditions is essential in ascertaining CO2 injectivity, migration and trapping in the pore space as a residual gas or supercritical fluid, and in assessing the suitability and safety of prospective CO2 storage sites. Because of lack of published data, the authors conducted a program of measuring the relative permeability and other displacement characteristics of CO2-brine systems for sandstone, carbonate and shale formations in central Alberta in western Canada. The tested formations are representative of the in-situ characteristics of deep saline aquifers in compacted on-shore North American sedimentary basins. The results show that the capillary pressure, interfacial tension, relative permeability and other displacements characteristics of CO2-brine systems depend on the in-situ conditions of pressure, temperature and water salinity, and on the pore size distribution of the sedimentary rock. This paper presents a synthesis and interpretation of the results.  相似文献   

16.
We use process-based modeling techniques to characterize the temporal features of natural biologically controlled surface CO2 fluxes and the relationships between the assimilation and respiration fluxes. Based on these analyses, we develop a signal-enhancing technique that combines a novel time-window splitting scheme, a simple median filtering, and an appropriate scaling method to detect potential signals of leakage of CO2 from geologic carbon sequestration sites from within datasets of net near-surface CO2 flux measurements. The technique can be directly applied to measured data and does not require subjective gap filling or data-smoothing preprocessing. Preliminary application of the new method to flux measurements from a CO2 shallow-release experiment appears promising for detecting a leakage signal relative to background variability. The leakage index of ±2 was found to span the range of biological variability for various ecosystems as determined by observing CO2 flux data at various control sites for a number of years.  相似文献   

17.
Leroy natural-gas storage site is an anticlinal, fault-bounded, aquifer-storage system located in Wyoming, USA. Based on its abundant data, uncontrolled leakage history and subsequent control by the facility operators, a modeling framework was developed for studying reservoir behavior, examining pressure and gas-inventory histories, as well as gas and brine leakage, and evaluating the sensitivity of that behavior to uncertainty about reservoir properties. A three-dimensional model capturing the bounding fault, layered geologic stratigraphy, and surface topography was calibrated by history data of reservoir pressure and gas inventory. The calibrated model predicted gas arrival at the ground surface that was consistent with the timing of observed gas bubbling into a creek. A global sensitivity analysis was performed to examine the parameters influencing fault leakage, and a geomechanical stability analysis was conducted to investigate the likelihood of fault reactivation. In general, it is shown that a discrete leakage pathway is required to explain the observed gas leakage and its subsequent operational control by reducing reservoir pressures. Specifically, the results indicate that fault leakage is a plausible explanation for the observed gas leakage. The results are relevant to other natural-gas storage sites, as well as other subsurface storage applications of buoyant fluids, such as CO2.  相似文献   

18.
Geological sequestration of anthropogenic CO2 appears to be a promising method for reducing the amount of greenhouse gases released to the atmosphere. Geochemical modelling of the storage capacity for CO2 in saline aquifers, sandstones and/or carbonates should be based on natural analogues both in situ and in the laboratory. The main focus of this paper has been to study natural gas emissions representing extremely attractive surrogates for the study and prediction of the possible consequences of leakage from geological sequestration sites of anthropogenic CO2 (i.e., the return to surface, potentially causing localised environmental problems). These include a comparison among three different Italian case histories: (i) the Solfatara crater (Phlegraean Fields caldera, southern Italy) is an ancient Roman spa. The area is characterised by intense and diffuse hydrothermal activity, testified by hot acidic mud pools, thermal springs and a large fumarolic field. Soil gas flux measurements show that the entire area discharges between 1200 and 1500 tons of CO2 per day; (ii) the Panarea Island (Aeolian Islands, southern Italy) where a huge submarine volcanic-hydrothermal gas burst occurred in November, 2002. The submarine gas emissions chemically modified seawater causing a strong modification of the marine ecosystem. All of the collected gases are CO2-dominant (maximum value: 98.43 vol.%); (iii) the Tor Caldara area (Central Italy), located in a peripheral sector of the quiescent Alban Hills volcano, along the faults of the Ardea Basin transfer structure. The area is characterised by huge CO2 degassing both from water and soil. Although the above mentioned areas do not represent a storage scenario, these sites do provide many opportunities to study near-surface processes and to test monitoring methodologies.  相似文献   

19.
A field facility located in Bozeman, Montana provides the opportunity to test methods to detect, locate, and quantify potential CO2 leakage from geologic storage sites. From 9 July to 7 August 2008, 0.3 t CO2 day−1 were injected from a 100-m long, ~2.5-m deep horizontal well. Repeated measurements of soil CO2 fluxes on a grid characterized the spatio-temporal evolution of the surface leakage signal and quantified the surface leakage rate. Infrared CO2 concentration sensors installed in the soil at 30 cm depth at 0–10 m from the well and at 4 cm above the ground at 0 and 5 m from the well recorded surface breakthrough of CO2 leakage and migration of CO2 leakage through the soil. Temporal variations in CO2 concentrations were correlated with atmospheric and soil temperature, wind speed, atmospheric pressure, rainfall, and CO2 injection rate.  相似文献   

20.
The capture and geological storage of CO2 can be used to reduce anthropogenic greenhouse gas emissions. To assess the environmental impact of potential CO2 leakage from deep storage reservoirs on the abundance and functional diversity of microorganisms in near-surface terrestrial environments, a natural CO2 vent (>90% CO2 in the soil gas) was studied as an analogue. The microbial communities were investigated using lipid biomarkers combined with compound-specific stable carbon isotope analyses, the determination of microbial activities, and the use of quantitative polymerase chain reactions (Q-PCR). With this complementary set of methods, significant differences between the CO2-rich vent and a reference site with a normal CO2 concentration were detected. The δ13C values of the plant and microbial lipids within the CO2 vent demonstrate that substantial amounts of geothermal CO2 were incorporated into the microbial, plant, and soil carbon pools. Moreover, the numbers of Archaea and Bacteria were highest at the reference site and substantially lower at the CO2 vent. Lipid biomarker analyses, Q-PCR, and the determination of microbial activities showed the presence of CO2-utilising methanogenic Archaea, Geobacteraceae, and sulphate-reducing Bacteria (SRB) mainly at the CO2 vent, only minor quantities were found at the reference site. Stable carbon isotopic analyses revealed that the methanogenic Archaea and SRB utilised the vent-derived CO2 for assimilatory biosynthesis. Our results show a shift in the microbial community towards anaerobic and acidophilic microorganisms as a consequence of the long-term exposure of the soil environment to high CO2 concentrations.  相似文献   

设为首页 | 免责声明 | 关于勤云 | 加入收藏

Copyright©北京勤云科技发展有限公司  京ICP备09084417号