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By Z. KLIMONT J. COFALA J. XING W. WEI C. ZHANG S. WANG J. KEJUN P. BHANDARI R. MATHUR P. PUROHIT P. RAFAJ A. CHAMBERS M. AMANN J. HAO 《Tellus. Series B, Chemical and physical meteorology》2009,61(4):602-617
Estimates of Asian emissions of air pollutants and carbonaceous aerosols and their mid-term projections have been changing significantly in the last years. The remote sensing community has shown that increase in NO x in Central East Asia is much stronger than any of the emission inventories or projections indicated so far. A number of studies reviewing older estimates appeared. Here, we review the key contributions and compare them to the most recent results of the GAINS model application for Asia and to the SRES projections used in the IPPC work. The recent projections indicate that the growth of emissions of SO2 in Asia should slow down significantly towards 2010 or even stabilize at the current level. For NO x , however, further growth is projected although it will be most likely slower that in the last decade, owing to introduction of measures in transport. Emissions of carbonaceous aerosols (black carbon and organic carbon) are expected to decline after 2010, largely due to reduced use of biofuels in residential sector and efficiency improvements. The estimates of these emissions are burdened with significantly larger uncertainties than SO2 and NO x ; even for the year 2000 the differences in estimates between studies are up to a factor of 2. 相似文献
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By HEATHER D. GRAVEN † BRITTON B. STEPHENS THOMAS P. GUILDERSON TERESA L. CAMPOS DAVID S. SCHIMEL J. ELLIOTT CAMPBELL RALPH F. KEELING 《Tellus. Series B, Chemical and physical meteorology》2009,61(3):536-546
Measurements of Δ14 C in atmospheric CO2 are an effective method of separating CO2 additions from fossil fuel and biospheric sources or sinks of CO2 . We illustrate this technique with vertical profiles of CO2 and Δ14 C analysed in whole air flask samples collected above Colorado, USA in May and July 2004. Comparison of lower tropospheric composition to cleaner air at higher altitudes (>5 km) revealed considerable additions from respiration in the morning in both urban and rural locations. Afternoon concentrations were mainly governed by fossil fuel emissions and boundary layer depth, also showing net biospheric CO2 uptake in some cases. We estimate local industrial CO2 :CO emission ratios using in situ measurements of CO concentration. Ratios are found to vary by 100% and average 57 mole CO2 :1 mole CO, higher than expected from emissions inventories. Uncertainty in CO2 from different sources was ±1.1 to ±4.1 ppm for addition or uptake of −4.6 to 55.8 ppm, limited by Δ14 C measurement precision and uncertainty in background Δ14 C and CO2 levels. 相似文献
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