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1.
The impact of urbanization is assessed by comparing values of the radiation parameters at an urban location with those of a rural site. Urban Delhi was divided according to land-use and the effects of urbanization was studied on incoming short-wave (K), albedo, incoming longwave (L, outgoing longwave (L), and net radiation (Q *), were individually studied at four representative sites (Rural, Commercial, Residential and Industrial). MaximumK was observed in the rural and commercial areas whereas highL was observed in the commercial and industrial locations. High depletion ofK of the order of 13% was observed for the industrial location in the winter season. An increase ofL in, the industrial location is of the same order as that of the commercial location, i.e. 20%. The residential location shows quite moderate (4.6%) depletion ofK in comparison with other sites.Nomenclature U Urban - R Rural - K Incoming Short-wave radiation - L Incoming Long-wave radiation - L Outgoing Long-wave radiation - Q * Net Radiation - Albedo - K * Net Short-wave radiation - L * Net Long-wave radiation  相似文献   

2.

In this study we present the seasonal chemical characteristics and potential sources of PM10 at an urban location of Delhi, India during 2010?2019. The concentrations of carbonaceous aerosols [organic carbon (OC), elemental carbon (EC), water soluble organic carbon (WSOC) and water insoluble organic carbon (WIOC)] and elements (Al, Fe, Ti, Cu, Zn, Mn, Pb, Cr, F, Cl, Br, P, S, K, As, Na, Mg, Ca, B, Ni, Mo, V, Sr, Zr and Rb) in PM10 were estimated to explore their possible sources. The annual average concentration (2010–2019) of PM10 was computed as 227?±?97 µg m?3 with a range of 34?734 µg m?3. The total carbonaceous aerosols in PM10 was accounted for 22.5% of PM10 mass concentration, whereas elements contribution to PM10 was estimated to be 17% of PM10. The statistical analysis of OC vs. EC and OC vs. WSOC of PM10 reveals their common sources (biomass burning and/or fossil fuel combustion) during all the seasons. Enrichment factors (EFs) of the elements and the relationship of Al with other crustal metals (Fe, Ca, Mg and Ti) of PM10 indicates the abundance of mineral dust over Delhi. Principal component analysis (PCA) extracted the five major sources [industrial emission (IE), biomass burning?+?fossil fuel combustion (BB?+?FFC), soil dust, vehicular emissions (VE) and sodium and magnesium salts (SMS)] of PM10 in Delhi, India. Back trajectory and cluster analysis of airmass parcel indicate that the pollutants approaching to Delhi are mainly from Pakistan, IGP region, Arabian Sea and Bay of Bengal.

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3.
Owing to the importance of middle atmosphere, recently, a Middle Atmospheric Dynamics (MIDAS) program was carried out during the period 2002?C2007 at Thumba (8.5°N, 77°E). The measurements under this program, involving regular radiosonde/rocket flights as well as atmospheric radars, provided long period observations of winds and temperature in the middle atmospheric region from which waves and oscillations as well as their forcing mechanisms particularly in the low-latitude middle atmosphere could be analyzed. However, a detailed analysis of the forcing mechanisms remains incomplete due to the lack of important measurements like ozone which is a significant contributor to atmospheric dynamics. Presently, profiles of ozone are available from TIMED/SABER (Thermosphere, Ionosphere, Mesosphere Energetics and Dynamics/Sounding of the Atmosphere using Broad Emission Radiometry) satellite globally from about 15 to 100?km, over multiple years since 2002. In this regard, a comprehensive study has been carried out on ozone and its variability at Quasi Biennial Oscillation (QBO) and Semiannual Oscillation (SAO) scales using TIMED/SABER ozone observations during the MIDAS campaign period. Before using the TIMED/SABER ozone measurements, an inter-comparison has been carried out with in situ measurements of ozone obtained under the Southern Hemisphere Additional Ozonesondes (SHADOZ) campaign for the year 2007 at few stations. The inter-comparison showed very good agreement between SABER and ozonesonde derived ozone profiles. After validating the SABER observations, ozone profiles are used extensively to study the QBO and SAO along with temperature and winds in the 20?C100?km height region. It is known that the SAO in mesosphere and stratosphere are in opposite phases, but the present study for the first time reports the aspect of opposite phases in the mesosphere itself. Thus, the present work attempts to study the long-period oscillations in stratosphere and mesosphere in ozone, temperature and winds simultaneously for the first time over this latitude. These observations provided a unique opportunity to explore long-period oscillations in chemistry, dynamics and thermal structure of the middle atmosphere simultaneously.  相似文献   

4.
PM10 samples were collected to characterize the seasonal and annual trends of carbonaceous content in PM10 at an urban site of megacity Delhi, India from January 2010 to December 2017. Organic carbon (OC) and elemental carbon (EC) concentrations were quantified by thermal-optical transmission (TOT) method of PM10 samples collected at Delhi. The average concentrations of PM10, OC, EC and TCA (total carbonaceous aerosol) were 222?±?87 (range: 48.2–583.8 μg m?3), 25.6?±?14.0 (range: 4.2–82.5 μg m?3), 8.7?±?5.8 (range: 0.8–35.6 μg m?3) and 54.7?±?30.6 μg m?3 (range: 8.4–175.2 μg m?3), respectively during entire sampling period. The average secondary organic carbon (SOC) concentration ranged from 2.5–9.1 μg m?3 in PM10, accounting from 14 to 28% of total OC mass concentration of PM10. Significant seasonal variations were recorded in concentrations of PM10, OC, EC and TCA with maxima during winter and minima during monsoon seasons. In the present study, the positive linear trend between OC and EC were recorded during winter (R2?=?0.53), summer (R2?=?0.59) and monsoon (R2?=?0.78) seasons. This behaviour suggests the contribution of similar sources and common atmospheric processes in both the fractions. OC/EC weight ratio suggested that vehicular emissions, fossil fuel combustion and biomass burning could be the major sources of carbonaceous aerosols of PM10 at the megacity Delhi, India. Trajectory analysis indicates that the air mass approches to the sampling site is mainly from Indo Gangetic plain (IGP) region (Uttar Pradesh, Haryana and Punjab etc.), Thar desert, Afghanistan, Pakistan and surrounding areas.  相似文献   

5.
We have studied long-term changes in tropospheric NO2 over South India using ground-based observations, and GOME and OMI satellite data. We have found that unlike urban regions, the region between Eastern and Western Ghat mountain ranges experiences statistically significant decreasing trend. There are few ground-based observatories to verify satellite based trends for rural regions. However, using a past study and recent measurements we show a statistically significant decrease in NOX and O3 mixing ratio over a rural location (Gadanki; 13.48° N, 79.18° E) in South India. In the ground-based records of surface NOX, the concentration during 2010–11 is found to be lower by 0.9 ppbv which is nearly 60 % of the values observed during 1994–95. Small but statistically significant decrease in noon-time peak ozone concentration is also observed. Noon-time peak ozone concentration has decreased from 34?±?13 ppbv during 1993–96 to 30?±?15 ppbv during 2010–11. NOX mixing ratios are very low over Gadanki. In spite of low NOX values (0.5 to 2 ppbv during 2010–11), ozone mixing ratios are not significantly low compared to many cities with high NOX. The monthly mean ozone mixing ratio varies from 9 ppbv to 37 ppbv with high values during Spring and low values during late Summer. Using a box-model, we show that presence of VOCs is also very important in addition to NOX in determining ozone levels in rural environment and to explain its seasonal cycle.  相似文献   

6.
Measurements of total ozone column and solar UV radiation under different atmospheric conditions are needed to define variations of both UV and ozone and to study the impact of ozone depletion at the Earth’s surface. In this study, spectral and broadband measurements of UV-B irradiance were obtained along with total ozone observations and aerosol optical depth measurements in the tropical urban region of Hyderabad, south India. We specifically used an Ultra-Violet Multifilter Rotating Shadow band Radiometer (UVMFR-SR), to measure UV irradiance in time and space. To assess the aerosol and O3 effects on ground-reaching UV irradiance, we used measurements from a Microtops II sun photometer in addition to the Tropospheric Ultraviolet Visible radiation (TUV) model. We also assessed the Defense Meteorological Satellite Program – Operational Line Scanner (DMSP-OLS) night time satellite data for inferring biomass burning fires during the study period. Results clearly suggested a negative correlation between the DMSP-OLS satellite derived fire count data and UVMFR-SR data suggesting that aerosols from biomass burning are directly attenuating UV irradiance in the study region. Also, correlation analysis between UV index and ozone measurements from sun photometer and TOMS-Ozone Mapping Instrument (OMI) indicated a clear decrease in ground reaching UV-B irradiance during higher ozone conditions. The higher levels are attributed to photochemical production of O3 during the oxidation of trace gases emitted from biomass burning. Results also suggested a relatively high attenuation in UV irradiance (~6% higher) from smoke particles than dust. We also found a relatively good agreement between the modeled (TUV) and measured UV irradiance spectra for different atmospheric conditions. Our results highlight the factors affecting UV irradiance in a tropical urban environment, south India.  相似文献   

7.
This study explores the influence of air gaseous pollutants–aerosols and solar zenith angle (SZA) on the spectral diffuse-to-direct beam E /E irradiances ratio. It does so using ground-based spectroradiometric measurements taken over the Athens atmosphere during May 1995. It was found that the spectral E /E ratio decreases rapidly with increasing wavelength and regression curves of the form E /E  = aλ?b fitted the experimental data. These curves are strongly modified by aerosols–air pollutants, aerosol optical properties, and SZA. The log–log plot of E /E versus λ reveals a significant departure from linearity, which is likely to be associated with aerosol physical properties and SZA effects. The effect of atmospheric turbidity, as expressed through the aerosol optical at 500 nm and SZA on the spectral E /E ratio, is investigated in detail for two discernible atmospheric conditions observed in the urban Athens atmosphere. The first case includes different atmospheric turbidity levels under the same SZA, while the second corresponds to different SZA values under the same turbidity levels. It was found that the correlation between E /E and spectral aerosol optical depth can be a useful tool in determining the aerosol optical properties and aerosol types composition.  相似文献   

8.
To stop global warming at well below 2° C, the bulk of the world’s fossil fuel reserves will have to be left in the ground. Coal is the fossil fuel with the greatest proportion that cannot be used, and various advocacy groups are campaigning for a ban on the opening of new coal mines. Recently, both China and the USA implemented temporary moratoria on the approval of new coal mining leases. This article examines whether these coal mining bans reflect the emergence of a global norm to keep coal under the ground. To that end, we review recent coal mining policies in the four largest coal producers and explain them comparatively with a framework based on interests, ideas and institutions. We find that the norm of keeping coal in the ground remains essentially contested. Even in those countries that have introduced some form of a coal mining moratorium, the ban can easily be, or has already been, reversed. To the extent that the norm of keeping coal in the ground has momentum, it is primarily due to non-climate reasons: the Chinese moratorium was mostly an instance of industrial policy (aiming to protect Chinese coal companies and their workers from the overcapacity and low prices that are hitting the industry), while the USA’s lease restrictions were mainly motivated by concerns over fiscal justice. We do not find evidence of norm internalisation, which means that the emerging norm fails to gain much traction amid relevant national actors and other (large) coal producing states. If proponents of a moratorium succeed in framing the issue in non-climate terms, they should have a greater chance of building domestic political coalitions in favour of the norm.  相似文献   

9.
The objective of this study is to make a comparison of the prediction performance of three techniques, Functional Trees (FT), Multilayer Perceptron Neural Networks (MLP Neural Nets), and Naïve Bayes (NB) for landslide susceptibility assessment at the Uttarakhand Area (India). Firstly, a landslide inventory map with 430 landslide locations in the study area was constructed from various sources. Landslide locations were then randomly split into two parts (i) 70 % landslide locations being used for training models (ii) 30 % landslide locations being employed for validation process. Secondly, a total of eleven landslide conditioning factors including slope angle, slope aspect, elevation, curvature, lithology, soil, land cover, distance to roads, distance to lineaments, distance to rivers, and rainfall were used in the analysis to elucidate the spatial relationship between these factors and landslide occurrences. Feature selection of Linear Support Vector Machine (LSVM) algorithm was employed to assess the prediction capability of these conditioning factors on landslide models. Subsequently, the NB, MLP Neural Nets, and FT models were constructed using training dataset. Finally, success rate and predictive rate curves were employed to validate and compare the predictive capability of three used models. Overall, all the three models performed very well for landslide susceptibility assessment. Out of these models, the MLP Neural Nets and the FT models had almost the same predictive capability whereas the MLP Neural Nets (AUC = 0.850) was slightly better than the FT model (AUC = 0.849). The NB model (AUC = 0.838) had the lowest predictive capability compared to other models. Landslide susceptibility maps were final developed using these three models. These maps would be helpful to planners and engineers for the development activities and land-use planning.  相似文献   

10.
The purpose of this paper is to analyze the trends and variability in extreme temperature indices and its impact on rice–wheat productivity over two districts of Bihar, India, which is part of the middle Indo-Gangetic Basin. Mann–Kendall non-parametric test was employed for detection of trend and Sen slope was determined to quantify the magnitude of such trends. We have analyzed 10 extreme temperature indices for monthly and seasonally. The influence of extreme temperature indices on rice–wheat productivity was determined using correlation analysis. As far as Patna is concerned, if the number of cool days during September ≥10, the rice productivity will increase due to the availability of sufficient duration to fill up the grain. However, higher warm days during all the months except June will affect the productivity. A significant negative correlation was noticed between maximum value of minimum temperature during September and rice productivity. Highly significant positive correlation was noticed between number of cool days during September with rice productivity while it was highly significant negative correlation in the case of number of warm days during the same month. As far as Samastipur is concerned, a negative correlation was noticed between wheat productivity and maximum value of maximum temperature (TXx) during February, but not statistically significant. The higher temperature may affect the kernel weight and thereby yield. It is seen that a critical value of TXx ≥29.2 °C will be harmful to wheat crop during February. A significant positive correlation of number of cool nights with wheat productivity also supports the above relationship. The critical values of extreme temperature indices during rice and wheat growing months provide an indicator to assess the vulnerability of rice–wheat productivity to temperature for Patna and Samastipur districts and there is a need to prepare an adaptive strategy and also develop thermo-insensitive rice–wheat high yielding varieties suitable for this region to sustain rice–wheat productivity under projected climate change situation.  相似文献   

11.
In the present study, an attempt has been made to examine the governing photochemical processes of surface ozone (O3) formation in rural site. For this purpose, measurements of surface ozone and selected meteorological parameters have been made at Anantapur (14.62°N, 77.65°E, 331 m asl), a semi-arid zone in India from January 2002 to December 2003. The annual average diurnal variation of O3 shows maximum concentration 46 ppbv at noon and minimum 25 ppbv in the morning with 1σ standard deviation. The average seasonal variation of ozone mixing ratios are observed to be maximum (about 60 ppbv) during summer and minimum (about 22 ppbv) in the monsoon period. The monthly daytime and nighttime average surface ozone concentration shows a maximum (55 ± 7 ppbv; 37 ± 7.3 ppbv) in March and minimum (28 ± 3.4 ppbv; 22 ± 2.3 ppbv) in August during the study period. The monthly average high (low) O3 48.9 ± 7.7 ppbv (26.2 ± 3.5 ppbv) observed at noon in March (August) is due to the possible increase in precursor gas concentration by anthropogenic activity and the influence of meteorological parameters. The rate of increase of surface ozone is high (1.52 ppbv/h) in March and lower (0.40 ppbv/h) in July. The average rate of increase of O3 from midnight to midday is 1 ppbv/h. Surface temperature is highest (43–44°C) during March and April months leading to higher photochemical production. On the other hand, relative humidity, which is higher during the rainy season, shows negative correlation with temperature and ozone mixing ratio. It can be seen that among the two parameters are measured, correlation of surface ozone with wind speed is better (R 2=0.84) in compare with relative humidity (R 2=0.66).  相似文献   

12.
13.
This research article aims at characterization of the sea-breeze circulation over Thumba (8.5°N,?76.9°E,?India) in the winter season from December 2008 to February 2009, when this mesoscale circulation over the study domain was prominent. The characteristics of sea-breeze circulation cell comprising sea-breeze and compensatory return flow are investigated for clear-sky and cloudy days. The study indicated delayed onset of sea-breeze on the cloudy days as compared to the clear-sky days and the vertical thickness of sea-breeze circulation cell was found to be larger for the clear-sky days. Vertical thickness of the return flow for both clear-sky and cloudy days was larger than that of the sea-breeze flow. Simultaneous observations of upper-air meteorological parameters obtained through balloon-borne GPS sonde ascents carried out from Thumba and its adjoining coastal ocean on 29 January 2009 as part of the Winter phase of Integrated Campaign for Aerosols, gases and Radiation Budget (W-ICARB) are utilized for a case study towards investigation of diurnal evolution of the sea-breeze circulation cell. Results obtained from this study indicated systematic evolution of sea-breeze circulation over Thumba, however, it was not very clear over ocean which is attributed to cloudy conditions that prevailed on the day of measurement.  相似文献   

14.
A comprehensive study on the chemistry of deposition and the concentration of tropospheric ozone and particulate sulfate in the ocean atmosphere was carried out for the data sets in 1990’s. It is important to study the atmospheric situation over the past years as well as the latest, especially in the East Asian region where emission amount of anthropogenic air pollutants have increased year by year due to rapid economic growth. The survey was conducted for 5 years in East Asia and West Oceania (35°N–35°S, 100–135°E) in August and September in 1990’s. The purpose of the survey was to study and understand the chemistry of deposition and the concentration of tropospheric ozone and particulate sulfate in the ocean atmosphere comprehensively in one project. Rainfall over the ocean was insufficiently neutralized. Gas and aerosol over the ocean were mature, i.e., well-mixed, during the period of the transportation. The characteristic latitudinal dependence was observed in the tropospheric ozone concentration, namely, higher in the southern hemisphere and lower in the northern hemisphere (approximately 25 ppb in the 10–40°S region and 5–15 ppb in the 20–40°N region). On the other hand, high concentrations of tropospheric ozone of over 30 ppb were observed in the northern hemisphere, which was attributable to the long-range transportation. The TSP concentration was approximately under the level of 40 μg m?3 irrespectively of the latitude; in contrast, the nss-SO4 2- concentration showed a clear latitudinal dependence, i.e., higher in the northern hemisphere and lower in the southern hemisphere. The background levels of the nss-SO4 2- concentration were approximately 0.5 μg m?3 in the 10–40°S region and 2–3 μg m?3 and 4–5 μg m?3 in the 0–20°N and 20–40°N regions, respectively.  相似文献   

15.
The developmental history of peatland and dry land vegetation within the Ob-Vasugan watershed of Western Siberia was characterized according to features of the plant communities and climatic changes which were revealed by stratigraphic, spore-pollen and C14 (carbon) data obtained from a vertical peat profile Vodorasdel. Changes in the paleoecological environment over the last 10000 years were divided into five periods. The climate was characterized in the Holocene according to these periods. At the watershed studied, peatland-forming processes started about 9510 years ago resulting in 550 cm of peat accumulation. The rate of peat accumulation within the watershed decreased over time from 1.9–0.3 mm year– 1.  相似文献   

16.
We report results of preliminary high-resolution in situ atmospheric measurements through the boundary layer and lower atmosphere over the southern coast of Perú. This region of the coast is of particular interest because it lies adjacent to the northern coastal edge of the sub-tropical south-eastern Pacific, a very large area of ocean having a persistent stratus deck located just below the marine boundary layer (MBL) inversion. Typically, the boundary layer in this region during winter is topped by a quasi-permanent, well-defined, and very large temperature gradient. The data presented herein examine fine-scale details of the coastal atmosphere at a point where the edge of this MBL extends over the coastline as a result of persistent onshore flow. Atmospheric data were gathered using a recently-developed in-house constructed, GPS-controlled, micro-autonomous-vehicle aircraft (the DataHawk). Measured quantities include high-resolution profiles of temperature, wind, and turbulence structure from the surface to 1,300 m.  相似文献   

17.
This work assessed homogeneity of the Institute of Astronomy, Geophysics and Atmospheric Sciences (IAG) weather station climate series, using various statistical techniques. The record from this target station is one of the longest in Brazil, having commenced in 1933 with observations of precipitation, and temperatures and other variables later in 1936. Thus, it is one of the few stations in Brazil with enough data for long-term climate variability and climate change studies. There is, however, a possibility that its data may have been contaminated by some artifacts over time. Admittedly, there was an intervention on the observations in 1958, with the replacement of instruments, for which the size of impact has not been yet evaluated. The station transformed in the course of time from rural to urban, and this may also have influenced homogeneity of the observations and makes the station less representative for climate studies over larger spatial scales. Homogeneity of the target station was assessed applying both absolute, or single station tests, and tests relatively to regional climate, in annual scale, regarding daily precipitation, relative humidity, maximum (TMax), minimum (TMin), and wet bulb temperatures. Among these quantities, only precipitation does not exhibit any inhomogeneity. A clear signal of change of instruments in 1958 was detected in the TMax and relative humidity data, the latter certainly because of its strong dependence on temperature. This signal is not very clear in TMin, but it presents non-climatic discontinuities around 1953 and around 1970. A significant homogeneity break is found around 1990 for TMax and wet bulb temperature. The discontinuities detected after 1958 may have been caused by urbanization, as the observed warming trend in the station is considerably greater than that corresponding to regional climate.  相似文献   

18.
CORALNet-UBC was installed in April 2008 as a “proof of concept” and the first facility in a proposed cross-Canada network of similar lidars. Despite its location on the wet West Coast of Canada, data recovery ranged from a low of 45% of the total time in December, when heavy snowfall interrupted operations, to a high of 90% in July. The facility has been a spectacular success in terms of its operational characteristics (as measured by data recovery), the range of phenomena observed and the research that it has spawned. Examples are provided of the types of phenomena observed since its initial deployment. These include observations of boundary layer structure, cloud signatures, forest fire plumes and evidence of singular long-range pollutant and volcanic transport events. Observations from CORALNet-UBC complement data from other aerosol measurement initiatives in the region and provide a rich source of information that is relevant to researchers, operational forecasters and air quality managers. Future research will be directed at elucidating the processes and phenomena revealed by the instrument as well as developing new products that exploit the real-time forecasting and public advisory potential of the facility.  相似文献   

19.
F. Giorgi  X. Bi  J. S. Pal 《Climate Dynamics》2004,22(6-7):733-756
We present an analysis of a multidecadal simulation of present-day climate (1961–1990) over Europe with the regional climate model RegCM nested within the global atmospheric model HadAMH. Climatic means, interannual variability and trends are examined, with focus on surface air temperature and precipitation. The RegCM driven by HadAMH fields is able to reproduce the basic features of the observed mean surface climate over Europe, its seasonal evolution and the regional detail due to topographic forcing. Surface air temperature biases are mostly less than 1–2 °C and precipitation biases mostly within 10–20%. The RegCM has more intense vertical transport of temperature and water vapor than HadAMH, which results in lower surface air temperatures and greater precipitation than found in the HadAMH simulation. In some cases this is in the direction of greater agreement with observations, while in others it is in the opposite direction. The simulation shows a tendency to overestimate interannual variability of temperature and precipitation compared to observations, particularly during summer and over the Mediterranean regions. It is shown that in DJF, MAM and SON the RegCM interannual variability is primarily determined by the boundary forcing from HadAMH, while in JJA the internal model physics and resolution effects dominate over many subregions of the domain, and the RegCM has higher interannual variability than HadAMH. The precipitation trends simulated by the nested modeling system for the period 1961–1990 capture some features of the observed trends, in particular the cold season drying over the Mediterranean regions. Ensembles of simulations are, however, needed for a more robust assessment of the models capability to simulate climatic trends. Overall, this simulation is of good quality compared with previous nested RegCM experiments and will constitute the basis for the generation of climate change scenarios over the European region to be reported in future work.  相似文献   

20.
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