北京地面紫外辐射（光谱）的观测与分析

通过对北京大气物理研究所与长春光机所合作研制的地基太阳紫外辐射光谱仪观测资料的分析，和用辐射传输模式UVSS计算的结果，对影响到达地面的UVB辐照度的主要因子太阳高度角（SZA）、臭氧总量和地表反照率进行了分析研究。最后对紫外光谱仪的观测资料做了总量和谱分析。     

紫外辐射传输模式计算与实际测量的比较

利用改进的离散坐标法紫外辐射传输模式,应用各种可测得的实际大气物理参数,模拟了1993年7月24日德国加尔米希-帕特科琛（Garmisch-Partenkirchen,47.47oN, 11.07oE）地面紫外辐射的全天分布,并与1993年秋天第三次欧洲紫外辐射光谱仪比对活动期间通过了严格绝对标定的奥地利英斯布鲁克（Innsbruck）大学的紫外光谱仪的实际观测资料进行了比较,进行了余弦响应订正后,计算与测量的绝对值差别很小,最大误差对地面UVB通量（280～320 nm）是0.07 W/m2（正午的通量为3.2 W/m2）。对UVA（320～400 nm）最大误差是2.6 W/m2（正午通量为54 W/m2）。计算与测量的平均偏差为5%～13%,这表明,地面紫外辐射水平也可以利用其他大气观测资料通过模式计算间接得到。     

紫外辐射如何影响人类

太阳辐射能量的波长范围较宽，对人类而言，其中大部分的太阳辐射是肉眼无法看得见的。波长越短，辐射强度越大，并且对于生物体潜在的危害也就越大。到达地球表面的紫外辐射，其波长在290～400nm(十亿分之一米)，这比可见光的波     

平流层臭氧变化对大气加热率及到达地面紫外辐射的影响

平流层臭氧的变化对平流层的温度结构，整个大气环流以及到达地面的紫外辐射均有影响。本文采用一个计算臭氧吸收太阳辐射的参数化方法和有关资料，研究了臭氧变化对大气最大加热率和到达地面的紫外辐射通量密度的影响情况。文中给出的参数化方法可直接应用于大气环流模式计算臭氧吸收太阳辐射的加热率。     

太阳辐射各因子的变化对太阳紫外辐射的影响

利用北京地区１９９０年太阳分光辐射的观测资料，计算了影响太阳紫外辐射的各因子的变化所引起的太阳紫外辐射的变化。当臭氧、水汽、气溶胶分别减少５％时，到达地面的太阳紫外辐射将分别增加０．８４％、０．２７％和１．９０％。在分析太阳紫外辐射的变化趋势时，应当全面考虑各个因子的影响。     

民勤地区紫外辐射的观测与模拟研究

利用2010年春季民勤加强观测实验的地面辐射资料,分析了民勤沙漠干旱区总紫外辐射的变化特征,并对该地区的紫外辐射进行了估算和模拟。结果表明,紫外辐射和太阳总辐射表现出一致的变化特征,层云对两者的反射能力比卷云强。2010年6月紫外辐射的瞬时最大值为55.92 W·m-2,平均日总量为1.07 MJ·m-2,紫外辐射与太阳辐射比例的平均值为4.7%,其变化范围在3%~9%之间。根据晴空指数(Kt)与最大紫外辐射(UV0)及太阳总辐射(G)建立了民勤地区紫外辐射(UV)的估算方程:UV=2.94+1.22×(Kt×UV0)和UV=0.047G,均能较好地估计该地区的地表紫外辐射。由于受输入参数精度的限制,辐射传输模式SBDART低估了晴空条件下的紫外辐射,低估的总平均值为1.12 W·m-2(约5.6%),变化范围在-2.8~0.2 W·m-2之间。     

亚音速飞机排放物对地面紫外辐射的影响

根据世界民航组织和世界气象组织有关专家对当前亚音速飞机排放量的估计和将来20年内增长的预测,用辐射传输模式估算了飞机排放物对地面紫外辐射水平的影响。计算使用DISORT程序,这是一个经过检验可以较好地包括多次散射作用的离散坐标法程序。分别检验了飞机排放煤烟、硫酸盐粒子和卷云的多次散射及引起的臭氧增加对地面280～400 nm紫外辐射的影响。结果表明：根据目前的估计和预测,飞机排放的煤烟和硫酸盐粒子对地面紫外辐射没有影响;引起的臭氧变化也不至于引起地面紫外辐射的变化。但如果天空存在一层卷云（光学厚度0.042）,就足以使得地面直射紫外辐射减少5%,总紫外辐射增加1%～2%。有资料表明,飞机排放的水汽可能使得某些地区卷云量增加了10%。因此,可能会对地面紫外辐射产生影响。     

北京地区太阳紫外辐射的观测与分析研究

利用北京地区太阳辐射和其它常规气象观测资料，得到了到达地面的太阳紫外辐射的计算公式，并将计算值与观测值进行了比较，两者吻合得比较好。最后给出了北京地区地面太阳紫外总辐射的变化趋势，计算结果表明，地面太阳紫外总辐射对大气浑浊度的变化比对大气臭氧总量的变化敏感得多。     

上海地区地面太阳紫外辐射的观测和分析

通过对上海地区2001～2003年地面太阳总辐射和紫外辐射观测资料的分析表明：（1）上海地区太阳辐射和紫外辐射年总量分别为4487．1MJ／m^2和149．6MJ/m^2。（2）紫外辐射的季节变化特征十分明显,夏半年（4-9月）各月极大紫外辐射强度远大于冬半年（10月～次年3月）,7月份最强,12月份最弱。（3）不同天气条件下,紫外辐射日变化显示出明显的差异,晴天强且稳定,多云天气波动较大,阴天则次之。（4）紫外辐射占总辐射的比例（η）也显示冬半年低,夏半年高的分布特征。（5）影响上海地区到达地面紫外辐射的主要因子有：太阳高度角的大小大致决定了到达地面紫外辐射的强弱,两者具有相近的年变化趋势;云、雨等天气类型是影响紫外辐射的重要因子;大气能见度对紫外辐射也有比较明显的影响。     

A Possible Photochemical Link Between Stratospheric and Near-Surface Ozone on Swiss Mountain Sites in Late Winter

Record high near-surface ozone concentrations at two elevated sites (Chaumont, 1140 m asl, and Rigi, 1030 m asl) in Switzerland were observed simultaneously with extremely low total ozone during a fair weather period in mid-February 1993. An analysis of ozone, temperature, humidity, and wind profiles suggests that the surface ozone peaks were most possibly generated within the region in a layer between about 1000 and 1500 m asl. Mean diurnal cycles of ozone concentration during the period shows a strong increase from late morning to late afternoon at Chaumont and at the same time a decrease at the high alpine site Jungfraujoch (3580 m asl). The different diurnal ozone cycles can both be explained photochemically by taking into account the large difference in NOx concentrations (about two orders of magnitude) between the sites. Photochemical processes are also indicated by the diurnal cycles of NO2 and NO concentration. As a strong photochemical activity is not expected in mid-February at 47°N, we hypothesize that the extremely low total ozone played a role. Total ozone controls the amount of UV-B radiation reaching the troposphere and thus influences photochemical processes. Using a radiation model, we calculated an increase in ozone photolysis at Chaumont and Jungfraujoch of 73% and 83%, respectively, on the day with the lowest total ozone (243 DU) compared to average February conditions (335 DU). It is suggested that total ozone changes have the potential to stimulate photochemistry sufficiently to produce the observed surface ozone peaks at Chaumont and Rigi of 61 and 64 ppbv, respectively. A fog layer just below Chaumont during these days probably also influenced photochemistry, but on a smaller spatial scale. Our empirical results on the influence of changing UV radiation on tropospheric photochemistry are in close agreement with model studies of other groups. Although this case study represents unique conditions, a distinct anticorrelation between near-surface ozone at Chaumont and total ozone also appears in other years (1992–1997) when selecting fair weather days in mid-February. However, other influences cannot be excluded. The selected days provide evidence of a significant photochemical source of ozone in the mid-latitude lower troposphere in late winter.     

辐射传输模式中地表参数对大气长波辐射的影响

本文利用Liou-Ou一维宽带辐射传输模式，对地表热力参数取值部分作了改进，使用模式大气和青藏高原实测资料对下垫面温度与地表空气温度两者不能合二为一的问题进行了分析，同时还讨论了下垫面温度的日变化对大气长波辐射通量日变化的影响及地表比辐射率的变化对大气长波辐射通量计算结果的修正作用。     

由GMS卫星资料获取我国夏季地表辐射收支

地表辐射收支是一个重要的基本辐射参数，本文导得卫星可见光和红外波段测值与地表辐射收支的基本关系，据此利用GMS静止气象卫星可见光和红外通道数值化资料和地面辐射收支观测资料，建立了几个由卫星资料估计地面辐射收支的模式，选择效果最佳的一种模式，通过内插方法求取全国辐射收支分布，回归效果与实测结果比较表明，方法有实际应用价值。     

一个三维Monte-Carlo地气耦合辐射传输模式

建立了一个可靠和较高计算效率的三维Monte-Carlo地气耦合辐射传输模式(3DMC).该模式在光子释放和定位、地气耦合、辐射率高分辨模拟计算和计算效率等方面有所发展.     

陆面过程模式中植被冠层短波辐射传输参数化方案研究进展

阐述植被冠层内短波辐射传输模式研究在陆面过程及陆气相互研究中的重要性,全面地回顾有关冠层短波辐射传输模式的研究进展,结合目前在陆面过程领域具有代表性的冠层短波辐射传输模式,指出当前在这一领域研究中存在并有待于解决的问题,探讨了未来的发展趋势.     

Characteristics of Surface Solar Radiation under Different Air Pollution Conditions over Nanjing,China: Observation and Simulation

Surface solar radiation (SSR) can affect climate, the hydrological cycle, plant photosynthesis, and solar power. The values of solar radiation at the surface reflect the influence of human activity on radiative climate and environmental effects, so it is a key parameter in the evaluation of climate change and air pollution due to anthropogenic disturbances. This study presents the characteristics of the SSR variation in Nanjing, China, from March 2016 to June 2017, using a combined set of pyranometer and pyrheliometer observations. The SSR seasonal variation and statistical properties are investigated and characterized under different air pollution levels and visibilities. We discuss seasonal variations in visibility, air quality index (AQI), particulate matter (PM₁₀ and PM_2.5), and their correlations with SSR. The scattering of solar radiation by particulate matter varies significantly with particle size. Compared with the particulate matter with aerodynamic diameter between 2.5 μm and 10 μm (PM_2.5?10), we found that the PM_2.5 dominates the variation of scattered radiation due to the differences of single-scattering albedo and phase function. Because of the correlation between PM_2.5 and SSR, it is an effective and direct method to estimate PM_2.5 by the value of SSR, or vice versa to obtain the SSR by the value of PM_2.5. Under clear-sky conditions (clearness index ≥0.5), the visibility is negatively correlated with the diffuse fraction, AQI, PM₁₀, and PM_2.5, and their correlation coefficients are ?0.50, ?0.60, ?0.76, and ?0.92, respectively. The results indicate the linkage between scattered radiation and air quality through the value of visibility.     

地面臭氧的变化规律和计算方法的初步研究Ⅰ.紫外波段

通过对广州鼎湖山近地面O3、NOx、太阳辐射、气象参数等项目的观测和理论分析,研究了地面O3与NOx等微量气体及太阳辐射的变化规律,详细讨论了紫外波段、不同天气条件地面O3与NOx,光化学反应、气溶胶、光化辐射等之间复杂的关系.用光能量传输与守恒的观点来考虑大气中与紫外辐射有关的主要过程,并以此来研究大气光化学过程中所遵循的能量规律,建立了一个简单、实用、省时的统计模式,用于计算地面O3浓度.结果表明,不同情况下计算值与观测值均吻合较好.     

大气辐射计算的吸收系数分布模式

全面论述了大气辐射计算中的吸收系数分布（#FKk#FS分布）模式,包括均匀路径的#FKk#FS分布模式以及非均匀路径的相关#FKk#FS分布模式。重点是利用吸收系数重排计算大气吸收气体分布函数和相关#FKk#FS分布函数的方法。某些结果系作者第一次公开发表。     

Four-stream Radiative Transfer Parameterization Scheme in a Land Surface Process Model

Accurate estimates of albedos are required in climate modeling. Accurate and simple schemes for radiative transfer within canopy are required for these estimates, but severe limitations exist. This paper developed a four-stream solar radiative transfer model and coupled it with a land surface process model. The radiative model uses a four-stream approximation method as in the atmosphere to obtain analytic solutions of the basic equation of canopy radiative transfer. As an analytical model, the four-stream radiative transfer model can be easily applied efficiently to improve the parameterization of land surface radiation in climate models. Our four-stream solar radiative transfer model is based on a two-stream short wave radiative transfer model. It can simulate short wave solar radiative transfer within canopy according to the relevant theory in the atmosphere. Each parameter of the basic radiative transfer equation of canopy has special geometry and optical characters of leaves or canopy. The upward or downward radiative fluxes are related to the diffuse phase function, the G-function, leaf reflectivity and transmission, leaf area index, and the solar angle of the incident beam. The four-stream simulation is compared with that of the two-stream model. The four-stream model is proved successful through its consistent modeling of canopy albedo at any solar incident angle. In order to compare and find differences between the results predicted by the four- and two-stream models, a number of numerical experiments are performed through examining the effects of different leaf area indices, leaf angle distributions, optical properties of leaves, and ground surface conditions on the canopy albedo. Parallel experiments show that the canopy albedos predicted by the two models differ significantly when the leaf angle distribution is spherical and vertical. The results also show that the difference is particularly great for different incident solar beams. One additional experiment is carried out to evaluate the simulations of the BATS land surface model coupled with the two- and four-stream radiative transfer models. Station observations in 1998 are used for comparison. The results indicate that the simulation of BATS coupled with the four-stream model is the best because the surface absorbed solar radiation from the four-stream model is the closest to the observation.