Spectra of surface wind speed and air temperature over the ocean in the mesoscale frequency range in JASIN-1978

Based on the data from an array of buoys during the JASIN-1978 field experiment made in an area northwest of Scotland, power spectra of surface wind speed and air temperature over the ocean in the mesoscale frequency range were studied. The averaged composite spectrum of wind speed for the whole period shows the existence of a spectral gap in the frequency range from 10^–4 to 5 × 10^–3 Hz. However, significant peaks in this range are often seen in particular spectra under certain weather conditions. Mesoscale spectral peaks of wind speed occur in 14 segments of the data record, approximately 10% of the total duration of the observations. In 4 of these segments, the mesoscale spectral peaks of both wind speed and air temperature occurred simultaneously. Several wave patterns of mesoscale atmospheric disturbances when mesoscale spectral peaks were seen are derived from phase differences between buoys. Significant mesoscale peaks in spectra appear in relatively strong winds and unstable or near-neutral atmospheric conditions, and none in stable atmospheric conditions. A criterion of wind speed and atmospheric stability is found for the mesoscale spectral peak appearance.     

Temperature stratification of the atmospheric boundary layer over the Deccan Plateau,India, during the summer monsoon

The vertical and horizontal temperature structure of the atmospheric boundary layer (ABL) were studied using aircraft observations made in the lowest 2.4 km above ground level during the summer monsoon.The vertical temperature structure of the ABL in the region may be classified into the following four categories.Category The ABL consisted of two layers of thickness 700–900 m separated by a thin transition layer. The lapse rates in the former two layers were dry adiabatic.Category The lowest layer of the ABL of thickness 400–600 m was adiabatically stratified and the overlying layer was stable with gradients of potential temperature 4–5°C km^–1. The stable layer contained a thin adiabatic stratified layer of 200–300 m thickness at a height of 1.5 km.Category The lowest 200–400 m layer of the ABL was adiabatically stratified and the overlying layer was stable with potential temperature gradients of 5–6 °C km¹.Category The ABL was mainly stable with potential temperature gradients of 6 °C km^–1 or greater. Occasionally thin layers with adiabatic stratification were found embedded in the ABL.The temperature distribution of the horizontal temperature at 900 m was mainly normal. The high-frequency portion of the spectra lying between 0.05 and 0.16 Hz (corresponding to wave length 1 km to 300 m) oscillated around the –\2/3 power law line. The spectral curve showed a significant peak at 0.011 Hz having a wave-length of 5 km.Department of Geoscience, North Carolina State University, Raleigh, NC, 27650, U.S.A.     

Small-scale atmospheric structure deduced from measurements of temperature,humidity and refractive index

Measurements have been made with fast-response multi-channel temperature, humidity and refractive index sensors flown to 2000 m on a tethered balloon to investigate small-scale fluctuations important in radio-wave scattering, their relation to atmospheric parameters, and their spatial variation in both one and three dimensions. Data from the three types of sensors at one point were consistent for frequencies up to about 8 Hz. Power spectra of data at various heights were computed over 0.1 to 10 Hz and generally showed slopes (on a log-log plot) close to - 5/3 above 1 Hz but ranged from –1.5 to – 3.5 at lower frequencies; in this range (f < 1 Hz) slopes were close to – 5/3 for negative Richardson number (Ri), provided temperature gradients were steeper than –1.1 °C 100 m^–1 and wind shears > 1.4 x 10^–2 s^–1 approx. Steeper slopes were generally associated with stable atmospheric conditions but no precise relation to the above parameters was found. Spectral density was a maximum for Ri –0.75.Cross-correlations of 0.5 were frequently observed between sensors 1 m apart in orthogonal directions; in the vertical, examples of negative correlation of vapour pressure were occasionally found over this spacing. Using four sensors spaced in line over 9 m, cross-spectrum phase calculations of drift speeds were found to be consistent with measured wind speeds. The ratio of identification distance (coherence=0.6) to scale size of irregularities ranged from 0.25 to 0.5 with no apparent relation to height or meteorological parameters.     

Seasonal variations of spectra of wind speed and air temperature in the mesoscale frequency range

Seasonal variations of the spectra of wind speed and air temperature in the mesoscale frequency range from 1.3 × 10^-4 to 1.5 × 10^-3 Hz (10 min to 2 h periods) have been studied through observations over land for one year. Spectrographs [time series of isopleths of spectral densities, f · S(f) vs f] of wind speed and air temperature contain occasional peaks that are attributed to short-lived mesoscale atmospheric activity with narrow frequency bands. Significant spectral peaks of wind speed were found in 19% of the total observations in winter, and in 15–16% in the other seasons; for air temperature, they occured in 12% of observations in autumn, and in 16–19% in the other seasons. The peaks most often occurred in the period range from 30 min to 1 h; most had durations less than 24 h. Mesoscale fluctuations of wind speed and air temperature were highly correlated, and in most cases, phase differences were 90–180 ° with air temperature leading wind speed. Significant spectral peaks of wind speed often occurred during northerly seasonal cold winds in winter, and accompanied tropical and/or mid-latitude cyclones in the other seasons. When the peaks occurred, wind speed was usually relatively high and the atmospheric surface layer was unstable.     

Thermal plumes and turbulence spectra in the atmospheric boundary layer

Experimental observations on the temperature and wind fields above flat grassy terrain have been obtained with an instrumented 92-m tower during intervals of strong insolation about midday. The turbulence characteristics of the air confirm that free convection prevailed at heights between 16 and 48 m, with some tendency for departure at higher levels. The spectra of temperature and vertical velocity contain gaps at wave numbers in the range 0.01–0.025 m^–1. These are attributed to natural thermal plumes that act as sources of extra energy input to the Kolmogorov-Obukhov-Corrsin scheme of turbulence in or at the low-wave number limit of the inertial subrange. Modified forms of the K-O-C spectral laws for thermally unstable air are derived which agree with the observed spectra over the whole range of wave numbers examined, and which contain the spectral gap at wave numbers corresponding to the thermal plume diameters.     

Methane emissions from a landfill measured by eddy correlation using a fast response diode laser sensor

We describe a fast response methane sensor based on the absorption of radiation generated with a near-infrared InGaAsP diode laser. The sensor uses an open path absorption region 0.5 m long; multiple pass optics provide an optical path of 50 m. High frequency wavelength modulation methods give stable signals with detection sensitivity (S/N=1, 1 Hz bandwidth) for methane of 65 ppb at atmospheric pressure and room temperature. Improvements in the optical stability are expected to lower the current detection limit. We used the new sensor to measure, by eddy correlation, the CH₄ flux from a clay-capped sanitary landfill. Simultaneously we measured the flux of CO₂ and H₂O. From seven half-hourly periods of data collected after a rainstorm on November 23, 1991, the average flux of CH₄ was 17 mmol m^–2 hr^–1 (6400 mg CH₄ m^–2 d^–1) with a coefficient of variation of 25%. This measurement may underrepresent the flux by 15% due to roll-off of the sensor response at high frequency. The landfill was also a source of CO₂ with an average flux of 8.1 mmol m^–2 hr^–1 (8550 mg CO₂ m^–2 d^–1) and a coefficient of variation of 26%. A spectral analysis of the data collected from the CH₄, CO₂, and H₂O sensors showed a strong similarity in the turbulent transfer mechanisms.     

Vertical profiles of small-scale temperature structure in the atmosphere

Measurements of air temperature fluctuations at frequencies from 1–100 Hz have been made with instruments carried by free-flying balloons. Structure functions and spectra of the temperature field have been calculated for various heights within the range 0.1–8 km above ground. The frequent occurrence of shallow regions, possibly layers, which exhibit locally enhanced values of the structure coefficient has been confirmed.     

Observations of the convective plume of a lake under cold-air advective conditions

Moderating effects of Lake Apopka, Florida on downwind surface temperatures were evaluated under cold-air advective conditions. Point temperature measurements north and south of the lake and data obtained from a thermal scanner flown at 1.6 km indicate that surface temperatures directly downwind may be higher than surrounding surface temperatures by as much as 5 °C under conditions of moderate winds (~4 m s^–1). No substantial temperature effects were observed with surface wind speed less than 1 m s^–1. Fluxes of sensible and latent heat from Lake Apopka were calculated from measurements of lake temperature, net radiation, relative humidity and air temperature above the lake. Bulk transfer coefficients and the Bowen ratio were calculated and found to be in agreement with reported data for non-advective conditions.IFAS Journal Series No. 1006.     

Seasonal variation of particulate polycyclic aromatic hydrocarbons associated with PM10 in Guangzhou, China

Polycyclic aromatic hydrocarbons (PAHs) are ubiquitous pollutants in the urban atmosphere. An investigation on seasonal variation of PAHs in the urban atmosphere of Guangzhou, China was conducted in this study. 112 PM10 (particulate matter with aerodynamic diameter < 10 μm) samples were collected at two sites between June 2002 and June 2003. PAHs were analyzed with GC–MS (gas chromatography–mass spectrometry). The result showed that PAHs exhibit distinct seasonal variation. The seasonal concentration for the ∑PAHs ranged from 8.11 to 106.26 ng m^− 3. The average ∑PAHs measured were highest in winter and lowest in summer. The PAHs distribution patterns were similar within each season at two sites. 5–6 ring PAHs were the abundant compounds, which accounted for 65–90% of ∑PAHs and benzo [b + k] fluoranthene dominated in four seasons. The PAHs concentration and distribution pattern fluctuated greatly in winter for the cold air current. Based on the different temperature in winter, the samples were split into two groups. PM10 and the abundance of the PAHs in winter-1 (temperature, 12–22 °C) were much greater than in winter-2 (temperature, 8–12 °C). In winter-1 benzo [b + k] fluoranthene and Indeno [1, 2, 3] pyrene dominated while chrysene and benzo [b + k] fluoranthene dominated in winter-2. Meteorological conditions such as wind speed and temperature had a strong influence on the seasonal variation. Potential sources of PAHs were identified using the molecular diagnostic ratios between PAHs. Results showed fossil fuel combustion may be the major source of PAHs at the two sites.     

A fast response,open path,infrared hygrometer,using a semiconductor source

Investigations were carried out as to the feasibility of using a semiconductor source in the design of a new rapid response, open-path hygrometer. A single-beam instrument was constructed employing an infrared light emitting diode (LED) as a source instead of the usual high energy, wideband filament. The spectral emission envelope encompassed the 1.87 m water absorption band. Electronic modulation and thermoelectrical cooling of the diode eliminated the conventional chopper wheel and stabilized the peak wavelength emission. Path length was 200 mm. Over a water vapour concentration range of 0–16 g m^–3, absorption varied by 2% in a linear fashion. At 10 Hz, the noise level was 0.1 g m^–3 rms. Hygrometer resolution and stability are constrained by the detector noise level, the small source emission in the absorption band and low frequency drift in the optical filter. Despite these problems, the new instrument showed comparable performance characteristics to a commercial Lyman- hygrometer. Latent heat fluxes measured with both instruments and a Kaijo-Denki, 3-D sonic anemometer agreed to within 4% over a range 0–350 W m^–2. Further improvements in performance can be anticipated with advances in detector and LED technology.     

Long-Term Ground Heat Flux and Heat Storage at a Mid-Latitude Site

We analyzed a long-term (37 year) record of monthly average below-ground temperatures, at depths ranging from the surface down to 12.8 m,to determine the ground heat flux. Temperatures at all depths have increased over the period, evidence of a non-zero mean ground heat flux. Analysis indicates an average downward flux out of the root zone (below 1.6m) over the period of approximately 1.1 MJ m^–2year^–1. The corresponding average flux through the bottomplane of measurement has been approximately 0.22 MJ m^–2year^–1, indicating that 20% of the heat storage duringthe period has been at depths greater than 12.8 m. Current representations of ground heat flux in global climate models are inadequate to realistically simulate these results. This warming, if it continues, could affect a range of biotic and abiotic below-ground processes.     

Turbulence Characteristics of the Stable Boundary Layer Over a Mid-Latitude Glacier. Part I: A Combination of Katabatic and Large-Scale Forcing

Profile and eddy-correlation (heights of 4 and 10 m) measurements performed on the Pasterze glacier (Austria) are used to study the characteristics of the stable boundary layer under conditions of katabatic and large-scale forcing. We consider cases where large-scale forcing results in a downslope (or following) ambient wind. The analysis of averaged spectra and cospectra reveals low frequency perturbations that have a large influence on the variances of temperature and horizontal wind components and also alter the cospectra of momentum and sensible heat flux. Only the spectrum of the vertical wind speed is comparable to universal spectra. The low frequency perturbations occur as brief intermittent events and result in downward entrainment of ambient air thereby producing enhanced downward sensible heat fluxes and downward as well as upward momentum fluxes with various magnitudes and timescales. After the variances were high pass filtered, the normalised standard deviations of wind speed and temperature compare favourably to findings in the literature within the range 0>z/L>0.5. For larger z/L they deviate as a result of an increased influence from low frequency perturbations and thus non-stationarity. In line with this, the turbulent kinetic energy budget (at 4 m height) indicates that production (shear) is in balance with destruction (buoyancy and dissipation) within the range 0>z/L>0.3. Non-dimensional gradients of wind speed within the range 0>z/L>0.3 have a slope of about 3.5. The scatter for the dimensionless temperature gradient is quite large, and the slope is comparable to that for wind speed gradients. For z/L>0.3 the imbalance in the turbulent kinetic energy budget grows and non-dimensional gradients for wind speed and temperature deviate considerably from accepted values as a result of increased non-stationarity. Average roughness lengths for momentum and sensible heat flux derived from wind speed and temperature profiles are respectively 1 × 10^-3 m and 6 × 10^-5 m, consistent with the literature. The ratio (z_0h/z_0m) compares to those predicted by surface renewal models. A variation of this ratio with the roughness Reynolds number is not indicated by our data.     

Coastal CCN measurements at Mace Head with enhanced concentrations in strong winds

Surface measurements of cloud condensation nuclei (CCN) number concentration (cm⁻³) are presented for unmodified marine air and for polluted air at Mace Head, for the years 1994 and 1995. The CCN number concentration active at 0.5% supersaturation is found to be approximately log-normal for marine and polluted air at the site. Values of geometric mean, median and arithmetic mean of CCN number concentration (cm⁻³) for marine air are in the range 124–135, 140–150 and 130–157 for the two years of data. Analysis of CCN number concentration for high wind speed, U, up to 20 m s⁻¹ show enhanced CCN production for U in excess of about 10–12 m s⁻¹. Approximately 7% increase in CCN per 1 m s⁻¹ increase in wind speed is found, up to 17 m s⁻¹. A relationship of the form log₁₀CCN=a+bU is obtained for the periods March 1994 and January, February 1995 for marine air yielding values a of 1.70; 1.90 and b of 0.035 for both periods.     

Simulation of Global Hydrogen Levels Using a Lagrangian Three-Dimensional Model

Many previous assessments of the global hydrogen budget have used assumed global averages of temperatures and levels of key reactants to calculate the magnitudes of the various sinks. Dry deposition is by far the largest hydrogen sink but has not been considered in detail in previous estimates of the hydrogen budget. Simulations of hydrogen using a global three-dimensional Lagrangian chemistry-transport model and two different dry deposition schemes were compared with surface measurements. An improved dry deposition scheme which included the effects of soil moisture gave better agreement between the modelled hydrogen levels and surface measurements. The seasonal variation in the hydrogen levels was also simulated much more accurately with the new dry deposition scheme. The model results at high southern latitudes were insensitive to the relative partitioning of the sources between fossil fuel combustion and biomass burning. The results indicate a global mean hydrogen dry deposition velocity of 5.3×10^–4 m s^–1 which is lower than the previously used 7×10^–4 m s^–1.     

Surface-layer scintillation measurements of daytime sensible heat and momentum fluxes

Line-averaged measurements of the structure parameter of refractive index (C _n ² ) were made using a semiconductor laser diode scintillometer above two markedly different surfaces during hours of positive net radiation. The underlying vegetation comprised in the first instance a horizontally homogeneous, pasture sward well-supplied with water, and in the second experiment, a sparse thyme canopy in a semi-arid environment. Atmospheric stability ranged between near neutral and strongly unstable (–20). The temperature structure parameterC _T ² computed from the optical measurements over four decades from 0.001 to 2 K² m^–2/3 agreed to within 5% of those determined from temperature spectra in the inertial sub-range of frequencies. Spectra were obtained from a single fine thermocouple sensor positioned near the midway position of the 100m optical path and at the beam propagation height (1.5m).With the inclusion of cup anemometer measurements, rule-of-thumb assumptions about surface roughness, and Monin-Obukhov similarity theory, path-averaged optical scintillations allow calculation of surface fluxes of sensible heat and momentum via a simple iterative procedure. Excellent agreement was obtained between these fluxes and those measured directly by eddy correlation. For sensible heat, agreement was on average close to perfect over a measured range of 0 to 500 W m^–2 with a residual standard deviation of 30 W m^–2. Friction velocities agreed within 2% over the range 0–0.9 m s^–1 (residual standard deviation of 0.06 m s^–1). The results markedly increase the range of validation obtained in previous field experiments. The potential of this scintillation technique and its theoretical foundation are briefly discussed.     

Fluxes of gases and particles above a deciduous forest in wintertime

Eddy-correlation measurements of the vertical fluxes of ozone, carbon dioxide, fine particles with diameter near 0.1 m, and particulate sulfur, as well as of momentum, heat and water vapor, have been taken above a tall leafless deciduous forest in wintertime. During the experimental period of one week, ozone deposition velocities varied from about 0.1 cm s^–1 at night to more than 0.4 cm s^-1 during the daytime, with the largest variations associated primarily with changes in solar irradiation. Most of the ozone removal took place in the upper canopy. Carbon dioxide fluxes were directed upward due to respiration and exhibited a strong dependence on air temperature and solar heating. The fluxes were approximately zero at air temperatures less than 5 °C and approached 0.8 mg m^–2 s^–1 when temperatures exceeded 15 °C during the daytime. Fine-particle deposition rates were large at times, with deposition velocities near 0.8 cm s^–1 when turbulence levels were high, but fluxes directed upward were found above the canopy when the surface beneath was covered with snow. Diffusional processes seemed to dominate fine-particle transfer across quasilaminar layers and subsequent deposition to the upper canopy. Deposition velocities for particulate sulfur were highly variable and averaged to a value small in magnitude as compared to similar measurements taken previously over a pine forest in summer.     

Changes in scavenging of particles by droplets due to weak electrification in clouds

Electrical charges on aerosol particles and droplets modify the droplet–particle collision efficiencies involved in scavenging, and the droplet–droplet and particle–particle collision efficiencies involved in coalescence of droplets and particles, even in only weakly electrified clouds and aerosol layers. This work places electrically enhanced scavenging, and the electrical inhibition of scavenging in the context of the microphysics of weakly electrified clouds.Collision efficiencies are calculated by numerical integration to obtain particle trajectories, that are determined by the complex interplay of electrical, gravitational and phoretic forces together with inertia. These modify the trajectory of a particle as it is carried by flow around the falling droplet. Conversely, the flow around the particle also modifies the trajectory of the droplet. The flows are specified analytically, using a hybrid of the Proudman–Pearson stream function for that region close to the droplet or particle, where it is accurate, merging into the exact Oseen stream function for larger distances, where that becomes accurate. The effect of the flow around the particle on the motion of the droplet was simulated using Langmuir's superposition technique on the hybrid stream functions. The treatment of inertia in the present calculations allows an extension of the scope of our previous work by a factor of 10 larger in particle size (10³ in mass). The coverage is extended to a wide range of atmospheric conditions and particle densities.The pressures and temperatures used in the models ranged from a representation of the lower troposphere at  1 km altitude (900 hPa, 10 °C) to that of the middle stratosphere at  30 km altitude (12 hPa, − 47 °C). The particles considered range from 0.1 μm to 10 μm radius; the droplet radii range from 4 μm to 50 μm; particle densities range from 300 kg m^− 3 to 2500 kg m^− 3; particle charges range from 2e to 100e with droplet charges of like sign of 100e; and relative humidities range from 10% to 100%.For the larger particles (radii greater than about 3 μm) interacting with the larger droplets (radii greater than about 15 μm) the effects of inertia increase with particle density and dominate at the larger densities. For particles with radii in the range 1–3 μm the ‘Greenfield Gap’ of very low collision efficiencies was found, and was determined to be due to the effects of the gravitational force causing a reduction of collisions of particles with the front of the droplet, and the effect of inertia overcoming the tendency for the weight to produce a collision in the slow velocity region in the rear. When the electrical or phoretic forces are sufficiently large the Greenfield Gap is closed.When the particles have radii < 3 μm inertial effects no longer dominate the collisions, although inertia modifies the weight effects for particles with radii down to about 0.5 μm. For charged aerosol particles with radii smaller than about 0.1 μm interacting with droplets or background aerosol particles smaller than a radius of about 15 μm, the long range electrical repulsive force is effective in opposing the phoretic forces and keeping the particle out of range of the short range attractive image force. Thus ‘electroscavenging’ gives way to ‘electroprotection’ against the scavenging or coagulation processes otherwise caused by Browninan diffusion or phoretic forces.In an atmosphere of temperature 10 °C and pressure 900 hPa the net phoretic force reduces to zero and becomes repulsive for particles with radii above about 2 μm (depending on particle conductivity). This enhances the development of the Greenfield Gap. However, the value of this radius (at which the net phoretic force is zero) increases strongly with decreasing temperature and pressure (increasing altitude) as expected from theory, and is about 5 μm in the middle troposphere and more than 10 μm in the stratosphere. Thus a net attractive phoretic force on particles extends into the 1–3 μm radius range in the upper troposphere; however, the weight and inertial effects can ensure the presence of the Greenfield Gap in that range for 2000 kg m^− 3 particles up to the middle stratosphere.     

Free convection frequency spectra of atmospheric turbulence over the sea

Frequency spectra of atmospheric turbulenceS (f) in the inertial subrange are considered in the free convection regime over the sea surface in a case of motionless instrument measurements (Eulerian frequency spectra). The frequency spectra formulaef _* S (f)/ ² =c (f _*/f)^5/3 for wind velocity (=1–3), temperature (=t) and humidity (=e) fluctuations are derived on the basis of similarity theory and the –5/3 law. These relations also can be derived from a consideration of convective large-scale advection of small eddies. The frequency scalef _* = (N ^{1 2}/)^1/2 (H/z ²)^1/3 is the lower bound of the inertial subrange and it is of order 10^–2 Hz.The spectra formulae are compared with direct measurements of atmospheric turbulence from the fixed research tower in the coastal zone of the Black Sea in calm weather. It is shown that these formulae are realized at least over two to three decades of the frequency range (approximately from 10^–2 to 10 Hz) and values of the numerical coefficients are found. The derived formulae can be used for calculations of sensible and latent heat fluxes by measuring the high-frequency range of spectra at a fixed point at low wind speeds when the conventional inertial dissipation method is not applicable.     

A comparison of turbulence statistics in the surface layer over plant canopies with those over several other surfaces

Turbulence statistics, including higher order moments, in the surface layer over plant canopies were compared with those observed over several different surfaces, using a nondimensional height (z – d)/z ₀: The values of (z – d)/z ₀extend over a very wide range from 10 over plant canopies to 10⁷ over the ocean. Several properties such as intensities of turbulence and skewness factors show a remarkable height-dependency in the air layer below (z – d)/z ₀ = 10², which is supposed to be much influenced by the underlying surface. In that layer, some peculiar phenomena, such as a downward energy transport and positive flux of shear stress, are frequently observed.     

An observational study of wind-induced waving of plants

The motions of individual plants and the turbulence statistics of surface winds measured near the top of a canopy are obtained over a wheat field and a rush field. Two typical cases of motions of individual plants are presented. The displacements of the ear of wheat (the plant height is 1.0 m) showed a natural oscillation in wind speeds of 1.6 m s^–1 measured at a height of 30 cm over a wheat canopy, while displacements of the stem of a rush plant were closely related to the fluctuations of surface winds in wind speeds of 1.7 m s^–1 measured at the top of the rush plant. The power spectra of displacements of a rush plant seem to support the negative seven-third power hypothesis proposed by Inoue. The frequency responses of displacements of plants to fluctuations of the instantaneous momentum flux are also presented.