Production of radionuclides by cosmic rays at mountain altitudes

Production rates of²²Na (T_1/2 = 2.6years) from aluminium by the action of cosmic rays are measured at the Mont Blanc (altitude 4600 m), the Aiguille du Midi (3840 m), and the Col du Lautaret (2070 m). They are2.3 ± 0.5,1.8 ± 0.3,and0.77 ± 0.18 atoms min^?1 kg^?1, respectively, in good agreement with the calculated production rates, 2.4, 1.7 and 0.6 atoms min^?1 kg^?1, respectively, at the three stations.Production rates of²⁴Na (T_1/2 = 15hours) from aluminium and magnesium are also measured at the Aiguille du Midi; the observed rates of3.4 ± 0.4and6.0 ± 1.7 atoms min^?1 kg^?1, respectively, agree well with the theoretically expected rates of 3.7 and 5.6 atoms min^?1 kg^?1.The production rates of³H,⁷Be,¹⁰Be,¹⁴C,²²Na,²⁶Al,³⁶Cl,³⁷Ar,³⁹Ar,⁵³Mn,⁵⁴Mn, and⁵⁵Fe in terrestrial rocks by the action of cosmic rays are calculated in order to show the possibility of applying the measurements of these cosmogenic radionuclides to the earth science.     

On the depth-dependent production of long-lived spallogenic53Mn in the St. Severin chondrite

The contents of spallogenic⁵³Mn and target elements for its production were determined in 80- to 400-mg samples from 13 different locations of the LL6 chondrite St. Severin, along the 34.8-cm drill core AIII. The⁵³Mn content increases from the surface to the center of the stone by ≈30%. The variation with depth is satisfactorily described by several models, presuming that appropriate primary and secondary particle fluxes are chosen. The⁵³Mn saturation activities (⁵³Mn^*) are linearly correlated with the spallogenic³He/²¹Ne and²²Ne/²¹Ne ratios, which suggests the possibility to eliminate uncertainties in the determination of⁵³Mn cosmic ray exposure ages arising from depth effects and terrestrial residence times.     

The unique cosmic-ray history of the Malakal chondrite

Cosmogenic radionuclides, including²²Na,²⁶Al and⁵⁴Mn, were measured in a sample of the recently-fallen Malakal hypersthene chondrite. The high²⁶Al activity, 79 ± 2 dpm/kg, greatly exceeds the levels expected from elemental production rates, shielding considerations, or comparisons with other ordinary chondrites, and can only be explained by exposure to a uniquely high cosmic-ray flux. Calculations including noble gas,³H, and⁵³Mn data from other laboratories require a two-stage irradiation. Malakal's most probable history is: exposure in excess of 4 m.y. to an effective cosmic-ray flux approximately three times that experienced by other chondrites, an orbit change (very possibly caused by a collision), and a final period of about 2 m.y. during which it was exposed to a “normal” cosmic-ray flux.     

Cosmogenic and radiogenic noble gases in the Dhajala chondrite

Whole rock and chondrules of the Dhajala chondrite were analyzed for Ne, Ar, Kr and Xe by total melting as well as by stepwise heating techniques. The cosmic ray exposure ages for the whole rock and the chondrules are6.2 ± 0.8 and6.3 ± 1.0m.y. as determined by the²¹Ne method and4.8 ± 1.5 and4.2 ± 2.0m.y. by the³⁸Ar method, respectively. The K-Ar age of the whole rock is4.2 ± 0.4b.y. The elemental composition of the trapped gas in this chondrite is of “planetary” type. The radiogenic¹²⁹Xe contents in the whole rock and chondrules are similar and this component is very retentively sited in the chondrules.     

Extra-terrestrial 53Mn in Antarctic ice

The reasons why⁵³Mn (a cosmogenic radionuclide with a half-life of 3.7 × 10⁶ y) appears as one of the best indicators of the presence of interplanetary dust are summarized. This paper reports the detection of⁵³Mn in pre-1952 snow samples collected on the Eastern Antarctic Plateau in the vicinity of Plateau Station. The measurements were carried out by neutron activation and X-ray spectrometry on three samples weighing a few hundred kg and covering each the time interval 1935–1950. The specific activity of⁵³Mn was found to be (0.82 ± 0.17) disint.min^?1/10³ tons of snow, corresponding to a deposition rate at Plateau Station of (2.2 ± 0.5) × 10^?5 disint. min^?1 m^?2 y^?1. The mean global deposition rate would be three times higher if⁵³Mn were assumed to behave in the same way as stratospheric⁹⁰Sr. By comparing this figure with existing data on the meteorite flux reaching the earth and with the galactic and solar production rates of⁵³Mn, it is concluded that the bulk of the⁵³Mn found at Plateau Station is associated with interplanetary dust in which it had been produced by the action of solar protons on iron. The deposition rate of extra-terrestrial dust-borne iron must be between 1.3 × 10^?5 and 1.3 × 10^?4 g m^?2 y^?1 at Plateau Station. These results support jointly with other studies the concept of an interplanetary zodiacal cloud of dust with a chemical composition and density not essentially different from chondritic meteorites, with a relatively ‘flat’ grain size distribution and a mass influx to the earth of the order of 10⁵ tons/y.     

Trapped solar wind He,Ne, and Ar and energetic He in Surveyor 3

The Apollo 12 mission brought back sections of the Surveyor 3 vehicle suitable for mass spectrometric studies of implanted solar wind and solar cosmic rays. Using this method, we have determined an average solar wind ⁴He flux of 6.1 × 10⁶ ions/cm² sec for the 31 months of exposure. We have also measured ⁴He/³He= 2700 ± 50;⁴He/²⁰Ne= 410 ± 30;²⁰Ne/²²Ne= 13.5 ± 0.2;²⁰Ne/³⁶Ar= 24.5 ± 2.5; and ³⁶Ar/³⁸Ar= 5.41 ± 0.20. These measurements provide solar wind values averaged over considerably longer periods of time than the Apollo Solar Wind Composition experiments and suggest that the short term SWC measurements during a period of high solar activity may not be a reliable measure of average solar wind composition.     

Beginning of the new solar cycle (cycle 24) in the large-scale open solar magnetic field

It is proposed to determined minimums of the 11-year solar cycles based on a minimal flux of the large-scale open solar magnetic field. The minimal fluxes before the finished cycle 23 (Carrington rotation CR 1904) and the started cycle 24 (CR 2054, April 2007) were equal to 1.8 × 10²² and 1.2 × 10²² μs, respectively. The long-term tendency toward an approach to a deep minimum of solar activity is confirmed. On the assumption that magnetic flux variations from minimums to maximums are proportional to each other, the anticipated value of the maximal Wolf number during cycle 24 is estimated as W _max = 80.     

Cosmic ray flux variations,modulated by the solar and terrestrial magnetic fields,and climate changes. Part 2: The time interval from ∼10000 to ∼100000 years ago

A joint analysis of paleodata on variations in cosmic ray fluxes, solar activity, geomagnetic field, and climate during the period from ～10000 to ～100000 years ago has been performed. Data on the time variations in the concentration of ¹⁴C and ¹⁰Be cosmogenic isotopes, which are generated in the Earth’s atmosphere under the action of cosmic ray fluxes modulated by solar activity and geomagnetic field variations, were used to detect variations in solar activity and the geomagnetic dipole. Information about climate changes has been obtained mainly from variations in the concentration of stable isotopes in the natural archives. A performed analysis indicates that the variations in cosmic ray fluxes under the action of variations in the geomagnetic field and solar activity are apparently one of the most effective natural factors of long-term climate changeability on a large time scale.     

Primordial gases in graphite-diamond-kamacite inclusions from the Haveröureilite

Stepwise heating experiments on separated graphite-diamond-kamacite aggregates have revealed a pronounced difference in the release patterns of spallogenic³He and trapped gases. About half the³He is released at T ? 920°C, without being accompanied by significant amounts of primordial gases; the latter, together with the remaining³He, is given off only at T ? 1200°C. Acid treatment of an aliquant dissolved about 2/3 of the total Fe in the sample but did not cause a significant change in the gas concentrations. It is concluded that (a) there is no evidence for a loss of spallogenic³He from the graphite-diamond-kamacite aggregates, (b) one major constituent of the aggregates - graphite - is almost void of trapped gases, (c) kamacite is not a main carrier of the gases. This leaves diamond as the most probable site of the primordial gases.The elemental abundance pattern in the noble gases is essentially as reported previously. In particular, the excellent correlation between relative depletion factors, normalized to the cosmic abundance ratios, and the respective ionisation energies is confirmed. Other important features of the trapped gases are a²⁰Ne/²²Ne ratio of 12.3 ± 0.6, intermediate between solar wind and solar flare implanted Ne,³⁶Ar/³⁸Ar = 5.20 ± 0.06 and a measured⁴⁰Ar/³⁶Ar ratio (before blank correction) of 0.0076.Possible modes of trapping of the noble gases are discussed.     

Cosmic-ray-produced53Mn in thirty-one meteorites

Cosmic-ray-produced⁵³Mn (t_½ = 3.7 × 10⁶years) has been determined by neutron activation analysis in twenty-two chondrites including three Antarctic meteorites: Yamato-7301 (j), -7305 (k) and -7304 (m).⁵³Mn was also measured in four mesosiderites, three iron meteorites, Bencubbin (unique) and Udei Station (iron with silicate inclusions). In addition, preliminary results for¹⁰Be (1.6 × 10⁶ years) were obtained in the Yamato meteorites using a low-background needle GM counter. Based on published values of rare gas ages, corrections were made for undersaturation; the average specific saturation activities of⁵³Mn were found in the range 450 ± 90dpm⁵³Mn/kg Fe in most of the chondrites and 490 ± 75dpm⁵³Mn/kg Fe in the mesosiderites. Two meteorites had extremely low contents of⁵³Mn: 102 ± 6 in Yamato-7301 and 48 ± 3dpm⁵³Mn/kg Fe in Bondoc. The Bondoc mesosiderite was already known to have a low concentration of cosmogenic radionuclides due to its large pre-atmospheric size. Several possible mechanisms are discussed to explain the low⁵³Mn activity in Yamato-7301: (1) long terrestrial age of about 7 m.y.; (2) low production rate of⁵³Mn due to heavy pre-atmospheric shielding (>70cm); (3) multi-stage irradiation history resulting in an undersaturation of⁵³Mn; and (4) a mechanism in which two or three of the above factors are combined. The ratio of⁵³Mn production rate in Ni to that in Fe has been estimated to be 1/3, based on the measurements of⁵³Mn in the metallic and silicate phases of St. Séverin meteorite, as well as on published results of some high-energy bombardment experiments.     

Behavior of the polar lower ionosphere during the solar flares in January 2005 according to the data of the partial reflections method

The results of the observations, using partial reflections, of the lower ionosphere over Tumannyi station in the Murmansk region (69.0° N, 35.7° E) during strong solar flares on January 15–20, 2005, are presented. The structure of the D region of the polar ionosphere and the effects of X-ray flares and fluxes of high energy protons on this region are considered. The anomalous values of electron density in the lower part of the D region, unusually low values of the height of the lower ionospheric boundary, complete or partial absorption of short and medium radiowaves, and bursts of the meter cosmic radio emission were detected during solar disturbances.     

VERTEX: manganese transport through oxygen minima

Manganese transport through a well-developed oxygen minimum was studied off central Mexico (18°N, 108°W) in October–November 1981 as part of the VERTEX (Vertical Transport and Exchange) research program. Refractory, leachable and dissolved Mn fractions associated with particulates caught in traps set at eight depths (120–1950 m) were analyzed. Particles entering the oxygen minimum had relatively large Mn loads; however, as the particulates sank further into the minimum, total Mn fluxes steadily decreased from 190 nmol m^?2 day^?1 at 120 m to 36 nmol m^?2 day^?1 at 400 m. Manganese fluxes then steadily increased in the remaining 800–1950 m, reaching rates of up to 230 nmol m^?2 day^?1 at 1950 m.Manganese concentrations were also measured in the water column. Dissolved Mn levels < 3.0 nmol kg^?1 were consistently observed within the 150–600 m depth interval. In contrast, suspended particulate leachable Mn amounts were especially low at those depths, and never exceeded 0.04 nmol kg^?1.The combined water column and particle trap data clearly indicate that Mn is released from particles as they sink through the oxygen minimum. Rate-of-change estimates based on trap flux data yield regeneration rates of up to 0.44 nmol kg^?1 yr^?1 in the upper oxygen minimum (120–200 m). However, only 30% of the dissolved Mn in the oxygen minimum appears to be from sinking particulate regeneration; the other 70% probably results from continental-slope-release-horizontal-transport processes.Dissolved Mn scavenges back onto particles as oxygen levels begin to increase with depth. Scavenging rates ranging from ?0.03 to ?0.09 nmol kg^?1 yr^?1 were observed at depths from 700 to 1950 m. These scavenging rates result in Mn residence times of 16–19 years, and scavenging rate constants on the order of 0.057 yr^?1. Manganese removal via scavenging on sinking particles below the oxygen minimum is balanced by Mn released along continental boundaries and transported horizontally via advective-diffusive processes.Manganese appears to be very weakly associated with particulates. Nevertheless, the amounts of Mn involved with sinking biogenic particles are large, and the resulting fluxes are on the same order of magnitude as those necessary to explain the excess Mn accumulating on the sea floor. The overall behavior of Mn observed in this, and other, studies strongly suggests some type of equilibrium occurring between dissolved and particulate phases. This equilibrium appears to shift in direct or indirect response to dissolved oxygen levels.     

26Al in iron meteorites and the constancy of cosmic ray intensity in the past

Cosmic-ray-produced²⁶Al in iron meteorites has been measured by low-level γγ-coincidence counting. The²⁶Al activities, in dpm/kg, are: Aroos3.0 ± 1.0, Braunau2.6 ± 0.5. Kayakent4.6 ± 1.5, N'Goureyma4.4 ± 1.1, Okahandja3.6 ± 0.9, Treysa4.0 ± 0.5. Exposure ages based on²⁶Al/²¹Ne are in agreement, within experimental error(±20%), with those based on³⁶Cl/³⁶Ar and³⁹Ar/³⁸Ar but the ages based on⁴⁰K/⁴¹K are higher by about 50%. The difference in exposure ages is probably caused by a real change of the cosmic ray intensity in the inner solar system.     

Recurrent variations of anomalous oxygen in association with a corotating interaction region

The fluxes of anomalous oxygen (E ranging from 3.5-6.8 MeV/amu), as measured by the EPAC instrument on ULYSSES, show a recurrent variation with the solar rotation period, which is anticorrelated with the fluxes of particles accelerated at the shocks of a corotating interaction region (CIR), and correlated with the fluxes of galactic cosmic rays known to be modulated by the CIR. The amplitude of this variation is much higher than expected for galactic cosmic rays of the same rigidity.     

Ti-V plots and the petrogenesis of modern and ophiolitic lavas

Radioactive and stable cosmogenic nuclides have been determined in the various fragments of the Kirin chondrite (H5). Experimental results obtained from our samples are described and compared with similar data obtained in other laboratories. Cosmogenic⁵⁴Mn,²²Na,⁶⁰Co,²⁶Al,⁵³Mn,⁴⁰K (in the metal phase), and light noble gases were measured. Based on these data, the irradiation history of this meteorite can be explained in terms of (1) a multi-stage exposure which involves a first-stage irradiation for 10⁷ years and a second stage for about 4×10⁵ years, and (2) depth effects in the productions of the nuclides in 4π(second stage) and 2π(first stage) geometries. These conclusions are consistent with those of our previous work which was based on a limited number of samples.     

Cosmic ray exposure ages of chondrites,pre-irradiation and constancy of cosmic ray flux in the past

A systematic calibration of the production rate of one specific cosmic-ray-produced nuclide in chondrites, that of²¹Ne, was achieved by using four independent methods:P₂₁(1.11) = 0.507 ± 0.039, 0.302 ± 0.013, 0.312 ± 0.017and0.292 ± 0.019 (in units of 10^?8 cm³ STP/g My) based on²⁶Al-age,⁵³Mn-age,⁸¹Kr-⁸³Kr and²²Na-²²Ne methods, respectively. These production rates are all normalized to a shielding parameter ratio²²Ne/²¹Ne= 1.11 and to the chemical composition of L chondrites. The results obtained by the latter three methods are in good agreement, but they disagree in a systematic way with the²⁶Al-age calibration. Based on these results, we recommend a valueP₂₁(1.11) = 0.31 and a production rate equation:P₂₁ = 4.845 P₂₁ (1.11) F[21.77(²²Ne/²¹Ne) ? 19.32]^?, whereF = 1.00 for L and LL, andF = 0.93 for H chondrites, for the calculation of cosmic ray exposure ages on the basis of Ne concentrations. In an attempt to assess possible causes for this discrepancy, we discuss the²⁶Al half-life measurements, we evaluate effects resulting from pre-irradiation of meteorites, and we discuss the evidence regarding the constancy of the cosmic ray flux in the past, in the light of some recent astronomical observations.     

Modulation of galactic cosmic rays in solar cycles 22–24: Analysis and physical interpretation

This work represents a physical interpretation of cosmic ray modulation in the 22nd–24th solar cycles, including an interpretation of an unusual behavior of their intensity in the last minimum of the solar activity (2008–2010). In terms of the Parker modulation model, which deals with regularly measured heliospheric characteristics, it is shown that the determining factor of the increased intensity of the galactic cosmic rays in the minimum of the 24th solar cycle is an anomalous reduction of the heliospheric magnetic field strength during this time interval under the additional influence of the solar wind velocity and the tilt angle of the heliospheric current sheet. We have used in the calculations the dependence of the diffusion tensor on the rigidity in the form K _ij ∝ R ^2?μ with μ = 1.2 in the sector zones of the heliospheric magnetic field and with μ = 0.8 outside the sector zones, which leads to an additional amplification of the diffusion mechanism of cosmic ray modulation. The proposed approach allows us to describe quite satisfactorily the integral intensity of protons with an energy above 0.1 GeV and the energy spectra in the minima of the 22nd–24th solar cycles at the same value of the free parameter. The determining factor of the anomalously high level of the galactic cosmic ray intensity in the minimum of the 24th solar cycle is the significant reduction of the heliospheric magnetic field strength during this time interval. The forecast of the intensity level in the minimum of the 25th solar cycle is provided.     

Cosmogenic neon produced from sodium in meteoritic minerals

Cosmogenic neon in sodium-rich oligoclase feldspar from the ordinary chondrites St. Severin and Guaren?a is characterized by an unusually high²²Ne/²¹Ne = 1.50 ± 0.02. This high ratio is due to the cosmogenic²²Ne/²¹Ne production ratio in sodium which is 2.9 ± 0.3, two to three times the production ratio in any other target element. The relative production rate of²¹Ne per gram sodium is one quarter the production rate per gram magnesium. The striking enrichment of²²Ne relative to²¹Ne in sodium arises from enhanced indirect production from²³Na via²²Na.The unusual composition of cosmogenic neon in sodium and sodium-rich minerals explains the high²²Ne/²¹Ne ratios observed in inclusions of the Allende carbonaceous chondrite, and observed during low-temperature extraction of neon from ordinary chondrites. The isotopic composition of cosmogenic neon released during the stepwise heating of a trapped gas-rich meteorite containing sodium-rich phases can be expected to vary, and use of a constant cosmogenic neon composition to derive the composition of the trapped gas may not be justified. Preferential loss of this²²Ne-enriched cosmogenic neon from meteoritic feldspar can result in a 2–3% drop in the measured cosmogenic²²Ne/²¹Ne ratio in a bulk meteorite sample. This apparent change in composition can lead to overestimation of the minimum pre-atmospheric mass of the meteorite by a factor of two.     

Cosmic ray flux variations, modulated by the solar and earth’s magnetic fields, and climate changes. 1. Time interval from the present to 10–12 ka ago (the Holocene Epoch)

Direct and indirect data on variations in cosmic rays, solar activity, geomagnetic dipole moment, and climate from the present to 10–12ka ago (the Holocene Epoch), registered in different natural archives (tree rings, ice layers, etc.), have been analyzed. The concentration of cosmogenic isotopes, generated in the Earth’s atmosphere under the action of cosmic ray fluxes and coming into the Earth archives, makes it possible to obtain valuable information about variations in a number of natural processes. The cosmogenic isotopes ¹⁴C in tree rings and ¹⁰Be in ice layers, as well as cosmic rays, are modulated by solar activity and geomagnetic field variations, and time variations in these concentrations gives information about past solar and geomagnetic activities. Since the characteristics of natural reservoirs with cosmogenic ¹⁴C and ¹⁰Be vary with climate changes, the concentrations of these isotopes also inform about climate changes in the past. A performed analysis indicates that cosmic ray flux variations are apparently the most effective natural factor of climate changes on a large time scale.     

Trapped solar and cosmogenic noble gas abundances in Apollo 15 and 16 deep drill samples

Abundances and isotopic compositions of all the stable noble gases have been measured in 19 different depths of the Apollo 15 deep drill core, 7 different depths of the Apollo 16 deep drill core, and in several surface fines and breccias. All samples analyzed from both drill cores contain large concentrations of solar wind implanted gases, which demonstrates that even the deepest layers of both cores have experienced a lunar surface history. For the Apollo 15 core samples, trapped⁴He concentrations are constant to within a factor of two; elemental ratios show even greater similarities with mean values of⁴He/²²Ne= 683±44,²²Ne/³⁶Ar= 0.439±0.057,³⁶Ar/⁸⁴Kr= 1.60±0.11·10³, and⁸⁴Kr/¹³²Xe= 5.92±0.74. Apollo 16 core samples show distinctly lower⁴He contents,⁴He/²²Ne(567±74), and²²Ne/³⁶Ar(0.229±0.024), but their heavy-element ratios are essentially identical to Apollo 15 core samples. Apollo 16 surface fines also show lower values of⁴He/²²Ne and²²Ne/³⁶Ar. This phenomenon is attributed to greater fractionation during gas loss because of the higher plagioclase contents of Apollo 16 fines. Of these four elemental ratios as measured in both cores, only the²²Ne/³⁶Ar for the Apollo 15 core shows an apparent depth dependance. No unambiguous evidence was seen in these core materials of appreciable variations in the composition of the solar wind. Calculated concentrations of cosmic ray-produced²¹Ne,⁸⁰Kr, and¹²⁶Xe for the Apollo 15 core showed nearly flat (within a factor of two) depth profiles, but with smaller random concentration variations over depths of a few cm. These data are not consistent with a short-term core accretion model from non-irradiated regolith. The Apollo 15 core data are consistent with a combined accretion plus static time of a few hundred million years, and also indicate variable pre-accretion irradiation of core material. The lack of large variations in solar wind gas contents across core layers is also consistent with appreciable pre-accretion irradiation. Depth profiles of cosmogenic gases in the Apollo 16 core show considerably larger concentrations of cosmogenic gases below ～65 cm depth than above. This pattern may be interpreted either as an accretionary process, or by a more recent deposition of regolith to the upper ～70 cm of the core. Cosmogenic gas concentrations of several Apollo 16 fines and breccias are consistent with ages of North Ray Crater and South Ray Crater of ～50·10⁶ and ～2·10⁶ yr, respectively.