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1.
江苏北部潮滩沉积物中~(137)Cs和~(210)pb的分布特征(英文)   总被引:1,自引:0,他引:1  
Seven cores were collected from different sediment zones of tidal flats at Xin-yanggang in north Jiangsu province in August 2007. Sediment grain-size distribution and radioisotopes of ~(137)Cs and ~(210)Pb analysis were carried out for these cores. Sediment rates of the cores and radioisotopes distribution in surface sediment in different zones of the tidal flat were calculated from the ~(137)Cs and ~(210)Pb activities in sediments cores. The results indicated that each tidal zone had experienced different evolution phases, hydrological dynamics in the tidal flats made the grain-size of the surface sediment change gradually. ~(137)Cs and ~(210)Pb activities on the superficial layer of the cores varied spatially and the reason was discussed. On tidal flats, the fluctuation of ~(137)Cs and ~(210)Pb activities in the cores reflected the special sedimentary characteristics. Vegetation affects the grain-size distribution and the vertical profiles of ~(137)Cs and ~(210)Pb in the upper depths. ~(137)Cs and ~(210)Pb chronology got the comparable average sediment rates on the tidal flat. The characteristics of ~(137)Cs and ~(210)Pb in the cores reflected various depositional dynamical environments in different tidal zones and gave information on the different evolvement phases of the tidal zones. Based on the information of grain-size distribution, texture of the cores, sediment rates and topography, the evolution lines of the tidal flat were reconstructed.  相似文献   

2.
Seven cores were collected from different sediment zones of tidal flats at Xinyanggang in north Jiangsu province in August 2007. Sediment grain-size distribution and radioisotopes of 137Cs and 210Pb analysis were carried out for these cores. Sediment rates of the cores and radioisotopes distribution in surface sediment in different zones of the tidal flat were calculated from the 137Cs and 210Pb activities in sediments cores. The results indicated that each tidal zone had experienced different evolution phases, hydrological dynamics in the tidal flats made the grain-size of the surface sediment change gradually. 137Cs and 210Pb activities on the superficial layer of the cores varied spatially and the reason was discussed. On tidal flats, the fluctuation of 137Cs and 210Pb activities in the cores reflected the special sedimentary characteristics. Vegetation affects the grain-size distribution and the vertical profiles of 137Cs and 210Pb in the upper depths. 137Cs and 210Pb chronology got the comparable average sediment rates on the tidal flat. The characteristics of 137Cs and 210Pb in the cores reflected various depositional dynamical environments in different tidal zones and gave information on the different evolvement phases of the tidal zones. Based on the information of grain-size distribution, texture of the cores, sediment rates and topography, the evolution lines of the tidal flat were reconstructed.  相似文献   

3.
Sediment cores collected from six sites in Lake Baikal as part of an extensive investigation of sediment records of recent environmental change were dated radiometrically by 210Pb. Although the results obtained were in some respects comparable to those obtained by previous 210Pb studies, there were some significant differences. Most notably, a core from abyssal depths in the centre of the middle basin appeared to record at least wo major episodes of rapid sedimentation, possibly caused by turbidity currents. All cores, including those from the North Basin, contained significant records of weapons test fallout 137Cs, though these were of little chronological value due to the long residence time of 137Cs in the water column. Models and budgets for sediment and radionuclide transport through Baikal are presented and used to help validate the 210Pb results.  相似文献   

4.
江苏王港盐沼的现代沉积速率   总被引:35,自引:0,他引:35  
江苏海岸湿地总面积超过5000km^2,但围垦活动的加剧使盐沼湿地面积迅速减少;为了达到海岸防护、保滩促淤的目的,先后引种了大米草和互花米草。通过采集江苏王港潮滩盐沼湿地9处柱状样和挖取探槽剖面,以及对沉积剖面样品进行^210Pb和^137Cs测年分析,探讨了^210Pb的本底及影响^210Pb富集的因素,估算了王港盐沼湿地的现代沉积速率。王港潮滩盐沼沉积物对^210Pb的吸附作用较弱;受风暴潮、生物扰动、物源变化及实验误差等因素的影响,在^210Pbex剖面上出现了数据异常点,将这些数据点剔除后计算得到的沉积速率为33cm yr^-1,^137Cs测年显示,该地区1963年以来的平均沉积速率3.1cm yr^-1,与^210Pb法及前人研究结果相一致。根据一个典型剖面的^137Cs测年数据分析,王港潮滩盐沼的沉积过程根据地貌特征的不同可分3个阶段,大米草覆盖阶段滩面高程迅速增加,互花米草的生长提高了滩面淤积速率。  相似文献   

5.
There is an important volume of published information on Lac Dufault (Québec) which describes the history of metal inputs over 70 years and the changes that occurred in the lake as a result of this contamination. We used this abundant source of chronological markers to test the hypothesis that lake sediments can provide true historical records of trace metal loading from metal mining. Sediment cores were obtained from the deepest zone of the lake (19 m). The sediments were dated using 210Pb and 137Cs and they were analyzed for total elemental concentrations (Ca, Cd, Cu, Fe, P, Pb, S, Zn). Metal profiles in the sediment core preserved the distinct signatures of different mine exploitations documented in the lake watershed. In particular, the core recorded: the beginning of industrialization in 1926; increasing sedimentation rates associated with perturbations in the lake watershed; the maximum of sediment [Cu] and the contemporary exploitation of ore bodies rich in Cu; the maximum of sediment [Fe] and the contemporary production of pyrite by a mining operation; the low sediment [Cu] and [Zn] in the 1950s and the low contemporary production of these metals by mining operations; the maximum of sediment [Cd] and the contemporary production of Cd by a subsequent mining operation. Anomalies in the distribution of 214Pb activities in sediments reflected the intensity of acid mine drainage (AMD). There is good evidence that the lake resisted acidification from this AMD for the last thirty years. Overall, our results support the thesis that profiles of sedimentary Cd, Cu, Zn, Pb and Fe levels reflect the past history of metal input to Lac Dufault.  相似文献   

6.
We examine sediment distribution patterns in seven Florida lakes and discuss implications for paleolimnological studies of shallow, subtropical lakes. The study lakes are highly productive and should exhibit thick organic sediment deposits, but organic sediments are often grossly lacking because basins are shallow, and frequent mixing, lack of stratification, and warm temperatures lead to breakdown of organic material.Organic sediment distribution patterns are highly variable. We observe three types of distribution patterns. When organic sediments are abundant, there may be (1) uniform sediment distribution. In lakes lacking organic sediments, there are (2) distribution to deeper areas if present, or (3) distribution to peripheral areas and embayments when deep waters are absent. We advocate the use of systematic mapping surveys to locate optimal coring sites for paleolimnological studies of shallow, wind-stressed lakes. Because numerous factors affect diagenesis and sediment redistribution, sediment abundance and location are not predictable. Sediment chronologies may be discontinuous and disturbed even in accumulation zones. The extent to which sedimentary records are discontinuous or disturbed is not quantifiable in any practical manner. 210Pb and 137Cs radioisotopic profiles provide qualitative evidence of the degree of stratigraphic disturbance. Total excess 210Pb inventories show that sediments are focused into depositional zones when sediment distribution is uneven. Excess 210Pb inventories are not informative about the completeness of sedimentary profiles unless small inventories suggest discontinuous sedimentation or erosional events. We present examples of disturbed and undisturbed profiles, and discuss how we use radioisotopic and geochemical evidence, and multiple cores to assess stratigraphic continuity.Journal Series No. R-04815 of the Florida Agricultural Experiment Station.  相似文献   

7.
云南抚仙湖近现代沉积速率变化研究   总被引:14,自引:0,他引:14  
王小雷  杨浩  丁兆运  杨本俊  张明礼 《地理学报》2011,66(11):1551-1561
借助GPS定位,采集了云南抚仙湖不同区域的7 个沉积物柱芯。通过对抚仙湖沉积物柱芯样品的放射性核素210Pb 和137Cs 测试分析,发现所有柱芯中均存在3 个公认的137Cs 计年时标(1954 年137Cs首次沉降、1963 年全球公认的137Cs最大沉降蓄积峰和1986 年前苏联切尔诺贝利核事故产生的137Cs 沉降蓄积峰),部分柱芯中存在20 世纪70 年代中期中国大气核试验形成的1975/1976 年次级蓄积峰,分析了该次级定年时标存在的合理性。借助210Pb CRS计年模式获得了抚仙湖过去百余年来的沉积年代,与137Cs 时标计年结果相比较存在一定偏差,对两种计年结果产生差异的可能原因进行了探讨。基于210Pb 和137Cs 计年结果,结合历史文献记载得出,自19 世纪中期以来,抚仙湖各个沉积物柱芯(FX6 除外) 的沉积速率变化规律具有相似性,大致可以划分为3 个阶段:A:自然演化阶段,B:人为扰动阶段,C:人为改造阶段。这种不稳定的沉积环境与抚仙湖地区相应历史时期的人类活动有密切关系,表明人类活动是影响短时间尺度下环境变化的主要驱动力。  相似文献   

8.
210Pb and 137Cs dating methods in lakes: A retrospective study   总被引:1,自引:0,他引:1  
210Pb has been used for more than two decades to provide the geochronology of annually deposited sediments and to construct pollution histories. Evidence from some lakes suggests that this radionuclide may be adequately mobile to compromise dating reliability. This study provides one test of that possibility by comparing recent measurements of 210Pb and trace metals to ones carried out more than 20 yrs in the past. 137Cs dating is used to confirm sediment accumulation rates in the recent cores. In the three Connecticut, USA, lakes studied, sediment accumulation rates changed abruptly to higher values between 40-50 yrs ago (increasing by factors of 2.2, 2.9, and 3.0). In all three lakes, rates calculated from 210Pb distributions both above and below this horizon agreed, within measurement uncertainty, in recent and older cores. Furthermore, when the older data were corrected for 20 yrs of burial, the changes in slope in 210Pb distributions occurred at the same depth in each pair of cores. The depth of sharp peaks in concentrations of trace metals also matched. In general, this evidence supports the idea that sediments in these lakes have simply been buried, without significant diagenetic remobilization of 210Pb and trace metals . Nevertheless, some important differences were also observed. For two of the three lakes, there was a significant difference in average sediment accumulation rate during the past 33 yrs as calculated from 137Cs and 210Pb in the recent cores. Most potential causes for this difference can be ruled out, and it appears that one of the two nuclides is remobilized compared to the other. There were also significant differences in the total inventories of both 210Pb and trace metals (both up to 2 ×) between recent and older cores in some cases. This may be due to dissimilar sediment focusing, since it is not known for certain whether the new cores were collected at exactly the same sites as in the past.  相似文献   

9.
Sediment cores collected from eight lakes along the western coast of Svalbard as part of a project investigating atmospheric pollution and environmental change in Arctic regions were dated radiometrically using natural (210Pb) and artificial (137Cs and 241Am) fallout radionuclides. At four sites the sedimentation rates were relatively uniform, and in consequence the 210Pb dates were relatively unambiguous. At the remaining sites there were irregularities in the 210Pb activity versus depth profiles, indicating significant variations in the net sediment accumulation rate during the past 120 years. At these sites, there were significant differences between 210Pb dates calculated using the two standard simple dating models, constant rate of supply (CRS) and constant initial concentration (CIC). In most cases, stratigraphic dates based on the 137Cs and 241Am records supported use of the CRS model, though at one site (Ossian Sarsfjellet) the CIC model appeared more appropriate. The irregularities in the 210Pb records were mainly caused by episodes of accelerated sedimentation due, for example, to inwash or slump events, though at some sites there appears to have been a systematic increase in sediment accumulation rates in recent decades. Sediment accumulation rates were generally lower at the northern sites, and higher at the more southerly locations. Mean sediment accumulation rates varied by an order of magnitude, ranging from 0.002 to 0.050 g cm−2 y−1 (0.02–0.10 cm y−1). 210Pb fluxes measured from the core inventories were mostly in the range 34–80 Bq m−2 y−1 typical of Arctic sites. Much higher values, recorded at two sites (Birgervatnet and Daltjørna), may be due to significant inputs from the catchments during spring thaw.  相似文献   

10.
长江中游网湖近代沉积环境演变及其对人类活动的响应   总被引:5,自引:2,他引:3  
史小丽  秦伯强 《地理研究》2013,32(5):808-816
采用放射性核素210Pb和137Cs计年方法,建立了长江中游网湖近代沉积物的年代序列,并对网湖沉积物的粒度组成、磁性参数、重金属元素、花粉组合以及营养盐含量等指标进行了分析。根据沉积指标垂直分布的综合特征,结合湖区史料,重建了网湖100年来沉积环境的演变过程。通过对沉积指标与湖区人口变化、工农业产值等数据的比对,发现中华人民共和国成立以后沉积物中TOC和TN浓度与人口变化存在较高的相关性,相关系数分别达到0.8892和0.8928(P<0.001);沉积物中重金属元素富集序列、营养盐富集序列与孢粉含量的变化序列与湖区人类活动具有较好的耦合性。表明网湖沉积指标可以敏感地反映湖区的人类活动。  相似文献   

11.
在广东省东南部惠州市的黄洞水库中取得沉积物柱芯,对其样品做了210Pb 和137Cs 比活度分析、粒度分析和孢粉及炭屑分析,并收集了这一水库邻近气象站的降水数据,计算了1960 年以来的年降水量、夏季(6-9 月) 降水量和24 小时暴雨量。利用上述210Pb和137Cs比活度分析结果建立了沉积物剖面的年代框架,结合孢粉浓度、炭屑浓度与降水量计算结果,对沉积剖面的粒度变化做出了解译,并初步推测1960-2009 年间水库所在流域的土壤侵蚀变化情况及其原因。研究表明,在该亚热带丘陵地区植被覆盖度较高的自然条件下,侵蚀作用对降水量波动和植被(尤其是乔木、灌木等木本植物) 覆盖度变化的响应十分灵敏,水库沉积物的粒度变化在一定程度上可以反映流域内土壤侵蚀相对强度的变化。  相似文献   

12.
Tidal flats, a precious resource that provides ecological services and land space for coastal zones, are facing threats from human activities and climate change. In this study, a robust decision tree for tidal flat extraction was developed to analyse spatiotemporal variations in the Bohai Rim region during 1984-2019 based on 9539 Landsat TM/OLI surface reflection images and the Google Earth Engine (GEE) cloud platform. The area of tidal flats significantly fluctuated downwards from 3551.22 to 1712.36 km2 in the Bohai Rim region during 1984-2019, and 51.31% of tidal flats were distributed near the Yellow River Delta and Liaohe River Delta during 2017-2019. There occurred a drastic spatial transition of tidal flats with coastline migration towards the ocean. Low-stability tidal flats were mainly distributed in reclamation regions, deltas, and bays near the estuary during 1984-2019. The main factors of tidal flat evolution in the Bohai Rim region included the direct impact of land cover changes in reclamation regions, the continuous impact of a weakening sediment supply, and the potential impact of a deteriorating sediment storage capability. The extraction process and maps herein could provide a reference for the sustainable development and conservation of coastal resources.  相似文献   

13.
Low‐energy gamma ray spectroscopy has been employed to estimate floodplain sedimentation rates using measurements of 210Pb in floodplain alluvium. The utility of the technique is assessed through the analysis of excess (unsupported) 210Pb profiles in three sediment cores taken from the floodplain of the Labasa River on Vanua Levu in northern Fiji. A low‐energy germanium spectrometer (LEGe) was used for the nondestructive determination of excess 210Pb in a region cultivated intensively with sugarcane. Measured average historical (c. 25 years) vertical accretion rates are between 2.2 and 4.4 cm yr?1. The findings are broadly comparable with published sedimentation rates from analyses of radionuclide profiles elsewhere in the tropical South Pacific Islands, but the rates are higher than those measured previously at the same Labasa River sites using 137Cs profiles. Accelerated soil erosion owing to cane burning and land tillage seems to be largely responsible for sediment production, although flood‐related effects such as channel accretion by coarse bedload and the emplacement of large organic debris also influence floodplain sedimentation. However, application of the 210Pb technique in Fiji (and perhaps neighbouring island countries) is found to have serious drawbacks compared to the more robust 137Cs method, owing principally to the low 210Pb concentrations in the sandy alluvial sediment tested.  相似文献   

14.
Sediment focusing in six small lake basins is inferred from sedimentary radionuclide profiles. The activities of137Cs and9+240Pu do not decrease to zero above the sub-surface maximum but tail off gradually. Similar behavior is observed in the sediments of three lakes for134Cs and60Co, which were added only to the lake. This upward tailing is not caused by bioturbation or erosion from the watershed. Sediment focusing is the likely cause, further substantiated by inventories in deep sediments of9+240Pu and210Pb that are twice as high as expected from atmospheric fallout. Inventories in deep sediments of137Cs are in several cases lower than expected from atmospheric fallout, and cannot be explained by hydraulic flushing from the lakes, as this would require unreasonable flushing rates. The low137Cs inventories and the sedimentary profiles of the137Cs/9+240Pu ratio are consistent with137Cs removal from the water column by boundary scavenging to shallow sediments. The profiles and inventories of all three nuclides could be reproduced with a simple three box model, assuming focusing of shallow sediments (50–60% of total sediment area) to deep sediments with a rate constant of 5–10% yr–1.This is the seventh of a series of papers to be published by this journal following the 20 th anniversary of the first application of210Pb dating of lake sediment. Dr P. G. Appleby is guest editing this series.  相似文献   

15.
Low-background gamma counting: applications for210Pb dating of sediments   总被引:1,自引:0,他引:1  
Sediment cores from three lakes were dated with210Pb using a constant rate of supply (CRS) model. We used low-background gamma counting to measure naturally occurring levels of210Pb,226Ra, and137Cs in sediment samples because sample preparation is simple and non-destructive,226Ra activity provides a direct measure of supported210Pb activity for each sample analyzed, and137Cs activity may provide an independent age marker for the 1962–1963 peak in atmospheric fallout of this radionuclide. In one core supported210Pb activity was estimated equally well from226Ra activity of each sampling interval or from the mean total210Pb activity of constant activity samples at depth. Supported210Pb activity was constant with depth in this core. In a short freeze core, determining226Ra activity of every sample proved advantageous in estimating supported210Pb activity because supported210Pb activity could be estimated from210Pb measurements only at the deepest sampling interval. Supported210Pb activity estimated from226Ra activity also yielded more precise estimates of highly variable sedimentation rates. In the third core226Ra activity exceeded210Pb activity at the top of the core and varied 20 fold with depth. This high input of226Ra in disequilibrium with210Pb is attributed to recent erosion of radium-bearing materials in the drainage basin. These data invalidate the assumption that supported210Pb activity is constant in sediment cores and can be estimated from the mean total210Pb activity at depths where210Pb activity is constant. We recommend using gamma counting or another independent assay of226Ra to validate the assumption of constant supported210Pb activity in sediment cores if there is reason to expect that226Ra activity varies with depth.This is the fourth of a series of papers to be published by this journal following the 20 th anniversary of the first application of210Pb dating of lake sediments. Dr. P.G. Appleby is guest editing this series.  相似文献   

16.
Spheroidal carbonaceous particles (SCP) from combustion of oil and coal have been quantified in cores from top sediments of Danish shallow lakes. Chronologies were provided by 210Pb-dating supplemented by measurements of other radionuclides (137Cs, 134Cs, 241Am). All cores show indications of sediment mixing but most still retain a characteristic SCP record. Deposition rates of SCP were low until the 1920s, increased strongly after World War II, reached maximum levels around 1970 and decreased thereafter. These results were used to infer a new chronology for a sediment core from a shallow lake, from which a 210Pb chronology had previously been published.SCP inventories are positively correlated with 210Pb inventories and dry matter accumulated since 1900, suggesting that absolute SCP accumulation rates may be more influenced by sedimentary processes than by atmospheric fluxes. The concentrations of SCP in surface sediments of the six lakes do, however, correlate with regional SO2 emissions.  相似文献   

17.
Reconstructing recent limnological history often relies on lead-210 dating to accurately ascribe a chronology to a sediment profile. In Lake Okeechobee, Florida, a large, shallow subtropical lake that may experience severe mixing, multiple dating methods are required to confirm that conformable sedimentation has been preserved and that the assumptions of the 210Pb method are satisfied. This study uses stratigraphic profiles of heavy metals, 137Cs, PCBs and pollen as independent dating markers to validate the sediment chronology as determined by 210Pb for three cores from the central mud zone of the lake. Unsupported 210Pb and most dating markers show distinct concentration/depth profiles, suggesting that the sediments have not been severely mixed for at least the last 75 years. Onset and maximum activity of the radioisotope 137Cs in the cores coincides with the 210Pb-dated interval of 1945–1970. This agrees well with the known timing of atmospheric deposition of 137Cs that resulted from above-ground nuclear testing during late 1940s until 1963. Sediment core profiles of atmospherically deposited metals such as Zn and Pb, which reflect regional increases during industrialization and decreases after regulation in the 1970s, exhibit expected concentration increases and peaks coinciding within 5–15 years of the predicted 210Pb dates. Uranium, a contaminant in some phosphate fertilizers, shows large concentration increases at core depths dated to be about 1950 by 210Pb, matching the intensification of agriculture after WWII. PCBs, which are expected to peak in the early 1970s, were measured in one core, and the observed peak corresponds to a 210Pb date of about 1960. Pollen makers were unable to verify specific events, but increases in disturbance taxa and declines in native types correspond generally with the expected dates assigned by 210Pb dating. Conformity between the 210Pb defined dates and independent markers of < ±15 years confirm that Lake Okeechobee sediments do preserve a sequential and reliable stratigraphic history of the lake, useful for reconstructing past limnological conditions.  相似文献   

18.
210Pb geochronologies should be validated with independent tracers such as 137Cs. In the cases with constant 210Pb activity in the topmost sediments, the presence of a distinct 137Cs peak within the 210Pb plateau has been used as a definitive demonstration of acceleration (increase in the sedimentation rate in recent years) versus fast mixing. Nevertheless, some limitations can be identified in the use of semiquantitative arguments, and a global understanding of the whole 137Cs activity profile is then required. Particularly, the incomplete mixing within the top sediment zone (described through the Incomplete Mixing Zone model) can explain quantitatively and simultaneously the 137Cs peak and the flattening in the 210Pb activity profile. This is demonstrated using selected examples from literature data. Thus, measured constant 210Pb activities in the top 6 cm of a sediment core from Lake Zürich. Nevertheless, they found 7Be only in the uppermost layer, the distinct 137Cs maximum at 6 cm depth, and undisturbed varves. The fast mixing seemed then opposed to common sense. The constant rate of supply model shows acceleration and it adequately matches the position of the 1963 137Cs peak. Nevertheless it fails to explain the whole 137Cs profile when handling time series of 137Cs atmospheric deposition. Finally, it is shown how the incomplete mixing of the activity (through the pore water) over a certain mass depth at the top sediment, with a finite value of the mixing coefficient, can quantitatively explain the whole activity versus mass depth profiles of 137Cs and 210Pb, and the presence of 7Be only in the uppermost sediment layer. A further validation of these ideas is presented from other literature data.  相似文献   

19.
Integrating remote sensing, geographic information system (GIS) and fractal theory, change characteristics of tidal flats and tidal creeks in the Huanghe (Yellow) River Delta over the period of 1986-2001 were discussed. The results show that evolutions of tidal fiats throughout the Huanghe River Delta are influenced by various factors, and that progressive succession and regression of tidal flats concur in different coastal segments of the delta. Human activities have played an increasingly important role in the succession process of tidal flats. Due to land reclamation in coastal zones of the delta in the last 15 years, lots of tidal flats were occupied, the artificial coastline migrated seaward (the maximum change rate was 0.8 kmyr^-1) and tidal creeks became sparser (the highest decreasing rate of length of tidal creeks was 14.9 kmyr^-1). Except for two coastal segments from the Tiaohe Estuary to the 106 Station and from the south of the Huanghe River mouth to the north of the Xiaodao River Estuary,fractal dimension values of tidal creeks in the remaining coastal segments of the delta decreased. In addition, the time dimension, sediment fluxes into the sea, waves and tidal-currents have profound influences on the evolution process of tidal flats. Four types of tidal flats-river-dominated tidal flats,tide-dominated tidal flats, wave-dominated tidal flats and man-dominated tidal flats can be identified.Owing to the intensification of human activities in coastal zones of the delta, man-dominated tidal flats have become the main kind of tidal flats.  相似文献   

20.
In 2008, three short sedimentary cores were collected from Nanyihu Lake in the lower Yangtze River Basin using a gravity corer. Heavy metals, including Pb, Cu, Zn, Cr, Ni, Mn, and major elements, including Al, Fe, K, Na, Mg and Ti, were measured. Radionuclides, including 210Pb and 137Cs, were analyzed to date the sediments. The significant Mn enrichment in the uppermost sediments of the three cores did not influence the distribution of Pb, Cu, Zn, Cr and Ni. The Pb, Cu, Zn, Cr and Ni contents have increased over the past 30–40 years. The decline of 206Pb/207Pb ratios toward the surface indicated increasing anthropogenic Pb loading to the lake sediments. However, the heavy metal enrichment was low overall because of the high sediment accumulation rates and the low anthropogenic heavy metal flux into the Nanyihu Lake.  相似文献   

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