Mineral magnetic characterization of sediment sources from an analysis of lake and floodplain sediments in the catchments of the Old Mill reservoir and Slapton Ley,South Devon,UK

Research on suspended sediment transport in the catchments of the Old Mill reservoir and Slapton Lower Ley, South Devon, has attempted to discriminate changing catchment sources on the basis of downcore variations in the mineral magnetic properties of lake, reservoir and floodplain sediments. Here, we examine these downcore variations and also explore the variability in catchment sources and the influence of topographic controls on mineral magnetic signatures of topsoils and subsoils. Particle size controls on the mineral magnetic signatures are explored by an analysis of a fractionated sediment sample, whilst the possible impact of diagenesis is assessed by an examination of the Mn profiles in the lake and reservoir sediments. From this analysis it is evident that the mineral magnetic signatures of well sorted floodplain deposits are more likely to reflect the particle size composition of the transported material. By contrast, the mineral magnetic record in the sediment of Slapton Ley appears to be most strongly influenced by dissolution of magnetic minerals. The sediment of the Old Mill reservoir provides the only suitable record for the application of a simple mixing model which is developed in order to quantify changes in the relative contribution of topsoil and subsoil through time. The research has important implications for attempting to reconstruct sediment sources in highly eutrophic lakes and emphasizes the uncertainty in the application of simple mixing models. © 1998 John Wiley & Sons, Ltd.     

Problems of core correlation,sediment source ascription and yield estimation in Ponsonby Tarn,West Cumbria,UK

A suite of 27 short cores, 10 of which have been used for magnetic measurements and four for radiometric dating, provides a framework for reconstructing the processes, patterns and rates of sedimentation in Ponsonby Tarn, a small artificial impoundment created towards the end of the 19th century, close to the Sellafield nuclear reprocessing plant in NW England. Spatial and temporal changes in sedimentation are reconstructed and evidence presented for non-synchroneity in magnetic property changes from core to core in the upper part of the sequence, as a result of sorting and selective deposition at different distances from the inflow to the Tarn. Magnetic measurements alone are therefore not a secure basis upon which to quantify sediment yield for defined time intervals at this site. The chronology, established mainly from ²¹⁰Pb and ¹³⁴Cs analyses, allows estimates of mean sediment yield per annum for four periods: prior to AD 1940, 1940–1964, 1964–1986 and 1986–1991. The rates of sediment accumulation have increased in recent times, especially since 1964, with evidence for input from both magnetically enhanced soils and gleyed alluvial and/or podsolized subsoil sources. Pre-1940 mean annual deposition within the present area of the lake is calculated as 19·5 t a⁻¹ and for the period since 1986 (the period of maximum sedimentation rates), as 111·3 t a⁻¹. These represent yields of 7·0 t km⁻² a⁻¹ and 39·8 t km⁻² a⁻¹, respectively, for the catchment as a whole. Rock magnetic evidence, based on measurements of both bulk samples and the finest particle size separates, suggests that bacterial magnetite, formed within the lake, contributes to the magnetic properties of the sediments, thus modifying the signatures relating to allochthonous sediment input. Copyright © 1999 John Wiley & Sons, Ltd.     

Fingerprinting upland sediment sources: particle size‐specific magnetic linkages between soils,lake sediments and suspended sediments

Accelerated erosion of fine‐grained sediment is an environmental problem of international dimensions. Erosion control strategies and targeting of mitigation measures require robust and quantitative identification of sediment sources. Here, we use magnetic ‘fingerprinting’ to characterize soils, and examine their affinity with and contribution to suspended sediments transported within two subcatchments feeding Bassenthwaite Lake, northwest England. A high‐resolution soil magnetic susceptibility survey was made using a field susceptometer (ZH Instruments, SM400 probe). Combining the spatial and vertical (down‐profile) soil magnetic data, a subset of soil profiles was selected for detailed, laboratory‐based magnetic remanence analyses. The magnetic properties of the catchment soils are highly particle size‐dependent. Magnetic analyses were performed on the 31–63 µm fraction, for particle size‐specific comparison both with the suspended sediments and lake sediments. Fuzzy cluster analysis groups the soil magnetic data into six clusters, apparently reflecting variations in parent material and horizon type, with three magnetically hard soils as unclassified outliers. Examination of the cluster affinity of the soils, suspended sediments and lake sediments indicates that topsoils of the upper Newlands Valley and subsoils around Keskadale Beck are a major source of the Newlands Beck suspended load, and the recent (post‐nineteenth century) sediments in the deep lake basin. Older lake sediments show strong affinity with a small number of the Derwent suspended sediments and one of the Glenderamackin soils. A large number of Derwent suspended sediments show no affinity with any of the soils or lake sediments, instead forming a coherent, discrete and statistically unclassified group, possibly resulting from mixing between the magnetically hard subsoils of the medium to high‐altitude Glenderamackin and Troutbeck areas and softer, lower altitude Glenderamackin soils. The lack of any affinity of these suspended sediments with the lake sediments may indicate deposition along the Derwent flood plain and/or in the shallow delta of Lake Bassenthwaite. Particle size‐specific magnetic fingerprinting is thus shown to be both highly discriminatory and quantitatively robust even within the homogeneous geological units of this catchment area. Such a methodological approach has important implications for small–large scale catchment management where sources of sediment arising from areas with uniform geology have been difficult to determine using other approaches, such as geochemical or radionuclide analyses. Copyright © 2009 John Wiley & Sons, Ltd.     

Use of composite fingerprints to determine the provenance of the contemporary suspended sediment load transported by rivers

Sediment fingerprinting appears to offer a valuable alternative to direct monitoring for elucidating the provenance of suspended sediment and the relative importance of spatial zones or subcatchments comprising larger (>500 km²) drainage basins. Against this background, a quantitative composite fingerprinting technique, incorporating both statistically verified multicomponent signatures and a multivariate sediment-mixing model, has been employed to determine the spatial origin of contemporary suspended sediment transported from the upper and middle reaches of the River Exe (601 km²) and River Severn (4325 km²) basins, UK. Spatial origin is addressed in terms of the relative contribution from three distinct geological subareas constituting each study basin. The consistency of the composite fingerprinting approach is examined using the estimates for mean and seasonal variations in source area contributions and also a comparison between the results obtained for individual flood events and alternative lines of evidence provided by flood travel times and the spatial distribution of precipitation. It is argued that fingerprinting estimates for sediment provenance are consistent with existing information on suspended sediment yields from different subcatchments within the study basins, although in the Severn, the role of storage and remobilization in producing signature ‘averaging’ may complicate comparison of the fingerprinting data with typical floodwater routing times. Validation represents the greatest problem for the cost–benefit of fingerprinting and scope still exists for further refinement of the procedures involved. © 1998 John Wiley & Sons, Ltd.     

Revisiting lake sediment budgets: How the calculation of lake lifetime is strongly data and method dependent

Lake sedimentation has a fundamental impact on lake lifetime. In this paper, we show how sensitive calculation of the latter is to the quality of data available and assumptions made during analysis. Based on the collection of a large new dataset, we quantify the sediment masses (1) mobilized on the hillslopes draining towards Lake Tana (Ethiopia), (2) stored in the floodplains, (3) transported into the lake, (4) deposited in the lake and (5) delivered out from the lake so as to establish a sediment budget. In 2012–2013, suspended sediment concentration (SSC) and discharge measurements were made at 13 monitoring stations, including two lake outlets. Altogether, 4635 SSC samples were collected and sediment rating curves that account for land cover conditions and rainfall seasonality were established for the 11 river stations, and mean monthly SSC was calculated for the outlets. Effects of the floodplain on rivers' sediment yield (SY) were investigated using measurements at both sides of the floodplains. SY from ungauged rivers was assessed using a model that includes catchment area and rainfall, whereas bedload and direct sediment input from lake shores were estimated. As a result, the gross annual SY was c. 39.55 (± 0.15) Mt, dominantly from Gilgel Abay and Gumara Rivers. The 2.57 (± 0.17) Mt sediment deposited in floodplains indicate that the floodplains serve as an important sediment sink. Moreover, annually c. 1.09 Mt of sediment leaves the lake through the two outlets. Annual sediment deposition in the lake was c. 36.97 (± 0.22) Mt and organic matter accumulation was 2.15 Mt, with a mean sediment trapping efficiency of 97%. Furthermore, SSC and SY are generally higher at the beginning of the rainy season because soils in cultivated fields are bare and loose due to frequent ploughing and seedbed preparation. Later in the season, increased crop and vegetation cover lead to a decrease in sediment production. Based on the established sediment budget with average rainfall, the lifetime of Lake Tana was estimated as 764 to 1032 years, which is shorter than what was anticipated in earlier studies. The sedimentation rate of Lake Tana (11.7 ± 0.1 kg m^?2 yr^?1) is in line with the sedimentation rates of larger lakes in the world, like Lake Dongting and Lake Kivu. Copyright © 2017 John Wiley & Sons, Ltd.     

Water and sediment geochemistry of an urban lake: Implications to weathering and anthropogenic activity

Lakes are sensitive ecosystems and respond quickly to any natural or anthropogenic contamination,particularly in urban areas due to poor planning and mismanagement in urban settlement, encroachment, and anthropogenic pollution. In the current study, water and sediment geochemistry are used along with available time series of geospatial data sets to assess: a) provenance and sources of pollution in the lake sediment and water, b) health risk using various sediment and water quality indices, and c...     

Combining suspended sediment monitoring and fingerprinting to determine the spatial origin of fine sediment in a mountainous river catchment

An excess of fine sediment (grain size <2 mm) supply to rivers leads to reservoir siltation, water contamination and operational problems for hydroelectric power plants in many catchments of the world, such as in the French Alps. These problems are exacerbated in mountainous environments characterized by large sediment exports during very short periods. This study combined river flow records, sediment geochemistry and associated radionuclide concentrations as input properties to a Monte Carlo mixing model to quantify the contribution of different geologic sources to river sediment. Overall, between 2007 and 2009, erosion rates reached 249 ± 75 t km^?2 yr^?1 at the outlet of the Bléone catchment, but this mean value masked important spatial variations of erosion intensity within the catchment (85–5000 t km^?2 yr^?1). Quantifying the contribution of different potential sources to river sediment required the application of sediment fingerprinting using a Monte Carlo mixing model. This model allowed the specific contributions of different geological sub‐types (i.e. black marls, marly limestones, conglomerates and Quaternary deposits) to be determined. Even though they generate locally very high erosion rates, black marls supplied only a minor fraction (5–20%) of the fine sediment collected on the riverbed in the vicinity of the 907 km² catchment outlet. The bulk of sediment was provided by Quaternary deposits (21–66%), conglomerates (3–44%) and limestones (9–27%). Even though bioengineering works conducted currently to stabilize gullies in black marl terrains are undoubtedly useful to limit sediment supply to the Bléone river, erosion generated by other substrate sources dominated between 2007 and 2009 in this catchment. Copyright © 2011 John Wiley & Sons, Ltd.     

The representation of sediment source group tracer distributions in Monte Carlo uncertainty routines for fingerprinting: An analysis of accuracy and precision using data for four contrasting catchments

Previous studies comparing sediment fingerprinting un-mixing models report large differences in their accuracy. The representation of tracer concentrations in source groups is perhaps the largest difference between published studies. However, the importance of decisions concerning the representation of tracer distributions has not been explored explicitly. Accordingly, potential sediment sources in four contrasting catchments were intensively sampled. Virtual sample mixtures were formed using between 10 and 100% of the retrieved samples to simulate sediment mobilization and delivery from subsections of each catchment. Source apportionment used models with a transformed multivariate normal distribution, normal distribution, 25th–75th percentile distribution and a distribution replicating the retrieved source samples. The accuracy and precision of model results were quantified and the reasons for differences were investigated. The 25th–75th percentile distribution produced the lowest mean inaccuracy (8.8%) and imprecision (8.5%), with the Sample Based distribution being next best (11.5%; 9.3%). The transformed multivariate (16.9%; 17.3%) and untransformed normal distributions (16.3%; 20.8%) performed poorly. When only a small proportion of the source samples formed the virtual mixtures, accuracy decreased with the 25th–75th percentile and Sample Based distributions so that when <20% of source samples were used, the actual mixture composition infrequently fell outside of the range of uncertainty shown in un-mixing model outputs. Poor performance was due to combined random Monte Carlo numbers generated for all tracers not being viable for the retrieved source samples. Trialling the use of a 25th–75th percentile distribution alongside alternatives may result in significant improvements in both accuracy and precision of fingerprinting estimates, evaluated using virtual mixtures. Caution should be exercised when using a normal type distribution, without exploration of alternatives, as un-mixing model performance may be unacceptably poor.     

A preliminary assessment of the spatial sources of contemporary suspended sediment in the Ohio River basin,United States,using water quality data from the NASQAN programme in a source tracing procedure

Reliable information on catchment scale suspended sediment sources is required to inform the design of management strategies for helping abate the numerous environmental issues associated with enhanced sediment mobilization and off‐site loadings. Since sediment fingerprinting techniques avoid many of the logistical constraints associated with using more traditional indirect measurement methods at catchment scale, such approaches have been increasingly reported in the international literature and typically use data sets collected specifically for sediment source apportionment purposes. There remains scope for investigating the potential for using geochemical data sets assembled by routine monitoring programmes to fingerprint sediment provenance. In the United States, routine water quality samples are collected as part of the US Geological Survey's revised National Stream Quality Accounting Network programme. Accordingly, the geochemistry data generated from these samples over a 10‐year period (1996–2006) were used as the basis for a fingerprinting exercise to assess the key tributary sub‐catchment spatial sources of contemporary suspended sediment transported by the Ohio River. Uncertainty associated with the spatial source estimates was quantified using a Monte Carlo approach in conjunction with mass balance modelling. Relative frequency weighted means were used as an alternative way of summarizing the spatial source contributions, thereby avoiding the need to use confidence limits. The results should be interpreted in the context of the routine, but infrequent nature, of the suspended sediment samples used to assemble geochemistry as a basis for the sourcing exercise. Nonetheless, the study demonstrates how routine monitoring samples can be used to provide some preliminary information on sediment provenance in large drainage basins. Copyright © 2011 John Wiley & Sons, Ltd.     

Quantitative reconstruction of Holocene sediment sources contributing to the central Jiangsu coast,China: New insights into source-to-sink processes

Coastal deltaic deposits are the primary locations for sediment storage on Earth, and quantifying their source contributions is a critical prerequisite for delineating S2S patterns in marginal seas. In most cases, quantification for the contribution by fine-grained sediments (i.e. particle size < 63 μm) is considered to be representative to constrain the overall sediment supply. However, this approach may be inappropriate because large differences exist between the two quantities. Here we propose an approach to solve the problem, which is based on the maximum number of tracers from multiple sediment size fractions incorporating the content of all size fractions of sediment. Using this approach, absolute source contributions during the Holocene are reconstructed that provide a first-order model for the S2S pattern of the central Jiangsu coast, China. The Huanghe River is the strongest driver for the Holocene sedimentation, with a mean contribution of ~72 ± 6% (1417 × 10⁸ t). The absolute contributions from the Changjiang and offshore areas were of secondary importance, (i.e. ~17 ± 1% (330 × 10⁸ t) and ~11 ± 5% (217 × 10⁸ t), respectively). The results show that a large difference between the relative and absolute source contributions and the assumption that the relative contribution represents the absolute contribution is invalid in a coastal setting. The impact of the Huanghe is mainly based on episodic events, such as the event of 1128–1855 AD . The model also reveals that the offshore sediments are as important as the Changjiang sediments for the central Jiangsu coast during the Holocene. Thus, the model provides both the time series and overall quantities of sediment supply during the formation and evolution of the Holocene tidal flats on the Jiangsu coast. Our findings shed new light on quantitative analysis of sediment sources applicable to future S2S studies of marginal seas. © 2020 John Wiley & Sons, Ltd.     

Subglacial drainage system changes of the Gulkana Glacier,Alaska: discharge and sediment load observations and modelling

Hydrological characteristics of englacial and subglacial drainage systems in Gulkana Glacier, Alaska, were examined by analysing temporal variations of discharge and sediment load in the proglacial Phelan Creek in 2001. From data plots on semi‐log paper, it appeared appropriate to separate both discharge and sediment load into fast and slow components. The two components were possibly produced by two different drainage systems: an englacial and subglacial, ‘channellized’ system in the ablation zone, and a subglacial, ‘distributed’ system in the accumulation zone. The data indicate the occurrence of an event during which part of the ‘distributed’ drainage system changed into the ‘channellized’ drainage system. The daily time‐series of discharge and sediment load were represented using a tank model. In the model, the drainage from an additional tank was added, supposing that a subglacial reservoir full of water and sediment collapsed slowly when the subglacial drainage system changed from distributed to channellized. The simulation with the collapsed tank gave much more reasonable results than those with no collapsed tank. The contribution of the collapsed tank to total sediment load is 24%, which is much larger than 9% to total discharge. Copyright © 2006 John Wiley & Sons, Ltd.     

Application of Bayesian model and discriminant function analysis to the estimation of sediment source contributions

Bayesian and discriminant function analysis (DFA) models have recently been used as tools to estimate sediment source contributions. Unlike existing multivariate mixing models, the accuracy of these two models remains unclear. In the current study, four well-distinguished source samples were used to create artificial mixtures to test the performance of Bayesian and DFA models. These models were tested against the Walling-Collins model, a credible model used in estimation of sediment source contributions estimation, as a reference. The artificial mixtures were divided into five groups, with each group consisting of five samples with known source percentages. The relative contributions of the sediment sources to the individual and grouped samples were calculated using each of the models. The mean absolute error (MAE) and standard error of (SE) MAE were used to test the accuracy of each model and the robustness of the optimized solutions. For the individual sediment samples, the calculated source contributions obtained with the Bayesian (MAE = 7.4%, SE = 0.6%) and Walling-Collins (MAE = 7.5%, SE = 0.7%) models produced results which were closest to the actual percentages of the source contributions to the sediment mixtures. The DFA model produced the worst estimates (MAE = 18.4%, SE = 1.4%). For the grouped sediment samples, the Walling-Collins model (MAE = 5.4%) was the best predictor, closely followed by the Bayesian model (MAE = 5.9%). The results obtained with the DFA model were similar to the values for the individual sediment samples, with the accuracy of the source contribution value being the poorest obtained with any of the models (MAE = 18.5%). An increase in sample size improved the accuracies of the Walling-Collins and Bayesian models, but the DFA model produced similarly inaccurate results for both the individual and grouped sediment samples. Generally, the accuracy of the Walling-Collins and Bayesian models was similar (p > 0.01), while there were significant differences (p < 0.01) between the DFA model and the other models. This study demonstrated that the Bayesian model could provide a credible estimation of sediment source contributions and has great practical potential, while the accuracy of the DFA model still requires considerable improvement.     

Suspended sediment load estimation and the problem of inadequate data sampling: a fractal view

Suspended sediment load estimation at high resolutions is an extremely difficult task, because: (1) it depends on the availability of high‐resolution water discharge and suspended sediment concentration measurements, which are often not available; (2) any errors in the measurements of these two components could significantly influence the accuracy of suspended sediment load estimation; and (3) direct measurements are very expensive. The purpose of this study is to approach this sampling problem from a new perspective of fractals (or scaling), which could provide important information on the transformation of suspended sediment load data from one scale to another. This is done by investigating the possible presence of fractal behaviour in the daily suspended sediment load data for the Mississippi River basin (at St. Louis, Missouri). The presence of fractal behaviour is investigated using five different methods, ranging from general to specific and from mono‐fractal to multi‐fractal: (1) autocorrelation function; (2) power spectrum; (3) probability distribution function; (4) box dimension; and (5) statistical moment scaling function. The results indicate the presence of multi‐fractal behaviour in the suspended sediment load data, suggesting the possibility of transformation of data from one scale to another using a multi‐dimensional model. Copyright © 2005 John Wiley & Sons, Ltd.     

Investigating mechanisms of stormflow generation by natural tracers and hydrometric data: a small catchment study in the Black Forest,Germany

The importance and interaction of various hydrological pathways and identification of runoff source areas involved in solute transport are still under considerable debate in catchment hydrology. To reveal stormflow generating areas and flow paths, hydrometric behaviour of throughfall, soil water from various depths, runoff, and respective concentrations of the environmental tracers ¹⁸O, Si, K, SO₄ and dissolved organic carbon were monitored for a 14‐week period in a steep headwater catchment in the Black Forest Mountains, Germany. Two stormflow hydrographs were selected and, based on ¹⁸O and Si, chemically separated into three flow components. Their sources were defined using mixing diagrams. Additional information about stormflow generating mechanisms was derived from recession analyses of the basin's complete 5‐year hydrograph record. By providing insight into storage properties and residence times of outflowing reservoirs of the basin, recession analysis proved to be a valuable tool in runoff model conceptualization. Its results agreed well with hydrometric and hydrochemical data. Supported by evaluation of 30 hillslope soil profiles a coherent concept of stormflow generation could be derived: whereas in many steeply sloped basins in the temperate region soil water from hillslopes appears to have an immediate effect on the shape of the stormflow hydrograph, its role at this basin is basically restricted to the recharge of the groundwater reservoir in the near‐channel area. Storm hydrograph peaks appear to be derived from a small direct runoff component supplemented by a fast delivery of baseflow from the groundwater reservoir in the valley bottom. Copyright © 2001 John Wiley & Sons, Ltd.     

Delayed delivery from the sediment factory: modeling the impact of catchment response time to tectonics on sediment flux and fluvio‐deltaic stratigraphy

The sediment flux from a catchment is driven by tectonics and climate but is moderated by the geomorphic response of the landscape system to changes in these two boundary conditions. Consequently, catchment response time and the non‐linear behavior of landscapes in response to boundary condition change control the downstream propagation of climatic or tectonic perturbations from catchments to neighboring basins. In order to investigate the impact of catchment response time on sediment flux, we integrated a spatially‐lumped numerical model PaCMod, with new routines simulating the evolution of landscape morphology and erosion rates under tectonic and climatic forcing. We subsequently applied the model to reconstruct the sediment flux from a tectonically perturbed catchment in central Italy. Finally, we coupled our model to DeltaSim, a process‐response model simulating fluvio‐deltaic stratigraphy, and investigated the impact of catchment response time on stratigraphy, using both synthetic scenarios and a real world system (Fucino Basin, central Italy). Our results demonstrate that the differential response of geomorphic elements to tectonic and climatic changes induces a complex sediment flux signal, and produces characteristic stratigraphic architectures and shoreline trajectories. Copyright © 2014 John Wiley & Sons, Ltd.