Long-term sediment yield in Crombie Reservoir catchment,Angus; and its regional significance within the Midland Valley of Scotland

Abstract

The drawdown of Crombie Reservoir in November 2001 afforded the opportunity to examine the exposed sediments trapped since impoundment in 1868. Direct measurements of infill depth enabled an isopachyte map to be produced. Gravimetric conversion using measured bulk densities and a trap efficiency term indicated a long-term catchment sediment yield of 59.1 t km^?2 year^?1. Core stratigraphy analysis indicated that sediments were dark brown/black cohesive silty-muds with multiple sandy sub-units, representing a combination of discrete flood events and previous drawdown surfaces. Dating, constrained by mineral magnetic and ¹³⁷Cs analysis, indicated that sedimentation rates have varied from 0.2 to 0.8 g cm^?2 year^?1, corresponding to a four-fold variation in catchment sediment yield (approximately 20–93 t km^?2 year^?1), most likely controlled by extensive conversion of moorland to woodland, and post-World War II agricultural expansion. The Crombie investigation is combined with other reservoir sedimentation surveys within the Midland Valley of Scotland. Area-specific sediment yields (t km^?2 year^?1) evidence a weak, though statistically significant (p > 0.05), positive correlation with catchment area (km²). The increase in area-specific yield with catchment area contradicts the decline, which is generally expected, and is taken to reflect the significance of channel erosion within water supply basins featuring mainly natural and semi-natural vegetation cover and low-intensity land management practices. With stable slopes channel erosion dominates and area-specific sediment yield increases downstream due to greater entrainment and transport potential. The high degree of scatter in the Midland Valley database reflects significant variations in the extent of land-use change and the local importance of agricultural improvements and afforestation practices.     

A mass balance approach to quantifying Pb storage and fluxes in an upland catchment of the Peak District,north‐central England

A mass balance model of the main Pb stores and fluxes for a typical organic‐rich upland catchment in the Peak District, UK, has been produced. The model, based on the Howden reservoir catchment, reveals that the majority of Pb in the catchment is stored within the soil (approximately 8·63 t km^?2). Soil Pb levels are extremely high and can only be explained as the result of centuries of atmospheric Pb deposition from surrounding urban–industrial conurbations, and mining and smelting activity within the Peak District National Park. The atmospheric Pb flux onto the Howden catchment is approximately 107 kg a^?1. The aquatic Pb flux is estimated at between 29·9 and 71·7 kg a^?1; thus, at present, catchment soils are acting as a sink for Pb pollution. The Howden reservoir acts as a secondary store for Pb eroded and leached from catchment soils, with approximately 80% re‐deposited in its sediments. It is estimated that 2·3% of the catchment soil Pb pool has been retained in the reservoir sediments over its 91 year lifespan. Although the catchment is currently acting as a Pb sink, the rate of change in the soil Pb pool is very small. Future change in climate or deposition chemistry could, however, transform catchment soils into a significant source of Pb to the aquatic environment and water supply. Copyright © 2008 John Wiley & Sons, Ltd.     

Spatial soil loss risk and reservoir siltation in semi-arid Tunisia

Abstract

Soil erosion vulnerability and extreme rainfall characteristics over the Mediterranean semi-arid region of Tunisia are crucial input for estimation of siltation rate in artificial reservoirs. A comprehensive high-resolution database on erosive rainfall, together with siltation records for 28 small reservoirs, were analysed for this region, the Tunisian Dorsal (the easternmost part of the Atlas Mountains). The general life-span of these reservoirs is only about 14 years. Depending on the soil degradation in the different catchments, the corresponding reservoirs display a wide range of soil erosion rates. The average soil loss was 14.5 t ha^?1 year^?1 but some catchments display values of up to 36.4 t ha^?1 year^?1. The maximum 15-min duration rainfall intensity was used to determine the spatial distribution of rainfall erosivity. The northwestern parts of the Tunisian Dorsal display the most extreme rainfall erosivity. Spatial erosion patterns are to some extent similar; however, they vary greatly according to their location in the “soil degradation cycle”. This cycle determines the soil particle delivery potential of the catchment. In general, the northwestern parts of the Dorsal display modest soil erosion patterns due to the already severely degraded soil structure. Here, the soil surface is often the original bedrock. However, the greatest soil erosion occurs in the mid-eastern parts of the Dorsal, which represents the “degradation front”. The latter corresponds to the area with highest erosion, which is continuously progressing westward in the Dorsal. The large variation between the erosive rainfall events and the annual soil loss rates was explained by two important factors. The first relates to the soil degradation cycle. The second factor corresponds to the degradation front with the highest soil loss rates. At present this front is located at 300 m altitude and appears to be moving along an 80-km westward path starting from the east coast. A better understanding of the above can be used to better manage soils and soil covers in the Tunisian Dorsal area and, eventually, to decrease the soil erosion and reservoir siltation risk.

Citation Jebari, S., Berndtsson, R., Bahri, A. & Boufaroua, M. (2010) Spatial soil loss risk and reservoir siltation in semi-arid Tunisia. Hydrol. Sci. J. 55(1), 121–137.     

Dynamics of soil erosion rates and controlling factors in the Northern Ethiopian Highlands – towards a sediment budget

This paper analyses the factors that control rates and extent of soil erosion processes in the 199 ha May Zegzeg catchment near Hagere Selam in the Tigray Highlands (Northern Ethiopia). This catchment, characterized by high elevations (2100–2650 m a.s.l.) and a subhorizontal structural relief, is typical for the Northern Ethiopian Highlands. Soil loss rates due to various erosion processes, as well as sediment yield rates and rates of sediment deposition within the catchment (essentially induced by recent soil conservation activities), were measured using a range of geomorphological methods. The area‐weighted average rate of soil erosion by water in the catchment, measured over four years (1998–2001), is 14·8 t ha^?1 y^?1, which accounts for 98% of the change in potential energy of the landscape. Considering these soil loss rates by water, 28% is due to gully erosion. Other geomorphic processes, such as tillage erosion and rock fragment displacement by gravity and livestock trampling, are also important, either within certain land units, or for their impact on agricultural productivity. Estimated mean sediment deposition rate within the catchment equals 9·2 t ha^?1 y^?1. Calculated sediment yield (5·6 t ha^?1 y^?1) is similar to sediment yield measured in nearby catchments. Seventy‐four percent of total soil loss by sheet and rill erosion is trapped in exclosures and behind stone bunds. The anthropogenic factor is dominant in controlling present‐day erosion processes in the Northern Ethiopian Highlands. Human activities have led to an overall increase in erosion process intensities, but, through targeted interventions, rural society is now well on the way to control and reverse the degradation processes, as can be demonstrated through the sediment budget. Copyright © 2007 John Wiley & Sons, Ltd.     

Hillslope erosion in a grassland environment: Calibration and evaluation of the SIBERIA landscape evolution model

Field measurement and modelling of soil erosion provides insights into landscape systems as well as the potential for enhanced landscape management. There are a number of field and numerical methods by which soil erosion and deposition can be quantified. Here we examine the capability of the SIBERIA landscape evolution model to quantify short-term erosion and deposition on a well-managed cattle grazing landscape on the east coast of Australia. The model is calibrated by two methods (1) a geomorphological approach using a site digital elevation model (DEM) and soil data and (2) a laboratory-scale flume. The two calibration processes resulted in similar model input parameters and estimated erosion rates of 3.1 t ha⁻¹ year⁻¹ and 4.4 t ha⁻¹ year⁻¹, respectively. These were found to closely match erosion rates estimated using the environmental tracer ¹³⁷Cs (2.7–4.8 t ha⁻¹ year⁻¹). However, erosion and deposition estimated at individual points along the hillslope was not well correlated with ¹³⁷Cs at the same position due to the temporal averaging of the model and microtopography. Sensitivity analysis showed the model was more sensitive to parameterisation than sub-DEM-scale topography. This places confidence in the model's ability to estimate erosion and deposition across an entire hillslope and catchment on decadal time scales. We also highlight the robustness and flexibility of the calibration methods.     

Assessment of soil erosion in a monsoon-dominated mountain river basin in India using RUSLE-SDR and AHP

The long-term average annual soil loss (A) and sediment yield (SY) in a tropical monsoon-dominated river basin in the southern Western Ghats, India (Muthirapuzha River Basin, MRB; area: 271.75 km²), were predicted by coupling the Revised Universal Soil Loss Equation (RUSLE) and sediment delivery ratio (SDR) models. Moreover, the study also delineated soil erosion risk zones based on the soil erosion potential index (SEPI) using the analytic hierarchy process (AHP) technique. Mean A of the basin is 14.36 t ha^?1 year^?1, while mean SY is only 3.65 t ha^?1 year^?1. Although the land use/land cover types with human interference show relatively lower A compared to natural vegetation, their higher SDR values reflect the significance of anthropogenic activities in accelerated soil erosion. The soil erosion risk in the MRB is strongly controlled by slope, land use/land cover and relative relief, compared to geomorphology, drainage density, stream frequency and lineament frequency.     

Seasonal patterns of suspended sediment load and erosion-transport assessment in a Mediterranean basin

ABSTRACT

To assess seasonal patterns of suspended sediment load and its erosion–transport interactions, 17 years of river monitoring data from the Isser River Basin (northwest Algeria) were studied, considering continuous and event-scale approaches. The results show significant differences in sediment yield and transport processes between dry and wet periods. A rate of 8 t ha^?1 year^?1 was estimated from continuous analysis, with values of 4.3 and 13 t ha^?1 year^?1 for wet and dry periods, respectively. Estimates of soil delivery ratio pointed to higher values during dry periods and the dominance of hillslope erosion processes. At the event scale, the hysteresis loops confirmed these seasonal patterns in transport dynamics. The calibration of the MUSLE model highlighted the severity of rainfall during the dry period. These results emphasize the importance of seasonality in erosion and transport processes with special relevance in terms of climate change predictions.     

Assessment of sediment yield in a small karst catchment by using 137Cs tracer technique

There is very thin soil layer in karst rocky desertification areas in Southwest China,sediment deposition and sediment yield in the karst area affects the development of vegetation greatly.In the present study,the ¹³⁷Cs technique was used to assess the rate of sediment deposition and sediment yield in a small karst catchment.The ¹³⁷Cs inventory within the depression varied between 800 m^-2 and 2,200 Bq m^-2,with the mean value of 1,500.1 Bq m^-2.The ¹³⁷Cs reference inventory at a nearby reference site was 805.9 Bq m^-2.It could be inferred to that sediment deposition had occurred in the catchment.The mean depth of sediments deposition in the depression was 6 cm and the deposition rate was approximately 0.13 cm yr^-1.The analysis of the topographic characteristics of the catchment revealed that the sediment deposition occurred mainly at the lower part of the small catchment.Although,there was a sinkhole in the depression,little sediment had drained out with runoff through the sinkhole,because the local people built ridges around the sinkholes for storing water.According to this,sediment yield rate in the small catchment was estimated to be approximately 19.25 to 27.5 t km^-2 yr^-1,and the extremely low sediment yield was maybe the main obstacle to vegetation restoration in karst rocky desertification areas.     

Sediment mobilization study on Cretaceous,Tertiary and Quaternary lithological formations of an external Rif catchment,Morocco

ABSTRACT

Soil erosion is a serious ecological problem in Mediterranean areas. The IntErO model based on the erosion potential method (EPM) and the modified universal soil loss equation (MUSLE) have been used to assess soil erosion in several basins. This study aimed to assess and evaluate the effectiveness of these methods for evaluating sediment production and deposition rates in the Arbaa Ayacha basin, Morocco, in order to estimate sediment fluxes on a catchment scale. Our findings suggest that the basin is strongly exposed to erosion owing to geological formations, slope and land use, with average losses of about 28.4 t ha^?1 year^?1. Erosion processes were evaluated at the erosion production (Eocene marly formations) and sedimentation zones (Quaternary terraces). The results of these models may be useful to address soil and water management in this region and to assess the impact of a river dam that will be built in the basin.     

Blanket peat erosion and sediment yield in an upland reservoir catchment in the southern Pennines,UK

This paper investigates temporal variations in fluxes of peat and other sediment in the catchment of March Haigh Reservoir, West Yorkshire. Long‐term estimates of sediment yield were derived from a study of reservoir sediments. Magnetic properties were used to correlate ten cores to a master profile dated using ²¹⁰Pb and ¹³⁷Cs. A ¹⁴C date suggests that most of the organic component of the sediment is allochthonous and derived from peat eroded from the catchment. Organic sediment yields suggest low catchment erosion rates between 1838 and 1963. Blanket peat erosion increased significantly after 1963, and peaked between 1976 and 1984. Estimates of total sediment yield range between 2 and 28 t km^?2 a^?1. These yields are significantly lower than those from some previous studies examining reservoir sedimentation in other blanket peat‐covered catchments. The low yield estimates may be due to relatively low rates of erosion in the basin, but may also be partly explained by maintenance of silt traps during the early life of the reservoir and removal of sediment by scouring. Sedimentation within the reservoir is spatially variable, and bathymetry and sediment source appear to be the dominant controls on sedimentation patterns within the reservoir. Copyright © 2005 John Wiley & Sons, Ltd.     

Spatial simulation of forest road effects on hydrology and soil erosion after a wildfire

Post-fire catchment and water utility managers throughout the world use predictive models to estimate potential erosion risks to aid in evaluating downstream impacts of increased runoff and erosion, and to target critical areas within a fire for applying mitigation practices. Erosion prediction can be complicated by forest road networks. Using novel GIS technology and soil erosion modelling, this study evaluated the effect of roads on surface runoff, erosion and sediment yields following a wildfire and determined that the predictive models were providing reasonable results. The GeoWEPP model was used to simulate onsite erosion and offsite sediment delivery before and after fire disturbance using a 2-m resolution DEM as the terrain layer. Erosion rates in excess of 4 Mg ha⁻¹ year⁻¹ were predicted mainly from steep moderate and high severity burn areas. Roads influenced surface runoff flow path distributions and sub-catchment delineations, affecting the spatial distribution of sediment detachment and transport. Roads tended to reduce estimated erosion on slopes below the roads but increases in erosion rates were estimated for road fillslopes. Estimated deposition amounts on roads and in sediment basins were similar to measured amounts. The results confirm that road prisms, culverts and road ditches influence sedimentation processes after wildfire, and they present opportunities to detain eroded sediments.     

Sediment production in large gullies of the Mediterranean area (NE Spain) from high‐resolution digital elevation models and geographical information systems analysis

Recent studies in the Mediterranean area have shown gully erosion to have a very significant contribution to total soil loss. In the Penedès vineyard region (NE Spain), between 15 and 27% of the land is affected by large gullies and gully‐wall retreat seems to be an ongoing process. Multi‐date digital elevation model (DEM) analysis has allowed computation of sediment production by gully erosion, showing that the sediment production rates are very high by the, up‐to‐date, usual global standards. Here, we present a study carried out using large‐scale multi‐date (1975 and 1995) aerial photographs (1 : 5000 and 1 : 7000) to monitor sediment yield caused by large gullies in the Penedès region (NE Spain). High‐resolution DEMs (1 m grid) were derived and analysed by means of geographical information systems techniques to determine the gully erosion rates. Rainfall characteristics within the same study period were also analysed in order to correlate with the soil loss produced. Mass movement was the main process contributing to total sediment production. This process could have been favoured by rainfalls recorded during the period: 58% of the events were of an erosive character and showed high kinetic energy and erosivity. A sediment production rate of 846 ± 40 Mg ha^?1 year^?1, a sediment deposition rate of 270 ± 18 Mg ha^?1 year^?1 and a sediment delivery ratio of 68·1% were computed for a gully area of 0·10 km². The average net erosion within the study period (1975–95) was 576 ± 58 Mg ha^?1 year^?1. In comparison with other methods, the proposed method also includes sediment produced by processes other than only overland flow, i.e. downcutting, headcutting, and mass movements and bank erosion. Copyright © 2003 John Wiley & Sons, Ltd.     

Long‐term sediment yield from a small catchment in southern Brazil affected by land use and soil management changes

Sediments produced from eroding cultivated land can cause on‐site and off‐site effects that cause considerable economic and social impacts. Despite the importance of soil conservation practices (SCP) for the control of soil erosion and improvements in soil hydrological functions, limited information is available regarding the effects of SCP on sediment yield (SY) at the catchment scale. This study aimed to investigate the long‐term relationships between SY and land use, soil management, and rainfall in a small catchment. To determine the effects of anthropogenic and climatic factors on SY, rainfall, streamflow, and suspended sediment concentration were monitored at 10‐min intervals for 14 years (2002–2016), and the land use and soil management changes were surveyed annually. Using a statistical procedure to separate the SY effects of climate, land use, and soil management, we observed pronounced temporal effects of land use and soil management changes on SY. During the first 2 years (2002–2004), the land was predominantly cultivated with tobacco under a traditional tillage system (no cover crops and ploughed soil) using animal traction. In that period, the SY reached approximately 400 t·km^?2·year^?1. From 2005 to 2009, a soil conservation programme introduced conservation tillage and winter cover crops in the catchment area, which lowered the SY to 50 t·km^?2·year^?1. In the final period (2010–2016), the SCP were partially abandoned by farmers, and reforested areas increased, resulting in an SY of 150 t·km^?2·year^?1. This study also discusses the factors associated with the failure to continue using SCP, including structural support and farmer attitudes.     

Development and testing of the Revised Morgan-Morgan-Finney (RMMF) soil erosion model under different pedological datasets

The study aims to investigate the effect of soil properties delineation on erosion modelling. To that end, the soil attributes of the Venetikos River catchment, northwestern Greece, are described using two pedological datasets, i.e. field samples and classification maps. The goal is to select the most appropriate for the accurate estimation of erosion. The Revised Morgan-Morgan-Finney (RMMF) model is developed per base map (annual or multi-annual), keeping all other parameters unchanged. Modelled sediment yield (SY) values are validated against “observed” ones, calculated utilizing the sediment rating curve methodology. Overall, the classification maps approach (164.35 t km^-2 year^?1) performed better than the soil samples one (82.97 t km^-2 year^?1), displaying higher convergence to the synthetic SY (548.9 t km^-2 year^?1). The discrepancy among approaches is attributed to the different computation methodologies (thus pedological background) used. Both approximations successfully identified the high-risk erosion areas. The same conclusions arose from the multi-annual application of the model.     

Quantification of bank erosion in a drained agricultural lowland catchment

The long‐term and current volumes of sediment exported from stream banks were calculated as potential sources of sediment in a large pond located at the catchment outlet of a small agricultural lowland basin strongly affected by anthropogenic pressure in France. Bank erosion was measured over a short period using a network of erosion pins along a small stream (1400 m long) to quantify the material exported during a single winter (2012–2013). The material exported by this same stream over the last 69 years was quantified using an original approach involving the comparison of a compilation of three‐dimensional historical stream redesign plans that date back to 1944 with the state of the banks in 2013 (differential global positioning system and LiDAR data). The results suggest that a global trend of material loss along the stream banks monitored by erosion pins, with an average erosion rate of 17.7 mm year^?1 and an average volume of exported material of 75 t km^?1. Over 69 years, this same stream exported an average of 36 t km^?1 year^?1, and the average loss of material from the banks throughout the whole catchment was estimated to be 14 t km^?1 year^?1. The contribution of bank material to the filling of the pond over the last 10 years is between 46% and 52% based on an extrapolation of erosion pin dynamics or between 27% and 30% based on the comparison of LiDAR data to the average historical profile extrapolated for the catchment. These results suggest that bank erosion represents a major source of sediment in degraded waters in traditionally understudied agricultural lowland catchments, where anthropogenic pressures are high.     

Estimation of soil erosion in the Xihanshui River Basin by using 137Cs technique

The Cesium-137 technique was used to estimate soil erosion in the Xihanshui River Basin.More than 100 samples were taken from 10 sites and 20 hillslopes with a 10cm diameter hand-operated core driller.Each sample was 60 cm long.The ¹³⁷Cs activity was analyzed by gamma spectrometry.The simplified mass balance model and the profile distribution model were used to calculate soil erosion and deposition rate.The local ¹³⁷Cs reference ranged from 1,600 to 2,402 Bq m^-2.The data shows an exponential decrease of mass concentration and amount with depth in an undisturbed soil profile.Soil erosion in the river basin is moderate or severe on cultivated land with annual erosion rates of 2,000-6,000 t km^-2yr^-1.In general,very severe or severe soil erosion occurred at the upper slope sections,moderate or severe soil erosion at the middle section,and moderate or slight soil erosion at the lower slope sections.On the slopes with natural vegetation,consisting of herbaceous and wood species,the erosion rate is much lower or not detectable.On the lower section of slopes with well-developed vegetation however,there was no soil loss,instead deposition occurred at a rate of more than 300 t km^-2 yr^-1.The slope gradient and vegetation cover affected soil erosion and deposition rates.In general,the rate of soil erosion was proportional to the slope gradient and inversely proportional to the degree of vegetative cover.     

Magnitude and processes of bank erosion at a small stream in Denmark

River banks are important sources of sediment and phosphorus to fluvial systems, and the erosion processes operating on the banks are complex and change over time. This study explores the magnitude of bank erosion on a cohesive streambank within a small channelized stream and studies the various types of erosion processes taking place. Repeat field surveys of erosion pin plots were carried out during a 4‐year period and observations were supplemented by continuous monitoring of volumetric soil water content, soil temperature, ground water level and exposure of a PEEP sensor. Bank erosion rates (17·6–30·1 mm year^?1) and total P content on the banks were relatively high, which makes the bank an important source of sediment and phosphorus to the stream, and it was estimated that 0·27 kg P_tot year^?1 ha^?1 may potentially be supplied to the stream from the banks. Yearly pin erosion rates exceeding 5 cm year^?1 were mainly found at the lower parts of the bank and were associated with fluvial erosion. Negative erosion pin readings were widespread with a net advance of the bank during the monitoring period mainly attributed to subaerial processes and bank failure. It was found that dry periods characterized by low soil water content and freeze–thaw cycles during winter triggered bank failures. The great spatial variability, in combination with the temporal interaction of processes operating at different scales, requires new tools such as 3‐D topographical surveying to better capture bank erosion rates. An understanding of the processes governing bank erosion is required for riparian management using vegetational measures as root size and structure play different roles when it comes to controlling bank erosion processes. Copyright © 2010 John Wiley & Sons, Ltd.     

Modeling soil erosion using a spatially distributed model in a karst catchment of northwest Guangxi,China

Reliable assessment of the spatial distribution of soil erosion is important for making land management decisions, but it has not been thoroughly evaluated in karst geo‐environments. The objective of this study was to modify a physically based, spatially distributed erosion model, the revised Morgan, Morgan and Finney (RMMF) model, to estimate the superficial (as opposed to subsurface creep) soil erosion rates and their spatial patterns in a 1022 ha karst catchment in northwest Guangxi, China. Model parameters were calculated using local data in a raster geographic information system (GIS) framework. The cumulative runoff on each grid cell, as an input to the RMMF model for erosion computations, was computed using a combined flow algorithm that allowed for flow into multiple cells with a transfer grid considering infiltration and runoff seepage to the subsurface. The predicted spatial distributions of soil erosion rates were analyzed relative to land uses and slope zones. Results showed that the simulated effective runoff and annual soil erosion rates of hillslopes agreed well with the field observations and previous quantified redistribution rates with caesium‐137 (¹³⁷Cs). The estimated average effective runoff and annual erosion rate on hillslopes of the study catchment were 18 mm and 0.27 Mg ha^?1 yr^?1 during 2006–2007. Human disturbances played an important role in accelerating soil erosion rates with the average values ranged from 0.1 to 3.02 Mg ha^?1 yr^?1 for different land uses. The study indicated that the modified model was effective to predict superficial soil erosion rates in karst regions and the spatial distribution results could provide useful information for developing local soil and water conservation plans. Copyright © 2014 John Wiley & Sons, Ltd.     

Mercury cycling during acid rain recovery at the forested Lesní potok catchment,Czech Republic

From 2011 to 2019, mercury (Hg) stores and fluxes were studied in the small forested catchment Lesní potok (LES) in the central Czech Republic using the watershed mass balance approach together with internal measurements. Mean input fluxes of Hg via open bulk deposition, beech throughfall and spruce throughfall during the periodwere 2.9, 3.9 and 7.6 μg m⁻² year⁻¹, respectively. These values were considerably lower than corresponding deposition Hg fluxes reported in the early years of the 21st century from catchments in Germany. Current bulk precipitation inputs at unimpacted Czech mountainous sites were lower than those in Germany. The largest Hg inputs to the catchment were via litterfall, averaging 22.6 and 17.8 μg m⁻² year⁻¹ for beech and spruce stands. The average Hg input, based on the sum of mean litterfall and throughfall deposition, was 23.0 μg m⁻² year⁻¹, compared to the estimated Hg output in runoff of 0.5 μg m⁻² year⁻¹, which is low compared to other reported values. Thus, only ~2% of Hg input is exported in stream runoff. Stream water Hg was only weakly related to dissolved organic carbon (DOC) but both concentrations were positively correlated with water temperature. The estimated total soil Hg pool averaged 47.5 mg m⁻², only 4% of which was in the O-horizon. Thus Hg in the O-horizon pool represents 72 years of deposition at the current input flux and 3800 years of export at the current runoff flux. Age-dating by ¹⁴C suggested that organic soil contains Hg from recent deposition, while mineral soil at 40–80 cm depth contained 4400-year old carbon, suggesting the soil had accumulated atmospheric Hg inputs through millennia to reach the highest soil Hg pool of the soil profile. These findings suggest that industrial era intensification of the Hg cycle is superimposed on a slower-paced Hg cycle during most of the Holocene.