On the production of cosmogenic nuclides in meteoroids by galactic protons

Abstract— A purely physical model is presented describing the depth- and size-dependence of the production of cosmogenic nuclides in meteoroids with radii up to 85 cm and in planetary surfaces by galactic cosmic ray protons. The model is based on Monte Carlo calculations of the intra- and internuclear cascades, by which depth- and size-dependent spectra of primary and secondary protons and of secondary neutrons are derived, and on experimental and theoretical thin-target cross sections of the underlying nuclear reactions. Model calculations are presented for production rates of ⁵³Mn, ²⁶Al, ²²Ne, and ²¹Ne in H- and L-chondrites and of ⁵³Mn and ²⁶Al in lunar surface material and compared with experimental data. From the analysis of ⁵³Mn and ²⁶Al in the Apollo 15 lunar drill core and in the L-chondrite Knyahinya GCR p-spectra and integral particle fluxes at 1 A.U. and in the meteoroid orbits averaged over the last 10 Ma are derived. An analysis of experimental depth profiles in four H- and L-chondrites demonstrates, that the new model is well capable of describing depth- and size-dependences of production rates of cosmogenic nuclides. Moreover, it is possible to determine exposure ages for these meteorites on the basis of the theoretical ²¹Ne production rates. The model calculations further explain the depth- and size-dependence of ²²Ne/²¹Ne-ratios and the dependences on these ratios of ²¹Ne, ²⁶Al and ⁵³Mn production rates. The future requirements for model calculations of cosmogenic nuclide production rates in extraterrestrial matter are outlined.     

Cosmogenic nuclides in the Brenham pallasite

Abstract— Cosmic‐ray‐produced (cosmogenic) nuclides were studied in fragments of the Brenham pallasite, a large stony iron meteorite. The contents of light noble gases (He, Ne, and Ar) and long‐lived radionuclides (¹⁰Be, ²⁶Al, ³⁶Cl, and ⁵³Mn), produced by nuclear reactions with cosmic rays, were measured in the separated metal and olivine phases from numerous samples representing a wide range of shielding conditions in the meteoroid. The distribution of cosmogenic nuclide concentrations in the metal follows patterns similar to that observed in large iron meteorites. Shielding effects were estimated from the relative proportions of low‐ and high‐energy reaction products. The production rates varied, from surface to interior, by a factor of more than several hundred. The ³⁶Cl‐³⁶Ar cosmic‐ray exposure age of Brenham is 156 ± 8 Myr. This determination is based on a multiple nuclide approach that utilizes cosmogenic nuclide pairs. This approach not only yields a “shielding independent” exposure age but also demonstrates that the production of cosmogenic nuclides occurred in a single stage. The depth profiles of ¹⁰Be in the stone phase and ⁵³Mn in the metal phase are shown superimposed on corresponding profiles from the Apollo 15 long drill core. Surprisingly low abundances of lithophile elements, such as K, U, and Th, provided a unique opportunity to examine the production systematics of those nuclides whose inventories typically have significant contributions from non‐cosmogenic sources, particularly radiogenic contributions. The U and Th contents of the olivine samples are extremely low, allowing detection of cosmogenic ⁴He production from oxygen, magnesium, silicon, and iron.     

Beryllium-10 and aluminum-26 in individual cosmic spherules from Antarctica

Abstract— We present data for the cosmogenic nuclides ¹⁰Be and ²⁶Al in a suite of 24 extraterrestrial spherules, collected from Antarctic moraines and deep sea sediments. All of the 10 large spherules collected in glacial till at Lewis Cliff are extraterrestrial. As in earlier work, the great majority of particles show prominent solar cosmic-ray (SCR) production of ²⁶Al, indicating bombardment ages on the order of 10⁶ years or even longer. These long ages are in direct contradiction to model ages for small particles in the inner Solar System and may require reconsideration of models of small particle lifetimes. A small fraction of the particles so far measured (6/42) possess cosmogenic radionuclide patterns consistent with predictions for meteoroid spall droplets. We believe that most of the spherules were bombarded in space primarily as bodies not much larger than their present size. The content of in situ produced ¹⁰Be and ²⁶Al in quartz pebbles in the same moraine suggests that these spherules may have on average a significant terrestrial age.     

Allan Hills 88019: An Antarctic H-chondrite with a very long terrestrial age

Abstract— We have measured the concentrations of the cosmogenic radionuclides ¹⁰Be, ²⁶Al and ³⁶Cl (half-lives 1.51 Ma, 716 ka, and 300 ka, respectively) in two different laboratories by accelerator mass spectrometry (AMS) techniques, as well as concentrations and isotopic compositions of stable He, Ne and Ar in the Antarctic H-chondrite Allan Hills (ALH) 88019. In addition, nuclear track densities were measured. From these results, it is concluded that the meteoroid ALH 88019 had a preatmospheric radius of (20 ± 5) cm and a shielding depth for the analyzed samples of between 4 and 8 cm. Using calculated and experimentally determined production rates of cosmogenic nuclides, an exposure age of ～40 Ma is obtained from cosmogenic ²¹Ne and ³⁸Ar. The extremely low concentrations of radionuclides are explained by a very long terrestrial age for this meteorite of 2 ± 0.4 Ma. A similarly long terrestrial age was found so far only for the Antarctic L-chondrite Lewis Cliff (LEW) 86360. Such long ages establish one boundary condition for the history of meteorites in Antarctica.     

Calibrating a physical model based on Geant4 to calculate cosmogenic nuclide production rates on lunar surface

A physical model based on the open‐source toolkit Geant4 for production rates of cosmogenic nuclei on the lunar surface is proposed and calibrated. The fluxes of proton and neutron beneath the lunar surface are obtained by simulating the physical processes between the cosmic‐ray particles and the lunar surface material. By combining the experimental proton cross sections and the a posteriori neutron cross sections, we calculate the production rate depth profiles of long‐lived nuclei (¹⁰Be, ¹⁴C, ²⁶Al, ³⁶Cl, and ⁵³Mn). Through comparing experimental and theoretical data for these nuclei, we find that for all the selected nuclei, experimental and theoretical production rate depth profiles agree well with each other by introducing a single normalization factor. It means that the physical model based on Geant4 can also reproduce the depth profiles of cosmogenic nuclei, and that this model can be used by everyone worldwide. In addition, we predict the production rates of three stable nuclei (²¹Ne, ²²Ne, and ³⁸Ar).     

Cosmic‐ray exposure ages of pallasites

We analyzed cosmogenic nuclides in metal and/or silicate (primarily olivine) separated from the main‐group pallasites Admire, Ahumada, Albin, Brahin, Brenham, Esquel, Finmarken, Glorieta Mountain, Huckitta, Imilac, Krasnojarsk, Marjalahti, Molong, Seymchan, South Bend, Springwater, and Thiel Mountains and from Eagle Station. The metal separates contained an olivine fraction which although small, <1 wt% in most cases, nonetheless contributes significantly to the budgets of some nuclides (e.g., up to 35% for ²¹Ne and ²⁶Al). A correction for olivine is therefore essential and was made using model calculations and/or empirical relations for the production rates of cosmogenic nuclides in iron meteoroids and/or measured elemental concentrations. Cosmic‐ray exposure (CRE) ages for the metal phases of the main‐group pallasites range from 7 to 180 Ma, but many of the ages cluster around a central peak near 100 Ma. These CRE ages suggest that the parent body of the main‐group pallasites underwent a major break‐up that produced most of the meteorites analyzed. The CRE age distribution for the pallasites overlaps only a small fraction of the distribution for the IIIAB iron meteorites. Most pallasites and IIIAB irons originated in different collisions, probably on different parent bodies; a few IIIABs and pallasites may have come out of the same collision but a firm conclusion requires further study. CRE ages calculated from noble gas and radionuclide data of the metal fraction are higher on average than the ²¹Ne exposure ages obtained for the olivine samples. As the metal and olivine fractions were taken in most cases from different specimens, the depth‐dependency of the production rate ratio ¹⁰Be/²¹Ne in metal, not accounted for in our calculations, may explain the difference.     

Cosmogenic activation in germanium and copper for rare event searches

Experiments looking for rare events like the direct detection of dark matter particles or the nuclear Double Beta Decay are operated in deep underground locations, to suppress or very effectively reduce the effect of cosmic rays; but cosmogenic activation produced at sea level in detectors and other materials can become a serious hazard for them. Copper and germanium are very frequently used in this kind of experiments requiring an ultra-low radioactive background and therefore have been chosen as activation targets in this work. First, the excitation functions for relevant induced long-lived radioactive isotopes have been estimated; special care has been taken in using those calculations giving the best agreement with measured production cross-sections and in distinguishing production by neutrons or by protons when relevant and possible. Then, the corresponding rates of production of the nuclides in natural and enriched (86% ⁷⁶Ge and 14% ⁷⁴Ge) germanium and copper have been evaluated considering two different cosmic ray spectra. Comparison of the obtained activation yields at surface with all the known previous results (based either on calculations or experiments) has allowed to draw conclusions on the general methodology for evaluating cosmogenic activation.     

Cosmogenic nuclides in core samples of the Chico L6 chondrite: Evidence for irradiation under high shielding

Abstract— Core samples were obtained from various locations of the ～ 105-kg Chico, NM, L6 chondrite in order to study the effects of large shielding on the production rates of cosmic-ray-produced nuclides. Relations between measured abundances of cosmogenic nuclides (¹⁰Be, ²⁶Al, and stable isotopes of He, Ne, and Ar) and the cosmogenic ²²Ne/²¹Ne ratio were determined and compared with recent model predictions of production rates. The measured ²²Ne/²¹Ne ratios (1.06-1.08) and significant variations observed in concentrations of cosmogenic ²¹Ne and ³He suggest an ～40-cm shielding gradient across Chico and irradiation within a large object (> 100-cm radius). Noble gas data indicate that Chico experienced greater shielding than chondrites Knyahinya or Keyes and similar to Jilin. Values of ¹⁰Be (average = 20.7 dpm/kg) and ²⁶Al (average = 71.1 dpm/kg) are nearly constant, however, and show no correlation with either ²²Ne/²¹Ne or ²¹Ne. Activities of ¹⁰Be and ²⁶Al suggest irradiation in a smaller object (～40–80 cm radius). The ²⁶Al activity and the ²⁶Al/¹⁰Be ratio (average value = 3.42) are both significantly larger than values for most other chondrites. These results could indicate a two-stage irradiation with t₁ ～ 104 Ma and t₂ ～ 4 Ma and a second-stage body the size of Knyahinya. The single stage, ¹⁰Be/²¹Ne exposure age for Chico is 65 Ma. The ²²Ne/²¹Ne ratio apparently becomes insensitive to shielding for objects the size of Chico. No substantial evidence exists for chondrites with ²²Ne/²¹Ne ratios significantly less than ～ 1.055.     

Energetic proton irradiation history of the howardite parent body regolith and implications for ancient solar activity

Abstract— Previous studies have shown that the Kapoeta howardite, as well as several other meteorites, contains excess concentrations of cosmogenic Ne in the darkened, solar-irradiated phase compared to the light, non-irradiated phase. The two explanations offered for the nuclear production of these Ne excesses in the parent body regolith are either from galactic cosmic-ray proton (GCR) irradiation or from a greatly enhanced flux of energetic solar “cosmic-ray” protons (SCR), as compared to the recent solar flux. Combining new isotopic data we obtained on acid-etched, separated feldspar from Kapoeta light and dark phases with literature data, we show that the cosmogenic ²¹Ne/²²Ne ratio of light phase feldspar (0.80) is consistent with only GCR irradiation in space for ～3 Ma. However, the ²¹Ne/²²Ne ratio (0.68) derived for irradiation of dark phase feldspar in the Kapoeta regolith indicates that cosmogenic Ne was produced in roughly equal proportions from galactic and solar protons. Considering a simple model of an immature Kapoeta parent body regolith, the duration of this early galactic exposure was only ～3–6 Ma, which would be an upper limit to the solar exposure time of individual grains. Concentrations of cosmogenic ²¹Ne in pyroxene separates and of cosmogenic ¹²⁶Xe in both feldspar and pyroxene are consistent with this interpretation. The near-surface irradiation time of individual grains in the Kapoeta regolith probably varied considerably due to regolith mixing to an average GCR irradiation depth of ～10 cm. Because of the very different depth scales for production of solar ～Fe tracks, SCR Ne, and GCR Ne, the actual regolith exposure times for average grains probably differed correspondingly. However, both the SCR ²¹Ne and solar track ages appear to be longer because of enhanced production by early solar activity. The SCR/GCR production ratio of ²¹Ne inferred from the Kapoeta data is larger by a at least a factor of 10 and possibly as much as a factor of ～50 compared to recent solar particle fluxes. Thus, this study indicates that our early Sun was much more active and emitted a substantially higher flux of energetic (>10 MeV/nucleon) protons.     

Interior textures,chemical compositions,and noble gas signatures of Antarctic cosmic spherules: Possible sources of spherules with long exposure ages

Abstract– The interior texture and chemical and noble gas composition of 99 cosmic spherules collected from the meteorite ice field around the Yamato Mountains in Antarctica were investigated. Their textures were used to classify the spherules into six different types reflecting the degree of heating: 13 were cryptocrystalline, 40 were barred olivine, 3 were porphyritic A, 24 were porphyritic B, 9 were porphyritic C, and 10 were partially melted spherules. While a correlation exists between the type of spherule and its noble gas content, there is no significant correlation between its chemical composition and noble gas content. Fifteen of the spherules still had detectable amounts of extraterrestrial He, and the majority of them had ³He/⁴He ratios that were close to that of solar wind (SW). The Ne isotopic composition of 28 of the spherules clustered between implantation‐fractionated SW and air. Extraterrestrial Ar, confirmed to be present because it had a ⁴⁰Ar/³⁶Ar ratio lower than that of terrestrial atmosphere, was found in 35 of the spherules. An enigmatic spherule, labeled M240410, had an extremely high concentration of cosmogenic nuclides. Assuming 4π exposure to galactic and solar cosmic rays as a micrometeoroid and no exposure on the parent body, the cosmic‐ray exposure (CRE) age of 393 Myr could be computed using cosmogenic ²¹Ne. Under these model assumptions, the inferred age suggests that the particle might have been an Edgeworth‐Kuiper Belt object. Alternatively, if exposure near the surface of its parent body was dominant, the CRE age of 382 Myr can be estimated from the cosmogenic ³⁸Ar using the production rate of the 2π exposure geometry, and implies that the particle may have originated in the mature regolith of an asteroid.     

The orbit and exposure history of the Piplia Kalan eucrite

Abstract— Cosmogenic radionuclides, particle tracks and rare gases have been measured in two fragments of the Piplia Kalan eucrite that fell in Rajasthan, India on 1996 June 20. The cosmic-ray exposure age of the meteorite is calculated to be 23 Ma, which is similar to ages of some other eucrites. The track density in feldspars and pyroxenes varies between 0.2 × 10⁶ to ～4.5 × 10⁶ cm^?2. The mass ablation of the meteorite, based on the distribution of track density in near-surface samples of the two fragments, is calculated to be ～75%, which corresponds to an entry velocity of ～17 km/s. The orbital parameters of the eucrite have been computed from the radiant of the meteor trail and the geocentric velocity. The best estimates are a = 2.47 AU, e = 0.62 and i = 7.54°, which is similar to the orbital elements of other meteorites, most of which have been inferred to originate within 2.6 AU of the Sun. The activity of the radionuclide ²⁶Al agrees with the expected production rate; whereas the shortlived radionuclides ²²Na, ⁵⁴Mn, ⁴⁶Sc etc. have levels that are consistent with the galactic cosmic-ray fluxes that are expected during the solar minimum period before the time of fall. All the cosmogenic effects (i.e., radio- and stable- nuclides and particle tracks) are consistent with the meteoroid having had a simple, one-stage exposure history in interplanetary space. Lower radio genic ages of U, Th-He (0.7 Ga) and K-Ar (3.6 Ga) indicate severe losses of ⁴He and ⁴⁰Ar, as observed in most eucrites. A Pu-Xe age, concordant with Angra dos Reis, shows that Piplia belongs to the “old” eucrite group.     

Cosmogenic effects in Mbale,L5/6 chondrite

Abstract— Measurements of particle tracks, cosmogenic radionuclides, and rare gas isotopes in Mbale indicate that the meteoroid had a simple, one-stage exposure for 30.2 Ma in interplanetary space. On the basis of the measured track production rates and ⁶⁰Co and ²⁶Al activities, the meteoroid is estimated to be a sphere with a radius of ～36 cm. The activities of several cosmogenic radionuclides (i.e., ⁵⁷Co, ⁵⁴Mn, ²²Na, ⁴⁴Ti, and ²⁶Al) in two fragments having different shielding, as estimated by their track density and ⁶⁰Co activity, provide the depth variation in their production rates. Cobalt-57, ⁵⁴Mn and ²²Na activities agree with the production that is expected around the maximum of the solar cycle 22 as calculated from the Sunspot numbers. The U, Th-⁴He and K-⁴⁰Ar ages are measured to be 0.54 Ga indicating a late thermal event which is in agreement with the thermal history of some other L group chondrites. The trapped N has δ¹⁵N of ?57 ± 4%o, which is much lighter than the average L-group chondrite value; this indicates the presence of an isotopically anomalous light N component.     

Simulation of the interaction of galactic cosmic‐ray protons with meteoroids: On the production of radionuclides in thick gabbro and iron targets irradiated isotropically with 1.6 GeV protons

Abstract— Thick spherical targets made of gabbro (R = 25 cm) and of steel (R = 10 cm) were irradiated isotropically with 1.6 GeV protons at the Saturne synchrotron at Laboratoire National Saturne (LNS)/CEN Saclay in order to simulate the interaction in space of galactic cosmic‐ray (GCR) protons with stony and iron meteoroids. Proton fluences of 1.32 × 10¹⁴ cm^?2 and 2.45 × 10¹⁴ cm^?2 were received by the gabbro and iron sphere, respectively, which corresponds to cosmic‐ray exposure ages of about 1.6 and 3.0 Ma. Both artificial meteoroids contained large numbers of high‐purity target foils of up to 28 elements at different depths. In these individual target foils, elementary production rates of radionuclides and rare gas isotopes were measured by x‐ and γ‐spectrometry, by low‐level counting, accelerator mass spectrometry (AMS), and by conventional rare gas mass spectrometry. Also samples of the gabbro itself were analyzed. Up to now, for each of the experiments, ～500 target‐product combinations were investigated of which the results for radionuclides are presented here. The experimental production rates show a wide range of depth profiles reflecting the differences between low‐, medium‐, and high‐energy products. The influence of the stony and iron matrices on the production of secondary particles and on particle transport, in general, and consequently on the production rates is clearly exhibited by the phenomenology of the production rates as well as by a detailed theoretical analysis. Theoretical production rates were calculated in an a priori way by folding depth‐dependent spectra of primary and secondary protons and secondary neutrons calculated by Monte Carlo techniques with the excitation functions of the underlying nuclear reactions. Discrepancies of up to a factor of 2 between the experimental and a priori calculated depth profiles are attributed to the poor quality of the mostly theoretical neutron excitation functions. Improved neutron excitation functions were obtained by least‐squares deconvolution techniques from experimental thick‐target production rates of up to five thick‐target experiments in which isotropic irradiations were performed. A posteriori calculations using the adjusted neutron cross sections describe the measured depth profiles of all these simulation experiments within 9%. The thus validated model calculations provide a basis for reliable physical model calculations of the production rates of cosmogenic nuclides in stony and iron meteorites as well as in lunar samples and terrestrial materials.     

New model calculations for the production rates of cosmogenic nuclides in iron meteorites

Abstract— Here we present the first purely physical model for cosmogenic production rates in iron meteorites with radii from 5 cm to 120 cm and for the outermost 1.3 m of an object having a radius of 10 m. The calculations are based on our current best knowledge of the particle spectra and the cross sections for the relevant nuclear reactions. The model usually describes the production rates for cosmogenic radionuclides within their uncertainties; exceptions are ⁵³Mn and ⁶⁰Fe, possibly due to normalization problems. When an average S content of about 1 ± 0.5% is assumed for Grant and Carbo samples, which is consistent with our earlier study, the model predictions for ³He, ²¹Ne, and ³⁸Ar are in agreement. For ⁴He the model has to be adjusted by 24%, possibly a result of our rather crude approximation for the primary galactic α particles. For reasons not yet understood the modeled ³⁶Ar/³⁸Ar ratio is about 30–40% higher than the ratio typically measured in iron meteorites. Currently, the only reasonable explanation for this discrepancy is the lack of experimentally determined neutron induced cross sections and therefore the uncertainties of the model itself. However, the new model predictions, though not yet perfect, enable determining the radius of the meteoroid, the exposure age, the sulphur content of the studied sample as well as the terrestrial residence time. The determination of exposure ages is of special interest because of the still open question whether the GCR was constant over long time scales. Therefore we will discuss in detail the differences between exposure ages determined with different cosmogenic nuclides. With the new model we can calculate exposure ages that are based on the production rates (cm³STP/(gMa)) of noble gases only. These exposure ages, referred to as noble gas exposure ages or simply ^3,4He, ²¹Ne, or ^36,38Ar ages, are calculated assuming the current GCR flux. Besides calculating noble gas ages we were also able to improve the ⁴¹K‐⁴⁰K‐and the ³⁶Cl‐³⁶Ar dating methods with the new model. Note that we distinguish between ³⁶Ar ages (calculated via ³⁶Ar production rates only) and ³⁶Cl‐³⁶Ar ages. Exposure ages for Grant and Carbo, calculated with the revised ⁴¹K‐⁴⁰K method, are 628 ± 30 Ma and 841 ± 19 Ma, respectively. For Grant this is equal to the ages obtained using ³He, ²¹Ne, and ³⁸Ar but higher than the 3⁶Ar‐ and ³⁶Cl‐³⁶Ar ages by ?30%. For Carbo the ⁴¹K‐⁴⁰K age is ?40% lower than the ages obtained using ³He, ²¹Ne, and ³⁸Ar but equal to the ³⁶Ar age. These differences can either be explained by our still insufficient knowledge of the neutron‐induced cross sections or by a long‐term variation of the GCR.     

Noble gases in enstatite chondrites I: Exposure ages,pairing, and weathering effects

Abstract— Cosmic‐ray exposure ages calculated from cosmogenic noble gas nuclides are reported for 57 enstatite (E) chondrites, 43 of them were measured for the first time. With a total of 62 individual E chondrites (literature and this data, corrected for pairing) the observed spectrum of ages ranges between 0.07 and 66 Ma. Three clusters seem to develop at about 3.5, 8, and 25 Ma, respectively. Since the uncertainty of ages is estimated to be ～20% (in contrast to 10 to 15% for ordinary chondrites) and the number of examined samples is still comparatively small, these peaks have to be confirmed by more measurements. Regarding the two subgroups, EH and EL chondrites, no systematic trend is apparent in the distribution of cosmic‐ray exposure ages. Several E chondrites yield significantly lower ³⁸Ar ages compared to those calculated from cosmogenic ³He and ²¹Ne. For these E chondrites, we suggest a reduction of cosmogenic ³⁸Ar as a result of weathering. In order to prove the possible influence of terrestrial alteration on the cosmogenic noble gas record of E‐chondritic material, we simulated terrestrial weathering in an experiment of 12 weeks duration. The treatment showed that a significant amount of cosmogenic ³⁸Ar is lost on Earth by the influence of water.     

Monte Carlo simulation of GCR neutron capture production of cosmogenic nuclides in stony meteorites and lunar surface

Abstract— A purely physical model based on a Monte Carlo simulation of galactic cosmic ray (GCR) particle interaction with meteoroids is used to investigate neutron interactions down to thermal energies. Experimental and/or evaluated excitation functions are used to calculate neutron capture production rates as a function of the size of the meteoroid and the depth below its surface. Presented are the depth profiles of cosmogenic radionuclides ³⁶Cl, ⁴¹Ca, ⁶⁰Co, ⁵⁹Ni, and ¹²⁹I for meteoroid radii from 10 cm up to 500 cm and a 2π irradiation. Effects of bulk chemical composition on n‐capture processes are studied and discussed for various chondritic and lunar compositions. The mean GCR particle flux over the last 300 ka was determined from the comparison of simulations with measured ⁴¹Ca activities in the Apollo 15 drill core. The determined value significantly differs from that obtained using equivalent models of spallation residue production.     

Exposure history of the Sutter's Mill carbonaceous chondrite

The Sutter's Mill (SM) carbonaceous chondrite fell in California on April 22, 2012. The cosmogenic radionuclide data indicate that Sutter's Mill was exposed to cosmic rays for 0.082 ± 0.008 Myr, which is one of the shortest ages for C chondrites, but overlaps with a small cluster at approximately 0.1 Myr. The age is significantly longer than proposed ages that were obtained from cosmogenic noble gas concentrations, which have large uncertainties due to trapped noble gas corrections. The presence of neutron‐capture ⁶⁰Co and ³⁶Cl in SM indicates a minimum preatmospheric radius of approximately 50 cm, and is consistent with a radius of 1–2 m, as derived from the fireball observations. Although a large preatmospheric size was proposed, one fragment (SM18) contains solar cosmic ray–produced short‐lived radionuclides, such as ⁵⁶Co and ⁵¹Cr. This implies that this specimen was less than 2 cm from the preatmospheric surface of Sutter's Mill. Although this conclusion seems surprising, it is consistent with the observation that the meteoroid fragmented high in the atmosphere. The presence of SCR‐produced nuclides is consistent with the high SCR fluxes observed during the last few months before the meteorite's fall, when its orbit was less than 1 AU from the Sun.     

Production of krypton and xenon isotopes in thick stony and iron targets isotropically irradiated with 1600 MeV protons

Abstract— Two spherical targets made of gabbro with a radius of 25 cm and of steel with a radius of 10 cm were irradiated isotropically with 1600 MeV protons at the SATURNE synchrotron at Laboratoire National Saturne (LNS)/CEN Saclay, in order to simulate the production of nuclides in meteorites induced by galactic cosmic‐ray protons in space. These experiments supply depth‐dependent production rate data for a wide range of radioactive and stable isotopes in up to 28 target elements. In this paper, we report results for ⁷⁸Kr, ^80–86Kr isotopes in Rb, Sr, Y and Zr and for ¹²⁴Xe, ¹²⁶Xe, ^128–132Xe, ¹³⁴Xe, ¹³⁶Xe isotopes in Ba and La. Krypton and xenon concentrations have been measured at different depths in the spheres by using conventional mass spectrometry. Based on Monte‐Carlo techniques, theoretical production rates are calculated by folding depth‐dependent spectra of primary and secondary protons and secondary neutrons with the excitation functions of the relevant nuclear reactions. The comparison of the model calculation results with experimental data in the thick target experiments performed at LNS and previously at CERN have allowed adjustments of the poorly known excitation functions of neutron‐induced reactions. Thus, for the two experiments at SATURNE, excellent agreement is obtained between experimental and calculated production rates for most Kr and Xe isotopes in all investigated target elements. Only Xe production in Ba in the gabbro is underestimated by the calculations by ?25%. This work validates the approach of the thin‐target model calculations of cosmogenic nuclide production rates in the attempt of modeling the interaction of galactic cosmic‐ray protons with stony and iron meteorites in space as well as with lunar samples.     

Cosmogenic production as a background in searching for rare physics processes

We revisit calculations of the cosmogenic production rates for several long-lived isotopes that are potential sources of background in searching for rare physics processes such as the detection of dark matter and neutrinoless double-beta decay. Using updated cosmic-ray neutron flux measurements, we use TALYS 1.0 to investigate the cosmogenic activation of stable isotopes of several detector targets and find that the cosmogenic isotopes produced inside the target materials and cryostat can result in large backgrounds for dark matter searches and neutrinoless double-beta decay. We use previously published low-background HPGe data to constrain the production of ³H on the surface and the upper limit is consistent with our calculation. We note that cosmogenic production of several isotopes in various targets can generate potential backgrounds for dark matter detection and neutrinoless double-beta decay with a massive detector, thus great care should be taken to limit and/or deal with the cosmogenic activation of the targets.     

Cosmogenic production as a background in searching for rare physics processes

We revisit calculations of the cosmogenic production rates for several long-lived isotopes that are potential sources of background in searching for rare physics processes such as the detection of dark matter and neutrinoless double-beta decay. Using updated cosmic-ray neutron flux measurements, we use TALYS 1.0 to investigate the cosmogenic activation of stable isotopes of several detector targets and find that the cosmogenic isotopes produced inside the target materials and cryostat can result in large backgrounds for dark matter searches and neutrinoless double-beta decay. We use previously published low-background HPGe data to constrain the production of ³H on the surface and the upper limit is consistent with our calculation. We note that cosmogenic production of several isotopes in various targets can generate potential backgrounds for dark matter detection and neutrinoless double-beta decay with a massive detector, thus great care should be taken to limit and/or deal with the cosmogenic activation of the targets.