中国主要城市群在灰霾污染下的近地面风场特征

利用2015-2016年全国PM2.5质量浓度站点资料及CCMP(Cross Calibrated Multi-Platform)风场再分析资料,对中国华北、长三角、珠三角以及四川盆地主要城市在PM2.5污染下的近地面风场及其影响进行统计分析.结果表明:(1)近地面风速与PM2.5质量浓度表现为负相关,低风速有利于PM...     

2007年冬季沈阳典型大气污染源PM10排放模拟

选取沈阳市区9个典型的大气污染源冬季的PM10排放浓度资料,利用MM5耦合CALPUFF对2007年12月至2008年2月沈阳城市区域气象场和排放PM10浓度分布进行月平均数值模拟.结果表明:冬季沈阳地区受高压控制,北风较强,并经过增强、减弱的过程,多呈现对大气污染物扩散不利的天气形势.高空为偏西风且风速较大时,地面和...     

日照市区PM10污染物特征及其与气象要素的关系

对2002年1月1日-2002年12月31日日照市环境监测中心提供的PM₁₀(可吸入颗粒物)日平均浓度资料和对应时段的日照市地面气象资料做了深入的分析,揭示了污染物PM₁₀变化特征及其随气象要素的变化规律。同时分析了主要污染物PM₁₀与地面风速、风向间的相关关系,发现日照市大于等于3级的PM₁₀污染日均出现在1-4月,地面风速对污染物PM₁₀浓度有一定影响,当地面风速超过5m/s时,3级及以上污染日很少出现,当地面风速超过6.5m/s时,随着风速的提高,污染物浓度呈下降趋势。污染物浓度呈明显的季节变化,冬、春季节明显高于夏、秋季节。     

Long-term size-segregated particle (PM10, PM2.5, PM1) characterization study at Melpitz -- influence of air mass inflow, weather conditions and season

Size-segregated high-volume (HV) quartz filter samples were collected daily at the Melpitz rural site in Germany for PM₁₀ (November 1992 until April 2012), and for PM_2.5 and PM₁ (January 2003 until April 2012, PM₁ sampled every sixth day). The samples were analysed for mass concentration (gravimetrically), water-soluble ions (ion-chromatography) and since 2003 for organic carbon (OC) and elemental carbon (EC) (thermography). The long-term measurements first show a decreasing trend for PM₁₀ (1993–2000) followed by a second period (2001–2011) with a mean mass concentration of about 22.4 μgm^?3 and an inter-annual variation of about?±?2.9 μgm^?3 (13% fluctuation margin). The absolute sulphate and calcium concentration (for the full period), as well as the EC concentration (time after 2003) decrease by about 50, 75 and 30% for PM₁₀, respectively. The nitrate concentration remains constant all the time. For the daily objective weather type classification (OWTC, 1993–2002) the highest PM₁₀ concentration was found for South-East (SE) and the lowest for North-West (NW) wind direction with 44 and 24 μgm^?3, respectively. These concentrations decrease for 2003–2011 in comparison to 1993–2002 by about 21% and 26%, respectively. The highest PM₁₀, PM_2.5 and PM₁ concentrations (2003–2011) were found for SE and the lowest for NW wind direction with about 34 and 17 μgm^?3 (PM₁₀), 28 and 19 μgm^?3 (PM_2.5) and 22 and 11 μgm^?3 (PM₁), respectively. The relative content of sulphate, OC and EC was the highest for SE wind direction. A differentiation into four categories for winter (Wi) and summer (Su) and air mass inflow from West (W) and East (E) was carried out. The highest PM concentrations were observed for WiE with the highest inter-annual fluctuation. In this category sulphate contents are largest. The lowest concentrations where found for SuW. The means for WiE show the strongest relative decreases, e.g. in PM₁₀ sulphate (1993–2011) and EC (2003–2011) by about 60% and 40%, respectively. Nitrate is an indicator for NO_x motor-car emissions. It shows a typical variation with maximum values in the middle of the week_, especially for air mass inflow from West. In contrast, chloride mostly originating from sea spray doesn’t show such a concentration pattern. The PM_2.5/PM₁₀ as well the PM₁/PM₁₀-ratio have the highest median (0.878 and 0.654) during WiE and the lowest (0.718 and 0.578) during SuW, respectively. For the ratio PM_2.5/PM₁₀ a slightly increasing trend was found (about 0.71 and 0.83 for 1995 and 2011, respectively). The increase is stronger in summer than in winter.     

Observed particle sizes and fluxes of Aeolian sediment in the near surface layer during sand-dust storms in the Taklamakan Desert

Monitoring, modeling and predicting the formation and movement of dust storms across the global deserts has drawn great attention in recent decades. Nevertheless, the scarcity of real-time observations of the wind-driven emission, transport and deposition of dusts has severely impeded progress in this area. In this study, we report an observational analysis of sand-dust storm samples collected at seven vertical levels from an 80-m-high flux tower located in the hinterland of the great Taklamakan Desert for ten sand-dust storm events that occurred during 2008–2010. We analyzed the vertical distribution of sandstorm particle grain sizes and horizontal sand-dust sediment fluxes from the near surface up to 80 m high in this extremely harsh but highly representative environment. The results showed that the average sandstorm grain size was in the range of 70 to 85 μm. With the natural presence of sand dunes and valleys, the horizontal dust flux appeared to increase with height within the lower surface layer, but was almost invariant above 32 m. The average flux values varied within the range of 8 to 14 kg m^?2 and the vertical distribution was dominated by the wind speed in the boundary layer. The dominant dust particle size was PM₁₀₀ and below, which on average accounted for 60–80 % of the samples collected, with 0.9–2.5 % for PM_0–2.5, 3.5–7.0 % for PM_0–10, 5.0–14.0 % for PM_0–20 and 20.0–40.0 % for PM_0–50. The observations suggested that on average the sand-dust vertical flux potential is about 0.29 kg m^?2 from the top of the 80 m tower to the upper planetary boundary layer and free atmosphere through the transport of particles smaller than PM₂₀. Some of our results differed from previous measurements from other desert surfaces and laboratory wind-dust experiments, and therefore provide valuable observations to support further improvement of modeling of sandstorms across different natural environmental conditions.     

The aerosol radiative effect on a severe haze episode in the Yangtze River Delta

Due to increased aerosol emissions and unfavorable weather conditions, severe haze events have occurred frequently in China in the last 10 years. In addition, the interaction between the boundary layer and the aerosol radiative effect may be another important factor in haze formation. To better understand the effect of this interaction, the aerosol radiative effect on a severe haze episode that took place in December 2013 was investigated by using two WRF-Chem model simulations with different aerosol configurations. The results showed that the maximal reduction of regional average surface shortwave radiation, latent heat, and sensible heat during this event were 88, 12, and 37 W m^–2, respectively. The planetary boundary layer height, daytime temperature, and wind speed dropped by 276 m, 1°C, and 0.33 m s^–1, respectively. The ventilation coefficient dropped by 8%–24% for in the central and northwestern Yangtze River Delta (YRD). The upper level of the atmosphere was warmed and the lower level was cooled, which stabilized the stratification. In a word, the dispersion ability of the atmosphere was weakened due to the aerosol radiative feedback. Additional results showed that the PM_2.5 concentration in the central and northwestern YRD increased by 6–18 μg m^–3, which is less than 15% of the average PM_2.5 concentration during the severely polluted period in this area. The vertical profile showed that the PM_2.5 and PM₁₀ concentrations increased below 950 hPa, with a maximum increase of 7 and 8 μg m^–3, respectively. Concentrations reduced between 950 and 800 hPa, however, with a maximum reduction of 3.5 and 4.5 μg m^–3, respectively. Generally, the aerosol radiative effect aggravated the level of pollution, but the effect was limited, and this haze event was mainly caused by the stagnant meteorological conditions. The interaction between the boundary layer and the aerosol radiative effect may have been less important than the large-scale static weather conditions for the formation of this haze episode.     

Factors affecting boundary-layer wind shear over the Indian Ocean during FGGE

Statistics on the vertical wind shear in the boundary layer over the Indian Ocean were examined for the causes of regional and seasonal changes. Low-level cloud motions and surface ship wind reports were used to define the vertical shear. Temperature data from the ship reports were analyzed for boundary-layer stability related to the observed shears. Smaller wind shears were found in areas of large negative air-sea temperature difference (unstable boundary layers). The thermal wind effects were very small over most of the tropical Indian Ocean. The largest factor affecting the speed shear was the strength of the wind itself. Larger speed shear was found under high wind conditions. A small reduction in the direction difference between cloud and ship observations also was found under higher speeds. The scatter of cloud-ship comparisons around the mean (dispersion) also decreased for higher wind speeds. Daily gridded cloud motion and ship wind speed data had a correlation coefficient of 0.8 with a scatter of 1.9 m s^-1 (r.m.s.) around the mean difference.     

风能资源数值模拟评估的分型方法研究

为了实现时间跨度较长(20—30年)的风能资源数值模拟评估,建立了一种新的分型方案,采用地面和探空观测资料,以风速、风向和最大混合层高度作为分型因子,针对每种类型随机抽取5%的日数进行真实算例的数值模拟。根据中国所有地区典型日的平均风能参数和30年观测平均结果的对比分析,得出以下结论:(1)中国所有分型站点挑选典型日的平均风速与30年平均风速的绝对误差均小于0.10 m/s,相对误差均低于6.50%;挑选典型日各风向频率值与30年结果的绝对误差平均值为0.28%—0.48%,风速频率绝对误差的平均值为0.09%—0.54%。(2)通过模拟区域分型站点以外探空气象站的风向频率和风速频率的对比检验发现:沿海地区风向频率绝对误差为0.27%—0.63%,风速频率绝对误差为0.14%—0.49%;内陆复杂山地风向频率绝对误差基本在0.57%以下,风速频率绝对误差为0.22%—0.60%;结果表明选取一个分型站点能够代表整个模拟区域内的风能资源特性。(3)根据沿海和内陆山地模拟区域重合范围内的探空站分型结果对比分析发现:对于模拟区域重合范围内的探空站,采用所有模拟区域分型站典型日结果加权平均后的风能参数对比误差大大低于各自模拟区域分型站点的对比误差。     

Mean wind speed profiles in the air basin of Moscow

Results of measurements of mean wind speed profiles and direction during two years in the center of the city of Moscow are presented. These measurements were performed with a Doppler acoustic profiler (sodar), which was used for continuous monitoring of the wind speed within the height range from 40 to 250–500 m. The averaged seasonal mean profiles are presented along with other observational data, including diurnal cycle parameters, wind speed and direction frequencies at chosen levels, and frequencies and duration of strong winds and calm weather.     

Using the OSPM Model on Pollutant Dispersion in an Urban Street Canyon

An observational campaign was conducted in the street canyon of Zhujiang Road in Nanjing city in 2007.Hourly mean concentrations of PM10 were measured at street and roof levels.The Operational Street Pollution Model(OSPM)street canyon dispersion model was used to calculate the street concentrations and the results were compared with the measurements.The results show that there is good agreement between measured and predicted concentrations.The correlation coecient R2 values(R2 is a measure of the correlation of the predicted and measured time series of concentrations)are 0.5319,0.8044,and 0.6630 for the scatter plots of PM10 corresponding to light wind speed conditions,higher wind speed conditions,and all wind speed conditions,respectively.PM10 concentrations tend to be smaller for the higher wind speed cases and decrease rapidly with increasing wind speed.The presentations of measured and modelled concentration dependence on wind direction show fairly good agreement.PM10 concentrations measured on the windward side are relatively smaller,compared with the corresponding results for the leeward side.This study demonstrates that it is possible to use the OSPM to model PM10 dispersion rules for an urban street canyon.     

Effect of wind vertical shear on diffusion characteristics in the mesoscale range

Using the turbulent statistical form of the vertical vortex diffusion coefficient K, in the planetary boundary layer (PBL) and Ekman spiral wind profile, the three-dimensional diffusion equation is solved by the numeri-cal method. The influences of vertical shear of both wind direction and wind speed on pollution trajectory and horizontal diffusion parameters σy are numerically analysed. The expressions of both pollution trajectory and σy, including the factor of wind shear, are obtained. The results show that the vertical shear of wind is important among all factors affecting the mesoscale dispersion. Specifically, from neutral to stable atmospheric conditions, vertical shear of wind makes greater contribution to σy than turbulence, thus it is the most important factor. In this paper, we have compared horizontal dispersion pattern with both Pasquill's dispersion pattern considering wind direction shear, and experimental data collected at 9 different sites rang-ing from 10 to 100 km, and the results show that our dispersion pattern is closer to the experimental values than Pasquill's results, and his correction to shear of wind direction is too large under the stable conditions.     

塔克拉玛干沙漠腹地贴地层风沙流结构研究

利用微梯度集沙仪在塔克拉玛干沙漠腹地塔中地区实测的2014年7—8月贴地层输沙量梯度观测资料(观测高度区间0~5 mm、5~15 mm、15~35 mm、35~85 mm),对沙尘天气过程贴地层风沙流结构进行了研究。结果表明:(1)沙尘天气(沙尘暴和扬沙)过程中,随着风速的增大,各高度层输沙量也随之增大。沙尘暴天气中,风速7.5 m·s~(-1)时,15~35 mm处的百分含量超过5~15 mm处的百分含量,风速7.5 m·s~(-1)时,15~35 mm处的百分含量达到最大,其余各高度含量变化不明显。扬沙天气中,风速8.0 m·s~(-1)时,百分含量最大值出现在35~85 mm高度处,占48.9%,风速8.0 m·s~(-1)时,大小依次为:15~35 mm(49.5%)35~85 mm(31.7%)0~5 mm(12.7%)5~15 mm(9.2%)。(2)两种天气过程中,沙粒的平均粒径在垂直高度上均呈现先减小后增大的趋势。粒径峰值均处在125~250 um,极细砂含量最高,细砂次之。与扬沙天气相比,沙尘暴天气过程中极细砂、细砂、中砂在各高度层上的含量略微下降,粉尘含量有所升高。     

基于风廓线雷达的湖北梅雨期暴雨中小尺度特征

针对2016年湖北梅雨期3次(“6·19”、“7·5”和“7·19”)暴雨过程,首先对比了汉口站探空数据与汉口、咸宁两个风廓线雷达站水平风速、风向,发现“6·19”和“7·5”过程汉口风廓线雷达站3 km以下水平风速和探空数据较为接近,而3次过程中咸宁风廓线雷达站8 km以下水平风向、风速和汉口站探空数据基本吻合。在此基础上利用风廓线雷达资料并结合常规、加密自动气象站资料,对3次过程中水平风场、平均垂直速度及其变率、水平风速垂直切变、大气折射率结构常数(C_(n)^(2))等进行分析。结果表明:(1)降水开始前西南风速明显增大,中层干冷空气入侵和地面冷池形成的中尺度偏东气流是“6·19”过程50站出现大于等于17.2 m·s^(-1)大风的主要原因,“7·5”和“7·19”过程西南急流长时间维持及1 km以下的偏东气流则是短时强降水持续时间较长的诱因;(2)梅雨期暴雨期间风廓线雷达观测的水平风速垂直切变、平均垂直速度及其变率随高度变化较小,较强上升运动区域主要集中在4 km高度以下;(3)C_(n)^(2)显示强降水发生前大气水汽含量有一增加过程,且整层水汽含量深厚,C_(n)^(2)大值区的消失对应降水结束。     

成都市PM2.5污染特征及其与地面气象要素的关系分析

为了解成都市PM_2.5污染特征及其与地面气象要素的关系,利用环境空气质量监测资料和地面气象观测资料,分析了PM_2.5质量浓度的季节、月和日变化特征,并分不同空气质量等级分析空气质量与地面气象要素的关系。结果表明：PM_2.5质量浓度具有明显的季节、月和日变化特征,且成都市区6个监测站的变化趋势比较一致;成都市相对湿度较大,地面风速较小,约62%的样本分布在相对湿度80%~100%,约85%的样本分布在地面风速0~2 m·s^-1,地面风速对成都市PM_2.5的水平输送、扩散、稀释不利;降水对PM_2.5的清除量随PM_2.5初始浓度、降雨持续时间和累积降雨量增加而增大。     

Influence of non-flat terrain and wind direction shear on canopy turbulence

We have analyzed eddy covariance data collected within open canopy to investigate the influence of non-flat terrain and wind direction shear on the canopy turbulence. The study site is located on non-flat terrain with slopes in both south-north and east-west directions. The surface elevation change is smaller than the height of roughness element such as building and tree at this site. A variety of turbulent statistics were examined as a function of wind direction in near-neutral conditions. Heterogeneous surface characteristics results in significant differences in measured turbulent statistics. Upwind trees on the flat and up-sloping terrains yield typical features of canopy turbulence while upwind elevated surface with trees yields significant wind direction shear, reduced u and w skewness, and negligible correlation between u and w. The directional dependence of turbulence statistics is due that strong wind blows more horizontally rather than following terrain, and hence combination of slope related momentum flux and canopy eddy motion decreases the magnitude of Sk _w and r _uw for the downslope flow while it enhances them for the upslope flow. Significant v skewness to the west indicates intermittent downdraft of northerly wind, possibly due to lateral shear of wind in the presence of significant wind direction shear. The effects of wind direction shear on turbulent statistics were also examined. The results showed that correlation coefficient between lateral velocities and vertical velocity show significant dependence on wind direction shear through change of lateral wind shear. Quadrant analysis shows increased outward interaction and reduced role of sweep motion for longitudinal momentum flux for the downslope flow. Multi-resolution analysis indicates that uw correlation shows peak at larger averaging time for the upslope flow than for the downslope flow, indicating that large eddy plays an active role in momentum transfer for the upslope flow. On the other hand, downslope flow shows larger velocity variances than other flows despite similar wind speed. These results suggest that non-flatness of terrain significantly influences on canopy-atmosphere exchange.     

PM10 Observed at a Meteorological Station in Beijing: Historical Trend and Implications

Inhalable particles (PM10), with aerodynamic equivalent diameters that are generally 10 micrometers or smaller, are basic pollutants in many areas, especially in northern China, and thus the pollution from PM10 inhalable particulate matter is a growing concern for public health. Independent long-term observations are necessary to evaluate the efficacy of PM10 reduction actions. Variations in the PM10 concentration from 2006 to 2017 at an observation station (NJ) in Beijing were recorded and analyzed. The average value ±1 standard deviation of daily mean PM10 concentrations was 138.8 ±96.1 μg m-3 for 1307 days (accounting for 34.7% of the total days), showing PM10 concentration exceeding the National Ambient Air Quality Standard (NAAQS) 24-h average of 150 μg m-3. Particulate concentration depended upon various meteorological conditions as also observed in this work: at low wind speed (<4 m s-1), the concentrations of PM10 revealed a downward trend with -19 μg m-3 per unit of wind speed, but when wind speed rose (>4 m s-1), the values increased by 49 μg m-3 per unit of wind speed. In Beijing, air masses from northwest China, especially from the Gobi Desert and other desert areas, had net contributions to long-range transport of natural dust, enhancing the PM10 concentrations by up to 29%. Overall, PM10 mass concentration showed a significant downward trend with -8.0 μg/m3/yr from 2006 to 2017. Although with higher fluctuations in recorded data, similar downward trends derived from the ) in 2017 still exceeded the NAAQS standard. The results showed that there is still a long way to go to reduce PM10 in Beijing.     

Effect of urbanization on the urban meteorology and air pollution in Hangzhou

Urbanization has a substantial effect on urban meteorology. It can alter the atmospheric diffusion capability in urban areas and therefore affect pollutant concentrations. To study the effects of Hangzhou’s urban development in most recent decade on its urban meteorological characteristics and pollutant diffusion, 90 weather cases were simulated, covering 9 weather types, with the Nanjing University City Air Quality Prediction System and high-resolution surface-type data and urban construction data for 2000 and 2010. The results show that the most recent decade of urban development in Hangzhou substantially affected its urban meteorology. Specifically, the average urban wind speed decreased by 1.1 m s ^?1; the average intensity of the heat island increased by 0.5°C; and the average urban relative humidity decreased by 9.7%. Based on one case for each of the nine weather types, the impact of urbanization on air pollution diffusion was investigated, revealing that the changes in the meteorological environment decreased the urban atmosphere’s diffusion capability, and therefore increased urban pollutant concentrations. For instance, the urban nitrogen oxides concentration increased by 2.1 μg m ^?3 on average; the fine particulate matter (diameter of 2.5 μm or less; PM_2.5) pollution concentration increased by 2.3 μg m ^?3 on average; in highly urbanized areas, the PM_2.5 concentration increased by 30 μg m ^?3 and average visibility decreased by 0.2 km, with a maximum decrease of 1 km; the average number of daily hours of haze increased by 0.46 h; and the haze height lifted by 100–300 m. The “self-cleaning time” of pollutants increased by an average of 1.5 h.     

Mass concentration of PM10 and PM2.5 fine-dispersed aerosol fractions in the Eastern Gobi Desert

Results are presented of monitoring measurements of the mass concentration of PM₁₀ (particles with the size of less than 10 μm) and PM_2.5 (less than 2.5 μm) fine-dispersed aerosol fractions at the Sainshand and Zamyn-Üüd stations located in the Gobi Desert of Mongolia. Revealed are the annual variations of the mass concentration of PM₁₀ and PM_2.5 fine-dispersed aerosol fractions at these stations in 2008. The maximum values of monthly mean concentration during the year were observed in May in the period of dust storms. On the days with the steady calm weather, the mass concentrations of PM₁₀ and PM_2.5 varied within 5–8 μg/m³ (PM₁₀) and 3–5 μg/m³ (PM_2.5) at the Sainshand station. During the dust storms, the maximum values of concentration exceeded 1400 μg/m³ (PM₁₀) and 380 μg/m³ (PM_2.5) that is by 28 (PM₁₀) and 15 (PM_2.5) times higher than the maximum permissible concentration for the European Union. Results are given of studying the frequency and duration of dust storms in recent 20 years (1991–2010) in the Eastern Gobi Desert.     

沙尘天气下输沙率的野外观测与分析

2014年7月—2014年8月借助风速仪、微梯度集沙仪,通过野外监测系统获取的试验数据,对塔中地区2014年7月—2014年8月沙尘天气过程中贴地层输沙率进行分析,得出:0～85 mm高度内,随着风速的增大,35～85 mm无论是绝对的输沙量还是相对的输沙量都减少。0～85 mm高度内,各层输沙率最大值均出现在风速为8 m·s-1左右,波动较为显著;最小值出现在6.5 m·s-1左右,波动不明显;沙尘天气中,输沙率最大值出现在5～15 mm高度,最小值出现在35～85 mm高度。扬沙天气中,风速9.2 m·s-1时,输沙率最大值在0～5 mm处。沙尘暴天气,拐点风速为7.5 m·s-1,7.5 m·s-1时,输沙率增加不显著,7.5 m·s-1时,输沙率增加显著。通过微梯度集沙仪获得的上述试验数据是风沙工程设计的一个极重要工程参数,具有重要的实践意义。     

武汉城市区域水陆风环流的形成与转化特征研究

大气细颗粒物PM_2.5污染引起的雾霾天气既与本地污染物排放密切有关,也受局地特殊的风场影响.本文以武汉城市区域为研究对象,分别研究了长江沿岸的江陆风环流、东湖沿岸湖陆风环流的形成与转化特征,发现江风、湖风开始时间均为07：00-08：00,一年中最大风速均能达到2 m/s左右,而春夏季江风的持续时间高于秋冬季,夏季湖风的持续时间高于春季.同时发现区域附近温度和相对湿度之间有明显的相关性,湿度变化趋势大体上跟温度变化趋势相反,且温度对相对湿度的影响存在一定的滞后性,延迟时间大约为1 h.