关于CAS FGOALS-f3-L模式中青藏高原地表温度偏差的归因分析

中国科学院全球海洋-大气-陆地耦合模式(FGOALS-f3-L)参加了耦合模式比较计划的第六阶段(CMIP6)试验,但是其对关键气候敏感地区青藏高原的地表温度的再现能力还不清楚.这项研究用再分析资料CFSR评估了FGOALS-f3-L模式对青藏高原地表温度的再现能力.结果表明,FGOALS-f3-L可以合理模拟整个高原上年平均地表温度的空间分布,但低估了整个高原上年平均地表温度.模拟的地表温度在整个高原上冬春季表现为冷偏差,夏秋季表现为暖偏差.基于地表能量平衡方程的进一步定量分析表明,地表反照率反馈(SAF)项极大地贡献了高原西部年平均,冬春季平均地表温度的冷偏差,而对高原东部是暖偏差贡献.与SAF项相比,地表感热项对地表温度偏差的贡献几乎相反,这大大抵消了SAF项引起的偏差.云辐射强迫项对高原东部的年平均和季节平均弱冷偏差有很大贡献.与高估的水蒸气含量有关的长波辐射项造成了夏秋季整个高原上大部分的暖偏差.该研究表明,提高FGOALS-f3-L中的陆面和云过程对降低高原上地表温度偏差至关重要.     

关于CAS FGOALS-f3-L模式中青藏高原地表温度偏差的归因分析（英文）

中国科学院全球海洋-大气-陆地耦合模式(FGOALS-f3-L)参加了耦合模式比较计划的第六阶段(CMIP6)试验,但是其对关键气候敏感地区青藏高原的地表温度的再现能力还不清楚.这项研究用再分析资料CFSR评估了FGOALSf3-L模式对青藏高原地表温度的再现能力.结果表明,FGOALS-f3-L可以合理模拟整个高原上年平均地表温度的空间分布,但低估了整个高原上年平均地表温度.模拟的地表温度在整个高原上冬春季表现为冷偏差,夏秋季表现为暖偏差.基于地表能量平衡方程的进一步定量分析表明,地表反照率反馈(SAF)项极大地贡献了高原西部年平均,冬春季平均地表温度的冷偏差,而对高原东部是暖偏差贡献.与SAF项相比,地表感热项对地表温度偏差的贡献几乎相反,这大大抵消了SAF项引起的偏差.云辐射强迫项对高原东部的年平均和季节平均弱冷偏差有很大贡献.与高估的水蒸气含量有关的长波辐射项造成了夏秋季整个高原上大部分的暖偏差.该研究表明,提高FGOALS-f3-L中的陆面和云过程对降低高原上地表温度偏差至关重要.     

Aerosol characteristics over the Tibetan Plateau simulated with a coupled aerosol–climate model (FGOALS-f3-L) 耦合气溶胶气候模式FGOALS-f3-L模拟青藏高原地区气溶胶特性

This study presents the simulated aerosol spatiotemporal characteristics over the Tibetan Plateau (TP) with a newly developed coupled aerosol–climate model (FGOALS-f3-L). The aerosol properties are simulated over the TP for the period 2002–11. The results indicate that soil dust, sulfate, and carbonaceous aerosols (black carbon (BC), organic carbon (OC) and BC/OC) account for 53.6%, 32.2%, and 14.2% of the total aerosol mass over the TP, respectively. The simulated aerosol surface mass concentrations and aerosol optical depths (AODs) are evaluated with ground-based and satellite observations, respectively. Underestimations of the aerosol surface mass concentration are found at the Lhasa site, especially for BC and OC. The spatial distribution and interannual variation of AOD are consistent with MODIS observations, with the RMSE of 0.081 and bias of 0.036. Due to the uncertainty of the parameterization of dust emissions, the model's performance in summer and autumn is much better than that in spring.摘要基于新耦合气溶胶气候模式FGOALS-f3-L模拟分析了2002–2011年青藏高原地区气溶胶时空分布特征.结果表明:青藏高原地区, 沙尘,硫酸盐,碳质气溶胶 (包括黑碳,有机碳和混合碳) 地表质量浓度分别占比为53.6%, 32.2%, 14.2%;在拉萨站点, 模拟的气溶胶地表质量浓度被低估, 尤其是黑碳和有机碳气溶胶;模拟的气溶胶光学厚度 (AOD) 时空分布与卫星观测结果较为一致, 均方根误差和偏差分别为0.081和0.036;由于模式中沙尘排放参数化的不确定性, 模式对AOD的模拟效果在夏季和秋季优于春季     

耦合气溶胶气候模式FGOALS-f3-L模拟青藏高原地区气溶胶特性

基于新耦合气溶胶气候模式FGOALS-f3-L模拟分析了2002-2011年青藏高原地区气溶胶时空分布特征.结果表明:青藏高原地区,沙尘,硫酸盐,碳质气溶胶(包括黑碳,有机碳和混合碳)地表质量浓度分别占比为53.6％,32.2％,14.2％;在拉萨站点,模拟的气溶胶地表质量浓度被低估,尤其是黑碳和有机碳气溶胶;模拟的气...     

耦合气溶胶气候模式FGOALS-f3-L模拟青藏高原地区气溶胶特性（英文）

基于新耦合气溶胶气候模式FGOALS-f3-L模拟分析了2002-2011年青藏高原地区气溶胶时空分布特征.结果表明:青藏高原地区,沙尘,硫酸盐,碳质气溶胶(包括黑碳,有机碳和混合碳)地表质量浓度分别占比为53.6%,32.2%,14.2%;在拉萨站点,模拟的气溶胶地表质量浓度被低估,尤其是黑碳和有机碳气溶胶;模拟的气溶胶光学厚度(AOD)时空分布与卫星观测结果较为一致,均方根误差和偏差分别为0.081和0.036;由于模式中沙尘排放参数化的不确定性,模式对AOD的模拟效果在夏季和秋季优于春季.     

Added Benefit of the Early-Morning-Orbit Satellite Fengyun-3E on the Global Microwave Sounding of the Three-Orbit Constellation

The three-orbit constellation can comprehensively increase the spatial coverage of polar-orbiting satellites, but the polar-orbiting satellites currently in operation are only mid-morning-orbit and afternoon-orbit satellites. Fengyun-3E(FY-3E) was launched successfully on 5 July 2021 in China. As an early-morning-orbit satellite, FY-3E can help form a complete three-orbit observation system together with the mid-morning and afternoon satellites in the current mainstream operational system. In th...     

Simulation of the Indian monsoon using the RegCM3–ROMS regional coupled model

A regional coupled atmosphere–ocean model was developed to study the role of air–sea interactions in the simulation of the Indian summer monsoon. The coupled model includes the regional climate model (RegCM3) as atmospheric component and the regional ocean modeling system (ROMS) as oceanic component. The two-way coupled model system exchanges sea surface temperature (SST) from the ocean to the atmospheric model and surface wind stress and energy fluxes from the atmosphere to the ocean model. The coupled model is run for four years 1997, 1998, 2002 and 2003 and the results are compared with observations and atmosphere-only model runs employing Reynolds SSTs as lower boundary condition. It is found that the coupled model captures the main features of the Indian monsoon and simulates a substantially more realistic spatial and temporal distribution of monsoon rainfall compared to the uncoupled atmosphere-only model. The intraseasonal oscillations are also better simulated in the coupled model compared to the atmosphere-only model. These improvements are due to a better representation of the feedbacks between the SST and convection and highlight the importance of air–sea coupling in the simulation of the Indian monsoon.     

Rain follows logging in the Amazon? Results from CAM3–CLM3

The impact of logging on precipitation in the Amazon region is investigated based on numerical experiments using the community atmosphere model version 3 coupled with the community land surface model version 3 (CAM3–CLM3). Three different representations of logging are examined, ranging from selective logging, to partial deforestation, to clear cut. Precipitation increases in response to modest selective logging, and decreases as the severity of logging progresses to partial deforestation and clear cut. Further experiments indicate that the increase of precipitation is mostly due to the decrease of surface albedo following selective logging, resulting from a low contrast between bare soil albedo and vegetation optical properties (i.e., leaf reflectance) in CLM3. This study demonstrates the complexity of representing land cover changes in climate models, and underlines the importance of accuracy in albedo measurement from satellite remote sensing.     

Downscaled simulations of the ECHAM5, CCSM3 and HadCM3 global models for the eastern Mediterranean–Black Sea region: evaluation of the reference period

The outputs of three GCMs, ECHAM5, CCSM3 and HadCM3, are downscaled for the eastern Mediterranean–Black Sea region for the period 1961–1990 using a regional climate model, RegCM3, to assess the capability of these models in simulating the climatology of the region. In addition, the NCEP/NCAR Reanalysis data are also downscaled for the same period to display the performance of the regional climate model for the same region, which constitutes a relatively complex terrain and rich variety of climates. The gridded observational dataset of CRU is primarily used in the evaluation of the models, however, a regional dataset, which is based on a relatively dense gauging network, is also used to see how it affects the performance measures of the models. The reanalysis simulation indicates that RegCM3 is able to simulate the precipitation and surface temperature as well as the upper level fields reasonably well. However, it tends to overestimate the precipitation over the mountainous areas. All three GCM models are found to be highly skilled in simulating the winter precipitation and temperature in the region. The two models, ECHAM5 and HadCM3, are also good at simulating the summer precipitation and temperature, but the CCSM3 simulation generates dryer and warmer conditions than the observations for the whole region, which are most likely a result of the dryness in the upper levels of the original outputs. The use of the regional observational dataset does not necessarily improve the pattern correlations, but it yields better match between the modeled and observed precipitation in terms of variability and root-mean-square difference. It could be said that the outputs of these GCMs can be used in the climate change downscaling and impact assessment studies for the region, given that their strengths and weaknesses that are displayed in the present study are considered.     

IAP／CAS的短期气候距平数值预测研究

本文介绍了中国科学院在气物理研究所（ＩＡＰ／ＣＡＳ）近十年来在短期气候距平数值预测研究方面的一些进展情况,首先介绍了近十年来准业务跨季度汛期降水预测的结果及评分,对预测的物理基础、预测可能性、集合预测方法、订正的必要性与方案进行了初步探讨,提出了我们的看法,发现预测中可能出现多平衡态,可以应用来改进不同区域的预测,并对些方法所作预测的特点、与经验半经验统计的相互配合、不同地区预测效果的差异、如何选     

Rate constants for the reactions of the NO3 radical with HCOOH/HCOO− and CH3COOH/CH3COO− in aqueous solution between 278 and 328 K

The kinetics of the aqueous phase reactions of NO₃ radicals with HCOOH/HCOO^– and CH₃COOH/CH₃COO^– have been investigated using a laser photolysis/long-path laser absorption technique. NO₃ was produced via excimer laser photolysis of peroxodisulfate anions (S₂O ₈ ^2– ) at 351 nm followed by the reactions of sulfate radicals (SO ₄ ^– ) with excess nitrate. The time-resolved detection of NO₃ was achieved by long-path laser absorption at 632.8 nm. For the reactions of NO₃ with formic acid (1) and formate (2) rate coefficients ofk ₁=(3.3±1.0)×10⁵ l mol^–1 s^–1 andk ₂=(5.0±0.4)×10⁷ l mol^–1 s^–1 were found atT=298 K andI=0.19 mol/l. The following Arrhenius expressions were derived:k ₁(T)=(3.4±0.3)×10¹⁰ exp[–(3400±600)/T] l mol^–1 s^–1 andk ₂(T)=(8.2±0.8)×10¹⁰ exp[–(2200±700)/T] l mol^–1 s^–1. The rate coefficients for the reactions of NO₃ with acetic acid (3) and acetate (4) atT=298 K andI=0.19 mol/l were determined as:k ₃=(1.3±0.3)×10⁴ l mol^–1 s^–1 andk ₄=(2.3±0.4)×10⁶ l mol^–1 s^–1. The temperature dependences for these reactions are described by:k ₃(T)=(4.9±0.5)×10⁹ exp[–(3800±700)/T] l mol^–1 s^–1 andk ₄(T)=(1.0±0.2)×10¹² exp[–(3800±1200)/T] l mol^–1 s^–1. The differences in reactivity of the anions HCOO^– and CH₃COO^– compared to their corresponding acids HCOOH and CH₃COOH are explained by the higher reactivity of NO₃ in charge transfer processes compared to H atom abstraction. From a comparison of NO₃ reactions with various droplets constituents it is concluded that the reaction of NO₃ with HCOO^– may present a dominant loss reaction of NO₃ in atmospheric droplets.     

Recent Advances in Dynamical Extra-Seasonal to Annual Climate Prediction at IAP／CAS

Recent advances in dynamical climate prediction at the Institute of Atmospheric Physics, Chinese Academy of Sciences (IAP/CAS) during the last five years have been briefly described in this paper. Firstly,the second generation of the IAP dynamical climate prediction system (IAP DCP-II) has been described,and two sets of hindcast experiments of the summer rainfall anomalies over China for the periods of 1980-1994 with different versions of the IAP AGCM have been conducted. The comparison results show that the predictive skill of summer rainfall anomalies over China is improved with the improved IAP AGCM in which the surface albedo parameterization is modified. Furthermore, IAP DCP-II has been applied to the real-time prediction of summer rainfall anomalies over China since 1998, and the verification results show that IAP DCP-II can quite well capture the large scale patterns of the summer flood/drought situations over China during the last five years (1998-2002). Meanwhile, an investigation has demonstrated the importance of the atmospheric initial conditions on the seasonal climate prediction, along with studies on the influences from surface boundary conditions (e.g., land surface characteristics, sea surface temperature).Certain conclusions have been reached, such as, the initial atmospheric anomalies in spring may play an important role in the summer climate anomalies, and soil moisture anomalies in spring can also have a significant impact on the summer climate anomalies over East Asia. Finally, several practical techniques(e.g., ensemble technique, correction method, etc.), which lead to the increase of the prediction skill for summer rainfall anomalies over China, have also been illustrated. The paper concludes with a list of criticalre quirements needed for the further improvement of dynamical seasonal climate prediction.     

Direct Climatic Effect of Dust Aerosol in the NCAR Community Atmosphere Model Version 3 （CAM3）

Direct climate responses to dust shortwave and longwave radiative forcing (RF) are studied using the NCAR Community Atmosphere Model Version 3 (CAM3). The simulated RF at the top of the atmosphere (TOA) is-0.45 W m-2 in the solar spectrum and +0.09 W m-2 in the thermal spectrum on a global average. The magnitude of surface RF is larger than the TOA forcing, with global mean shortwave forcing of-1.76 W m-2 and longwave forcing of +0.31 W m-2 . As a result, dust aerosol causes the absorption of 1.1 W m-2 in t...     

Assimilation of FY-3D MWTS-Ⅱ Radiance with 3D Precipitation Detection and the Impacts on Typhoon Forecasts

Precipitation detection is an essential step in radiance assimilation because the uncertainties in precipitation would affect the radiative transfer calculation and observation errors. The traditional precipitation detection method for microwave only detects clouds and precipitation horizontally, without considering the three-dimensional distribution of clouds.Extending precipitation detection from 2D to 3D is expected to bring more useful information to the data assimilation without using the a...     

Preliminary Evaluation of a Revised Zhang-McFarlane Convection Scheme Using the NCAR CCM3 GCM

l. IntroductiOnThe parameterizat1on of atmospheric convection is one of the most challenging issues inglobal climate modeling. Since convection interacts strongly with clouds and the large--scalecirculation, its representation in GCMs has a tremendous impact on the slmulation of theglobal climate and its variations. For example, in the National Center for Atmospheric Re-search (NCAR) Community Climate Model Version 2 (CCM2), excessive surface 1atent heatflux in the tropics was simulate…     

Effect of Increasing CO_2 on the Stratospheric Level of CO and O_3

Production and destruction processes of carbon monoxide (CO) and ozone (O3) are examined in the light of increasing amount of atmospheric carbon dioxide (CO2). It is found that doubling of CO2 will increase the stratospheric concentration of CO and will have positive effect on O3 concentration.     

Assimilation of ERS‐2 scatterometer winds using the Canadian 3D‐var

Abstract

The goal of this study is to evaluate the impact of incorporating the marine surface winds retrieved from the ERS‐2 scatterometer in the Canadian three‐dimensional variational analysis system, (3D‐var). The aspects of the 3D‐var most relevant to the assimilation of surface ‐wind observations and a general method for resolving the directional ambiguity of the retrieved scatterometer ‐winds are first described. A comparison ‐with 6‐h forecasted winds is then made to demonstrate that these data are of high quality, but exhibit a speed bias that can be removed by increasing their amplitudes by about 5%. The analysis increment from a single scatterometer wind observation is calculated to illustrate the response of the 3D‐var to surface wind observations. As a consequence of the forecast error covariance model, the assimilation of surface wind observations produces meteorologically consistent increments for both the rotational and divergent wind components and the mass field. The results from a series of cross‐validation experiments using ship‐based wind data demonstrate a positive impact of assimilating scatterometer winds and the effectiveness of a simple method for estimating and removing the speed bias. The impact of assimilating scatterometer data within a short assimilation cycle is also evaluated. Overall, the results show that including scatterometer data in the analysis decreases the 6‐h forecast error of surface wind by 13%. Over the northern extra‐tropics the improvement is only 4% and for the southern extra‐tropics it is 16%. Results from a series of two‐day forecasts produced using the analyses from the assimilation cycles with and without retrieved scatterometer winds included are also presented. Using radiosonde observations at 850 hPa, 500 hPa, 250 hPa and 100 hPafor verification, the impact on the forecasts is nearly neutral in the northern hemisphere and the tropics. Conversely, a significant positive impact is found on both wind and mass fields in the southern hemisphere over the entire two‐day forecast.     

A study of the formation of N2O in the reaction of NO3(A2E′) with N2

The rate of formation of N₂O via the thermochemically favourable reaction of NO₃(A²E) with N₂, which would represent an additional source of stratospheric N₂O and therefore NO_x, has been investigated. Mixtures of NO₂+O₃ in synthetic air were photolysed at 662 nm. No evidence was found for the production of N₂O via this pathway, the upper limit for the quantum yield of nitrous oxide formation being % MathType!MTEF!2!1!+-% feaafeart1ev1aaatCvAUfeBSjuyZL2yd9gzLbvyNv2CaerbuLwBLn% hiov2DGi1BTfMBaeXafv3ySLgzGmvETj2BSbqefm0B1jxALjhiov2D% aebbfv3ySLgzGueE0jxyaibaiiYdd9qrFfea0dXdf9vqai-hEir8Ve% ea0de9qq-hbrpepeea0db9q8as0-LqLs-Jirpepeea0-as0Fb9pgea% 0lrP0xe9Fve9Fve9qapdbaqaaeGacaGaaiaabeqaamaabaabcaGcba% GaeqOXdy2aaSbaaSqaamaaBaaameaadaWgaaqaamaaBaaabaGaamOt% amaaBaaabaGaaGOmaiaad+eaaeqaaaqabaaabeaaaeqaaaWcbeaatu% uDJXwAK1uy0HMmaeHbfv3ySLgzG0uy0HgiuD3BaGqbaOGae8hzIqOa% aGimaiaac6cacaaI2aGaaiyjaaaa!4E60!\[\phi _{_{_{_{N_{2O} } } } } \le 0.6\% \]. However, a dark conversion of NO_x to N₂O was observed and is attributed tentatively to a heterogeneous reaction on the wall of the reaction vessel. This process, although most likely to be insignificant in the atmosphere, needs to be taken into consideration in laboratory investigations or field studies of N₂O emission or deposition.