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MODEL STUDY OF THE EFFECT OF SOIL NO EMISSIONS ON SURFACE OZONE
作者姓名:韩志伟  胡非  张美根  朱江
作者单位:State Key Laboratory of Atmospheric Boundary Physics and Atmospheric Chemistry Institute of Atmospheric Physics,Chinese Academy of Sciences,Beiiing 100029,China,State Key Laboratory of Atmospheric Boundary Physics and Atmospheric Chemistry,Institute of Atmospheric Physics,Chinese Academy of Sciences,Beiiing 100029,China,Frontier Research System for Global Change,Kanagawa 236-0061,Japan,International Centre for Climate and Environmental Sciences,Institute of Atmospheric Physics.Chinese Academy of Sciences,Beijing 100029,China
基金项目:The research is supported by the Knowledge Innovation Project(KZCX2-204)and Hundred Talents Program(Research on Natural Cybernetics)by Chinese Academy of Sciences.
摘    要:The effect of soil NO emissions on surface ozone in autumn in East China has been studied byusing TCTM(Troposphere Chemical Transport Model)with the input of meteorological variablesfrom RAMS.The chemical mechanism for ozone variation caused by soil emissions has also beeninvestigated.The model results reveal that soil NO emissions are important to regional ozoneformation and distribution and the effect of soil NO emissions shows spatial inhomogeneity.Ozoneover most areas in northern China decreases with maximum average decrement reaching 5 ppbwhile it increases over most areas of central and southern China with maximum average incrementreaching 7 ppb caused by soil NO emissions.This situation of ozone variation is mainly determinedby nonlinear photochemical mechanism.For the low NOx areas(≤3 ppb),ozone increases as NOxincreases;for the high NOx areas(>3 ppb),ozone decreases as NOx increases.The effect of soilNO emissions on ozone depends on the transition value and NOx concentrations.


MODEL STUDY OF THE EFFECT OF SOIL NO EMISSIONS ON SURFACE OZONE
HAN Zhiwei HU Fei State Key Laboratory of Atmospheric Boundary Physics and Atmospheric Chemistry.MODEL STUDY OF THE EFFECT OF SOIL NO EMISSIONS ON SURFACE OZONE[J].Acta Meteorologica Sinica,2002(4).
Authors:HAN Zhiwei HU Fei State Key Laboratory of Atmospheric Boundary Physics and Atmospheric Chemistry
Institution:HAN Zhiwei HU Fei State Key Laboratory of Atmospheric Boundary Physics and Atmospheric Chemistry,Institute of Atmospheric Physics,Chinese Academy of Sciences.Beijing 100029,China ZHANG Meigen Frontier Research System for Global Change.Kanagawa 236-0061,Japan ZHU Jiang International Centre for Climate and Environmental Sciences.Institute of Atmospheric Physics Chinese Academy of Sciences.Beijing 100029,China
Abstract:
Keywords:model study  soil NO emissions  ozone  photochemical mechanism  transition value
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