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Nitrogen compound emission from biomass burning in tropical African savanna FOS/DECAFE 1991 experiment (Lamto,Ivory Coast)
Authors:Robert Delmas  Jean Pierre Lacaux  Jean Claude Menaut  Luc Abbadie  Xavier Le Roux  Gunter Helas  Jurgen Lobert
Institution:(1) Laboratoire d'Aérologie (URA CNRS 354), Université Paul Sabatier, Toulouse, France;(2) Laboratoire d'Ecologie, Ecole Normale Supérieure, Paris, France;(3) Max Planck Institut für Chemie, Mainz, Germany
Abstract:Gaseous nitrogen compounds (NO x , NO y , NH3, N2O) were measured at ground level in smoke plumes of prescribed savanna fires in Lamto, in the southern Ivory Coast, during the FOS/DECAFE experiment in January 1991. During the flaming phase, the linear regression between deltaNO x ] and deltaCO2] (differences in concentration between smoke plumes and atmosheric background) results volumic emission ratio deltaNO x ]/deltaCO2]=1.37×10–3 with only slight differences between heading and backing fires. Nearly 90% of the nitrogen oxides are emitted as NO. Average emission ratios of other compounds are: 1.91, 0.047, and 0.145×10–3 for NO y , NH3 and N2O, respectively. The emission ratios obtained during this field experiment are compred with corresponding values measured during former experiments with the same plant species in combustion chambers. An accurate determination of both the biomass actually burned and of the plant nitrogen content, allows an assessment of emission fluxes of N-compounds from Guinean savanna burns. Preliminary results dealing with the influence of fire on biogenic emissions from soils are also reported.
Keywords:biomass burning  savanna fires  biogenic emissions  nitrogen compounds
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