贵州和四川盆地云量的气候研究

贵州和四川盆地是我国云量最多的地区,素有“天无三日晴”和“蜀犬吠日”之说,盆地西缘的雅安古时还有“雅州天漏”的谚语。从全球日照百分率分布推知,川黔地区也是世界上天气最阴沉的地区之一。川黔之阴一向为国内外气象界所注意,本文根据1951—1980     

TEM evidence for intracellular accumulation of lead by bacteria in subsurface environments

We monitored near-surface atmospheric fallout (15-cm above ground) and soil solution (at 15, 35 and 55 cm below ground) derived nanoparticles over an 8-month period by collecting the particles directly onto TEM grids in anthropogenically-influenced (vineyard) and pristine (native forest) sites in France. Particle clusters trapped on the grid were selected randomly and individual particles were binned into eight different groups (euhedral clays, weathered clays, salts, oxi-hydroxides, bacteria, non-living organic matter, aggregates and undetermined). Bacteria represent 9–23% of the collected nanoparticle area (ave. 9.4% and 18% for two atmospheric collection sites and ave. 23% for soil infiltration samples). Bacteria were most often associated with non-living organic matter and comprised a variety of morpho-types. Interestingly, 45% of all the bacteria analyzed by transmission electron microscopy and electron dispersive spectroscopy (TEM-EDX) showed the presence of intracellular grains significantly enriched in lead and phosphorus. Intracellular sequestration of Pb into polyphosphate bodies has been observed in the laboratory, but this is the first observation of this phenomenon in a natural environment. Furthermore, this suggests that microbial-bound Pb may be an important transport mechanism in subsurface environments.     

环球海洋大气气溶胶化学研究

1986年11月—1987年5月,在中国第三次南极考察和环球科学考察期间,收集了58个海洋气溶胶样品,采用中子活化法分析了Al,V,Mn,I,Br,Mg,Na,Cl等元素。应用因子分析、回归分析和富集因子分析对气溶胶中元素进行分类、定量评估和来源判别,讨论不同来源元素的特征,计算各主要来源的贡献分量。结果表明,海洋气溶胶中Al的99.99％是来自陆源地壳风化物,Na的99.2％。和Cl的99.99％是来自海水,V的91.4％。来自陆源污染物。因此,Al可作为海洋气溶胶中陆源地壳风化物的示踪元素,Na和Cl可作为海水源示踪元素,非地壳源的V则可选择为陆源污染物的示踪元素。     

气溶胶光学厚度的时空变化

在大气中气溶胶微粒是一种重要的大气微量成分。气溶胶光学厚度也是大气校正所需的重要大气参数，同时也是海洋水色卫星主要的数据产品。由于气溶胶光学厚度的时空变化较大，所以如何准确获取大气校正和卫星数据产品真实性检验所需的气溶胶光学厚度则是至关重要的。在简述气溶胶光学性质的基础上，并结合2002年6月HY—1南海实验数据来阐述现场气溶胶光学厚度的准确获取。     

Numerical study of droplet size dependent chemistry in oceanic,wintertime stratus cloud at southern mid-latitudes

Cloud droplet chemistry is modelled for the first 150 m of rise in a wintertime, mid-latitude, marine stratus cloud using observations made at and near the Cape Grim Baseline Station as a source of input parameters. The emphasis in this work was to study the variation in droplet chemistry as a function of both droplet size and nucleus composition, with a particular focus on the way in which oxidation of dissolved sulfur dioxide varied.At 150 m above the condensation level, solute concentration as a function of droplet size was found to increase by as much as 2 to 3 orders of magnitude for only a factor of 2 increase in droplet radius, primarily as a consequence of the 1/r dependence in the droplet growth equation. This type of size dependence exists at all levels in the model cloud, and has a significant influence on oxidation rate of sulfur dioxide in droplets growing on sulfate nuclei, oxidation by ozone being favoured in the smallest droplets, but oxidation by hydrogen peroxide being favoured in the larger droplets. Oxidation by ozone is favoured at all sizes in droplets formed on sea-salt nuclei as a result of the initially high alkalinity of these droplets, and in the cloud overall is calculated to be the more important oxidation pathway. Although based on a simplified chemical scheme, these results suggest that both size-dependent and nucleus-dependent chemistry of cloud droplets may need to be considered explicitly in cloud modelling work.Volume-weighted mean pH values in the range 5 to 6 were predicted from sensitivity studies in which input variables were varied over reasonable ranges, in agreement with two sets of bulk cloud-water pH data obtained by aircraft near Cape Grim.     

北京晴天紫外波段气溶胶光学厚度反演与分析

利用太阳一大气紫外光谱辐射计(SAUVS)，测量到达北京地表的太阳直接和散射紫外光谱辐射，给出反演大气气溶胶光学厚度的一种方法。结果表明：在紫外波段，大气气溶胶的光学厚度随波长的增加而单调减小，用指数函数可以很好地拟合反演结果。统计得到了3个水平能见度状况下拟合函数的系数值，与全球气溶胶监测网络(AERONET)北京站的资料对比，表明反演结果基本合理。     

海盐气溶胶和硫酸盐气溶胶在云微物理过程中的作用

利用大气气溶胶和云分档模式研究海盐气溶胶和硫酸盐气溶胶在云微物理过程中的作用, 计算结果表明:云中液态水含量随高度的分布并不随海盐、硫酸盐的数目以及云团上升速度的变化而变化; 随着云滴数目的增加, 云滴的有效半径会减小; 硫酸盐对云滴数目影响起主导作用, 海盐在水汽相对充足情况下增加了云滴数目, 在水汽相对不足的情况下减少了云滴数目; 硫酸盐粒子浓度特别强的情况下 (人类活动污染比较严重时), 如果水汽相对不足, 云滴数目会明显小于硫酸盐粒子浓度; 而海盐粒子的存在, 加剧了水汽的供应不足, 从而可以在很大程度上进一步降低云滴数目。也就是说, 在有些情况下, 如果不考虑海盐气溶胶的作用, 硫酸盐气溶胶对云特性的影响会被过高估计。     

近20年全球总云量变化趋势分析

利用ISCCP月平均云气候资料集的总云量资料, 采用趋势分析的方法, 得到1983年7月至2001年9月近20年来全球平均总云量的变化趋势, 并分析云量变化的可能原因。近20年全球增温幅度加快, 研究这期间云的变化, 对气候研究和模拟具有重要的意义。结果表明:平均大气环流决定总云量的分布;全球平均总云量的变化趋势在20世纪80年代末发生逆转, 即由增加转为减少;全球平均云量呈减少的变化趋势, 2000年与1987年相比, 减少量约占平均总云量的4%;从地理位置上看, 云量的变化存在区域性差异, 热带和中纬度地区的总云量减少较多, 高纬度地区云量略有增加, 其中南极大陆云量增加较多。     

MODIS多光谱云相态识别技术的应用研究

介绍了卫星多光谱云相态识别的基本原理, 并给出了EOS/ MODIS云相态识别的流程。针对简单和复杂云场, 利用个例并结合无线电探空资料与MODI S三通道合成图肯定了多光谱云相态识别的合理性和实际效果。文中对几个特定天气系统(西南涡旋和西太平洋台风)下大面积云场相态分析的结果表明:多光谱云相态识别技术有一定应用价值, 且需要引入可见光技术来减少红外谱段对多层云覆盖和薄卷云的相态分析误差。