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Evolution of aerosol vertical distribution during particulate pollution events in Shanghai 下载免费PDF全文
A set of micro pulse lidar(MPL)systems operating at 532 nm was used for ground-based observation of aerosols in Shanghai in 2011.Three typical particulate pollution events(e.g.,haze)were examined to determine the evolution of aerosol vertical distribution and the planetary boundary layer(PBL)during these pollution episodes.The aerosol vertical extinction coefficient(VEC)at any given measured altitude was prominently larger during haze periods than that before or after the associated event.Aerosols originating from various source regions exerted forcing to some extent on aerosol loading and vertical layering,leading to different aerosol vertical distribution structures.Aerosol VECs were always maximized near the surface owing to the potential influence of local pollutant emissions.Several peaks in aerosol VECs were found at altitudes above 1 km during the dust-and bioburning-influenced haze events.Aerosol VECs decreased with increasing altitude during the local-polluted haze event,with a single maximum in the surface atmosphere.PM2.5 increased slowly while PBL and visibility decreased gradually in the early stages of haze events;subsequently,PM2.5 accumulated and was exacerbated until serious pollution bursts occurred in the middle and later stages.The results reveal that aerosols from different sources impact aerosol vertical distributions in the atmosphere and that the relationship between PBL and pollutant loadings may play an important role in the formation of pollution. 相似文献
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Reconstructed light extinction coefficients using chemical compositions of PM<Subscript>2.5</Subscript> in winter in Urban Guangzhou,China 总被引:8,自引:0,他引:8
The objective of this study was to reconstruct light extinction coefficients (b ext ) according to chemical composition components of particulate matter up to 2.5 μm in size (PM 2.5 ). PM 2.5 samples were collected at the monitoring station of the South China of Institute of Environmental Science (SCIES, Guangzhou, China) during January 2010, and the online absorbing and scattering coefficients were obtained using an aethalometer and a nephelometer. The measured values of light absorption coefficient by particle (b ap ) and light scattering coefficient by particle (b sp ) significantly correlated (R 2 > 0.95) with values of b ap and b sp that were reconstructed using the Interagency Monitoring of Protected Visual Environments (IMPROVE) formula when RH was <70%. The measured b ext had a good correlation (R 2 > 0.83) with the calculated b ext under ambient RH conditions. The result of source apportionment of b ext showed that ammonium sulfate [(NH 4 ) 2 SO 4 ] was the largest contributor (35.0%) to b ext , followed by ammonium nitrate (NH 4 NO 3 , 22.9%), organic matter (16.1%), elemental carbon (11.8%), sea salt (4.7%), and nitrogen dioxide (NO 2 , 9.6%). To improve visibility in Guangzhou, the effective control of secondary particles like sulfates, nitrates, and ammonia should be given more attention in urban environmental management. 相似文献
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2010年在代表长三角区域背景地区的浙江省临安区域大气本底站开展了对大气细粒子PM2.5为期1年的地面观测,并对细粒子中水溶性离子和碳组分的季节变化特征进行了分析。临安2010年大气中PM2.5质量浓度平均为 (58.2±50.8) μg·m-3,PM2.5质量浓度季节变化明显。利用HYSPLIT4模式计算了2010年临安72 h后向轨迹,根据轨迹计算与聚类结果,结合地面观测的PM2.5数据进行了分析。研究表明:临安地区因受到长江三角洲区域及偏北气流引起的污染传输影响,呈现出高细粒子水平特征。PM2.5中总水溶性离子年平均质量浓度为 (28.5±17.7) μg·m-3,占PM2.5质量浓度的47%。其中,气溶胶组分SO42-,NO3-和NH4+所占比例最大,共占总水溶性离子的69%。PM2.5中有机碳和元素碳的年平均质量浓度分别为 (10.1±6.7) μg·m-3和 (2.4±1.8) μg·m-3。有机碳和元素碳质量浓度显著相关,表明有机碳和元素碳主要来自相同的排放源。 相似文献
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风廓线雷达以测风为主要目的设计,没有充分考虑强度的定量测量。如果能够实现强度定量测量将大大扩展风廓线雷达的应用范围。首要的扩展应用就是可以获取雨滴谱分布、解决降水定量测量准确性问题。若实现强度定量测量,需要解决的一个关键技术问题是如何由其功率谱数据准确计算噪声功率。该文根据风廓线雷达功率谱估计方法、依据噪声频域统计特性,提出了一种计算风廓线雷达功率谱噪声功率的方法,并利用风廓线雷达实测功率谱数据进行检验。检验结果表明:即便在有降水或存在地物时,该方法仍可以准确、快速分辨出噪声功率谱, 且客观有效。 相似文献
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通过对我国北方地区影响日光温室生产的主要气候因素进行分析,从光、温、风、雪4个方面选取了冬季总辐射、日光温室生产季阴天日数、年极端最低气温、冬季平均气温、生产季月最大风速平均值、年最大积雪深度平均值6个因子作为气候适宜性区划指标,采用加权指数求和的评价方法建立综合气候适宜性区划指标模型,在利用层次分析法对区划指标进行量化分析确定其权重的基础上,借助GIS技术,得到北方地区日光温室发展的气候适宜性区划图。为了细化区划结果,将研究区域气候特征明显不同的典型区域分别进行进一步区划。结果表明:该方法不仅理论性较强,与实际相吻合的区划结果也说明该方法还具有良好的实用性。 相似文献
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西藏波龙斑岩铜金矿床成矿斑岩年代学、岩石化学特征及其成矿意义 总被引:12,自引:0,他引:12
波龙斑岩铜金矿床是近年来在青藏高原中部发现的最大的斑岩型矿床,波龙矿床发育两期花岗闪长斑岩和一期花岗斑岩,两期花岗闪长斑岩是波龙矿床的成矿斑岩。本文开展了波龙矿床三期斑岩锆石U-Pb年龄、全岩岩石地球化学和Sr-Nd-Hf同位素组成分析。锆石U-Pb测年结果显示,三期斑岩在120Ma集中侵位。两期花岗闪长斑岩均富集轻稀土、大离子亲石元素,亏损重稀土、高场强元素,Eu异常不明显,显示出岛弧岩浆岩的特征;两期花岗闪长斑岩的(87Sr/86Sr)i值分别为0.70562-0.70711和0.70567-0.70850,εNd(t)分别为-4.0--3.1和-8.0--2.4,εHf(t)值分别变化于2.5-6.9和3.3-6.9,表明两期花岗闪长斑岩起源于新生的下地壳;花岗斑岩也具有岛弧岩浆岩的岩石化学特征,但其具有较高εNd(t)值(-0.7--0.2)和εHf(t)值(1.3-12.2),可能表明花岗斑岩也起源于下地壳,但有更多幔源物质混入。波龙斑岩铜金矿床形成于班公湖-怒江洋壳向北俯冲末期,其成岩-成矿可能与洋壳俯冲关系密切,但波龙矿床的三期斑岩均起源于新生的下地壳,可能表明在120Ma南羌塘地块南缘开始逐步加厚。 相似文献
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