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31.
The diffusion of an ion in porewaters cannot occur independently of the other ions in solution as a result of Coulombic coupling, as well as from other effects not considered here. Unfortunately, a longstanding disagreement exists about the correct form and meaning of the equations that describe Coulombic coupling in porewaters, i.e., Ben-Yaakov [Am. J. Sci. 281 (1981) 974] vs. Lasaga [Am. J. Sci. 281 (1981) 981]. This paper re-examines this controversy by reformulating the problem starting from fundamental concepts of mass and charge conservation. We show that these antagonistic formulations are both valid and, in fact, equivalent, when the different interpretations of charge balance are resolved. Most of the disagreements between Ben-Yaakov and Lasaga are then shown to result from differing methods of solution, not fundamental disparities in their models. We note, however, that the explanation for the concept of “stationary” gradients of nonreacting ions as given Ben-Yaakov is inaccurate, and such gradients do lead to diffusive fluxes that are counterbalanced by electrochemical migrational fluxes to produce no net flux (excluding advective flux). We further find that the bicarbonate diffusive flux will not balance the diffusional charge flux of sulfate during its reduction if advection is present. This latter imbalance generates compensating fluxes in the other nonreacting ions. We have applied our theory to a simplified case of sulfate reduction in a marine sediment. The results show that nonreacting ions do diffuse and that with normally expected values of porewater advection, the ratio of the bicarbonate to the sulfate flux can be far different than the ideal value of −2. 相似文献
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时域瞬变场电磁场有限差分法 总被引:1,自引:2,他引:1
模拟电磁场在地下介质中的传播规律是理解地下介质响应的重要手段,直接应用有限差分法在时间域对二维、三维瞬变场进行数值分析是一种有效方法。应用反映电磁场基本规律的麦克斯韦方程组,导出时域场量的齐次扩散方程,对所研究的空间区域作差分离散,源作为初始条件加入,采用合适的边界条件,利用差分方程进行计算,从而得到场量的数值结果,展现瞬变场在地下随时间扩散的全过程,对电磁场的瞬态响应有更加直观的了解。 相似文献
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针对吉林市铁合金厂排污口下游江水的污染情况,设计研究江段,分段、分层取样。通过野外与室内实验,分析研宄了江水污染物的主要成分,并对NH4^ 的纵向、横向、垂向上的分布特征及其影响因素进行了详细研究。结果表明,垂直方向污染物扩散可以瞬时完成,在极短的时间内基本能达到完全混合;在横向和纵向上,岸边排放污染物一般只在近岸扩散,污染范围一般也只在靠近排污口一带;随着离排污口距离增大,污染物浓度降低,横向变化率较纵向大。本研究为排污口的污染物控制与治理、水资源保护提供了科学依据。 相似文献
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Postglacial topographic evolution of glaciated valleys: a stochastic landscape evolution model 总被引:1,自引:0,他引:1
The retreat of valley glaciers has a dramatic effect on the stability of glaciated valleys and exerts a prolonged influence on the subsequent fluvial sediment transport regime. We have studied the evolution of an idealized glaciated valley during the period following retreat of ice using a numerical model. The model incorporates a stochastic process to represent deep‐seated landsliding, non‐linear diffusion to represent shallow landsliding and an approximation of the Bagnold relation to represent fluvial sediment transport. It was calibrated using field data from several recent surveys within British Columbia, Canada. We present ensemble model results and compare them with results from a deterministic linear‐diffusion model to show that explicit representation of large landslides is necessary to reproduce the morphology and channel network structure of a typical postglacial valley. Our model predicts a rapid rate of fluvial sediment transport following deglaciation with a subsequent gradual decline, similar to that inferred for Holocene time. We also describe how changes in the model parameters affect the estimated magnitude and duration of the paraglacial sediment pulse. Copyright © 2005 John Wiley & Sons, Ltd. 相似文献
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Evolution of the Magma Chamber beneath Usu Volcano since 1663: a Natural Laboratory for Observing Changing Phenocryst Compositions and Textures 总被引:2,自引:1,他引:2
We have investigated the evolution of an active silicic magma-feedingsystem beneath Usu volcano, Japan, where eight eruptions havebeen recorded since AD 1663. All magmatic products contain similartypes of plagioclase and orthopyroxene phenocrysts that consistof homogeneous cores with uniform compositions, and a zonedmantle that increases in size with time. The compositions ofplagioclase and orthopyroxene phenocrysts vary gradually andregularly with time, as do the bulk-rock compositions. The textureof these phenocrysts also changes systematically, caused byprogressive crystal growth, dissolution and diffusion. On thebasis of these observations, we conclude that the same magma-feedingsystem has persisted at Usu volcano since AD 1663. Compositionalvariation of magnetite phenocrysts differs from that of plagioclaseand orthopyroxene, because magnetite has large diffusion coefficientsand should represent magmatic conditions immediately beforethe eruption. Most pumices from Usu volcano contain two typesof magnetite phenocryst, each with a different composition andcrystallization temperature, indicating that two magmas mixedbefore each eruption (approximately several days before). Theend-members changed with time: rhyolite + basaltic andesite(1663); dacite ± rhyolite (1769, 1822, 1853); dacite± dacite (1977, 2000). The temperature of the magma apparentlyincreases with time, and the increase can be explained by sequentialtapping from a magma chamber with a thermal and chemical gradientin addition to injection of high-temperature magma. KEY WORDS: continuous existence of magma chamber; dacite; dissolution and diffusion of phenocrysts; magma mixing; magnetite 相似文献
39.
Plastic Deformation and Recrystallization of Garnet: A Mechanism to Facilitate Diffusion Creep 总被引:5,自引:0,他引:5
Elongate and deformed garnets from Glenelg, NW Scotland, occurwithin a thin shear zone transecting an eclogite body that hasundergone partial retrogression to amphibolite facies at circa700°C. Optical microscopy, back-scattered electron imaging,electron probe microanalysis and electron back-scatter diffractionreveal garnet sub-structures that are developed as a functionof strain. Subgrains with low-angle misorientation boundariesoccur at low strain and garnet orientations are dispersed, aroundrational crystallographic axes, across these boundaries. Towardshigh-strain areas, boundary misorientations increase and thereis a loss of crystallographic control on misorientations, whichtend towards random. In high-strain areas, a polygonal garnetmicrostructure is developed. The garnet orientations are randomlydispersed around the original single-crystal orientation. Somegarnet grains are elongate and Ca-rich garnet occurs on thefaces of elongate grains oriented normal to the foliation. Commonly,the garnet grains are admixed with matrix minerals, and, wherein contact with other phases, garnet is well faceted. We suggestthat individual garnet porphyroclasts record an evolution fromlow-strain conditions, where dislocation creep and recoveryaccommodated deformation, through increasing strain, where dynamicrecrystallization occurred by subgrain rotation, to higheststrains, where recrystallized grains were able to deform bydiffusion creep assisted grain boundary sliding with associatedrotations. KEY WORDS: diffusion creep; EBSD; garnet; plastic deformation; recrystallization 相似文献
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基于一维地下水渗透方程详细推导其有限差分解算过程,引入不同于显式差分的隐式差分和中心差分格式,对比分析不同差分格式对地下水模拟结果及其相应地下水重力效应的影响,并对其中的层间参数取值和非线性方程的线性化问题进行探讨。结果表明,在日本Isawa扇形地区超导台站,不同层间参数加权公式能够引起最大约0.15 μGal的重力效应差异,影响在1.9%以内;不同差分格式和线性化方法组合形式能够引起最大约0.12 μGal的重力效应差异,影响在1.5%以内。 相似文献