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LI Jijun LU Shuangfang WU Wei XUE Haitao XU Qingxi GENG Jie YU Yinghua 《《地质学报》英文版》2011,85(5):1203-1210
In order to discuss the role and influence of water during the generation of natural gas, the participation mechanism of water during the evolution of organic matter and its influences were summarized. In addition, we carried out an anhydrous cracking experiment of oil extracted from the Feixianguan Formation source rock in a closed system, which led to the establishment of the kinetic models for describing carbon and hydrogen isotopic fractionation during gas generation from organic matter. The models were calibrated and then applied to the northeastern Sichuan Basin. By combining a series of gas generation experiments from octadecane pyrolysis without water or with distilled water in varying mass proportions, several results were proved: (1) the hydrogen isotopic composition of natural gas becomes lighter with the participation of formation water; (2) we can quantitatively study the hydrogen isotopic fractionation with the kinetic model for describing carbon isotopic fractionation; (3) more abundant and reliable geological information can be obtained through the combined application of carbon and hydrogen isotopic indices. 相似文献
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随着分析技术的进步,δ13C观测在全球碳循环研究中越来越受到重视。在讨论关于碳循环中δ13C的Suess效应、分布特征和同位素分馏等基本概念的基础上,结合现有的观测事实,介绍应用δ13C辨别碳的源汇问题的方法,通过比较不同KeelingPlot方法分析该方法在研究大气CO2背景特征中的意义。着重讨论δ13C在研究大气C... 相似文献
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鄂尔多斯盆地苏里格地区奥陶系马家沟组马五段白云岩的地球化学特征 总被引:1,自引:0,他引:1
苏里格地区奥陶系马家沟组马五段白云岩是重要的油气储集层.多年来,马家沟组白云岩的成因一直是地质研究者讨论的热点话题.对苏里格地区马家沟组马五段白云岩的微量元素及C、O、Sr同位素地球化学资料的分析表明,微量元素表现为高铁、低锰、低锶、低钠;白云石、白云质角砾和孔洞充填白云岩的δ13C和δ18O值较为近似,且白云岩的δ1... 相似文献
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Zhen Tao Quanzhou Gao Wenping Guo Zhengang Wang Yongling Zhang Chenji Xie Xiakun Huang Hongwei Zhong 《山地科学学报》2011,8(5):694-703
A whole year analysis of riverine dissolved organic carbon (DOC) concentrations in the Xijiang River (XJR), South China, showed that the mean riverine DOC concentration (1.24 mg L-1) in the XJR was notably lower than the averaged value (5.75 mg L-1) of the global riverine DOC concentration in several major rivers. There is an inconspicuous monthly fluctuation of the DOC signal in the XJR, but on a semi-yearly time scale, however, the riverine DOC concentration had significant difference between hydrological... 相似文献
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人工经济林在中国南方种植面积大,并有不断增加的趋势.人工经济林生态系统受人为周期性经营活动影响比较大,是重要的流动性碳库.因此,选择福建省建瓯市万木林自然保护区内本地条件基本一致的毛竹(Phyllostachys heterocycla)、柑橘(Citrus reticulata Blanco)和锥栗(Castanea henryi)作为研究对象,探讨其土壤有机碳含量及其垂直分布特征,结果表明:3种林地土壤剖面有机碳含量的变化范围分别为毛竹林5.91~19.18 g.kg-1、柑橘5.70~13.31g.kg-1、锥栗3.84~10.78 g.kg-1,3种林地土壤有机碳含量随着深度的增加呈现递减趋势;3种林地0~20 cm、20~40 cm层土壤有机碳含量与40~60 cm、60~80 cm、80~100 cm各层均存在显著性差异(P<0.05);3种林地间土壤有机碳储量均存在显著性差异(P<0.05);使用对数方程对3种林地土壤有机碳含量随土壤深度的变化进行拟合均达到显著水平(P<0.05);土壤有机碳含量与土壤全N、C/N比之间存在一定的相关性,特别是3种林地土壤有机碳含量均与土壤全N含量的相关性最好(... 相似文献
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基于能源消费的中国不同产业空间的碳足迹分析 总被引:10,自引:2,他引:8
Using energy consumption and land use data of each region of China in 2007,this paper established carbon emission and carbon footprint model based on energy consumption,and estimated the carbon emission amount of fossil energy and rural biomass energy of dif-ferent regions of China in 2007.Through matching the energy consumption items with indus-trial spaces,this paper divided industrial spaces into five types:agricultural space,living & industrial-commercial space,transportation industrial space,fishery and water conservancy space,and other industrial space.Then the author analyzed the carbon emission intensity and carbon footprint of each industrial space.Finally,advices of decreasing industrial carbon footprint and optimizing industrial space pattern were put forward.The main conclusions are as following:(1) Total amount of carbon emission from energy consumption of China in 2007 was about 1.65 GtC,in which the proportion of carbon emission from fossil energy was 89%.(2) Carbon emission intensity of industrial space of China in 2007 was 1.98 t/hm2,in which,carbon emission intensity of living & industrial-commercial space and of transportation in-dustrial space was 55.16 t/hm2 and 49.65 t/hm2 respectively,they were high-carbon-emission industrial spaces among others.(3) Carbon footprint caused by industrial activities of China in 2007 was 522.34 106 hm2,which brought about ecological deficit of 28.69 106 hm2,which means that the productive lands were not sufficient to compensate for carbon footprint of industrial activities,and the compensating rate was 94.5%.As to the regional carbon footprint,several regions have ecological profit while others have not.In general,the present ecologi-cal deficit caused by industrial activities was small in 2007.(4) Per unit area carbon footprint of industrial space in China was about 0.63 hm2/hm2 in 2007,in which that of living & indus-trial-commercial space was the highest (17.5 hm2/hm2).The per unit area carbon footprint of different industrial spaces all presented a declining trend from east to west of China. 相似文献