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ZHAO Mingliang WEI Xianfeng LIU Xuemeng DONG Xueyang YU Rilei WAN Shengbiao JIANG Tao 《中国海洋大学学报(英文版)》2018,(3)
Due to their structural diversity and variety of biological activities, marine natural products have been the subject of extensive study. These compounds, especially phospholipid polycyclic aromatic hydrocarbons, have a wide range of pharmacological applications, including embedded DNA and central nervous system, anti-tumor, anti-virus, anti-parasite, anti-bacterial, and antithrombotic effects. Unfortunately, the insufficient drug sources have limited the development of these compounds. In this study, we isolated salinpostin compounds from a fermentation solution of marine-derived Salinospora sp., which has a common bicyclic enol-phosphotriester core framework, as well as potent and selective antimalarial activities against P. falciparum with EC_(50)=50 nmolL~(-1). The chemical synthesis of these compounds in greater quantities is necessary for their use in bioactivity studies. Thus we explored a short route with high yields and mild reaction conditions, which can generate combinatorial libraries for drug discovery and lead optimization. We developed a new total synthesis method for six cyclic enol-phosphotriester salinipotin compounds and their diastereomers. For the total synthesis of cyclipostin P, we prepared cyclic enol-phosphotriester salinipostin compounds in 10 steps from a readily accessible starting material, 1,3-dihydroxyacetone, and obtained an overall yield of 1.29%. We fully characterized these compounds by proton nuclear magnetic resonance(~1H-NMR), carbon-13 NMR(~(13)C-NMR), and high-resolution mass spectrometry(HRMS) analyses, and found they coincide absolutely with the same compounds reported previously. 相似文献
44.
2001—2020年黄河流域植被覆盖变化及其影响因素 总被引:4,自引:3,他引:1
基于MODIS NDVI植被指数和气象数据集,以集合经验模态分解、趋势分析和随机森林回归分析等方法,分析了黄河流域2001—2020年植被覆盖时空变化特征,并对其气候驱动因素进行探讨。结果表明:(1)2001—2020年黄河流域植被覆盖整体呈显著增长趋势,增速为0.055/10a (P<0.05),2010年之前增速(0.067/10a)大于2010年之后的增速(0.051/10a)。(2)空间上,植被覆盖增加区域主要分布在陕北黄土高原、甘肃省东南部、内蒙古自治区河套平原等退耕还林还草生态工程实施区域,而植被覆盖显著下降区域则集中在关中平原城市群、黄淮海平原以及青藏高原等区域。(3)气温、降水和CO2浓度等对黄河流域植被生长起到正向促进作用,且绝对敏感性依次降低,而大气饱和水汽压差、太阳辐射等对植被生长起到抑制作用。本研究结果可为评估气候变化对黄河流域植被覆盖变化的综合影响提供参考依据。 相似文献
45.
六盘山东麓晚更新世以来黄土粒度指示的物源特征及演变 总被引:4,自引:0,他引:4
在宁夏长城塬完整的晚更新世-全新世黄土-古土壤剖面(长城塬剖面)进行高分辨率采样,对125个样品的粒度数据做了粒度端元分析,并对各端元组分含量在地层深度尺度上做了小波分析。结果认为:端元分析法可以把代表4 种不同动力的沉积端元分离出来。端元1可能代表了西风带控制下的由高空气流搬运的远源粉尘物质;端元2可能代表了沉积物沉积后在东亚夏季风作用下的风化以及成壤改造作用;端元3可能代表了后期的淋溶作用动力特征;端元4可能代表了东亚冬季风作用下典型的风成黄土粗颗粒组分特征。根据小波分析认为各端元组分含量在不同的深度上均存在着准周期变化,指示了相对应的时间尺度上古季风变化具有准周期性的特征,同时也说明了沉积剖面一直处于较为连续沉积状态,比较完整地记载了各沉积动力过程。各端元组分在不同的时间尺度上具有不同的准周期性特征。 相似文献
46.
Zhao Anzhou Zhang Anbing Liu Xianfeng Cao Sen 《Theoretical and Applied Climatology》2018,132(1-2):555-567
Theoretical and Applied Climatology - Extreme drought, precipitation, and other extreme climatic events often have impacts on vegetation. Based on meteorological data from 52 stations in the Loess... 相似文献
47.
引入调节变量的入境旅游对消费物价影响分析——基于1999~2014年香港季度数据的实证研究 总被引:2,自引:2,他引:0
引入调节变量,采用香港1999~2014年的季度统计数据建立一个新实证模型,利用Pearson相关性分析方法、计量经济学非平稳数据分析方法和Granger因果关系检验方法系统分析了入境旅游、经济增长和消费物价之间的关系。研究结果表明:① 入境旅游、经济增长和消费物价之间存在相关性和稳定的长期均衡关系;入境旅游对消费物价的带动性高于经济增长。② 入境旅游与消费物价、经济增长和消费物价、入境旅游和经济增长之间都存在单向Granger因果关系,入境旅游发展必然带动经济增长并影响消费物价。③ 入境旅游对消费物价产生影响的原因主要是入境游客规模扩大和结构单一;负面影响主要表现在影响当地底层民众生活品质、损害当地旅游形象和主客感情;对策主要为拓展入境旅游类型并使旅游发展红利惠及底层民众。 相似文献
48.
完善碳排放清单,是进行减排工作的基础,为了查明煤田火区对大气碳排放的贡献量,以煤氧复合作用学说为理论基础,从不同的研究思路出发,提出了烧失煤量法和排放通量法两种火区碳排放量计算模型。在明确模型中关键参数“释放因子”“排放系数α”“排放通量”“排放系数β”的具体含义的基础上,重点对各参数所对应的获取途径进行了研究论述:(1)释放因子通过在室内进行煤自燃模拟实验得出;(2)排放系数α通过煤岩吸附实验结合火区实地勘测得出;(3)排放通量通过对火区现场煤自燃气体排放及环境因素的实时监测得出;(4)排放系数β通过对遥感图像裂隙信息的提取得到。上述两种计算模型在我国乌达实验区进行了实际应用,并对其可实现性进行了检验。 相似文献
49.
An evolutionary economic geography perspective on types of operation development in West Lake,China 总被引:1,自引:0,他引:1
The types of operation play a key role in facilitating tourism consumption and economic development in a tourism destination. By adopting evolutionary economic geography theory, the paper analyzes the types of operation in West Lake Scenic Area from 1978 to 2013. First, an evolution process consisting of four stages is underpinned, and they are: the new establishment stage, the preliminary development stage, the speedup development stage, and the stabilized maturity stage. Specifically, the distinct characteristics associated with operation types are compared and evaluated at different stages throughout the process. The evolution trees are introduced to scrutinize types of operation development. The results of evolution trees demonstrate the substantial increase in both numbers and types. Second, by applying GIS spatial analysis, the paper also analyzes the spatial evolution characteristics on the types of operation, and the results unveil the co-existence of centripetal and centrifugal forces: the processes of spatial agglomeration and spatial dispersion. More specifically, we recognize the spatial process includes the emergence of node and concentration(1978–1995), the sparse distribution and intensity reduction(1996–2002), the patchy distribution and spatial agglomeration intensification(2003–2008), the dispersed distribution and core area agglomeration(2009–2013). Lastly, path dependence on resource endowment, government and market innovation, knowledge learning and spillover can reasonably explain the types of operation evolution. In conclusion, the evolutionary economic geography theories provide new theoretical and empirical perspectives for tourism policy analysis. At the same time, our comprehensive evidences impart more comprehensive insights and offer useful managerial and policy implications. 相似文献
50.
Huaizhan Li Guangli Guo Jianfeng Zha Yan He Zhiyong Wang Shuangyu Qin 《Environmental Earth Sciences》2017,76(20):704
We studied an underground coal gasification technique using strip mining-face mining gasifier controlled retraction injection technology (SMFM). This green mining approach offers several advantages over conventional strip mining but the stress distribution and stability of SMFM operations remain largely untested. In particular, hyperbolic coking pillars are used in SMFM compared with rectangular pillars used in traditional strip mining, which can influence the ultimate bearing capacity and stability. We use numerical simulations to investigate the influence of different factors (arch height, pillar height and width, mechanical characteristics), under the coupling effect of high temperature, on the ultimate bearing capacity of hyperbolic pillars. Our results indicate that arch height has a strong influence on pillar stress, while changes in pillar width and height are less significant. A stability evaluation method is proposed and tested on a case study in Inner Mongolia. Our theoretical results have practical significance for the promotion and application of SMFM. 相似文献