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31.
Margaret C. Graham John G. Farmer Ian W. Oliver Angus B. MacKenzie Robert M. Ellam 《中国地球化学学报》2006,25(B08):112-112
Natural uranium has three isotopes, ^238U, ^235U and ^234U, with natural abundances of 99.27 atom %, 0.72% and 0.0055%, respectively. Only ^235U is fissile and the production of nuclear fuel and nuclear weapons involves enrichment of uranium in ^235U. This process also results in separation of ^234U from ^238U, leaving depleted uranium (DU), with typical ^234U/^238U and ^235U/^238U activity ratios of about 0.19 and 0.013, respectively, as a waste product. The high density, high melting and boiling points and chemical stability of uranium and the availability of DU in relatively pure form mean that DU has many uses, including armour-piercing munitions. Such munitions have been developed in the UK since the 1960s and testing has been carried out by the Ministry of Defence (MoD) at firing ranges such as Dundrennan, SW Scotland and Eskmeals, NW England. The firing of DU munitions can result in the dispersion of DU and its combustion products (oxides) as aerosols or as larger fragments, with the potential for human exposure either directly at the site of detonation or via post-depositional migration in the environment. The aim of this work was to investigate the potential environmental mobility of DU by characterizing the associations of U in soil porewaters with increasing distance from a firing site. To this end, several soil cores located down-wind of the firing site at Dundrennan, near Kirkcudbright, SW Scotland, were collected in May 2006. These were sectioned on-site into 1- or 2-cm depth intervals and porewaters were isolated by centfifugation (10 minutes; 8873 g) on return to the laboratory. Following filtration through 0.2-micron cellulose nitrate filters, the porewaters were analyzed by ICP-QMS (U concentration) and ICP-OES (Fe, Al, Ca, Mg, Mn concentrations). Sub-samples were also subjected to centrifugal ultrafiltration (100, 30, and 3 kD) and to gel electrophoretic fractionation (agarose; 0.045 M Tris-borate; 20 mA, 30 minutes). Results showed that U was present at up to 4 μg/L in the soil porewater and that the associations of U varied with sample location and soil depth. 相似文献
32.
Teddy W. Sudinda Teddy 《中国地球化学学报》2006,25(B08):156-157
Flood and desiccation are perceived as two most critical and influential disasters which contradict between causes and consequences. Flood occurs when the water surface could no longer flow the whole water flow, thus, the water flooded. Contradicted to that, desiccation occurs when the water flow contains a low volume of water deposit, thus, the water requirement exceeds the available potential. That condition was caused by land utilization as the consequences due to the increased land requirement for housing or industrial needs. An attempt to overcome the flood, nowadays, is implemented mostly in a structural way, through building canals, implementing rivers normalization, building gateways or building flood control pump which are more directed toward the flood direction in order to increase the surface flow in an immediate maner to the sea. However, the effort to overcome the flood its self, could be more effective if followed by an effort to increase the soil ability to absorb natural recharge or artificial recharge or by refilling the water into the earth surface. Absorption reservoir used as one of technology alternatives (artificial recharge) could also be used to support the attempt to overcome flood and desiccation. Absorption reservoir is a dam which was designed according to the basic principles, such as the bottom surface of the reservoir that has a high permeability surface; the surface of the reservoir water is higher (higher aquifer) along with a high permeability, considering the availability of water source that has been absorbed and its quality; considering the aquifer category on the water absorption dam; 相似文献
33.
Huiwen HSIAO Susanne M. Ullrich Trevor W. Tanton 《中国地球化学学报》2006,25(B08):233-233
This research aims to establish the risks of hurnan exposure to modeling approach. The study site was located on the River Nura 1990s, an acetaldehyde production plant located in the industrial high environmental mercury levels, based on a quantitative risk in central Kazakhstan. From the 1950s until its closure in the mid city of Temirtau released mercury-containing wastewater into the river. River sediments are highly contaminated with mercury up to a distance of 25 km and beyond. In addition, a local power station released an estimated 6 million tonnes of fly-ash into the water and the mercury has become quite tightly associated with the ash deposits. River water, fish and agricultural land in the floodplain are also contaminated with mercury, yet the risks posed to the local population have not been evaluated to date. In June and July 2005, we took samples of soil, interior and exterior dust, drinking water, and food from individual households, communal areas and markets. Additionally, water and sediment samples and fish were taken from the river. Interviews were conducted with householders to establish their age and body weight, general living conditions and sources of irrigation and drinking water. A food frequency questionnaire (FFQ) was designed to investigate the frequencies of consumption of several common regional food items, including fish from the fiver and/or local market. Human hair samples were also collected to estimate the mercury bioburden and to enable the validity of the modeling approach to be established. The paper expands on the main pathways of contamination and looks at linkages between exposure pathways and mercury concentrations found in human hair. Uncertainties inherent in risk analysis as well as their influence on the relative importance of different exposure routes are also discussed. 相似文献
34.
近40年来西藏高原气候变化特征分析 总被引:5,自引:0,他引:5
本文利用西藏高原近40年来的逐月气象数据,通过时间序列分析和非参数Mann—Kendall检验方法,对西藏高原日照时数、平均气温、小型蒸发皿蒸发量和降水量4个基本气象要素变化特征进行了较为全面的分析,揭示了近40年来西藏高原气候变化的主要特征.结果表明:(1)日照时数是西北部长,东南部短,且东南部呈一定的下降趋势,西北部呈一定的上升趋势;(2)年平均气温以0℃和5℃为界划分为3个区,研究区全年总体表现出升温趋势,藏西地区的气温变化趋势大于藏东地区;(3)蒸发量年变化很大,研究区整体呈下降趋势,空间上表现为从西部向东部逐渐减少的趋势,其中仅西部和东南部小部分地区呈现出上升趋势,其余地区都为下降趋势;(4)降水趋势变率空间分布上的基本规律是:其大小由东往西逐渐减小,藏中和藏东为上升趋势,藏西为下降趋势.另外,4个要素各月与各季节的变化趋势与年变化趋势间表现出很好的一致性. 相似文献
35.
36.
南苏鲁芝麻房石榴石橄榄岩中橄榄石的“C”类组构及其形成条件探讨 总被引:5,自引:6,他引:5
上地幔地震的各向异性主要归因于橄榄石的优选方位,不同的橄榄石优选方位模式可以作为上地幔不同动力学作用的指示剂。不同应力和含水量条件下的高温变形实验已经确定出五类橄榄石组构模式(“A”型、“B”型、“C”型、“D”型和“E”型)。本文运用电子背散射(EBSD)技术对来自苏鲁超高压变质带南部的芝麻房石榴石橄榄岩的橄榄石进行了优选方位测定,不同变形程度的橄榄石均显示了[100]轴近垂直于面理和[001]轴近平行于线理的特征,为“C”类组构模式,可见组构类型与变形程度没有关系,并且橄榄石组构所显示的NW向SE的剪切指向,与围岩-正、副片麻岩中形成于折返过程的石英优选方位所显示的SE向NW的剪切指向完全不同,说明芝麻房石榴石橄榄岩中橄榄石的“C”类组构是折返前形成的。结合橄榄石结构水的测量和已有的芝麻房石榴石橄榄岩形成的温压条件,推测该组构形成于含水俯冲带中,认为芝麻房石榴石橄榄岩的原岩来自于高含水的上部地幔楔碎块,与俯冲的陆壳物质一起经历了超高压变质作用并最终折返至地表。 相似文献
37.
苏鲁超高压变质岩区深部流体He-Ar的系统关系:中国大陆科学钻探工程在线流体监测的解析 总被引:3,自引:1,他引:3
中国大陆科学钻探工程在线监测从泥浆中分离出的气体地球化学组成揭示了一段重要的气体异常,从2004年12月24日夜里开始到12月29日晚上结束。从12月10日到24日晚上11点30分的气体的Ar、He和N2基本上沿着趋势A分布,而12月26日早上7点半到29日晚上7点半的数据沿趋势C分布。相对于趋势A,趋势C中的气体含有相对升高的Ar,Ar/He和Ar/N2的平均值分别为3653和0.0142,明显高于空气的比值1800和0.0119。趋势A中的气体的Ar/He和Ar/N2比值分别围绕1851和0.0118变化,其中的Ar/He比值稍微高于空气的比值,但Ar/N2比值近似于空气比值,表明背景地下流体含非常低的Ar,而He和N2主要是大气组分。在趋势A和趋势C之间的数据(时间段B)具有和空气接近的Ar/N2比值,但平均Ar/He比值为3265,明显高于空气比值,反映了该段气体具有相对亏损的He。苏鲁-大别山地区的热年代学研究已经表明云母和角闪石的Ar/Ar的冷却年龄大大地高于磷灰石或锆石的He的冷却年龄,说明Ar在超高压变质地体折返早期就已封闭,而He一直保持开放状态,直到超高压变质岩接近地表。这种Ar和He对温度变化的不同反应,导致大部分的He在超高压岩石折返过程中脱气并释放到空气中,Ar则相对圈闭在固体岩石或封闭的断裂带中。在He-Ar的系统关系上,表现为来自于超高压岩石或断裂带中的流体具有富集Ar、亏损He及升高的Ar/He比值。气体组分从趋势A向趋势C的骤然跳跃,反映了地下流体组分的强烈变化,即具有相对富集Ar的深部流体的贡献大大增强。 相似文献
38.
CCSD在线流体监测捕获的气体地球化学异常与2004年9.3级苏门答腊地震可能的超远程关系 总被引:5,自引:0,他引:5
中国大陆科学钻探工程在线流体地球化学监测在2004年12月10至2005年1月10日之间捕获到一段重要的气体地球化学异常。该异常从2004年12月24日晚上11点半开始到12月29日晚上7点半结束,其中在12月26日早上7点半到29日晚7点半这段异常非常特殊,表现出流体地球化学的剧烈变化。具体表现为流体组分从基本上不含Ar、He及N2跳跃到富含Ar、但亏损He和N2。该异常发生在2004年9.3级苏门答腊地震前1个半小时。由于CCSD现场离苏门答腊地震震中距离大于4170公里,大于该地震破裂长度1200公理的3倍,该地震在CCSD现场产生的静态应力变化微乎其微,不足以导致CCSD现场深部岩石或封闭破裂的岩石物理性质剧烈变化,因而可以排除静态激发效应的作用。在我国的云南和广东等地所观测到的地震异常和地下水位变化等表明2004年苏门答腊地震的动态激发效应主要沿东北方向,这和大地震的动态激发具有方向性一致。而CCSD现场就位于该方向上。我们推测2004年苏门答腊地震所产生的面波在CCSD现场激发的动态效应,导致库仑型失稳,增进深部岩石或破裂带的渗透率,释放富含Ar但亏损He和N2的流体,产生CCSD所观测到的气体异常。 相似文献
39.
地下圆形衬砌隧道对沿线地震动的影响(II):数值结果 总被引:5,自引:3,他引:5
利用地下圆形衬砌隧道对入射平面P波和SV波散射级数解答,定量分析了入射波长、入射角度、隧道直径、衬砌刚度等因素对沿线地表位移放大作用的影响。计算结果表明,当入射频率较低时,地下隧道的存在对地表位移幅值影响不大;而当入射频率较高时,地表位移幅值可以达到无隧道情况的4.5倍以上;衬砌情况下地表位移幅值可以高出非衬砌情况的87.8%。建议在地铁的规划设计中考虑地下隧道的建设对隧道沿线设计地震动的影响。 相似文献
40.