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101.
Hitoshi Sakai Thomas J. Casadevall James G. Moore 《Geochimica et cosmochimica acta》1982,46(5):729-738
Eighteen basalts and some volcanic gases from the submarine and subaerial parts of Kilauea volcano were analyzed for the concentration and isotope ratios of sulfur. By means of a newly developed technique, sulfide and sulfate sulfur in the basalts were separately but simultaneously determined. The submarine basalt has 700 ± 100 ppm total sulfur with δ34SΣs of . The sulfate/sulfide molar ratio ranges from 0.15 to 0.56 and the fractionation factor between sulfate and sulfide is . On the other hand, the concentration and δ34SΣs values of the total sulfur in the subaerial basalt are reduced to 150 ± 50 ppm and , respectively. The sulfate to sulfide ratio and the fractionation factor between them are also smaller, 0.01 to 0.25 and +3.0‰, respectively. Chemical and isotopic evidence strongly suggests that sulfate and sulfide in the submarine basalt are in chemical and isotopic equilibria with each other at magmatic conditions. Their relative abundance and the isotope fractionation factors may be used to estimate the and temperature of these basalts at the time of their extrusion onto the sea floor. The observed change in sulfur chemistry and isotopic ratios from the submarine to subaerial basalts can be interpreted as degassing of the SO2 from basalt thereby depleting sulfate and 34S in basalt.The volcanic sulfur gases, predominantly SO2, from the 1971 and 1974 fissures in Kilauea Crater have δ34S values of 0.8 to 0.9%., slightly heavier than the total sulfur in the submarine basalts and definitely heavier than the subaerial basalts, in accord with the above model. However, the δ34S value of sulfur gases (largely SO2) from Sulfur Bank is 8.0%., implying a secondary origin of the sulfur. The δ34S values of native sulfur deposits at various sites of Kilauea and Mauna Loa volcanos, sulfate ions of four deep wells and hydrogen sulfide from a geothermal well along the east rift zone are also reported. The high δ34S values (+5 to +6%.o) found for the hydrogen sulfide might be an indication of hot basaltseawater reaction beneath the east rift zone. 相似文献
102.
103.
A sulfur isotope fractionation of 20.0 ± 0.2‰ was measured between aqueous sulfide and sulfate at 300°C and 1000 bars using gold-cell hydrothermal solution equipment. The value is 2‰ smaller than previously published values. Rates of exchange were determined as a function of pH and total sulfur content. Initial mean 34S concentration was changed to approach equilibrium from two directions. Half-times ranged from 3.4 to 8.2 days, with shorter times obtained for more acid and more concentrated solutions.The sulfate-sulfide isotope temperature scale based on theory should be revised according to this new fractionation factor. The rate data permit assessment of the extent to which equilibrium may be attained in some natural systems. For example, the lack of agreement between temperatures based on sulfide mineral pairs and sulfide-sulfate mineral pairs from Kuroko ore deposits of Japan might imply that the residence time of sulfate and sulfide in Kuroko solutions was not longer than 1000 years, if the present kinetic data are correct. Geothermal systems such as the Wairakei system of New Zealand may reach sulfur isotope equilibrium between sulfate and sulfide in 300 years at 300°C, but would be increasingly removed from equilibrium at lower temperatures if residence times were 300 years or less. 相似文献
104.
Oxygen isotope study of metamorphic and granitic rocks of the Yanai district in the Ryoke belt,Japan
18O/16O ratios have been obtained for 134 whole-rocks and minerals from metamorphic and granitic rocks of the Yanai district in the Ryoke belt, Southwest Japan. The 18O/16O ratios of pelitic rocks of the marginal metamorphic zone decrease progressively with increasing metamorphic grade. In the gneiss-granite complex (zone of migmatite [1]), the most characteristic feature of the rocks is that oxygen isotopic homogenization proceeds on both local and regional scales in parallel with “granitization” or chemical homogenization. Granitic rocks of various origin are fairly uniform in isotopic composition with δ 18O of quartz of 12 to 14‰ (SMOW) and δ 18O of biotite of 7 to 9‰ and are about 3 to 4‰ enriched in 18O compared to other Cretaceous granites of non-metamorphic terranes in Japan. The high 18O/16O ratios of granitic rocks of this district were discussed in relation to the 18O-depletion in metasediments. Oxygen isotopic fractionations among coexisting minerals from various rock-types of the gneiss-granite complex indicate that these minerals were formed under near isotopic equilibrium at a temperature of about 600 to 700° C. Some abnormal fractionations of quartz-biotite pairs also were obtained for rocks which had undergone a progressive 18O-depletion or 18O-enrichment. This is due to high resistivity of quartz and contrastive susceptibility of biotite to isotopic exchange during metamorphism and “granitization”. 相似文献
105.
Ryutaro Sakai Minoru Kusakabe Masami Noto Teruaki Ishii 《Earth and Planetary Science Letters》1990,100(1-3)
Many serpentinite seamounts occur over a region 20–120 km west of the trench axis in the Izu-Ogasawara-Mariana forearc regions. The hydrogen and oxygen isotopic compositions of serpentine from these regions indicate that there are at least two kinds of waters responsible for serpentinization: seawater and water derived from dehydration of the descending slab. Serpentine from two Mariana and two Torishima samples with microscopically ductile and sheared texture (sheared-type) have lowerδD(−63to−52‰) and slightly higherδ18O values (+6.1 to +8.2‰) than that of other nine Ogasawara samples with mesh texture (mesh-type) (δD= −43to−49‰ andδ18O= +5.8to+6.7‰). This suggests that the sheared-type serpentine with lowerδD and slightly higherδ18O values was formed within the wedge mantle by interaction with water derived from a descending slab. The sheared texture is likely to have been produced during diapiric uplift. The unaltered portion of the ultramafic bodies later interacted with seawater after emplacement at or near the seafloor, resulting in formation of the mesh-type serpentine with higherδD values. 相似文献
106.
Oxygen and carbon isotope compositions were determined for calcites from the Green Tuff formations of Miocene age in Japan. Values of
18O from 24 calcites in altered rocks from 5 districts range from –2 to +16SMOW, in most cases from 0 to +8SMOW. The low
18O values rule out the possibility of their low-temperature origin or any significant contribution of magmatic fluid in the calcite precipitation. These values, coupled with their mineral assemblages, suggest that the calcites formed from meteoric hydrothermal solutions which caused propylitic alteration after the submarine strata became emergent.Values of
13C from the calcites show a wide variation from –17 to 0PDB. Calcites from different districts have different ranges of
13C values, indicating that there was no homogeneous reservoir of carbon at the time the calcite formed, and that the carbon had local sources. Carbon isotopic compositions of calcite within ore deposits in the Green Tuff formations range from –19 to 0PDB, similar to those of calcite in the altered rocks in the same district, suggesting that the carbon in ore calcites was likely supplied from the surrounding rocks through activity of meteoric hydrothermal solutions. 相似文献
107.
We present simulation results of X-type coalescence of two current-loops, by using a 3-D resistive MHD code. The results are compared with the limb flare observed by Yohkoh on 2 August, 1993 at 08:30 UT, which is a good example of partial X-type coalescence. It is shown that the maximum temperature enhancement near the cross-point of the two loops, obtained from the simulation, agrees well with the observations when the plasma is 0.08. 相似文献
108.
The Ou Backbone Range strikes northwards through the central northeastern Japan arc and is bounded on both sides by the active reverse Uwandaira and Sen'ya faults. We have applied a traveltime inversion method (seismic tomography) with spatial velocity correlation to active and passive seismic data in order to investigate a three-dimensional (3-D) velocity structure. The data set contains 33,993 P- and 18,483 S-wave arrivals from 706 natural sources and 40 blasts, as well as 2803 P-wave traveltime data from 10 explosions detonated during the 1997 controlled source experiment. The traveltime inversion reveals a zone beneath the Ou Backbone Range in which P-wave velocities (VP) are approximately 6–8% lower than the average velocity at equivalent depths. The low VP and a low VP to S-wave velocity (VS) ratio (VP/VS) of about 1.65 suggest the presence of aqueous fluids in the middle crust. 相似文献
109.
The 18O/16O ratios were analyzed for 35 volcanic rocks from the Izu-Hakone region, Oki-Dogo Island, Asama Volcano and Kiso-Ontake Volcano in the Japanese Islands. The 18O-enrichment in magma during crystallization differentiation is recognized in every rock series. The magnitude of solid-liquid isotope fractionation in the magma of tholeiite series is similar to that of alkali rock series, while the apparent isotope fractionation of calc-alkali rock series is larger than that of the above two series. The
18O value of the tholeiite magma in the Izu- Hakone region is +5.7 relative to SMOW, which suggests its origin from the fresh upper mantle material. The primary magma of the calc-alkali rock series in Asama Volcano is assumed to have the
18O value similar to or slightly higher than that of the Izu-Hakone primary magma. The alkali rock series of Oki-Dogo Island in the continental side of the island arc is by 1 heavier than the Izu-Hakone rock suite. This may imply that Oki-Dogo rock series might have exchanged their oxygen with 18O-rich crustal materials, or they might have originated from somewhat 18O-rich upper mantle material. 相似文献
110.
Atsushi Nozaki Ryuichi Majima Koji Kameo Saburo Sakai Atsuro Kouda Shungo Kawagata Hideki Wada Hiroshi Kitazato 《Island Arc》2014,23(2):157-179
We present field and core observations, nannofossil biostratigraphy, and stable oxygen isotope fluctuations in foraminiferal tests to describe the geology and to construct an age model of the Lower Pleistocene Nojima, Ofuna, and Koshiba Formations (in ascending order) of the middle Kazusa Group, a forearc basin‐fill succession, exposed on the northern Miura Peninsula on the Pacific side of central Japan. In the study area, the Nojima Formation is composed of sandy mudstone and alternating sandy mudstone and mudstone, the Ofuna Formation of massive mudstone, and the Koshiba Formation of sandy mudstone, muddy sandstone, and sandstone. The Kazusa Group contains many tuff beds that are characteristic of forearc deposits. Thirty‐six of those tuff beds have characteristic lithologies and stratigraphic positions that allow them to be traced over considerable distances. Examination of calcareous nannofossils revealed three nannofossil datum planes in the sequences: datum 10 (first appearance of large Gephyrocapsa), datum 11 (first appearance of Gephyrocapsa oceanica), and datum 12 (first appearance of Gephyrocapsa caribbeanica). Stable oxygen isotope data from the tests of the planktonic foraminifer Globorotalia inflata extracted from cores were measured to identify the stratigraphic fluctuations of oxygen isotope ratios that are controlled by glacial–interglacial cycles. The observed fluctuations were assigned to marine isotope stages (MISs) 49–61 on the basis of correlations of the fluctuations with nannofossil datum planes. Using the age model obtained, we estimated the ages of 24 tuff beds. Among these, the SKT‐11 and SKT‐12 tuff beds have been correlated with the Kd25 and Kd24 tuff beds, respectively, of the Kiwada Formation on the Boso Peninsula. The Kd25 and Kd24 tuff beds are widely recognized in Pleistocene strata in Japan. We used our age model to date SKT‐11 at 1573 ka and SKT‐12 at 1543 ka. 相似文献