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81.
Kinetic parameters were determined for the first time, via open-system pyrolyses, on algaenans (highly resistant biomacromolecules that are selectively preserved during kerogen formation) isolated from extant microalgae. Parallel studies were also carried out on 10 kerogens exhibiting, with one exception, a low level of maturity. These kerogens included samples chiefly derived from the selective preservation of the above algaenans and samples mainly, or almost exclusively, derived from the “natural vulcanization” pathway. Important differences in activation energy (Ea) distributions were observed between the four algaenans investigated and correlated with their chemical structures. The kerogens predominantly derived from algaenan-selective preservation (Pula alginite, NE 70 and BJ 248 Torbanites, Rundle Oil Shale) also exhibited pronounced differences in Ea distributions. These distributions provided: (i) information on the diversity of the source materials; and (ii) reflected the occurrence of important differences in chemical structures and thermal behaviour between three of the tested kerogens, even though they are all classified as low maturity type I. The Kimmeridge Clay samples and the Lorca Oil Shale showed broad Ea distributions shifted to low energies when compared with the above algaenans and kerogens. Such shifts reflect an important (or even almost exclusive for some of these kerogens) contribution of materials originating from sulphur incorporation into various lipids during early diagenesis. Finally, the kinetic data derived for the nine low maturity fossil samples were extrapolated to a very low, geological heating rate of 3°C Ma−1 and the generation rate curves and cumulative yield curves thus obtained were compared. 相似文献
82.
A series of experiments on the fluid-absent melting of a quartz-rich aluminous metagreywacke has been carried out. In this
paper, we report the chemical composition of the phases present in the experimental charges as determined by electron microprobe.
This analytical work includes biotite, plagioclase, orthopyroxene, garnet, cordierite, hercynite, staurolite, gedrite, oxide,
and glass, over the range 100–1000 MPa, 780–1025 °C. Biotites are Na- and Mg-rich, with Ti contents increasing with temperature.
The compositions of plagioclase range from An17 to An35, with a significant orthoclase component, and are always different from the starting minerals. At high temperature, plagioclase
crystals correspond to ternary feldspars with Or contents in the range 11–20 mol%. Garnets are almandine pyrope grossular
spessartine solid solutions, with a regular and significant increase of the grossular content with pressure. All glasses are
silicic (SiO2 = 67.6–74.4 wt%), peraluminous, and leucocratic (FeO + MgO = 0.9–2.9 wt%), with a bulk composition close to that of peraluminous
leucogranites, even for degrees of melting as high as 60 vol.%. With increasing pressure, SiO2 contents decrease while K2O increases. At any pressure, the melt compositions are more potassic than the water-saturated granitic minima. The H2O contents estimated by mass balance are in the range 2.5–5.6 wt%. These values are higher than those predicted by thermodynamic
models. Modal compositions were estimated by mass balance calculations and by image processing of the SEM photographs. The
positions of the 20 to 70% isotects (curves of equal proportion of melt) have been located in the pressure-temperature space
between 100 MPa and 1000 MPa. With increasing pressure, the isotects shift toward lower temperature between 100 and 200 MPa,
then bend back toward higher temperature. The melting interval increases with pressure; the difference in temperature between
the 20% and the 70% isotects is 40 °C at 100 MPa, and 150 °C at 800 MPa. The position of the isotects is interpreted in terms
of both the solubility of water in the melt and the nature of the reactions involved in the melting process. A comparison
with other partial melting experiments suggests that pelites are the most fertile source rocks above 800 MPa. The difference
in fertility between pelites and greywackes decreases with decreasing pressure. A review of the glass compositions obtained
in experimental studies demonstrates that partial melting of fertile rock types in the crust (greywackes, pelites, or orthogneisses)
produces only peraluminous leucogranites. More mafic granitic compositions such as the various types of calk-alkaline rocks,
or mafic S-type rocks, have never been obtained during partial melting experiments. Thus, only peraluminous leucogranites
may correspond to liquids directly formed by partial melting of metasediments. Other types of granites involve other components
or processes, such as restite unmixing from the source region, and/or interaction with mafic mantle-derived materials.
Received: 11 July 1995 / Accepted: 27 February 1997 相似文献
83.
Several stratigraphic sequences in the Upper Carboniferous (Pennsylvanian) in Kansas (Midcontinent, USA) were analyzed quantitatively for periodic repetitions. The sequences were coded by lithologic type into strings of datasets. The strings then were analyzed by an adaptation of a one-dimensional Fourier transform analysis and examined for evidence of periodicity. The method was tested using different states in coding to determine the robustness of the method and data. The most persistent response is in multiples of 8–10 ft (2.5–3.0 m) and probably is dependent on the depositional thickness of the original lithologic units. Other cyclicities occurred in multiples of the basic frequency of 8–10 with persistent ones at 22 and 30 feet (6.5–9.0 m) and large ones at 80 and 160 feet (25–50 m). These levels of thickness relate well to the basic cyclothem and megacyclothem as measured on outcrop. We propose that this approach is a suitable one for analyzing cyclic events in the stratigraphic record. 相似文献
84.
In situ flow-through attenuated total reflectance (ATR) Fourier transform infrared (FTIR) spectroscopy has been used to investigate the formation, and step-wise oxidation, of sulfoxyanions at the pyrite surface during oxidation by molecular oxygen. The surface was studied under two different pH regimes (pH 2.5 and pH 5.6) and under two light conditions (dark and ultraviolet light). It was experimentally observed that multiple sulfoxyanions were present at the pyrite surface during oxidation by molecular oxygen, spectroscopically illustrating the concept of sulfur step-wise oxidation. The results from photochemical experiments were complex and suggest a dependence on both pH and surface speciation. 相似文献
85.
Particles in shear enclose important information about a rock's past and can potentially be used to decipher the kinematic history and mechanical behavior of a certain outcrop or region. Isolated rigid clasts in shear zones often exhibit systematic inclinations with respect to the shear-plane at small angles, tending towards the instantaneous stretching direction of the shear zone. This shape preferred orientation cannot be easily explained by any of the analytical theories used in geology. It was recently recognized that a weak mantle surrounding the clast or a slipping clast–matrix interface might be responsible for the development of the observed inclinations. Physical considerations lead us to conjecture that such mantled, rigid clasts can be effectively treated as voids that are not allowed to change their shape. The resulting equivalent void conjecture agrees well with numerical and field data and has the following important geological implications. (i) Clasts in shear zones can have stable positions in simple shear without the requirement of an additional pure shear component. (ii) The stable orientation can be approached either syn- or antithetically; hence, the clast can rotate against the applied shear sense. (iii) The strain needed to develop a strong shape preferred orientation is small (γ≈1) and therefore evaluations based on other theories may overestimate strain by orders of magnitude. (iv) The reconstruction of far-field shear flow conditions and kinematic vorticity analysis must be modified to incorporate these new findings. 相似文献
86.
Marcus B. Lane 《The Australian geographer》2005,36(3):283-299
This paper tracks the changing role of public participation in planning thought. In doing so, the paper shows that the role of public participation in planning is largely determined by the nature of the planning enterprise being undertaken. The definition of the planning problem, the kinds of knowledge used in planning practice, and the conceptualisation of the planning and decision-making context are the important determinants of the extent of participation offered to the public. The paper therefore contributes to thinking about how to evaluate public participation by showing that it can only be understood in terms of the decision-making context in which it is embedded. Specifically, it makes little sense to evaluate public participation in terms that are not shared by the planning model itself 相似文献
87.
Ruth Lane Damian Lucas Frank Vanclay Sophie Henry Ian Coates 《The Australian geographer》2005,36(3):351-367
Emerging approaches to environmental governance require a greater level of community participation than did previous approaches in which these responsibilities largely rested with government agencies. There is consequently a need for increased engagement with NRM among a broad community sector. This paper examines initiatives by two prominent government agencies, the Murray–Darling Basin Commission (MDBC) and the National Museum of Australia (NMA), to engage school children from regional communities using education programs that focus on place and environmental health. We focus on the MDBC's International Riverhealth Conference held in Mildura in 2003 and the associated Murray–Darling Basin TalkBack Classroom sponsored by the NMA and the Parliamentary Education Office (PEO). We explore how key themes of local scale, place-based identities, youth voice and critical engagement are developed in these programs and consider how they relate to the environmental agency of children. We then reflect on the potential for the kinds of environmental agency promoted through these programs to help build the capacity of local communities to progress larger goals of environmental restoration and sustainability in the Murray–Darling Basin. The evaluation research reported here forms part of the Committing to Place research project, an Australian Research Council Linkage grant involving the University of Tasmania, the National Museum of Australia and the Murray–Darling Basin Commission. 相似文献
88.
89.
Atika Karim Mostafa Berkhli Daniel Vachard Nicolas Tribovillard Beate Orberger 《Comptes Rendus Geoscience》2005,337(5):525-532
The unexplored area of Azarhare in central Morocco is studied thanks to three sections composed of five lithological facies Main biostratigraphical and sedimentological results concern (1) the identification of Late Visean biozones, with important presence of problematic algae Ungdarella, (2) the regional extension of deposit sequences SD5, SD6 and SD7 previously defined, (3) and an analysis of the diagenetic kaolinite. To cite this article: A. Karim et al., C. R. Geoscience 337 (2005). 相似文献
90.