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排序方式: 共有371条查询结果,搜索用时 46 毫秒
31.
Quantification of carbon flow from stable isotope fractionation in rice field soils with different organic matter content 总被引:1,自引:0,他引:1
Rice fields are an important source for the greenhouse gas methane produced by acetoclastic and hydrogenotrophic methanogenesis. Fractionation of 13C/12C can in principle be used to quantify the relative contribution of these pathways, but our knowledge of isotopic fractionation during reduction of CO2 and turnover of acetate in different methanogenic environments is still scarce. We therefore measured δ13C signatures in two types of anoxic Italian rice field soils, one with high and one with low degradable organic matter (OM) content. Both soils were incubated in the presence and absence of methyl fluoride, a specific inhibitor of acetoclastic methanogenesis. Optimization of methyl fluoride concentration resulted in complete inhibition of acetoclastic methanogenesis. CH4 was then exclusively produced by hydrogenotrophic methanogenesis, allowing determination of the isotopic signatures and fractionation factors specific for this methanogenic pathway. Acetate, which was then no longer consumed, accumulated and was used for determination of the isotopic signature of the fermentatively produced acetate (both total acetate and methyl carbon of acetate). Hence, all isotopic signatures, including fractionation factors were determined for the methanogenic soil. These data, were then used for computation of the relative contribution of the two methanogenic pathways. In the high OM soil, the contribution of acetoclastic methanogenesis to total CH4 production increased simultaneously with decreasing acetate concentration. In the low OM soil, methanogenesis from H2/CO2 was clearly greater than theoretically expected. Furthermore, isotope fractionation of hydrogenotrophic methanogenesis indicated that the in situ energy status of methanogens strongly depended on the availability of organic carbon in the rice field soil system. Collectively, our data show that the study of isotopic fractionation in methanogenic environments allows a deeper insight into the ongoing processes, which may be quite different in the same ecosystem with different content of degradable OM. 相似文献
32.
Gérard Thuillier Michel Hersé Paul C. Simon Dietrich Labs Holger Mandel Didier Gillotay Thomas Foujols 《Solar physics》1998,177(1-2):41-61
The SOLSPEC instrument has been built to carry out solar spectral irradiance measurements from 200 to 3000 nm. It consists of three spectrometers designed to measure the solar spectral irradiance in ultraviolet, visible, and infrared domains. It flew with the ATLAS I mission in March 1992. This paper is dedicated to the visible part of the solar spectrum. Comparisons with recent data are shown and differences below 450 nm are discussed. 相似文献
33.
34.
Dr. Christoph Hoffmann 《International Journal of Earth Sciences》1977,66(1):465-477
Until now (Smith, 1965) it was thought that in the central Damara Belt, South West Africa, the Red Granite and the Salem Granodiorite are two magmatic bodies separated by (essentially) marbles. Three places were discovered, where the marbles are missing; in all three places the Red Granite intrudes the Salem Granodiorite. Experimental melting done with samples from two of these localities allows to appraise the likely conditions during the intrusion of the Red Granite (680° C, 4 kb H2O-pressure).The White Granites — until now thought to be late or post kinematic — are a geologically heterogeneous group, at least in one place such an intrusion precedes that of the Red Granite.
Zusammenfassung Bis jetzt dachte man (Smith, 1965) daß im Zentralbereich des Damara-Orogens, Südwest Afrika, der Rote Granit und der Salem Granodiorit zwei magmatische Körper wären, die überall von (im wesentlichen) Marmoren getrennt seien. Es wurden drei Gegenden entdeckt, an denen die Marmore fehlen; an allen drei Stellen intrudiert der Rote Granit in den Salem Granodiorit. Schmelz-Experimente mit Proben von zwei dieser Lokalitäten erlauben die Bedingungen abzuschätzen, die während der Intrusion des Roten Granites geherrscht haben (680° C, 4 kb H2O-Druck).Die Weißen Granite — von denen man bis jetzt glaubte, sie seien spät-oder nachkinematisch — sind eine geologisch heterogene Gruppe. Mindestens an einer Stelle geht eine Intrusion der Weißen Granite derjenigen der Roten Granite voraus.
Résumé Jusqu'à présent (Smith, 1965) on a pensé que dans la zone centrale de l'orogène de Damara (Sud-Ouest Africain) le Granite Rouge et la Granodiorite de Salem étaient deux plutonites séparées partout par des couches de marbres. On a découvert trois endroits où les marbres n'existent pas et où le Granite Rouge forme des intrusions recoupant la Granodiorite de Salem.Des essais de fusibilité sur des échantillons provenant de deux de ces localité permettent d'estimer les conditions d'intrusion du Granite Rouge (680° C avec des pressions H2O de 4–5 kb).Les Granites blancs (acceptés jusqu'à présent comme tardi orogéniques) forment géologiquement une groupe hétérogène. En un endroit au moins, une intrusion de Granite blanc est recoupée par une intrusion du Granite Rouge, plus jeune.
(SMITH, 1965), , , - , , . 3 , , . , , , (680° C, 4 ). , , -, , . , - , .相似文献
35.
Giancarlo Bellucci Joern Helbert Francesca Altieri Dennis Reiss Jean-Pierre Bibring Stephan van Gasselt Harald Hoffmann Yves Langevin Gerhard Neukum Franois Poulet 《Icarus》2007,192(2):361-377
In this paper we report about a small region on the northern scarp of Olympus Mons showing an increase of the 3 μm hydration band in the OMEGA spectra, together with low superficial temperatures. Although water ice clouds can occurs on the flank of big martian volcanoes, radiative transfer modeling indicates that atmospheric water ice alone cannot justify the shape of the observed band. A fit of the 1.9–3 μm absorption features is obtained by hypothesizing that the study region consists of a mixture of dust and water ice covered by an optically thin (τ=0.08 at 3 μm) layer of dust. Thermal modeling also suggests that water ice in this region may be stable during most of the martian year due to the saturation of the atmosphere. If water ice is responsible for the observed spectral behavior, it might consist of a number of ice or snow patches possibly deposited in small depressions. 相似文献
36.
Helen V. McGregor Lydie Dupont Jan-Berend W. Stuut Holger Kuhlmann 《Quaternary Science Reviews》2009,28(15-16):1434-1448
Understanding past human–climate–environment interactions is essential for assessing the vulnerability of landscapes and ecosystems to future climate change. This is particularly important in southern Morocco where the current vegetation is impacted by pastoralism, and the region is highly sensitive to climate variability. Here, we present a 2000-year record of vegetation, sedimentation rate, XRF chemical element intensities, and particle size from two decadal-resolved, marine sediment cores, raised from offshore Cape Ghir, southern Morocco. The results show that between 650 and 850 AD the sedimentation rate increased dramatically from 100 cm/1000 years to 300 cm/1000 years, and the Fe/Ca and pollen flux doubled, together indicating higher inputs of terrestrial sediment. Particle size measurements and end-member modelling suggest increased fluvial transport of the sediment. Beginning at 650 AD pollen levels from Cichorioideae species show a sharp rise from 10% to 20%. Pollen from Atemisia and Plantago, also increase from this time. Deciduous oak pollen percentages show a decline, whereas those of evergreen oak barely change. The abrupt increase in terrestrial/fluvial input from 650 to 850 AD occurs, within the age uncertainty, of the arrival of Islam (Islamisation) in Morocco at around 700 AD. Historical evidence suggests Islamisation led to population increase and development of southern Morocco, including expanded pastoralism, deforestation and agriculture. Livestock pressure may have changed the vegetation structure, accounting for the increase in pollen from Cichorioideae, Plantago, and Artemisia, which include many weedy species. Goats in particular may have played a dominant role as agents of erosion, and intense browsing may have led to the decline in deciduous oak; evergreen oak is more likely to survive as it re-sprouts more vigorously after browsing. From 850 AD to present sedimentation rates, Fe/Ca ratios and fluvial discharge remain stable, whereas pollen results suggest continued degradation. Pollen results from the past 150 years suggest expanded cultivation of olives and the native argan tree, and the introduction of Australian eucalyptus trees. The rapidly increasing population in southern Morocco is causing continued pressure to expand pastoralism and agriculture. The history of land degradation presented here suggests that the vegetation in southern Morocco may have been degraded for a longer period than previously thought and may be particularly sensitive to further land use changes. These results should be included in land management strategies for southern Morocco. 相似文献
37.
Holger L. Fröhlich Lutz Breuer Hans‐Georg Frede Johan A. Huisman Kellie B. Vaché 《水文研究》2008,22(12):2028-2043
The link between spatiotemporal patterns of stream water chemistry and catchment characteristics for the mesoscale Dill catchment (692 km2) in Germany is explored to assess the catchment scale controls on water quality and to characterize water sources. In order to record the spatiotemporal pattern, ‘snapshot sampling’ was applied during low, mean and high flow, including 73 nested sites throughout the catchment. Water samples were analysed for the elements Li, B, Na, Mg, Al, K, Ca, V, Cr, Mn, Fe, Co, Ni, Cu, Zn, Rb, Sr, Mo, Ba, Pb and U using inductively‐coupled‐plasma mass spectrometry, and for electric conductivity and pH. Principle component analysis and hierarchical cluster analysis were used to find typical element associations and to group water samples according to their hydrochemical fingerprints. This revealed regional hydrochemical patterns of water quality which were subsequently related to catchment attributes to draw conclusions about the controls on stream chemistry. It was found that various lithologic signals and anthropogenic point source inputs controlled the base flow hydrochemistry. During increased flows, stream waters were diluted causing additional hydrochemical variability in response to heterogeneous precipitation inputs and differences in aquifer storage capacities. The hydrochemical patterns further displayed in‐stream mixing of waters. This implied, that stream waters could be apportioned to the identified water sources throughout the catchment. The basin‐wide hydrochemical variability has the potential to outrange the tracer signatures typically inferred in studies at the hillslope scale and is able to strongly influence the complexity of the catchment output. Both have to be considered for further catchment scale tracer and modelling work. Despite the likelihood of non‐conservative behaviour, the minor and trace elements enhanced the rather qualitative discrimination of the various groundwater types, as the major cations were strongly masked by point source inputs. Copyright © 2007 John Wiley & Sons, Ltd. 相似文献
38.
Modification of fluid inclusions in quartz by deviatoric stress I: experimentally induced changes in inclusion shapes and microstructures 总被引:1,自引:1,他引:0
Alexandre Tarantola Larryn W. Diamond Holger Stünitz 《Contributions to Mineralogy and Petrology》2010,160(6):825-843
Fluid inclusions in quartz are known to modify their shapes and microstructures (textures) during weak plastic deformation.
However, such changes have not been experimentally demonstrated and criteria are not available to relate them to paleostress
conditions. To address these issues, quartz crystals containing natural CO2–H2O–NaCl fluid inclusions have been experimentally subjected to compressive deviatoric stresses of 90–250 MPa at 700°C and ~600 MPa
confining pressure. Strains of up to 1% cause the inclusions to develop irregular shapes and to generate microcracks in crystallographic
planes oriented subperpendicular to the major compression axis, σ
1. The uniform alignment of the microcracks imparts a planar fabric to the samples. The microcracks heal and form swarms of
tiny satellite inclusions. These new inclusions lose H2O by diffusion, thereby triggering plastic deformation of the surrounding quartz via H2O-weakening. Consequently, the quartz samples deform plastically only in domains originally rich in inclusions. This study
shows that fluid inclusions deformed by deviatoric stresses may indeed record information on paleostress orientations and
that they play a key role in facilitating crystal-plastic deformation of quartz. 相似文献
39.
The Epupa Metamorphic Complex constitutes the southwestern margin of the Congo Craton and is exposed in a hilly to mountainous terrain of northwestern Namibia, bordering the Kunene River and extending into southern Angola. It consists predominantly of granitoid gneisses which are migmatized over large areas. This migmatization locally led to anatexis and produced crustal-melt granites such as the Otjitanda Granite. We have undertaken reconnaissance geochemical studies and single zircon U–Pb SHRIMP and Pb–Pb evaporation dating of rocks of the Epupa Complex. The granitoid gneisses, migmatites and anatectic melts are similar in composition and constitute a suite of metaluminous to peraluminous, calc-alkaline granitoids, predominantly with volcanic arc geochemical signatures. The zircon protolith ages for the orthogneisses range from 1861 ± 3 to 1758 ± 3 Ma. Anatexis in the migmatitic Epupa gneisses was dated from a melt patch at 1762 ± 4 Ma, and the anatectic Otjitanda Granite has a zircon age of 1757 ± 4 Ma. Migmatization and anatexis therefore occurred almost immediately after granitoid emplacement and date a widespread high-temperature Palaeoproterozoic event at ∼1760 Ma which has not been recorded elswhere in northern Namibia. The Nd isotopic systematics of all dated samples are surprisingly similar and suggest formation of the protolith from a source region that probably separated from the depleted mantle about 2.4–2.0 Ga ago. A major Archaean component in the source area is unlikely. 相似文献
40.
In this article, an approach for the efficient numerical solution of multi-species reactive transport problems in porous media
is described. The objective of this approach is to reformulate the given system of partial and ordinary differential equations
(PDEs, ODEs) and algebraic equations (AEs), describing local equilibrium, in such a way that the couplings and nonlinearities
are concentrated in a rather small number of equations, leading to the decoupling of some linear partial differential equations
from the nonlinear system. Thus, the system is handled in the spirit of a global implicit approach (one step method) avoiding
operator splitting techniques, solved by Newton’s method as the basic algorithmic ingredient. The reduction of the problem
size helps to limit the large computational costs of numerical simulations of such problems. If the model contains equilibrium
precipitation-dissolution reactions of minerals, then these are considered as complementarity conditions and rewritten as
semismooth equations, and the whole nonlinear system is solved by the semismooth Newton method. 相似文献