气溶胶对云宏微观特性和降水影响的研究进展

气溶胶—云—降水相互作用是当今大气科学研究的热点和前沿问题.概述性地回顾了气溶胶对云宏微观特性和降水影响的研究进展,分别讨论了气溶胶对层状云、对流云等典型云系的动力和微物理过程的影响,总结了国内外研究关于气溶胶对云宏微观特性影响的可能的物理解释.回顾外场观测及数值研究表明,气溶胶对云液态水含量、地面降水及光学厚度的影响...     

气溶胶影响云和降水的机理和观测研究进展

气溶胶对云和降水的影响,对于气候系统、大气环境以及水循环至关重要。气溶胶粒子作为云凝结核和大气冰核影响云的微物理过程,进而影响雨、雪、雹和其他形式的降水。近年来,在理解气溶胶的化学成分,气溶胶微物理特性以及气溶胶作为云凝结核和大气冰核影响云降水等方面已取得重大进展。本文对于气溶胶的概念、来源以及气溶胶的直接和间接效应进行了简要概述,重点总结了国内外在气溶胶影响云和降水的机理研究方面的成果,回顾了近年来利用卫星、地面观测设备、机载探测设备等对气溶胶和云进行遥感观测和直接观测所获得的观测事实并讨论了其可能的物理机制,在总结前人研究成果的基础上对未来的研究方向进行了讨论。     

气溶胶对北京地区不同类型云降水影响的数值模拟

利用耦合Milbrandt双参数显式云方案的WRF模式,在大陆型和海洋型气溶胶浓度背景下,对北京地区暴雨、中雨和微量降水等3次云降水过程进行了数值模拟研究。结果表明,气溶胶的增加对北京地区云降水有多方面的影响：（1）影响地面降水量。随着气溶胶浓度的增加,北京地区的暴雨、中雨和微量降水平均累计降水量分别减少了23.8%,...     

华北地区秋冬季气溶胶污染与不同类型降水的关系

气溶胶对降水的影响具有很大的不确定性,正确理解和认识气溶胶对不同类型降水的影响对提高天气预报的准确度和全球气候变化具有重要意义。利用GPM-DPR观测资料和MERRA-2再分析资料分析了气溶胶污染与华北地区2014—2020年秋、冬季对流云降水和层状云降水的关系。结果表明:与清洁状况相比,气溶胶污染状况下对流云降水的降水强度有所增强,雨顶高度更高。在污染状态下对流云降水具有粒径小但数浓度高的降水粒子,潜热加热率更高。气溶胶污染与层状云降水的降水强度、雨顶高度等宏观特征不存在明显相关。层状云降水相比对流云降水更容易受到大气水汽条件和垂直上升运动的影响。因此,在气象条件主导降水的情况下,气溶胶污染对华北地区层状云降水的影响很难通过GPM-DPR和MERRA-2数据观测到。      

利用GRAPES模式研究气溶胶对云和降水过程的影响

在GRAPES中尺度模式的双参数微物理方案中加入了气溶胶活化参数化过程,实现了对云滴数浓度的预报。选取不同季节两个降水过程进行模拟,并分别开展了不同气溶胶背景下的两个试验进行对比分析,研究气溶胶对云和降水可能的影响。结果表明:气溶胶浓度增加后,因为活化产生了更多尺度较小的云滴,抑制了云雨的自动转化,使大气中滞留了更多的云水,暖云降水减小;另一方面,云水的增加会使冰相粒子,尤其是雪和霰通过碰并云水等过程而增大,最后融化成雨增加冷云降水,同时冰相粒子增加会释放更多的潜热,促进上升气流的发展,进一步增加冷云降水。气溶胶对降水的影响存在空间不一致性,暖云较厚的地方暖雨过程受到的抑制明显,使地面降水减小,冷云厚度相对较厚时,冷云降水的增加会大于暖云降水的抑制,使地面降水增加。同时由于在云降水发展的不同阶段冷暖云的变化,气溶胶对降水的影响也存在着时间不一致性。     

气溶胶对秦岭山脉地形云降水的影响

以华山站为影响站,其周围华阴、渭南、西安为对比站,通过对影响站与对比站降水之比--地形强化因子(Ro)的变化趋势以及Ro与能见度变化关系的分析,研究了气溶胶对秦岭地形云降水的影响.结果表明:有观测以来Ro逐年递减,1980年后Ro递减更快,减幅达20%;Ro的减小趋势与能见度递减、气溶胶递增相吻合,说明气溶胶的增加抑制了地形云降水;华山1980年后的年平均雨量比1980年前减少了15%,达132mm,而平原地区的减少量不超过3%(16mm).分析气溶胶抑制地形云降水的物理过程发现,Ro的递减主要是减少了中小雨(日雨量小于30mm)的天数,而对大于30mm的降水影响较小,说明气溶胶对浅薄的生命期较短的地形云降水的抑制作用更明显;在以动力强迫抬升为主的春秋季,气溶胶对地形云降水的抑制作用明显强于平原地区,1980--2004年间降水减少了20%～30%;在热力作用下,气溶胶对地形云降水的抑制作用与平原地区相当.     

中国北方沙尘气溶胶对云和降水影响的数值模拟研究

已有的研究表明中国北方千旱半干旱地区是对流层沙尘气溶胶的主要来源之一,对当地乃至全球气候都有重要的意义.利用数值模拟研究方法探讨不同干燥程度的大气背景环境下,沙尘气溶胶数浓度对混合云形成和发展的可能影响,并采用析因试验讨论了主次影响因素.结果表明:沙尘气溶胶的增加导致降水减少、延长了云在空中存在的时间,改变了云的空间结构和微观结构.析因分析表明干旱半干旱气候背景条件下,混合云的累计降水量对沙尘气溶胶数浓度变化的敏感性要高于对大气环境湿度的敏感性;沙尘气溶胶数浓度增加导致云累计降水量的减少;沙尘气溶胶数浓度和大气环境湿度对云的累计降水量的影响是复杂的,研究结果可以用于指导降水预报业务.     

秦岭地区气溶胶对地形云降水的抑制作用

以华山站为影响站, 周围的西安、渭南和华阴作为对比站, 通过影响站与对比站降水之比——地形强化因子(Ro)的变化趋势以及Ro与能见度关系的分析, 定量研究了秦岭地区气溶胶对地形云降水的抑制作用。Ro的演变分析表明: 有观测以来Ro逐年递减, 减幅为14%～20%, 即影响站与对比站相比降水量减少了14%～20%; Ro的减少趋势与能见度递减、气溶胶递增相吻合, 说明气溶胶的增加抑制了地形云降水。Ro的递减主要是减少了中小雨 (日雨量小于30 mm) 的天数, 这种影响对浅薄的生命期较短的地形云降水作用更明显, 对于华山站, 30 mm以下的降水都会受到入云气溶胶的抑制作用, 而西安站为5 mm以下, 入云气溶胶浓度越高, 就有越厚的降水云受气溶胶影响而抑制降水; 在以动力强迫抬升为主的春秋季, 气溶胶抑制华山地形云降水20%左右, 最大可达25%; 在热对流条件下, 气溶胶对地形云和对平原地区云的抑制作用基本相当。不同风速风向下Ro的变化趋势表明, Ro递减随风速增大而加快, 迎风向 (240°～30°) 大风 (≥5 m/s) 时减少降水超过30%。由Ro与能见度关系的定量分析发现, 当能见度在14 km时Ro为1.8左右, 随着能见度的降低Ro逐渐减小, 当能见度小于8 km时,R0约为1.2, 减小了30%左右; 华山对于华阴的Ro与能见度呈线性关系, 相关系数达0.81。最后, 根据研究结果归纳出气溶胶抑制秦岭地区地形云降水的初步物理模型。     

吸湿性催化剂在暖云降水初始阶段的作用

引言用人工播撒吸湿性催化剂或者人工喷水催化对流云,以加速降水发展和增加降水量,已经引起了许多科学家的注意。从专门的模拟研究得知,这类健化技术的前途是大有希望的。然而,这类有用的计算,关键在于准确预报自然云的发展趋势。据最近对大气气溶胶的测量结果,大气中一般的气溶胶直径并不止10微米,并     

云降水物理与人工影响天气研究进展

2011年,云降水物理与人工影响天气研究主要在暖云数值模式研制及模拟、云物理过程对降水影响、冰雹物理过程、效果检验、南方冻雨的微物理过程以及华北气溶胶特征等方面取得如下研究成果。     

气溶胶-气候耦合模式系统BCC_AGCM2.0.1_CAM气候态模拟的初步评估

本文讨论了国家气候中心第二代大气环流模式BCC_AGCM2.0.1和加拿大气溶胶理化模式CAM所组成的耦合模式系统对5种典型气溶胶(硫酸盐、黑碳、有机碳、沙尘和海盐)和气候要素的模拟效果。结果表明,耦合系统对5种典型气溶胶的模拟总体上比较合理,尤其是对硫酸盐、沙尘和海盐的模拟比BCC_AGCM2.0.1原有的月平均气溶胶资料有很大的改进。耦合系统模拟的全球平均气候态参量与观测/再分析资料比较一致,在总云量、陆地表面温度和降水等方面要略优于原月平均气溶胶资料的模拟结果。耦合系统对沙尘和海盐气溶胶模拟的改进使得撒哈拉沙漠和南半球中纬度海洋大气顶净太阳辐射的模拟也有所改进,而这将直接影响地表温度尤其是陆地表面温度。而不同气溶胶方案在赤道海洋上引起的云反馈不仅引起辐射的改变,还将对降水产生明显影响。     

The aerosol module in the INM RAS climate model

The aerosol module is included into the INM RAS climate model. The module computes the evolution of main aerosols: sea salt, mineral dust, sulfate aerosol, and black and organic carbon. Aerosol surface fluxes, advection, gravitational sedimentation, surface absorption, and scavenging by precipitation are taken into account to compute aerosol concentration variations. Model aerosol distribution is used to compute radiation fluxes. The ten-year run of the climate model is performed. The climatology of model aerosol is considered. The aerosol mass, integral source values, optical thickness, and radiative forcing are presented. The results are compared with the data of other models and observations.     

Aerosol direct forcing of the summer Indian monsoon as simulated by the NCAR CAM3

In this study, the effects of aerosols on the simulation of the Indian monsoon by the NCAR Community Atmosphere Model CAM3 are measured and investigated. Monthly mean 3D mass concentrations of soil dust, black and organic carbons, sulfate, and sea salt, as output from the GOCART model, are interpolated to mid-month values and to the horizontal and vertical grids of CAM3. With these mid-month aerosol concentrations, CAM3 is run for a period of approximately 16 months, allowing for one complete episode of the Indian monsoon. Responses to the aerosols are measured by comparing the mean of an ensemble of aerosol-induced monsoon simulations to the mean of an ensemble of CAM3 simulations in which aerosols are omitted, following the method of Lau et al. (2006) in their experiment with the NASA finite volume general circulation model. Additionally, an ensemble of simulations of CAM3 using climatological mid-month aerosol concentrations from the MATCH model is composed for comparison. Results of this experiment indicate that the inclusion of aerosols results in drops in surface temperature and increases in precipitation over central India during the pre-monsoon months of March, April, and May. The presence of aerosols induces tropospheric shortwave heating over central India, which destabilizes the atmosphere for enhanced convection and precipitation. Reduced shortwave heating and enhanced evaporation at the surface during April and May results in reduced terrestrial emission to cool the lower troposphere, relative to simulations with no aerosols. This effect weakens the near-surface cyclonic circulation and, consequently, has a negative feedback on precipitation during the active monsoon months of June and July.     

中国区域气溶胶对东亚夏季风的可能影响（I）：硫酸盐气溶胶的影响

利用NCAR的新一代GCM CAM3.0模式离线耦合一个气溶胶同化系统,模拟研究了中国区域硫酸盐气溶胶的直接气候效应对东亚夏季风及其降水的影响。结果显示：中国区域硫酸盐气溶胶引起全球平均的直接辐射强迫为-0.25 W/m²,中国内陆约25°N以北普遍降温,而海表温度升高。由此导致海陆温差缩小,东亚夏季风强度减弱,中国地区季风降水明显减少,而尤以积云降水减少起主要作用。硫酸盐气溶胶对中国地区的对流活动起抑制作用。     

中国区域气溶胶对东亚夏季风的可能影响（I）：硫酸盐气溶胶的影响

 利用NCAR的新一代GCM CAM3.0模式离线耦合一个气溶胶同化系统,模拟研究了中国区域硫酸盐气溶胶的直接气候效应对东亚夏季风及其降水的影响。结果显示：中国区域硫酸盐气溶胶引起全球平均的直接辐射强迫为-0.25 W/m²,中国内陆约25°N以北普遍降温,而海表温度升高。由此导致海陆温差缩小,东亚夏季风强度减弱,中国地区季风降水明显减少,而尤以积云降水减少起主要作用。硫酸盐气溶胶对中国地区的对流活动起抑制作用。     

夏季硫酸盐和黑碳气溶胶对中国云特性的影响

利用WRF-Chem（Weather Research and Forecasting model coupled with Chemistry）模式研究2006年8月1日—9月1日中国区域硫酸盐和黑碳气溶胶对云特性的影响。模式验证利用了卫星和地面观测的气象要素、化学物质浓度、气溶胶光学特性和云微物理特性。模式性能评估表明该模式能较好地抓住气象要素（温度、降水、相对湿度和风速）的量级和空间分布特征。通过与地面观测和MODIS卫星数据对比发现,尽管模式模拟还存在偏差,但还是能较好模拟出气溶胶物种的地表浓度、气溶胶光学厚度（AOD）、云光学厚度（COD）、云量（CLDF）、云顶云滴有效半径（CER）和云水路径（LWP）。通过两个敏感性试验（分别增加二氧化硫和黑碳排放量至控制试验排放的3倍）与控制试验的对比发现硫酸盐比黑碳更易成为云凝结核,在中国东部云顶云滴数浓度和其它云特性参数对二氧化硫排放增加的响应均从北向南呈递增,这与地面湿度分布有关。云滴有效半径对硫酸盐气溶胶的响应符合气溶胶第一间接效应的定义,即硫酸盐气溶胶增多,云滴数浓度增加,云滴有效半径减少,但是对黑碳气溶胶的响应在各区域不尽相同。还发现黑碳对云量的影响远大于硫酸盐,主要原因是由于黑碳气溶胶直接辐射效应（对太阳光的吸收）导致的云的“燃烧”作用。      

Direct Climatic Effect of Aerosols and Interdecadal Variations over East Asia Investigated by a Regional Coupled Climate-chemistry/aerosol Model

The direct climatic effect of aerosols for the 1980-2000 period over East Asia was numerically investigated by a regional scale coupled climate-chemistry/aerosol model,which includes major anthropogenic aerosols(sulfate,black carbon,and organic carbon) and natural aerosols(soil dust and sea salt) .Anthropogenic emissions used in model simulation are from a global emission inventory prepared for the Intergovernmental Panel on Climate Change Fifth Assessment Report(IPCC AR5) ,whereas natural aerosols are calculated online in the model.The simulated 20-year average direct solar radiative effect due to aerosols at the surface was estimated to be in a range of-9--33 W m-2 over most areas of China,with maxima over the Gobi desert of West China,and-12 W m-2 to-24 W m-2 over the Sichuan Basin,the middle and lower reaches of the Yellow River and the Yangtze River.Aerosols caused surface cooling in most areas of East Asia,with maxima of-0.8-C to-1.6-C over the deserts of West China,the Sichuan Basin,portions of central China,and the middle reaches of the Yangtze River. Aerosols induced a precipitation decrease over almost the entire East China,with maxima of-90 mm/year to-150 mm/year over the Sichuan Basin,the middle reaches of the Yangtze River and the lower reaches of the Yellow River.Interdecadal variation of the climate response to the aerosol direct radiative effect is evident,indicating larger decrease in surface air temperature and stronger perturbation to precipitation in the 1990s than that in the 1980s,which could be due to the interdecadal variation of anthropogenic emissions.     

Direct Radiative Forcing and Climatic Effects of Aerosols over East Asia by RegCM3

The authors used a high-resolution regional climate model(RegCM3) coupled with a chemistry/aerosol module to simulate East Asian climate in 2006 and to test the climatic impacts of aerosols on regionalscale climate.The direct radiative forcing and climatic effects of aerosols(dust,sulfate,black carbon,and organic carbon) were discussed.The results indicated that aerosols generally produced negative radiative forcing at the top-of-the-atmosphere(TOA) over most areas of East Asia.The radiative forcing induced by aerosols exhibited significant seasonal and regional variations,with the strongest forcing occurring in summer.The aerosol feedbacks on surface air temperature and precipitation were clear.Surface cooling dominated features over the East Asian continental areas,which varied in the approximate range of-0.5 to-2°C with the maximum up to-3-C in summer over the deserts of West China.The aerosols induced complicated variations of precipitation.Except in summer,the rainfall generally varied in the range of-1 to 1 mm d-1 over most areas of China.     

Particulate carbon content in rain at various temperate and tropical locations

Particulate organic and black carbon concentrations in rain were determined in various source or remote regions, in order to gain information on the incorporation of atmospheric carbonaceous particles in hydrometeors. The analyses of rainwaters indicate that all the samples contained particles derived from combustion. Data obtained on a sample basis, show an important areal and temporal variability of the composition of rain carbonaceous particles, a variability which is reported to that of the black carbon to total carbon ratio, Cb/Ct, ranging from 10 to 72%. In addition to the fluctuations of the aerosol atmospheric burden, these variations may be related to alterations of the organic fraction of the particles or their involvement in in-cloud nucleation processes during atmospheric transport. Also, a comparison of the mean relative abundance of black carbon in aerosols and in rainwaters, gives evidence of a partial disappearance of the organic particles, a phenomenon which could be due to their dissolution when incorporated in the hydrometeors. Precipitation scavenging ratio values of black carbon particles, which range from 100 to 370, are similar to those found for sulphate anthropogenic aerosols. Due to their hygroscopic properties and mean size, black carbon aerosols could possibly trace the physico-chemical processes involved in the incorporation of fine combustion particles into hydrometeors. It is also suggested that smoke particles may act as cloud condensation nuclei (CCN). Consequently, emissions of particulates derived from combustion in some tropical or industrial regions could result locally in alteration of cloud albedo and precipitation regimes.     

Episode Simulation of Asian Dust Storms with an Air Quality Modeling System

A dust deflation module was developed and coupled with the air quality modeling system RAMS-CMAQ to simultaneously treat all the major tropospheric aerosols（i.e.,organic and black carbons,sulfate,nitrate, ammonia,soil dust,and sea salt）.Then the coupled system was applied to East Asia to simulate Asian dust aerosol generation,transport and dry/wet removal processes during 14-25 March 2002 when two strong dust storms occurred consecutively.To evaluate model performance and to analyze the observed features of dust aerosols over the East Asian region,model results were compared to concentrations of suspended particulate matter of 10μm or less(PM₁₀;1-h intervals) at four remote Japanese stations and daily air pollution index （API） values for PM₁₀ at four large Chinese cities.The modeled values were generally in good agreement with observed data,and the model reasonably reproduced two dust storm outbreaks and generally predicted the dust onset and cessation times at each observation site.In addition,hourly averaged values of aerosol optical thickness（AOT） were calculated and compared with observations at four Aerosol Robotic Network （AERONET） stations to assess the model’s capability of estimating dust aerosol column burden.Analysis shows that modeled and observed AOT values were generally comparable and that the contribution of dust aerosols to AOT was significant only with regard to their source regions and their transport paths.