基于格点资料的四川大气混合层高度特征及与空气质量的关系

基于2018年1月~2020年12月中国气象局陆面数据同化系统（CLDAS）资料，利用罗氏法计算四川省大气混合层高度，分析其时空分布特征，并结合大气环境空气质量监测数据，讨论大气混合层高度变化与空气质量的关系。结果表明:四川省大气混合层高度呈西高东低分布特征。盆地与攀西地区、川西高原大气混合层高度季节变化有显著性差异，盆地春季最高，秋季最低；川西高原和攀西地区秋季最高，夏季最低。四川省各地区大气混合层高度月、日变化趋势基本一致。四川省大气混合层高度与O₃质量浓度呈显著正相关关系，与PM_2.5质量浓度呈显著负相关关系。      

珠三角地区日最大混合层高度及其对 区域空气质量的影响

大气混合层高度是影响大气扩散的主要因子之一,其对空气质量评估与污染物的存储量及分布起着重要作用。利用2014年4月至2018年3月珠三角地区香港（沿海站点）和清远（内陆站点）气象探空数据,采用干绝热曲线法估算代表大气垂直方向上大气混合能力的最大混合层高度,探讨沿海与内陆地区混合层高度的差异性,并将最大混合层高度估算值与地面观测的污染物浓度进行相关性分析。结果表明：珠三角沿海与内陆地区的混合层变化具有典型局地特征,沿海日最大混合层高度普遍低于内陆,两地平均高度分别为982 m和1198 m。区域混合层高度的空间差异性由多方面原因造成,其中温度日较差起到关键作用。由于海洋水体的气温调节作用,沿海地区温度日较差较小,因此混合层发展相对较低。珠三角地区各污染物浓度与混合层高度的相关性有较大差异,其中以CO为代表的一次污染物与混合层高度间呈显著负相关,以O₃为代表的二次污染物与混合层高度间则呈显著正相关,而颗粒物作为多源性污染物（既有一次排放,又有二次生成）,其与混合层高度之间的相关性较弱。     

青藏高原东部大气探空廓线的气候特征分析

通过对青藏高原东部地区近几年部分探空资料的分析,得出了一些有意义的结论。结果表明:冬季,青藏高原东侧地区在对流层下部存在明显的逆温现象,在逆温层之下,大气相对湿度大,水汽随高度减小的幅度小,大气处于中性层结状况;在此逆温层之上,大气相对湿度小。在逆温层底部有大量的水汽堆积,在空中形成明显的逆湿层,而在高原主体上并没有此逆温层的存在,高原东侧各站逆温层底的高度差别不大。夏季,青藏高原东侧地区20时可以存在明显的混合层,混合层的高度在成都站最小,重庆站最大,而高原主体混合层高度大于东侧地区。旱年混合层高度大于涝年。8时和20时,冬季大气温、湿垂直特性变化不明显,而夏季具有明显的变化。夏季,降水过程明显抑制混合层的发展,在暴雨过程及其前后,混合层有明显的成熟、消亡、重新建立的特征。     

青藏高原东部大气探空廓线的气候特征分析

通过对青藏高原东部地区近几年部分探空资料的分析,得出了一些有意义的结论。结果表明：冬季,青藏高原东侧地区在对流层下部存在明显的逆温现象,在逆温层之下,大气相对湿度大,水汽随高度减小的幅度小,大气处于中性层结状况;在此逆温层之上,大气相对湿度小。在逆温层底部有大量的水汽堆积,在空中形成明显的逆湿层,而在高原主体上并没有此逆温层的存在,高原东侧各站逆温层底的高度差别不大。夏季,青藏高原东侧地区20时可以存在明显的混合层,混合层的高度在成都站最小,重庆站最大,而高原主体混合层高度大于东侧地区。旱年混合层高度大于涝年。8时和20时,冬季大气温、湿垂直特性变化不明显,而夏季具有明显的变化。夏季,降水过程明显抑制混合层的发展,在暴雨过程及其前后,混合层有明显的成熟、消亡、重新建立的特征。     

编程求解混合层高度的方法

在t-lnp图上利用08时、14时气压和最低气温、最高气温,经过坐标转换求解早晨、中午混合层的气压和温度,然后根据等温大气压高公式计算混合层高度.该计算方法用VB 6.0编程,可自动从当日报文中读取数据,计算出混合层高度值,也可根据数值预报结果计算次日混合层高度.     

编程求解混合层高度的方法

在t-lnp图上利用08时、14时气压和最低气温、最高气温，经过坐标转换求解早晨、中午混合层的气压和温度，然后根据等温大气压高公式计算混合层高度。该计算方法用VB6．0编程，可自动从当日报文中读取数据，计算出混合层高度值，也可根据数值预报结果计算次日混合层高度。     

北京城市大气混合层与气溶胶垂直分布观 测研究

2002年3～10月在北京大学利用微脉冲激光雷达(MPL)观测了气溶胶时空变化。提出一种反演混合层高度的方法,这种方法减小了仪器订正的误差,反演的混合层高度与探空测量结果有很好的一致性。利用该方法计算了观测期间晴天无云天气条件下的混合层高度,分析了混合层高度及其增长率的日变化、季节变化,初步研究了混合层高度和近地面气溶胶分布的相互关系,分析了表征大气扩散能力的通风系数的日变化。结果表明,利用MPL监测城市混合层是可行的和优越的。     

一个混合层高度发展的数值模拟试验

本文利用在ＨＥＩＦＥ期间戈壁地区采集的资料，并用一个考虑由地表热力及动力强的害和高空下沉等因子控制的零阶跳跃模式，对该地区白天混层高度增长的机制进行了数值模拟分析，结果表明：白天混合层高的增长受来自祁连山强烈的下沉冷空气的影响较大，使其高度的增长受到抑制，且最大值出现的时间超前，其结果与声雷达回波强度确定的混合层高度吻合较好。     

基于激光雷达和微波辐射计观测确定混合层高度方法的比较

利用苏州地区2010年1月4,7,16日和2月4日4天的激光雷达及微波辐射计观测资料,比较了不同遥感手段探测晴天大气混合层高度的差异,发现试验期间该地区的混合层高度在300~1500 m之间。利用梯度法、标准偏差法、小波法从激光雷达数据中提取混合层高度并进行了对比,结果表明三种方法都能较好地反演混合层高度并且一致性较好,三者差异主要存在于大气边界层的发展和消亡阶段;梯度法和小波法结果无明显差异,而标准偏差法结果稍高于其他方法。在此基础上,利用微波辐射计探测的大气温度,使用温度梯度法估算大气混合层高度,并与激光雷达探测结果进行了比较,结果表明,大多数情况下激光雷达探测结果高于微波辐射计观测结果;两种遥感手段有较好的相关性,相关系数为0.76。激光雷达同微波辐射计结果存在差异,尤其是在边界层的发展和消散阶段,这是由两种遥感手段探测原理不同造成的。     

激光雷达和探空反演的混合层高度对比分析

本文利用2016年12月至2017年11月期间晴朗少云天气下的成都微脉冲激光雷达观测数据反演的混合层高度,与温江探空资料确定的混合层高度进行了对比和误差分析,结果表明:基于探空资料和激光雷达数据反演的混合层高度具有较好的一致性,两者相关系数达0.75,激光雷达反演的混合层高度略低于基于探空资料确定的值,在混合层高度为1000～2000m时,两种方法计算所得的值偏差幅度最小,约为20%;在1000m以内和2000m以上,偏差幅度略有增大,为26%;两种方法反演的混合层高度变化趋势较为一致,均呈现出12月、1月较低,4月、5月较高的特点;混合层高度具有明显的日变化特征:上午混合层高度迅速增高,午后增长速度减慢并发展到最大高度,日落后迅速降低;混合层内相对湿度的增加、残留层的存在是导致激光雷达反演混合层高度时产生较大误差的原因之一。     

热带西太平洋边界层的多层结构分析

本文主要利用第一次“中美热带西太平洋海气相互作用联合调查”所获得的海洋水文、气象及大气探测资料,分析了热带西太平洋暖水区边界层大气层结特征,指出热带西太平洋边界层大气具有多层结构和多层送温现象,边界层内各层厚度及气温、位温、混合比随高度的变化趋势如下:超绝热层位于地面以上50m左右,气温、位温、混合比迅速减小,系绝热不稳定层;第一层为混合层,平均厚度为351m,位温、混合比变化不明显;混合层上又是逆温层大多为30—100m厚,位温迅速增大,混合比迅速减小,系绝对稳定层;700—1000m为浅对流云活跃层,     

Convective mixing in the monsoon boundary layer

Aerological observations over a tropical inland station collected during different phases of the Indian summer monsoon have been used to study the convective mixing in the monsoon boundary layer. The mixing line (ML) model for the thermodynamic structure of a partially cloudy boundary layer has been used to estimate the mixing by convection. The ML model together with the saturation point approach is able to depict different convective mixing regimes in the monsoon boundary layer.     

Application of Linear Thermodynamics to the Atmospheric System.Part Ⅱ: Exemplification of Linear Phenomenological Relations in the Atmospheric System

将边界层相似性理论同线性热力学理论结合，间接地以观测实验事实证明大气边界层内线性唯象关系是成立的，而且线性湍流输送系数同相应的线性唯象系数成正比关系。但实验事实表明，大涡对流的混合层线性唯象系数成正比关系。但实验事实表明，大涡对流的混合层线性唯象关系是不成立的，混合层内湍流输送过程是一种强的非线性过程。所以，对流边界层是一种远离平衡态非线性区的热力学状态。地转风和热成风是一种大气系统特有的动力过程和热力过程和交叉耦合现象，这是大气系统交叉耦合现象的一个实际例证。     

Meso-scale variations of the urban mixing height

Local variations in the summertime mixing height over metropolitan St. Louis, Missouri, are examined in order to evaluate the dynamical and thermodynamical influences of an urban area. Case studies employing aircraft, lidar, pilot balloon and radiosonde data from Project METROMEX show variations in the height of a temperature inversion which caps a deep mixing layer. A dome-like lifting of the inversion structure occurs over the urban-industrial center with subsidence of the inversion layer at the perimeter of the metropolitan area. The maximum amplitude of the dome occurs shortly after mid-day, suggesting that thermal influences are primarily responsible.     

黑河绿洲区不均匀下垫面大气边界层结构的大涡模拟研究

采用RAMS模式中大涡模拟的方法,加入高分辨率的植被和土壤资料,模拟了黑河（张掖地区）不均匀下垫面条件下大气边界层演变过程。分析了模拟的地表通量、边界层的平均结构和湍流二阶量,并用黑河试验的观测资料检验了模式的模拟性能。结果表明,模拟的平均结构较好地展现了不均匀下垫面条件下边界层内从稳定层结到混合层发展,夹卷层形成,底层逆温层出现,混合层过渡到残留层等的演变过程,呈现出了从初始的稳定边界层发展到对流边界层,最后又形成夜问稳定边界层的日变化规律。湍流二阶量的分析显示,在非均匀下垫面条件下边界层内湍流二阶量的垂直分布与边界层的发展相对应,白天湍流二阶量出现两个峰值,分别位于近地层和混合层顶。与观测资料和现有研究的对比表明,RAMS中陆面模块（LEAF）地表参数不能较好地反映黑河地区的植被特征,模拟的白天地表感热和潜热通量偏小,气温白天偏低、夜间偏高,相对湿度也有偏差。     

Observations of reversal of mixing ratio in the atmospheric boundary layer over the Arabian sea

Analysis of the radiosonde observations over the Arabian sea region during MONSOON-77 and MONEX-79 has revealed a reversal in the mixing ratio (QR) above the inversion/stable layer in the atmospheric boundary layer. The reversal could be attributed to the detrainment of cloudy air originating in the deep moist convection which has penetrated the inversion layer in nearby areas. It was noticed that the soundings in which a reversal of mixing ratio was not observed, were associated with meteorological conditions favourable for deep convection.     

Numerical simulation for the effects of PBL and the surface on pollutant concentrations

On the basis of theoretical and experimental results of study of planetary boundary layer (PBL), the physical parameters describing the structure of PBL are calculated by using the data obtained from a meteor-ological tower and the effects of PBL and the surface on pollutant concentrations are numerically simulated with a time-dependent two-dimensional advection and diffusion equation.It is shown that the diurnal variation of PBL results in that of concentration. The height of mixing layer is an important factor to determine the ground-level concentration. As for an elevated point source, the height of mixing layer, growing from lower to higher than the releasing height is a necessary condition for the phenomenon of fumigation. It is also shown that the surface may be considered as a boundary with perfect reflection when Vd ≤ 0.001 m s-1, but has an important effect on concentration and must be carefully dealt with when Vd ≤ 0.01 m s-1.     

Evaluation of Mixing-Height Retrievals from Automatic Profiling Lidars and Ceilometers in View of Future Integrated Networks in Europe

The determination of the depth of daytime and nighttime mixing layers must be known very accurately to relate boundary-layer concentrations of gases or particles to upstream fluxes. The mixing-height is parametrized in numerical weather prediction models, so improving the determination of the mixing height will improve the quality of the estimated gas and particle budgets. Datasets of mixing-height diurnal cycles with high temporal and spatial resolutions are sought by various end users. Lidars and ceilometers provide vertical profiles of backscatter from aerosol particles. As aerosols are predominantly concentrated in the mixing layer, lidar backscatter profiles can be used to trace the depth of the mixing layer. Large numbers of automatic profiling lidars and ceilometers are deployed by meteorological services and other agencies in several European countries providing systems to monitor the mixing height on temporal and spatial scales of unprecedented density. We investigate limitations and capabilities of existing mixing height retrieval algorithms by applying five different retrieval techniques to three different lidars and ceilometers deployed during two 1-month campaigns. We studied three important steps in the mixing height retrieval process, namely the lidar/ceilometer pre-processing to reach sufficient signal-to-noise ratio, gradient detection techniques to find the significant aerosol gradients, and finally quality control and layer attribution to identify the actual mixing height from multiple possible layer detections. We found that layer attribution is by far the most uncertain step. We tested different gradient detection techniques, and found no evidence that the first derivative, wavelet transform, and two-dimensional derivative techniques have different skills to detect one or multiple significant aerosol gradients from lidar and ceilometer attenuated backscatter. However, our study shows that, when mixing height retrievals from a ultraviolet lidar and a near-infrared ceilometer agreed, they were 25?C40% more likely to agree with an independent radiosonde mixing height retrieval than when each lidar or ceilometer was used alone. Furthermore, we point to directions that may assist the layer attribution step, for instance using commonly available surface measurements of radiation and temperature to derive surface sensible heat fluxes as a proxy for the intensity of convective mixing. It is a worthwhile effort to pursue such studies so that within a few years automatic profiling lidar and ceilometer networks can be utilized efficiently to monitor mixing heights at the European scale.     

A parameterization of the nocturnal ozone reduction in the residual layer by verticla downward mixing during summer smog situations using sodar data

The reduction of ozone in the nocturnal residual layer by vertical mixing to the surface was investigated for several summer smog episodes on the Swiss plateau in the years 1990 and 1991. Using a limited data set of SODAR measurements and surface ozone concentrations, a parameterization of the ozone depletion in the nocturnal residual layer due to vertical mixing to the ground is proposed. This model is not intended to be physically complete but is rather simple with limited input information required. The nocturnal ozone reduction within the whole planetary boundary layer (nocturnal boundary layer plus residual layer) over the complex terrain of the Swiss plateau for the days investigated is between 20 and 50%.