THE IMPACT OF RELATIVE HUMIDITY ON THE RADIATIVE PROPERTY AND RADIATIVE FORCING OF SULFATE AEROSOL*

With the data of complex refractive index of sulfate aerosol,the radiative properties of the aerosol under 8 relative humidity conditions are calculated in this paper.By using the concentration distribution from two CTM models and LASG GOALS/AGCM,the radiative forcing due to hygroscopic sulfate aerosol is simulated.The results show that:(1)With the increase of relative humidity,the mass extinction coefficiency factor decreases in the shortwave spectrum;single scattering albedo keeps unchanged except for a little increase in longwave spectrum,and asymmetry factor increases in whole spectrum.(2)Larger differences occur in radiative forcingsimulated by using two CTM data,and the global mean forcing is -0.268 and -0.816 W/m²,respectively.(3)When the impact of relative humidity on radiative property is taken into account,the distribution pattern of radiative forcing due to the wet particles is very similar to that of dry sulfate,but the forcing value decreases by 60%.     

THE IMPACT OF RELATIVE HUMIDITY ON THE RADIATIVE PROPERTY AND RADIATIVE FORCING OF SULFATE AEROSOL

With the data of complex refractive index of sulfate aerosol,the radiative properties of theaerosol under 8 relative humidity conditions are calculated in this paper.By using the concentrationdistribution from two CTM models and LASG GOALS/AGCM,the radiative forcing due tohygroscopic sulfate aerosol is simulated.The results show that:(1)With the increase of relativehumidity,the mass extinction coefficiency factor decreases in the shortwave spectrum;singlescattering albedo keeps unchanged except for a little increase in longwave spectrum,andasymmetry factor increases in whole spectrum.(2)Larger differences occur in radiative forcingsimulated by using two CTM data,and the global mean forcing is—0.268 and—0.816 W/m~2,respectively.(3)When the impact of relative humidity on radiative property is taken into account,the distribution pattern of radiative forcing due to the wet particles is very similar to that of drysulfate,but the forcing value decreases by 60%.     

硫酸盐和烟尘气溶胶辐射特性及辐射强迫的模拟估算

利用已有的硫酸盐和烟尘气溶胶折射指数资料，精确计算了这两种气溶胶从太阳短波到红外谱段的辐射特性。然后，在LLNL化学输送模式(CTM)模拟的硫酸盐和烟尘气溶胶资料及改进的气溶胶参数化基础上，在国内首次用GCM估算了这两种气溶胶引起的全球辐射强迫。结果表明:(1)西欧是全球最大的硫酸盐辐射强迫中心，最大值出现在夏季，达-5.0W/m2；(2)烟尘强迫的最大中心出现在夏季的南美和非洲中南部，为4.0W/m2；(3)南半球大陆人为气溶胶的强迫不容忽视；(4)某些地区人为气溶胶的强迫在量值上可与CO2等温室气体引起的强迫相比拟。     

一个简单的雪晶辐射参数化方案及雪晶辐射对中尺度降水的影响

文章提出一个简单的雪晶辐射性质参数化方案, 并利用1998年6月8日华南暴雨资料研究了雪晶的辐射性质对于中尺度降水的影响。结果表明:雪晶的辐射性质对中尺度降水的影响是不可忽略的, 白天尤为显著; 它能够明显地改变中尺度降水的局部特征, 特别是降水中心的强度和位置, 而对降水的分布影响不大。因此, 建立独立的雪晶辐射参数化对提高中尺度模式对中尺度降水的预报能力是必要的。     

Four-stream Radiative Transfer Parameterization Scheme in a Land Surface Process Model

Accurate estimates of albedos are required in climate modeling. Accurate and simple schemes for radiative transfer within canopy are required for these estimates, but severe limitations exist. This paper developed a four-stream solar radiative transfer model and coupled it with a land surface process model. The radiative model uses a four-stream approximation method as in the atmosphere to obtain analytic solutions of the basic equation of canopy radiative transfer. As an analytical model, the four-stream radiative transfer model can be easily applied efficiently to improve the parameterization of land surface radiation in climate models. Our four-stream solar radiative transfer model is based on a two-stream short wave radiative transfer model. It can simulate short wave solar radiative transfer within canopy according to the relevant theory in the atmosphere. Each parameter of the basic radiative transfer equation of canopy has special geometry and optical characters of leaves or canopy. The upward or downward radiative fluxes are related to the diffuse phase function, the G-function, leaf reflectivity and transmission, leaf area index, and the solar angle of the incident beam. The four-stream simulation is compared with that of the two-stream model. The four-stream model is proved successful through its consistent modeling of canopy albedo at any solar incident angle. In order to compare and find differences between the results predicted by the four- and two-stream models, a number of numerical experiments are performed through examining the effects of different leaf area indices, leaf angle distributions, optical properties of leaves, and ground surface conditions on the canopy albedo. Parallel experiments show that the canopy albedos predicted by the two models differ significantly when the leaf angle distribution is spherical and vertical. The results also show that the difference is particularly great for different incident solar beams. One additional experiment is carried out to evaluate the simulations of the BATS land surface model coupled with the two- and four-stream radiative transfer models. Station observations in 1998 are used for comparison. The results indicate that the simulation of BATS coupled with the four-stream model is the best because the surface absorbed solar radiation from the four-stream model is the closest to the observation.     

利用ERBE资料分析中国地区云辐射强迫的时空变化

利用１９８５￣１９８８年４年的ＥＲＢＥ资料,分析和揭示了我国大陆地区云辐射强迫变化的一些基本事实。结果发现：云强迫存在很大的区域差异和较强的季节变化,其中川黔地区是全国最大的云强迫负值区,其次是长江中下游地区和华北地区青藏高原为正、负值的过渡区,高原北侧的西北干旱区冬季为较弱的云强迫正值区。此外,云强迫还具有一定的年际变化。     

中国沙漠沙尘气溶胶对沙漠源区及北太平洋地区大气辐射加热的影响

针对2001年春季中国沙漠和北太平洋上空沙尘气溶胶的空间分布情况，利用辐射传输模式，分别计算了沙尘气溶胶对沙漠和海洋大气的辐射加热（冷却）率，并讨论了低云、中云、高云对辐射加热率的影响。结果表明:春季，位于中国沙漠和太平洋上空的沙尘层对大气具有明显的加热作用。当沙漠上空光学厚度为1.0，海洋上空光学厚度为0.3时，取春季平均太阳高度角，沙尘层对应的净辐射加热率分别为2.8 K/d和0.4 K/d。由于WMO推荐的沙尘模型比东亚沙尘模型对太阳辐射吸收强，采用该模型计算得到的中国沙漠和海洋上空的加热率比采用东亚沙尘模型分别高1.5 K/d和0.2 K/d。沙尘对大气的加热率很大程度上依赖于沙尘的大气载荷。这种依赖性首先受太阳高度角的影响， 其次也受地表反照率的影响。云对沙尘层辐射加热（冷却）率的影响与云的高度和厚度有关。低云能够加热沙漠和海洋上空的沙尘大气，冷却地面和洋面。中、高云冷却沙漠上空的沙尘层。在海洋上空，中云对云层以上的沙尘层有加热作用，对云层以下的沙尘层有冷却作用。高云对海洋上空沙尘层的辐射加热（冷却）率的影响比较小，加热还是冷却，取决于云的厚度，当云层较薄时，加热沙尘层，而当云层较厚的时候，有可能冷却沙尘层。     

Direct Climatic Effect of Dust Aerosol in the NCAR Community Atmosphere Model Version 3 （CAM3）

Direct climate responses to dust shortwave and longwave radiative forcing (RF) are studied using the NCAR Community Atmosphere Model Version 3 (CAM3). The simulated RF at the top of the atmosphere (TOA) is-0.45 W m-2 in the solar spectrum and +0.09 W m-2 in the thermal spectrum on a global average. The magnitude of surface RF is larger than the TOA forcing, with global mean shortwave forcing of-1.76 W m-2 and longwave forcing of +0.31 W m-2 . As a result, dust aerosol causes the absorption of 1.1 W m-2 in t...     

黑碳气溶胶辐射强迫全球分布的模拟研究

利用一个改进的辐射传输模式,结合全球气溶胶数据集（GADS）,计算晴空条件下冬夏两季黑碳气溶胶的直接辐射强迫在对流层顶和地面的全球分布。计算结果表明,与温室气体引起的整层大气都是正的辐射强迫不同,黑碳气溶胶的辐射强迫在对流层顶为正值,而在地面的辐射强迫却是负值。作者从理论上解释了造成这种结果的原因。对北半球冬季和夏季而言,在对流层顶黑碳气溶胶的全球辐射强迫的平均值分别为0.085W/m2和0.155 W/m2,在地面则分别为-0.37 W/m2和-0.63 W/m2。虽然气溶胶的辐射强迫主要依赖于其本身的光学性质和在大气中的浓度,太阳高度角和地表反照率对黑碳气溶胶的辐射强迫会产生很大的影响。研究指出:黑碳气溶胶在对流层顶正的辐射强迫和在地面负的辐射强迫的绝对值都随太阳天顶角的余弦和地表反照率的增加线性增大;地表反照率对黑碳气溶胶辐射强迫的强度和分布都有重要影响。黑碳气溶胶的辐射强迫分布具有明显的纬度变化特征,冬夏两季的大值区都位于30°N~90°N之间,表明人类活动是造成黑碳气溶胶辐射强迫的主要原因。     

青藏高原地气系统云辐射强迫的气候学特征

利用ＥＲＢＥ－Ｓ４和ＩＳＣＣＰ－Ｃ２月平均资料着重分析了青藏高原这一特殊气候区域地气系统云辐射强拓的气候学特征，分析结果表明，冬，夏季云对气系统辐射强迫的场分布形势有明显的差异，对于地气系统长波辐射，冬季高原主体云强迫高值区，夏季云强迫空间变化平缓，高原主体平均云的温室效应春季最大，秋季最小，云使地气系统射出长波辐射年平均减少４５．６Ｗ／ｍ＾２对于地气系统短波辐射，冬季高原地区云强迫相对高值区，夏     

THE RADIATIVE EFFECTS OF ANTHROPOGENIC AEROSOLS OVER CHINA AND THEIR SENSITIVITY TO SOURCE EMISSION

In this paper,the RIEMS 2.0 model,source emission in 2006 and 2010 are used to simulate the distributions and radiative effects of different anthropogenic aerosols over China.The comparison between the results forced by source emissions in 2006 and 2010 also reveals the sensitivity of the radiative effects to source emission.The results are shown as follows:(1) Compared with those in 2006,the annual average surface concentration of sulfate in 2010 decreased over central and eastern China with a range of-5 to 0 μg/m~3;the decrease of annual average aerosol optical depth of sulfate over East China varied from 0.04 to 0.08;the annual average surface concentrations of BC,OC and nitrate increased over central and eastern China with maximums of 10.90,11.52 and 12.50μg/m~3,respectively;the annual aerosol optical depths of BC,OC and nitrate increased over some areas of East China with extremes of 0.006,0.007 and 0.008,respectively.(2)For the regional average results in 2010,the radiative forcings of sulfate,BC,OC,nitrate and their total net radiative forcing at the top of the atmosphere over central and eastern China were-0.64,0.29,-0.41,-0.33 and-1.1 W/m~2,respectively.Compared with those in 2006,the radiative forcings of BC and OC in 2010 were both enhanced,while that of sulfate and the net radiative forcing were both weakened over East China mostly.(3)The reduction of the cooling effect of sulfate in 2010 produced a warmer surface air temperature over central and eastern China;the maximum value was 0.25 K.The cooling effect of nitrate was also slightly weakened.The warming effect of BC was enhanced over most of the areas in China,while the cooling effect of OC was enhanced over the similar area,particularly the area between Yangtze and Huanghe Rivers.The net radiative effect of the four anthropogenic aerosols generated the annual average reduction and the maximum reduction were-0.096 and-0.285 K,respectively,for the surface temperature in 2006,while in 2010 they were-0.063 and-0.256 K,respectively.In summary,the change in source emission lowered the cooling effect of anthropogenic aerosols,mainly because of the enhanced warming effect of BC and weakened cooling effect of scattering aerosols.     

一个三维Monte-Carlo地气耦合辐射传输模式

建立了一个可靠和较高计算效率的三维Monte-Carlo地气耦合辐射传输模式(3DMC).该模式在光子释放和定位、地气耦合、辐射率高分辨模拟计算和计算效率等方面有所发展.     

大气气溶胶变化对农业影响的研究进展

随着工业化和城市化的迅速发展,大气气溶胶含量和种类明显增加,它们通过直接吸收和反射太阳辐射以及改变其它辐射强迫因子(云、臭氧)的大小间接影响地气系统的能量收支,从而影响气候。气溶胶变化对气候的影响已有较多的研究,而对植被(农业)的影响是一个相对较新的研究领域,文章简要概述了大气气溶胶辐射强迫效应和大气气溶胶对农业的影响研究现状及国内外主要研究成果,并对气溶胶监测方法及模式评估方面可能存在的问题作了简单的分析。     

利用多模传输理论求解块状云的辐射特征

实际云层在水平与垂直方向都是不均匀的,但为了便于计算,绝大多数关于云辐射的理论模式,都采用平面平行模式.到目前为止,解决三维空间辐射传输问题的方法仍然不多.一般采用统计方法和二流近似法,但这两种方法分别在计算机时和计算精度上受到限制.作者在三维多模传输理论与辐射传输计算程序软件包--DISORT的基础上,发展出计算三维孤立云块多次散射过程的一套程序(MM-DISORT),并由此初步探讨了云块的三维立体结构对云的短波吸收的影响.     

卫星对地观测中大气与地表辐射贡献的参数化

卫星对地观测定量遥感地表与大气特性是当前地球科学与应用研究的关键手段之一。在定量遥感中区分大气和地表在地-气系统对空间散射辐射中各自的贡献与作用是关键的一步。这一问题的核心是基于辐射传输方程的数值计算建立起适合应用于遥感反演中分离大气与地表贡献的参数化表达式。本文对特定的气溶胶气候类型和可见/近红外波段建立起定量的表达形式,并对表达式的物理含义和拟合精度进行了分析。最后讨论了其应用的可行性和进一步的工作。     

Modeling Study of the Global Distribution of Radiative Forcing by Dust Aerosol

To quantitatively understand the dust aerosol effects on climate change,we calculated the global distribution of direct radiative forcing due to dust aerosol under clear and cloudy skies in both winter and summer,by using an improved radiative transfer model and the global distribution of dust mass concentration given by GADS (Global Aerosol Data Set).The results show that the global means of the solar forcing due to dust aerosol at the tropopause for winter and summer are –0.48 and –0.50 W m-2 ,respectivel...     

南半球中高纬度区域不同类型云的辐射特性

利用CloudSat的2B-CLDCLASS-LIDAR云分类产品和2B-FLXHR-LIDAR辐射产品4 a（2007-2010年）的数据,定量分析了单层云（高云、中云、低云）和3种双层云（如:高云与中云共存、高云与低云共存以及中云与低云共存）在南半球中高纬度（40°-65°S）的云量、云辐射强迫和云辐射加热率。其中云辐射加热率定义为有云时的大气加热率廓线与晴空大气加热率廓线的差值。结果表明:研究区域盛行单层低云和单层中云,其云量分别为44.1%和10.3%。并且,中云重叠低云在双层云中云量也是最大（8.7%）。不同类型云的云量也显著影响着其云辐射强迫。单层低云在大气层顶、地表以及大气中的净云辐射强迫分别是-64.8、-56.5和-8.4 W/m2,其绝对值大于其他类型云。虽然单层的中云在大气层顶和地表的净辐射强迫也为负值,但其在大气中的净云辐射强迫为正值（2.3 W/m2）。最后,讨论了不同类型云对大气中辐射能量垂直分布的影响。所有类型云的短波（或长波）云辐射加热率都随高度升高表现为由负值转为正值（或由正值转为负值）。对于大部分云,其净云辐射加热率主要由长波云辐射加热率决定。这些研究结果旨在为模式中云重叠参数化方案在区域的适用性评估及改进提供观测依据。      

影响地面紫外辐射的因素分析

通过作者改进的离散坐标法（DISORT）辐射传输模式和部分观测资料考察了臭氧总量及其垂直分布、二氧化硫、气溶胶及火山气溶胶、地表反照率、太阳天顶角对到达地面紫外辐射的影响,以及云与紫外辐射的相互作用,给出了一些最主要的结果。此外,还简要地介绍了国内外紫外辐射观测研究的一些进展,特别是欧盟委员会资助开展的“确定UV-B辐射观测网标准”的科学计划。     

A Review of Aerosol Optical Properties and Radiative Effects

Atmospheric aerosols influence the earth's radiative balance directly through scattering and absorbing solar radiation, and indirectly through affecting cloud properties. An understanding of aerosol optical properties is fundamental to studies of aerosol effects on climate. Although many such studies have been undertaken, large uncertainties in describing aerosol optical characteristics remain, especially regarding the absorption properties of different aerosols. Aerosol radiative effects are considered as either positive or negative perturbations to the radiation balance, and they include direct, indirect (albedo effect and cloud lifetime effect), and semi-direct effects. The total direct effect of anthropogenic aerosols is negative (cooling), although some components may contribute a positive effect (warming). Both the albedo effect and cloud lifetime effect cool the atmosphere by increasing cloud optical depth and cloud cover, respectively. Absorbing aerosols, such as carbonaceous aerosols and dust, exert a positive forcing at the top of atmosphere and a negative forcing at the surface, and they can directly warm the atmosphere. Internally mixed black carbon aerosols produce a stronger warming effect than externally mixed black carbon particles do. The semi-direct effect of absorbing aerosols could amplify this warming effect. Based on observational (ground-and satellite-based) and simulation studies, this paper reviews current progress in research regarding the optical properties and radiative effects of aerosols and also discusses several important issues to be addressed in future studies.     

海洋-大气耦合辐射传输模式

本文在已有的DISORT大气辐射传输模式基础上，耦合进一个海洋反射模式，在海洋反射模式部分，考虑了风生海表毛细波对海表双向反射的作用以及海洋中叶绿素、悬浮物、溶解有机物对海洋反射光谱的影响，同时，为应用方便，为此模式配套了完整的大气温、压、湿、微量气体、气溶胶及太阳地外谱数据集；此海洋反射模式和海洋-大气耦合辐射传输模式已与1995年9月5日黄海海面反射光谱的实测资料和飞行实验中的光谱仪测量数据进行了对比验证，模拟结果与实测数据基本上符合。