Cloud contribution to the daily and annual radiation budget in a mountainous valley

An automated-ventilated radiation station has been set up in a mountainous valley at the Logan Airport in northern Utah, USA, since mid-1995, to evaluate the daily and annual radiation budget components, and develop an algorithm to study cloudiness and its contribution to the daily and annual radiation. This radiation station (composed of pyranometers, pyrgeometers and a net radiometer) provides continuous measurements of downward and upward shortwave, longwave and net radiation throughout the year. The surface temperature and pressure, the 2-m air temperature and humidity, precipitation, and wind at this station were also measured. A heated rain gauge provided precipitation information. Using air temperature and moisture and measured downward longwave (atmospheric) radiation, appropriate formula (among four approaches) was chosen for computation of cloudless-skies atmospheric emissivity. Considering the additional longwave radiation during the cloudy skies coming from the cloud in the waveband which the gaseous emission lacks (from 8–13 μm), an algorithm was developed which provides continuous 20-min cloud information (cloud base height, cloud base temperature, percent of skies covered by cloud, and cloud contribution to the radiation budget) over the area during day and night. On the partly-cloudy day of 3 February, 2003, for instance, cloud contributed 1.34 MJ m^− 2 d^− 1 out of 26.92 MJ m^− 2 d^− 1 to the daily atmospheric radiation. On the overcast day of 18 December, 2003, this contribution was 5.77 MJ m^− 2 d^− 1 out of 29.38 MJ m^− 2 d^− 1. The same contribution for the year 2003 amounted to 402.85 MJ m^− 2 y^− 1 out of 9976.08 MJ m^− 2 y^− 1. Observations (fog which yielded a zero cloud base height and satellite cloud imaging data) throughout the year confirmed the validity of the computed data. The nearby Bowen ratio station provided the downward radiation and net radiation data. If necessary, these data could be substituted for the missing data at the radiation station. While the automated surface observing systems (ASOS) ceilometer at the Logan airport provides only the overhead cloud information, the proposed algorithm provides this information over the valley. The proposed algorithm is a promising approach for evaluation of the cloud base temperature, cloud base height, percent of skies covered by cloud, and cloud contribution to the daily and annual radiation budget at local and regional scales.     

Contribution of the MODIS instrument to observations of deep convective storms and stratospheric moisture detection in GOES and MSG imagery

Past studies based on the NOAA/AVHRR and GOES I-M imager instruments have documented the link between certain storm top features referred to as the “cold-U/V” shape in the 10–12 μm IR band imagery and plumes of increased 3.7/3.9 μm band reflectivity. Later, similar features in the 3.7/3.9 μm band have been documented in the AVHRR/3 1.6 μm band imagery.The present work focuses on storm top observations utilizing the MODIS data. The MODIS instrument (available onboard NASA's EOS Terra and Aqua satellites) provides image data with significantly better geometrical resolution (in some of its bands) and broader range of spectral bands as compared to that from AVHRR/3 observations. One of the goals of this study is to evaluate the contribution of this new instrument to observations of convective storm tops. Besides the cloud top features linked to storm top microphysics and morphology, the paper also addresses the possibility of detection of lower stratospheric water vapor above cold convective storm tops. This issue is explored utilizing MODIS as well as GOES and MSG imagery.In addition, the paper discusses an alternative interpretation of the “cold-U/V” patterns at the top of intense storms by a mechanism of “plume masking” as suggested by some of the observations.     

Effects of prescribed initial cloud droplet spectra on convective cloud and precipitation developments under different thermodynamic conditions: A modeling and observational study

A two-dimensional cloud model with bin microphysics was used to investigate the effects of cloud condensation nuclei (CCN) concentrations and thermodynamic conditions on convective cloud and precipitation developments. Two different initial cloud droplet spectra were prescribed based on the total CCN concentrations of maritime (300 cm^− 3) and continental (1000 cm^− 3) air masses, and the model was run on eight thermodynamic conditions obtained from observational soundings. Six-hourly sounding data and 1-hourly precipitation data from two nearby weather stations in Korea were analyzed for the year 2002 to provide some observational support for the model results.For one small Convective Available Potential Energy (CAPE) ( 300 J kg^− 1) sounding, the maritime and continental differences were incomparably large. The crucial difference was the production of ice phase hydrometeors in the maritime cloud and only water drops in the continental cloud. Ice phase hydrometeors and intrinsically large cloud drops of the maritime cloud eventually lead to significant precipitation. Meanwhile negligible precipitation developed from the continental cloud. For the three other small CAPE soundings, generally weak convective clouds developed but the maritime and continental clouds were of the same phases (both warm or both cold) and their differences were relatively small.Model runs with the four large CAPE ( 3000 J kg^− 1) soundings demonstrated that the depth between the freezing level (FL) and the lifting condensation level (LCL) was crucial to determine whether a cloud becomes a cold cloud or not, which in turn was found to be a crucial factor to enhance cloud invigoration with the additional supply of freezing latent heat. For two large CAPE soundings, FL–LCL was so deep that penetration of FL was prohibitive, and precipitation was only mild in the maritime clouds and negligible in the continental clouds. Two other soundings of similarly large CAPE had small FL–LCL, and both the maritime and continental clouds became cold clouds. Precipitation was strong for both but much more so in the maritime clouds, while the maximum updraft velocity and the cloud top were slightly higher in continental clouds. Although limited to small CAPE cases, more precipitation for smaller FL–LCL for a selected group of precipitation and thermodynamic sounding data from Korea was in support of these model results in its tendency.These results clearly demonstrated that the CCN effects on cloud and precipitation developments critically depended on the given thermodynamic conditions and not just the CAPE but the entire structure of the thermodynamic profiles had to be taken into account.     

中国东部大陆和邻近海域暖云特性时空分布及其与气象条件的关系

基于2003~2016年MODIS/Aqua（MODerate resolution Imaging Spectroradiometer）云产品资料（MYD08_D3）,分析了中国东部大陆及其邻近海域云量（CF）、云滴有效半径（CER）、和液水路径（LWP）的空间分布以及季节变化,并结合同期ERA-Interim再分析资料的850 hPa垂直速度（ω_850hPa）、低对流层稳定度（LTS）、以及MODIS/Aqua水汽产品中的大气可降水量（PWV）资料,分析了云宏微观物理量与动力、热力及水汽条件之间的关系。从空间分布来看,夏季由日本海至中南半岛存在一个东北西南走向的云量高值区,覆盖我国东部地区,冬季云量高值区位于我国南方地区和东部海域上空;云滴有效半径冬、夏分布类似,均为由东南洋面至西北内陆递减;夏季液水路径分布较为均一,冬季空间差异很大,30°N是明显的高低值分界线,这与冬季水汽的分布密切相关。陆地和海洋上云量均呈冬高夏低的变化趋势,陆地大于海洋,而云滴有效半径和液水路径则为夏高冬低,海洋大于陆地。总体来说,云量与PWV和LTS均表现为正相关、与ω_850hPa呈负相关,表明低层的上升运动有利于水汽向上输送、凝结形成云,但稳定的大气层结又会阻碍云进一步向上发展,使其被限制在底层空间,由于本文的研究对象为暖云,多为中低云,因而云量较高;云滴有效半径和液水路径均与LTS、ω_850hPa表现为负相关,但是对PWV的变化不是很敏感,表明水汽并不是影响云滴尺度和液水路径的主导因素,其主要受动力、热力抬升作用的影响;以上关系在不同区域、不同季节的表现存在一定差异。     

Influence of the total atmospheric optical depth and cloud cover on solar irradiance components

Broadband solar irradiance data obtained in the spectral range 400–940 nm at Kwangju, South Korea from 1999–2000 have been analyzed to investigate the effects of cloud cover and atmospheric optical depth on solar radiation components. Results from measurements indicate that the percentage of direct and diffuse horizontal components of solar irradiance depend largely on total optical depth (TOD) and cloud cover. During summer and spring, the percentages of diffuse solar irradiance relative to the global irradiance were 5.0% and 4.9% as compared to 2.2% and 3.0% during winter and autumn. The diffuse solar irradiance is higher than the direct in spring and summer by 24.2%, and 40.6%, respectively, which may largely be attributed to the attenuation (scattering) of radiation by heavy dust pollution and large cloud amount. In cloud-free conditions with cloud cover ≤2/10, the fraction of the direct and diffuse components were 66.0% and 34.0%, respectively, with a mean daily global irradiance value of 7.92±2.91 MJ m⁻² day⁻¹. However, under cloudy conditions (with cloud cover ≥8/10), the diffuse and direct fractions were 97.9% and 2.2% of the global component, respectively. The annual mean TOD under cloudless conditions (cloud cover≤2/10) yields 0.74±0.33 and increased to as much as 3.15±0.67 under cloudy conditions with cloud amount ≥8/10. An empirical formula is derived for estimating the diffuse and direct components of horizontal solar irradiance by considering the total atmospheric optical depth (TOD). Results from statistical models are shown for the estimation of solar irradiance components as a function of TOD with sufficient accuracy as indicated by low standard error for each solar zenith angle (SZA).     

Cloud condensation nuclei measurements at Mace Head, Ireland, over the period 1994–2002

Analyses of cloud condensation nuclei (CCN) number concentrations (cm^− 3) measured at the Mace Head Atmospheric Research Station, near Carna, County Galway, Ireland, using a DH Associates Model M1 static thermal diffusion cloud chamber over the period from March 1994 to September 2002 are presented in this work. Air masses are defined as being ‘marine’ if they originate from a wind direction of 180–300° and ‘continental’ air masses are defined as originating from a wind direction of 45–135°. Air masses without such filtering were classified as ‘undefined’ air masses. Air masses were found to be dominated by marine sector air, re-affirming Mace Head as a baseline atmospheric research station. CCN levels for specific air masses at Mace Head were found to be comparable with earlier studies both at Mace Head and elsewhere. Monthly averaged clean marine (wind direction of 180–300° and black carbon absorption coefficient < 1.425 Mm^− 1) CCN and marine CCN varied between 15–247 cm^− 3 and 54–670 cm^− 3, respectively. As expected, significant increases in number concentration were found in continentally sourced CCN over that of marine CCN and were found to follow a log-normal distribution significantly tighter than that of clean marine air masses. No significant trend was found for CCN over the 9-year period. While polluted continental air masses showed a slight increase in CCN concentrations over the winter months, most likely due to increased fuel usage and a lower mixed boundary layer, the dominance of marine sector air arriving at Mace Head, which generally consists of background CCN concentrations, reduced seasonal differences for polluted air. Marine air showed a distinct seasonal pattern, with elevated values occurring over the spring and summer seasons. This is thought to be due to enhanced biogenic aerosol production as a result of phytoplankton bloom activity in the North Atlantic.     

Comparison between MODIS-derived Day and Night Cloud Cover and Surface Observations over the North China Plain

Satellite and human visual observation are two of the most important observation approaches for cloud cover. In this study, the total cloud cover(TCC) observed by MODIS onboard the Terra and Aqua satellites was compared with Synop meteorological station observations over the North China Plain and its surrounding regions for 11 years during daytime and7 years during nighttime. The Synop data were recorded eight times a day at 3-h intervals. Linear interpolation was used to interpolate the Synop data to the MODIS overpass time in order to reduce the temporal deviation between the satellite and Synop observations. Results showed that MODIS-derived TCC had good consistency with the Synop observations; the correlation coefficients ranged from 0.56 in winter to 0.73 in summer for Terra MODIS, and from 0.55 in winter to 0.71 in summer for Aqua MODIS. However, they also had certain differences. On average, the MODIS-derived TCC was 15.16%higher than the Synop data, and this value was higher at nighttime(15.58%–16.64%) than daytime(12.74%–14.14%). The deviation between the MODIS and Synop TCC had large seasonal variation, being largest in winter(29.53%–31.07%) and smallest in summer(4.46%–6.07%). Analysis indicated that cloud with low cloud-top height and small cloud optical thickness was more likely to cause observation bias. Besides, an increase in the satellite view zenith angle, aerosol optical depth, or snow cover could lead to positively biased MODIS results, and this affect differed among different cloud types.     

The spatial and temporal variability of fog and its relation to fog oases in the Atacama Desert, Chile

Fog has been studied in the Atacama Desert of Chile for the past ten years. This paper analyzes its temporal and spatial variability, relying in part on satellite images (GOES) to analyze the frequent orographic fog and the low cloud deck (stratocumulus, Sc) that generates advective fog in the area. Fog water fluxes were measured with Standard Fog Collectors (SFC). Field trips and observers provided information on cloud top and base and the presence of fog. Vegetation in fog oases were used to confirm the results of these surveys.The Sc moves onshore into the continent with different intensities depending on season and time of day. The maximum spatial extent occurs during winter and at night. Fog is frequent in the coastal cliffs, where fog water fluxes of 7.0 L m^− 2 day^− 1 were measured using a SFC. It is less frequent 12 km inland, where the collection rates were less than 1 L m^− 2 day^− 1. The height of the fog collector above the ground affected the collection rate. The highest fog water fluxes were recorded at Alto Patache at altitudes of between 750 and 850 m a.s.l. The growth or thickness of the cloud is important in the collection of fog water. The information that GOES provides on the altitude of the top of low clouds is used to analyze this factor. Fog oases are described and analyzed in relation to how the geographical location of fog influences the growth of vegetation.     

General circulation model simulation of mild nuclear winter effects

The climatic effects of an elevated uniform global layer of purely absorbing smoke of absorption optical depth 0.2 have been simulated using a version of the 9-level spectral model of McAvaney et al. (1978). The model was run at rhomboidal wave number 21 with convective adjustment, prognostic precipitation and soil hydrology, but fixed zonally averaged climatological cloud and fixed sea surface temperature, for constant January and July conditions with and without smoke absorption. Results show a reduction in convective rainfall in the tropics and monsoonal regions of the order of 50%, with diurnal average soil surface coolings of several degrees C except in those locations where the reduction in soil moisture is sufficient to effectively stop evaporation at the surface. In that case, small increases in temperature may occur. Results over Australia are consistent with the zonal mean picture. Run in a diurnal cycle mode, the model shows that daily maximum temperatures are more strongly affected, with soil surface coolings of the order of 2°–3° C in summer (with some local warmings) and 4°–6° C in winter. Overninght minimum temperatures cool by only 1°–2° C in both summer and winter. Possible effects of a lowering of sea surface temperature, variations in cloud cover, neglect of scattering by smoke, and infrared absorption and emission by the smoke are discussed.     

基于2014～～2017年Ka毫米波雷达数据分析北京地区云宏观分布特征

本文利用2014年1月至2017年12月Ka毫米波雷达数据对北京地区云宏观特征进行统计分析。云出现率方面，4年平均值约36.3%；冬季最低，夏季最大；月出现率值9月最大，12月最小；出现率日变化有季节差异，春夏两季呈现中午（11:00，北京时间，下同）开始逐步升高至下午17:00后逐步下降的特点，增高幅度大于15%；冬、秋两季日变化特征不显著。高度方面，4年平均云底高约4.9 km，平均云顶高约7.2 km；云顶高和云底高的月变化特征明显，从年初1月开始逐步上升，在6月达到峰值，而后下降到12月达到低值；3～10月，高云（云底高>5 km)占约一半左右比例；厚度小于1 km的云在各月中所占比例最高；厚度1～4 km的云，厚度越大所占比例越低；特别地，厚度大于4 km的云所占比例在4～9月中仅次于厚度小于1 km云的比例。4年期间，北京地区单层云居多约占66.7%，两层云占比约25.2%，两层以上云占8.1%；冬季约80%的云为单层云，而6～9月云层分布变化最多，其中9月单层云比例最低约为40%。本文基于4年高时空分辨率雷达数据对北京地区云分布特征，特别是云垂直分布特征在数值上准确刻画，该项工作在已有云气候研究中尚未见开展，所获得的知识将对了解地区气候特征、区域模式云参数化选择提供参考。     

中国地区三种地表反照率产品比较北大核心

利用2007—2011年MODIS、GlobAlbedo和ERA-Interim的3种地表反照率产品,借助地理信息系统(Geographic Information System,GIS)空间化技术,对中国地区3种地表反照率产品进行了对比分析。结果表明:3种产品与气象站观测值的时间分布趋势一致,冬季高夏季低,且相关性较高。3种产品中,MODIS与GlobAlbedo的绝对差异值最小,ERA-Interim与MODIS、GlobAlbedo的绝对差异值较大。3种产品在青藏高原和西北山地区域表现出较大的差异,且差异表现为冬半年高,夏半年低。3种产品之间相关性最高的是MODIS与GlobAlbedo,最低的是MODIS与ERA-Interim,3种产品在40°N以北具有较好的相关性。且在夏季和冬季地表反照率均值的表现说明,ERA-Interim相比MODIS、GlobAlbedo难以反映地表反照率受地形和土地覆被的影响。     

北京地区地基辐射计与卫星云特性参数对比研究

利用2019年MODIS卫星数据、葵花-8卫星数据和天空辐射计观测数据分析北京城区云光学特性的时空分布特征。结果表明,北京地区的云光学厚度(Cloud optical depth,COD)和云滴有效半径(Cloud drop effective radius,CER)呈现明显的季节变化特征。北京地区COD主要分布特征为南部地区较高而北部地区较低,且夏季COD值明显高于其他季节,最高值为20左右。CER在春季和夏季呈现相反的区域分布特征,春季北京地区南低北高,夏季北京地区南高北低,而秋冬季CER明显低于春夏两季。通过将天空辐射计观测数据与卫星观测结果对比分析发现二者在COD方面一致性较高, r分别为0.69和0.66,MODIS对于CER数据的一致性较差,r值为0.053而葵花-8一致性较好r值为0.53。     

An airborne two-stage impactor for chemical analysis of size-segregated cloud drops

Aqueous concentrations of ionic species observed in cloud water studies often have been in conflict with expectations from model predictions. These inconsistencies result from the size-dependent chemical composition of cloud drops during different stages in the lifetime of a cloud. To study this phenomenon, droplets of clouds need to be collected in different size ranges with high resolution in space and time. The only possibility for this kind of study is the use of an aircraft. Therefore, during the last several years, an attempt was made to develop a mobile cascade impactor, which can be installed outside an aircraft. The cloud water sampled in different size fractions can be transferred into the interior of the aircraft during the measuring flight. The collector is able to sample two size fractions. For continental clouds, the cutoffs are chosen to be >5 and >13.5 μm in diameter. For maritime clouds, the cutoff for the first stage could be shifted to 18.6 μm by lowering the nozzle speed. Prior to field application, the collector was characterized with the aid of “calibration fogs” produced in the laboratory with different drop sizes and different chemical compositions. The characterization included the examination of the cutoffs and the reliability of the sampling procedure with regard to the subsequent chemical analysis. With a collection period of 2 min, collection rates in the order of 0.1–1 cm³ min⁻¹ can be obtained. The collector characterized in this manner was successfully used during measuring flights in clouds over northern Germany. Preliminary concentrations of NH₄⁺, SO₄²⁻ and Cl⁻ found in the two size fractions of the cloud drops are presented.     

Seasonal variations of spectra of wind speed and air temperature in the mesoscale frequency range

Seasonal variations of the spectra of wind speed and air temperature in the mesoscale frequency range from 1.3 × 10^-4 to 1.5 × 10^-3 Hz (10 min to 2 h periods) have been studied through observations over land for one year. Spectrographs [time series of isopleths of spectral densities, f · S(f) vs f] of wind speed and air temperature contain occasional peaks that are attributed to short-lived mesoscale atmospheric activity with narrow frequency bands. Significant spectral peaks of wind speed were found in 19% of the total observations in winter, and in 15–16% in the other seasons; for air temperature, they occured in 12% of observations in autumn, and in 16–19% in the other seasons. The peaks most often occurred in the period range from 30 min to 1 h; most had durations less than 24 h. Mesoscale fluctuations of wind speed and air temperature were highly correlated, and in most cases, phase differences were 90–180 ° with air temperature leading wind speed. Significant spectral peaks of wind speed often occurred during northerly seasonal cold winds in winter, and accompanied tropical and/or mid-latitude cyclones in the other seasons. When the peaks occurred, wind speed was usually relatively high and the atmospheric surface layer was unstable.     

复杂地形区陆面资料对WRF模式模拟性能的影响

本文利用WRF（Weather Research and Forecasting）模式耦合Noah陆面过程模式,对比研究了使用不同精度陆面资料:WRF默认陆面资料、中国1 km分辨率数字高程模型数据集、2006年MODIS（MODerate-resolution Imaging Spectroradiometer）土地利用和植被覆盖度资料,WRF模式对兰州地区冬季气象场模拟结果的差异。结果表明,近地面气温对陆面资料的精度非常敏感,而风场对陆面资料的精度不敏感,WRF模式对气温的模拟效果好于对风场模拟。采用高精度且时效性好的陆面资料后,WRF模拟的近地面气温准确率提高了15.8%,模拟的夜间气温改进幅度较白天大。陆面资料可影响整个边界层温度场分布,准确的陆面资料对提高WRF模式模拟近地面乃至整个边界层气象场至关重要。尽管风速模拟误差较大,但总体上WRF模式能较准确地模拟出研究区的风场演变特征。使用新的陆面资料后WRF模拟的风速误差略有减小,风向误差略有增加。干旱半干旱区冬季数值模拟需要注意土壤湿度初值和模式初始积分时刻对模拟结果的影响。     

Black carbon relationships with emissions and meteorology in Xi'an, China

Aerosol black carbon (BC) was measured every 5 min at Xi'an, China from September 2003 to August 2005. Daily BC concentrations ranged from 2 to 65 μg m^− 3, averaging 14.7 ± 9.5 μg m^− 3 and displayed clear summer minima and winter maxima. BC typically peaked between 0800 and 1000 LST and again between 2000 and 2200 LST, corresponding with morning and evening traffic combined with nighttime residential cooking and heating. The nocturnal peak was especially evident in winter, when more domestic heating is used and pollutant-trapping surface-inversions form earlier than in summer. BC frequency distributions the most commonly occurring concentrations occurred between 5 and 10 μg m^− 3 in all four seasons. BC ranged from 1.6% and 15.6%, and averaged 8.3% of PM_2.5. A clear inverse relationship between BC and wind speed (WS) was found when WS was below 2.5 to 3.0 m s^− 1, implying a local origin for BC. Mixed layer depths (MLDs) were shallower during BC episodes compared to cleaner conditions.     

Optical observations of transient luminous events associated with winter thunderstorms near the coast of Israel

We report the results of two observation campaigns conducted during the Northern Hemisphere winters of 2005–6 and 2006–7 aiming to detect transient luminous events (TLEs) above winter thunderstorms in the vicinity of Israel and the eastern coastline of the Mediterranean Sea. In 10 out of 31 different observation nights we detected 66 events: 56 sprites and 10 Elves. The detection ranges varied from 250 to 450 km. Sprites were found to be produced by active cells with a vertical dimension of 5–9 km and cloud top temperature ~ − 40 °C, embedded in a much larger matrix of stratiform precipitating cloudiness. This configuration closely resembles the conditions for winter sprites in the Hokuriku region of Japan. Synchronized with the optical observations, ELF data were recorded at two observation stations in Israel and Hungary in order to qualify and quantify parameters of the parent lightning discharge associated with the TLEs. These stations are located 500 km and 2100 km respectively from the Eastern Mediterranean Sea, where most TLEs occur. Among the optically observed TLE events, we found that all the ELF signals were produced solely by positive cloud-to-ground flashes (+ CGs), most of which were recorded in Israel (88%) and Hungary (77%). Calculation of the Charge Moment Change showed average values of 1400 ± 600 C km, with some extreme events exceeding 3500 C km. The average time delay between the ELF transient of the parent + CG and the observed sprites was 55 ms, with shorter delays for column sprites (42 ± 34 ms) compared to carrot sprites (68 ± 34). Furthermore, based on the ELF data, there were no early identifiable precursors to TLE occurrence in the regional lightning activity. From the spatial formation of the observed columniform sprites, we propose that columniform sprites are sometimes arranged in a 3-dimensional circular pattern, thus mapping the instantaneous electric field in the mesosphere.     

The Great Dun Fell Experiment 1995: an overview

During March and April of 1995 a major international field project was conducted at the UMIST field station site on Great Dun Fell in Cumbria, Northern England. The hill cap cloud which frequently envelopes this site was used as a natural flow through reactor to examine the sensitivity of the cloud microphysics to the aerosol entering the cloud and also to investigate the effects of the cloud in changing the aerosol size distribution, chemical composition and associated optical properties. To investigate these processes, detailed measurements of the cloud water chemistry (including the chemistry of sulphur compounds, organic and inorganic oxidised nitrogen and ammonia), cloud microphysics and properties of the aerosol and trace gas concentrations upwind and downwind of the cap cloud were undertaken. It was found that the cloud droplet number was generally strongly correlated to aerosol number concentration, with up to 2000 activated droplets cm⁻³ being observed in the most polluted conditions. In such conditions it was inferred that hygroscopic organic compounds were important in the activation process. Often, the size distribution of the aerosol was substantially modified by the cloud processing, largely due to the aqueous phase oxidation of S(IV) to sulphate by hydrogen peroxide, but also through the uptake and fixing of gas phase nitric acid as nitrate, increasing the calculated optical scattering of the aerosol substantially (by up to 24%). New particle formation was also observed in the ultrafine aerosol mode (at about 5 nm) downwind of the cap cloud, particularly in conditions of low total aerosol surface area and in the presence of ammonia and HCl gases. This was seen to occur at night as well as during the day via a mechanism which is not yet understood. The implications of these results for parameterising aerosol growth in Global Climate Models are explored.     

基于多源卫星资料的中国地区云宏微观特征研究

利用2007—2016年国际卫星云气候计划（International Satellite Cloud Climatology Project,ISCCP）、云和地球辐射能量系统（Clouds and the Earth''s Radiant Energy System,CERES）和中分辨率成像光谱仪（Moderate Resolution Imaging Spectroradiometer,MODIS）卫星反演云产品,对比分析了不同数据反演的中国地区云系结构的宏微观特征,并采用复合评价指标定量评估了不同数据之间时间和空间上的一致性。结果表明：三套卫星数据都能较好地反演出中国地区总云量呈南高北低、东高西低、夏高冬低的分布特征,但通过比较时间技巧（Temporal Skill,S_T）及空间技巧（Spatial Skill,S_S）复合评价指标及其各项分量发现,与MODIS相比,CERES与ISCCP数据反演的总云量时间序列演变特征明显更为一致,且其评分均有南方优于北方,夏季优于冬季的特征;进一步分析不同高度云量的S_T评分发现,CERES和ISCCP两套数据在南方地区的总云量差异主要来自于低云量的绝对偏差,而北方地区的偏差则同时存在于低云和中云;对比分析MODIS和CERES反演的云滴有效半径发现,高云对应的冰相云一致性较高,而中低云相对应的液相云的偏差则有夏季高于冬季的规律。针对夏季液相和冰相云滴粒径及概率密度分析则表明,相比CERES数据,MODIS对夏季液水和冰水粒子的有效半径在不同地区均有不同程度的高估,液（冰）水谱宽则更宽（窄）。     

东亚地区云垂直结构的CloudSat卫星观测研究

本文利用卫星CloudSat同时结合了与其同轨道的卫星CALIPSO(Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations)2007至2009年3年的观测资料,将东亚地区划分为六个研究区域,着重研究了东亚地区云垂直分布的统计特征.结果表明:东亚地区不同高度的云量之和具有明显的季节变化趋势,夏季最大,春秋次之,冬季最小.海洋上空的单层云量最大值出现在冬季,而在陆地上空则出现在夏季.从云出现概率来看,东亚地区单层云出现的概率在春、夏、秋、冬季节依次为52.2%,48.1%,49.2%和51.9%,而多层(2层和2层以上)云出现的概率在春、夏、秋、冬季节分别为24.2%,31.0%,19.7%,15.8%.云出现的总概率和多层云出现的概率,在六个区域都呈现出夏季最大,冬季最小;对4个季节都呈现出东亚南部比东亚北部大,海洋上空比陆地上空大的特点,表明云出现的总概率的季节变化主要由多层云出现的概率的变化决定.东亚地区云系统中最高层云云顶的高度,在夏季最高,为15.9 km,在冬季最低,为8.2 km;在东亚南部和海洋上空较高,平均为15.1 km;在东亚北部较低,平均为12.1 km,且呈现东亚南北部之间差异较大的特点.东亚地区云系统的云层厚度基本位于1 km到3 km之间,且夏季大,冬季小;对同一季节,不同区域的云层厚度差别较小;当多层云系统中的云层数目增加时,云层的平均厚度减少,且较高层的云层平均厚度大于较低层的.云层间距的概率分布基本呈单峰分布,出现峰值范围的云层间距在1到3 km之间,各区域之间没有明显差别,季节变化也不大.本文的研究为在气候模式中精确描述云的垂直结构提供了有用的参数化依据.