温室气体和硫酸盐气溶胶的辐射强迫作用

对GOALS4 .0海 陆 气耦合模式的相关部分进行了改进 ,主要改进包括温室气体的扩充和硫酸盐气溶胶“显式”方案的引入 ,并引入 2 0世纪温室气体的实际浓度变化以及硫循环模式模拟的硫酸盐气溶胶的三维全球浓度分布 ,模拟了温室气体和硫酸盐气溶胶造成的辐射强迫的空间分布和时间变化。全球平均的温室气体和硫酸盐气溶胶的辐射强迫分别为 2 .17W /m2 和 - 0 .2 9W /m2 ;温室气体造成的辐射强迫在空间上呈现明显的纬向结构 ,最大值 (大于 2 .5W/m2 )和最小值 (小于 1W /m2 )分别位于副热带和两极地区 ,在北半球主要工业区硫酸盐气溶胶的辐射强迫绝对值接近温室气体的辐射强迫值 (大于 - 2 .0W /m2 )。     

Global warming potentials modified for surface radiative forcing for use in surface energy balance models

The radiative impact of greenhouse gases in warming the Earth varies significantly, depending on whether one considers the forcing at the tropopause or at the surface. Compared to the former, the surface forcing for some greenhouse gases is reduced by the interference of water vapour. Hence, we calculate alternative surface global warming potentials (SGWPs) that are derived from the surface forcing radiation of greenhouse gases for potential use in surface radiative energy balance models (SREBMs). For gases with a large water vapour overlap, the SGWPs are typically 30% smaller than current GWPs; for gases with relatively little overlap, the SGWPs are larger by more than 33%. These results may be used in conjunction with SREBMs as an additional means of calculating climate change, and may lead to an altered emissions budget compared to that outlined by the current Kyoto agreement.     

Modeling Study of the Effect of Anthropogenic Aerosols on Late Spring Drought in South China

In this study,the mechanisms underlying the decadal variability of late spring precipitation in South China are investigated by using the latest Community Earth System Model version 1 （CESM1）.We aim to unravel the effects of different climate forcing agents such as aerosols and greenhouse gases （GHGs） on the decadal variation of precipitation,based on transient experiments from pre-industry （for year 1850） to present-day （for year 2000）.Our results reveal that：（1） CESM1 can reproduce the climatological features of atmospheric circulation and precipitation for the late spring in South China; （2） only simulations including the forcing of anthropogenic aerosols can reproduce the observed decreasing trend of late spring precipitation from 1950-2000 in South China; （3） aerosols affect the decadal change of precipitation mainly by altering the large-scale atmospheric circulation,and to a less extent by increasing the lower-tropospheric stability to inhibit the convective precipitation; and （4） in comparison,other climate forcing agents such as GHGs have much smaller effects on the decadal change of spring precipitation in South China.     

A Model for Estimating Future Emissions of Sulfur Hexafluoride and Perfluorocarbons

Sulfur hexafluoride (SF₆), perfluoromethane (CF₄) and perfluoroethane (C₂F₆) are strong greenhouse gases with long (>1000 year) atmospheric residence times. We derive emission factors for the major anthropogenic sources and project future emissions for 5 regions and the world. Although firms in many industrialized countries are already limiting emissions, without further policy intervention global emissions will rise 150% (CF₄ and C₂F₆) and 210% (SF₆) between 1990 and 2050; radiative forcing will increase 0.026 W m^-2. Full application of available low-cost and costless policies in industrialized nations would cut that radiative forcing by one-quarter. Increased forcing due to these gases is small (<2%) relative to other gases but permanent on the timescale of human civilization. We also quantify plausible manipulations to governmental data that will be used to determine compliance with the 1997 Kyoto Protocol, which includes commitments for industrialized countries to regulate these and other greenhouse gases. More complete and transparent data are urgently needed. West European nations, for example, can cut their emissions of these gases by half by 2010 simply by manipulating emission factors within the current bounds of uncertainty.     

Climatic changes associated with a global “2°C-stabilization” scenario simulated by the ECHAM5/MPI-OM coupled climate model

In this study, concentrations of the well-mixed greenhouse gases as well as the anthropogenic sulphate aerosol load and stratospheric ozone concentrations are prescribed to the ECHAM5/MPI-OM coupled climate model so that the simulated global warming does not exceed 2°C relative to pre-industrial times. The climatic changes associated with this so-called “2°C-stabilization” scenario are assessed in further detail, considering a variety of meteorological and oceanic variables. The climatic changes associated with such a relatively weak climate forcing supplement the recently published fourth assessment report by the IPCC in that such a stabilization scenario can only be achieved by mitigation initiatives. Also, the impact of the anthropogenic sulphate aerosol load and stratospheric ozone concentrations on the simulated climatic changes is investigated. For this particular climate model, the 2°C-stabilization scenario is characterized by the following atmospheric concentrations of the well-mixed greenhouse gases: 418 ppm (CO₂), 2,026 ppb (CH₄), and 331 ppb (N₂O), 786 ppt (CFC-11) and 486 ppt (CFC-12), respectively. These greenhouse gas concentrations correspond to those for 2020 according to the SRES A1B scenario. At the same time, the anthropogenic sulphate aerosol load and stratospheric ozone concentrations are changed to the level in 2100 (again, according to the SRES A1B scenario), with a global anthropogenic sulphur dioxide emission of 28 TgS/year leading to a global anthropogenic sulphate aerosol load of 0.23 TgS. The future changes in climate associated with the 2°C-stabilization scenario show many of the typical features of other climate change scenarios, including those associated with stronger climatic forcings. That are a pronounced warming, particularly at high latitudes accompanied by a marked reduction of the sea-ice cover, a substantial increase in precipitation in the tropics as well as at mid- and high latitudes in both hemispheres but a marked reduction in the subtropics, a significant strengthening of the meridional temperature gradient between the tropical upper troposphere and the lower stratosphere in the extratropics accompanied by a pronounced intensification of the westerly winds in the lower stratosphere, and a strengthening of the westerly winds in the Southern Hemisphere extratropics throughout the troposphere. The magnitudes of these changes, however, are somewhat weaker than for the scenarios associated with stronger global warming due to stronger climatic forcings, such as the SRES A1B scenario. Some of the climatic changes associated with the 2°C-stabilization are relatively strong with respect to the magnitude of the simulated global warming, i.e., the pronounced warming and sea-ice reduction in the Arctic region, the strengthening of the meridional temperature gradient at the northern high latitudes and the general increase in precipitation. Other climatic changes, i.e., the El Niño like warming pattern in the tropical Pacific Ocean and the corresponding changes in the distribution of precipitation in the tropics and in the Southern Oscillation, are not as markedly pronounced as for the scenarios with a stronger global warming. A higher anthropogenic sulphate aerosol load (for 2030 as compared to the level in 2100 according to the SRES A1B scenario) generally weakens the future changes in climate, particularly for precipitation. The most pronounced effects occur in the Northern Hemisphere and in the tropics, where also the main sources of anthropogenic sulphate aerosols are located.     

Stratospheric Temperature Changes and Ozone Recovery in the 21st Century

Increasing greenhouse gases and likely ozone recovery will be the two most important factors influencing changes in stratospheric temperatures in the 21st century. The radiative effect of increasing greenhouse gases will cause cooling in the stratosphere, while ozone recovery will lead to stratospheric warming. To investigate how stratospheric temperatures change under the two opposite forcings in the 21st century, we use observed ozone and reanalysis data as well as simulation results from four coupled oceanic and atmo- spheric general circulation models （GISS-ER, GFDL-CM20, NCAR-CCSM3, and UKMO-HadCM3） used in the IPCC （Intergovernment Panel for Climate Change） Fourth Assessment Report （AR4）. Observational analysis shows that total column ozone and lower stratospheric temperatures all show increasing in the past 10 years, while middle stratospheric temperatures demonstrate cooling. IPCC AR4 simulations show that greenhouse forcing alone will lead to stratospheric cooling. However, with forcing of both increasing greenhouse gases and ozone recovery, the middle stratosphere will be cooled, while the lower stratosphere will be warmed. Warming magnitudes vary from one model to another. UKMO-HadCM3 generates relatively strong warming for all three greenhouse scenarios, and warming extends to 40 hPa. GFDL-CM20 and NCAR-CCSM3 produce weak warming, and warming mainly exists at lower levels, below about 60 hPa. In addition, we also discuss the effect of temperature changes on ozone recovery.     

Transient climatic response to an increase of greenhouse gases

The physical factors governing the transient climatic response to an increase of greenhouse gases are discussed, reasons for remaining uncertainties are identified, and recent climate modelling results are briefly summarized. The relevance of the transient response, and of uncertainties in the transient response, to questions such as the applicability of equilibrium climate model simulations to a gradual greenhouse gas increase, the verification of model projections, rates of climatic change, and the impacts of preventative strategies for dealing with the buildup of greenhouse gases is also discussed.     

Climatic variability within an equilibrium greenhouse simulation

A simulation of the possible consequences of a doubling of the CO₂ content of the atmosphere has been performed with a low resolution global climatic model. The model included the diurnal and seasonal cycles, computed sea ice amount and cloud cover, and used implied oceanic heat fluxes to represent transport processes in the oceans. A highly responsive 2-layer soil moisture formulation was also incorporated. Twenty year equilibrated simulations for control (1 × CO₂) and greenhouse (2 × CO₂) conditions were generated. The major emphasis of the analysis presented here is on the intra-annual and interannual variability of the greenhouse run with respect to the control run. This revealed considerable differences from the time-averaged results with occasions of marked positive and negative temperature deviations. Of particular interest were the periods of negative temperature departures compared to the control run which were identified, especially over the Northern Hemisphere continents. Temporal and spatial precipitation and soil moisture anomalies also occurred, some of which were related to the surface temperature changes. Substantial sea surface temperature anomalies were apparent in the greenhouse run, indicating that a source of climatic forcing existed in addition to that due to doubling of the CO₂. Comparison of the intra-annual and interannual variability of the control run with that of the greenhouse run suggests that, in many situations, it will be difficult to identify a greenhouse signal against the intrinsic natural variability of the climatic system.     

Radiation indices of climate-forming factors and their estimates under anthropogenic climate changes

Predictions of expected climate changes are mainly based on the use of large climate models. In the results of these models, it is difficult sometimes to single out the effects and role of separate climate-forming factors. The estimates of such effects are needed for the activities on the mitigation of negative consequences of climate changes on various temporal and spatial scales. Therefore, the methods of computation and comparison of climate-forming factor indices such as the radiative forcing, global warming potential, climate forcing efficiency, et al. are of special importance. Presented is a brief review of indices of principal anthropogenic factors influencing the atmospheric radiation regime on global and local scales such as greenhouse gases, atmospheric aerosols, and radiative properties of the Earth??s surface. The rates of changes in these indices are assessed, as well as their contribution to the variations of climatic characteristics. The examples of these rates are given.     

硫酸盐和烟尘气溶胶辐射特性及辐射强迫的模拟估算

利用已有的硫酸盐和烟尘气溶胶折射指数资料，精确计算了这两种气溶胶从太阳短波到红外谱段的辐射特性。然后，在LLNL化学输送模式(CTM)模拟的硫酸盐和烟尘气溶胶资料及改进的气溶胶参数化基础上，在国内首次用GCM估算了这两种气溶胶引起的全球辐射强迫。结果表明:(1)西欧是全球最大的硫酸盐辐射强迫中心，最大值出现在夏季，达-5.0W/m2；(2)烟尘强迫的最大中心出现在夏季的南美和非洲中南部，为4.0W/m2；(3)南半球大陆人为气溶胶的强迫不容忽视；(4)某些地区人为气溶胶的强迫在量值上可与CO2等温室气体引起的强迫相比拟。     

An investigation into the mechanisms of changes in mid-latitude mean sea level pressure as greenhouse gases are increased

When greenhouse gases are increased in coupled GCM experiments there is both a direct effect and an indirect effect due to changes in the surface conditions. In this study we carry out experiments with a perpetual winter atmosphere only model in order to investigate the influence of changes to the surface conditions (sea surface temperatures, sea-ice and snow amount) on the Northern Hemisphere winter mid-latitude mean sea level pressure response. The surface conditions for the perpetual winter model experiments are prescribed from time averages of the HadCM2 control and greenhouse gas experiments. Forcing the perpetual winter model with the HadCM2 greenhouse gas surface conditions produces a negative mean sea level pressure (MSLP) response across both Northern Hemisphere ocean basins, as was found in the coupled model HadCM2 experiment. Additional PW model experiments show that the sea surface temperature forcing from the HadCM2 greenhouse gas experiment dominates the snow and soil moisture content forcings. The sea-ice forcing from the HadCM2 greenhouse gas experiment reduces MSLP at high latitudes. In the north Pacific region MSLP decreases when the global mean warming is applied to the sea surface temperature forcing field at all open sea points. In the north Atlantic region the increased tropics to mid-latitude meridional sea surface temperature gradient is required for MSLP to decrease. These experiments show that the MSLP response in the Northern Hemisphere mid-latitude storm track regions is sensitive to the non-local sea surface temperature anomaly pattern.     

BCC_CSM1．1全球模式中极端气温变化的归因分析

利用1°×1°的ERA-Interim再分析资料和气候系统模式BCC_CSM1．1历史模拟（Historical）试验及气候归因试验（只考虑温室气体变化Historica1GHG试验和只考虑自然强迫变化的Historica1Nat试验）的结果,考查了BCC_CSM1．1模式对中国和全球陆地地区极端气温指数的模拟能力,并在此基础上分析了温室气体和自然强迫这两种外强迫的变化对极端气温变化的贡献。结果表明：BCC_CSM1．1可以对中国乃至全球陆地区域极端气温指数的气候态及其变化趋势进行合理模拟,主要偏差表现为模式对极端低温指数模拟值偏低,而对极端高温指数模拟值偏高。对于20世纪末极端气温指数的变化,只有考虑了温室气体变化的外强迫时,模式可以再现再分析资料中极端气温的变化趋势。这表明温室气体的变化对极端气温的变化有着关键性的影响。     

Impact of the Montreal protocol and its amendments on the rate of change of global radiative forcing

Increases in chlorinated and brominated halocarbons are believed to be responsible for the depletion of stratospheric ozone observed over much of the globe in the past decade or so. Ozone depletion is in turn believed to lead to a negative radiative forcing, tending to cool the stratosphere and the surface. We show that the increasing atmospheric concentrations of ozone-depleting halocarbons and onset of related ozone depletion likely led to a negative forcing of the climate system in the 1980s that slowed significantly the rate of change of total anthropogenic radiative forcing due to the combined effect of all greenhouse gases over that decade. Within the next decade, emissions of these halocarbons are expected to rapidly decrease, with corresponding impacts on ozone and radiative forcing. As the emissions of ozone-depleting gases are reduced and eventually phased out, the rate of ozone depletion is expected to decrease and eventually reverse. All other things being equal, we show that the change from deepening ozone depletion in the 1980s to ozone increases in the future should lead to a pronounced increase in the decadal rate of change of anthropogenic greenhouse forcing of the next few decades, perhaps to levels unprecedented in this century.     

Direct Radiative Forcing of Anthropogenic Aerosols over Oceans from Satellite Observations

Anthropogenic aerosols play an important role in the atmospheric energy balance. Anthropogenic aerosol optical depth (AOD) and its accompanying shortwave radiative forcing (RF) are usually simulated by nu- merical models. Recently, with the development of space-borne instruments and sophisticated retrieval algorithms, it has become possible to estimate aerosol radiative forcing based on satellite observations. In this study, we have estimated shortwave direct radiative forcing due to anthropogenic aerosols over oceans in all-sky conditions by combining clouds and the Single Scanner Footprint data of the Clouds and Earth’s Radiant Energy System (CERES/SSF) experiment, which provide measurements of upward shortwave fluxes at the top of atmosphere, with Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol and cloud products. We found that globally averaged aerosol radiative forcing over oceans in the clear-sky conditions and all-sky conditions were -1.03±0.48 W m-2 and -0.34 ±0.16 W m-2, respectively. Direct radiative forcing by anthropogenic aerosols shows large regional and seasonal variations. In some regions and in particular seasons, the magnitude of direct forcing by anthropogenic aerosols can be comparable to the forcing of greenhouse gases. However, it shows that aerosols caused the cooling effect, rather than warming effect from global scale, which is different from greenhouse gases.     

CMIP6情景中主要温室气体和气溶胶排放强度的时空分布特征分析

基于不同共享社会经济路径（Shared Socioeconomic Pathways, SSPs）形成的8组最新的未来可能情景（SSPx-y情景）,被用于第六次耦合模式比较计划（CMIP6）,以据此来预估未来气候变化的可能幅度和趋势。本文主要对比分析了8组SSPx-y新情景中主要温室气体和气溶胶排放数据的基准年排放强度分布、未来排放强度的时空变化、以及在6个典型区域排放强度的逐年变化等特征。结果表明:二氧化碳（CO₂）、甲烷（CH₄）、黑碳（BC）、二氧化硫（SO₂）在基准年的排放强度高值区都位于东亚和南亚。相比于基准年,2100年CO₂和CH₄在高和低辐射强迫情景下表现出的排放强度变化有显著差异。此外,所有情景下2100年的BC和SO₂全球平均排放强度都弱于基准年的排放强度。在时间变化上,随着生物质能碳捕获与封存技术的不断进步,所有地区在4组不超过3.4 W/m2的低辐射强迫情景下,CO₂排放强度到2100年都呈现负值。其中,南美洲的负排放最强,2100年在SSP5-3.4情景下该地区的排放强度为－0.3 kg m－2 a－1。最后,对比东亚和南亚排放强度的逐年变化可以发现,在各情景所描述的未来发展过程中,东亚的减排行动的成效都要好于南亚。     

过去0.8 Ma期间的地表温度数值模拟研究

使用一个改进的二维能量平衡模式模拟了过去0.8 Ma冰期-间冰期旋回期间北半球各纬度带的地表温度,并以65°N的地表温度为代表与南极冰芯记录进行了比较.通过敏感性试验,分析了日射量、温室气体、沙尘气溶胶强迫和水汽反馈的辐射-气候效应.结果显示,日射量变化不足以解释冰期-间冰期旋回期间北半球的地表温度变化,大气温室气体(...     

Anthropogenic and natural causes of climate change

We test for causality between radiative forcing and temperature using multivariate time series models and Granger causality tests that are robust to the non-stationary (trending) nature of global climate data. We find that both natural and anthropogenic forcings cause temperature change and also that temperature causes greenhouse gas concentration changes. Although the effects of greenhouse gases and volcanic forcing are robust across model specifications, we cannot detect any effect of black carbon on temperature, the effect of changes in solar irradiance is weak, and the effect of anthropogenic sulfate aerosols may be only around half that usually attributed to them.     

A DIAGNOSTIC STUDY OF FEEDBACK MECHANISM IN GREENHOUSE EFFECTS SIMULATED BY NCAR CCM1

This paper describes a diagnostic study of the feedback mechanism in greenhouse effects of increased CO_2 and oth-er trace gases(CH_4,N_2O and CFCs),simulated by general circulation model.The study is based on two sensitivity exper-iments for doubled CO_2 and the inclusion of other trace gases,respectively,using version one of the community climatemodel(CCM1)developed at the National Centre for Atmospheric Research.A one-dimensional(1-D)and atwo-dimensional(2-D)radiative-convective models are used to diagnose the feedback effect.It shows that thefeedback factors in global and annual mean conditions are in the sequence of surface albedo,water vapor amount,watervapor distribution,cloud height,critical lapse rate and cloud cover,while in zonal and annual mean conditions in thetropical region the above sequence does not change except the two water vapor terms being the largest feedback compo-nents.Among the feedback components,the total water vapor feedback is the largest(about 50%).The diagnosis alsogives a very small feedback of either the cloud cover or the lapse rate,which is substantially different from the 1-Dfeedback analysis by Hansen et al.(1984).The small lapse rate feedback is considered to be partly caused by theconvective adjustment scheme adopted by CCM1 model.The feedback effect for doubled CO_2 is very different from that of the addition of other trace gases because of theirdifferent vertical distributions of radiative forcing although the non-feedback responses of surface air temperature forboth cases are almost the same.For instance,the larger forcing at surface by the addition of other trace gases can causestronger surface albedo feedback than by doubled CO_2.Besides,because of the negative forcing of doubled CO_2 in thestratosphere,cloud height feedback is more intense.The larger surface forcing in the case of other trace gases can also in-fluence atmospheric water vapor amount as well as the water vapor distribution,which will in turn have strongerfeedback effects.All these indicate that it is incorrect to use“effective CO_2”to replace other trace gases in the generalcirculation model.     

RCP4.5: a pathway for stabilization of radiative forcing by 2100

Representative Concentration Pathway (RCP) 4.5 is a scenario that stabilizes radiative forcing at 4.5?W?m^?2 in the year 2100 without ever exceeding that value. Simulated with the Global Change Assessment Model (GCAM), RCP4.5 includes long-term, global emissions of greenhouse gases, short-lived species, and land-use-land-cover in a global economic framework. RCP4.5 was updated from earlier GCAM scenarios to incorporate historical emissions and land cover information common to the RCP process and follows a cost-minimizing pathway to reach the target radiative forcing. The imperative to limit emissions in order to reach this target drives changes in the energy system, including shifts to electricity, to lower emissions energy technologies and to the deployment of carbon capture and geologic storage technology. In addition, the RCP4.5 emissions price also applies to land use emissions; as a result, forest lands expand from their present day extent. The simulated future emissions and land use were downscaled from the regional simulation to a grid to facilitate transfer to climate models. While there are many alternative pathways to achieve a radiative forcing level of 4.5?W?m^?2, the application of the RCP4.5 provides a common platform for climate models to explore the climate system response to stabilizing the anthropogenic components of radiative forcing.     

Climate effect of ozone changes caused by present and future air traffic

 The potential of aircraft-induced ozone changes to force a substantial climate impact is investigated by means of simulations with an atmospheric general circulation model, coupled to a mixed layer ocean model. We present results from several numerical experiments that are based on ozone change patterns for 1992 aviation and on a future scenario for the year 2015. In both cases, the climate signal is statistically significant. The strength of the ozone impact is of comparable magnitude to that arising from aircraft CO₂ emissions, thus meaning a non-negligible contribution to the total climate effect of aviation emissions. There are indications of a characteristic signature of the aircraft ozone related temperature response pattern, distinctly different from that associated with the increase of well-mixed greenhouse gases. Likewise, the climate sensitivity to non-uniform ozone changes including a strong concentration perturbation at the tropopause may be higher than the climate sensitivity to uniform changes of a greenhouse gas. In a hierarchy of experiments, for which the spatial structure of an aircraft-related ozone perturbation was left fixed, while the amplitude of the perturbation was artificially increased, the climate signal depends in a non-linear way on the radiative forcing. Received: 10 September 1998 / Accepted: 4 May 1999