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1.
A global two-dimensional (altitude-latitude) chemistry transport model is used to follow the changes in the tropospheric distribution of the two major radiatively active trace gases, methane and ozone, following step changes to the sustained emissions of the short-lived trace gases methane, carbon monoxide and non-methane hydrocarbons. The radiative impacts were dependent on the latitude chosen for the applied change in emissions. Step change global warming potentials (GWPs) were derived for a range of short-lived trace gases to describe their time-integrated radiative forcing impacts for unit emissions relative to that of carbon dioxide. The GWPs show that the tropospheric chemistry of the hydrocarbons can produce significant indirect radiative impacts through changing the tropospheric distributions of hydroxyl radicals, methane and ozone. For aircraft, the indirect radiative forcing impact of the NO x emissions appears to be greater than that from their carbon dioxide emissions. Quantitative results from this two-dimensional model study must, however, be viewed against the known inadequacies of zonally-averaged models and their poor representation of many important tropospheric processes.  相似文献   

2.
Today's climate policy is based on the assumption that the location of emissions reductions has no impact on the overall climate effect. However, this may not be the case since reductions of greenhouse gases generally will lead to changes in emissions of short-lived gases and aerosols. Abatement measures may be primarily targeted at reducing CO2, but may also simultaneously reduce emissions of NOx, CO, CH4 and SO2 and aerosols. Emissions of these species may cause significant additional radiative forcing. We have used a global 3-D chemical transport model and a radiative transfer model to study the impact on climate in terms of radiative forcing for a realistic change in location of the emissions from large-scale sources. Based on an assumed 10% reduction in CO2 emissions, reductions in the emissions of other species have been estimated. Climate impact for the SRES A1B scenario is compared to two reduction cases, with the main focus on a case with emission reductions between 2010 and 2030, but also a case with sustained emission reductions. The emission reductions are applied to four different regions (Europe, China, South Asia, and South America). In terms of integrated radiative forcing (over 100 yr), the total effect (including only the direct effect of aerosols) is always smaller than for CO2 alone. Large variations between the regions are found (53–86% of the CO2 effect). Inclusion of the indirect effects of sulphate aerosols reduces the net effect of measures towards zero. The global temperature responses, calculated with a simple energy balance model, show an initial additional warming of different magnitude between the regions followed by a more uniform reduction in the warming later. A major part of the regional differences can be attributed to differences related to aerosols, while ozone and changes in methane lifetime make relatively small contributions. Emission reductions in a different sector (e.g. transportation instead of large-scale sources) might change this conclusion since the NOx to SO2 ratio in the emissions is significantly higher for transportation than for large-scale sources. The total climate effect of abatement measures thus depends on (i) which gases and aerosols are affected by the measure, (ii) the lifetime of the measure implemented, (iii) time horizon over which the effects are considered, and (iv) the chemical, physical and meteorological conditions in the region. There are important policy implications of the results. Equal effects of a measure cannot be assumed if the measure is implemented in a different region and if several gases are affected. Thus, the design of emission reduction measures should be considered thoroughly before implementation.  相似文献   

3.
The radiative impact of greenhouse gases in warming the Earth varies significantly, depending on whether one considers the forcing at the tropopause or at the surface. Compared to the former, the surface forcing for some greenhouse gases is reduced by the interference of water vapour. Hence, we calculate alternative surface global warming potentials (SGWPs) that are derived from the surface forcing radiation of greenhouse gases for potential use in surface radiative energy balance models (SREBMs). For gases with a large water vapour overlap, the SGWPs are typically 30% smaller than current GWPs; for gases with relatively little overlap, the SGWPs are larger by more than 33%. These results may be used in conjunction with SREBMs as an additional means of calculating climate change, and may lead to an altered emissions budget compared to that outlined by the current Kyoto agreement.  相似文献   

4.
We use recent advances in time series econometrics to estimate the relation among emissions of CO2 and CH4, the concentration of these gases, and global surface temperature. These models are estimated and specified to answer two questions; (1) does human activity affect global surface temperature and; (2) does global surface temperature affect the atmospheric concentration of carbon dioxide and/or methane. Regression results provide direct evidence for a statistically meaningful relation between radiative forcing and global surface temperature. A simple model based on these results indicates that greenhouse gases and anthropogenic sulfur emissions are largely responsible for the change in temperature over the last 130 years. The regression results also indicate that increases in surface temperature since 1870 have changed the flow of carbon dioxide to and from the atmosphere in a way that increases its atmospheric concentration. Finally, the regression results for methane hint that higher temperatures may increase its atmospheric concentration, but this effect is not estimated precisely.  相似文献   

5.
RCP4.5: a pathway for stabilization of radiative forcing by 2100   总被引:3,自引:2,他引:1  
Representative Concentration Pathway (RCP) 4.5 is a scenario that stabilizes radiative forcing at 4.5?W?m?2 in the year 2100 without ever exceeding that value. Simulated with the Global Change Assessment Model (GCAM), RCP4.5 includes long-term, global emissions of greenhouse gases, short-lived species, and land-use-land-cover in a global economic framework. RCP4.5 was updated from earlier GCAM scenarios to incorporate historical emissions and land cover information common to the RCP process and follows a cost-minimizing pathway to reach the target radiative forcing. The imperative to limit emissions in order to reach this target drives changes in the energy system, including shifts to electricity, to lower emissions energy technologies and to the deployment of carbon capture and geologic storage technology. In addition, the RCP4.5 emissions price also applies to land use emissions; as a result, forest lands expand from their present day extent. The simulated future emissions and land use were downscaled from the regional simulation to a grid to facilitate transfer to climate models. While there are many alternative pathways to achieve a radiative forcing level of 4.5?W?m?2, the application of the RCP4.5 provides a common platform for climate models to explore the climate system response to stabilizing the anthropogenic components of radiative forcing.  相似文献   

6.
Among anthropogenic perturbations of the Earths atmosphere, greenhouse gases and aerosols are considered to have a major impact on the energy budget through their impact on radiative fluxes. We use three ensembles of simulations with the LMDZ general circulation model to investigate the radiative impacts of five species of greenhouse gases (CO2, CH4, N2O, CFC-11 and CFC-12) and sulfate aerosols for the period 1930–1989. Since our focus is on the atmospheric changes in clouds and radiation from greenhouse gases and aerosols, we prescribed sea-surface temperatures in these simulations. Besides the direct impact on radiation through the greenhouse effect and scattering of sunlight by aerosols, strong radiative impacts of both perturbations through changes in cloudiness are analysed. The increase in greenhouse gas concentration leads to a reduction of clouds at all atmospheric levels, thus decreasing the total greenhouse effect in the longwave spectrum and increasing absorption of solar radiation by reduction of cloud albedo. Increasing anthropogenic aerosol burden results in a decrease in high-level cloud cover through a cooling of the atmosphere, and an increase in the low-level cloud cover through the second aerosol indirect effect. The trend in low-level cloud lifetime due to aerosols is quantified to 0.5 min day–1 decade–1 for the simulation period. The different changes in high (decrease) and low-level (increase) cloudiness due to the response of cloud processes to aerosols impact shortwave radiation in a contrariwise manner, and the net effect is slightly positive. The total aerosol effect including the aerosol direct and first indirect effects remains strongly negative.  相似文献   

7.
Increasing atmospheric concentrations of greenhouse gases are expected to result in global climatic changes over the next decades. Means of evaluating and reducing greenhouse gas emissions are being sought. In this study an existing simulation model of a tropical savanna woodland grazing system was adapted to account for greenhouse gas emissions. This approach may be able to be used in identifying ways to assess and limit emissions from other rangeland, agricultural and natural ecosystems.GRASSMAN, an agricultural decision-support model, was modified to include sources, sinks and storages of greenhouse gases in the tropical and sub-tropical savanna woodlands of northern Australia. The modified model was then used to predict the changes in emissions and productivity resulting from changes in stock and burning management in a hypothetical grazing system in tropical northeastern Queensland. The sensitivity of these results to different Global Warming Potentials (GWPs) and emission definitions was then tested.Management options to reduce greenhouse gas emissions from the tropical grazing system investigated were highly sensitive to the GWPs used, and to the emission definition adopted. A recommendation to reduce emissions by changing burning management would be toreduce fire frequency if both direct and indirect GWPs of CO2, CH4, N2O, CO and NO are used in evaluating emissions, but toincrease fire frequency if only direct GWPs of CO2, CH4 and N2O are used. The ability to reduce greenhouse gas emissions from these systems by reducing stocking rates was also sensitive to the GWPs used. In heavily grazed systems, the relatively small reductions in stocking rate needed to reduce emissions significantly should also reduce the degradation of soils and vegetation, thereby improving the sustainability of these enterprises.The simulation studies indicate that it is possible to alter management to maximise beef cattle production per unit greenhouse gases or per unit methane emitted, but that this is also dependent upon the emission definition used. High ratios of liveweight gain per unit net greenhouse gas emission were found in a broadly defined band covering the entire range of stocking rates likely to be used. In contrast, high values of liveweight gain per unit anthropogenic greenhouse gas emission were found only at very low stocking rates that are unlikely to be economically viable.These results suggest that policy initiatives to reduce greenhouse gas emissions from tropical grazing systems should be evaluated cautiously until the GWPs have been further developed and the implications of emission definitions more rigorously determined.  相似文献   

8.
The RCP2.6 emission and concentration pathway is representative of the literature on mitigation scenarios aiming to limit the increase of global mean temperature to 2°C. These scenarios form the low end of the scenario literature in terms of emissions and radiative forcing. They often show negative emissions from energy use in the second half of the 21st century. The RCP2.6 scenario is shown to be technically feasible in the IMAGE integrated assessment modeling framework from a medium emission baseline scenario, assuming full participation of all countries. Cumulative emissions of greenhouse gases from 2010 to 2100 need to be reduced by 70% compared to a baseline scenario, requiring substantial changes in energy use and emissions of non-CO2 gases. These measures (specifically the use of bio-energy and reforestation measures) also have clear consequences for global land use. Based on the RCP2.6 scenario, recommendations for further research on low emission scenarios have been formulated. These include the response of the climate system to a radiative forcing peak, the ability of society to achieve the required emission reduction rates given political and social inertia and the possibilities to further reduce emissions of non-CO2 gases.  相似文献   

9.
Under the Paris Agreement, countries are encouraged to submit long-term low greenhouse gas emissions development strategies. Such strategies will merge emissions goals with socio-economic objectives and enable countries to increase their ambition over time, thus offering an opportunity to close the gap between the current emissions trajectory and the Agreement’s ‘well below 2°C’ target. China is in the process of preparing its own long-term strategy. We argue in this article that non-CO2 greenhouse gases (NCGGs) should be an essential component of China’s long-term low-emissions strategy. To incorporate NCGGs into China’s long-term low-emissions development strategy, key scientific and institutional challenges should be addressed, such as uncertainty about the accuracy of NCGG emissions inventories; uncertainty about future projections of NCGG emissions; and institutional coordination deficits and imbalanced policy approaches. Overcoming these barriers will have significant implications for climate change mitigation and can open a path for the development of concrete follow-up actions.

Key policy insights

  • Non-CO2 greenhouse gases (NCGGs) make up around 17% of China’s GHG emissions, but China has no quantified target to limit or reduce these gases.

  • NCGG emissions mitigation should be an essential component of China's long-term low-emissions strategy, which is currently under development.

  • Considerable uncertainty exists over both historical NCGG emissions data and forecasts. This poses challenges to developing a comprehensive multi-gas strategy.

  • Institutional challenges must also be addressed, such as fragmentation of responsibility for NCGGs.

  相似文献   

10.
An emission pathway for stabilization at 6?Wm?2 radiative forcing   总被引:1,自引:0,他引:1  
Representative Concentration Pathway 6.0 (RCP6) is a pathway that describes trends in long-term, global emissions of greenhouse gases (GHGs), short-lived species, and land-use/land-cover change leading to a stabilisation of radiative forcing at 6.0 Watts per square meter (Wm?2) in the year 2100 without exceeding that value in prior years. Simulated with the Asia-Pacific Integrated Model (AIM), GHG emissions of RCP6 peak around 2060 and then decline through the rest of the century. The energy intensity improvement rates changes from 0.9% per year to 1.5% per year around 2060. Emissions are assumed to be reduced cost-effectively in any period through a global market for emissions permits. The exchange of CO2 between the atmosphere and terrestrial ecosystem through photosynthesis and respiration are estimated with the ecosystem model. The regional emissions, except CO2 and N2O, are downscaled to facilitate transfer to climate models.  相似文献   

11.
Anthropogenic aerosols play an important role in the atmospheric energy balance. Anthropogenic aerosol optical depth (AOD) and its accompanying shortwave radiative forcing (RF) are usually simulated by nu- merical models. Recently, with the development of space-borne instruments and sophisticated retrieval algorithms, it has become possible to estimate aerosol radiative forcing based on satellite observations. In this study, we have estimated shortwave direct radiative forcing due to anthropogenic aerosols over oceans in all-sky conditions by combining clouds and the Single Scanner Footprint data of the Clouds and Earth’s Radiant Energy System (CERES/SSF) experiment, which provide measurements of upward shortwave fluxes at the top of atmosphere, with Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol and cloud products. We found that globally averaged aerosol radiative forcing over oceans in the clear-sky conditions and all-sky conditions were -1.03±0.48 W m-2 and -0.34 ±0.16 W m-2, respectively. Direct radiative forcing by anthropogenic aerosols shows large regional and seasonal variations. In some regions and in particular seasons, the magnitude of direct forcing by anthropogenic aerosols can be comparable to the forcing of greenhouse gases. However, it shows that aerosols caused the cooling effect, rather than warming effect from global scale, which is different from greenhouse gases.  相似文献   

12.
The global three-dimensional Lagrangian chemistry-transport model STOCHEM has been used to follow the changes in the tropospheric distributions of the two major radiatively-active trace gases, methane and tropospheric ozone, following the emission of pulses of the short-lived tropospheric ozone precursor species, methane, carbon monoxide, NOx and hydrogen. The radiative impacts of NOx emissionswere dependent on the location chosen for the emission pulse, whether at the surface or in the upper troposphere or whether in the northern or southern hemispheres. Global warming potentials were derived for each of the short-lived tropospheric ozone precursor species by integrating the methane and tropospheric ozone responses over a 100 year time horizon. Indirect radiative forcing due to methane and tropospheric ozone changes appear to be significant for all of the tropospheric ozone precursor species studied. Whereas the radiative forcing from methane changes is likely to be dominated by methane emissions, that from tropospheric ozone changes is controlled by all the tropospheric ozone precursor gases, particularly NOxemissions. The indirect radiative forcing impacts of tropospheric ozone changes may be large enough such that ozone precursors should be considered in the basket of trace gases through which policy-makers aim to combat global climate change.  相似文献   

13.
Increases in chlorinated and brominated halocarbons are believed to be responsible for the depletion of stratospheric ozone observed over much of the globe in the past decade or so. Ozone depletion is in turn believed to lead to a negative radiative forcing, tending to cool the stratosphere and the surface. We show that the increasing atmospheric concentrations of ozone-depleting halocarbons and onset of related ozone depletion likely led to a negative forcing of the climate system in the 1980s that slowed significantly the rate of change of total anthropogenic radiative forcing due to the combined effect of all greenhouse gases over that decade. Within the next decade, emissions of these halocarbons are expected to rapidly decrease, with corresponding impacts on ozone and radiative forcing. As the emissions of ozone-depleting gases are reduced and eventually phased out, the rate of ozone depletion is expected to decrease and eventually reverse. All other things being equal, we show that the change from deepening ozone depletion in the 1980s to ozone increases in the future should lead to a pronounced increase in the decadal rate of change of anthropogenic greenhouse forcing of the next few decades, perhaps to levels unprecedented in this century.  相似文献   

14.
Based on univariate correlation and coherence analyses and considering the physical basis of the relationships, a simple multiforced (multiple) statistical concept is used which correlates observational climatic time series simultaneously with volcanic, solar, ENSO, and the anthropogenic greenhouse gases forcing. This is appropriate to remove some natural climate noise in the observed data and to evaluate the components (signals) possibly due to the anthropogenic greenhouse gas forcing (CO2, or equivalent CO2 implying additional gases) during industrial time. In this paper, we apply this technique to 100 global box data time series 1890–1985, of the surface air temperature, using observed data from Hansen and Lebedeff. The results are presented in terms of latitudinal-seasonal and regional trends, where the observed trend patterns are compared with the hypothetical signals (statistical assessments) possibly due to anthropogenic greenhouse forcing. These latter signals can be amplified to enable a comparison with corresponding results from general circulation model (GCM) CO2 doubling experiments. These observed-statistical assessments lead to results which are, at least qualitatively and in respect to the zonal mean temperatures, very similar to some GCM experiments indicating the maximum CO2 doubling signals (statistical assessment > 12 K) in the arctic winter. However, these signals are moderate in the tropics and in the Southern Hemisphere (global average 2.8–4.4 K). As far as the industrial signals are concerned (observed period) these signals are somewhat larger (maximum 7 K, global average 0.5–0.9 K) than the observed trends (maximum 5 K, global average 0.5 K). Phase shifts of cause and effect may amplify these signals but are very uncertain.This paper was presented at the International Conference on Modelling of Global Climate Change and Variability, held in Hamburg 11–15 September 1989 under the auspices of the Meteorological Institute of the University of Hamburg and the Max Planck Institute for Meteorology. Guest Editor for these papers is Dr. L. Dümenil  相似文献   

15.
The global three-dimensional Lagrangian chemistry-transport model STOCHEM has been used to follow changes in the tropospheric distributions of methane CH4 and ozone O3 following the emission of pulses of the oxides of nitrogen NO x . Month-long emission pulses of NO x produce deficits in CH4 mixing ratios that bring about negative radiative forcing (climate cooling) and decay away with e-folding times of 10–15 years. They also produce short-term excesses in O3 mixing ratios that bring about positive radiative forcing (climate warming) that decay over several months to produce deficits, with their attendant negative radiative forcing (climate cooling) that decays away in step with the CH4 deficits. Total time-integrated net radiative forcing is markedly influenced by cancellation between the negative CH4 and long-term O3 contributions and the positive short-term O3 contribution to leave a small negative residual. Consequently, total net radiative forcing from NO x emission pulses and the global warming potentials derived from them, show a strong dependence on the magnitudes, locations and seasons of the emissions. These dependences are illustrated using the Asian continent as an example and demonstrate that there is no simple robust relationship between continental-scale NO x emissions and globally-integrated radiative forcing. We find that the magnitude of the time-integrated radiative forcing from NO x -driven CH4 depletion tends to approach and outweigh that from ozone enhancement, leaving net time-integrated radiative forcings and global warming potentials negative (climate cooling) in contrast to the situation for aircraft NO x (climate warming). Control of man-made surface NO x emissions alone may lead to positive radiative forcing (climate warming).  相似文献   

16.
This paper discusses methodological issues relevant to the calculation of historical responsibility of countries for climate change (‘The Brazilian Proposal’). Using a simple representation of the climate system, the paper compares contributions to climate change using different indicators: current radiative forcing, current GWP-weighted emissions, radiative forcing from increased concentrations, cumulative GWP-weighted emissions, global-average surface-air temperature increase and two new indicators: weighted concentrations (analogue to GWP-weighted emissions) and integrated temperature increase. Only the last two indicators are at the same time ‘backward looking’ (take into account historical emissions), ‘backward discounting’ (early emissions weigh less, depending on the decay in the atmosphere) and ‘forward looking’ (future effects of the emissions are considered) and are comparable for all gases. Cumulative GWP-weighted emissions are simple to calculate but are not ‘backward discounting’. ‘Radiative forcing’ and ‘temperature increase’ are not ‘forward looking’. ‘Temperature increase’ discounts the emissions of the last decade due to the slow response of the climate system. It therefore gives low weight to regions that have recently significantly increased emissions. Results of the five different indicators are quite similar for large groups (but possibly not for individual countries): industrialized countries contributed around 60% to today’s climate change, developing countries around 40% (using the available data for fossil, industrial and forestry CO2, CH4 and N2O). The paper further argues including non-linearities of the climate system or using a simplified linear system is a political choice. The paper also notes that results of contributions to climate change need to be interpreted with care: Countries that developed early benefited economically, but have high historical emission, and countries developing at a later period can profit from developments in other countries and are therefore likely to have a lower contribution to climate change.  相似文献   

17.
The surface energy fluxes simulated by the CSIRO9 Mark 1 GCM for present and doubled CO2 conditions are analyzed. On the global scale the climatological flux fields are similar to those from four GCMs studied previously. A diagnostic calculation is used to provide estimates of the radiative forcing by the GCM atmosphere. For 1 × CO2, in the global and annual mean, cloud produces a net cooling at the surface of 31 W m–2. The clear-sky longwave surface greenhouse effect is 311 W m–2, while the corresponding shortwave term is –79 W m–2. As for the other GCM results, the CSIRO9 CO2 surface warming (global mean 4.8°C) is closely related to the increased downward longwave radiation (LW ). Global mean net cloud forcing changes little. The contrast in warming between land and ocean, largely due to the increase in evaporative cooling (E) over ocean, is highlighted. In order to further the understanding of influences on the fluxes, simple physically based linear models are developed using multiple regression. Applied to both 1 × CO2 and CO2 December–February mean tropical fields from CSIRO9, the linear models quite accurately (3–5 W m–2 for 1 × CO2 and 2–3 W m–2 for CO2) relate LW and net shortwave radiation to temperature, surface albedo, the water vapor column, and cloud. The linear models provide alternative estimates of radiative forcing terms to those from the diagnostic calculation. Tropical mean cloud forcings are compared. Over land, E is well correlated with soil moisture, and sensible heat with air-surface temperature difference. However an attempt to relate the spatial variation of LWt within the tropics to that of the nonflux fields had little success. Regional changes in surface temperature are not linearly related to, for instance, changes in cloud or soil moisture.  相似文献   

18.
Global Warming Potentials: 2. Accuracy   总被引:1,自引:1,他引:0  
This paper exposes flaws in the mathematical structure of the Global Warming Potential (GWP) concept. These lead to errors when emissions changes in different greenhouse gases are compared. The most fundamental problem is that the unit impulse response functions from which GWPs, and many of their proposed alternatives, are constructed provide an incomplete representation of the relationship between emissions and radiative forcing. Additional errors occur when GWPs are used to compare finite-length emissions changes.  相似文献   

19.
We identify and remove the main natural perturbations (e.g. volcanic activity, ENSOs) from the global mean lower tropospheric temperatures (T LT ) over January 1979 - June 2017 to estimate the underlying, potentially human-forced trend. The unaltered value is +0.155 K dec?1 while the adjusted trend is +0.096 K dec?1, related primarily to the removal of volcanic cooling in the early part of the record. This is essentially the same value we determined in 1994 (+0.09 K dec?1, Christy and McNider, 1994) using only 15 years of data. If the warming rate of +0.096 K dec?1 represents the net T LT response to increasing greenhouse radiative forcings, this implies that the T LT tropospheric transient climate response (ΔT LT at the time CO2 doubles) is +1.10 ± 0.26 K which is about half of the average of the IPCC AR5 climate models of 2.31 ± 0.20 K. Assuming that the net remaining unknown internal and external natural forcing over this period is near zero, the mismatch since 1979 between observations and CMIP-5 model values suggests that excessive sensitivity to enhanced radiative forcing in the models can be appreciable. The tropical region is mainly responsible for this discrepancy suggesting processes that are the likely sources of the extra sensitivity are (a) the parameterized hydrology of the deep atmosphere, (b) the parameterized heat-partitioning at the oceanatmosphere interface and/or (c) unknown natural variations.  相似文献   

20.
Deforestation in Brazilian Amazonia is a significant source of greenhouse gases today and, with almost 90% of the originally forested area still uncleared, is a very large potential source of future emissions. The 1990 rate of loss of forest (13.8 × 103 km2/year) and cerrado savanna (approximately 5 × 103 km2/year) was responsible for releasing approximately 261 × 106 metric tons of carbon (106 t C) in the form of CO2, or 274–285 × 106 t of CO2-equivalent C considering IPCC 1994 global warming potentials for trace gases over a 100-year horizon. These calculations consider conversion to a landscape of agriculture, productive pasture, degraded pasture, secondary forest, and regenerated forest in the proportions corresponding to the equilibrium condition implied by current land-use patterns. Emissions are expressed as net committed emissions, or the gases released over a period of years as the carbon stock in each hectare deforested approaches a new equilibrium in the landscape that replaces the original forest. For low and high trace gas scenarios, respectively, 1990 clearing produced net committed emissions (in 106 t of gas) of 957–958 for CO2, 1.10–1.42 for CH4, 28–35 for CO, 0.06–0.16 for N2O, 0.74–0.74 for NOx and 0.58–1.16 for non-methane hydrocarbons.  相似文献   

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