Depositional rates and dating techniques of modern deposits in the Brno reservoir (Czech Republic) during the last 70 years

Facies analysis, magnetic susceptibility, and analysis of grain size, TOC content and isotopes (¹³⁷Cs, ²¹⁰Pb, ²²⁶Ra, ²²⁸Ra, and ²³⁸U concentrations) were used to determine the history of the modern deposits of the Brno reservoir. The sedimentary succession can be subdivided into two main units. The lower unit is formed predominantly by medium- to coarse-grained silty sands and is interpreted as a fluvial succession deposited before the Svratka River was dammed. The upper unit consists of brownish planar laminated silts and rarely of clayey or sandy silts and is interpreted as a product of the reservoir deposition. The concentrations of ²³⁸U reflect the history of uranium mining in the upper part of the Svratka River catchment. As a consequence, ²¹⁰Pb radionuclide concentrations cannot be used for establishing a sediment chronology. Concentrations of ¹³⁷Cs show two marked peaks, the upper of which is attributed to the Chernobyl reactor accident in 1986, and the lower one is attributed to the maximum rate of atomic weapons testing in 1963. From these peaks, mean depositional rates of 3.2 cm year⁻¹ for the time period of 1986–2007 and of 3.4 cm year⁻¹ between 1963 and 1986 are calculated. Based on the known age of the reservoir, which was constructed in 1939, we can also calculate mean depositional rate for the time period of 1939–1963, which is 3.1 cm year⁻¹.     

A 140-year record of recent changes in aquatic productivity in a remote,tropical alpine lake in the Rwenzori Mountain National Park,Uganda

Environmental change in many tropical, alpine habitats remains poorly resolved due to an absence of proximate and sustained observations. In the Rwenzori Mountains of East Africa, glaciers have receded rapidly over the last century, and here we assess the impact of this recession through palaeolimnological analyses of a 45 cm sediment core (Buju3) from Lake Bujuku which is closest to the ice-fields and partly supplied by melt water in-flows. ²¹⁰Pb and ¹³⁷Cs suggest that Buju3 has an average sedimentation rate of 2.9 mm year⁻¹ and the base of the core can be dated to 1864 ± 20 years. Contemporary diatom taxa found in the lake are dominated by Tabellaria flocculosa and Synedra spp., but also include Achnanthes minutissima and Fragilaria pinnata. However, the diatom flora for Buju3 is less diverse and dominated by small, tychoplanktonic species of Fragilaria. Over the period associated with glacial recession, organic carbon isotope analysis (δ¹³C) suggests a small but distinct increase in within-lake productivity, which increases in rate since the mid 1970s up to the present day, in line with a shift towards increased algal productivity (as highlighted by C/N ratios). However, the diatom and pollen records appear rather insensitive to changes in glacier recession since the late 19th century.     

Post-depositional 137Cs Mobility in the Sediments of Three Shallow Coastal Lagoons, SW England

We present ¹³⁷Cs profiles for three low lying coastal lagoons in Southwest England that show a decline in activity with sediment depth. ¹³⁷Cs inventories are lower than expected by comparison with local reference inventories despite the fact that sampling was undertaken in the deep-water zone of each lake where sediment and ¹³⁷Cs focusing would be expected. At all three locations, lake sediment ⁷Be and unsupported ²¹⁰Pb (²¹⁰Pb_un) inventories are not significantly lower than the local reference inventory. ¹³⁷Cs inventories in the study cores range from 38 to 95% of local reference inventories. The standing water level and mud: water interface at two sites are below maximum tide level and, at all three sites, salinity increases significantly in the water columns between low and high tide and in the pore waters of the underlying sediments. We suggest that the difference in hydrostatic pressure between sea level and standing water levels in the lagoons forces salt water up through the sediment column and that monovalent cations (especially Na⁺ and K⁺) replace ¹³⁷Cs on exchange sites leading to the upward migration and loss of ¹³⁷Cs. Rising sea levels may therefore contribute to remobilisation and release of ¹³⁷Cs to the aquatic environment from the sediments of coastal lagoons.     

Anthropogenic radionuclides in the water column and a sediment core from the Alboran Sea: application to radiometric dating and reconstruction of historical water column radionuclide concentrations

Global fallout is the main source of anthropogenic radionuclides in the Mediterranean Sea. This work presents ¹³⁷Cs, ^239+240Pu and ²⁴¹Am concentrations in the water column in the southwest Alboran Sea, which was sampled in December 1999. A sediment core was taken at 800 m depth in the area (35°47′ N, 04°48′ W). ²¹⁰Pb, ²²⁶Ra, ¹³⁷Cs and ^239+240Pu specific activities were measured at multiple depths in the core for dating purposes. ¹³⁷Cs and ^239+240Pu profiles did not show defined peaks that could be used as time markers, and they extended up to depths for which the ²¹⁰Pb-based constant rate of supply (CRS) dating model provided inconsistent dates. These profiles can be useful to test dating models, understood as particular solutions of a general advection–diffusion problem, if the time series of radionuclide inputs into the sediment is provided. Thus, historical records of depth-averaged ¹³⁷Cs and ^239+240Pu concentrations in water, and their corresponding fluxes into the sediment, were reconstructed. A simple water-column model was used for this purpose, involving atmospheric fallout, measured distribution coefficient (k _d) values, and a first-estimate of sedimentation rates. A dating model of constant mixing with constant sedimentation rate was applied successfully to three independent records (unsupported ²¹⁰Pb, ¹³⁷Cs and ^239+240Pu), and provided the objective determination of mixing parameters and mass sedimentation rate. These results provide some insight into the fate of atmospheric inputs to this marine environment and, particularly, into the contribution from the Chernobyl accident.     

Biogeochemical records of paleoenvironmental changes in Nainital Lake,Kumaun Himalayas,India

Rapid urbanization and increased tourism around Nainital Lake in the Kumaun Himalayan region in north India has raised concerns about sediment and water pollution. Lead-210 dated sediment cores from the lake represent ~95 years of accumulation and yield a mean sedimentation rate of ~4.7 mm year⁻¹. Total organic carbon (TOC), percent N and S and their atomic C/N and C/S ratios, stable isotopes (δ¹³C, δ¹⁵N, and δ³⁴S), and specific biomarkers (n-alkanes and pigments) were measured in the core. Organic matter is primarily derived from in-lake algal production and TOC flux varies from 1.0 to 3.5 g m⁻² year⁻¹. Sediments are anoxic (Eh −328 to −187 mV) and have low (0.10–0.30 g m⁻² year⁻¹) N, but high (0.37–1.0 g m⁻² year⁻¹) S flux. Shifts in δ¹³C, δ¹⁵N, and δ³⁴S suggest in-lake microbial processes dominated by denitrification and sulfate reduction. The sediments are dominated by short-chain hydrocarbons with low Carbon Preference Index values. The pigments indicate a gradual shift to cyanobacterial domination of the phytoplankton community in recent years. Despite an increase in external input of nutrients, the trophic state of the lake has remained largely unchanged, and the perceived human-induced impacts are limited.     

A chronological assessment of Lake Okeechobee (Florida) sediments using multiple dating markers

Reconstructing recent limnological history often relies on lead-210 dating to accurately ascribe a chronology to a sediment profile. In Lake Okeechobee, Florida, a large, shallow subtropical lake that may experience severe mixing, multiple dating methods are required to confirm that conformable sedimentation has been preserved and that the assumptions of the ²¹⁰Pb method are satisfied. This study uses stratigraphic profiles of heavy metals, ¹³⁷Cs, PCBs and pollen as independent dating markers to validate the sediment chronology as determined by ²¹⁰Pb for three cores from the central mud zone of the lake. Unsupported ²¹⁰Pb and most dating markers show distinct concentration/depth profiles, suggesting that the sediments have not been severely mixed for at least the last 75 years. Onset and maximum activity of the radioisotope ¹³⁷Cs in the cores coincides with the ²¹⁰Pb-dated interval of 1945–1970. This agrees well with the known timing of atmospheric deposition of ¹³⁷Cs that resulted from above-ground nuclear testing during late 1940s until 1963. Sediment core profiles of atmospherically deposited metals such as Zn and Pb, which reflect regional increases during industrialization and decreases after regulation in the 1970s, exhibit expected concentration increases and peaks coinciding within 5–15 years of the predicted ²¹⁰Pb dates. Uranium, a contaminant in some phosphate fertilizers, shows large concentration increases at core depths dated to be about 1950 by ²¹⁰Pb, matching the intensification of agriculture after WWII. PCBs, which are expected to peak in the early 1970s, were measured in one core, and the observed peak corresponds to a ²¹⁰Pb date of about 1960. Pollen makers were unable to verify specific events, but increases in disturbance taxa and declines in native types correspond generally with the expected dates assigned by ²¹⁰Pb dating. Conformity between the ²¹⁰Pb defined dates and independent markers of < ±15 years confirm that Lake Okeechobee sediments do preserve a sequential and reliable stratigraphic history of the lake, useful for reconstructing past limnological conditions.     

A lake sediment record of Pb mining from Ullswater,English Lake District,UK

Lake sediments can be significantly impacted by industrial activities. These impacts vary among sites and include both local point sources and atmospherically-derived pollution. Here we present results of a lake sediment pollution record from Ullswater, UK, where lead mining activities have taken place within the catchment since 1690, although large-scale mining did not begin until 1840. Metal concentration data from 12 cores taken along a lake bed transect illustrate that lead mining at Greenside Mine had a significant impact on the lake sediments. High Pb concentrations were identified throughout Ullswater, and exhibited a spatial gradient from south to north, with concentrations decreasing with greater distance from the main source of input at Glenridding. Furthermore, inter-element correlations exhibit spatial variation that reflects the processes by which they are incorporated into the lake sediment record. Together, these observations illustrate potential shortcomings in palaeoenvironmental reconstructions and pollution studies based on single cores from large and morphologically variable lakes. Sedimentation rates were estimated by matching this pollution record with the historical record of mining activities. Within Ullswater, sedimentation rates from 1840 to the present varied from 0.67 to 2.33 mm year⁻¹ with a mean of 1.4 mm year⁻¹; highest sedimentation rates were observed in the deepest section of the lake and close to the main inputs, and lowest sedimentation rates were observed in the northern part of the lake, furthest from the main input. Despite the considerable changes in mining techniques and production, there is little evidence to suggest significant changes in sedimentation rates over time.     

Lithological and geochemical record of anthropogenic changes in recent sediments of a small and shallow lake (Lake Pusty Staw,northern Poland)

The article presents the results of lithological and geochemical investigations of recent sediments of Lake Pusty Staw. The analysed sediments document about 300 years of the history of this lake. Historical materials indicate that significant changes in the catchment of the lake took place from the beginning of the 18th century (deforestation and afforestation) followed by 19th century tourist development, and 20th century industrialisation. The sediments were dated using the ²¹⁰Pb and ¹³⁷Cs method and core lithology. These made it possible to establish a reliable chronology to the year 1730. The calculated sedimentation rates ranged between 0.17 and 0.83 cm year^–1. There was a period of intensified erosion caused by land clearance between 1734 and 1810, which resulted in an acceleration in sedimentation rate (0.36 cm year^–1) and a change of lithological type of sediment from detritus gyttja to clayey gyttja. On the basis of Cu, Zn, Cd and Pb content in the sediments, it was determined that the beginning of pollution of the lake dates back to the 19th century and was caused probably by the existence of a health resort. A systematic increase in pollution occurred in the 20th century as a result of industrial plants. Normalised with respect to Al, the content of heavy metals in polluted sediments was from several to twenty times higher than in sediments of the preindustrial period, and a comparison of historical materials with changes of sediments in most cases made it possible to identify the direct causes of the increase in pollution.     

Difficulties in interpreting fast mixing in the radiometric dating of sediments using 210Pb and 137Cs

²¹⁰Pb geochronologies should be validated with independent tracers such as ¹³⁷Cs. In the cases with constant ²¹⁰Pb activity in the topmost sediments, the presence of a distinct ¹³⁷Cs peak within the ²¹⁰Pb plateau has been used as a definitive demonstration of acceleration (increase in the sedimentation rate in recent years) versus fast mixing. Nevertheless, some limitations can be identified in the use of semiquantitative arguments, and a global understanding of the whole ¹³⁷Cs activity profile is then required. Particularly, the incomplete mixing within the top sediment zone (described through the Incomplete Mixing Zone model) can explain quantitatively and simultaneously the ¹³⁷Cs peak and the flattening in the ²¹⁰Pb activity profile. This is demonstrated using selected examples from literature data. Thus, measured constant ²¹⁰Pb activities in the top 6 cm of a sediment core from Lake Zürich. Nevertheless, they found ⁷Be only in the uppermost layer, the distinct ¹³⁷Cs maximum at 6 cm depth, and undisturbed varves. The fast mixing seemed then opposed to common sense. The constant rate of supply model shows acceleration and it adequately matches the position of the 1963 ¹³⁷Cs peak. Nevertheless it fails to explain the whole ¹³⁷Cs profile when handling time series of ¹³⁷Cs atmospheric deposition. Finally, it is shown how the incomplete mixing of the activity (through the pore water) over a certain mass depth at the top sediment, with a finite value of the mixing coefficient, can quantitatively explain the whole activity versus mass depth profiles of ¹³⁷Cs and ²¹⁰Pb, and the presence of ⁷Be only in the uppermost sediment layer. A further validation of these ideas is presented from other literature data.     

Wind control on the accumulation of heavy metals in sediment of Lake Ulubat,Anatolia, Turkey

Freshwater Lake Ulubat (z _mean = 1.5–2.0 m and Area = ~138 km²), NW Anatolia, Turkey was filled in by fine-to-medium-grain silts during the late Holocene. Deposition in Lake Ulubat has been 1.6 cm year⁻¹ for the last 50 years, but the sedimentation rate over the last ~1,600 years was lower (0.37 mm year⁻¹). The organic matter and carbonate contents of the infill show cyclic changes that reflect environmental fluctuations. The silt-dominated lithology and the vertically uniform heavy metal distributions are probably due to wind-controlled sedimentation in the lake. Heterogeneous mud, derived from a large, mountainous drainage basin, is deposited in the lake mostly during summer, June to October, when conditions are hot and calm. Winter months are stormier and sediments are re-suspended due to the shallow water depth and the effect of waves on the lake bottom. It is likely that re-suspended sediments, particularly fine-grained particles, together with the heavy metals, are transported out of the lake via the outlet, especially during periods of high lake level. This resuspension and removal process probably caused the lake sediments to become silt-dominated and depleted in heavy metals. The role of broad shallow lakes in sequestering sediments and heavy metals can be described more accurately when wind data are considered. Such information may also be helpful for land-use planning in downstream areas.     

Assessing the utility of 210Pb geochronology for estimating sediment accumulation rates on river floodplains in Fiji

Low‐energy gamma ray spectroscopy has been employed to estimate floodplain sedimentation rates using measurements of ²¹⁰Pb in floodplain alluvium. The utility of the technique is assessed through the analysis of excess (unsupported) ²¹⁰Pb profiles in three sediment cores taken from the floodplain of the Labasa River on Vanua Levu in northern Fiji. A low‐energy germanium spectrometer (LEGe) was used for the nondestructive determination of excess ²¹⁰Pb in a region cultivated intensively with sugarcane. Measured average historical (c. 25 years) vertical accretion rates are between 2.2 and 4.4 cm yr^?1. The findings are broadly comparable with published sedimentation rates from analyses of radionuclide profiles elsewhere in the tropical South Pacific Islands, but the rates are higher than those measured previously at the same Labasa River sites using ¹³⁷Cs profiles. Accelerated soil erosion owing to cane burning and land tillage seems to be largely responsible for sediment production, although flood‐related effects such as channel accretion by coarse bedload and the emplacement of large organic debris also influence floodplain sedimentation. However, application of the ²¹⁰Pb technique in Fiji (and perhaps neighbouring island countries) is found to have serious drawbacks compared to the more robust ¹³⁷Cs method, owing principally to the low ²¹⁰Pb concentrations in the sandy alluvial sediment tested.     

Mixing, sediment accumulation and focusing using 210Pb and 137Cs

The Portil lagoon is a natural freshwater reservoir located at the southwest of Spain, near the coast. In its surroundings an important tourist complex has been developed since the earlier 1970s. This has resulted in increased loads of nutrients, specially during summer months. In order to evaluate the impact from humans on the lagoon caused by anthropogenic activities, we have determined vertical profiles of excess ²¹⁰Pb and ¹³⁷Cs in a sediment core taken from its bottom. Vertical profile of excess ²¹⁰Pb seems to indicate that the sediment core was affected by large-scale mixing processes. Nevertheless this possibility was ruled out based on the shape of the ¹³⁷Cs vertical distribution after modelling the ¹³⁷Cs profile considering large-scale mixing. The chronology developed from ²¹⁰Pb and ¹³⁷Cs has allowed us to calculate the temporal evolution of the mass sedimentation rate during the last century. This mass sedimentation rate increased in 1973: from 0.08(2) g cm^-2 a^-1 in the period 1900-1973 to 0.17(5) g cm^-2 a^-1 in the period 1973-1995. This increase could be related to land-movements in the drainage area and to permitted sewage inputs into the lagoon, both with its origin in the growing/running of the surrounding tourist complex.     

Using unsupported lead-210 measurements to investigate soil erosion and sediment delivery in a small Zambian catchment

Traditional techniques used to assemble information on rates of erosion and soil redistribution possess many important limitations. As a result, the use of environmental radionuclides, and more particularly ¹³⁷Cs measurements, has attracted increasing attention in recent years as a means of obtaining spatially distributed information on rates of erosion and deposition. The application of the ¹³⁷Cs approach is, however, hampered in some areas of the world where ¹³⁷Cs inventories are low and the low concentrations of ¹³⁷Cs found in soils and sediments cause problems for laboratory analysis. These problems will increase as time progresses due to the radioactive decay of the existing inventory, most of which was deposited as fallout ca. 40 years ago. This contribution explores the potential for using another fallout radionuclide, namely unsupported ²¹⁰Pb, as an alternative to ¹³⁷Cs, in the small (63 km²) Upper Kaleya catchment in southern Zambia where ¹³⁷Cs inventories are already very low. The approach employed with unsupported ²¹⁰Pb is similar to that used for ¹³⁷Cs, although the essentially constant fallout of unsupported ²¹⁰Pb through time means that the resulting estimates of erosion and soil redistribution rates reflect a longer period of time (ca. 100 years rather than ca. 40 years). The estimates of erosion and deposition rates derived from the unsupported ²¹⁰Pb measurements are used to construct typical sediment budgets for the three main land-use types in the Upper Kaleya catchment, namely, commercial cultivation, communal cultivation and bush grazing. The results obtained from the unsupported ²¹⁰Pb are compared with equivalent results based on ¹³⁷Cs measurements provided by a previous investigation undertaken in the study catchment. The two sets of results are highly consistent. The study reported confirms the viability of using unsupported ²¹⁰Pb as an alternative to ¹³⁷Cs in this environment and demonstrates that conjunctive use of both radionuclides can provide additional information on the erosional history of a study area.     

Evaluating the mobility of137Cs,239+240Pu and210Pb from their distributions in laminated lake sediments

Post-depositional mobility of¹³⁷Cs,^239+240Pu and²¹⁰Pb was assessed in six small lake basins by comparing sedimentary nuclide profiles with their known fallout history. Laminae couplets, when present, were determined to be varves because the¹³⁷Cs and^239+240Pu 1963 fallout peaks are present in laminae couplets corresponding to years 1962–1964. There is no evidence of mobility of²¹⁰Pb, because 1) mass accumulation rates based on²¹⁰Pb agree with those based on¹³⁷Cs and^239+240Pu peak depths and with those based on varve counts, and 2)²¹⁰Pb ages agree with varve ages. Significant mobility of¹³⁷Cs is evident from the penetration of¹³⁷Cs to depths 15–20 cm deeper than^239+240Pu. Deep penetration of¹³⁷Cs in spite of a sharp gradient below the peak is interpreted by a numerical model to suggest that¹³⁷Cs is present in two distinct forms in these sediments, 67–82% as an immobile form and 18–33% reversibly adsorbed with a K _d of approximately 5000. The profiles can be interpreted equally well assuming a small portionof the total¹³⁷Cs was present as an extremely mobile phase (K _d 5000) in the months to years following peak fallout, slowly becoming more strongly adsorbed. High NH ₄ ⁺ concentrations in porewaters may enhance diffusion of the mobile form of¹³⁷Cs, but not of the immobile form of¹³⁷Cs that defines the sharp gradient. Mobility of¹³⁷Cs is likely also enhanced by the low clay content and the high porosity of these sediments. Thus the first detection of¹³⁷Cs in the sediments cannot automatically be assumed to correspond to a date of 1952 (initial testing of thermonuclear weapons), although the depth of the peak can be assumed to correspond to 1963 (the year of maximum fallout from testing of thermonuclear weapons).^239+240Pu is a more reliable sediment chronometer than¹³⁷Cs because it is significantly less mobile.This is the sixth of a series of papers to be published by this journal following the 20 ^th anniversary of the first application of²¹⁰Pb dating of lake sediments. Dr P.G. Appleby is guest editing this series.     

Distribution of <Superscript>137</Superscript>Cs and <Superscript>210</Superscript>Pb in sediments of tidal flats in north Jiangsu Province

Seven cores were collected from different sediment zones of tidal flats at Xinyanggang in north Jiangsu province in August 2007. Sediment grain-size distribution and radioisotopes of ¹³⁷Cs and ²¹⁰Pb analysis were carried out for these cores. Sediment rates of the cores and radioisotopes distribution in surface sediment in different zones of the tidal flat were calculated from the ¹³⁷Cs and ²¹⁰Pb activities in sediments cores. The results indicated that each tidal zone had experienced different evolution phases, hydrological dynamics in the tidal flats made the grain-size of the surface sediment change gradually. ¹³⁷Cs and ²¹⁰Pb activities on the superficial layer of the cores varied spatially and the reason was discussed. On tidal flats, the fluctuation of ¹³⁷Cs and ²¹⁰Pb activities in the cores reflected the special sedimentary characteristics. Vegetation affects the grain-size distribution and the vertical profiles of ¹³⁷Cs and ²¹⁰Pb in the upper depths. ¹³⁷Cs and ²¹⁰Pb chronology got the comparable average sediment rates on the tidal flat. The characteristics of ¹³⁷Cs and ²¹⁰Pb in the cores reflected various depositional dynamical environments in different tidal zones and gave information on the different evolvement phases of the tidal zones. Based on the information of grain-size distribution, texture of the cores, sediment rates and topography, the evolution lines of the tidal flat were reconstructed.     

Paleolimnological assessment of recent environmental change in Lake Baikal: sediment chronology

Sediment cores collected from six sites in Lake Baikal as part of an extensive investigation of sediment records of recent environmental change were dated radiometrically by ²¹⁰Pb. Although the results obtained were in some respects comparable to those obtained by previous ²¹⁰Pb studies, there were some significant differences. Most notably, a core from abyssal depths in the centre of the middle basin appeared to record at least wo major episodes of rapid sedimentation, possibly caused by turbidity currents. All cores, including those from the North Basin, contained significant records of weapons test fallout ¹³⁷Cs, though these were of little chronological value due to the long residence time of ¹³⁷Cs in the water column. Models and budgets for sediment and radionuclide transport through Baikal are presented and used to help validate the ²¹⁰Pb results.     

Palaeovariations in the East-Asian Monsoon Regime Geochemically Recorded in Varved Sediments of Lake Sihailongwan (Northeast China, Jilin Province). Part 2: a 200-Year Record of Atmospheric Lead-210 Flux Variations and its Palaeoclimatic Implications

Palaeovariations of the atmospheric ²¹⁰Pb flux in Northeast China (Long Gang area, Jilin province), quantified by high resolution ²¹⁰Pb measurements on seasonally laminated sediments of Lake Sihailongwan are presented on decadal scale. The mean flux of unsupported ²¹⁰Pb between 1790 and 1970 for the centre of the lake basin is 517 Bq m⁻² yr⁻¹ with maximum deviations between −23% and +27% of this value. Flux rates above this average were found between 1783 and 1813, around 1836, and between 1860 and 1901. The mean ²¹⁰Pb^exc flux rates derived were clearly lower around 1821, 1908, 1930, and 1953. The ²¹⁰Pb^exc flux reached its minimum of 344 Bq m⁻² yr⁻¹ during the period 1977–1982. The atmospheric flux of unsupported ²¹⁰Pb is correlated with the precipitation frequency during the summer monsoon and shows coinciding variability with geochemical proxies that document the groundwater inflow into the lake. Al₂O₃-rich dust of remote provenance scavenged by wet-deposition in the rainy season is the major carrier of the atmospheric ²¹⁰Pb^exc flux.     

Environmental Change and Atmospheric Contamination on Svalbard: Sediment Chronology

Sediment cores collected from eight lakes along the western coast of Svalbard as part of a project investigating atmospheric pollution and environmental change in Arctic regions were dated radiometrically using natural (²¹⁰Pb) and artificial (¹³⁷Cs and ²⁴¹Am) fallout radionuclides. At four sites the sedimentation rates were relatively uniform, and in consequence the ²¹⁰Pb dates were relatively unambiguous. At the remaining sites there were irregularities in the ²¹⁰Pb activity versus depth profiles, indicating significant variations in the net sediment accumulation rate during the past 120 years. At these sites, there were significant differences between ²¹⁰Pb dates calculated using the two standard simple dating models, constant rate of supply (CRS) and constant initial concentration (CIC). In most cases, stratigraphic dates based on the ¹³⁷Cs and ²⁴¹Am records supported use of the CRS model, though at one site (Ossian Sarsfjellet) the CIC model appeared more appropriate. The irregularities in the ²¹⁰Pb records were mainly caused by episodes of accelerated sedimentation due, for example, to inwash or slump events, though at some sites there appears to have been a systematic increase in sediment accumulation rates in recent decades. Sediment accumulation rates were generally lower at the northern sites, and higher at the more southerly locations. Mean sediment accumulation rates varied by an order of magnitude, ranging from 0.002 to 0.050 g cm⁻² y⁻¹ (0.02–0.10 cm y⁻¹). ²¹⁰Pb fluxes measured from the core inventories were mostly in the range 34–80 Bq m⁻² y⁻¹ typical of Arctic sites. Much higher values, recorded at two sites (Birgervatnet and Daltjørna), may be due to significant inputs from the catchments during spring thaw.     

Twentieth century eutrophication of the St. Croix River (Minnesota–Wisconsin,USA) reconstructed from the sediments of its natural impoundment

Evaluation of land-use effects on coastal and marine ecosystems requires better understanding of the role of rivers in regulating mass transport from terrestrial to oceanic environments. Here we take advantage of the presence of a riverine lake to use paleoecological techniques to quantify impacts of logging, European-style agriculture, urbanization and continued terrestrial disturbance on mass transport and water quality in the northern drainage of the Mississippi River. Two 2-m sediment-cores recovered in 1999 from Lake St. Croix, a natural impoundment of the St. Croix River, were dated using ²¹⁰Pb and ¹³⁷Cs, and analyzed for historical changes (c. 1840–present) in sediment magnetic susceptibility, inorganic and organic matter content, biogenic silica, fossil pigments, and diatom microfossils. Inorganic sediment accumulation increased threefold between the mid-1800s and present, whereas clear signs of eutrophication were only evident after the mid-twentieth century when biogenic silica accumulation increased sixfold, diatom accumulation rates increased 20- to 50- fold, and the diatom community shifted from predominantly benthic species to assemblages composed mainly of planktonic taxa. Similarly, fossil pigment concentrations increased during the 1960s, and diatom-inferred total phosphorus (DI-TP) increased from ~30 μg TP l⁻¹ c. 1910 to ~60 μg l⁻¹ since 1990, similar to historical records since 1980. Together, these patterns demonstrate that initial land clearance did not result in substantive declines in water quality or nutrient mass transport, instead, substantial degradation of downstream environments was restricted to the latter half of the twentieth century. This is one of eight papers dedicated to the “Recent Environmental History of the Upper Mississippi River” published in this special issue of the Journal of Paleolimnology. D. R. Engstrom served as guest editor of the special issue.     

210Pb、137Cs 计年法在现代海岸带沉积速率 研究中的应用述评

²¹⁰Pb、¹³⁷Cs 计年法已被国内外广泛用于湖泊、河流和海洋现代沉积速率的研究中。本文在 回顾了210Pb、137Cs 计年法应用于海岸带沉积速率研究的现状以及存在问题的基础上, 根据海岸带 沉积环境特征分析了²¹⁰Pb、¹³⁷Cs 计年法在应用中应当注意的问题, 包括采样精准性, 样品分离的 分辨率, 数据校正方法的选择及两种方法的相互印证等。从几个方面探讨了提高沉积速率测定精 度的可能性, 同时指出, ²¹⁰Pb、¹³⁷Cs 的扩散混合模型的建立, ¹³⁷Cs 沉积滞后的问题, 以及¹³⁷Cs、²¹⁰Pb 计年法的应用范围等仍有待深入探讨。