Two-moment bulk stratiform cloud microphysics in the grid-point atmospheric model of IAP LASG (GAMIL)

A two-moment bulk stratiform microphysics scheme, including recently developed physically-based droplet activation/ice nucleation parameterizations has been implemented into the Grid-point Atmospheric Model of IAP LASG (GAMIL) as an effort to enhance the model’s capability to simulate aerosol indirect effects. Unlike the previous one-moment cloud microphysics scheme, the new scheme produces a reasonable representation of cloud particle size and number concentration. This scheme captures the observed spatial variations in cloud droplet number concentrations. Simulated ice crystal number concentrations in cirrus clouds qualitatively agree with in situ observations. The longwave and shortwave cloud forcings are in better agreement with observations. Sensitivity tests show that the column cloud droplet number concentrations calculated from two different droplet activation parameterizations are similar. However, ice crystal number concentration in mixed-phased clouds is sensitive to different heterogeneous ice nucleation formulations. The simulation with high ice crystal number concentration in mixed-phase clouds has less liquid water path and weaker cloud forcing. Furthermore, ice crystal number concentration in cirrus clouds is sensitive to different ice nucleation parameterizations. Sensitivity tests also suggest that the impact of pre-existing ice crystals on homogeneous freezing in old clouds should be taken into account.     

Aerosol Indirect Effects on Warm Clouds in the Grid-Point Atmospheric Model of IAP LASG (GAMIL)

Aerosol indirect effects on warm clouds are estimated in the Grid-point Atmospheric Model of the State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics,Institute of Atmospheric Physics(IAP LASG)(GAMIL) with a new two-moment cloud microphysics scheme using two different physically-based aerosol activation parameterizations:Abdul-Razzak and Ghan,and Nenes and Seinfeld.The annual global mean changes in shortwave cloud forcing from preindustrial times to present day(a measure of the aerosol indirect effects) estimated from these two parameterizations are remarkably similar:0.76 W m?2 with the Abdul-Razzak and Ghan parameterization,and 0.78 W m?2 with the Nenes and Seinfeld parameterization.Physically-based parameterizations can provide robust representations of aerosol effects on droplet nucleation,meaning that aerosol activation is no longer the most uncertain factor in modeling aerosol indirect effects.     

Direct Radiative Forcing of Anthropogenic Aerosols over Oceans from Satellite Observations

Anthropogenic aerosols play an important role in the atmospheric energy balance. Anthropogenic aerosol optical depth (AOD) and its accompanying shortwave radiative forcing (RF) are usually simulated by nu- merical models. Recently, with the development of space-borne instruments and sophisticated retrieval algorithms, it has become possible to estimate aerosol radiative forcing based on satellite observations. In this study, we have estimated shortwave direct radiative forcing due to anthropogenic aerosols over oceans in all-sky conditions by combining clouds and the Single Scanner Footprint data of the Clouds and Earth’s Radiant Energy System (CERES/SSF) experiment, which provide measurements of upward shortwave fluxes at the top of atmosphere, with Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol and cloud products. We found that globally averaged aerosol radiative forcing over oceans in the clear-sky conditions and all-sky conditions were -1.03±0.48 W m-2 and -0.34 ±0.16 W m-2, respectively. Direct radiative forcing by anthropogenic aerosols shows large regional and seasonal variations. In some regions and in particular seasons, the magnitude of direct forcing by anthropogenic aerosols can be comparable to the forcing of greenhouse gases. However, it shows that aerosols caused the cooling effect, rather than warming effect from global scale, which is different from greenhouse gases.     

不同形状冰晶权重假定对冰云光学和辐射特性的影响

在BCC_RAD辐射传输模式和包含多形状冰晶粒子的冰云光学性质参数化方案的基础上,详细分析了不同冰晶粒子权重选取对冰云光学和辐射特性的影响。结果显示,不同形状冰晶粒子权重的选取对长波带平均消光系数、单次散射比、不对称因子和短波带平均不对称因子均有较大的影响。冰晶粒子权重选取对长波辐射通量有很大影响:对长波向下辐射通量,权重选择不同可在云底处造成高达10.50 W/m2的差别;对长波向上辐射通量,权重选择不同可在云顶处造成高达15.05 W/m2的差别。冰晶粒子权重选择对短波辐射通量也存在较大影响:对短波向下辐射通量,权重选择不同可在云底处造成高达12.48 W/m2的差别;对短波向上辐射通量,权重选择不同可在云顶处造成高达10.23 W/m2的差别。冰晶粒子权重选择对长波加热率影响较大,在云顶处和云底处分别可达1.31和-2.06 K/d。研究表明,不同形状冰晶粒子权重的选取对冰云光学性质和辐射计算均有较大的影响,在长波区间尤其明显。      

Lidar remote sounding of cirrus clouds and comparison of simulated fluxes with surface and METEOSAT observations

Three cirrus cloud cases have been remotely sounded near Paris by a ground-based backscatter lidar and broadband radiometers. Some cirrus properties (optical depth, emissivity, height) are derived from these measurements and used to compare radiative transfer calculations to surface and METEOSAT observations of broadband irradiances.For a useful comparison, the three cirrus cases were selected to have different morphologies and optical properties: June 29, 1993—thin cirrus cloud (thickness 1.5 km, optical depth 0.22); September 6, 1993—thick cirrus cloud (thickness 5 km, optical depth 2.7); and November 16, 1993—inhomogeneous and geometrically thick cirrus cloud (thickness 3.5–6.5 km) but optically thin (optical depth 0.82).At surface, the differences between measurements and model range from 1.5 to 4 Wm⁻² for longwave fluxes, and from 20 to 70 Wm⁻² for shortwave fluxes.At the top of the atmosphere, the differences between METEOSAT measurements and model are in fair agreement for longwave fluxes (up to 50 Wm⁻²). However, unexpected high differences are found for shortwave fluxes (up to 144 Wm⁻²) due to cirrus clouds heterogeneities and uncertainties in their microphysical properties and especially the occurrence of high reflectivity due to horizontally oriented ice crystals at the cloud top, which are not taken into account by the Model presently.     

气候模式分辨率对气溶胶气候效应模拟结果的影响

气候模式分辨率作为影响模式模拟结果的重要因素,其对气溶胶与云相互作用的影响尚未全面认识。利用公共大气模型CAM5.3在3种分辨率（2°、1°、0.5°）下,分别采用2000年和1850年气溶胶排放情景进行试验,检验提高分辨率是否能改进气候模式的模拟能力,分析不同分辨率下气溶胶气候效应的异同,探索模式分辨率对气溶胶气候效应数值模拟结果的影响。通过观测资料与模式结果对比发现,提高分辨率可以明显改进模式对总云量、云短波辐射强迫的模拟能力,0.5°分辨率下模拟结果与观测更接近,其他变量并无明显改善。在不同分辨率下,全球平均的气溶胶气候效应较为一致,总云量、云水路径均增加,云短波和长波辐射强迫均加强,而云顶的云滴有效半径和降水均减小,地面气温降低。不同分辨率下,气溶胶增加引起的气溶胶光学厚度、云水路径、地面温度、云短波和长波辐射强迫变化的纬向平均分布相似但大小存在差异;而降水和云量变化的纬向分布与大小均存在较大差异,在区域尺度上还存在较大的不确定性。全球平均而言, 0.5°分辨率下气溶胶的间接辐射强迫相比1°分辨率下的结果降低了2.5%,相比2°分辨率下的结果降低了6.4%。提高模式分辨率可以部分改进模式模拟能力,同时,气溶胶的间接效应随着模式分辨率的提高而减弱。但气溶胶引起的云量、降水的变化在不同分辨率下差异较大,存在较大的不确定性。      

Impact of primary ice nucleation parameterizations on the formation and maintenance of cirrus

Different ice nucleation algorithms are implemented in a cloud microphysical scheme and numerical simulations of clouds are performed using a three-dimensional mesoscale model. The predicted ice crystal fields are found to be sensitive to the different modes of calculation of the number of deposition/ condensation freezing nuclei and contact freezing nuclei. Also a time and supercooling dependence of this sensitivity is established.The general features of the cirrus clouds observed by the research aircraft Falcon during the 1989 (International Cirrus Experiment) mission ICE212 are compared to those of the cirrus clouds generated by the model. The cloud top height, the cloud ice content and the ice number concentrations seem to be reproduced well.     

Effects of arctic sulphuric acid aerosols on wintertime low-level atmospheric ice crystals,humidity and temperature at Alert,Nunavut

The effect of pollution-derived sulphuric acid aerosols on wintertime arctic lower atmospheric ice crystals is investigated. These anthropogenic aerosols differ from natural background aerosols by their number concentration, strong solubility and reduced homogeneous freezing temperature when internally mixed with other compounds. Furthermore, observations suggest that the ice-forming nuclei concentration is reduced by one to four orders of magnitude when the sulphuric acid aerosol concentration is high.Simulations performed using a column model and analysis of observed data for the period of 1991–1994 at Alert (82° 30'N, 62°20'W) are used to assess the changes of the boundary layer cloud characteristics by sulphuric acid aerosols and the potential effect on arctic climate. Results show that aerosol acidification leads to depletion of the ice crystal number concentration and an increase of its mean size. As a result, low-level precipitating ice crystals occur more frequently than ice fog and thick nonprecipitating clouds during high concentration of pollution-derived aerosols. This result is in agreement with observations that indicate an increase by more than 50% of the frequency of precipitating ice crystals when the weight proportion of sulphuric acid is greater than its mean value of 20% of the total aerosol mass. Consequently, the ice crystal size increases and number decreases, and the sedimentation flux of ice crystals and the dehydration rate of the lower troposphere are accelerated in the presence of high sulphuric acid aerosol concentration. As a result, the infrared radiation flux reaching the surface and the greenhouse effect are decreased. This process is referred to as the dehydration–greenhouse feedback. One-dimensional simulation for Alert during the period of 1991 to 1994 shows that a negative cloud radiative forcing of −9 W m⁻² may occur locally as a result of the enhanced dehydration rate produced by the aerosol acidity.     

An Algorithm for Detecting Ice Cloud at Different Altitudes by Combining Dual CrIS Full Spectrum Resolution CO2 Channels

Using infrared sensors to detect ice clouds in different atmospheric layers is still a challenge. The different scattering and absorption properties of longwave and shortwave infrared channels can be utilized to fulfill this purpose.In this study, the release of Suomi-NPP Cross-track Infrared Sounder(Cr IS) full spectrum resolution is used to select and pair channels from longwave(～ 15 μm) and shortwave(～4.3 μm) CO_2 absorption bands under stricter conditions, so as to better detect ice clouds. Besides, the differences of the weighting function peaks and cloud insensitive level altitudes of the paired channels are both within 50 h Pa so that the variances due to atmospheric conditions can be minimized. The training data of clear sky are determined by Visible Infrared Imaging Radiometer Suite(VIIRS) cloud mask product and used to find the linear relationship between the paired longwave and shortwave CO_2 absorption channels. From the linear relationship, the so-called cloud emission and scattering index(CESI) is derived to detect ice clouds. CESI clearly captures the center and the ice cloud features of the Super Typhoon Hato located above 415 h Pa. Moreover, the CESI distributions agree with cloud top pressure from the VIIRS in both daytime and nighttime in different atmospheric layers.     

典型站点气溶胶对云特性的影响

结合Cloud Sat对云的主动观测和MODIS(MODerate-Resolution Imaging Spectroradiometer)对气溶胶的被动反演,研究了典型站点气溶胶对云的宏观、微观和辐射特性的影响。结果表明,气溶胶对大陆性和海洋性站点的云均有显著影响。1)随气溶胶光学厚度(Aerosol Optical Depth,AOD)增加,水汽含量较弱站点的低层(高层)云量呈减小(增加)趋势,而水汽条件较强站点的各层云量均增大,且具有较高(较低)云顶的云层发生概率在各个站点都呈增加(减小)趋势。2)AOD的增大导致各站点云滴和冰晶粒子的有效半径均减小、大气层顶的短波和长波云辐射强迫均增强、短波云辐射强迫绝对值的加强更显著、长波云辐射强迫增加的幅度相对更大。3)气象要素在AOD大(小)值情况下的变化表明,大尺度动力条件并不能解释云的上述特性随AOD的显著改变。     

基于CMIP6强迫模拟分析人为气溶胶的气候效应(二)——诊断方法在分类评估中的重要性

对气溶胶气候效应开展分类评估并探讨诊断方法的合理性。人为气溶胶辐射效应对计算云辐射强迫的影响为0.38 W·m~(-2)。诊断评估气溶胶对云辐射强迫的影响需要排除这个偏差。两种基于不同试验设计诊断得出的半直接效应分别为0.21和0.09 W·m~(-2),存在显著差异。主要原因可能是人为气溶胶影响云辐射强迫的不同机制之间在模式模拟过程中不断地相互交织,不是简单的线性叠加关系。模式诊断得出的Twomey效应不仅包括Twomey效应本身,还包括Twomey效应引起的部分快速调整。总之,利用模式评估分析人为气溶胶气候效应需要注意审查试验设计和诊断方法的合理性。     

Data-driven Estimation of Cloud Effects on Surface Irradiance at Xianghe,a Suburban Site on the North China Plain

Clouds are a dominant modulator of the energy budget. The cloud shortwave radiative effect at the surface (CRE) is closely related to the cloud macro- and micro-physical properties. Systematic observation of surface irradiance and cloud properties are needed to narrow uncertainties in CRE. In this study, 1-min irradiance and Total Sky Imager measurements from 2005 to 2009 at Xianghe in North China Plain are used to estimate cloud types, evaluate cloud fraction (CF), and quantify the sensitivities of surface irradiance with respect to changes in CF whether clouds obscure the sun or not. The annual mean CF is 0.50, further noting that CF exhibits a distinct seasonal variation, with a minimum in winter (0.37) and maximum in summer (0.68). Cumulus occurs more frequently in summer (32%), which is close to the sum of the occurrence of stratus and cirrus. The annual CRE is –54.4 W m^–2, with seasonal values ranging from –29.5 W m^–2 in winter and –78.2 W m^–2 in summer. When clouds do not obscure the sun, CF is a dominant factor affecting diffuse irradiance, which in turn affects global irradiance. There is a positive linear relationship between CF and CRE under sun-unobscured conditions, the mean sensitivity of CRE for each CF 0.1 increase is about 1.2 W m^–2 [79.5° < SZA (Solar Zenith Angle) < 80.5°] to 7.0 W m^–2 (29.5° < SZA < 30.5°). When clouds obscure the sun, CF affects both direct and diffuse irradiance, resulting in a non-linear relationship between CF and CRE, and the slope decreases with increasing CF. It should be noted that, although only data at Xianghe is used in this study, our results are representative of neighboring areas, including most parts of the North China Plain.     

基于IASI双二氧化碳通道的一种不同高度云检测算法

利用红外高光谱探测仪（Infrared Atmospheric Sounding Interferometer,IASI）在二氧化碳吸收带的长短波红外通道对云反应程度的不同来探测云。依据不同通道的权重函数峰值高度和云不敏感层高度将IASI长短波红外通道进行配对,成功配对的长短波红外通道晴空亮温之间建立线性回归模型,即通过长波红外通道亮温可以线性回归得到配对的短波通道亮温,将短波通道的晴空回归亮温和观测亮温之差定义为云指数。权重函数峰值高度位于383 hPa的云指数空间分布和云成分为冰的空间分布较为一致,尤其在赤道和低纬度地区。权重函数峰值高度位于790 hPa的云指数空间分布和低云云顶气压也有较好的一致性。     

Impacts of greenhouse gases and aerosol direct and indirect effects on clouds and radiation in atmospheric GCM simulations of the 1930–1989 period

Among anthropogenic perturbations of the Earths atmosphere, greenhouse gases and aerosols are considered to have a major impact on the energy budget through their impact on radiative fluxes. We use three ensembles of simulations with the LMDZ general circulation model to investigate the radiative impacts of five species of greenhouse gases (CO₂, CH₄, N₂O, CFC-11 and CFC-12) and sulfate aerosols for the period 1930–1989. Since our focus is on the atmospheric changes in clouds and radiation from greenhouse gases and aerosols, we prescribed sea-surface temperatures in these simulations. Besides the direct impact on radiation through the greenhouse effect and scattering of sunlight by aerosols, strong radiative impacts of both perturbations through changes in cloudiness are analysed. The increase in greenhouse gas concentration leads to a reduction of clouds at all atmospheric levels, thus decreasing the total greenhouse effect in the longwave spectrum and increasing absorption of solar radiation by reduction of cloud albedo. Increasing anthropogenic aerosol burden results in a decrease in high-level cloud cover through a cooling of the atmosphere, and an increase in the low-level cloud cover through the second aerosol indirect effect. The trend in low-level cloud lifetime due to aerosols is quantified to 0.5 min day^–1 decade^–1 for the simulation period. The different changes in high (decrease) and low-level (increase) cloudiness due to the response of cloud processes to aerosols impact shortwave radiation in a contrariwise manner, and the net effect is slightly positive. The total aerosol effect including the aerosol direct and first indirect effects remains strongly negative.     

Direct Climatic Effect of Dust Aerosol in the NCAR Community Atmosphere Model Version 3 （CAM3）

Direct climate responses to dust shortwave and longwave radiative forcing (RF) are studied using the NCAR Community Atmosphere Model Version 3 (CAM3). The simulated RF at the top of the atmosphere (TOA) is-0.45 W m-2 in the solar spectrum and +0.09 W m-2 in the thermal spectrum on a global average. The magnitude of surface RF is larger than the TOA forcing, with global mean shortwave forcing of-1.76 W m-2 and longwave forcing of +0.31 W m-2 . As a result, dust aerosol causes the absorption of 1.1 W m-2 in t...     

Radiative energy partition and cloud radiative forcing at a Po valley site

Values of downward and upward flux densities of solar and terrestrial radiation were continuously recorded between 1 December 2001 and 30 November 2002 using a four-components radiometer at S. Pietro Capofiume (SPC) in northern Italy (44°39′N, 11°37′E, alt. 11 m a.m.s.l.), which is characterized by a weakly-reflective surface. The aim of the study was to investigate the effects of clouds on surface radiation balance (SRB); the cloud fraction (N) has been retrieved through the inverted form of the parameterization proposed by Kasten and Czeplak [Solar Energy 24 (1980) 177] and cloud types estimated following the methodology of Duchon and O'Malley [J. Appl. Meteorol. 38 (1999) 132]. The cloud radiative forcing (CRF) was evaluated through the Bintanja and Van den Broeke [Int. J. Climatol. 16 (1996) 1281] formula and then associated with cloud type. Experimental results showed that during the measuring period the net shortwave (Sw) balance always decreased with increasing N, whereas the net longwave (Lw) balance increased in all seasons. The net radiation available at the surface decreased with increasing N in all seasons except in winter, where no significant dependency was detected.The analysis of the cloud radiative forcing indicates that all seasons were characterized by a net cooling of the surface except winter, where clouds seem to have no effects on the surface warming or cooling. Taking into account the dependence on solar radiation cycle, an intercomparison between the retrieved cloud types seems to indicate that the effect of stratus was a slight cooling whereas that of cumulus clouds was a stronger cooling of the surface. On the contrary, cirrus clouds seem to have slight warming effect on the surface.The annual trends of mean monthly values of shortwave and longwave radiation balances confirmed that the measurement site is characterized by a temperate climate. Moreover, in spite of the cooling effect of clouds, a monthly radiative energy surplus is available all year long for surface–atmosphere energy exchanges. The analysis is also instrumental for the detection of SRB variations.     

The Arctic surface energy budget as simulated with the IPCC AR4 AOGCMs

Ensembles of simulations of the twentieth- and twentyfirst-century climate, performed with 20 coupled models for the Intergovernmental Panel on Climate Change (IPCC) Fourth Assessment, provide the basis for an evaluation of the Arctic (70°–90°N) surface energy budget. While the various observational sources used for validation contain differences among themselves, some model biases and across-model differences emerge. For all energy budget components in the twentieth-century simulations (the 20C3M simulation), the across-model variance and the differences from observational estimates are largest in the marginal ice zone (Barents, Kara, Chukchi Seas). Both downward and upward longwave radiation at the surface are underestimated in winter by many models, and the ensenmble mean annual net surface energy loss by longwave radiation is 35 W/m², which is less than for the NCEP and ERA40 reanalyses but in line with some of the satellite estimates. Incoming solar radiation is overestimated by the models in spring and underestimated in summer and autumn. The ensemble mean annual net surface energy gain by shortwave radiation is 39 W/m², which is slightly less than for the observational based estimates, In the twentyfirst-century simulations driven by the SRES A2 scenario, increased concentrations of greenhouse gasses increase (average for 2080–2100 minus average for 1980–2000 averages) the annual average ensemble mean downward longwave radiation by 30.1 W/m². This was partly counteracted by a 10.7 W/m² reduction in downward shortwave radiation. Enhanced sea ice melt and increased surface temperatures increase the annual surface upward longwave radiation by 27.1 W/m² and reduce the upward shortwave radiation by 13.2 W/m², giving an annual net (shortwave plus longwave) surface radiation increase of 5.8 W/m² , with the maximum changes in summer. The increase in net surface radiation is largely offset by an increased energy loss of 4.4 W/m² by the turbulent fluxes.     

Vertical Structures of Convective and Stratiform Clouds in Boreal Summer over the Tibetan Plateau and Its Neighboring Regions

Cloud is essential in the atmosphere, condensing water vapor and generating strong convective or large-scale persistent precipitation. In this work, the relationships between cloud vertical macro- or microphysical properties, radiative heating rate, and precipitation for convective and stratiform clouds in boreal summer over the Tibetan Plateau (TP) are analyzed and compared with its neighboring land and tropical oceans based on CloudSat/CALIPSO satellite measurements and TRMM precipitation data. The precipitation intensity caused by convective clouds is twofold stronger than that by stratiform clouds. The vertical macrophysics of both cloud types show similar features over the TP, with the region weakening the precipitation intensity and compressing the cloud vertical expansion and variation in cloud top height, but having an uplift effect on the average cloud top height. The vertical microphysics of both cloud types under conditions of no rain over the TP are characterized by lower-level ice water, ice particles with a relatively larger range of sizes, and a relatively lower occurrence of denser ice particles. The features are similar to other regions when precipitation enhances, but convective clouds gather denser and larger ice particles than stratiform clouds over the TP. The atmospheric shortwave (longwave) heating (cooling) rate strengthens with increased precipitation for both cloud types. The longwave cooling layer is thicker when the rainfall rate is less than 100 mm d^?1, but the net heating layer is typically compressed for the profiles of both cloud types over the TP. This study provides insights into the associations between clouds and precipitation, and an observational basis for improving the simulation of convective and stratiform clouds over the TP in climate models.     

The representation of tropical upper tropospheric water in EC Earth V2

Tropical upper tropospheric humidity, clouds, and ice water content, as well as outgoing longwave radiation (OLR), are evaluated in the climate model EC Earth with the aid of satellite retrievals. The Atmospheric Infrared Sounder and Microwave Limb Sounder together provide good coverage of relative humidity. EC Earth’s relative humidity is in fair agreement with these observations. CloudSat and CALIPSO data are combined to provide cloud fractions estimates throughout the altitude region considered (500–100?hPa). EC Earth is found to overestimate the degree of cloud cover above 200?hPa and underestimate it below. Precipitating and non-precipitating EC Earth ice definitions are combined to form a complete ice water content. EC Earth’s ice water content is below the uncertainty range of CloudSat above 250?hPa, but can be twice as high as CloudSat’s estimate in the melting layer. CERES data show that the model underestimates the impact of clouds on OLR, on average with about 9?W?m^?2. Regionally, EC Earth’s outgoing longwave radiation can be ～20?W?m^?2 higher than the observation. A comparison to ERA-Interim provides further perspectives on the model’s performance. Limitations of the satellite observations are emphasised and their uncertainties are, throughout, considered in the analysis. Evaluating multiple model variables in parallel is a more ambitious approach than is customary.     

Elicitation of Expert Judgments of Aerosol Forcing

A group of twenty-four leading atmospheric and climate scientists provided subjective probability distributions that represent their current judgment about the value of planetary average direct and indirect radiative forcing from anthropogenic aerosols at the top of the atmosphere. Separate estimates were obtained for the direct aerosol effect, the semi-direct aerosol effect, cloud brightness (first aerosol indirect effect), and cloud lifetime/distribution (second aerosol indirect effect). Estimates were also obtained for total planetary average forcing at the top of the atmosphere and for surface forcing. Consensus was strongest among the experts in their assessments of the direct aerosol effect and the cloud brightness indirect effect. Forcing from the semi-direct effect was thought to be small (absolute values of all but one of the experts' best estimates were ≤0.5 W/m²). There was not agreement about the sign of the best estimate of the semi-direct effect, and the uncertainty ranges some experts gave for this effect did not overlap those given by others. All best estimates of total aerosol forcing were negative, with values ranging between −0.25 W/m² and −2.1 W/m². The range of uncertainty that a number of experts associated with their estimates, especially those for total aerosol forcing and for surface forcing, was often much larger than that suggested in 2001 by the IPCC Working Group 1 summary figure (IPCC, 2001).