区域酸性沉降的数值研究 II. 个例模拟和试验

利用建立的区域酸性污染物沉降模式，配合中尺度模式MM4预报的气象场，以1991年6月12～14日淮河流域的一次降雨过程作为实例，对我国东半部及其相邻地区的酸沉降进行了数值模拟和试验研究。结果表明，模式基本上能够模拟出区域酸性沉降的特征，具有良好的综合模拟性能和广阔的应用前景。     

中国西南和华南地区硫沉降数值模拟

利用CMAQ(Community Multi-scale Air Quality)模式模拟了中国西南和华南地区的硫沉降。模式中详细考虑了气象过程、气相与液相化学过程、非均相化学过程、气溶胶过程和干湿沉降过程对SO2输送、转化和沉降过程的影响。通过与IMPACTS小流域的观测资料的比较,显示了该模式系统能够较好地模拟SO2在大气中的转化以及干湿沉降过程。在此基础之上,分析了不同季节该区域的硫沉降和向外输送的情况,并且模拟了该区域2002年全年的硫沉降分布状况,这为该区域有效地污染治理奠定了基础。     

区域酸性沉降的数值研究 I. 模式

建立了一个三维时变的欧拉型区域酸性污染物沉降模式，模式包括源排放、平流输送、湍流扩散、干沉积、气相化学、液相化学及湿清除等六大部分。考虑到计算条件的承受能力和应用性的要求，在把握酸沉降形成的关键过程的前提下，合理地简化设计模式。相对于国内已有的工作，本模式在干沉积、气相化学、液相化学和湿清除等方面均有所改进。     

区域模式和GCM对青藏高原和西北地区气候模拟结果的对比分析

使用一个区域模式与大气环流模式（ＧＣＭ）嵌套,模拟了我国西北及青藏高原地区夏季气候的平均状态。将区域模式与ＧＣＭ嵌套的模拟结果和ＧＣＭ单独使用时的模拟结果与观测场进行了对比分析和相关分析。结果表明：ＧＣＭ模式拟出了我国西北和青藏高原地区夏季大尺度气候的基本特征,对降水的模拟也基本合理,但无法分辨出较小系统。区域模式与ＧＣＭ嵌套拟结果有明显改善,它可成功地再现西北及青藏高原地区夏季的区域气候特征（包     

地气相互作用的自适应多级模拟

自适应多级模拟（ＡＭＭ）方法能将大气模式和陆面水文模式安全耦合，并保持其大尺度（大气）分量和区域（陆地）分量间的一致性，用这个方法研究了三个个例。     

初始条件和边界条件对区域模式模拟青藏高原区域气候的影响

用ＧＦＤＬ气候场及ＧＣＭ的模拟结果分别为区域模式（ＭＭ４）提供初始条件和边界条件,模拟了青藏高原地区夏季区域气候特征,通过比较不同初始条件和边界条件时区域模式的模拟结果,分析了初始条件和边界条件对模拟结果的影响,虽然这两种方法都模拟出青藏高原附近的主要区域气候特征,但ＧＦＤＬ提供初始条件和边界条件对ＭＭ４的模拟结果明显优于用ＧＣＭ提供初始条件和边界条件时的模拟结果,特别是高层,ＧＣＭ输出结果与实际     

黑风暴的沙尘形成与输送参数化及中尺度数值试验

西北地区典型黑风暴和强沙尘暴都是在特定大尺度环流背景和中尺度系统相互作用下发生和发展的，而中、低空强锋区相伴的强冷锋移经沙源充足的大沙漠区是黑风暴和强沙尘暴形成和发展的必要条件。为了研究黑风暴和沙尘暴的沙尘形成、输送及沉降机制，本文提出了一种沙尘源、汇项的参数化方案和一个沙尘输送方程，进而引入已有的ＭＭ４中尺度数值模式模拟系统；应用这个改进和发展的模式模拟系统基本成功地模拟了“９３．５”黑风暴的天气系统演变及其沙尘浓度的近地层和垂直分布以及沙尘的沉降与输送。模拟结果分析表明，用包括沙尘输送方程及其沙尘源、汇项参数化方案的中尺度数值模式来研究黑风暴的沙尘形成、输送和沉降机制是一种具有应用前景的方法。     

有限区域卫星云图资料变分分析的试验研究

资料分析在数值预报中的重要性受到越来越多的关注，星目前常规探测网的时空局限性，利用分辨率较高的非常规资料势在必行。该文利用一个有限区域中尺度模式ＭＭ４，采用变分分析技术对有限区域的常规探空资料和非常规云图资料进行变分分析和数值模拟。     

我国燃煤汞沉降的数值模拟

利用CMAQ-Hg(Community Multi-scale Air Quality-Mercury)模式模拟了我国燃煤排放的大气汞在我国区域的沉降分布状况,其中气象模式为MM5.模式中包括了三种价态汞(气态元素汞(GEM)、气态活性汞(RGM)和颗粒汞(PHg))的气相、液相、非均相化学反应过程以及输送、干湿沉降等物理过程.中国燃煤排放的大气汞中RGM所占比例较高,约为58.4%～66.8%,这导致我国汞沉降量较大.模拟结果表明,在我国的西南地区、华东地区以及京津塘地区燃煤汞的沉降较高,在这些区域的沉降通量高达2～6μg m-2mon-1.燃煤大气汞排放形态对汞的沉降有重要影响,减少燃煤汞排放中RGM的比例能够显著降低我国区域汞的沉降通量.     

东亚酸沉降模式不确定性分析

酸沉降会对生态环境造成危害。要控制和减少酸沉降,就要了解酸沉降的幅度和不确定性,而模式研究是获得这些因子的重要工具。用东亚酸沉降模式比较计划（MICS-AsiaⅡ）中7个模式模拟的2001年7月和12月东亚地区酸沉降数据及东亚酸沉降监测网络（EANET）的观测数据,通过相关分析发现多模式模拟的平均值可表现东亚地区酸沉降的分布特征。采用各个模式与模拟结果平均值的离散程度来表征这些模式在东亚地区的不确定性,简要分析了目前模式模拟东亚酸沉降的不确定及其产生原因,可为制定酸沉降的控制措施提供依据。     

中层大气行星波在臭氧的季节和年际变化中输运作用的数值研究──Ⅰ．常定流的情况

本文构造了一个３４层球坐标原始方程波－流相互耦合谱模式，利用此模式从拉格朗日平均环流的观点研究了在常定流下行星波对臭氧的输运作用。研究结果表明，行星波对臭氧的输运有明显的季节变化，在北半球冬季，由于行星波上传到平流层而大大增强了中高纬地区向极地向下的Ｏ３输运；并且还表明，热带纬向风的ＱＢＯ不仅通过影响东、西风切变而引起热带Ｏ３分布的年际变化，而且通过影响行星波的传播引起了行星波对Ｏ３输运的年际变化，这表现为当热带纬向风处于东风位相时，中高纬地区行星波对Ｏ３的输运比西风位相时强。     

准定常行星被对大气中臭氧输运的动力作用

本文从拉格朗日平均环流观点讨论了行星波对大气中Ｏ３。的输运作用。理论分析表明，当行星波是定常保守时，行星波对大气中Ｏ３没有输运作用；而非定常的行星被对大气中ｏ。有明显的输运作用，它可以强迫出一个正的输运环流、即从热带上升，而从高纬下沉的环流；此外，只有当耗散的行星波传播到平流层才会在平流层强迫出输运环流。为了说明行星波对大气中Ｏ３输运的动力作用，本文还利用一组３４层波－流相互耦合球坐标原始方程谱模式计算了地球大气中行星波对Ｏ３变化的作用，其计算的Ｏ３变化与实际观测到的Ｏ３分布变化很相似。     

北半球冬季行星波的传播及其输运作用

利用变换欧拉平均方程讨论了行星波动力学。观测和模拟结果都表明,在北半球冬季准定常行星波的经向传播存在两支波导。一支为高纬度波导,另一支则为低纬度波导。这些结果与理论分析相当一致。通过对EP通量进一步的研究表明,平流层爆发性增温是沿高纬度波导传播的异常行星波与平均气流相互作用的结果。而热带风场的准两年周期振荡（QBO）是低纬度平流层下层大气纬向平均流的一个重要年际变化,它可以影响行星波沿低纬度波导的传播;此外,由一个行星波一平均流耦合模式模拟的结果表明,这个热带风场的变化还可以通过波流相互作用调制行星波沿高纬度波导的传播。 行星波对臭氧的输运作用在文中也进行了分析。行星波强迫出的剩余平均环流表明,耗散的行星波有强的输运作用;向北的涡动热量输送可以强迫出一个正的输运环流,其在低纬度上升并在高纬度下沉。同时研究还表明,热带风场的QBO对行星波传播的调制对输运环流也有重要影响,模式结果表明,在QBO的东风位相期间行星波引起的输运作用明显增强,其结果可用于解释平流层高纬度臭氧的年际变化。     

西太平洋地区大气边界层内臭氧的季节变化及其影响因子分析

利用臭氧探空资料,分析了西太平洋地区香港(Hong Kong)、那霸(Naha)和札幌(Sapporo)三个站点2000~2010年期间大气边界层内臭氧(O₃)的季节分布和年变化趋势。结果表明,三个站点O₃的季节分布存在明显的差异。其中,那霸和香港大气边界层内O₃季节平均呈双峰值分布,其峰值分别出现在春季和秋季;而札幌站为单峰分布,峰值出现在春季。造成季节分布差异的主要原因包括人为污染源和自然因素如气象条件。另外,三个站点大气边界层内O₃均呈上升趋势。其中札幌、那霸上升最快,分别达0.80 ppb a-1和0.77 ppb a-1。(ppb表示10-9,下同)香港的年际增长较不明显,但秋季增长却非常明显,高达1.21 ppb a-1。结合GOME (Global Ozone Monitoring Experiment) 和SCIAMACHY (Scanning Imaging Absorption Spectro Meter for Atmospheric Chartography)卫星反演的NO₂数据发现,过去10年中国京津唐和东北地区的对流层内NO₂柱总量增加极为迅速。这些O₃前体物通过远距离输送是导致札幌、那霸O₃浓度增加的主要原因之一。珠江三角洲人为污染源的增加及偏北气流的影响,是导致香港地区秋季O₃增加的主要原因。     

On the Importance of Reliable Background Concentrations of Ozone for Regional Scale Photochemical Modelling

Ozone throughout the troposphere is subject of significant temporal and spatial variability due to photochemical production in the planetary boundary layer and free troposphere, stratospheric intrusions, convective events and long range transport. However, high resolving observations of ozone in the troposphere are generally rare today. That is of special disadvantage for limited area models, which represent mathematically a differential equation system with an initial and boundary problem. As ozone concentrations usually increase from the earth surface to the stratosphere, a proper choice of the background ozone concentrations is necessary to reproduce or even predict the amount and distribution of ozone in a specific region of interest.In this paper the impact of background concentrations of ozone on regional scale model results is analysed during a summer smog episode over Europe. For this purpose ozone is artificially partitioned into individual categories. For each category, transport and chemical transformation is calculated separately. Initial and boundary concentrations of ozone dominate total ozone concentrations increasingly with height. But also in the planetary boundary layer they contribute with more than 30% to thetotal ozone changes and are therefore far from being negligible. Moderately modified assumptions of background ozone concentrations reveal an uncertainty of near surface ozone concentrations of 5–15%depending on the weather situation.     

Involvement of the Brewer–Dobson circulation in changes of stratospheric temperature and ozone

Wintertime temperature and ozone in the Northern Hemisphere stratosphere vary significantly between years. Largely random, those variations are marked by compensating changes at high and low latitudes, a feature that reflects the residual mean circulation of the stratosphere. Interannual changes of temperature and ozone each track anomalous forcing of the residual circulation. This relationship is shown to be obeyed even over the Arctic, where transport is augmented by heterogeneous chemical processes that destroy ozone. Chlorine activation obeys a similar relationship, reflecting feedback between changes of the residual circulation and anomalous photochemistry.Changes of stratospheric dynamical and chemical structure are found be accompanied by coherent changes in the troposphere. Vertically extensive, they reflect inter-dependent changes in the stratosphere and troposphere, which are coupled by the residual circulation through transfers of mass. The corresponding structure is shown to share major features with empirical modes of interannual variability associated with the AO and its cousin, the NAO.A 3D model of dynamics and photochemistry is used to simulate anomalous temperature and ozone. Driven by anomalous wave activity representative of that observed, the model reproduces the salient structure of observed interannual changes. Anomalous temperature and ozone follow in the integrations from anomalous downwelling, which, under disturbed conditions, renders temperature over the Arctic anomalously warm, and from anomalous poleward transport, which renders Arctic ozone anomalously rich.Accompanying random interannual changes in the observed record was a systematic decline of Northern Hemisphere temperature and ozone during the 1980s and early 1990s. Comprising decadal trends, these systematic changes are shown to have the same essential structure and seasonality as random changes, which, in turn, vary coherently with anomalous forcing of the residual circulation. Implications of the findings to the interpretation of stratospheric trends are discussed in light of anomalous residual motion, photochemistry, and feedback between them.     

Influence of Vertical Eddy Diffusivity Parameterization on Daily and Monthly Mean Concentrations of O3 and NOy

Two parameterization schemes for vertical eddy diffusivity were utilized to investigate their impacts on both the daily and monthly mean concentrations of ozone and NOy, which are the major fractions of the sum of all reactive nitrogen species, i.e., NOy=NO＋NO2＋HNO3＋PAN. Simulations indicate that great changes in the vertical diffusivity usually occur within the planetary boundary layer （PBL）. Daily and monthly mean concentrations of NOy are much more sensitive to changes in the vertical diffusivity than those of ozone and ozone and NOy levels only at or in （relatively） clean sites and areas, where long-range transport plays a crucial role, display roughly equivalent sensitivity. The results strongly suggest that a widely-accepted parameterization scheme be selected and the refinement of the model＇s vertical resolution in the PBL be required, even for regional and long-term studies, and ozone only being examined in an effort to judge the model＇s performance be unreliable, and NOy be included for model evaluations.     

Finite-amplitude, neutral baroclinic eddies and mean flows in an internally heated rotating fluid: 1. Numerical simulations and quasi-geostrophic ‘free modes’

A series of numerical simulations of steady wave flows in a rotating fluid annulus, subject to internal heating and various thermal boundary conditions, is examined to characterise their structures, energetics and potential vorticity transport properties. The last of these characteristics, together with more conventional scaling considerations, indicate the possibility of applying quasi-geostrophic theory to the interior flow in a formulation similar to the inviscid, adiabatic models of Kuo and White.The analytical model of White, describing finite amplitude, neutral baroclinic eddies and mean flows as illustrations of the Charney-Drazin non-acceleration theorem, is then extended to include uniform diabatic heating and the effects of different forms of lateral shear in the background mean zonal flow. Like the solutions discussed by White, those obtained in the present paper consist of steady, internal jet, mean zonal flows, and baroclinic and barotropic Rossby wave components, all having the same three-dimensional wavenumber. Provided the diabatic heating is proportional to the stratification of the background flow, measured by the square of the Brunt-Vaisälä frequency N, the potential vorticity equation remains homogeneous. All the solutions are then characterised by zero net transfer of potential vorticity despite the possibility of non-zero eddy fluxes of heat or momentum and non-trivial Lorenz energy cycles.A series of particular three-component solutions (which, like some of the solutions discussed by White, do not obey conventional lateral boundary conditions) is examined as possible theoretical analogues of the steady waves observed in the numerical simulations of the laboratory flows, and is found to agree encouragingly well in the spatial variations of their mean flows, eddy stream function (pressure) and eddy fluxes of heat and momentum. Potential vorticity fluxes in the numerical simulations are relatively small (though crucially non-zero), supporting the possible analogy with the analytical model and exposing some limitations of the latter in not accounting for weak dissipation and forcing processes present in the laboratory flows.Further implications of the results are discussed, including possible analogies between the laboratory experiments and certain features in planetary atmospheres and oceans.     

对流层气溶胶的直接气候效应对平流层的影响

通过WACCM-3模式中气溶胶光学厚度与卫星资料的对比发现,模式可以很好地再现全球气溶胶的主要分布特征,但在一些区域还存在数值上的差异。利用数值试验研究对流层气溶胶的直接气候效应对平流层气候的影响,结果表明:对流层气溶胶对平流层气候有明显影响,平流层化学过程在这一影响中起重要作用,而对流层气溶胶对平流层辐射的影响不是其直接气候效应对平流层影响的主要原因。其机制可能是对流层气溶胶改变对流层的辐射平衡,影响对流层的温度和大气环流,进而影响行星波的上传,使得平流层气候发生变化;影响区域主要位于高纬度和极地地区,南半球的变化比北半球大,温度变化最大达10 K,纬向风变化最大可达12 m/s,臭氧体积分数最多减少0.8×10-6。     

Effect of basic state on seasonal variation of convectively coupled Rossby wave

Convectively coupled equatorial Rossby (ER) waves display maximum varability over the northern hemisphere during boreal summer and over the southern hemisphere during boreal winter. It suggests that the seasonal variation of ER waves is significantly affected by the annual cycle of basic state. However, which specific environmental factor plays a determining role remains obscure. This study investigates the background influence on the seasonal variation of ER wave by employing an intermediate anomaly atmospheric model. By prescribing boreal summer/winter seasonal mean state as the model’s basic state, the authors found that the model is able to simulate the trapping of the ER wave purtrubation over the northern/southern hemisphere as in observation. Further sensitivity experiments suggest that the moisture distribution plays a major role in modulating the ER wave structure while the mosoonal flows play a minor role.