A Review of Research on Human Activity Induced Climate ChangeⅠ. Greenhouse Gases and Aerosols

Extensive research on the sources and sinks of greenhouse gases, carbon cycle modeling, and the characterization of atmospheric aerosols has been carried out in China during the last 10 years or so. This paper presents the major achievements in the fields of emissions of greenhouse gases from agricultural lands, carbon cycle modeling, the characterization of Asian mineral dust, source identification of the precursors of the tropospheric ozone, and observations of the concentrations of atmospheric organic compounds. Special, more detailed Information on the emissions of methane from rice fields and the physical and chemical characteristics of mineral aerosols are presented.     

人类活动对气候影响的研究Ⅰ.温室气体和气溶胶

近5年来中国在温室气体源和汇,碳循环,气溶胶以及对流层臭氧等方面都进行了大量的研究.作者着重介绍农田温室气体排放,碳循环模式,亚洲沙尘气溶胶,对流层臭氧前体物的来源以及大气有机化合物的浓度观测等方面的主要研究成果,特别是关于稻田甲烷排放和沙尘气溶胶的物理化学特性方面的研究成果.     

温室气体和硫酸盐气溶胶的辐射强迫作用

对GOALS4 .0海 陆 气耦合模式的相关部分进行了改进 ,主要改进包括温室气体的扩充和硫酸盐气溶胶“显式”方案的引入 ,并引入 2 0世纪温室气体的实际浓度变化以及硫循环模式模拟的硫酸盐气溶胶的三维全球浓度分布 ,模拟了温室气体和硫酸盐气溶胶造成的辐射强迫的空间分布和时间变化。全球平均的温室气体和硫酸盐气溶胶的辐射强迫分别为 2 .17W /m2 和 - 0 .2 9W /m2 ;温室气体造成的辐射强迫在空间上呈现明显的纬向结构 ,最大值 (大于 2 .5W/m2 )和最小值 (小于 1W /m2 )分别位于副热带和两极地区 ,在北半球主要工业区硫酸盐气溶胶的辐射强迫绝对值接近温室气体的辐射强迫值 (大于 - 2 .0W /m2 )。     

Principles of monitoring of anthropogenic greenhouse gas emissions and sinks

Principles and substantiation of a system of monitoring anthropogenic greenhouse gas emissions and sinks are considered. The basic task of the system is to estimate the anthropogenic contribution to the atmospheric greenhouse gas concentrations and possible climate effect. The major attention is paid to the system of indirect or “computational” monitoring of anthropogenic greenhouse gases. A multifunctional information system is described in the context of its application for solving a number of other ecological problems. It can be used as an instrumental basis for estimating ecological efficiency of measures aimed at reducing emissions and increasing greenhouse gas uptake. The effect should be considered in totality for all greenhouse gases and most hazardous pollutants. Monitoring of anthropogenic greenhouse gas emissions and sinks includes observations (using modeling) of integral indicators of ecosystems and can be used as part of ecological monitoring (for example, dynamics of soil carbon balance of agroecosystems and forest cenoses). The connection of the monitoring of anthropogenic greenhouse gas emissions and sinks with the satellite monitoring enlarges the possible applications of this information system.     

Impact of carbonaceous aerosol emissions on regional climate change

The past and future evolution of atmospheric composition and climate has been simulated with a version of the Max Planck Institute Earth System Model (MPI-ESM). The system consists of the atmosphere, including a detailed representation of tropospheric aerosols, the land surface, and the ocean, including a model of the marine biogeochemistry which interacts with the atmosphere via the dust and sulfur cycles. In addition to the prescribed concentrations of carbon dioxide, ozone and other greenhouse gases, the model is driven by natural forcings (solar irradiance and volcanic aerosol), and by emissions of mineral dust, sea salt, sulfur, black carbon (BC) and particulate organic matter (POM). Transient climate simulations were performed for the twentieth century and extended into the twenty-first century, according to SRES scenario A1B, with two different assumptions on future emissions of carbonaceous aerosols (BC, POM). In the first experiment, BC and POM emissions decrease over Europe and China but increase at lower latitudes (central and South America, Africa, Middle East, India, Southeast Asia). In the second experiment, the BC and POM emissions are frozen at their levels of year 2000. According to these experiments the impact of projected changes in carbonaceaous aerosols on the global mean temperature is negligible, but significant changes are found at low latitudes. This includes a cooling of the surface, enhanced precipitation and runoff, and a wetter surface. These regional changes in surface climate are caused primarily by the atmospheric absorption of sunlight by increasing BC levels and, subsequently, by thermally driven circulations which favour the transport of moisture from the adjacent oceans. The vertical redistribution of solar energy is particularly large during the dry season in central Africa when the anomalous atmospheric heating of up to 60 W m⁻² and a corresponding decrease in surface solar radiation leads to a marked surface cooling, reduced evaporation and a higher level of soil moisture, which persists throughout the year and contributes to the enhancement of precipitation during the wet season.     

可持续发展背景下的黑碳减排

 黑碳气溶胶是环境大气中浓度较低的一种气溶胶粒子组分,因其对光的吸收作用,及其对空气质量和人体健康的影响,而成为当前国际气候变化和环境研究中关注的热点问题之一。本文围绕黑碳的减排问题,介绍黑碳的来源、全球分布,讨论全球温室气体减排和区域空气质量控制对黑碳减排的影响,综述控制和改善燃烧条件、减少开放式生物质燃烧和黑碳封存等减排黑碳的措施。文章还分析了黑碳未能成为全球减排共识的原因,并对中国有关黑碳减排的政策选择提出了建议。     

Warming of an elevated layer over Africa

This paper analyzes trends of temperatures over Africa and seeks to quantify the most significant processes. Observations of air temperature reveal significant warming trends in the 925–600 hPa layer over tropical west Africa and the east Atlantic. This is related to the influence of desert dust and biomass burning emissions on the atmospheric energy budget. We calculate a net radiative absorption of ～??20 W m^???2. The southern (northern) plume is rich in short-lived greenhouse gases (dust aerosols), and the atmospheric response, according to a simplified radiative transfer model, is a >3°C heating of the 2–4 km layer. The observed pattern of warming coincides with a mixture of dust, black carbon and short-lived greenhouse gases in space, time and height. Physical forcing provides a secondary source of regional warming, with sinking motions over the Sahel. The elevated warm layer stabilizes the lower atmosphere over and west of Africa, so drying trends may be anticipated.     

Non-Kyoto radiative forcing in long-run greenhouse gas emissions and climate change scenarios

Climate policies must consider radiative forcing from Kyoto greenhouse gases, as well as other forcing constituents, such as aerosols and tropospheric ozone that result from air pollutants. Non-Kyoto forcing constituents contribute negative, as well as positive forcing, and overall increases in total forcing result in increases in global average temperature. Non-Kyoto forcing modeling is a relatively new component of climate management scenarios. This paper describes and assesses current non-Kyoto radiative forcing modeling within five integrated assessment models. The study finds negative forcing from aerosols masking (offsetting) approximately 25 % of positive forcing in the near-term in reference non-climate policy projections. However, masking is projected to decline rapidly to 5–10 % by 2100 with increasing Kyoto emissions and assumed reductions in air pollution—with the later declining to as much as 50 % and 80 % below today’s levels by 2050 and 2100 respectively. Together they imply declining importance of non-Kyoto forcing over time. There are however significant uncertainties and large differences across models in projected non-Kyoto emissions and forcing. A look into the modeling reveals differences in base conditions, relationships between Kyoto and non-Kyoto emissions, pollution control assumptions, and other fundamental modeling. In addition, under climate policy scenarios, we find air pollution and resulting non-Kyoto forcing reduced to levels below those produced by air pollution policies alone—e.g., China sulfur emissions fall an additional 45–85 % by 2050. None of the models actively manage non-Kyoto forcing for climate implications. Nonetheless, non-Kyoto forcing may be influencing mitigation results, including allowable carbon dioxide emissions, and further evaluation is merited.     

A coupled model study on the intensification of the Asian summer monsoon in IPCC SRES Scenarios

The Asian summer monsoon is an important part of the climate system. Investigating the response of the Asian summer monsoon to changing concentrations of greenhouse gases and aerosols will be meaningful to understand and predict climate variability and climate change not only in Asia but also globally. In order to diagnose the impacts of future anthropogenic emissions on monsoon climates, a coupled general circulation model of the atmosphere and the ocean has been used at the Max-Planck-Institute for Meteorology. In addition to carbon dioxide, the major well mixed greenhouse gases such as methane, nitrous oxide, several chlorofluorocarbons, and CFC substitute gases are prescribed as a function of time. The sulfur cycle is simulated interactively, and both the direct aerosol effect and the indirect cloud albedo effect are considered. Furthermore, changes in tropospheric ozone have been pre-calculated with a chemical transport model and prescribed as a function of time and space in the climate simulations. Concentrations of greenhouse gases and anthropogenic emissions of sulfur dioxide are prescribed according to observations （1860-1990） and projected into the future （1990-2100） according to the Scenarios A2 and B2 in Special Report on Emissions Scenarios （SRES, Nakcenovic et al., 2000） developed by the Intergovernmental Panel on Climate Change （IPCC）. It is found that the Indian summer monsoon is enhanced in the scenarios in terms of both mean precipitation and interannual variability. An increase in precipitation is simulated for northern China but a decrease for the southern part. Furthermore, the simulated future increase in monsoon variability seems to be linked to enhanced ENSO variability towards the end of the scenario integrations.     

Greenhouse-gas versus aerosol forcing and African climate response

There are many indicators that human activity may change climate conditions all around the globe through emissions of greenhouse gases. In addition, aerosol particles are emitted from various natural and anthropogenic sources. One important source of aerosols arises from biomass burning, particularly in low latitudes where shifting cultivation and land degradation lead to enhanced aerosol burden. In this study the counteracting effects of greenhouse gases and aerosols on African climate are compared using climate model experiments with fully interactive aerosols from different sources. The consideration of aerosol emissions induces a remarkable decrease in short-wave solar irradiation near the surface, especially in winter and autumn in tropical West Africa and the Congo Basin where biomass burning is mainly prevailing. This directly leads to a modification of the surface energy budget with reduced sensible heat fluxes. As a consequence, temperature decreases, compensating the strong warming signal due to enhanced trace gas concentrations. While precipitation in tropical Africa is less sensitive to the greenhouse warming, it tends to decrease, if the effect of aerosols from biomass burning is taken into account. This is partly due to the local impact of enhanced aerosol burden and partly to modifications of the large-scale monsoon circulation in the lower troposphere, usually lagging behind the season with maximum aerosol emissions. In the model equilibrium experiments, the greenhouse gas impact on temperature stands out from internal variability at various time scales from daily to decadaland the same holds for precipitation under the additional aerosol forcing. Greenhouse gases and aerosols exhibit an opposite effect on daily temperature extremes, resulting in an compensation of the individual responses under the combined forcing. In terms of precipitation, daily extreme events tend to be reduced under aerosol forcing, particularly over the tropical Atlantic and the Congo basin. These results suggest that the simulation of the multiple aerosol effects from anthropogenic sources represents an important factor in tropical climate change, hence, requiring more attention in climate modelling attempts.     

Modeling Methane Emissions from Paddy Rice Fields under Elevated Atmospheric Carbon Dioxide Conditions

Methane(CH4 ) emissions from paddy rice fields substantially contribute to the dramatic increase of this greenhouse gas in the atmosphere.Due to great concern about climate change,it is necessary to predict the effects of the dramatic increase in atmospheric carbon dioxide(CO2 ) on CH4 emissions from paddy rice fields.CH4MOD 1.0 is the most widely validated model for simulating CH4 emissions from paddy rice fields exposed to ambient CO2(hereinafter referred to as aCO2 ).We upgraded the model to CH4MOD 2.0 b...     

Impacts of greenhouse gases and aerosol direct and indirect effects on clouds and radiation in atmospheric GCM simulations of the 1930–1989 period

Among anthropogenic perturbations of the Earths atmosphere, greenhouse gases and aerosols are considered to have a major impact on the energy budget through their impact on radiative fluxes. We use three ensembles of simulations with the LMDZ general circulation model to investigate the radiative impacts of five species of greenhouse gases (CO₂, CH₄, N₂O, CFC-11 and CFC-12) and sulfate aerosols for the period 1930–1989. Since our focus is on the atmospheric changes in clouds and radiation from greenhouse gases and aerosols, we prescribed sea-surface temperatures in these simulations. Besides the direct impact on radiation through the greenhouse effect and scattering of sunlight by aerosols, strong radiative impacts of both perturbations through changes in cloudiness are analysed. The increase in greenhouse gas concentration leads to a reduction of clouds at all atmospheric levels, thus decreasing the total greenhouse effect in the longwave spectrum and increasing absorption of solar radiation by reduction of cloud albedo. Increasing anthropogenic aerosol burden results in a decrease in high-level cloud cover through a cooling of the atmosphere, and an increase in the low-level cloud cover through the second aerosol indirect effect. The trend in low-level cloud lifetime due to aerosols is quantified to 0.5 min day^–1 decade^–1 for the simulation period. The different changes in high (decrease) and low-level (increase) cloudiness due to the response of cloud processes to aerosols impact shortwave radiation in a contrariwise manner, and the net effect is slightly positive. The total aerosol effect including the aerosol direct and first indirect effects remains strongly negative.     

Emissions, Concentrations, & Temperature: A Time Series Analysis

We use recent advances in time series econometrics to estimate the relation among emissions of CO₂ and CH₄, the concentration of these gases, and global surface temperature. These models are estimated and specified to answer two questions; (1) does human activity affect global surface temperature and; (2) does global surface temperature affect the atmospheric concentration of carbon dioxide and/or methane. Regression results provide direct evidence for a statistically meaningful relation between radiative forcing and global surface temperature. A simple model based on these results indicates that greenhouse gases and anthropogenic sulfur emissions are largely responsible for the change in temperature over the last 130 years. The regression results also indicate that increases in surface temperature since 1870 have changed the flow of carbon dioxide to and from the atmosphere in a way that increases its atmospheric concentration. Finally, the regression results for methane hint that higher temperatures may increase its atmospheric concentration, but this effect is not estimated precisely.     

The RCP greenhouse gas concentrations and their extensions from 1765 to 2300

We present the greenhouse gas concentrations for the Representative Concentration Pathways (RCPs) and their extensions beyond 2100, the Extended Concentration Pathways (ECPs). These projections include all major anthropogenic greenhouse gases and are a result of a multi-year effort to produce new scenarios for climate change research. We combine a suite of atmospheric concentration observations and emissions estimates for greenhouse gases (GHGs) through the historical period (1750?C2005) with harmonized emissions projected by four different Integrated Assessment Models for 2005?C2100. As concentrations are somewhat dependent on the future climate itself (due to climate feedbacks in the carbon and other gas cycles), we emulate median response characteristics of models assessed in the IPCC Fourth Assessment Report using the reduced-complexity carbon cycle climate model MAGICC6. Projected ??best-estimate?? global-mean surface temperature increases (using inter alia a climate sensitivity of 3°C) range from 1.5°C by 2100 for the lowest of the four RCPs, called both RCP3-PD and RCP2.6, to 4.5°C for the highest one, RCP8.5, relative to pre-industrial levels. Beyond 2100, we present the ECPs that are simple extensions of the RCPs, based on the assumption of either smoothly stabilizing concentrations or constant emissions: For example, the lower RCP2.6 pathway represents a strong mitigation scenario and is extended by assuming constant emissions after 2100 (including net negative CO₂ emissions), leading to CO₂ concentrations returning to 360 ppm by 2300. We also present the GHG concentrations for one supplementary extension, which illustrates the stringent emissions implications of attempting to go back to ECP4.5 concentration levels by 2250 after emissions during the 21^st century followed the higher RCP6 scenario. Corresponding radiative forcing values are presented for the RCP and ECPs.     

Assessment of atmospheric emissions of pollutants and greenhouse gases from the civil aviation of Russia

Presented are the results of computation of emissions of pollutants and greenhouse gases from civil aircrafts in the first decade of the 21st century (from 2000 to 2012). It is revealed that in 2012 the emissions of pollutants to the atmospheric surface layer were reduced by 22.0–61.4% as compared with 2000, and those of greenhouse gases, by 30.6–62.3%. Environmental conditions in the area of large airports can remain rather strained. It is demonstrated that in 2012 the emissions of the majority of pollutants and greenhouse gases to the upper tropospheric layer increased by 41.9–48.5 and 43.7%, respectively, as compared with 2000. The inflow of gaseous compounds of different types of activity to the atmosphere can increase the total negative effect.     

IPCC《气候变化与土地特别报告》解读

总结了IPCC《气候变化与土地特别报告》中有关陆气相互作用、粮食系统与粮食安全、土地退化和荒漠化、可持续土地管理等的主要结论,分析了报告中争议较大的粮食系统温室气体排放、生物质能源、土地温室气体通量等问题。我国在粮食系统全生命周期温室气体排放量估算、基于遥感测量和地面测量的大气浓度等数据反演温室气体排放量等方面需要深入研究。同时,我国要继续加强可持续土地管理,提高相应的技术措施和能力建设。     

Precipitation: A Parameter Changing Climate and Modified by Climate Change

This paper discusses two aspects of climate modeling, the deep water formation in the North Atlantic and precipitation changes due to climate change caused by anthropogenic emissions of greenhouse gases. The deep water formation is strongly influenced by the precipitation, and the precipitation is affected by the concentration of the greenhouse gases in the atmosphere and by the atmospheric and oceanic circulation. The experiments discussed here have been performed independently to test the stability of the thermohaline circulation of the North Atlantic and to investigate changes in precipitation due to anthropogenic greenhouse gas emissions. The precipitation changes in a climate change environment are sufficient in some simulations to decrease the thermohaline circulation noticeably. However, it appears that the amount of freshwater needed to bring the circulation to a collapse is magnitudes larger than the anticipated change in precipitation due to anthropogenic activities within the next 100 years. The precipitation changes, on the other hand, might change regionally quite drastically towards more extreme situations, thereby putting additional stress on vegetation and enhancing soil erosion.     

A Global Inventory of Burned Areas at 1 Km Resolution for the Year 2000 Derived from Spot Vegetation Data

Biomass burning constitutes a major contribution to global emissions of carbon dioxide, carbon monoxide, methane, greenhouse gases and aerosols. Furthermore, biomass burning has an impact on health, transport, the environment and land use. Vegetation fires are certainly not recent phenomena and the impacts are not always negative. However, evidence suggests that fires are becoming more frequent and there is a large increase in the number of fires being set by humans for a variety of reasons. Knowledge of the interactions and feedbacks between biomass burning, climate and carbon cycling is needed to help the prediction of climate change scenarios. To obtain this knowledge, the scientific community requires, in the first instance, information on the spatial and temporal distribution of biomass burning at the global scale. This paper presents an inventory of burned areas at monthly time periods for the year 2000 at a resolution of 1 kilometer (km) and is available to the scientific community at no cost. The burned area products have been derived from a single source of satellite-derived images, the SPOT VEGETATION S1 1 km product, using algorithms developed and calibrated at regional scales by a network of partners. In this paper, estimates of burned area, number of burn scars and average size of the burn scar are described for each month of the year 2000. The information is reported at the country level. This paper makes a significant contribution to understanding the effect of biomass burning on atmospheric chemistry and the storage and cycling of carbon by constraining one of the main parameters used in the calculation of gas emissions.     

Responses of East Asian summer monsoon to historical SST and atmospheric forcing during 1950–2000

The East Asian summer monsoon (EASM) circulation and summer rainfall over East China have experienced large decadal changes during the latter half of the 20th century. To investigate the potential causes behind these changes, a series of simulations using the national center for atmospheric research (NCAR) community atmospheric model version 3 (CAM3) and the geophysical fluid dynamics laboratory (GFDL) atmospheric model version 2.1 (AM2.1) are analyzed. These simulations are forced separately with different historical forcing, namely tropical sea surface temperature (SSTs), global SSTs, greenhouse gases plus aerosols, and a combination of global SSTs and greenhouse gases plus aerosols. This study focuses on the relative roles of these individual forcings in causing the observed monsoon and rainfall changes over East Asia during 1950–2000. The simulations from both models show that the SST forcing, primarily from the Tropics, is able to induce most of the observed weakening of the EASM circulation, while the greenhouse gas plus (direct) aerosol forcing increases the land-sea thermal contrast and thus enhances the EASM circulation. The results suggest that the recent warming in the Tropics, especially the warming associated with the tropical interdecadal variability centered over the central and eastern Pacific, is a primary cause for the weakening of the EASM since the late 1970s. However, a realistic simulation of the relatively small-scale rainfall change pattern over East China remains a challenge for the global models.     

Towards the Construction of Climate Change Scenarios

Climate impacts assessments need regional scenarios of climate change for a wide range of projected emissions. General circulation models (GCMs) are the most promising approach to providing such information, but as yet there is considerable uncertainty in their regional projections and they are still too costly to run for a large number of emission scenarios. Simpler models have been used to estimate global-mean temperature changes under a range of scenarios. In this paper we investigate whether a fixed pattern from a GCM experiment scaled by global-mean temperature changes from a simple model provides an acceptable estimate of the regional climate change over a range of scenarios. Changes estimated using this approximate approach are evaluated by comparing them with results from ensembles of a coupled ocean-atmosphere model. Five specific emissions scenarios are considered. For increases in greenhouse gases only, the 'error' in annual mean temperature for the cases considered is smaller than the sampling error due to the model's internal variability. The method may break down for scenarios of stabilisation of concentrations, because the patterns change as the model approaches equilibrium. The inclusion of large local perturbations due to sulphate aerosols can lead to significant deviations of the temperature pattern from that obtained using greenhouse gases alone. Combining separate patterns for the responses to greenhouse gases and aerosols may improve the accuracy of approximation. Finally, the accuracy of the scaling approach is more difficult to assess for deriving changes in regional precipitation because many of the regional changes are not statistically significant in the climate change projections considered here. If precipitation changes are only marginally significant in other models, the apparent disagreement between different models may be as much due to sampling error as to genuine differences in model response.