Aerosol characteristics at Patiala during ICARB—2006

The spectral AOD measurements have been made for the first time over Patiala during multi-platform field campaign ICARB—2006 using a Multi-Wavelength Radiometer (MWR) along with the suspended particulate matter measurements with a high volume sampler. Spectral AOD has higher values in May in comparison to March and April. The monthly mean AOD values at 500 nm are 0.26 ± 0.08, 0.36 ± 0.19 and 0.58 ± 0.20 for the months of March, April and May respectively. The mean AOD is more during afternoon in comparison to forenoon at all wavelengths. The atmospheric turbidity is higher in May and is attributed to dust transported by southerly winds prevailing during this month. The Ångström parameter α varies between zero and 0.68 while β ranges from 0.1 to 0.9. The columnar water vapour content ranges from 0.12 to 2.92 cm, having a mean value of 1.06 ± 0.648 cm. The mean total suspended particulate matter is 334.41 ± 97.56 μgm/m³, an indication of high aerosol loading over Patiala during the campaign period.     

Characteristics of spectral aerosol optical depths over India during ICARB

Spectral aerosol optical depth (AOD) measurements, carried out regularly from a network of observatories spread over the Indian mainland and adjoining islands in the Bay of Bengal and Arabian Sea, are used to examine the spatio-temporal and spectral variations during the period of ICARB (March to May 2006). The AODs and the derived Ångström parameters showed considerable variations across India during the above period. While at the southern peninsular stations the AODs decreased towards May after a peak in April, in the north Indian regions they increased continuously from March to May. The Ångström coefficients suggested enhanced coarse mode loading in the north Indian regions, compared to southern India. Nevertheless, as months progressed from March to May, the dominance of coarse mode aerosols increased in the columnar aerosol size spectrum over the entire Indian mainland, maintaining the regional distinctiveness. Compared to the above, the island stations showed considerably low AODs, so too the northeastern station Dibrugarh, indicating the prevalence of cleaner environment. Long-range transport of aerosols from tshe adjoining regions leads to remarkable changes in the magnitude of the AODs and their wavelength dependencies during March to May. HYSPLIT back-trajectory analysis shows that enhanced long-range transport of aerosols, particularly from the west Asia and northwest coastal India, contributed significantly to the enhancement of AOD and in the flattening of the spectra over entire regions; if it is the peninsular regions and the island Minicoy are more impacted in April, the north Indian regions including the Indo Gangetic Plain get affected the most during May, with the AODs soaring as high as 1.0 at 500 nm. Over the islands, the Ångström exponent (α) remained significantly lower (～1) over the Arabian Sea compared to Bay of Bengal (BoB) (～1.4) as revealed by the data respectively from Minicoy and Port Blair. Occurrences of higher values of α, showing dominance of accumulation mode aerosols, over BoB are associated well with the advection, above the boundary layer, of fine particles from the east Asian region during March and April. The change in the airmass to marine in May results in a rapid decrease in α over the BoB.     

Atmospheric aerosol characteristics retrieved using ground based solar extinction studies at Mohal in the Kullu valley of northwestern Himalayan region,India

Aerosol parameters are measured using a ground-based Multi-wavelength Radiometer (MWR) at Mohal (31.90°N, 77.11°E, 1154 m amsl) in the Kullu valley during clear sky days of a seasonal year. The study shows that the values of spectral aerosol optical depths (AODs) at 500 nm and the Ångstrom turbidity coefficient ‘β’ (a measure of columnar loading in atmosphere) are high (0.41 ± 0.03, 0.27 ± 0.01) in summer, moderate (0.30 ± 0.03, 0.15 ± 0.03) in monsoon, low (0.19 ± 0.02, 0.08 ± 0.01) in winter and lowest (0.18 ± 0.01, 0.07 ± 0.01) in autumn, respectively. The Ångstrom wavelength exponent ‘α’ (indicator of the fraction of accumulation-mode particles to coarse-mode particles) has an opposite trend having lowest value (0.64 ± 0.06) in summer, low (0.99 ± 0.10) in monsoon, moderate (1.20 ± 0.15) in winter and highest value (1.52 ± 0.03) in autumn. The annual mean value of AOD at 500 nm, ‘α’ and ‘β’ are 0.24 ± 0.01, 1.06 ± 0.09 and 0.14 ± 0.01, respectively. The fractional asymmetry factor is more negative in summer due to enhanced tourists’ arrival and also in autumn months due to the month-long International Kullu Dussehra fair. The AOD values given by MWR and satellite-based moderate resolution imaging spectro-radiometer have good correlation of 0.76, 0.92 and 0.97 on diurnal, monthly and seasonal basis, respectively. The AODs at 500 nm as well as ‘β’ are found to be highly correlated, while ‘α’ is found to be strongly anti-correlated with temperature and wind speed suggesting high AODs and turbidity but low concentration of fine particles during hot and windy days. With wind direction, the AOD and ‘β’ are found to be strongly anti-correlated, while ‘α’ is strongly correlated.     

Latitudinal and longitudinal variation in aerosol characteristics from Sun photometer and MODIS over the Bay of Bengal and Arabian Sea during ICARB

Spatial variations in aerosol optical properties as function of latitude and longitude are analysed over the Bay of Bengal and Arabian Sea during ICARB cruise period of March–May 2006 from in situ sun photometer and MODIS (Terra, Aqua) satellite measurements. Monthly mean 550 nm aerosol optical depths (AODs) over the Bay of Bengal and Arabian Sea show an increase from March to May both in spatial extent and magnitude. AODs are found to increase with latitude from 4°N to 20°N over the Bay of Bengal while over Arabian Sea, variations are not significant. Sun photometer and MODIS AODs agree well within ±1σ variation. Bay of Bengal AOD (0.28) is higher than the Arabian Sea (0.24) latitudinally. Aerosol fine mode fraction (FMF) is higher than 0.6 over Bay of Bengal, while FMF in the Arabian Sea is about 0.5. Bay of Bengal α(～1) is higher than the Arabian Sea value of 0.7, suggesting the dominance of fine mode aerosols over Bay of Bengal which is corroborated by higher FMF values over Bay of Bengal. Air back trajectory analyses suggest that aerosols from different source regions contribute differently to the optical characteristics over the Bay of Bengal and Arabian Sea.     

Characterization of aerosol type based on aerosol optical properties over Baghdad,Iraq

Aerosol optical depth (AOD), Angstrom exponent (AE), and ozone monitoring instrument aerosols index (OMI-AI) data, derived from MODerate Resolution Imaging Spectroradiometer (MODIS) and OMI sensor on board NASA’s Aqua satellite and NASA-Aura satellite platforms, have been analyzed and classified over Baghdad, Iraq, for an 8-year period (2008–2015). In order to give an obvious understanding of temporal inconsistency in the characteristics and classification of aerosols during each season separately, PREDE POM-02 sky radiometer measurements of AOD, carried out during a 2-year period (2014–2015), were compared with MODIS–Aqua AODs. On seasonal bases, MODIS–Aqua AODs corroborate well with ground-based measurements, with correlation coefficients ranging between 0.74 and 0.8 and RMSE ranging from 0.097 to 0.062 during spring and autumn seasons respectively. The overall satellite- and ground-based measurement comparisons showed a good agreement with correlation coefficients of 0.78 and RMSE of 0.066. These results suggest that MODIS–Aqua gives a good estimate of AOD. Analysis of MODIS–Aqua data for the 8-year period showed that the overall mean AOD, AE, and OMI-AI over Baghdad were 0.44?±?0.16, 0.77?±?0.29, and 1.34?±?0.33 respectively. AOD records presented a unique peak which was extended from mid-spring (April) to mid-summer (July) while the AE annual variability indicated a more complicated behavior with minimum values during the period from late spring (May) to early autumn (September). The maximum AOD and OMI-AI values occurred during summer while their minimum values occurred during winter. The AE showed an opposite behavior to that of AOD such that the highest AE values occurred during autumn and winter and the lowest values happened during spring and summer. This behavior may be attributed to the domination of coarse aerosol particles during autumn and winter seasons and fine aerosol particles during spring and summer seasons. A Hybrid Single-Particle Lagrangian Integrated Trajectory model was utilized to determine the source of air mass transport and to recognize the variability of aerosol origin regions. Finally, AOD, AE, and OMI-AI values have been employed to identify several aerosol types and to present seasonal heterogeneity in their contribution based on their origins.     

Physical and optical characteristics of atmospheric aerosols during ICARB at Manora Peak,Nainital: A sparsely inhabited,high-altitude location in the Himalayas

Collocated measurements of the optical and physical properties of columnar and near-surface aerosols were carried out from Manora Peak, Nainital (a sparsely inhabited, high altitude location, ～2 km above mean sea level, in the Himalayas), during the Integrated Campaign for Aerosols, gases and Radiation Budget (ICARB) under the Geosphere Biosphere Programme of the Indian Space Research Organization (ISRO-GBP). Under this, observational data of spectral aerosol optical depths (AOD), mass concentration of aerosol black carbon (M _B ), mass concentration (M _T ) and number concentration (N _t ) of composite (total) aerosols near the surface and meteorological parameters were collected during the period February 15 to April 30, 2006. Though very low (<0.1 at 500 nm) AODs were observed during clear days, as much as a four-fold increase was seen on hazy days. The Ångström exponent (α), deduced from the spectral AODs, revealed high values during clear days, while on hazy days α was low; with an overall mean value of 0.69 ± 0.06 for the campaign period. BC mass concentration varied between 0.36 and 2.87 μg m^?3 and contributed in the range 0.7 to 1.8% to the total aerosol mass. Total aerosol number concentration and BC mass concentration showed diurnal variation with a midnight and early morning minimum and a late afternoon maximum; a pattern quite opposite to that seen in low altitude stations. These are attributed to the dynamics of the atmospheric boundary layer.     

Trends in aerosol optical properties over Eastern Europe based on MODIS-Aqua

This study provides characteristics of aerosol columnar properties, measured over ten countries in Eastern Europe from 2002 to 2019. Aerosol optical depth (AOD) and Ångström exponent (AE) were obtained with the Moderate Resolution Imaging Spectroradiometer (MODIS) Collection 6.1 merged Dark Target and Deep Blue aerosol product. The product is validated using ground-based Aerosol Robotic Network (AERONET) situated at Minsk, Belsk, Moldova and Kyiv. The results showed that 76.15% of retrieved AOD data are within the expected error. It was established that 64.2% of AOD points are between 0 and 0.2 and 79.3% of all AE points are over 1. Mean AOD values in the region vary from 0.130 ​± ​0.04 (Moldova) to 0.193 ​± ​0.03 (Czech Republic) with mean value in the region 0.162 ​± ​0.05. Seasonal mean AOD (AE) values were at the maximum during the summer from 0.231 ​± ​0.05 (1.482 ​± ​0.09 in winter) to minimum 0.087 ​± ​0.04 during the winter (1.363 ​± ​0.17 in summer). Gradual AOD reduction is observed in all countries with annual trend from −0.0050 (Belarus) to −0.0029 (Russia). Finally, the relationship between AOD and AE was studied to classify various aerosol types and showed seasonal non-uniformity of their contribution depending on variation in sources. The entire region is under significant impact of various aerosol types, including clean continental (СС), mixed (MX) and anthropogenic/burning (AB) aerosols types that are at 59.77%, 24.72%, and 12.97% respectively. These results form an important basis for further regional studies of air quality and distribution of sources of pollution.     

Study of total column atmospheric aerosol optical depth,ozone and precipitable water content over Bay of Bengal during BOBMEX-99

The spatial and temporal variations in aerosols and precursor gases over oceanic regions have special importance in the estimation of radiative forcing parameters and thereby in the refinement of general circulation models. Extensive observations of the columnar aerosol optical depth (AOD), total column ozone (TCO) and precipitable water content (PWC) have been carried out using the on-line, multi-band solar radiometers onboard ORV Sagar Kanya (Cruise # SK 147B) over Bay of Bengal during 11th–28th August 1999. Aerosol optical and physical properties (optical depth and angstrom parameter) have been estimated at six wavelengths covering from UV to NIR (380–1020 nm) while TCO and PWC have been determined using the UV band around 300 nm and NIR band around 940 nm, respectively. Added, concurrent meteorological and satellite observations during this field phase of BOBMEX-99 have been utilized to investigate spectral-temporal variations of AOD, TCO and PWC in marine environment. The results indicate lower AODs (around 0.4 at characteristic wavelength of 500 nm) and size distributions with abundance of coarse-mode particles as compared to those aerosols of typical land origin. An interesting result that is found in the present study is the significant reduction in AOD at all wavelengths from initial to later part of observation period due to cloud-scavenging and rain-washout effects as well as signature of coastal aerosol loading. The clear-sky daytime diurnal variation of TCO shows gradual increase during post-sunrise hours, broad maximum during afternoon hours and gradual decrease during pre-sunset hours, which is considered to be due to photochemical reactions. The diurnal variation curve of PWC showed maximum (~ 4 cm) during morning hours and gradual decrease (~ 3.5 cm) towards evening hours, which are found to be greater as compared to typical values over land. Another interesting feature observed is that although the PWC values are very high, there was no proportionate or appreciable enhancement in AOD—a feature that can be utilized to infer composition of aerosols over the study region.     

新疆地区不同下垫面气溶胶光学特性的分析

利用太阳光度计CE318资料,对新疆地区3个观测站点（阿克达拉、乌鲁木齐、塔中）所代表的草场、城市和沙漠下垫面的440 nm波长处气溶胶光学厚度（AOD）和440~870 nm之间的Angstrom波长指数（AE）进行了统计分析,结果表明：三个站点的AOD年均值塔中站最大、乌鲁木齐站次之、阿克达拉站最小。其中阿克达拉站点的AOD全年变化不大,其月均值均小于0.3;乌鲁木齐站点AOD则表现出明显的季节性变化,冬春季的AOD月均值是夏秋季节的2.17倍;塔中站全年的AOD表现为单峰型,大值时段主要集中在3-7月。三个站点的AE年均值阿克达拉站最大、乌鲁木齐站次之、塔中站最小。阿克达拉和乌鲁木齐站点的AOD以人为排放等小粒径气溶胶为主,塔中站的AOD主要为沙尘等大粒径气溶胶。从年际变化来看,乌鲁木齐站AOD总体呈下降趋势,塔中站和阿克达拉站AOD总体呈上升趋势。乌鲁木齐霾天气的AOD日均值分布在0.35~1.21之间,塔中站沙尘天气的AOD日均值范围为0.30~2.05。     

Evaluation and comparison of CMIP6 models and MERRA-2 reanalysis AOD against Satellite observations from 2000 to 2014 over China

Rapid industrialization and urbanization along with a growing population are contributing significantly to air pollution in China. Evaluation of long-term aerosol optical depth (AOD) data from models and reanalysis, can greatly promote understanding of spatiotemporal variations in air pollution in China. To do this, AOD (550 nm) values from 2000 to 2014 were obtained from the Coupled Model Inter-comparison Project (CIMP6), the second version of Modern-Era Retrospective analysis for Research, and Applications (MERRA-2), and the Moderate Resolution Imaging Spectroradiometer (MODIS; flying on the Terra satellite) combined Dark Target and Deep Blue (DTB) aerosol product. We used the Terra-MODIS DTB AOD (hereafter MODIS DTB AOD) as a standard to evaluate CMIP6 Ensemble AOD (hereafter CMIP6 AOD) and MERRA-2 reanalysis AOD (hereafter MERRA-2 AOD). Results show better correlations and smaller errors between MERRA-2 and MODIS DTB AOD, than between CMIP6 and MODIS DTB AOD, in most regions of China, at both annual and seasonal scales. However, significant under- and over-estimations in the MERRA-2 and CMIP6 AOD were also observed relative to MODIS DTB AOD. The long-term (2000–2014) MODIS DTB AOD distributions show the highest AOD over the North China Plain (0.71) followed by Central China (0.69), Yangtse River Delta (0.67), Sichuan Basin (0.64), and Pearl River Delta (0.54) regions. The lowest AOD values were recorded over the Tibetan Plateau (0.13 ± 0.01) followed by Qinghai (0.19 ± 0.03) and the Gobi Desert (0.21 ± 0.03). Large amounts of sand and dust particles emitted from natural sources (the Taklamakan and Gobi Deserts) may result in higher AOD in spring compared to summer, autumn, and winter. Trends were also calculated for 2000–2005, for 2006–2010 (when China introduced strict air pollution control policies during the 11th Five Year Plan or FYP), and for 2011–2014 (during the 12th FYP). An increasing trend in MODIS DTB AOD was observed throughout the country during 2000–2014. The uncontrolled industrialization, urbanization, and rapid economic development that mostly occurred from 2000 to 2005 probably contributed to the overall increase in AOD. Finally, China's air pollution control policies helped to reduce AOD in most regions of the country; this was more evident during the 12th FYP period (2011–2014) than during the 11th FYP period (2006–2010). Therefore this study strongly advises the authority to retain or extend these policies in the future for improving air quality.     

Influence of circulation parameters on the AOD variations over the Bay of Bengal during ICARB

MODIS (Moderate Resolution Imaging Spectroradiometer) level-3 aerosol data, NCEP (National Centers for Environmental Prediction) reanalysis winds and QuikSCAT ocean surface winds were made use of to examine the role of atmospheric circulation in governing aerosol variations over the Bay of Bengal (BoB) during the first phase of the ICARB (Integrated Campaign for Aerosols, gases and Radiation Budget) campaign (March 18–April 12, 2006). An inter-comparison between MODIS level-3 aerosol optical depth (AOD) data and ship-borne MICROTOPS measurements showed good agreement with correlation 0.92 (p < 0.0001) and a mean MODIS underestimation by 0.01. During the study period, the AOD over BoB showed high values in the northern/north western regions, which reduced towards the central and southern BoB. The wind patterns in lower atmospheric layers (> 850 hPa) indicated that direct transport of aerosols from central India was inhibited by the presence of a high pressure and a divergence over BoB in the lower altitudes. On the other hand, in the upper atmospheric levels, winds from central and northern India stretched south eastwards and converged over BoB with a negative vorticity indicative of a downdraft. These wind patterns pointed to the possibility of aerosol transport from central India to BoB by upper level winds. This mechanism was further confirmed by the significant correlations that AOD variations over BoB showed with aerosol flux convergence and flux vorticity at upper atmospheric levels (600–500 hPa). AOD in central and southern BoB away from continental influences displayed an exponential dependence on the QuikSCAT measured ocean surface wind speed. This study shows that particles transported from central and northern India by upper atmospheric circulations as well as the marine aerosols generated by ocean surface winds contributed to the AOD over the BoB during the first phase of ICARB.     

Optical and radiative properties of aerosols over Abu Dhabi in the United Arab Emirates

The present study is on the aerosol optical and radiative properties in the short-wave radiation and its climate implications at the arid city of Abu Dhabi (24.42 ^°N, 54.61 ^°E, 4.5 m MSL), in the United Arab Emirates. The direct aerosol radiative forcings (ARF) in the short-wave region at the top (TOA) and bottom of the atmosphere (BOA) are estimated using a hybrid approach, making use of discrete ordinate radiative transfer method in conjunction with the short-wave flux and spectral aerosol optical depth (AOD) measurements, over a period of 3 years (June 2012–July 2015), at Abu Dhabi located at the south-west coast of the Arabian Gulf. The inferred microphysical properties of aerosols at the measurement site indicate strong seasonal variations from the dominance of coarse mode mineral dust aerosols during spring (March–May) and summer (June–September), to the abundance of fine/accumulation mode aerosols mainly from combustion of fossil-fuel and bio-fuel during autumn (October–November) and winter (December–February) seasons. The monthly mean diurnally averaged ARF at the BOA (TOA) varies from ?13.2 Wm^?2 (～?0.96 Wm^?2) in November to ?39.4 Wm^?2 (?11.4 Wm^?2) in August with higher magnitudes of the forcing values during spring/summer seasons and lower values during autumn/winter seasons. The atmospheric aerosol forcing varies from + 12.2 Wm^?2 (November) to 28.2 Wm^?2 (June) with higher values throughout the spring and summer seasons, suggesting the importance of mineral dust aerosols towards the solar dimming. Seasonally, highest values of the forcing efficiency at the surface are observed in spring (?85.0 ± 4.1 W m^?2 τ ^?1) followed closely by winter (?79.2 ± 7.1 W m^?2 τ ^?1) and the lowest values during autumn season (?54 ± 4.3 W m^?2 τ ^?1). The study concludes with the variations of the atmospheric heating rates induced by the forcing. Highest heating rate is observed in June (0.39 K day ^?1) and the lowest in November (0.17 K day ^?1) and the temporal variability of this parameter is linearly associated with the aerosol absorption index.     

Detection of marine aerosols with IRS P4-Ocean Colour Monitor

The atmospheric correction bands 7 and 8 (765nm and 865nm respectively) of the Indian Remote Sensing Satellite IRS P4-0CM (Ocean Colour Monitor) can be used for deriving aerosol optical depth (AOD) over the oceans. A retrieval algorithm has been developed which computes the AOD using band 7 data by treating the ocean surface as a dark background after removing the Rayleigh path radiance in the sensor-detected radiances. This algorithm has been used to detect marine aerosol distributions at different coastal and offshore locations around India. A comparison between OCM derived AOD and the NOAA operational AOD shows a correlation ∼0.92 while that between OCM derived AOD and the ground-based sun photometer measurements near the coast of Trivandrum shows a correlation of ∼0.90.     

Impact of dust events on aerosol optical properties over Iraq

The spatial and temporal characteristics of aerosol optical properties (AOP) were analyzed in order to find out the hotspot aerosol sources over Iraq and surrounding regions. The correlation of AOP with the frequency of dust events (dust storm (DS), rising dust (RD), suspended dust (SD)) over 12 Iraqi stations is evaluated during the study period (January 2005–December 2014). The AOP: aerosol absorption optical depth (AAOD), aerosol extinction optical depth (AOD), and aerosol single scattering albedo (SSA) at 388 and 500 nm and aerosol index (AI), are derived from the Ozone Monitoring Instrument (OMI) on board the Aura satellite. Three well-known spatial interpolation techniques: inverse distance weighting, radial basis function with three sub-types, and kriging with three sub-types, are examined in ArcGIS software. Statistical analysis is applied to compute the station probability of dust events and its correlation with AOP. Results showed that the spline with the lowest RMSE and MPE near zero is the optimum method for estimating AOP. The spatial mean of AAOD, AOD, and AI (SSA) have the same pattern with high (low) mean values over the south and northwest of Iraq, Kuwait, and the northeast of Saudi Arabia. The seasonal variability of AAOD and AOD over the Iraqi stations showed that high (low) values occurred during spring and summer (winter) and concluded that AAOD is a responsible component for variation in AOD. DS and RD probability is higher over stations in the middle and south of Iraq than the stations in the north. High SD probability is over Mosul, Baghdad, and Nasiriya stations. The correlation of AOP with dust events suggests that the AAOD component is more important in the study of DS than SSA and AI while AI is a good index for the study of RD and SD in the study region.     

Variations in sulphate aerosols concentration during winter monsoon season for two consecutive years using a general circulation model

During the field cruises of the Indian Ocean Experiment (INDOEX) extensive measurements on the atmospheric chemical and aerosol composition are undertaken to study the long-range transport of air pollution from south and southeast Asia towards the Indian Ocean during the dry monsoon season in 1998 and 1999. The present paper discusses the temporal and spatial variations in aerosols and aerosol forcing during the winter monsoon season (January-March) for INDOEX first field phase (FFP) in 1998 and INDOEX intensive field phase (IFP) in 1999. An interactive chemistry/aerosol model (LMDZ.3.3) is used to investigate the variation in the spatial distribution of tropospheric sulphate aerosols during 1998 and 1999. The model results depict major enhancement in the sulphate aerosol concentrations, radiative forcing (RF) and optical depth over the Indian subcontinent and adjoining marine areas between INDOEX-FFP and IFP. A significant increase in transport of sulphate aerosols from the continents to the Indian Ocean region has also been simulated during the winter monsoon in 1999. The mean RF over INDOEX-FFP in 1998 is found to be ?1.2 Wm^–2 while it increased to ?1.85 Wm^–2 during INDOEX-IFP in 1999. Model results reveal a mean sulphate aerosol optical depth (AOD) of 0.08 and 0.14 over Indian subcontinent during 1998 and 1999, respectively. The model results suggest that elevated AOD downwind of source regions in India can significantly affect the regional air quality and adjoining marine environments.     

Lidar observation of aerosol stratification in the lower troposphere over Pune during pre-monsoon season of 2006

Lidar observations of aerosol vertical distributions in the lower troposphere along with observations of horizontal and vertical winds from collocated UHF radar (Wind Profiler) over a tropical Indian station, Pune during the pre-monsoon season (March–May) of 2006 as part of an ISRO-GBP national campaign (ICARB) have been examined. Lidar vertical profiles showed high aerosol concentrations in the surface layers and a subsequent gradual decrease with height. Results showed the presence of an elevated stratified aerosol layer around 2000–3500m height which persisted throughout the months of March and April. Observed strong vertical gradients in both horizontal and vertical winds in the lower troposphere seem to be a possible cause for the formation of elevated aerosol layers. Further, high daytime temperatures accompanied by dry conditions at the surface help to enhance the aerosol loading in the lower layers over this location.     

Impact of aerosols from the Asian Continent on the adjoining oceanic environments

Aerosol optical depth (AOD) at 630 nm wavelength over the oceanic regions adjoining the Asian Continent is examined using a seven-year long data base derived from the Advanced Very High Resolution Radiometer (AVHRR) on board NOAA satellite to study the mean spatial and temporal variations as well as to understand the impact of aerosols advecting from the continent. Depending on the prevailing meteorological conditions and nature of synoptic circulation, the AOD over the oceanic region shows a systematic annual variation. This annual pattern inturn also shows an inter-annual variability because of the corresponding variations in the meteorological features over the continent as well as small-scale deviations in the nature of synoptic circulation. The annual variation over the oceanic regions also shows a pronounced spatial heterogeneity depending on the influence of continental aerosols. Making use of the wind speed dependence of sea-salt AOD at far-oceanic environments and monthly mean wind speeds at small grids of size 5° × 5°, the annual variation of sea-salt AOD at different locations is studied to understand the spatial heterogeneity of this component. The residual component obtained by subtracting this from the measured AOD is the non-oceanic component due to advection from continent. The source regions for major continental advections are delineated from the analysis of air-mass back trajectories at appropriate locations identified from the annual pattern of non-oceanic component. The long-term effect of the continental impact is examined from the mean trend of AOD over the three major oceanic regions. This study shows that the continental influence is most significant over the Arabian Sea, followed by the Bay of Bengal and is almost insignificant in most of the regions over the Southern Hemispheric Indian Ocean, except for the effect of smoke aerosols over a few locations near Indonesia and Madagascar.     

Airborne measurements of submicron aerosols across the coastline at Bhubaneswar during ICARB

Airborne measurements of the number concentration and size distribution of aerosols from 13 to 700 nm diameter have been made at four vertical levels across a coastline at Bhubaneswar (20°25′N, 85°83′E) during the Integrated Campaign for Aerosols, gases and Radiation Budget (ICARB) programme conducted in March–April 2006. The measurements made during the constant-level flights at 0.5, 1, 2 and 3 km altitude levels extend ～100 km over land and ～150km over ocean. Aerosol number concentrations vary from 2200 to 4500 cm^?3 at 0.5 km level but are almost constant at ～ 6000 cm^?3 and ～ 800 cm^?3 at 2 and 3 km levels, respectively. At 1km level, aerosol number concentration shows a peak of 18,070 cm^?3 around the coastline. Most of the aerosol size distribution curves at 0.5 km and 1 km levels are monomodal with a maxima at 110nm diameter which shifts to 70 nm diameter at 2 and 3 km levels. However, at the peak at 1 km level, number concentration has a bimodal distribution with an additional maximum appearing in nucleation mode. It is proposed that this maxima in nucleation mode at 1 km level may be due to the formation and transport of new particles from coastal regions.     

Volatile properties of atmospheric aerosols during nucleation events at Pune,India

Continuous measurements of aerosol size distributions in the mid-point diameter range 20.5–500 nm were made from October 2005 to March 2006 at Pune (18°32′N, 73°51′E), India using Scanning Mobility Particle Sizer (SMPS). Volatilities of atmospheric aerosols were also measured at 40°, 125°, 175°, 300° and 350°C temperatures with Thermodenuder–SMPS coupled system to determine aerosol volatile fractions. Aerosols in nucleated, CCN and accumulated modes are characterized from the measured percentage of particles volatized at 40°, 125°, 175°, 300° and 350°C temperatures. Averaged monthly aerosol concentration is at its maximum in November and gradually decreases to its minimum at the end of March. The diurnal variations of aerosol concentrations gradually decrease in the night and in early morning hours (0400–0800 hr). However, concentration attains minimum in its variations in the noon (1400–1600 hr) due to higher ventilation factor (product of mixing height and wind speed). The half an hour averaged diurnal variation of aerosol number concentration shows about 5 to 10-fold increase despite the ventilation factor at higher side before 1200 hr. This sudden increase in aerosol concentrations is linked with prevailing conditions for nucleation bursts. The measurement of volatile fraction of ambient aerosols reveals that there are large number of highly volatile particles in the Aitken mode in the morning hours and these volatile fractions of aerosols at temperatures <150°C are of ammonium chloride and ammonium sulfate, acetic and formic acids.     

Analysis of marine aerosol optical depth retrieved from IRS-P4 OCM sensor and comparison with the aerosol derived from SeaWiFS and MODIS sensor

Aerosol optical depth is regularly derived from SeaWiFS and MODIS sensor and used by the scientific community in various climatic studies. In the present study an attempt has been made to retrieve the aerosol optical depth using the IRS-P4 OCM sensor data and a comparison has been carried out using few representative datasets. The results show that the IRS-P4 OCM retrieved aerosol optical depth is in good agreement with the aerosols retrieved from SeaWiFS as well as MODIS. The RMSE are found to be ±0.0522 between OCM and SeaWIFS and ±0.0638 between OCM and MODIS respectively. However, IRS-P4 OCM sensor retrieved aerosol optical depth is closer to SeaWiFS (correlation = 0.88, slope = 0.96 and intercept = ?0.013) compared to MODIS (correlation = 0.75, slope = 0.91 and intercept = 0.0198). The mean percentage difference indicates that OCM retrieved AOD is +12% higher compared to SeaWiFS and +8% higher compared to MODIS. The mean absolute percentage between OCM derived AOD and SeaWiFS is found to be less (16%) compared to OCM and MODIS (20%).