Stratospheric aerosol measurements in the Arctic winter of 1996/1997 with the M‐55 Geophysika high‐altitude research aircraft

In‐situ aerosol measurements were performed in the northern hemispheric stratosphere up to altitudes of 21 km between 13 November 1996 and 14 January 1997, inside and outside of the polar vortex during the Airborne Polar Experiment (APE) field campaign. These are measurements of particle size distributions with a laser optical particle counter of the FSSP‐300 type operated during 9 flights on the Russian M‐55 high‐altitude research aircraft Geophysika. For specific flights, the FSSP‐300 measurements are compared with balloon‐borne data (launched from Kiruna, Sweden). It was found that the stratospheric aerosol content reached levels well below the background concentrations measured by the NASA operated ER‐2 in 1988/89 in the northern hemisphere. During the APE campaign, no PSC particle formation was observed at flight altitudes although the temperatures were below the NAT condensation point during one flight. The measured correlations between ozone and aerosol give an indication of the subsidence inside the 1996/97 polar vortex. Despite the lower aerosol content in the winter 1996/97 compared to the 1989 background, the heterogeneous reactivity of the aerosol (as calculated from the measured data with additional model input) is comparable. This is due to the dependency of the reactive uptake coefficients on the atmospheric water vapor content. Under the described assumptions the reaction rates on the background aerosol are significantly smaller than for competing gas phase chlorine activation, as can be expected for stratospheric background conditions especially inside the polar vortex.     

Interannual variations in total ozone fields at high latitudes of the Northern Hemisphere, November to March 1998–2005

Synoptic analysis of monthly and daily mean total ozone fields is carried out using ground-based (Roshydromet) and TOMS measurements. Large interannual changes in the evolution of the stratospheric polar vortex and the North Pacific anticyclone influence the formation and dynamics of the winter-spring ozone fields in the stratosphere of high northern latitudes. The analysis shows considerable variations in the direction of zonal ozone transport from the sector of ozone inflow from low latitudes and accumulation in the Far East depending on the winter polar stratosphere temperature and the quasi-biennial oscillation (QBO) phase. In years with the easterly QBO phase and the warm polar stratosphere, ozone at the end of winter is transported to northeastern Canada and Atlantic. In years with the easterly phase and cold polar stratosphere, ozone transport is directed to northern Eurasia. These characteristics will be verified on extensive observational data.     

2019-2020冬季北半球超强极涡事件

2019-2020冬季北极平流层极涡异常并且持续的偏强,偏冷.利用NCEP再数据和OMI臭氧数据,本文分析了此次强极涡事件中平流层极涡的动力场演变及其对地面暖冬天气和臭氧低值的影响.此次强极涡的形成是由于上传行星波不活跃.持续的强极涡使得2020年春季的最后增温出现时间偏晚.平流层正NAM指数向下传播到地面,与地面AO指数和NAO指数相一致,欧亚大陆和北美地面气温均比气候态偏暖,在欧亚大陆的一些地区,2020年1月和2月的气温甚至偏高了 10K.2020年2月以来北极臭氧出现了2004年以来的最低值,2020年3-4月60°-90°N的平均臭氧柱总量比气候态偏低了 80DU.     

Observed and simulated precursors of stratospheric polar vortex anomalies in the Northern Hemisphere

The Northern Hemisphere stratospheric polar vortex is linked to surface weather. After Stratospheric Sudden Warmings in winter, the tropospheric circulation is often nudged towards the negative phase of the Northern Annular Mode (NAM) and the North Atlantic Oscillation (NAO). A strong stratospheric vortex is often associated with subsequent positive NAM/NAO conditions. For stratosphere?Ctroposphere associations to be useful for forecasting purposes it is crucial that changes to the stratospheric vortex can be understood and predicted. Recent studies have proposed that there exist tropospheric precursors to anomalous vortex events in the stratosphere and that these precursors may be understood by considering the relationship between stationary wave patterns and regional variability. Another important factor is the extent to which the inherent variability of the stratosphere in an atmospheric model influences its ability to simulate stratosphere?Ctroposphere links. Here we examine the lower stratosphere variability in 300-year pre-industrial control integrations from 13 coupled climate models. We show that robust precursors to stratospheric polar vortex anomalies are evident across the multi-model ensemble. The most significant tropospheric component of these precursors consists of a height anomaly dipole across northern Eurasia and large anomalies in upward stationary wave fluxes in the lower stratosphere over the continent. The strength of the stratospheric variability in the models was found to depend on the variability of the upward stationary wave fluxes and the amplitude of the stationary waves.     

The cause of the spring strengthening of the Antarctic polar vortex

The stratospheric polar vortex strengthening from late winter to spring plays a crucial role in polar ozone depletion. The Arctic polar vortex reaches its peak intensity in mid-winter, whereas the Antarctic vortex usually strengthens in early spring. As a result, the strong ozone depletion is observed every year over the Antarctic, while over the Arctic short-term ozone loss occasionally occurs in late winter or early spring. However, the cause of such a difference in the life cycles of the Arctic and Antarctic polar vortices is still not completely clear. Based on the ERA-Interim reanalysis data, we show a high agreement between the seasonal variations of temperature in the subtropical lower stratosphere and zonal wind in the subpolar and polar lower stratosphere in the Southern Hemisphere. Thus, the spring strengthening of the Antarctic polar vortex can occur due to the seasonal temperature increase in the subtropical lower stratosphere in this period.     

涡动在南北半球平流层极涡崩溃过程中作用的比较

比较了南北半球春季平流层极涡的崩溃过程以及涡动在此崩溃过程中的作用。极涡的崩溃时间以平流层极夜急流核区最后一次西风转换为东风的时间来确定。结果表明南北半球平流层极涡的崩溃过程有着共同的特点,涡动和非绝热加热过程都对极涡的崩溃起着重要的作用,在极涡崩溃前平流层行星尺度波动活动明显,极涡崩溃以后,这种波动活动便迅速减弱。其中从对流层上传的行星波决定着极涡的具体崩溃时间。两个半球的差别主要表现在南半球极涡崩溃过程一般始于平流层高层,然后逐渐下传,而北半球这种下传不是很明显。其次,北半球平流层极涡崩溃偏晚年,极涡的减弱有两次过程,第一次为快速变化过程,第二次变化比较缓慢,而南半球平流层极涡崩溃无论早晚年只有一次减弱过程。长期的变化趋势分析表明南北半球平流层极涡的崩溃时间逐渐推迟,特别是20世纪90年代中后期以来,这种推迟更加明显。进一步的研究还发现,伴随着平流层极涡的崩溃过程平流层和对流层存在强烈的动力耦合,南北半球极涡迅速减弱前,各自半球的环状模指数也由负指数增加为正指数,表明低层环流对于平流层极涡的崩溃起到重要的作用;同时极涡不同强度所对应的低层环状模指数也不同,这可能与不同强度平流层极涡对于上传的行星波的反射有关。     

Stratospheric Polar Vortex Splitting in December 2009

Abstract

The 2009–10 Arctic stratospheric winter, in comparison with other recent winters, is mainly characterized by a major Sudden Stratospheric Warming (SSW) in late January associated with planetary wavenumber 1. This event led to a large increase in the temperature of the polar stratosphere and to the reversal of the zonal wind. Unlike other major SSW events in recent winters, after the major SSW in January 2010 the westerlies and polar vortex did not recover to their pre-SSW strength until the springtime transition. As a result, the depletion of the ozone layer inside the polar vortex over the entire winter was relatively small over the past 20 years. The other distinguishing feature of the 2010 winter was the splitting of the stratospheric polar vortex into two lobes in December. The vortex splitting was accompanied by an increase in the temperature of the polar stratosphere and a weakening of the westerlies but with no reversal. The splitting occurred when, in addition to the high-pressure system over northeastern Eurasia and the northern Pacific Ocean, the tropospheric anticyclone over Europe amplified and extended to the lower stratosphere. Analysis of wave activity in the extratropical troposphere revealed that two Rossby wave trains propagated eastward to the North Atlantic several days prior to the vortex splitting. The first wave train propagated from the subtropics and mid-latitudes of the eastern Pacific Ocean over North America and the second one propagated from the northern Pacific Ocean. These wave trains contributed to an intensification of the tropospheric anticyclone over Europe and to the splitting of the stratospheric polar vortex.     

The Role of Stationary and Transient Planetary Waves in the Maintenance of Stratospheric Polar Vortex Regimes in Northern Hemisphere Winter

Using 1958-2002 NCEPNCAR reanalysis data, we investigate stationary and transient planetary wave propagation and its role in wave-mean flow interaction which influences the state of the polar vortex (PV) in the stratosphere in Northern Hemisphere (NH) winter. This is done by analyzing the Eliassen-Palm (E-P) flux and its divergence. We find that the stationary and transient waves propagate upward and equatorward in NH winter, with stronger upward propagation of stationary waves from the troposphere to the stratosphere, and stronger equatorward propagation of transient waves from mid-latitudes to the subtropics in the troposphere. Stationary waves exhibit more upward propagation in the polar stratosphere during the weak polar vortex regime (WVR) than during the strong polar vortex regime (SVR). On the other hand, transient waves have more upward propagation during SVR than during WVR in the subpolar stratosphere, with a domain of low frequency waves. With different paths of upward propagation, both stationary and transient waves contribute to the maintenance of the observed stratospheric PV regimes in NH winter.     

Effects of meridional sea surface temperature changes on stratospheric temperature and circulation

Using a state-of-the-art chemistry-climate model,we analyzed the atmospheric responses to increases in sea surface temperature （SST）.The results showed that increases in SST and the SST meridional gradient could intensify the subtropical westerly jets and significantly weaken the northern polar vortex.In the model runs,global uniform SST increases produced a more significant impact on the southern stratosphere than the northern stratosphere,while SST gradient increases produced a more significant impact on the northern stratosphere.The asymmetric responses of the northern and southern polar stratosphere to SST meridional gradient changes were found to be mainly due to different wave properties and transmissions in the northern and southern atmosphere.Although SST increases may give rise to stronger waves,the results showed that the effect of SST increases on the vertical propagation of tropospheric waves into the stratosphere will vary with height and latitude and be sensitive to SST meridional gradient changes.Both uniform and non-uniform SST increases accelerated the large-scale Brewer-Dobson circulation （BDC）,but the gradient increases of SST between 60°S and 60°N resulted in younger mean age-of-air in the stratosphere and a larger increase in tropical upwelling,with a much higher tropopause than from a global uniform 1.0 K SST increase.     

2007/2008和2008/2009冬季平流层强、弱极涡事件对应的行星波活动的对比分析

在对逐日气象资料进行纬向谐波分析的基础上, 对比和讨论了2007/2008年冬季强极涡期间和2008/2009冬季弱极涡期间平流层和对流层不同波数的行星波的变化特征, 特别关注强极涡或弱极涡发生之后, 500 hPa 沿60°N和30°N行星波1波和2波振幅和位相的差异, 以及相应的500 hPa位势场的差异, 进而讨论为什么不同的平流层极涡异常会对东亚有不同的影响, 特别讨论为什么同一种极涡异常, 对我国南北方近地面气温的影响会不同。结果表明:平流层极涡发生异常时, 平流层行星波活动有明显的异常。随着极涡异常的下传, 对流层行星波的振幅和位相也有明显的变化, 而且, 对于不同的纬度带, 其变化又有不同, 表现为:2008年1月强极涡发生之后, 500 hPa行星波1波和2波的扰动都向南伸, 而2009年1月的弱极涡(SSW)期间和之后, 1波和2波的扰动都偏北; 在对流层, 强极涡和弱极涡发生之后不但行星波1波和2波的振幅有所差异, 其位相也有明显的不同。特别是, 其位相的差异还随纬度而变化。就同一年(或者说对于同是强极涡或者同是弱极涡)而言, 无论是1波还是2波, 在60°N和30°N附近的扰动相比, 几乎反位相。这样就使得它们的500 hPa 位势场也有明显不同:在东半球, 主要表现为乌拉尔高压和东亚大槽的强度和位置不同。2008年1月强极涡发生之后, 乌拉尔高压和东亚大槽东移, 不利于冷空气向欧亚大陆北部(包括我国北方)的输送, 使这些地区的温度偏高;而2009年1月弱极涡之后, 东亚大槽西退, 利于冷空气向欧亚大陆北部输送, 导致这些地区较冷。对于同一种极涡异常(如2008强极涡或者2009弱极涡)由于南方和北方行星波扰动的位相不同, 对南方和北方冷暖空气的输送也就不一样。所以同一种极涡异常对(我国)南北地区的温度影响是不同的。     

Continuous Ozone Depletion over Antarctica After 2000 and Its Relationship with the Polar Vortex

Observations have shown highly variable ozone depletion over the Antarctic in the 2000s, which could affect the long-term ozone trend in this region as well as the global ozone recovery. By using the total column ozone data （1979-2011）, interannual variation of the springtime Antarctic ozone tow is investigated, together with its relationship with the polar vortex evolution in the lower stratosphere. The results show that springtime Antarctic ozone depletion has continued in the 2000s, seemingly contradicting the consensus view of a global ozone recovery expected at the beginning of the 21st century. The spring Antarctic polar vortex in the lower stratosphere is much stronger in the 2000s than before, with a larger area, delayed breakup time, and greater longevity during 2000-2011. Fhrther analyses show that the recent continuation of springtime Antarctic ozone depletion could be largely attributed to the abnormal variation of the Antarctic polar vortex.     

The exceptionally strong and persistent Arctic stratospheric polar vortex in the winter of 2019–2020: 2019-2020冬季北半球超强极涡事件

The Arctic stratospheric polar vortex was exceptional strong, cold and persistent in the winter and spring of 2019–2020. Based on reanalysis data from the National Centers for Environmental Prediction/National Center for Atmospheric Research and ozone observations from the Ozone Monitoring Instrument, the authors investigated the dynamical variation of the stratospheric polar vortex during winter 2019–2020 and its influence on surface weather and ozone depletion. This strong stratospheric polar vortex was affected by the less active upward propagation of planetary waves. The seasonal transition of the stratosphere during the stratospheric final warming event in spring 2020 occurred late due to the persistence of the polar vortex. A positive Northern Annular Mode index propagated from the stratosphere to the surface, where it was consistent with the Arctic Oscillation and North Atlantic Oscillation indices. As a result, the surface temperature in Eurasia and North America was generally warmer than the climatology. In some places of Eurasia, the surface temperature was about 10 K warmer during the period from January to February 2020. The most serious Arctic ozone depletion since 2004 has been observed since February 2020. The mean total column ozone within 60°–90°N from March to 15 April was about 80 DU less than the climatology.摘要2019-2020冬季北极平流层极涡异常并且持续的偏强,偏冷.利用NCEP再数据和OMI臭氧数据, 本文分析了此次强极涡事件中平流层极涡的动力场演变及其对地面暖冬天气和臭氧低值的影响.此次强极涡的形成是由于上传行星波不活跃.持续的强极涡使得2020年春季的最后增温出现时间偏晚.平流层正NAM指数向下传播到地面, 与地面AO指数和NAO指数相一致, 欧亚大陆和北美地面气温均比气候态偏暖, 在欧亚大陆的一些地区, 2020年1月和2月的气温甚至偏高了10K.2020年2月以来北极臭氧出现了2004年以来的最低值, 2020年3-4月60°–90°N的平均臭氧柱总量比气候态偏低了80DU.     

Interaction of atmospheric chemistry and climate and its impact on stratospheric ozone

The interactively coupled chemistry-climate model ECHAM4.L39(DLR)/CHEM is employed in sensitivity calculations to investigate feedback mechanisms of dynamic, chemical, and radiative processes. Two multi-year model simulations are carried out, which represent recent atmospheric conditions. It is shown that the model is able to reproduce observed features and trends with respect to dynamics and chemistry of the troposphere and lower stratosphere. In polar regions it is demonstrated that an increased persistence of the winter vortices is mainly due to enhanced greenhouse gas mixing ratios and to reduced ozone concentration in the lower stratosphere. An additional sensitivity simulation is investigated, concerning a possible future development of the chemical composition of the atmosphere and climate. The model results in the Southern Hemisphere indicate that the adopted further increase of greenhouse gas mixing ratios leads to an intensified radiative cooling in the lower stratosphere. Therefore, Antarctic ozone depletion slightly increases due to a larger PSC activity, although stratospheric chlorine is reduced. Interestingly, the behavior in the Northern Hemisphere is different. During winter, an enhanced activity of planetary waves yields a more disturbed stratospheric vortex. This "dynamical heating" compensates the additional radiative cooling due to enhanced greenhouse gas concentrations in the polar region. In connection with reduced stratospheric chlorine loading, the ozone layer clearly recovers.     

Link between Arctic ozone and the stratospheric polar vortex

The stratospheric ozone layer protects life on earth by preventing solar ultraviolet radiation from reaching the surface. Owing to the large population in the Northern Hemisphere and extreme ozone loss in the Arctic, changes in Arctic stratospheric ozone (ASO) and their causes have attracted broad attention recently. Using monthly mean data during the period 1980–2020 from MERRA-2, the relationship between the stratospheric polar vortex (SPV) and ASO, along with the relative contributions of chemical and dynamic processes associated with the SPV to changes in ASO, were examined in this study. Results showed that the ASO in March has a strong out-of-phase link with the strength of the SPV in March, with no obvious lead–lag correlations, i.e., an increase (decrease) in ASO corresponds to a weakened (strengthened) SPV. Further analysis suggested that the strong out-of-phase link between the SPV and ASO is related to changes in Brewer–Dobson circulation (BDC). Strong SPV events, accompanied by a low temperature condition and weakened upward propagation of planetary waves over the Arctic in the stratosphere, result in weakened BDC. The weakened downwelling at high latitudes tends to transport less ozone-rich air in the upper stratosphere at lower latitudes into the lower stratosphere at high latitudes, facilitating a decrease in ASO. The BDC's vertical velocity plays the dominant role in modulating ASO.摘要利用1980–2020年MERRA-2资料, 分析了平流层极涡 (Stratospheric polar vortex, SPV) 和北极臭氧 (Arctic stratospheric ozone, ASO) 的关系, 评估了与SPV相关的化学, 动力过程在其中的相对作用. 结果表明, 3月份ASO与同期SPV强度反相关最大. SPV-ASO二者反相关与平流层剩余环流 (Brewer-Dobson circulation, BDC) 变化密切相关. 强SPV伴随的北极平流层低温条件和行星波向上传播减弱, 导致BDC减弱, 减弱的BDC下沉支将低纬度平流层上层臭氧含量较低的空气输送到北极平流层低层, 从而导致ASO减少. BDC垂直速度在其中起主导作用.     

Overview of the Major 2012-2013 Northern Hemisphere Stratospheric Sudden Warming：Evolution and Its Association with Surface Weather

In this study, we analyzed the dynamical evolution of the ma jor 2012-2013 Northern Hemisphere （NH） stratospheric sudden warming （SSW） on the basis of ERA-Interim reanalysis data provided by the ECMWF. The intermittent upward-propagating planetary wave activities beginning in late November 2012 led to a prominent wavenumber-2 disturbance of the polar vortex in early December 2012. However, no major SSW occurred. In mid December 2012, when the polar vortex had not fully recovered, a mixture of persistent wavenumber-1 and -2 planetary waves led to gradual weakening of the polar vortex before the vortex split on 7 January 2013. Evolution of the geopotential height and Eliassen-Palm flux between 500 and 5 hPa indicates that the frequent occurrence of tropospheric ridges over North Pacific and the west coast of North America contributed to the pronounced upward planetary wave activities throughout the troposphere and stratosphere. After mid January 2013, the wavenumber-2 planetary waves became enhanced again within the troposphere, with a deepened trough over East Asia and North America and two ridges between the troughs. The enhanced tropospheric planetary waves may contribute to the long-lasting splitting of the polar vortex in the lower stratosphere. The 2012-2013 SSW shows combined features of both vortex displacement and vortex splitting. Therefore, the anomalies of tropospheric circulation and surface temperature after the 2012-2013 SSW resemble neither vortex-displaced nor vortex-split SSWs, but the combination of all SSWs. The remarkable tropospheric ridge extending from the Bering Sea into the Arctic Ocean together with the resulting deepened East Asian trough may play important roles in bringing cold air from the high Arctic to central North America and northern Eurasia at the surface.     

北半球冬季平流层温度和Brewer-Dobson环流对11 a太阳循环的响应

采用北京气候中心大气辐射模式(BCC-RAD)、日本气象厅JRA-55月平均再分析资料,研究了北半球冬季低纬度平流层上、下两个温度异常区对太阳周期的响应及其机制。结果表明,太阳活动偏强年,低纬度的上平流层温度暖异常是由臭氧短波加热异常引起的,它在中纬度的上平流层激发出异常强西风,阻碍行星波正常上传,由波破碎驱动的Brewer-Dobson环流也减弱,该环流上升支减弱的动力加热作用导致了低纬度的下平流层暖异常。     

A Study of Ozone Laminae Using Diabatic Trajectories, Contour Advection and Photochemical Trajectory Model Simulations.

In this paper, we show that the rate of ozone loss in both polar and mid-latitudes, derived from ozonesonde and satellite data, has almost the same vertical distribution (although opposite sense) to that of ozone laminae abundance. Ozone laminae appear in the lower stratosphere soon after the polar vortex is established in autumn, increase in number throughout the winter and reach a maximum abundance in late winter or spring. We indicate a possible coupling between mid-winter, sudden stratospheric warmings (when the vortex is weakened or disrupted) and the abundance of ozone laminae using a 23-year record of ozonesonde data from the World Ozone Data Center in Canada combined with monthly-mean January polar temperatures at 30 hPa.Results are presented from an experiment conducted during the winter of 1994/95, in phase II of the Second European Stratospheric And Mid-latitude Experiment (SESAME), in which 93 ozone-enhanced laminae of polar origin observed by ozonesondes at different time and locations are linked by diabatic trajectories, enabling them to be probed twice or more. It is shown that, in general, ozone concentrations inside laminae fall progressively with time, mixing irreversibly with mid-latitude air on time-scales of a few weeks. A particular set of laminae which advected across Europe during mid February 1995 are examined in detail. These laminae were observed almost simultaneously at seven ozonesonde stations, providing information on their spatial scales. The development of these laminae has been modelled using the Contour Advection algorithm of Norton (1994), adding support to the concept that many laminae are extrusions of vortex air. Finally, a photochemical trajectory model is used to show that, if the air in the laminae is chemically activated, it will impact on mid-latitude ozone concentrations. An estimate is made of the potential number of ozone molecules lost each winter via this mechanism.     

一次寒潮降温过程的等熵位涡和热力学分析

通过等熵位涡和热力学能量方程的各项诊断对2018年1月上旬我国东部一次寒潮天气过程进行分析,重点给出垂直运动在寒潮降温中的作用。结果表明：此次寒潮天气过程主要受蒙古国南部的横槽转竖影响,巴尔喀什湖东部和西伯利亚地区及其北部为引起这次寒潮的主要冷空气源地。欧亚大陆北部和极区对流层高层和平流层低层的高位涡强冷空气沿着等熵面向南向下平流,引导强冷空气侵袭我国东部。等熵位涡大值区的东侧对应上升运动区,有利于降水的产生。寒潮期间风场平流引起的850 hPa强降温区主要位于东南沿海地区,降温幅度最高可达6×10^-4 K·s^-1,而东北地区在整个寒潮期间冷平流强度较弱,最大降温幅度仅约为1×10^-4 K·s^-1。通过计算东南沿海和东北地区区域平均风场平流和垂直运动引起850 hPa温度变化,得出寒潮期间两地的温度总降幅约为1×10^-4 K·s^-1。东南沿海地区的寒潮主要由风场的冷平流引起,而东北地区则是由冷平流和垂直上升运动的共同作用引起。垂直方向上,东北地区冷空气能影响的高度要远高于东南沿海地区。     

Decadal Variation of the Impact of La Niña on the Winter Arctic Stratosphere

The impact of La Ni?a on the winter Arctic stratosphere has thus far been an ambiguous topic of research. Contradictory results have been reported depending on the La Ni?a events considered. This study shows that this is mainly due to the decadal variation of La Ni?a's impact on the winter Arctic stratosphere since the late 1970 s. Specifically,during the period1951–78,the tropospheric La Ni?a teleconnection exhibits a typical negative Pacific–North America pattern,which strongly inhibits the propagation of the planetary waves from the extratropical troposphere to the stratosphere,and leads to a significantly strengthened stratospheric polar vortex. In contrast,during 1979–2015,the La Ni?a teleconnection shifts eastwards,with an anomalous high concentrated in the northeastern Pacific. The destructive interference of the La Ni?a teleconnection with climatological stationary waves seen in the earlier period reduces greatly,which prevents the drastic reduction of planetary wave activities in the extratropical stratosphere. Correspondingly,the stratospheric response shows a less disturbed stratospheric polar vortex in winter.     

Chemistry–Climate Interactions of Stratospheric and Mesospheric Ozone in EMAC Long-Term Simulations with Different Boundary Conditions for CO2, CH4, N2O,and ODS

Abstract

To evaluate future climate change in the middle atmosphere and the chemistry–climate interaction of stratospheric ozone, we performed a long-term simulation from 1960 to 2050 with boundary conditions from the Intergovernmental Panel on Climate Change A1B greenhouse gas scenario and the World Meteorological Organization Ab halogen scenario using the chemistry–climate model ECHAM5/MESSy Atmospheric Chemistry (EMAC). In addition to this standard simulation we performed five sensitivity simulations from 2000 to 2050 using the rerun files of the simulation mentioned above. For these sensitivity simulations we used the same model setup as in the standard simulation but changed the boundary conditions for carbon dioxide (CO₂), methane (CH₄), nitrous oxide (N₂O), and ozone-depleting substances (ODS). In the first sensitivity simulation we fixed the mixing ratios of CO₂, CH₄, and N₂O in the boundary conditions to the amounts for 2000. In each of the four other sensitivity simulations we fixed the boundary conditions of only one of CO₂, CH₄, N₂O, or ODS to the year 2000.

In our model simulations the future evolution of greenhouse gases leads to significant cooling in the stratosphere and mesosphere. Increasing CO₂ mixing ratios make the largest contributions to this radiative cooling, followed by increasing stratospheric CH₄, which also forms additional H₂O in the upper stratosphere and mesosphere. Increasing N₂O mixing ratios makes the smallest contributions to the cooling. The simulated ozone recovery leads to warming of the middle atmosphere.

In the EMAC model the future development of ozone is influenced by several factors. 1) Cooler temperatures lead to an increase in ozone in the upper stratosphere. The strongest contribution to this ozone production is cooling due to increasing CO₂ mixing ratios, followed by increasing CH₄. 2) Decreasing ODS mixing ratios lead to ozone recovery, but the contribution to the total ozone increase in the upper stratosphere is only slightly higher than the contribution of the cooling by greenhouse gases. In the polar lower stratosphere a decrease in ODS is mainly responsible for ozone recovery. 3) Higher NO_x and HO_x mixing ratios due to increased N₂O and CH₄ lead to intensified ozone destruction, primarily in the middle and upper stratosphere, from additional NO_x; in the mesosphere the intensified ozone destruction is caused by additional HO_x. In comparison to the increase in ozone due to decreasing ODS, ozone destruction caused by increased NO_x is of similar importance in some regions, especially in the middle stratosphere. 4) In the stratosphere the enhancement of the Brewer-Dobson circulation leads to a change in ozone transport. In the polar stratosphere increased downwelling leads to additional ozone in the future, especially at high northern latitudes. The dynamical impact on ozone development is higher at some altitudes in the polar stratosphere than the ozone increase due to cooler temperatures. In the tropical lower stratosphere increased residual vertical upward transport leads to a decrease in ozone.