从紫外到中红外谱区冰的光学常数与温度关系的研究

本文简要地讨论了冰的结构及其光学特性,并应用经典的极化理论研究了冰的光学常数与频谱和温度的关系,计算了从紫外到中红外谱区、在地球大气温度范围内冰的光学常数。对计算结果的分析表明,在高空卷云的散射和辐射传输的理论计算中,温度对云中冰晶光学常数的影响必须考虑。     

A case study of cirrus layers with variable 3.74 µm reflection properties in the first FIRE experiment, 2 November 1986

Summary Remotely sensed scanning radiometer and lidar data on cirrus clouds were obtained during the cirrus FIRE IFO experiment in November 1986 from the ER-2 aircraft plat-form.Data were examined particularly on 2 November for an area in the vicinity of Wausau, Wisconsin where unusual effects were noticed in bispectral histograms from various channels in the scanner data.After calibration of the data in spectral channels of both the Scan Cloud Radiometer (SCR) and Multichannel Cloud Radiometer (MCR) instruments, including direct comparison between compatible channels in the two instruments, it was found that the 0.856 µm SCR channel gave good data, whereas the 0.665 µm and 0.74 µm SCR channels gave large offsets, when compared with the MCR 0.754 µm data. The latter channel was found to compare well in a second comparison with coincident AVHRR channel satellite data. Similarly, the SCR 11.17 µm data gave consistent results and the SCR 3.74 µm data were carefully calibrated.Bispectral histograms formed between 0.856 µm, 3.74 µm and 11.17 µm SCR channel data indicated that some coherent layers of cirrus clouds were giving enhanced solar reflectance at 3.74 µm, indicative of small (~ <25 µm radius) particles, whereas other neighbouring layers gave little reflectance.A comparison of 0.856 µm reflections with 11.17 µm absorption optical depth indicated that the small particles where probably ice crystals. A comparison of 3.74 µm solar albedo and 11.17 µm absorption optical depths of these layers with theoretical calculations for ice spheres indicated a mode radius of about 8 µm for the cloud particle size distribution. An estimate from similar recent calculations on hexagonal ice crystals indicated that the retrieved effective radius would be increased to 25 µm. The difference between the two retrieved radii was a measure of the uncertainty in the retrievals, considering also differences in the assumed size distributions.Qualitative comparison with ER-2 lidar data gave a tentative identification of the reflecting layers.The results demonstrate the power of the 3.74 µm channel for identification of small-particle layers in cirrus.With 9 Figures     

Average ice crystal size and bulk short-wave single-scattering properties of cirrus clouds

The bulk single-scattering properties of cirrus clouds required for driving the radiation scheme in large-scale climate models are computed with respect to various size distributions and ice crystal shapes. It is shown that the average ice crystal size, defined as the ratio of total volume to the total projected area, can well-characterize the effect of various size distributions in determining the bulk radiative properties of cirrus clouds. Details of the size distributions are not significant in specifying the radiative properties of these clouds if the effective average size is thus defined. Therefore, the ratio of the total volume to the total projected area is an ideal parameter for describing the bulk single-scattering properties. The effect of ice crystal shape is not critical in the parameterization of the extinction coefficient and single-scattering albedo. However, the various crystal habits must be accounted for in the parameterization of the asymmetry parameter. The resulting parameterization is intended for radiative transfer calculations involving cirrus clouds in large-scale models.     

Ice cloud microphysics,radiative transfer and large-scale cloud processes

Summary Parameterization programs for cloud microphyscs and radiative transfer involving ice clouds have been developed in terms of the mean effective size and ice water path. The mean effective size appears to be adequate in representing the ice crystal size distribution for radiative parameterizations. For a given ice water path, smaller mean effective sizes reflect more solar radiation, emit more IR radiation and enhance net radiative heating/cooling at the cloud top and bottom than larger sizes. The presence of small ice crystals may generate steeper lapse rates in clouds. A 3-D global cloud model that prescribes the horizontal wind fields in a 24 hour period is used to investigate the sensitivity of the mean effective size of ice crystals on the simulation of radiative heating, temperature, cloud cover and ice water content. A variation in the mean effective size from 75 to 50 m in a 24 hour prediction on simulation generates more cooling above the high cloud top and a decrease of temperature. These results lead to an increase of high cloud cover in some latitudes by as much as 4% and, at the same time, a decrease of middle cloud cover by 3–4% in latitudes between 60°S and 60°N.With 7 Figures     

Ice microphysics and climatic temperature feedback

The potential effects of ice microphysics involving ice crystal size distribution and ice water path (IWP) on climatic temperature perturbations are investigated by using a one-dimensional radiative-turbulent climate model. We define a mean effective size, denoting the width of ice crystals weighted by the geometric cross section area, to represent ice crystal size distribution. Based on aircraft measurements, both the mean effective size and IWP are related to temperature and may be parameterized as functions of temperature. The radiative properties of cirrus clouds are further parameterized in terms of these two basic cloud physics parameters. Using CO₂ doubling as the radiative forcing, feedbacks among temperature, the mean effective size and IWP, and the radiative properties of clouds are analyzed from the model results. We show that overall, a positive feedback associated with ice microphysics and the coupled radiative transfer is produced by temperature increase.     

Determination of cirrus radiative parameters from combination between active and passive remote sensing measurements during FRENCH/DIRAC 2001

In the context of the next AQUA Train satellite experiment, airborne measurements were carried out to simulate satellite measurements. They were conducted between September 25 and October 12, 2001, off the coast of southern France over the Atlantic Ocean and over the Mediterranean Sea, respectively. During the intensive Field Radiation Experiment on Natural Cirrus and High-level clouds (FRENCH/DIRAC 2001), natural ice clouds were sampled from in situ and remote sensing measurements. On October 5 and 7, 2001, cirrus cloud decks were described by a complete data set acquired by: (i) in situ microphysical instruments onboard the TBM-700 aircraft: PMS probe, and Polar Nephelometer (ii) and downward-looking radiative instruments onboard the Mystère 20 aircraft: an infrared radiometer, a lidar, a visible imager with polarisation capabilities, and a middle infrared radiometer. Moreover, classical thermodynamical measurements were carried out onboard the Mystère 20. Mean microphysical characteristics of cirrus deck are derived from interpretation of remote sensing measurements. These properties are compared with those derived from in situ microphysical measurements in order to evaluate the radiative impact of natural cirrus clouds.     

Remote sensing of cloud liquid water

Summary A method is presented to infer cloud liquid water path (LWP in kg/m²) over the ocean from passive microwave measurements of SSM/I. The algorithm to retrieve LWP is based on simulated satellite observations. They are calculated with a radiative transfer model applied to about 3000 radiosonde ascents over the Atlantic Ocean. Since radiosonde observations do not contain direct information about cloud water and ice, these parameters are parameterized based on relative humidity and temperature using modified adiabatic liquid water density profiles. A multiple linear regression is applied to the simulated radiances and the calculated LWP to derive the algorithm. The retrieval accuracy based on the regression analysis including instrumental noise is 0.03 kg/m². Validation of the LWP-algorithm was pursued through a comparison with measurements of a ground-based 33 GHzmicrowave radiometer on board of R.V. Poseidon during the International Cirrus Experiment 1989 at the North Sea (ICE'89). The LWP values agree within the range of uncertainty caused by the different sampling characteristics of the observing systems. The retrieval accuracy for clear-sky cases determined using colocated METEOSAT data over the North Sea is 0.037 kg/m² and confirms the accuracy estimated from regression analysis for the low liquid water cases.The algorithm was used to derive maps of monthly mean LWP over the Atlantic Ocean. As an example the Octobers of the 5 years 1987–1991 were selected to demonstrate the interannual variability of LWP. The results were compared with the cloud water content produced by the climate model ECHAM-T2 from the Max-Planck-Institut Hamburg.Observations during ICE'89 were used to check the accuracy of the applied radiative transfer model. Brightness temperatures were calculated from radiosonde ascents launched during the overpass of DMSP-F8 in cloud-free situations. The channel-dependent differences range from about –2 to 3 K.The possibility to identify different cloud types using microwave and infrared observations was examined. The main conclusion is that simultaneous microwave and infrared measurements enable the separation of dense cirrus and cirrus with underlying water clouds. A classification of clouds with respect to their top heights and LWP was carried out using a combination of SSM/I derived LWP and simultaneously recorded Meteosat IR-data during ICE'89.With 11 Figures     

Lidar remote sounding of cirrus clouds and comparison of simulated fluxes with surface and METEOSAT observations

Three cirrus cloud cases have been remotely sounded near Paris by a ground-based backscatter lidar and broadband radiometers. Some cirrus properties (optical depth, emissivity, height) are derived from these measurements and used to compare radiative transfer calculations to surface and METEOSAT observations of broadband irradiances.For a useful comparison, the three cirrus cases were selected to have different morphologies and optical properties: June 29, 1993—thin cirrus cloud (thickness 1.5 km, optical depth 0.22); September 6, 1993—thick cirrus cloud (thickness 5 km, optical depth 2.7); and November 16, 1993—inhomogeneous and geometrically thick cirrus cloud (thickness 3.5–6.5 km) but optically thin (optical depth 0.82).At surface, the differences between measurements and model range from 1.5 to 4 Wm⁻² for longwave fluxes, and from 20 to 70 Wm⁻² for shortwave fluxes.At the top of the atmosphere, the differences between METEOSAT measurements and model are in fair agreement for longwave fluxes (up to 50 Wm⁻²). However, unexpected high differences are found for shortwave fluxes (up to 144 Wm⁻²) due to cirrus clouds heterogeneities and uncertainties in their microphysical properties and especially the occurrence of high reflectivity due to horizontally oriented ice crystals at the cloud top, which are not taken into account by the Model presently.     

Sensitivity Study of Anthropogenic Aerosol Indirect Forcing through Cirrus Clouds with CAM5 Using Three Ice Nucleation Parameterizations

Quantifying the radiative forcing due to aerosol–cloud interactions especially through cirrus clouds remains challenging because of our limited understanding of aerosol and cloud processes. In this study, we investigate the anthropogenic aerosol indirect forcing (AIF) through cirrus clouds using the Community Atmosphere Model version 5 (CAM5) with a state-of-the-art treatment of ice nucleation. We adopt a new approach to isolate anthropogenic AIF through cirrus clouds in which ice nucleation parameterization is driven by prescribed pre-industrial (PI) and presentday (PD) aerosols, respectively. Sensitivities of anthropogenic ice AIF (i.e., anthropogenic AIF through cirrus clouds) to different ice nucleation parameterizations, homogeneous freezing occurrence, and uncertainties in the cloud microphysics scheme are investigated. Results of sensitivity experiments show that the change (PD minus PI) in global annual mean longwave cloud forcing (i.e., longwave anthropogenic ice AIF) ranges from 0.14 to 0.35 W m^–2, the change in global annual mean shortwave cloud forcing (i.e., shortwave anthropogenic ice AIF) from–0.47 to–0.20 W m^–2, and the change in net cloud forcing from–0.12 to 0.05 W m^–2. Our results suggest that different ice nucleation parameterizations are an important factor for the large uncertainty of anthropogenic ice AIF. Furthermore, improved understanding of the spatial and temporal occurrence characteristics of homogeneous freezing events and the mean states of cirrus cloud properties are also important for constraining anthropogenic ice AIF.     

Correlations between microphysical properties of large-scale semi-transparent cirrus and the state of the atmosphere

By making use of TOVS Path-B satellite retrievals and ECMWF reanalyses, correlations between bulk microphysical properties of large-scale semi-transparent cirrus (visible optical thickness between 0.7 and 3.8) and thermodynamic and dynamic properties of the surrounding atmosphere have been studied on a global scale. These clouds constitute about half of all high clouds. The global averages (from 60°N to 60°S) of mean ice crystal diameter, D_e, and ice water path (IWP) of these clouds are 55 μm and 30 g m⁻², respectively. IWP of these cirrus is slightly increasing with cloud-top temperature, whereas D_e of cold cirrus does not depend on this parameter. Correlations between D_e and IWp of large-scale cirrus seem to be different in the midlatitudes and in the tropics. However, we observe in general stronger correlations between D_e and IWP and atmospheric humidity and winds deduced from the ECMWF reanalyses: D_e and IWP increase both with increasing atmospheric water vapour. There is also a good distinction between different dynamical situations: In humid situations, IWP is on average about 10 gm⁻² larger in regions with strong large-scale vertical updraft only that in regions with strong large-scale horizontal winds only, whereas the mean D_e of cold large-scale cirrus decreases by about 10 μm if both strong large-scale updraft and horizontal winds are present.     

Characteristics of cirrus clouds and its radiative properties based on lidar observation over Chung-Li, Taiwan

In this paper, characterization of cirrus clouds are made by using data from ground based polarization lidar and radiosonde measurements over Chung-Li (24.58°N, 121.10°E), Taiwan for a period of 1999–2006. During this period, the occurrence of cirrus clouds is about 37% of the total measurement nights over the lidar site. Analysis of the measurement gives the statistical characteristics about the macrophysical properties such as occurrence height, ambient temperature, and its geometrical thickness while the microphysical properties are interpreted in terms of extinction coefficient, optical depth, effective lidar ratio and depolarization ratio. The effective lidar ratio has been retrieved by using the simulation technique of backscattered lidar signals. The effect of multiple scattering has been taken into the account by a model calculation. Summer (Jun–Aug) shows the maximum appearances of cirrus due to its formation mechanism. It is shown that tropopause cirrus clouds may occur with a probability of about 24%. These clouds are usually optically thin and having laminar in structure with some cases resembling the characteristics similar to that of polar stratospheric clouds (PSCs). The radiative properties of the cirrus clouds are also discussed in detail by the empirical equations with results show a positive feedback on any climate change.     

Short-wave radiation flux divergence in arctic cirrus: a case study

Radiation and particle measurements have been performed with an aircraft in deep cirrus cloud fields near the island of Svalbard. The data of 12 March 1993, when measurements at 10 different levels could be obtained, are used in a comparative study with radiative transfer calculations. In a first analysis, the cirrus cloud field was assumed to be horizontally homogeneous and invariable during the time of measurements (frozen properties). Calculations of the up and downward radiative flux densities showed root mean square differences of 9 Wm⁻² from the measurements. To estimate the possible effect of changes of the optical properties of cirrus with time, the flux densities in the upper part (6000–8500 m) and the lower part (3000–5500 m) of the cirrus cloud were analyzed separately. In these simulations, the optical thickness in the lower (upper) part was increased (decreased) by 50%. By this treatment, most of all calculated flux densities were within one standard deviation of the natural variability in each leg. Finally, the effect of inhomogeneities in the cloud field on the solar flux density has been simulated using a Monte Carlo method, since the upper part of the cirrus field has indeed been very inhomogeneous. This paper is a result of a collaborative effort between the MRI in Tsukuba, Japan, and the GKSS in Geesthacht, Germany.     

Airborne and lidar measurements of aerosol and cloud particles in the troposphere over Alert Canada in April 1986

As a component of the Canadian Arctic Haze Study, held coincident with the second Arctic Gas and Aerosol Sampling Program (AGASP II), vertical profiles of aerosol size distribution (0.17 m), light scattering parameters and cloud particle concentrations were obtained with an instrumented aircraft and ground-based lidar system during April 1986 at Alert. Northwest Territories. Average aerosol number concentrations range from about 200 cm^–3 over the Arctic ice cap to about 100 cm^–3 at 6 km. The aerosol size spectrum is virtually free of giant or coarse aerosol particles, and does not vary significantly with altitude. Most of the aerosol volume is concentrated in the 0.17–0.50 m size range, and the aerosol number concentration is found to be a good surrogate for the SO₄ ⁼ concentration of the Arctic haze aerosol. Comparison of the aircraft and lidar data show that, when iced crystal scattering is excluded, the aerosol light scattering coefficient and the lidar backscattering coefficient are proportional to the Arctic haze aerosol concentration. Ratios of scattering to backscattering, scattering to aerosol number concentration, and backscattering to aerosol number concentration are 15.3 steradians, 1.1×10^–13 m², and 4.8×10^–15 m² sr^–1, respectively. Aerosol scattering coefficients calculated from the measured size distributions using Mie scattering agree well with measured values. The calculations indicate the aerosol absorption optical depth over 6 km to range between 0.011 and 0.018. The presence of small numbers of ice crystals (10–20 crystals 1^–1 measured) increased light scattering by over a factor of ten.     

Effects of horizontal orientation on the radiative properties of ice clouds

Transfer of radiation through cirrus consisting of non-sphericalice crystals randomly oriented in a plane (2D model) is solved by using the discrete-ordinates method. The model is employed to determine the radiative flux properties and the intensity distribution of cirrus for both solar and thermal infrared ra-diation. Comparison of the 2D cloud model with the conventional 3D cloud model, i.e., randomly oriented in a three- dimensional space, shows that the preferential orientation of ice crystals has a substantial effect on the cloud solar albedo. The difference in the cloud albedo computed from the two models can be as large as 8% for a cirrus of 2 km thickness. On the thermal infrared side, although the flux emission for cirrus is less affected by the orientation of ice crystals, the difference in the upward radiance using 2D and 3D models is also significant.     

Ice crystal shape effects on solar radiative properties of Arctic mixed-phase clouds—Dependence on microphysical properties

Based on 1-year cloud measurements with radar and microwave radiometer broadband solar radiative transfer simulations were performed to quantify the impact of different ice crystal shapes of Arctic mixed-phase clouds on their radiative properties (reflectance, transmittance and absorptance). The ice crystal shape effects were investigated as a function of microphysical cloud properties (ice volume fraction f_i, ice and liquid water content IWC and LWC, mean particle diameter D_m^I and D_m^W of ice/water particle number size distributions, NSDs).The required NSDs were statistically derived from radar data. The NSD was composed of a liquid and a solid mode defined by LWC, D_m^W (water mode) and IWC, D_m^I (ice mode). It was found that the ratio of D_m^I and D_m^W determines the magnitude of the shape effect. For mixed-phase clouds with D_m^I ≤ 27 μm a significant shape effect was obtained. The shape effect was almost insensitive with regard to the solar zenith angle, but highly sensitive to the ice volume fraction of the mixed-phase cloud. For mixed-phase clouds containing small ice crystals (D_m^I ≤ 27 μm) and high ice volume fractions (f_i > 0.5) crystal shape is crucial. The largest shape effects were observed assuming aggregates and columns. If the IWC was conserved the shape effect reaches values up to 0.23 in cloud reflectance and transmittance. If the ice mode NSD was kept constant only a small shape effect was quantified (≤ 0.04).     

用红外和水汽两个通道的卫星测值指定云迹风的高度

提出了一种改进的用红外和水汽两个通道的测值指定云迹风高度的算法。利用红外水汽散点图和云迹风本身自动地将有低云的目标区、有半透明卷云的目标区、有密蔽高云的目标区分开。在有低云的目标区和有密蔽高云的目标区用红外一个通道指定云高。在有半透明卷云的目标区用红外和水汽两个通道指定云高。在用两个通道的测值指定云高时，假定卷云高度以上不存在水汽，以红外和水汽两个通道亮温相同这个方程与两个通道辐射测值线性相关的方程联立解出云的高度     

The microstructure of selected, small, isolated, cumulus clouds near Red Deer, Alberta

Physical experiments designed to explore the potential of rain augmentation through airborne glaciogenic seeding on small, isolated non-precipitating cumuliform clouds near Red Deer, Alberta were carried out during the period 1982–1985. The microstructure of 90 cumulus congestus clouds have been documented through repeated in-situ sampling using a cloud physics instrumented aircraft platform. Observations from the inspection passes of 57 clouds seeded with either dry ice pellets or silver iodide pyrotechnics, and all the passes of 33 natural clouds are presented.Measurements of the cloud droplet concentration indicate that Alberta cumulus clouds are typically continental in nature, with an average droplet concentration of 535 cm⁻³ and an average droplet diameter of 10.6 μm. Alberta clouds have average liquid water contents of 0.57 g m⁻³, with a peak 1-sec value of 3.17 g m⁻³. The 1-km average liquid water contents are 0.83 g m⁻³, with a peak value of 2.81 g m⁻³. Cloud lifetimes vary between 11 and 20 minutes. Concentrations of naturally occurring ice crystals are found to be low. The average maximum 1-km ice concentration was 31⁻¹, and the peak 1-km concentration was 73.11⁻¹ in the natural cloud dataset. Evidence of precipitation-sized particles was detected in 21% (7 of 33) of the clouds, and precipitation below cloud base was detected in 6% (2 of 33) of the clouds.A comparison of the Alberta cloud characteristics to the cumulus clouds from different locations showed that there are some distinct differences between Alberta clouds and the clouds from the other regions.     

Cirrus Cloud Macrophysical and Optical Properties over North China from CALIOP Measurements

Two years of mid-latitude cirrus cloud macrophysical and optical properties over North China are described from Earth-orbiting Cloud-Aerosol Lidar with Orthogonal Polarization(CALIOP) satellite measurements. Global cloud climatological studies based on active remote sensing data sets benefit from more accurate resolution of vertical structure and more reliable detection of optically thin layers.The mean values for cirrus cases over North China are 0.19±0.18 for infrared emittance,0.41±0.68 for visible optical depth, 0.26±0.12 for integrated depolarization ratio,and 0.72±0.22 for integrated color ratio.When studied using reasonable assumptions for the relationship between extinction and ice crystal backscatter coefficients,our results show that most of the cirrus clouds profiled using the 0.532μm channel data stream correspond with an optical depth of less than 1.0.The dependence of cirrus cloud properties on cirrus cloud mid-cloud temperature and geometry thickness are generally similar to the results derived from the ground-based lidar, which are mainly impacted by the adiabatic process on the ice cloud content.However,the differences in macrophysical parameter variability indicate the limits of spaceborne-lidar and dissimilarities in regional climate variability and the nature and source of cloud nuclei in different geographical regions.     

冰晶性质对卷云辐射特征影响的模拟研究

介绍了SBDART辐射模式和libRadtran程序包，并利用这两个模式模拟分析了当卷云内冰晶性质如有效半径、冰晶含量以及形状变化时，卷云反照率的变化。模拟分析表明，在相同条件下，不同形状冰晶构成的卷云反照率有所不同，同种冰晶构成的卷云在不同波长的反照率也不同。总的来说，不论是由何种形状冰晶构成的卷云，随着卷云内冰晶含量增大，有效半径减小，卷云反照率增大。这些工作将有助于增进对lib Radtran程序包和卷云性质的了解。     

Satellite-derived outgoing longwave radiation,surface temperature and sea ice concentration off the coast of Adélie-Land,Eastern Antarctica

Summary Outgoing longwave radiation (OLR) as seen from satellite (NOAA-series), and sea ice concentration in Mer Dumont d'Urville, Eastern Antarctica were analyzed. For the time period 1974–1990 available radiative flux data showed a slight increase of 1.8 W/m² or 1% for the period. If thistrend should continue — trends over a 16-year period in any geophysical data is a rather questionable concept in isolation — a 4°C warming would be observed from space for this polar region over a century. The observed increase is, however, in agreement with Dumont d'Urville, the only ground station within the study area, which displayed a similar temperature increase (Periard and Pettré, 1991). Further it is in agreement with the general temperature increase which has been observed for the high southern latitudes (Boden et al., 1990). In addition, models of climatic change due to increased CO₂ and other trace gases predict for polar regions values of similar size.Sea ice concentration showed a slight decrease for the time period 1974–1989, for which data were available. However, a relationship existed between the radiative flux and the ice concentration, not only for the actual data, but also for the deviation series with the annual cycles removed. A correlation factor of –0.74 was found; the sensitivity for an increase of 10% in ice concentration was –2.9 W/m². This represents a temperature change as seen from space of about 1°C for a 10% change in sea ice concentration.With 7 Figures