城市化环境大气污染模型动力学问题

城市化环境大气污染动力学问题是城市环境大气污染形成机理及其治理原理研究中核心理论问题,该文从城市化环境大气污染各类复杂的交叉影响因素角度,初步描述了城市环境大气多尺度相互作用;城市建筑群及其周边地形影响;下垫面及陆面过程对城市环境大气动力结构形成的影响效应;城市环境水-土-气污染形成的多圈层相互作用等问题.并且综合分析探讨了城市环境大气污染的动力学特征及其影响作用.通过理论问题的讨论,给出了本项目开展的BECAPEX现场观测试验的设计实施和城市污染"大锅盖"特征结构研究的科学问题.     

北京城市大气环境污染机理与调控原理

该文主要介绍了科技部国家重点基础研究发展规划项目“首都北京及周边地区大气、水、土环境污染机理及调控原理”大气分项目的研究成果。项目分别于2001年和2003年重点开展了BECAPEX科学试验 (Beijing City Air Pollution Experiment)。BECAPEX试验同步进行城市边界层气象与大气化学观测, 通过卫星遥感、地面观测, 即城市空间和地面以及点与面结合的技术途径, 以揭示北京城市污染“空气穹隆”大气化学结构特征及其变化规律, 为城市环境大气动力-化学模式提供基本科学参数, 给出城市边界层大气物理化学过程综合模型, 为提高城市环境大气物理-化学过程耦合模式的准确性和可靠性提供科学依据。该项目揭示了北京城区和城近郊区城市边界层结构与湍流特征, 城市大气污染垂直结构特征; 发现了城市大气污染空间结构多尺度特征, 其中包括大气污染源影响和城市热岛多尺度特征; 揭示了城市大气重污染过程周边源影响域, 以及北京及周边地区气溶胶影响域和区域气候响应; 提出了北京市典型污染源排放清单; 发展了城市气象模式系统, 包括冠层模式、街谷环流和热力结构以及城市高大建筑群周围风环境数值模拟; 发展了空气质量模式技术, 包括二次气溶胶模拟试验、北京地区SO₂污染的长期模拟及不同类型排放源影响的计算与评估、影响北京地区的沙尘暴输送模拟、区域化学输送模式中NO_x和O₃源示踪法, 城市尺度的大气污染CAPPS模式及统计模型的应用、大气污染及紫外辐射数值预报模式和CMAQ-MOS空气质量预报方法; 改进了美国公共多尺度空气质量预报模式, 建立了CMAQ-MOS区域空气质量动力-统计模型预报模式, 以及发展的源同化技术, 突破了当前空气质量模式技术“瓶颈”, 使模式预报准确率明显提高。     

北方局地夏末气溶胶光学特性综合观测分析

本文对中国北方相近地理经度不同纬度的三个试验点（内蒙草原生态定位站、北京、新乡）夏末季节大气气溶胶特性进行了地面粒子计数和整层光学遥感等综合观测。分析结果表明，这三个试验点地面和整层气溶胶数浓度通常有内蒙较小，北京居中，新乡最大的特征。文中提出了浓度比这个参量，它可以定量描述地面源气溶胶对整层大气气溶胶的相对贡献。据此分析可知内蒙地面源较弱，与该地区人类活动稀少相对应。由浓度比推测，新乡除近地面城市空气污染较严重外，滨临的黄河河面水汽蒸发作用也是促成气溶胶浓度增大的原因。     

2017年冬季长沙一次重度霾污染天气过程气象成因分析

利用空气质量监测资料、常规气象资料,根据气象条件的水平和垂直扩散能力,以及地面湿度和动力条件等分析了2017年1月27—29日长沙地区这次严重空气污染事件的污染特征。结果表明:污染发生时段,南支槽不断加深东移,槽前势力强盛的西南气流将孟加拉湾一带的水汽向长沙地区输送,进一步增加了该地区的空气湿度。同时,持续东移的脊前暖平流对长沙中低层大气增温有显著影响,为稳定的大气层结创造了有利条件。长沙处于弱高压的底后部,受大范围的弱鞍型场及均压场控制,地面有暖倒槽发展,且由于高压较弱,导致地面和低空的风速较小,不利于污染物的水平扩散,同时有利于夜间地面的辐射降温。稳定的大气环流形势为霾天气和严重污染提供了持续稳定的大气环境场,逆温结构和稳定温度层结在一定程度上减弱了大气在垂直方向上的湍流交换和热力对流,大气中的污染颗粒不易扩散,为此次污染事件的维持、加剧提供了重要的气象条件。长沙地区处在罗霄山脉和雪峰山脉之间的湘江故地,受周边地形阻挡的影响,污染物在下沉气流的控制下聚集到长沙地区后,很难通过水平输送离开,这也是造成此次霾污染的原因之一。     

人为热对城市边界层结构影响研究

为研究不同人为热源引入方案对城市边界层结构模拟性能的影响，以杭州地区为例，在区域边界层模式（RBLM）中引入一种新人为热源处理方案，即对城市中的人为热排放分层考虑，将低层的人为热源加入地表能量平衡方程，将高层人为热源分布与建筑物高度和密度联系起来，加入热量方程中，同时考虑了人为热源强度的日变化。数值试验结果表明，这是一种比较合理的处理方案。人为热源引入方案对城市边界层结构的影响表现在:气温、湍流动能增加，并通过湍流交换输送到较高层大气；大气不稳定度增加，混合层高度最高抬升了400 m；城市地区上升速度增加，热岛环流加强；白天人为热源一般为太阳辐射的10%～20%，对地气交换的影响较小。夜间没有了太阳辐射能量，对地气交换的影响比日间更明显；冬季低层湍流活动加强，湍能约增加40%，大气层结稳定度降低。     

福州城市空气污染对太阳辐射的影响

本文通过1962—1985年大气辐射过程、大气透明度和大气混浊度的变化,间接推断福州大气质量的长期演变及空气污染的季节变化。结果表明,直接辐射量减少,大气透明度的降低和大气混浊度的提高,都反映了城市空气污染的逐步发展,归因于空气中颗粒物的增加。本文所讨论的大气污染物混浊因子T_R,可以较客观地反映福州空气污染的年变化。     

Further Development of the Vegetated Urban Canopy Model Including a Grass-Covered Surface Parametrization and Photosynthesis Effects

The vegetated urban canopy model (VUCM), which includes parametrizations of urban physical processes for artificial surfaces and vegetated areas in an integrated system, has been further developed by including physical processes associated with grass-covered surfaces in urban pervious surfaces and the photosynthesis effects of urban vegetation. Using measurements made from three urban/suburban sites during the BUBBLE field campaign in 2002, the model’s performance in modelling surface fluxes (momentum flux, net radiation, sensible and latent heat fluxes and storage heat flux) and canopy air conditions (canopy air temperature and specific humidity) was critically evaluated for the non-precipitation and the precipitation days. The observed surface fluxes at the urban/suburban sites were significantly altered by precipitation as well as urban vegetation. Especially, the storage heat at urban surfaces and underlying substrates varied drastically depending on weather conditions while having an important role in the formation of a nocturnal urban surface layer. Unlike the nighttime canopy air temperature that was largely affected by the storage-heat release, the daytime canopy air conditions were highly influenced by the vertical turbulent exchange with the overlying atmosphere. The VUCM well reproduced these observed features in surface fluxes and canopy air conditions at all sites while performing well for both the non-precipitation and the precipitation days. The newly implemented parametrizations clearly improved the model’s performance in the simulation of sensible and latent heat fluxes at the sites, more noticeably at the suburban site where the vegetated area fraction is the largest among the sites. Sensitivity analyses for model input parameters in VUCM elucidated the relative importance of the morphological, aerodynamic, hydrological and radiative/thermal properties in modelling urban surface fluxes and canopy air conditions for daytime and nighttime periods. These results suggest that the VUCM has great potential for urban atmospheric numerical modelling for a range of cities and weather conditions in addition to having a better physical basis in the representation of urban vegetated areas and associated physical processes.     

CALPUFF模型在合肥地区SO2大气环境容量测算中的应用

在对合肥地区污染源调查的基础上,利用CALPUFF模型模拟了合肥地区大气污染物SO₂质量浓度场,通过与现场监测结果对比分析了模型的适用性,并根据模拟结果研究了不同排放源对合肥地区大气污染的贡献情况,建立了大气污染物传递矩阵;通过综合考虑城市区域的大气扩散能力、污染源贡献和大气环境质量目标等,采用线性规划模型测算了合肥市的大气环境容量.     

Nighttime convection in the interior of a dense Douglas fir forest

Infrared radiative surface temperatures as observed over a dense Douglas fir forest during stable atmospheric conditions are analyzed. It is shown that the concept of a single surface temperature to describe both the thermal coupling and the radiative coupling between atmosphere and forest fails when longwave cooling is large and wind speeds are low. In such cases a decoupling of the radiative surface temperature from the air temperature aloft is observed. Conditions for decoupling are formulated in terms of an appropriate Richardson number. It is shown that a convective surface temperature comes into play that is coupled to the forest interior air temperature. Observed radiative surface temperature is then composed of this convective surface temperature and the aerodynamic surface temperature. Forest interior air temperature during nighttime is, in general, lower than air temperature above the canopy. A simple two-layer canopy model is used to explain this phenomenon in terms of the distribution of atmospheric sensible heat flux and storage heat flux over the two canopy layers.     

大气边界层物理与大气环境过程研究进展

总结了近5年来中国科学院大气物理研究所大气边界层物理和大气化学国家重点实验室(LAPC)在第二代超声风速温度仪研制、城市边界层研究、复杂地形大气边界层探测与数值模拟、湍流机理研究、大气污染模式发展与应用等领域的主要进展,其中,第二代超声风速温度仪的野外对比测试结果表明其主要性能完全达到了国际先进水平;北京城市化发展使得北京325 m气象塔周边近地面流场已经具备了典型城市粗糙下垫面的流场特征,近地面夏季平均风速呈现非常明显的逐年递减趋势;北京沙尘暴大风时期湍流运动主要是小尺度湍涡运动,而大风的概率分布偏离高斯分布,风速较大的一侧概率分布呈指数迅速衰减,大风中风速很大的部分具有分形特征;珠穆朗玛峰北坡地区两次综合强化探测实验是迄今为止在青藏高原大型山地中实施的针对山地环流和物质／能量交换最为全面和连续的大气过程探测实验;白洋淀地区的观测研究表明,非均匀边界层具有一般边界层不具备的特点,无论是边界层结构还是湍流输送方面,水、陆边界层之间存在一定的差异,凸显其地表非均匀性的作用;为了解决不同尺度、不同类型的大气污染问题和实际应用,研制或发展完善了多套大气污染模式系统,包括全球大气化学模式、区域大气污染数值模式、城市大气污染数值模式和微小尺度(如街区尺度)范围内污染物输送扩散模式。     

Sensitivity experiments performed with an energy balance atmosphere model coupled to an advection-diffusion ocean model

Summary In this paper a simple climate model is presented which is used to perform some sensitivity experiments. The atmospheric part is represented by a vertically and zonally averaged layer in which the surface air temperature, radiative fluxes at the surface and at the top of the atmosphere, the turbulent fluxes between atmosphere and surface and the snow cover are calculated. This atmospheric layer is coupled to a two-dimensional advection-diffusion ocean model in which the zonal overturning pattern is prescribed. The ocean model evaluates the temperature distribution, the amount of sea-ice and the meridional and vertical heat fluxes. The present-day climate simulated by the model compares reasonably well with observations of the seasonal and latitudinal distribution of temperature, radiation, surface alebdo, sea-ice and snow cover and meridional energy fluxes. Then, the sensitivity of the model-simulated present-day climate to perturbations in the incident solar radiation at the top of the atmosphere is investigated. The temperature response displays large latitudinal and seasonal variations, which is in qualitative agreement with results obtained with other climate models. It is found that the seasonal variation of sea-ice cover (and hence, the effective oceanic heat capacity) is one of the most important elements determining seasonal variations in climate sensitivity. Differences in sensitivity between the seasonal and annual mean version of the model are discussed. Finally, the equilibrium response to perturbations in some selected model variables is presented; these variables include meridional diffusion coefficients, drag coefficient, sea-ice thickness, atmospheric CO₂-concentration and cloud optical thickness.With 13 Figures     

Environmental process and convergence belt of atmospheric NO2 pollution in North China

Both surface environmental monitoring and satellite remote sensing show that North China is one of the regions that are heavily polluted by NO₂. Using the NO₂ monitoring data from 18 major cities in the region, the tropospheric NO₂ column density data from the Ozone Monitoring Instrument (OMI) on the Aura satellite, and the observations from the China Meteorological Administration network, this paper analyzes a regional NO₂ pollution event in February 2007 over North China, examines the convergence of the pollutant, and identies its correlation with the atmospheric background conditions. The results show that daily mean NO₂ concentrations derived from surface observations are consistent with the mean values of the OMI measurements, with their correlation coeficient reaching 0.81. The correlations of NO₂ concentration with general weather patterns and sequential changes of temperature structure from 925 hPa down to the surface indicate that the weather fronts, high pressure and low pressure systems in the atmosphere play a role in changing the temporal and spatial evolutions of NO₂ through removing, accumulating or converging of the pollutant, respectively. It is also found that the eastern Taihang Mountains is most heavily polluted by NO₂ in North China. Based on a model that correlates NO₂ column density with surface wind vector, the relation of the NO₂ concentrations in six major cities in North China to the surrounding wind field is analyzed. The results show that the maximum wind field is associated with the highest frequency of pollution events, and under certain large-scale atmospheric conditions together with the topographic effect, small- and meso-scale wind fields often act to transport and converge pollutants, and become a major factor in forming the heaviest NO₂ pollution event in North China. Analysis of the causes for the severe NO₂ pollution event in this study may shed light on understanding, forecasting, and mitigating occurrences of heavy NO₂ pollution.     

Aspects Of The Atmospheric Surface Layers On Mars And Earth

The structures of mean flow and turbulence in the atmospheric surface boundary layer have been extensively studied on Earth, and to a far less extent on Mars, where only the Viking missions and the Pathfinder mission have delivered in-situ data. Largely the behaviour of surface-layer turbulence and mean flow on Mars is found to obey the same scaling laws as on Earth. The largest micrometeorological differences between the two atmospheres are associated with the low air density of the Martian atmosphere. Together with the virtual absence of water vapour, it reduces the importance of the atmospheric heat flux in the surface energy budget. This increases the temperature variation of the surface forcing the near-surface temperature gradient and thereby the diabatic heat flux to higher values than are typical on the Earth, resulting in turn in a deeper daytime boundary layer. As wind speed is much like that of the Earth, this larger diabatic heat flux is carried mostly by larger maximal values of T_*, the surface scale temperature. The higher kinematic viscosity yields a Kolmogorov scale of the order of ten times larger than on Earth, influencing the transition between rough and smooth flow for the same surface features.The scaling laws have been validated analysing the Martian surface-layer data for the relations between the power spectra of wind and temperature turbulence and the corresponding mean values of wind speed and temperature. Usual spectral formulations were used based on the scaling laws ruling the Earth atmospheric surface layer, whereby the Earth's atmosphere is used as a standard for the Martian atmosphere.     

昆明和北京两幢建筑物表面热力效应的观测对比

利用昆明、北京两座城市内建筑物为研究对象, 对其不同朝向外墙壁面、屋顶面表面温度及壁面近旁气温进行了观测, 分析了建筑物外墙壁面表面温度及其近旁气温的垂直分布以及壁面、屋顶对周围大气的热力效应特征, 并对两座城市内建筑物的热力状况进行了比较分析。研究表明:建筑物表面温度受太阳辐射的影响要比近旁气温大得多, 一般说来, 壁面昼间是热源, 夜间是热汇; 受研究对象所在的大区域气候、人类活动等影响, 建筑物外表面的热力效应有许多异同; 建筑物屋顶面与近旁空气间的平均热通量基本为正值, 呈现较强的热源效应, 其热力效应强度与太阳辐射呈现正相关; 城市建筑物的外表面 (壁面、屋顶面) 已成为城市区域内有别于城市地面, 且对城市立体气候的形成具有不可忽视影响的热力作用面。     

大气环境数值模拟研究新进展

近五年来,中国科学院大气物理研究所(简称大气所)在大气环境数值模拟方面取得了丰硕的成果,通过自主发展和引进,建立了完备的多尺度、多成分的大气环境数值模式,包括全球大气化学输送模式、区域和城市空气质量预报模式。大气所利用这些模式研究各种空间尺度上污染物浓度时空分布以及污染物的输送和演变,研究了多种污染过程的成因和污染变化规律,在污染物输送、低对流层臭氧高污染、区域及城市污染等方面取得了很多成果,并对区域或城市空气质量进行业务化实时预报。大气所还拓展了我国大气环境模拟研究的新领域:大气化学资料同化、污染模式集合预报、污染源反演新方法。初步建立了空气质量模式的资料同化系统(分别基于最优插值技术和集合卡曼滤波技术)和多模式集合预报体系,提高了模式预报水平;在污染源反演新方法方面进行了初步的探索。结合我国目前仍然面临着的大气环境问题,对今后大气环境数值模式的发展方向进行了展望。     

A Review of Atmospheric Chemistry Research in China: Photochemical Smog, Haze Pollution, and Gas-Aerosol Interactions

In this paper we present a review of atmospheric chemistry research in China over the period 2006-2010, focusing on tropospheric ozone, aerosol chemistry, and the interactions between trace gases and aerosols in the polluted areas of China. Over the past decade, China has suffered severe photochemical smog and haze pollution, especially in North China, the Yangtze River Delta, and the Pearl River Delta. Much scientific work on atmospheric chemistry and physics has been done to address this large-scale, complex environmental problem. Intensive field experiments, satellite data analyses, and model simulations have shown that air pollution is significantly changing the chemical and physical characters of the natural atmosphere over these parts of China. In addition to strong emissions of primary pollutants, photochemical and heterogeneous reactions play key roles in the formation of complex pollution. More in-depth research is recommended to reveal the formation mechanism of photochemical smog and haze pollution and their climatic effects at the urban, regional, and global scales.     

Effect of urbanization on the urban meteorology and air pollution in Hangzhou

Urbanization has a substantial effect on urban meteorology. It can alter the atmospheric diffusion capability in urban areas and therefore affect pollutant concentrations. To study the effects of Hangzhou’s urban development in most recent decade on its urban meteorological characteristics and pollutant diffusion, 90 weather cases were simulated, covering 9 weather types, with the Nanjing University City Air Quality Prediction System and high-resolution surface-type data and urban construction data for 2000 and 2010. The results show that the most recent decade of urban development in Hangzhou substantially affected its urban meteorology. Specifically, the average urban wind speed decreased by 1.1 m s ^?1; the average intensity of the heat island increased by 0.5°C; and the average urban relative humidity decreased by 9.7%. Based on one case for each of the nine weather types, the impact of urbanization on air pollution diffusion was investigated, revealing that the changes in the meteorological environment decreased the urban atmosphere’s diffusion capability, and therefore increased urban pollutant concentrations. For instance, the urban nitrogen oxides concentration increased by 2.1 μg m ^?3 on average; the fine particulate matter (diameter of 2.5 μm or less; PM_2.5) pollution concentration increased by 2.3 μg m ^?3 on average; in highly urbanized areas, the PM_2.5 concentration increased by 30 μg m ^?3 and average visibility decreased by 0.2 km, with a maximum decrease of 1 km; the average number of daily hours of haze increased by 0.46 h; and the haze height lifted by 100–300 m. The “self-cleaning time” of pollutants increased by an average of 1.5 h.     

Sensitivity of the thermohaline circulation in coupled oceanic GCM — atmospheric EBM experiments

We analyze the sensitivity of the oceanic thermohaline circulation (THC) regarding perturbations in fresh water flux for a range of coupled oceanic general circulation — atmospheric energy balance models. The energy balance model (EBM) predicts surface air temperature and fresh water flux and contains the feedbacks due to meridional transports of sensible and latent heat. In the coupled system we examine a negative perturbation in run-off into the southern ocean and analyze the role of changed atmospheric heat transports and fresh water flux. With mixed boundary conditions (fixed air temperature and fixed surface fresh water fluxes) the response is characterized by a completely different oceanic heat transport than in the reference case. On the other hand, the surface heat flux remains roughly constant when the air temperature can adjust in a model where no anomalous atmospheric transports are allowed. This gives an artificially stable system with nearly unchanged oceanic heat transport. However, if meridional heat transports in the atmosphere are included, the sensitivity of the system lies between the two extreme cases. We find that changes in fresh water flux are unimportant for the THC in the coupled system.     

鄂尔多斯市城区发展对局地大气环境影响的数值模拟

选取鄂尔多斯市东胜区为代表区域。基于该区域1961-2006年定时地面气象观测资料,2002-2006年08时、20时各标准层探空以及2001-2006年主要污染源源强、1961-2006年社会经济数据、2002年卫星遥感反演资料、2003-2020年城市总体规划资料等,利用区域边界层模式模拟方法,分析鄂尔多斯市城市化进程对局地大气环境的影响。结果表明:东胜区发展后(2020年)气温低于现状(2002),使城区中心气温与周边地区气温差异变小,对城区大气环境的改善较为有利。东胜城区扩展后,在污染严重的冬季,气流辐合区域减少,辐散能力增强,对减轻城区污染和改善大气环境有利。城区拓展后由于下垫面等布局发生变化, 气流场变化较大,但从污染物的扩散能力来看,按规划发展后城区污染轻于现状。     

城市中水体布局对大气环境的影响

城市下垫面状况在很大程度上决定城市大气物理环境的特征。在城市区域增加湿地等自然地表有利于城市的减温增湿,促使局地流场发生变化,改善局地微气象条件以及大气物理环境。城市规划大气物理环境多尺度数值模拟系统为城市规划大气物理环境定量评估提供了有效的模拟工具。利用该系统中的城市尺度模式模拟了水体布局为集中型和分散型,水体面积占有率分别为4%、8%、12%和16%条件下,城市大气温度、湿度、风速、城市大气扩散条件的变化及其对城市大气环境的影响,利用北京市城市水体气象观测数据,分析了水体周边和商业区、交通区温、湿度的差异,并对模式模拟结果进行了验证,揭示了城市水体布局对城市大气物理环境影响的可能机制。模拟和观测结果显示,城市水体布局会对城市微气象环境产生一定影响。无论分散型或集中型布局,城市水体面积的增加,都在一定程度上使城市气温降低、湿度增加、平均风速增大。比较而言,分散型水体布局对城市区域微气象环境的影响更为显著。