沈阳近地层大气颗粒物浓度垂直变化特征及与气象因子的关系

利用2018年10月1日至2019年9月30日沈阳地区三个高度大气颗粒物浓度和气象要素逐时观测资料,分析了不同高度颗粒物浓度时间变化特征及其与气象要素的关系.结果表明:不同高度的颗粒物浓度均存在明显的季节变化,秋冬季数值明显高于春夏季.冬季,三个高度的PM2.5平均浓度为54.98±12.67μg·m-3、63.77±...     

稻麦轮作农田区大气边界层高度的日变化和季节特征

利用2015年7月至2016年5月寿县稻麦轮作农田区观测站地基多通道微波辐射计观测的高时间分辨率温度廓线资料,结合位温梯度法,计算了该站点的大气边界层高度,分析了边界层高度的日、月和季节演变规律。结果显示,晴朗天气情况下,边界层高度具备典型的日变化特征,随着地面温度的升高边界层高度不断增大。其最大平均值通常出现在午后,8月平均高度最高,超过1520m,1月最低,只有520m。而且边界层高度具有季节变化趋势,春季(3—5月)、夏季(6—8月)、秋季(9—11月)和冬季(12月至次年2月)平均高度分别为436m,499m,377m和322m。将边界层高度结果与FNL和ERA-Interim数据进行对比,发现在白天时间段(08:00—19:00)FNL和ERA-Interim比观测平均值分别高258m,346m,夜间时间段(19:00至次日08:00)比观测平均值分别低144m,102m。     

Measuring Sensible Heat Flux Density over Pasture Using the ct2-Profile Method

Two large-aperture infrared scintillometers were positioned at heights (z) of 10 and 1.5 m with beams propagated horizontally over pasture for distances of 3.1 km and 141 m, respectively. From each scintillometer a half-hourly average value of the path-averaged, temperature-structure parameter (CT2) was obtained in unstable atmospheric conditions. The result suggested CT2 to scale with height as z-2/3. Using the CT2-profile method a path-averaged measure of the Obukhov length (L0) was calculated for each half-hour period, whence L0 was used to determine the friction velocity, u* and the surface-layer temperature scaling parameter, T*. The scintillometer-based sensible heat flux density Hsc was then calculated from Hsc = Cpu*T*. A time series of half-hourly averaged Hsc compared to Hec obtained by the eddy covariance method agreed to within 10%, with R2 = 0.67, for a range of unstable conditions (- 0.2 z/L0 - 0.01).     

气流输送对北京大气污染物体积分数的影响

利用HYSPLIT后向轨迹模式和2004年8月—2007年12月NCEP再分析气象资料,计算每天15:00抵达北京地区10、100和500m高度上的后向气流轨迹.对整个研究时段、采暖季和非采暖季期间的后向气流轨迹分别进行聚类分析,得到这3个时段到达北京地区的主要后向气流轨迹聚类.其中整个研究时段的后向气流轨迹分成3个聚类,采暖季和非采暖季的后向气流轨迹都分成5个聚类.结合各段时间中国科学院大气物理研究所观测的大气污染物体积分数资料,分析不同时段气流输送作用对北京主要大气污染物体积分数的影响.发现采暖季和非采暖季北京气体污染物体积分数高值主要集中在来自风速较小的西北方气流聚类.采暖季污染物体积分数低值主要出现在偏北方向风速较大的后向气流轨迹聚类.非采暖季污染物体积分数低值主要出现在偏北低速气流聚类和西北向高速气流轨迹聚类中.从各时段污染物最值分布情况可以看出:在风速较大的后向气流轨迹聚类影响下,北京的污染物体积分数较低;途经了较严重工业排放地带的后向气流轨迹聚类会使北京气体污染物体积分数显著增高.此外,虽然非采暖季的大气污染物分布与气流输送的影响基本符合,但各聚类污染物分布结果与气流输送作用的影响存在偏差.     

基于微波辐射计和气溶胶激光雷达的边界层高度研究及应用

分别基于微波辐射计温湿度廓线资料的气块法、位温法和比湿法,地面气象资料的罗氏法及气溶胶激光雷达数据的梯度法,计算得出广州地区大气边界层高度,对比分析5种边界层高度结果及其与气象条件、空气质量之间的关系,结合典型大气污染过程分析边界层高度对PM_2.5、O₃浓度的影响。结果显示:（1）利用位温法、气块法、罗氏法、比湿法和梯度法计算得出广州地区平均边界层高度分别为2 207 m、1 239 m、901 m、717 m和660 m,位温法显著高估了广州地区的边界层高度;（2）利用气块法得出的混合层高度日变化能够较好地表征白天大气边界层演变特征,利用气块法和比湿法得出的白天混合层高度与近地面O₃浓度有显著的正相关关系,相关系数在0.5以上,在O₃污染防治中,应同时考虑边界层内垂直输送的影响;（3）利用梯度法得出的边界层高度在污染天气时与PM_2.5浓度的相关性较好,能较好地表现出大气污染情况,在PM_2.5污染天气过程分析中具有较好的应用价值。      

Dynamical controls on the diurnal cycle of temperature in complex topography

We examine the climatological diurnal cycle of surface air temperature in a 6 km resolution atmospheric simulation of Southern California from 1995 to the present. We find its amplitude and phase both have significant geographical structure. This is most likely due to diurnally-varying flows back and forth across the coastline and elevation isolines resulting from the large daily warming and cooling over land. Because the region’s atmosphere is generally stably stratified, these flow patterns result in air of lower (higher) potential temperature being advected upslope (downslope) during daytime (nighttime). This suppresses the temperature diurnal cycle amplitude at mountaintops where diurnal flows converge (diverge) during the day (night). The nighttime land breeze also advects air of higher potential temperature downslope toward the coast. This raises minimum temperatures in land areas adjacent to the coast in a manner analogous to the daytime suppression of maximum temperature by the cool sea breeze in these same areas. Because stratification is greater in the coastal zone than in the desert interior, these thermal effects of the diurnal winds are not uniform, generating spatial structures in the phase and shape of the temperature diurnal cycle as well as its amplitude. We confirm that the simulated characteristics of the temperature diurnal cycle as well as those of the associated diurnal winds are also found in a network of 30 observation stations in the region. This gives confidence in the simulation’s realism and our study’s findings. Diurnal flows are probably mainly responsible for the geographical structures in the temperature diurnal cycle in other regions of significant topography and surface heterogeneity, their importance depending partly on the degree of atmospheric stratification.     

1991年江淮暴雨期地气通量与混合层结构的研究

本文用１９９１年５—７月江淮及其北部地区的地面与高空资料根据３种不同的整体公式对地表通量（动量、感热和潜热通量）进行了估算，并对混合层结构进行了研究，揭示出这次持续性特大暴雨中陆面过程的一些特征，主要结果如下：１．地表通量依赖于大气稳定度，稳定度越强，地表通量越小。不稳定状况下平均地表动量通量为０．０１５４Ｎ／ｍ２，向上的感热和潜热平均值分别为２５．７Ｗ／ｍ２和１３２．３Ｗ／ｍ２；稳定状况下，地表动量通量为０．００６Ｎ／ｍ２，感热和潜热通量平均是向下输送的，分别为－１．５Ｗ／ｍ２和２．５Ｗ／ｍ２。２．地表通量与降水过程密切有关。雨期的动量通量略小于非雨期，而雨期的感热与潜热通量明显小于非雨期，雨量越大，这两种通量愈小。３．地表通量具有明显日变化。动量、感热和潜热通量的最大值出现在下午２时左右，最小值出现在凌晨２时左右。４．混合层与雨期关系密切，雨期的混合层高度较非雨期低，这时地表感热和潜热通量小；而非雨期情况相反     

The Impact of the Afternoon Planetary Boundary-Layer Height on the Diurnal Cycle of CO and $$\hbox {CO}_{2}$$ Mixing Ratios at a Low-Altitude Mountaintop

Mountaintop trace-gas mixing ratios are often assumed to represent free atmospheric values, but are affected by valley planetary boundary-layer (PBL) air at certain times. We hypothesize that the afternoon valley–PBL height relative to the ridgetop is important in the diurnal cycle of mountaintop trace-gas mixing ratios. To investigate this, we use, (1) 4-years (1 January 2009–31 December 2012) of CO and \(\hbox {CO}_{2}\) mixing-ratio measurements and supporting meteorological observations from Pinnacles (\(38.61^{\circ }\hbox {N}\), \(78.35^{\circ }\hbox {W}\), 1017 m a.s.l.), which is a monitoring site in the Appalachian Mountains, (2) regional \(\hbox {O}_{3}\) mixing-ratio measurements, and (3) PBL heights determined from a nearby sounding station. Results reveal that the amplitudes of the diurnal cycles of CO and \(\hbox {CO}_{2}\) mixing ratios vary as a function of the daytime maximum valley–PBL height relative to the ridgetop. The mean diurnal cycle for the subset of days when the afternoon valley–PBL height is at least 400 m below the ridgetop shows a daytime CO mixing-ratio increase, implying the transport of PBL air from the valley to the mountaintop. During the daytime, on days when the PBL heights exceed the mountaintop, PBL dilution and entrainment cause CO mixing ratios to decrease. This decrease in CO mixing ratio, especially on days when PBL heights are at least 400 m above the ridgetop, suggests that measurements from these days can be used as with afternoon measurements from flat terrain in applications requiring regionally-representative measurements.     

Diurnal Variations of Air Pollution and Atmospheric Boundary Layer Structure in Beijing During Winter 2000／2001

The diurnal variations of gaseous pollutants and the dynamical and thermodynamic structures of the atmospheric boundary layer (ABE) in the Beijing area from January to March 2001 are analyzed in this study using data from the Beijing City Air Pollution Observation Field Experiment (BECAPEX). A heavy pollution day (22 February) and a good air quality day (24 February) are selected and individually analyzed and compared to reveal the relationships between gaseous pollutants and the diurnal variations of the ABL. The results show that gaseous pollutant concentrations exhibit a double-peak-double-valley-type diurnal variation and have similar trends but with different magnitudes at different sites in Beijing. The diurnal variation of the gaseous pollutant concentrations is closely related to (with a 1-2 hour delay of) changes in the atmospheric stability and the mean kinetic energy in the ABL.     

Evaluation of MM5 mesoscale model at local scale for air quality applications over the Swedish west coast: Influence of PBL and LSM parameterizations

Summary The performance of MM5 mesoscale model (Version 3.6.3) using different planetary boundary layer (PBL) and land surface model (LSM) parameterizations is evaluated and compared using high temporal and spatial resolution G?TE2001 campaign data at local scale (a few kilometers) over the Greater G?teborg area along the Swedish west coast during 7–20 May 2001. The focus is on impact of PBL and LSM parameterizations on simulated meteorological variables important for air quality applications such as global radiation, diurnal cycle of near-surface air temperature and wind, diurnal cycle intensity, near-surface vertical temperature gradient, nocturnal temperature inversion, boundary layer height, and low-level jet (LLJ). The model performance for daytime and nighttime and under different weather conditions is also discussed. The purpose is to examine the performance of the model using different PBL and LSM parameterizations at local scale in this area for its potential applications in air quality modeling. The results indicate that the influence of PBL and LSM parameterizations on simulated global radiation, diurnal cycle of near-surface air temperature and wind speed, diurnal cycle intensity, vertical temperature gradient, nocturnal temperature inversion and PBL heights, which are critical parameters for air quality applications, is evident. Moreover, the intensity and location of LLJ are simulated well by all schemes, but there also exist some differences between simulated results by using different PBL and LSM schemes. Therefore, the choice of PBL and LSM parameterizations is important for MM5 applications to air quality studies. Correspondence: Junfeng Miao, Department of Earth Sciences, G?teborg University, P.O. Box 460, 405 30 G?teborg, Sweden     

森林近地层大气湍流特性观测分析

利用长白山森林生态系统定位研究站观测资料,及2003年8月和9月涡旋相关资料,分析和比较了该地区近地层包括风速、风向、大气稳定度在内的平均场特征,以及湍流强度、无量纲化风脉动方差相似性和地表通量变化特征。结果表明:(1)8月和9月稳定度都基本集中在0附近;(2)风速2 m·s-1的环境中,湍流发展最为旺盛,随着风速的增大湍流强度先迅速减小,当风速增大到3 m·s-1后,湍流强度偏离0值变大了一些,再继续增大到一定风速大小以后,湍流强度基本不随风速变化;(3)无量纲化三维风脉动方差符合Monin-Obukhov相似理论的"1/3"定律,其最佳通用相似函数在稳定和不稳定条件下都可以拟合得到;(4)地表通量均表现出明显的日变化特征,8月以潜热为主,感热较小;9月仍以潜热为主,但是相比8月明显偏小,感热变化不大。     

Static Stability of the Troposphere Over the Southeastern Beaufort Sea–Amundsen Gulf Region of the Western Maritime Arctic

The characterization of the static stability of the troposphere over the western maritime Arctic remains limited in spite of its significance to both atmospheric thermodynamics and dynamics. Field observations of microwave radiometric temperature profiles from the International Polar Year, Circumpolar Flaw Lead System Study (late November 2007 to mid-July 2008) and the ArcticNet field campaign (mid-July to early November 2009) provided a unique opportunity to characterize the static stability of the troposphere over the southeastern Beaufort Sea–Amundsen Gulf region. Notably, the monthly median atmospheric boundary layer (<2000?m) static stability profile for April and the profile for May clearly revealed an inversion elevated above a thermal internal boundary layer, whereas the median summer static stability profiles had very strong surface-based inversions. These profiles have been linked to the seasonal evolution of sea-ice cover in Amundsen Gulf. The monthly static stability profiles for the free atmosphere (2000–10,000?m) revealed an annual cycle. The average static stability of the lower troposphere (2000–5000?m) had a minimum of 3.3?±?0.5?K?km^?1 in July and a maximum of 4.5?±?0.5?K?km^?1 in January and February. In the upper troposphere (>5000–8000?m), the average static stability had a minimum of 2.9?±?0.6?K?km^?1 in June and August and a maximum of 5.3?±?0.8?K?km^?1 in January. The monthly median heights of the tropopause also had an annual cycle. The maximum of 9750?m occurred in June, July, and August. The minimum tropopause height of 8000?m occurred in December, January, and March. The seasonal cycles of static stability in the free atmosphere and the seasonal cycle in the height of the tropopause can be attributed to regional as well as synoptic-scale forcing. This analysis will contribute to the understanding of the thermodynamics and dynamics of a data-sparse region of the Arctic by providing a “snapshot” of the state of the atmosphere through a composite annual cycle.     

Interaction of secondary circulations with the summer monsoon and diurnal rainfall over Hong Kong

A complete yearly record (1988) of surface measurements is used to examine the atmospheric diurnal secondary circulations over the entire area of Hong Kong in conjunction with spatial and temporal variations of surface temperature, wind speed and rainfall. Evidence of atmospheric diurnal secondary circulations is found at 10 sites. The occurrence of a summer morning rainfall maximum over the coast results from the interaction of the large-scale summer monsoon and local mesoscale secondary circulations. The afternoon onshore secondary circulation accelerates the advection of warm, humid unstable air and, coupled with the upward orographic lifting, produces enhanced rainfall along windward mountain ridges.Dynamical and scaling considerations suggest that the blocking effect is negligible and the primary forcing mechanism is land-sea temperature difference, but terrain effects are also important. Although the secondary circulation system's strength and timing vary, the circulation behaves like a classic sea-land breeze circulation, complicated by superimposed mountain-valley breezes.     

An Improvement of the Louis Scheme for the Surface Layer in an Atmospheric Modelling System

The Louis scheme for calculating the vertical eddy fluxes within the atmospheric surface layer is improved by broadening the original assumptions. In our approach, the momentum and heat transfer roughness lengths (z₀ and z_T respectively) can be different, and z₀ need not be negligibly small compared with the lowest height (z) in modelling. For these conditions, we choose more consistent wind and potential temperature profile forms, then derive new algorithms for calculating fluxes. Improvement is demonstrated for a wide range of z/L (L is the Obukhov length), z/z₀ and z₀ z_T, by comparing these fluxes with those derived from a theoretical surface-layer model. The improved algorithms can be used in atmospheric modelling systems for more varied surfaces and a wide range of atmospheric stability.     

Evaluation of the vegetated urban canopy model (VUCM) and its impacts on urban boundary layer simulation

The vegetated urban canopy model (VUCM) is implemented in a meteorological model, the Regional Atmospheric Modeling System (RAMS), for urban atmospheric modeling. The VUCM includes various urban physical processes such as in-canyon radiative transfer, turbulent energy exchanges, substrate heat conduction, and in-canyon momentum drag. The coupled model RAMS/VUCM is evaluated and then used to examine its impacts on the dynamic and thermodynamic structure of the urban boundary layer (UBL) in the Seoul metropolitan area. The spatial pattern of the nocturnal urban heat island (UHI) in Seoul is quite well simulated by the RAMS/VUCM. A statistical evaluation of 2-m air temperature reveals a significant improvement in model performance, especially in the nighttime. The RAMS/VUCM simulates the diurnal variations of surface energy balance fluxes realistically. This contributes to a reasonable UBL formation. A weakly unstable UBL is formed in the nighttime with UBL heights of about 100–200 m. When urban surfaces are represented in the RAMS using a land surface model of the Land Ecosystem-Atmosphere Feedback (LEAF), the RAMS/LEAF produces strong cold biases and thus fails to simulate UHI formation. This is due to the poor representation or absence of important urban physical processes in the RAMS/LEAF. This study implies that urban physical processes should be included in numerical models in order to reasonably simulate meteorology and air quality in urban areas and that the VUCM is one of the promising urban canopy models.     

Distribution of convective energy at upper level in South Korea and the possibility of artificial showery rain caused by activated CAPE

This paper reports a theoretical study on the possibility of inducing artificial showery rain using the convective available potential energy, which is naturally stored in the troposphere. We calculated the environmental parameters (frequency of climatic values, extreme value of stability index, etc.) in the upper troposphere using rawinsonde data from six main stations in Korea from 2001 to 2008 and examined the temporal spatial convective energy according to region. Our results showed that convective available potential energy, which can induce artificial rainfall, existed in the troposphere mainly in summer and were low in other seasons. Its value was found to be highest during late afternoon and in inland regions. We examined the vertical structure of the atmosphere using moisture convergence and vertical velocity (omega) and found that precipitation occurred under strong real latent instability conditions with high convective available potential energy (>3,000?J/kg) in summer and was characterized by moisture convergence at 1,000?C400?hPa, moisture divergence at 400?C300?hPa, and continuous ascending air current at 1,000?C300?hPa (?C??), on average. However, precipitation still did not occur in more than half the cases with high convective available potential energy because, according to the analysis, convective rainfall is affected to a greater extent by the value of convective inhibition than by convective available potential energy. It was also verified that in spite of zero convective inhibition, if the updrafts at a lower level were not sufficient to generate high convective available potential energy at a level higher than the level of free convection, convective rainfall would not occur under real latent instability. Therefore, we suggest it might be possible during the summer to secure the water resources in regions without precipitation by inducing ascending air current artificially under unstable atmospheric conditions to induce showery rain.     

Two Types of Diurnal Variations in Heavy Rainfall during July over Korea※

This study examined the characteristics of the diurnal variations of heavy rainfall (≥110 mm in 12 hours) in Korea and the related atmospheric circulation for July from 1980?2020. During the analysis period, two dominant pattens of diurnal variation of the heavy rainfall emerged: all-day heavy rainfall (AD) and morning only heavy rainfall (MO) types. For the AD-type, the heavy rainfall is caused by abundant moisture content in conjunction with active convection in the morning (0000?1200, LST; LST = UTC + 9) and the afternoon hours (1200?2400 LST). These systems are related to the enhanced moisture inflow and upward motion induced by the strengthening of the western North Pacific subtropical high and upper-tropospheric jet. For the MO-type, heavy rainfall occurs mostly in the morning hours; the associated atmospheric patterns are similar to the climatology. We find that the atmospheric pattern related to severe heavy rainfalls in 2020 corresponds to a typical AD-type and resembles the 1991 heavy-rainfall system in its overall synoptic/mesoscale circulations. The present results imply that extremely heavy rainfall episodes in Korea during the 2020 summer may occur again in the future associated with the recurring atmospheric phenomenon related to the heavy rainfall.     

Boundary-layer effects on mountain waves: a new look at some historical studies

Early studies of mountain waves reported various results that have rarely been investigated since. These include: large-amplitude mountain waves above an unstable boundary layer much higher than the mountains; a repeated downwind drift and upwind jump of mountain waves; and larger vertical wind magnitude near sunrise and/or sunset. These are investigated using over 3,000 radiosondes and meso-strato-troposphere (MST) radar. Superadiabatic temperature gradients are found beneath mountain waves, explainable by convection which appears to raise the mountain-wave launching height. Movement of mountain-wave patterns is studied by a new method using height–time vertical wind data. A swaying motion of mountain waves, with period of a few minutes, appears to be equally upwind and downwind, rather than asymmetric at the heights measurable. Also, vertical wind shows no change in mean, variance or extreme values near sunrise and sunset, despite the expected diurnal changes of boundary-layer structure. An explanation for differences between MST radar and other measurements and models of mountain waves is suggested in terms of more than one variety of mountain wave. Type 1 has stable air near the ground; type 2 is above a convective/turbulent boundary layer of significant height as compared to the mountains.     

宜昌冬季两次降水过程大气边界层的观测分析

利用宜昌2007年12月10-25日的加密观测资料,分析了两次低值系统经过宜昌时大气边界层的温湿风廓线结构及其日变化特征。结果表明：位温廓线具有明显的日变化特征,对流边界层在白天出现和发展,其高度可达600m,而稳定边界层在夜间出现和发展,其高度可达300m,降水会抑制对流边界层和稳定边界层的发展;湿度廓线结构及其日变化与对流边界层的发展有关,总体上湿度随高度减小,贴近地面的薄层湿度随高度减小较快,而混合层内湿度随高度变化较小,出现降水时,近地层的湿度有明显增加,大气边界层内湿度随高度快速平稳减小;风速廓线结构比较复杂,总体上风速随高度增大,在大气边界层低层有时会出现一个风速极大值,风速廓线没有明显的日变化特征,大气边界层内风向变化较大,但以偏东风为主。     

Some Basic Properties of the Surrogate Subgrid-Scale Heat Flux in the Atmospheric Boundary Layer

The development of improved subgrid-scale (SGS) models for large-eddy simulation of scalar transport in the atmospheric boundary layer requires an improved understanding of basic properties of the SGS fluxes. High frequency atmospheric wind speed and temperature data sampled at a height of 1.7 m are used to measure SGS heat fluxes and dissipation of temperature variance, by means of one-dimensional filtering and invoking Taylor's hypothesis. Conditional averaging is used to isolate interesting features of the SGS signals, and to relate them to the large-scale characteristics of the flow, such as the presence of coherent structures. Both mean and conditionally averaged SGS quantities are compared with those obtained using a standard eddy-diffusivity model. Within the limitations imposed by the one-dimensional data analysis, we observe that the model appears unable to reproduce important features of the real signals, such as the negative dissipation of temperature variance associated with strong negative resolved temperature gradients due to the ejection of warm air under unstable atmospheric stability conditions.